Comparison Between Historic Nuclear Explosion Yield Formulas
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45 MILITARY TECHNOLOGY, WEAPONRY, AND NATIONAL DEF↗
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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.
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THE INITIATION AND GROWTH OF EXPLOSION IN THE CONDENSED PHASE
Crystallography - thermal decomposition of explosive crystals - effect of fission fragments - initiation and growth of explosion
THERMAL DECOMPOSITION↗
Novel application of neutrinos to evaluate U.S. nuclear weapons performance
There is a growing realization that neutrinos can be used as a diagnostic tool to better understand the inner workings of a nuclear weapon. Robust estimates demonstrate that an Inverse Beta Decay (IBD) neutrino scintillation detector built at the Nevada Test Site with a 1000-ton active target mass at a standoff distance of 500 m would detect thousands of antineutrino events per nuclear test. This would provide less than 4% statistical error on the measured antineutrino rate and 5% error on antineutrino energy. Extrapolating this to an error on the test device explosive yield requires knowledge from evaluated nuclear databases, non-equilibrium fission rates, and assumptions on internal neutron fluxes. Initial calculations demonstrate that the total number of neutrinos emitted per fission in the first 10 3 s after a short pulse of 239 Pu fission is about a factor of two less than that from Pu fissioning under steady state conditions. Furthermore, there are significant energy spectral differences as a function of time after the pulse that must be considered. These and other model dependencies will be discussed in the paper. In the absence of nuclear weapons testing, many of the technical and theoretical challenges of a full nuclear test could be mitigated with a low cost smaller scale 20 ton fiducial mass IBD demonstration detector placed near a pulsed reactor. Potential reactors include the Texas A&M University TRIGA 1 GW–10 ms pulsed facility or the Sandia Annular Core Research Reactor. The short duty cycle and repeatability of pulses would provide critical real environment testing and measurements, which would be valuable for planning a possible real test shot in the future. Furthermore, the antineutrino rate as a function of time data would provide unique constraints on fission databases and model assumptions. Finally, there are impactful science drivers such as sensitive searches for ∼1 eV 2 sterile neutrinos and ∼MeV scale axions.
72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
Fast neutron activation of ubiquitous materials
Nuclear explosions expose ubiquitous materials to large numbers of neutrons, producing a variety of radioactive isotopes. To simulate such phenomena from both fission and thermonuclear explosions, we irradiated 29 different targets with approximately 3 and 14 MeV neutrons and measured the beta-delayed gamma rays using germanium detectors. Therefore, for each neutron energy, the expected radioisotopes, half-lives, and gamma ray energies were deduced. From measurements of the ratios of activities of the radionuclides produced by neutron irradiations, we were able to identify several materials that are particularly sensitive to the neutron energy spectra.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
Innovative nuclear thermal propulsion technology evaluation - Results of the NASA/DOE task team study
In response to findings from two NASA/DOE nuclear propulsion workshops, six task teams were created to continue evaluation of various propulsion concepts, from which evolved an innovative concepts subpanel to evaluate thermal propulsion concepts which did not utilize solid fuel. This subpanel endeavored to evaluate each concept on a level technology basis, and to identify critical issues, technologies, and early proof-of-concept experiments. Results of the concept studies including the liquid core fission, the gas core fission, the fission foil reactors, explosively driven systems, fusion, and antimatter are presented.
Howe, Steven D.↗
Measurements at the southern magnetic conju- gate region of the fission debris from the starfish nuclear detonation
Measurement of fission products from Star Fish high-altitude nuclear explosion with recording gamma-ray spectrometer
RECORDING INSTRUMENT↗
Nuclear fission reaction simulations in compact stars
Type-Ia supernovas are powerful stellar explosions that provide important distance indicators in cosmology. Recently, we proposed a new Type-Ia supernova mechanism that involves a nuclear fission chain-reaction in an isolated white dwarf [Phys. Rev. Lett. 126, 131101 (2021)]. Here, in this work, we perform novel reaction network simulations of the actinide-rich first solids in a cooling white dwarf. The network includes neutron-capture and fission reactions on a range of U and Th isotopes with various possible values for 235 U enrichment. We find, for modest 235 U enrichments, neutron capture on 238 U and 232 Th can breed additional fissile nuclei so that a significant fraction of all U and Th nuclei may fission during the chain reaction. Finally, we compute the energy release from the fission chain reaction for various uranium enrichments; a novel result that is a necessary input for thermal diffusion simulations of carbon ignition.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
Measurements at the southern magnetic conjugate region of the fission debris from the starfish nuclear detonation.
Fission products of Star Fish high-altitude nuclear detonation measured at southern magnetic conjugate region
STAR FISH PROJECT↗
Effect of shock on fission track dating of apatite and sphene crystals from the Hardhat and Sedan undergound nuclear explosions
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Fleischer, R. L.↗
Analysis of 127 Xe tracer measurements using a net counts method
A suite of measurement systems were deployed as part of the Physical Experiment 1 series of experiments, which involved detonating chemical explosives along with radionuclide tracers in an underground cavity, at the Nevada National Security Site (NNSS) in the United States. One of the radionuclide tracers, 127 Xe was released from the containment following the explosion and detected on a SAUNA Q B sampler situated approximately 3.5 km away. The system uses a beta-gamma coincidence detector system to measure fission product radioisotopes of xenon relevant to nuclear explosion monitoring. In this work we use the coincidence measurement data to analyse and interpret the results from the SAUNA Q B system, to calculate the measured 127 Xe activity concentration(s).
98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗
Ignition of Carbon Burning from Nuclear Fission in Compact Stars
Abstract Type Ia supernovae (SN Ia) are powerful stellar explosions that provide important distance indicators in cosmology. Recently, we proposed a new SN Ia mechanism that involves a nuclear fission chain reaction in an isolated white dwarf (WD). The first solids that form as a WD starts to freeze are actinide rich and potentially support a fission chain reaction. In this Letter, we explore thermonuclear ignition from fission heating. We perform thermal diffusion simulations and find at high densities, above about 7 × 10 8 g cm −3 , that fission heating can ignite carbon burning. This could produce an SN Ia or another kind of astrophysical transient.
79 ASTRONOMY AND ASTROPHYSICS↗
Partitioning of Radionuclides in Various Streams of the Mo-99 Purification Process
The Universal Neutron Irradiator (UNI) was designed to irradiate a small volume of uranium solution and to achieve high fission power without creating a large radionuclide (RN) inventory. The UNI system is equipped with a fully enclosed off-gas system with online hydrogen gas monitoring to prevent the production of an explosive atmosphere, as well as storage cylinders for capturing fission gases. It also includes a catalytic recombiner in the target capsule (to immediately recombine radiolytic hydrogen and oxygen gas in the system) and access ports for sampling the target solution and capsule headspace. In UNI Phase I experiments, 50 mL of uranyl sulfate solution was irradiated at 0.3–0.5 W/mL fission power using a tantalum target assembly to produce photoneutrons via irradiation with an electron beam. The purposes of the Phase I experiments were to test the efficacy of adding 200 ppm Fe 2+ to the target solution to prevent uranyl peroxide precipitation under representative irradiation conditions, and to monitor iodine speciation in the irradiated uranyl sulfate solution. The focus of the UNI Phase II experiments was to use an irradiated uranyl sulfate solution containing a mixture of fission products and monitor their distribution in various streams during the primary recovery column (titania-based column) that separates Mo-99 from uranium. Irradiations were designed to create sufficient activity for tracking their distribution in various processing streams using a combination of gamma counting and inductively coupled plasma mass spectrometry (ICP-MS) analyses. Obtained data will be used to better understand the composition of waste streams, accumulation of RN on the titania column, and identify what RNs accumulate in the uranyl sulfate solution. Furthermore, this knowledge will allow us to determine waste classifications for various streams produced during the Mo-99 purification process and develop an appropriate waste clean-up strategy.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
Neutronics Modeling of the pulsed plasma rocket reactor using rattlesnake
In the pulsed plasma rocket (PPR) reactor, neutron induced fission processes are utilized to implement a series of pulsed micro-explosions of very high power and eject plasma as a propellant. More specifically, projectiles (bullets) composed of moderated uranium are sent through the chamber of an unmoderated uranium barrel. By inducing rapid fission within the bullets, a plasma can be generated with appropriate delivery of neutrons. This study aims to assess the neutronics performance of the PPR reactor during normal operations using the MOOSE-based Rattlesnake code through the evaluation of the impact of the movement of the fuel bullet and the rotation of control drums on the criticality of the system. The Monte Carlo (MC) code Serpent 2 was employed to generate material-based cross sections for use in Rattlesnake and the reference neutronics solution. Cubit was used to generate the mesh for the Rattlesnake model. Parametric studies were conducted to evaluate the best approaches for cross section and mesh generation to ensure accurate results from Rattlesnake. As part of the verification process, the eigenvalue results of the system at various fuel bullet positions were obtained using Rattlesnake and compared with the reference solutions. The acceptable differences show that the Rattlesnake model with appropriate cross section and mesh generation procedure is a sufficiently accurate approximation of the continuous energy (CE) MC model for micro-sized reactors like the PPR reactor. Next, the impact of the rotation of the control drums on the system criticality was evaluated using the verified model. It was shown that the high-fidelity simulation using the deterministic code Rattlesnake can produce sufficiently accurate results for the evaluation of the reactor's neutronics performance in different phases of the normal operation with acceptable computational cost.
21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗
External Pulsed Plasma Propulsion (EPPP) Analysis Maturation
External Pulsed Plasma Propulsion (EPPP) systems are at the stage of engineering infancy with evolving paradigms for application. performance and general characteristics. Recent efforts have focused on an approach that employs existing technologies with near term EPPP development for usage in interplanetary exploration and asteroid/comet deflection. if mandated. The inherent advantages of EPPP are discussed and its application to a variety of propulsion concepts is explored. These include, but are not limited to, utilizing energy sources such as fission. fusion and antimatter, as well as, improved chemical explosives. A mars mission scenario is presented as a demonstration of its capability using existing technologies. A suggested alternate means to improve EPPP efficiencies could also lead to a heavy lift (non-nuclear) launch vehicle capability. Conceivably, true low-cost, access to space is possible using advanced explosive propellants and/or coupling the EPPP vehicle to a "beam propellant" concept. EPPP systems appear to offer an approach that can potentially cover ETO through interstellar transportation capability. A technology roadmap is presented that shows mutual benefits pertaining to a substantial number of existing space propulsion and research areas.
Bonometti, Joesph A.↗
127 Xe quantification method development and intercomparison exercise
Monitoring of the atmosphere for fission products ( 131m Xe, 133m Xe, 133 Xe, and 135 Xe) is performed by various laboratories to detect nuclear explosions. Quantification of 127 Xe is not routinely performed by laboratories measuring atmospheric radioxenon because it is not a fission product. 127 Xe was recently detected by a ground-based beta-gamma air monitoring system. When measured using beta-gamma coincidence detector systems, such as those in use on the International Monitoring System (IMS) of the Comprehensive Nuclear-Test-Ban Treaty (CTBT), 127 Xe can interfere with the quantification of fission product radioxenon due to overlap of the 127 Xe beta-gamma coincidence signatures with those of fission product radioxenon. Here, this work demonstrates quantification of 127 Xe at different laboratories with different measurement techniques. Production and purification of 127 Xe was performed by neutron activation of enriched 126 Xe. The purified 127 Xe was then split between laboratories, and detection and quantification methods were developed. At Idaho National Laboratory, a quantification method involving high purity germanium detectors was devised that included self-attenuation correction. At AWE, a beta-gamma coincidence counting method, as used in support of the IMS, was modified to enable the measurement and analysis of the 127 Xe samples. Corrections were made for self-attenuation, which showed a strong xenon volume dependency, for some coincidence signatures. The gas sample activity concentration was used as the comparison metric and it showed excellent agreement between the methods.
98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗
A Review of Nuclear Forensics: 2016-2020
The study of nuclear forensics harkens back to the Manhattan Project-era, when scientists first started to analyze the debris from the 1945 Trinity test. Political turmoil stemming from the Cold War and the rehabilitation of Germany following WWII has led to new challenges in international security involving nuclear proliferation. Nuclear materials have, on occasion, been lost, misplaced, or stolen from former Soviet countries, and illicit materials have been interdicted all over the world. The National Technical Nuclear Forensics Center (NTNFC) was established in 2006, and has been at the forefront of drive to advance nuclear forensic capabilities in the United States. The ultimate goal of nuclear forensics is to examine nuclear and other radioactive materials using analytical techniques to determine origin and history of the material, particularly in the context of law enforcement investigations. Nuclear forensics can be divided into two parts: predetonation and post-detonation. Pre-detonation forensics, as the name implies, is the investigation of a nuclear material or weapon that has not been detonated or involved in an explosion, whereas postdetonation forensics is the study of activation or fission products in debris or the environment following the use of a nuclear or radiological dispersal device (RDD). Both parts require a number of analytical chemical and radiochemical techniques to determine identification of the material. Many advancements in analytical techniques, including rapidity, sample size, and forensic signatures have been made in recent years. The analytical methods that can be used in a nuclear forensic investigation, such as mass spectrometry and gamma spectroscopy, have been described in detail in previous reviews, including Straub et.al, and will not be explained here. This review will discuss recent publications (from 2016 to present) describing advancements of techniques such as radiochronometry, morphology, development of novel reference materials, and inter-laboratory collaborations for both pre- and post-detonation nuclear forensics.
37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
Drops in Space: Super Oscillations and Surfactant Studies
An unprecedented microgravity observation of maximal shape oscillations of a surfactant-bearing water drop the size of a ping pong ball was observed during a mission of Space Shuttle Columbia as part of the second United States Microgravity Laboratory-USML-2 (STS-73, October 20-November 5, 1995). The observation was precipitated by the action of an intense sound field which produced a deforming force on the drop. When this deforming force was suddenly reduced, the drop executed nearly free and axisymmetric oscillations for several cycles, demonstrating a remarkable amplitude of nonlinear motion. Whether arising from the discussion of modes of oscillation of the atomic nucleus, or the explosion of stars, or how rain forms, the complex processes influencing the motion, fission, and coalescence of drops have fascinated scientists for centuries. Therefore, the axisymmetric oscillations of a maximally deformed liquid drop are noteworthy, not only for their scientific value but also for their aesthetic character. Scientists from Yale University, the Jet Propulsion Laboratory (JPL) and Vanderbilt University conducted liquid drop experiments in microgravity using the acoustic positioning/manipulation environment of the Drop Physics Module (DPM). The Yale/JPL group's objectives were to study the rheological properties of liquid drop surfaces on which are adsorbed surfactant molecules, and to infer surface properties such as surface tension, Gibb's elasticity, and surface dilatational viscosity by using a theory which relies on spherical symmetry to solve the momentum and mass transport equations.
Apfel, Robert E.↗
Fission gas trapped in Chornobyl fuel microparticles reveals details of reactor operations
The isotopic ratios of fission gas would provide important source information of a nuclear fuel sample found in the environment. However, it is believed that during a reactor accident like Chornobyl all fission gas is lost and that the radioactive particles found in the Chornobyl Exclusion Zone today are depleted in gases by the initial explosion and subsequent fire. We disprove this hypothesis by detection and analysis of trapped krypton and xenon in these particles. Our analysis of krypton and xenon isotopes by noble gas mass spectroscopy in combination with resonance ionization mass spectrometry establishes that important information about reactor operations like age, neutron flux and plutonium fission fraction can still be reconstructed from individual micrometer-sized particles even after decades of weathering in the environment.
Chornobyl↗