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Lawrence Livermore National Laboratory and Sandia National Laboratory Nuclear Accident Dosimetry Support of IER 252 and the Dose Characterization of the Flattop Reactor at the DAF

In support of IER 252 “Characterization of the Flattop Reactor at the NCERC”, LLNL performed ROSPEC measurements of the neutron spectrum and deployed 129 Personnel Nuclear Accident Dosimeters (PNAD) to establish the need for height corrections and verification of neutron spectrum evaluation of the fluences and dose. A very limited number of heights (typically only one or two heights) can be measured using neutron spectrometers, therefore it was important to determine if any height correction would be needed in future intercomparisons and studies. Specific measurement positions around the Flatttop reactor are provided in Figure 1. Table 1 provides run and position information for LLNL measurements. The LLNL ROSPEC (R2) was used for run numbers 1 – 7, and vi. PNADs were positioned on trees during run numbers 9, 11, and 13.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Blind Intercomparison of Nuclear Accident Dosimetry using the Flattop Reactor at NCERC

The purpose of this exercise was to continue United States, United Kingdom, and France collaborative activities performing Nuclear Accident Dosimetry intercomparison. IER 148 was the inaugural intercomparison exercise using the Godiva reactor at the DAF. In contrast to IER 148, in the current exercise participants were “blind” to the known doses during the exercise, to simulate the dosimetry response to a real criticality incident. This document is the Final Exercise (CED-x) Report for IER-253, “International Intercomparison Exercise for Nuclear Accident Dosimetry at the DAF Using Flattop.” The report describes the structure and results of the exercise consisting of two irradiations. The details of all dosimetry elements and their placement in proximity to Flattop on support stands or phantoms was unknown to participating laboratories. The participating laboratories in this report are deidentified and the report summarizes participant results from the intercomparison. The exercise occurred during the week of May 21, 2018.

42 ENGINEERING↗

The First ICNC February 10-12, 1981 [Slides]

The first meeting that became the International Conference on Nuclear Criticality—ICNC—was held at the Los Alamos National Laboratory in February 1981. This presentation includes information on that meeting, including several experiments performed around that time period.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Sensitivity Data File Formats

The format of the TSUNAMI-A sensitivity data file produced by SAMS for cases with deterministic transport solutions is given in Table 6.3.A.1. The occurrence of each entry in the data file is followed by an identification of the data contained on each line of the file and the FORTRAN edit descriptor denoting the format of each line. A brief description of each line is also presented. A sample of the TSUNAMI-A data file for the Flattop-25 sample problem is provided in Figure 6.3.A.1. Here, only two profiles out of the 130 computed are shown.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

National Criticality Experiments Research Center (NCERC) - capabilities and recent measurements

The National Criticality Experiments Research Center (NCERC) located at the Device Assembly Facility (DAF) at the Nevada National Security Site (NNSS) and operated by Los Alamos National Laboratory (LANL) is home to four critical assemblies which are used to support of range of missions, including nuclear criticality safety and nuclear nonproliferation. Additionally, subcritical systems can also be assembled at NCERC. NCERC is providing critical and subcritical experiments valuable to the nuclear data community and experiments performed at NCERC are often published as benchmarks in the International Criticality Safety Benchmark Evaluation Project (ICSBEP) Handbook. This manuscript will give a broad overview of recent experiments performed at NCERC, upcoming experiments, and why integral measurements are important and useful to the nuclear data community. The four critical assemblies are GODIVA IV, FLATTOP, COMET, and PLANET. GODIVA IV is a cylindrical metal fast burst reactor, the fourth in the GODIVA series that dates back to the 1950’s. FLATTOP is an highly enriched uranium (HEU) or Pu core reflected by natural uranium. COMET and PLANET are vertical lift assemblies, where one half of the reactor can be lifted to the upper half of the reactor to create a critical system. Some recent experiments include various critical intermediate energy assemblies with lead, and subcritical measurements of plutonium reflected by copper, tungsten, and nickel. Work is also underway to make a better measurement of the critical mass of neptunium, using a neptunium sphere surrounded by nickel shells. Additionally, measurements will be performed next year with HEU shells from Rocky Flats. These HEU shells will be stacked together to make larger systems, allowing for a large range of criticality (from subcritical to delayed critical). Other upcoming measurements include an HEU critical assembly sensitive to intermediate energy neutrons.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

Preservation of kinetics parameters generated by Monte Carlo calculations in two-step deterministic calculations

The generation of accurate kinetic parameters such as mean generation time Λ and effective delayed neutron fraction β eff via Monte Carlo codes is established. Employing these in downstream deterministic codes warrants another step to ensure no additional error is introduced by the low-order transport operator when computing forward and adjoint fluxes for bilinear weighting of these parameters. Another complexity stems from applying superhomogenization (SPH) equivalence in non-fundamental mode approximations, where reference and low-order calculations rely on a 3D full core model. In these cases, SPH factors can optionally be computed for only part of the geometry while preserving reaction rates and K-effective, but the impact of such approximations on kinetics parameters has not been thoroughly studied. This paper aims at studying the preservation of bilinearly-weighted quantities in the Serpent–Griffin calculation procedure. Diffusion and transport evaluations of IPEN/MB-01, Godiva, and Flattop were carried out with the Griffin reactor physics code, testing available modeling options using Serpent-generated multigroup cross sections and equivalence data. Verifying Griffin against Serpent indicates sensitivities to multigroup energy grid selection and regional application of SPH equivalence, introducing significant errors; these were demonstrated to be reduced through the use of a transport method together with a finer energy grid.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

ATF Transient Prescription Tests in TREAT

EXECUTIVE SUMMARY The Transient Reactor Test facility (TREAT) was constructed in the late 1950’s and provided thousands of transient irradiations before being placed in standby mode in 1994. In 2017, it resumed operation in order to reclaim its crucial role in nuclear-heated safety research. TREAT is a transient reactor where inherently-safe core physics, a nimble transient rod drive system, and a philosophy of continual facility improvement work together to enable flexible power maneuvers for fuel safety research. While the facility’s flexible design and multi-mission nature saw historic experiments for numerous transient types, TREAT was not specifically adapted to optimize or demonstrate its full performance capability for Light Water Reactor (LWR) postulated accidents including Hot Zero Power Reactivity Initiated Accidents (HZP-RIA) and Loss of Coolant Accidents (LOCA). The physics of HZP-RIA drive very brief pulses with fairly large energy excursions. TREAT is currently capable of approaching HZP-RIA pulse widths through transients initiated on a large step insertion of reactivity and terminated shortly thereafter by rapid re-insertion of the transient rods (“clipping”). LOCAs are postulated to occur quite differently, starting from normal power operations followed by a long period of lower power decay heat. TREAT is able to simulate LOCA events with an initial flattop transient for tens of seconds, followed by a sizeable power reduction, to a longer segment where specimen fission heating represents internal decay heat generation. Two reactor physics testing campaigns were undertaken to address the HZP-RIA type transients, neither of which had been performed in any great measure historically to address data gaps in the timing, repeatability of clipping and effect of dynamic transient rod motions on core-to-specimen fission power coupling. The first campaign, referred to as the Accident Tolerant Fuel (ATF) transient prescription tests, employed dosimeters in the core to characterize the effect of rod motions on specimen power coupling for clipped, unclipped, and low-level steady state operations each with approximately the same moderate core energy release. This campaign was accompanied by efforts to measure dosimetry and compare results to analytic predictions. The other HZP-RIA campaign, referred to as Narrow Pulse Width (NPW) transient prescriptions, employed higher step insertions with increased core energy release to demonstrate TREAT’s capability in achieving the narrowest-possible pulse width. Additionally, a series of LOCA transient prescriptions were also performed to demonstrate how well TREAT could perform long-duration shaped transients. Both NPW and LOCA transient prescriptions did not include dosimeters but used existing plant power instrumentation to produce transient power data. All three transient prescription campaigns were successfully carried out in TREAT. The ATF-3 transient prescriptions showed that TREAT can perform clipped transients with remarkable repeatability. Measurement and modeling both showed that the power coupling in small, fissile dosimeters does not change by more than 8% between clipped, unclipped, and steady state runs while uncertainty sources in both the modeling and measurement methods were identified and found to be on the order of 20% in total. Overall, the ATF-3 transient prescription tests were successful in determining repeatability and consistency of dosimeter power coupling, developing processes for modeling and measuring this crucial parameter, and demonstrating the need for continued efforts in transient prescription work at TREAT in support of future experiment design and post test data interpretation. The NPW and LOCA transient prescriptions were also successfully performed to exhibit TREAT’s capability for these important LWR accident categories. The NPW transients showed pulse widths of ~90 ms, which were the narrowest ever achieved in TREAT to date and relevant for the upper end range of HZP-RIA simulation. This effort provided crucial data for calibrating kinetic models to be used in enhanced pulse-narrowing strategies in upcoming irradiations. Similarly, The LOCA transient prescriptions showed that TREAT can simulate the needed nuclear heating and event time scales for LOCA fuel safety research and provided essential data for future experiment design.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

The National Criticality Experiments Research Center: Capability Expansion and Experiments in the Last Three Years

The National Criticality Experiments Research Center (NCERC) is a general purpose criticality experiments facility located inside the Device Assembly Facility (DAF) at the Nevada National Security Site (NNSS). Critical experiments containing any special nuclear material, any enrich ment/separation, most physical forms, and any configuration are possible within the constraints of the defined safety basis. NCERC draws upon physical assets and experimental knowledge to solve some of the most difficult problems with respect to criticality safety, reactor physics, and reactor kinetics. In terms of physical assets, NCERC houses hundreds of kilograms of special nuclear material with a majority consisting of highly enriched uranium (HEU) and weapons grade plutonium (WGPu). NCERC is home to four critical assembly machines: Comet, Planet, Flattop, and Godiva IV. To support various derivative diagnostics on fissioning systems, NCERC houses a count room to measure irradiated samples and dosimeters. This paper will step through each of these capabilities explaining recently completed work and upgrades.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Radiative pulsed L-mode operation in ARC-class reactors

Abstract A new ARC-class, highly-radiative, pulsed, L-mode, burning plasma scenario is developed and evaluated as a candidate for future tokamak reactors. Pulsed inductive operation alleviates the stringent current drive requirements of steady-state reactors, and operation in L-mode affords ELM-free access to ∼ 90 % core radiation fractions, significantly reducing the divertor power handling requirements. In this configuration the fusion power density can be maximized despite L-mode confinement by utilizing high-field to increase plasma densities and current. This allows us to obtain high gain in robust scenarios in compact devices with P fus > 1000 MW despite low confinement. We demonstrate the feasibility of such scenarios here; first by showing that they avoid violating 0D tokamak limits, and then by performing self-consistent integrated simulations of flattop operation including neoclassical and turbulent transport, magnetic equilibrium, and radiofrequency current drive models. Finally we examine the potential effect of introducing negative triangularity with a 0D model. Our results show high-field radiative pulsed L-mode scenarios are a promising alternative to the typical steady state advanced tokamak scenarios which have dominated tokamak reactor development.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Investigating Fission Reaction Rate Ratio Sensitivities [Abstract]

Reaction rate ratios are a measurable parameter for reactor and criticality applications. A number of foil irradiations and fission chamber measurements have been performed for critical assemblies at Los Alamos National Laboratory starting in the 1950’s including (i) Godiva, a bare HEU spherical assembly; (ii) Flattop-25, a spherical assembly consisting of an HEU core and a natural uranium reflector; (iii) Jezebel, a bare 239 Pu assembly; and (iv) Flattop-Pu, a spherical assembly consisting of a 239Pu core and a natural uranium reflector. Fission ratio data for 238 U(n,f)/ 235 U(n,f), 237 Np(n,f)/ 235 U(n,f), 233 U(n,f)/ 235 U(n,f) and 239 Pu(n,f)/ 235 U(n,f) were obtained and reported. The EUCLID (Experiments Underpinned by Computational Learning for Improvements in nuclear Data) project at Los Alamos National Laboratory (LANL) aims to constrain nuclear data by using a suite of measurement types beyond k-effective. Recent investigations include the use of pulsed spheres for nuclear data validation and other measurement methods of interest. One focus of the work is to determine if other methods are complimentary to the critical experiments utilized for nuclear data validation. It is anticipated the investigations will help inform methods that may be utilized in machine learning algorithms for nuclear validation. In order to use a measurement type for nuclear validation, it is necessary to obtain cross-section sensitivities for parameters. This work looks at reaction rate ratio sensitivities with SENSMG and Monte Carlo N-Particle R Code Version 6.21.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Data from Rossi-alpha and pulsed neutron prompt neutron time decay measurements at the Oak Ridge Critical Experiments Facility

This report briefly describes the Rossi-alpha and pulsed neutron prompt neutron time decay measurements performed at the Oak Ridge Critical Experiments Facility. This description includes the measurement equipment, type of data, and how to access the actual data from Records Management Services at Oak Ridge National Laboratory and the Nuclear Criticality Safety Benchmark Program (NCSBEP) of the Idaho National Laboratory. Most of the data were acquired between 1960 and 1975 on weapons-grade enriched uranium metal assemblies. Also included are measurements of the same type performed at Los Alamos National Laboratory by Oak Ridge National Laboratory with the JEZEBEL and FLATTOP criticality assemblies and other plutonium metal parts. The purpose of this report is to allow future mining of the data for publication of additional information that can be used to verify calculational methods and nuclear cross sections. These data can be used to create reactor physics benchmarks for the Nuclear Energy Agency’s International Handbook of Evaluated Reactor Physics Experiments. Present calculational methods can be used to directly calculate the measured data. The prompt neutron decay is more neutron spectrum sensitive than other measured quantities, particularly for interacting fissile metal systems where the flight time of neutrons between interacting sections is a large part of the neutron lifetime.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Flattop Critical Assembly [Slides]

Objectives: Gain a working knowledge of the design of the Flattop critical assembly; Gain a working knowledge of how changes in reflector location can affect the criticality of a system; and, Understand the concept of temperature-dependent reactivity feedback.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

CSEWG Meeting Minutes

Work has been done at LANL to validate various updated evaluations from ENDF/BVIII.1b0 including: Fe, Cu, Si, U, Pu. Continuous energy tables were processed with NJOY2016 and output to ACE files. For non-Pu legacy critical benchmarks, all calculations were within the experimental benchmark uncertainty, with some benchmarks having shown lower bias using ENDF/B-VIII.1b0. In HST systems, ENDF/B-VIII.0 shows reasonable results above the thermal leakage fraction. ENDF/B-VIII.0.1 is doing slightly worse than ENDF/B- VIII.0. b0.2 and it also includes a new 19 F evaluation, so more work is needed to examine its impact. 233 U thermal and intermediate bare and water-reflected benchmarks agree well with ENDF/B-VIII.0. From ENDF/B-VIII.0 to ENDF/B-VIII.0b0.1, HMF-007 C/E are increasing and the new 19 F evaluation is helping the HMF-007 cases containing Teflon which have historically had high C/E. The Pu legacy benchmark suite is within experimental uncertainty with the exception of THOR. The INDEN evaluation followed by LANL gave the lowest mean absolute bias, but it remains difficult to make a determination on which Pu evaluation is the best. INDEN performs slightly better for the JEZEBEL series, while the LANL Pu evaluation is better for THOR and flattop benchmarks. For the PMI benchmark series INDEN outperforms the LLNL evaluation. For the PST benchmark series ENDF/B-VIII.0 and LLNL Pu evaluations are better than the INDEN evaluation. C/E ratios for Jezebel and Godiva reaction rate ratios show all the Pu evaluations are very close to one another, making it again difficult to say which is best. When examining neutron reactor kinetics parameters, each Pu evaluation is once again very close. Each individual Pu evaluation seems to have advantages in their own applications.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Modelling and experiment to stabilize disruptive tearing modes in the ITER baseline scenario in DIII-D

Abstract The achievement of high gain, stationary conditions in a tokamak scenario aimed at producing fusion energy in the ITER Project is crucial to the demonstration that this form of energy can be used in future reactors to provide cheap and clean energy globally. Disruptions are a challenge for the fusion energy field, in particular for the ‘ITER Baseline Scenario’ (IBS), as reproduced in the DIII-D tokamak. This work shows that a solution has been found for the m = 2/ n = 1 tearing modes that have consistently caused disruptions in the IBS: stable operation down to zero input torque was achieved by modifying the current density profile at the beginning of the pressure flattop and the ELM character later in the discharges, guided by previous results showing that the most likely cause of these instabilities is the current density profile. The coupling between sawteeth, n>2 modes and the 2/1 TMs is shown to not be statistically significant, nor the leading origin for the evolution towards instability. Ideal and resistive MHD modeling provide positive verification that a steeper ‘well’ in the region of the q = 2 rational surface leads to worse ideal stability, higher tearing index Δ’ and lower threshold Δ’ c for resistive instabilities, consistent with the experimental results. This provides confidence that the methods used in this work can be extrapolated to other devices and applied to avoid disruptions in ITER and pulsed fusion devices worldwide.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

The time-dependent simulation of CFETR baseline steady-state scenarios

One of the key issues to achieve the phase I mission of China fusion engineering test reactor (CFETR) is steady-state operation with a modest fusion power up to 200 MW. To examine this feasibility, time-dependent modeling of CFETR baseline scenario is performed. The time-dependent scenario design examines actual discharge features, including auxiliary heating and current drive scheme, equilibrium, transport, PF coil systems and plasma control system during the plasma evolution. During plasma current ramp-up, 10 MW of EC or LH heating is used to effectively save volt–second consumption to a reasonable level within magnet coil capability and to reduce li for better plasma control. Three reference scenarios are designed to target full non-inductive operation with different external heating and current drive (H&CD), which are NB + EC, NB + LH, and LH + EC, respectively. Two scenarios with neutral beams reach the required fusion power of CFETR phase I target, while for LH + EC scenario the fusion power and confinement is somewhat lower. A reversed magnetic shear with q min > 2 is sustained with off-axis current drive and bootstrap current for all cases examined. Ideal MHD analysis shows that both large toroidal mode number n ballooning mode and low n kink mode are stable in the three reference cases independent of whether the current is totally relaxed or not. The L mode and H–L back transition ramp-down are designed to successfully reduce the plasma current to 2 MA and keep li below 2 with ramp-down rate of 80 kA s -1 . The H–L back transition ramp-down yields improvements in the power transfer and coil current evolution as well as the li evolution. The heating and current drive characteristics of three auxiliary heating sources are indicated by scanning studies. A 2D scan of NB energy and tangency radius indicates the features of NB power deposition, current drive, torque and shine through issue. Both ramp-up and flattop are considered in the scanning of radio frequency parameters. For EC waves, the ramp-up phase constrains the parameter space more. The 2D scan of EC launch angle shows that EC waves launched above the midplane yield a better CD efficiency than using a midplane launcher. Specifically, 10 MW of EC waves launched from LFS above the midplane yield a maximum on axis driven current of about 0.55 MA, while waves launched from top yield a maximum near edge driven current of about 0.45 MA in the region of ρ > 0.5. Scanning of n $\parallel$ in LH spectrum shows that n $\parallel$ should be set around 1.7 to get enough penetration (inside ρ = 0.7) for current drive and avoid strong accessibility problem. It is found that LH waves launched from HFS drives more current than that launched from LFS when n $\parallel$ is small. The maximum LH driven current reaches 1.1 MA with 10 MW of LH power launched from HFS.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Preliminary Activation Wire Analysis for the POKER Experiment Flattop Irradiation

Activation foils, or in this case wires, are commonly deployed to critical experiments at the Na tional Criticality Experiments Research Center (NCERC) to provide additional neutron diagnostics and provide additional energy-dependent responses to tie back to neutronic and/or multi-physics simulations.

07 ISOTOPE AND RADIATION SOURCES↗

On benchmarking of simulations of particle transport in ITER

We present results of benchmarking of core particle transport simulations by a collection of codes widely used in transport modelling of tokamak plasmas. Our analysis includes formulation of transport equations, difference between electron and ion solvers, comparison of modules of the pellet and edge gas fuelling on the ITER baseline scenario. During the first phase of benchmarking we address the particle transport effects in the stationary phase. Firstly, simulations are performed with identical sources, sinks, transport coefficients, and boundary conditions prescribed in the flattop H-mode phase. The transformation of ion particle transport equations is introduced so to directly compare their results to electron transport solvers. Moreover, the pellet fuelling models are benchmarked in various conditions to evaluate the dependency of the pellet deposition on the pellet volume, injection side, pedestal and separatrix parameters. Thirdly, edge gas fuelling is benchmarked to assess sensitivities of source profile predictions to uncertainties in plasma conditions and detailed model assumptions. At the second phase, we address particle transport effects in the time-evolving plasma including the current ramp-up to the ramp-down phase. The ion and the electron solvers are benchmarked together. Differences between the simulation results of the solvers are investigated in terms of equilibrium, grid resolution, radial coordinate, radial grid distribution, and plasma volume evolution term. We found that the selection of the radial coordinate can yield prominent differences between the solvers mainly due to differences in the edge grid distribution. The simulations reveal that electron and ion solvers predict noticeably different density peaking for the same diffusion and pinch velocity while with the peaked profile of helium, expected in fusion reactors. The fuelling benchmarking demonstrates that gas puffing is not efficient for core fuelling in H-modes and density control should be done by the high field side pellet injection in contrast to present machines.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗