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DOE OSTI2020

Structure retrieval in liquid-phase electron scattering

Electron scattering on liquid samples has been enabled recently by the development of ultrathin liquid sheet technologies. The data treatment of liquid-phase electron scattering has been mostly reliant on methodologies developed for gas electron diffraction, in which theoretical inputs and empirical fittings are often needed to account for the atomic form factor and remove the inelastic scattering background. In this work, we present an alternative data treatment method that is able to retrieve the radial distribution of all the charged particle pairs without the need of either theoretical inputs or empirical fittings. Here, the merits of this new method are illustrated through the retrieval of real-space molecular structure from experimental electron scattering patterns of liquid water, carbon tetrachloride, chloroform, and dichloromethane.

74 ATOMIC AND MOLECULAR PHYSICS↗

DOE OSTI2021

Convergent close-coupling calculations of electrons scattering on electronically excited molecular hydrogen

We use the adiabatic-nuclei molecular convergent close-coupling method to perform calculations of 0.01–1000 eV electrons scattering on the c 3 Π u , a 3 $Σ$$^{+}_{g}$, B 1 $Σ$$^{+}_{u}$, C 1 Π u , and EF 1 $Σ$$^{+}_{g}$ states of H 2 in the v=0 vibrational level. Elastic, superelastic, ionization, and grand-total cross sections are presented, as well as cross sections for excitation of the n=2–3 singlet and triplet states of H 2 (where n is the atomic-limit principle quantum number). Comparison with available theoretical results is made. Good agreement is found with the recent R-matrix results [J. Phys. B 53, 245203 (2020)] for most of the exchange and dipole-forbidden transitions, but not for the dipole-allowed transitions. Here, the sources of disagreement were found to be an unconverged partial-wave expansion and the utilization of the fixed-nuclei approximation (as opposed to adiabatic-nuclei) in the R-matrix calculations.

74 ATOMIC AND MOLECULAR PHYSICS↗

DOE OSTI2021

Experimental Investigation and Monte Carlo Simulation of Quasielastic Electron Scattering From Helium-3 Clusters in Helium-4

Experiment E04-018 was conducted in Hall A of the Jefferson National Laboratory (JLab) from November 2006 through July 2007. The experiment used the two superconducting, high-resolution magnetic spectrometers of Hall A to detect scattered electrons and recoil nuclei. One goal of this experiment was to provide accurate data on the elastic charge form factor of 4He to high momentum transfers (up to Q2 = 77 fm?2). The purpose of this thesis is to analyze and simulate a very unique and unexpected class of data from this experiment. The work performed involved the analysis of electron scattering data with the 4He target of the JLab E04-018 experiment and Monte Carlo simulation studies of elastic and quasielastic electron scattering from the 4He and 3He few-body nuclear systems. The results of this experiment and the simulations provide insights into the existence of A = 3 clustering in 4He, and possibly in heavier nuclei.

Alahmade, Walaa↗

DOE OSTI2023

Neutron Skin Measurement of 208Pb and 48Ca Using Parity Violating Electron Scattering

Parity-violating electron scattering experiments (PVES) provides a clean probe of neutron densities that is model independent and free from strong interaction uncertainties in interpretation. The PREX-2 and CREX experiments were run in 2019 and 2020 at Jefferson laboratory measured the nucleon skin thickness, the difference between the r.m.s. neutron radius Rn and the r.m.s. proton radius Rp, of 208Pb and 48Ca via parity violating electroweak asymmetry in the elastic scattering of longitudinally polarized electrons. PREX-2 experiment was performed with 950 MeV electrons scattered at a 5¿ angle with Q2 = 0.00616 ± 0.00004 (GeV/c)2, while CREX used 2182 MeV electrons at the same angle with Q2 = 0.0297 ± 0.0002 (GeV/c)2. For PREX-2 the measured asymmetry was AP V = 550 ± 16 (stat.) ± (syst.) ppb, which corresponds to Rskin = 0.278 ± 0.078 (exp.) ± 0.012 (theo.) fm. The CREX asymmetry was AP V = 2668 ± 106 (stat.) ± 40 (syst.) ppb, which corresponds to Rskin = 0.121 ± 0.026 (exp.) ±0.024 (model) fm. One of the crucial systematic uncertainty that PREX-2 and CREX were sensitive to was the non-parity violating asymmetries that resulted from the helicity correlated false asymmetries in the polarized electron beam. There was a lot of work put towards understanding and suppressing the asymmetries arising from these effects. The parity violating asymmetry measurement required a very precise determination of the electron beam polarization. To accurately determine the beam polarization, a Compton polarimeter was used during both PREX-2 and CREX. A careful alignment of the laser to the Fabry-Perot cavity, data analysis and systematic control was employed to get a precise beam polarization result for the experiments. The PREX-2 measurement has broad implications for increasing our knowledge about neutron star structure and the equation of state of nuclear matter. The combined PREX and CREX results will have implications for future energy density functional calculations and the theory of nuclear structure.

Premathilake, Sachinthani↗

DOE OSTI2023

Potential Constraints to Neutrino-Nucleus Interactions Based on Electron Scattering Data

A thorough understanding of neutrino-nucleus interactions physics is crucial to achieving precision goals in broader neutrino physics programs. The complexity of nuclei comprising the detectors and limited understanding of their weak response constitutes one of the biggest systematic uncertainties in neutrino experiments - both at intermediate energies affecting the short- and long-baseline neutrino programs as well as at lower energies affecting coherent scattering neutrino programs. While electron and neutrino interactions are different at the primary vertex, many underlying relevant physical processes in the nucleus are the same in both cases, and electron scattering data collected with precisely controlled kinematics, large statistics and high precision allows one to constrain nuclear properties and specific interaction processes. To this end, electron-nucleus scattering experiments provide vital complementary information to test, assess and validate different nuclear models and event generators intended to be used in neutrino experiments. In fact, for many decades, the study of electron scattering off a nucleus has been used as a tool to probe the properties of that nucleus and its electromagnetic response. While previously existing electron scattering data provide important information, new and proposed measurements are tied closely to what is required for the neutrino program in terms of expanding kinematic reach, the addition of relevant nuclei and information on the final states hadronic system.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2023

Electron Scattering from 1-Methyl-5-Nitroimidazole: Cross-Sections for Modeling Electron Transport through Potential Radiosensitizers

In this study, we present a complete set of electron scattering cross-sections from 1-Methyl-5-Nitroimidazole (1M5NI) molecules for impact energies ranging from 0.1 to 1000 eV. This information is relevant to evaluate the potential role of 1M5NI as a molecular radiosensitizers. The total electron scattering cross-sections (TCS) that we previously measured with a magnetically confined electron transmission apparatus were considered as the reference values for the present analysis. Elastic scattering cross-sections were calculated by means of two different schemes: The Schwinger multichannel (SMC) method for the lower energies (below 15 eV) and the independent atom model-based screening-corrected additivity rule with interferences (IAM-SCARI) for higher energies (above 15 eV). The latter was also applied to calculate the total ionization cross-sections, which were complemented with experimental values of the induced cationic fragmentation by electron impact. Double differential ionization cross-sections were measured with a reaction microscope multi-particle coincidence spectrometer. Using a momentum imaging spectrometer, direct measurements of the anion fragment yields and kinetic energies by the dissociative electron attachment are also presented. Cross-sections for the other inelastic channels were derived with a self-consistent procedure by sampling their values at a given energy to ensure that the sum of the cross-sections of all the scattering processes available at that energy coincides with the corresponding TCS. This cross-section data set is ready to be used for modelling electron-induced radiation damage at the molecular level to biologically relevant media containing 1M5NI as a potential radiosensitizer. Nonetheless, a proper evaluation of its radiosensitizing effects would require further radiobiological experiments.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2024

Simulations, Modeling and Data Analysis of Parity Violating Electron Scattering Experiments

In the Standard Model (SM) of nuclear and particle physics, parity violation is incorporated through the representation of the weak interaction as a chiral gauge interaction. Only the left-handed components of particles and right-handed components of antiparticles participate in weak interactions in the Standard Model. This implies that parity is asymmetric for the weak interaction. Parity violating electron scattering (PVES) experiments are designed to probe the physics parameters related to the SM, with the possibility to discover physics beyond the SM (BSM) by measuring the parity violating asymmetry ¿¿¿ of longitudinally polarized electrons scattered off unpolarized targets with high precision. This dissertation will be focused on two PVES experiments, the next 208Pb Lead Radius Experiment (PREX-II), and the Measurement of a Lepton-Lepton Electroweak Reaction (MOLLER) experiment, as well as in some small sections, the Calcium Radius Experiment (CREX) and P2 experiment which are also PVES experiments). PREX-II and CREX experiments, performed in Hall A at the Thomas Jefferson National Accelerator Facility (Jefferson Lab), measured ¿¿¿ in the elastic scattering of longitudinally polarized electrons from 208Pb and 48Ca targets to provide a precise model independent determination of the neutron skin thickness of 208Pb and 48Ca nuclei, respectively. The MOLLER experiment, proposed to start in 2027 and also to be performed in Hall A at Jefferson Lab, is to measure ¿¿¿ of longitudinally polarized electrons scattered off unpolarized electrons (Møller scattering) to determine the weak charge of electrons ¿¿¿ and the weak mixing angle ¿¿ with high precision. As for the P2 experiment, which will be performed at the upcoming MESA accelerator in Mainz Germany, it is to measure the weak charge of proton ¿¿¿ using ¿¿¿ in the elastic electron-proton scattering of polarized electrons off unpolarized protons. The final results from the PREX-II experiment are presented as ¿¿¿=550±16 (¿¿¿¿)±8 (¿¿¿¿) parts-per-billion (ppb). Combining the PREX-I and PREX-II results, the neutron skin thickness from PREX experiments is determined as ¿¿-¿¿=0.283±0.071 ¿¿ in 208Pb. This thesis lists the software and computational contribution of the author to these PVES experiments, including writing scripts and software to help with the PREX-II/CREX experiments, analyzing data to provide useful information and systematic uncertainty for the PREX-II experiment, modeling and simulations for the MOLLER, and providing an alternative design of an electronic equipment for the P2 experiment.

Chen, Yufan↗

DOE OSTI2024

Simulations, Modeling and Data Analysis of Parity Violating Electron Scattering Experiments

Chen, Yufan↗

DOE OSTI2021

Dependence of dark matter - electron scattering on the galactic dark matter velocity distribution

The rate of dark matter-electron scattering depends on the underlying velocity distribution of the dark matter halo. Importantly, dark matter-electron scattering is particularly sensitive to the high-velocity tail, which differs significantly amongst the various dark matter halo models. In this work, we summarize the leading halo models and discuss the various parameters which enter them. We recommend updated values for these parameters based on recent studies and measurements. Furthermore, we quantify the dependence of the dark matter-electron scattering rate on the choice of halo model and parameters, and demonstrate how these choices propagate to the predicted cross-section limits. The rate is most sensitive to changes in the circular velocity v 0 ; in silicon targets, we find that the changes in the rate predictions can range from Script $\mathcal{O}$(0.01%) to Script $\mathcal{O}$(100%) for contact interactions and Script $\mathcal{O}$(10%) to Script $\mathcal{O}$(100%) for long-range interactions.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2021

Development and Use of an Ultra-High Resolution Electron Scattering Apparatus

In this LDRD project, we developed a versatile capability for high-resolution measurements of electron scattering processes in gas-phase molecules, such as ionization, dissociation, and electron attachment/detachment. This apparatus is designed to advance fundamental understanding of these processes and to inform predictions of plasmas associated with applications such as plasma-assisted combustion, neutron generation, re-entry vehicles, and arcing that are critical to national security. We use innovative coupling of electron-generation and electron-imaging techniques that leverages Sandia’s expertise in ion/electron imaging methods. Velocity map imaging provides a measure of the kinetic energies of electrons or ion products from electron scattering in an atomic or molecular beam. We designed, constructed, and tested the apparatus. Tests include dissociative electron attachment to O2 and SO2, as well as a new method for studying laser-initiated plasmas. This capability sets the stage for new studies in dynamics of electron scattering processes, including scattering from excited-state atoms and molecules.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2022

General tensor structure for electron scattering in terms of invariant responses

The general structure of semi-inclusive polarized electron scattering from polarized spin-1/2 targets is developed for use at all energy scales, from modest-energy nuclear physics applications to use in very high energy particle physics. The leptonic and hadronic tensors that enter in the formalism are constructed in a general covariant way in terms of kinematic factors that are frame dependent but model independent and invariant response functions which contain all of the model-dependent dynamics. In the process of developing the general problem the relationships to the conventional responses expressed in terms of the helicity components of the exchanged virtual photon are presented. For semi-inclusive electron scattering with polarized electrons and polarized spin-1/2 targets one finds that 18 invariant response functions are required, each depending on four Lorentz scalar invariants. Additionally it is shown how the semi-inclusive cross sections are related via integrations over the momentum of the selected coincidence particle and sums over open channels.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2025

Convergent close-coupling calculations of electron scattering on LiH

Cross sections for electron scattering on the ground state of LiH are calculated using the molecular convergent close-coupling method. The fixed-nuclei approximation is utilized, and calculations are performed at the mean internuclear separation of 3.06 𝑎 0 for projectile energies ranging from 0.1 to 500 eV. Here, a model-potential approach is utilized to treat the LiH molecule as a two-electron system, and good agreement is found with the literature for various properties of the structure model. Cross sections are presented for elastic scattering, excitation to several electronic states, and ionization. Comparison is made with existing results, and qualitative agreement is found with small close-coupling calculations at low projectile energies. Good agreement is found with first-order results at high projectile energies.

74 ATOMIC AND MOLECULAR PHYSICS↗

DOE OSTI2024

X-ray Spectral-Timing Pipeline to Investigate an Electron-Scattering Time Delay in Black Hole Accretion Disks [Slides]

The soft lag in black hole X-ray binaries (BHXRBs) refers to the time delay for the soft, thermal disk to respond to hard, variable coronal irradiation. This time lag increases from less than 1 ms to ~10 ms during the hard-to-soft state transition. Interpretations of soft lag trends appeal to changing the light-travel path via an evolving coronal height and/or inner accretion disk radius. Both interpretations neglect a time delay contribution from the reprocessing of irradiation inside the disk, where electron-scattering opacity dominates. A new theory considering a thermalization (electron scattering) time delay in the disk can plausibly produce ~10 ms time delays in the intermediate state. To further investigate the impacts of adding a time delay component from electron scattering in the disk, we are creating a spectral-timing pipeline that can analyze NICER (Neutron Star Interior Composition Explorer) X-ray observations of BHXRBs in outburst. In the near future, we will apply this spectral timing pipeline to develop a reverberation lag model from simulations that include the thermalization time delay from electron scattering in the disk.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2022

Complete collision data set for electrons scattering on molecular hydrogen and its isotopologues: III. Vibrational excitation via electronic excitation and radiative decay

We present state-resolved cross sections for vibrational excitation via electronic excitation followed by radiative decay (ERD), for electrons scattering on all bound vibrational levels of the ground electronic state ($X\hspace{1.5 mm} ^1Σ_g^+$) of molecular hydrogen and its isotopologues (H 2 , HD, HT, D 2 , DT and T 2 ). We consider excitation of the singlet $\textit{n}$ = 2–3 states (where n refers to the united-atoms-limit principle quantum number) and account for all possible decay pathways back to the bound vibrational levels of the ground electronic state ($X\hspace{1.5 mm} ^1Σ_g^+$) to produce an estimate for the ERD cross sections. A selection of the results are presented in graphical form and a full data set is provided as both numerical values and analytic fit functions in supplementary data files. The uncertainty in the cross sections is estimated to be 11%, except for scattering on the highest bound vibrational level of HD, HT, D 2 , and DT, where the uncertainty is 21%. The data can be downloaded from the MCCC database at mccc-db.org.

74 ATOMIC AND MOLECULAR PHYSICS↗

DOE OSTI2025

Electroweak observables in neutrino-electron scattering from a muon storage ring

We investigate the sensitivity of a companion neutrino detector situated in the plane of a high-energy, high-intensity muon storage ring to elastic ν μ and ν e scattering on electrons (EνES). Assuming a muon collider with center-of-mass energies of up to 10 TeV, we report sensitivity to the weak couplings g V and g A up to around 0.05% relative error, and sensitivity to the weak mixing angle in the momentum transfer Q ∈ [10 −2 , 2] GeV range up to around 0.03% relative error. EνES measurements with high-energy muon storage rings allow one to directly interrogate the momentum-transfer regime associated with the NuTeV anomaly. This level of precision allows unique sensitivity to the momentum-dependence of sin 2 θ W . We estimate that with the neutrinos from a E μ = 1.5 TeV (or higher) muon collider, the hypothesis that sin 2 θ W does not “run” can be safely ruled out.

electroweak precision physics↗

DOE OSTI2025

The importance of electron scattering in the analysis of actinide X-ray spectroscopy

Abstract Manifestations of electron scattering in X-ray spectroscopy have been evident for decades. Here, it will be shown that the proper interpretation of variants of X-ray Absorption Spectroscopy (XAS) of actinide materials must include an accurate treatment of features caused by electron scattering, i.e., EXAFS or Extended X-ray Absorption Fine Structure. These EXAFS features can be of such low energy that they are within ten to twenty electron volts of the Unoccupied Density of States (UDOS), immediately above the Fermi Energy or Band Gap. The adaption of simple models using the FEFF simulation program will be presented, including the demonstration of the robust nature of the results from different models. Graphical abstract

Tobin, J. G. (ORCID:0000000322943301)↗

DOE OSTI2025

Influence of neutrino-electron scattering and neutrino-pair annihilation on hypermassive neutron star

Here, we investigate the influence of inelastic neutrino microphysics in general-relativistic magnetohydrodynamics simulations of a hypermassive neutron star. In particular, we include species/energy groups coupled neutrino-matter interactions, such as inelastic neutrino-electron scattering and electron-positron annihilation kernels, into simulations up to 50 ms. Neutrino-electron inelastic scattering is known to have effective neutrino-matter energy exchange. We show that, with neutrino-electron inelastic scattering, simulations predict 75% higher disc mass with slightly different mass-averaged compositions, and 18% more ejected mass with similar distributions. The enhancement of the mass of the disc and the ejecta results in stronger baryon pollution, leading to less favorable jet launching environments. Furthermore, neutrino luminosities are about 50%, 40%, and 30% higher for electron neutrino, electron antineutrino, and heavy-lepton neutrinos. In contrast, we do not see any significant impacts due to electron-positron annihilation.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2022

An overview of how parity-violating electron scattering experiments are performed at CEBAF

Parity-violating electron-scattering experiments represent an important focus of the nuclear physics experimental program at the Continuous Electron Beam Accelerator Facility (CEBAF) at Jefferson Lab. These experiments pose significant challenges because the scattering asymmetries can be very small, of the order parts-per-million and smaller. To succeed, the properties of the electron beam such as current, position, size and energy, must be very nearly identical in the two electron-polarization spin states (parallel and anti-parallel relative to the direction of beam motion at the scattering target). This paper describes the origins of unwanted helicity-correlated beam asymmetries present on the electron beam and methods to minimize them to acceptable levels.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗