Electron and Positron Scattering Cross Sections from CO 2 : A Comparative Study over a Broad Energy Range (0.1–5000 eV)
Not Available
37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
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Results for “Electron & positron scattering”
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Convergent close-coupling calculations of electron scattering on HeH +
Here, we use the molecular convergent close-coupling (MCCC) method to perform calculations of 10–1000 eV electron scattering on the ground state of HeH + . Cross sections are presented for excitation of the n = 2 – 3 singlet and triplet states (where n is the united-atoms-limit principle quantum number), as well as ionization. We also present cross sections for He + and H + ion production following dissociative excitation and ionization. The He + production cross section is compared with the measurements of Lecointre, Jureta, Urbain, and Defrance [J. Lecointre, J. J. Jureta, X. Urbain, and P. Defrance, J. Phys. B At. Mol. Opt. Phys. 47, 015203 (2014)]. We find that the MCCC results are up to 30% higher than experiment.
74 ATOMIC AND MOLECULAR PHYSICS↗
Orientation-dependent enhanced ionization in acetylene revealed by ultrafast cross-polarized pulse pairs
We investigate the orientation dependence of enhanced ionization (EI) during strong-field-driven nuclear motion in acetylene (C 2 H 2 ). Here, we both initiate and probe molecular dynamics in acetylene with intense 6-fs cross-polarized pulse pairs, separated by a variable delay. Following multiple ionization by the first pulse, acetylene undergoes simultaneous elongation of the carbon-carbon and carbon-hydrogen bonds, enabling further ionization by the second pulse and the formation of a very highly charged state, [C 2 H 2 ] 6+ . At small interpulse delays (< 20 fs), this enhancement occurs when the molecule is aligned to the probe pulse. Conversely, at large delays (> 40 fs), formation of [C 2 H 2 ] 6+ occurs when the molecule is aligned to the pump pulse. By analyzing the polarization and time dependence of sequentially ionized [C 2 H 2 ] 6+ , we resolve two transient alignments that both contribute to a large increase in the multiple ionization yield. In conclusion, this cross-polarized pulse pair scheme uniquely enables selective probing of deeply bound orbitals, providing new insights on orientation-dependent EI in highly charged hydrocarbons.
Atomic & molecular clusters↗
Linear polarization fractions of Fulcher- α fluorescence in electron collisions with H 2
We apply the molecular convergent close-coupling method to the calculation of linear polarization fractions for Fulcher-band fluorescence following electron-impact excitation of the H 2 d 3 Π u state. Furthermore, the results exhibit the opposite threshold behavior compared to the only previous calculations, but are in agreement with the most recent measurements for the Q(1), R(1), and Q(3) transitions.
72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
Retrieval of the molecular orientation distribution from atom-pair angular distributions
Imaging laser-induced rotational dynamics is an important and active field due to its applications in capturing reactions in the molecular frame and in molecular imaging. Experimental measurement of the molecular orientation distribution, as a function of the Euler angles, has only been demonstrated for special cases when the detectable signal is generated along the molecular symmetry axis. Here we developed the general theory that maps the probability density distribution of the molecular orientation to the atom-pair angular distributions for nonlinear molecules. With the theory, the molecular orientation distribution can be retrieved from the measured atom-pair angular distribution, which we demonstrate experimentally using ultrafast electron diffractive imaging of impulsively aligned trifluoro-iodomethane molecules. Here, the retrieved molecular orientation distribution is in good agreement with direct numerical simulations of the time-dependent Schrodinger equation using the experimental conditions. Unlike the existing retrieval methods, the retrieval method does not require solving Schrodinger equation, works for any alignment method, and is in principle applicable to asymmetric top molecules.
74 ATOMIC AND MOLECULAR PHYSICS↗
Dynamics of resonant low-energy electron attachment to ethanol-producing hydroxide anions
Here, the dynamics of dissociative electron attachment to ethanol is experimentally investigated at the Feshbach resonance formed with incident electron energies near 9.5 eV. Highly differential laboratory-frame momentum distributions of OH – fragments are measured for a series of energies spanning the resonance width, using the velocity-map-imaging technique. The OH – kinetic-energy distribution indicates that the C-O breaking dissociation process could either be a three-body dissociation or a two-body dissociation with significant rovibrational excited fragments. The small, but significant, anisotropy in the OH – angular distribution provides signatures of the molecular symmetry of the associated resonant state under the axial recoil approximation, which assumes the dissociation is much faster than any rotation of the dissociation axis. Within these assumptions, the 9.5-eV Feshbach resonance can be assigned to the electronic transition from the ($10a'$) orbital with its ground-state C s symmetry to the empty ($4a''$) level, involving the simultaneous electron attachment. This dynamics could be a model for C-O dissociation in larger alcohols and ethers.
74 ATOMIC AND MOLECULAR PHYSICS↗
All-Order Full-Coulomb Quantum Spectral Line-Shape Calculations
Understanding how atoms interact with hot dense matter is essential for astrophysical and laboratory plasmas. Interactions in high-density plasmas broaden spectral lines, providing a rare window into interactions that govern, for example, radiation transport in stars. However, up to now, spectral line-shape theories employed at least one of three common approximations: second-order Taylor treatment of broadening operator, dipole-only interactions between atom and plasma, and classical treatment of perturbing electrons. In this Letter, we remove all three approximations simultaneously for the first time and test the importance for two applications: neutral hydrogen and highly ionized magnesium and oxygen. Finally, we found 15%–50% change in the spectral line widths, which are sufficient to impact applications including white-dwarf mass determination, stellar-opacity research, and laboratory plasma diagnostics.
79 ASTRONOMY AND ASTROPHYSICS↗
Competing ionization and dissociation: Extension of the energy-dependent frame transformation to the gerade symmetry of H 2
This article solves two major tasks that frequently arise in the theory of electron collisions with a target molecular cation. First, it extends the energy-dependent frame transformation (EDFT) treatment, which is needed to map fixed-nuclei electron-molecule scattering matrices into an energy-dependent laboratory-frame scattering matrix with vibrational channel indices. The EDFT mapping can now be carried out even when the target molecule possesses multiple low-energy potential curves, significantly transcending previous applications. Second, it implements a method to extract the rest of the full laboratory-frame scattering matrix, i.e., the columns and rows describing input and/or output dissociation channels. The treatment is benchmarked in this article against the essentially exact solution of a refined two-dimensional model of the singlet gerade Σ symmetry of H 2 . Our tests demonstrate that the theory accurately maps fixed-nuclei scattering information, of the type provided by existing electron-molecule computer codes, into a laboratory-frame scattering matrix that includes both ionization and dissociation. Furthermore, this treatment can provide a general framework applicable to a broad class of electron collision processes involving diatomic target ions, suitable for an accurate description of challenging processes such as dissociative recombination.
74 ATOMIC AND MOLECULAR PHYSICS↗
First Measurement of Hard Exclusive π − Δ + + Electroproduction Beam-Spin Asymmetries off the Proton
Not Available
72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
First Study of Reaction Ξ 0 n → Ξ − p Using Ξ 0 -Nucleus Scattering at an Electron-Positron Collider
Not Available
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
Fast calculation of diffraction patterns from an ensemble of aligned molecules
We report an algorithm to calculate electron diffraction patterns for molecules with anisotropic angular distribution, which is significantly faster than existing methods. The algorithm uses a transform to convert the molecular orientation distribution, which is a function of three Euler angles, to the atom-pair distribution functions which depend on the polar and azimuthal angles. The diffraction signal can then be calculated from the atom-pair distributions. We demonstrate the computation method numerically by calculating electron diffraction patterns for a symmetric top molecule (trifluoroiodomethane) and an asymmetric top molecule (formaldehyde) and show that it reduces the calculation time by approximately two orders of magnitude compared to the standard brute-force method. Here, the method can also be applied to the calculation of x-ray diffraction patterns.
74 ATOMIC AND MOLECULAR PHYSICS↗
Quantum vacuum processes in the extremely intense light of relativistic plasma mirror sources
Abstract The advent of petawatt-class laser systems allows generating electromagnetic fields of unprecedented strength in a controlled environment, driving increasingly more efforts to probe yet unobserved processes through their interaction with the quantum vacuum. Still, the lowest intensity scale governing these effects lies orders of magnitude beyond foreseen capabilities, so that such endeavor is expected to remain extremely challenging. In recent years, however, plasma mirrors have emerged as a promising bridge across this gap, by enabling the conversion of intense infrared laser pulses into coherently focused Doppler harmonic beams lying in the X-UV range. In this work, we present predictions on the quantum vacuum signatures produced when such beams are focused to intensities between 10 24 and 10 28 W cm −2 , specifically photon–photon scattering and electron–positron pair creation. These signatures are computed via the stimulated vacuum formalism, combined with a model of perfectly focused beam built from PIC-generated harmonics spectra, and implemented on state-of-the-art massively parallel numerical tools. In view of identifying experimentally favorable configurations, we also consider the coupling of the focused harmonic beam with an auxiliary optical beam, and provide comparison with other established schemes. Our results show that a single coherently focused harmonic beam can produce as much scattered photons as two infrared pulses in head-on collision, and confirm that the coupling of the harmonic beam to an auxiliary beam gives rise to significant levels of inelastic scattering, and hence holds the potential to strongly improve the attainable signal to noise ratios in experiments.
70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
Final state interactions for high energy scattering off atomic electrons
We consider the scattering of high energy leptons off bound atomic electrons focusing primarily on final state interactions between the outgoing energetic electron, and the heavy residual charged “debris” in the final state. These effects are inherently absent from calculations for a free electron at rest. Coulomb exchanges are enhanced by the large number of electrons in the atomic debris, and are unsuppressed by nonrelativistic velocities in the debris. We find that these exchanges can be resummed using operator methods, and cancel at the level of the cross section until at least 𝑂(𝛼 3 ). Furthermore, we argue that both final and initial state Coulomb exchanges (enhanced by the number of electrons in the atom) do not affect the cross section until at least 𝑂(𝛼 3 ). Transverse photon couplings to nonrelativistic electrons are proportional to their small velocities, and rotational invariance suppresses their contribution to 𝑂(𝛼 3 ). Our results are relevant for precision experiments involving neutrinos, electrons, positrons, and muons scattering off of atomic electrons in a fixed target.
Atoms↗
Elastic scattering and rotational excitation of H 2 by electron impact: Convergent close-coupling calculations
We apply the adiabatic-nuclei molecular convergent close-coupling (MCCC) method to the study of elastic scattering and rotational excitation of H 2 by 0.01–20-eV electrons. Integral cross sections are presented for all rotational transitions with |ΔN| ≤ 2 and N i = 0–31 within the v = 0 vibrational level and differential cross sections for a selection of transitions. Agreement with the available measurements and previous calculations is mostly excellent, depending on the transition and incident energy. Finally, we suggest possible reasons, and argue for the accuracy of the MCCC data.
74 ATOMIC AND MOLECULAR PHYSICS↗
Close-coupling approach to electron scattering with multielectron targets
Momentum-space close coupling calculations of electron scattering require removal of spurious and unphysical solutions. Here, we demonstrate here that removal of these solutions involve regulator operators that enforce Pauli exclusion selection rules in addition to removing spurious solutions. The form of a regular operator for e-H scattering has already been established, but a general extension to the multielectron case has been elusive. Here we present a general method for scattering on multielectron targets, atoms, or molecules, ensuring that the scattering solutions obey Pauli-exclusion selection rules. The regulator operator is obtained by finding the null space vectors of the 𝑁+1 electrons of the projectile and target atom scattering system. We demonstrate that this general procedure reduces to the e-H result and provide examples for He- and Li-like targets as well as guidance for implementation.
74 ATOMIC AND MOLECULAR PHYSICS↗
Attosecond time delays in the body frame for photodetachment from molecular anions
Attosecond time delays in molecular photoionization at low energies are dominated by the contribution of the Coulomb phase, which diverges as the energy of the photoelectron decreases towards zero. With calculations on core-electron ejection from CN – and C 2 – we demonstrate that in photodetachment of molecular anions the absence of the long-range Coulomb interaction in the final state can reveal the delays of narrow low-energy shape resonances that do not generally occur in photoionization. Delays of several femtoseconds can be associated with such resonances. Finally, the angular dependence of photodetachment time delays in the body frame is highly sensitive to short-range anisotropies in the electron-molecule interaction as well as to the initial state.
74 ATOMIC AND MOLECULAR PHYSICS↗
Elastic positron–proton scattering at low Q$^2$
Systematic differences in the the proton's charge radius, as determined by ordinary atoms and muonic atoms, have caused a resurgence of interest in elastic lepton scattering measurements. The proton's charge radius, defined as the slope of the charge form factor at Q$^2$=0, does not depend on the probe. Any difference in the apparent size of the proton, when determined from ordinary versus muonic hydrogen, could point to new physics or need for the higher order corrections. While recent measurements seem to now be in agreement, there is to date no high precision elastic scattering data with both electrons and positrons. A high precision proton radius measurement could be performed in Hall B at Jefferson Lab with a positron beam and the calorimeter based setup of the PRad experiment. This measurement could also be extended to deuterons where a similar discrepancy has been observed between the muonic and electronic determination of deuteron charge radius. A new, high precision measurement with positrons, when viewed alongside electron scattering measurements and the forthcoming MUSE muon scattering measurement, could help provide new insights into the origins of the proton radius puzzle, and also provide new experimental constraints on radiative correction calculations.
72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
Influence of neutrino-electron scattering and neutrino-pair annihilation on hypermassive neutron star
Here, we investigate the influence of inelastic neutrino microphysics in general-relativistic magnetohydrodynamics simulations of a hypermassive neutron star. In particular, we include species/energy groups coupled neutrino-matter interactions, such as inelastic neutrino-electron scattering and electron-positron annihilation kernels, into simulations up to 50 ms. Neutrino-electron inelastic scattering is known to have effective neutrino-matter energy exchange. We show that, with neutrino-electron inelastic scattering, simulations predict 75% higher disc mass with slightly different mass-averaged compositions, and 18% more ejected mass with similar distributions. The enhancement of the mass of the disc and the ejecta results in stronger baryon pollution, leading to less favorable jet launching environments. Furthermore, neutrino luminosities are about 50%, 40%, and 30% higher for electron neutrino, electron antineutrino, and heavy-lepton neutrinos. In contrast, we do not see any significant impacts due to electron-positron annihilation.
79 ASTRONOMY AND ASTROPHYSICS↗