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Experimental Observations of Nuclear Activity in Deuterated Materials Subjected to a Low-Energy Photon Beam

Exposure of highly deuterated materials to a low-energy (nom. 2 MeV) photon beam resulted in nuclear activity of both the parent metals of hafnium and erbium and a witness material (molybdenum) mixed with the reactants. Gamma spectral analysis of all deuterated materials, ErD2.8+C36D74+Mo and HfD2+C36D74+Mo, showed that nuclear processes had occurred as shown by unique gamma signatures. For the deuterated erbium specimens, posttest gamma spectra showed evidence of radioisotopes of erbium ((163)Er and (171)Er) and of molybdenum ((99)Mo and (101)Mo) and by beta decay, technetium (99mTc and 101Tc). For the deuterated hafnium specimens, posttest gamma spectra showed evidence of radioisotopes of hafnium (180mHf and 181Hf) and molybdenum ((99)Mo and (101)Mo), and by beta decay, technetium ((99m)Tc and (101)Tc). In contrast, when either the hydrogenated or non-gas-loaded erbium or hafnium materials were exposed to the gamma flux, the gamma spectra revealed no new isotopes. Neutron activation materials showed evidence of thermal and epithermal neutrons. CR-39 solid-state nuclear track detectors showed evidence of fast neutrons with energies between 1.4 and 2.5 MeV and several instances of triple tracks, indicating (is) greater than 10 MeV neutrons. Further study is required to determine the mechanism causing the nuclear activity.

Steinetz, Bruce M.↗

Nuclear Data Sheets for A = 163

The available data from the various reaction and decay studies leading to nuclides having mass number A=163 have been reviewed. These data are summarized and presented, together with adopted level schemes and properties, for nuclides from Eu (Z=63) through Os (Z=76). {sup 163}Eu represents a new addition to these nuclides. Level structures are now known for {sup 163}Ta and {sup 163}W through high-spin studies and recoil-decay tagging techniques. Several radioactive decays in this mass chain are not known at all or poorly established. No {beta} or {gamma}-ray data are available for {sup 163}Re-{sup 163}W-{sup 163}Ta-{sup 163}Hf {epsilon} decay chain. Those for {sup 163}Hf-{sup 163}Lu-{sup 163}Yb {epsilon} decay chain and {sup 163}Eu-{sup 163}Gd-{sup 163}Tb {beta}{sup -} decay chain are very sketchy. This evaluation is an update and revision of the previous one (2000Si01)

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Thermal properties of holmium-implanted gold films for a neutrino mass experiment with cryogenic microcalorimeters

In a microcalorimetric neutrino mass experiment using the radioactive decay of {sup 163}Ho, the radioactive material must be fully embedded in the microcalorimeter absorber. One option that is being investigated is to implant the radioactive isotope into a gold absorber, as gold is successfully used in other applications. However, knowing the thermal properties at the working temperature of microcalorimeters is critical for choosing the absorber material and for optimizing the detector performance. In particular, it is paramount to understand if implanting the radioactive material in gold changes its heat capacity. We used a bolometric technique to measure the heat capacity of gold films, implanted with various concentrations of holmium and erbium (a byproduct of the {sup 163}Ho fabrication), in the temperature range 70 mK–300 mK. Our results show that the specific heat capacity of the gold films is not affected by the implant, making this a viable option for a future microcalorimeter holmium experiment.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗