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DUAL-PARTICLE DOSEMETER BASED ON ORGANIC SCINTILLATOR

Abstract Traditionally available handheld dosemeters are generally sensitive to only one type of radiation: neutrons or photons. Some dosemeters also rely on very specific attenuation correlations between response and dose, are not scalable in size and multiple dosemeters are required to characterise mixed-particle fields. The research presented here serves as a proof-of-concept for a method to simultaneously measure dose rates from neutrons and photons using a particle discriminating organic scintillation detector without the need for spectral deconvolution. The method was compared with traditional instruments and to simulation. Isotopic photon dose rates measured with this method were within 4% of simulated truth, whereas fission spectrum neutron dose rates were measured within 21%. Measurements of dose rates from both particles agree with simulated truth better than traditional instruments. This new method allows for measurement of dose equivalent from both neutrons and photons with a single instrument and no reliance on spectral deconvolution.

Miller, C. A.↗

Efficiency of a radiophotoluminescence glass dosemeter for low-earth-orbit space radiation

Chips of a radiophotoluminescence glass dosemeter (RPLG) were used for measurements of space radiation during a 9.8 d Shuttle-Mir mission (STS-91) at an altitude of 400 km and an inclination of 51.65 degrees. Two of RPLG chips were put into each of 59 positions in or on a life-size human phantom. The RPLG values equivalent to 137Cs gamma ray absorbed doses were found to be systematically lower than those of a Mg2SiO4:Tb thermoluminescence dosemeter (TDMS). In comparison with the organ or tissue absorbed dose and dose equivalent values that were estimated using a combination of TDMS and plastic nuclear track detectors, the efficiencies of the RPLG chips were about 80% for the water absorbed dose and about 40% for the dose equivalent. Whereas the percentage values will change during different missions, such additional information obtained from small RPLG chips is useful for improving the reliability of radiation dosimetry in space.

NASA Discipline Radiation Health↗

Extra dose due to extravehicular activity during the NASA4 mission measured by an on-board TLD system

A microprocessor-controlled on-board TLD system, 'Pille'96', was used during the NASA4 (1997) mission to monitor the cosmic radiation dose inside the Mir Space Station and to measure the extra dose to two astronauts in the course of their extravehicular activity (EVA). For the EVA dose measurements, CaSO4:Dy bulb dosemeters were located in specially designed pockets of the ORLAN spacesuits. During an EVA lasting 6 h, the dose ratio inside and outside Mir was measured. During the EVA, Mir crossed the South Atlantic Anomaly (SAA) three times. Taking into account the influence of these three crossings the mean EVA/internal dose rate ratio was 3.2. Internal dose mapping using CaSO4:Dy dosemeters gave mean dose rates ranging from 9.3 to 18.3 microGy h-1 at locations where the shielding effect was not the same. Evaluation results of the high temperature region of LiF dosemeters are given to estimate the mean LET.

NASA Experiment Number 9401704↗

Microprocessor controlled portable TLD system

An up-to-date microprocessor controlled thermoluminescence dosemeter (TLD) system for environmental and space dose measurements has been developed. The earlier version of the portable TLD system, Pille, was successfully used on Soviet orbital stations as well as on the US Space Shuttle, and for environmental monitoring. The new portable TLD system, Pille'95, consists of a reader and TL bulb dosemeters, and each dosemeter is provided with an EEPROM chip for automatic identification. The glow curve data are digitised and analysed by the program of the reader. The measured data and the identification number appear on the LED display of the reader. Up to several thousand measured data together with the glow curves can be stored on a removable flash memory card. The whole system is supplied either from built-in rechargeable batteries or from the mains of the space station.

NASA Discipline Radiation Health↗

Oxy-fluorophosphate glass doped SmO{sup 3+} as solid state dosimeter via spectroscopic techniques

In the present work, collective studies on optical, structural and magnetic properties of 0.5% SmO{sup 3+} ions in new easily melting fluorophosphate glass of the basic composition 70P{sub 2}O{sub 5}–20AlF{sub 3}–10NaF were carried out. The same combined spectral measurements (UV–Vis, FTIR, and ESR) were repeated after successive gamma irradiation. These collective spectral studies are expected to throw some insight on the effect of host fluorophosphate glass on these selected spectral properties of samarium ions together with identifying the effects of gamma irradiation on both the host fluorophosphate glass and on samarium ions and reaching to the resultant generated induced defects. The experimental results exhibit that, the slope of the UV–Vis line is sufficiently high in order to this tool is preferable to be elected as a suitable tool for the dosimetric purpose for this glass composition. The results in this manuscript propose that it is possible to use these techniques to determine if the glass sample may be used as solid-state dosimeters for gamma dose measurements in the range from 0.1 up to 15 kGy due to their linearity with the absorbed dose, color change, low fading for time periods up to 25 days and good response reproducibility.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

First Step in Validating the Radiological Inventories of the Current French Nuclear Fleet - 19000

To anticipate the evolution of the mechanical characteristics of its PWR vessels, EDF developed a vessels fluence monitoring program. This program was based on vessel samples and neutron dosimeters deployed between the fuel assemblies and vessels. These samples and dosimeters are regularly analyzed in laboratories. To calculate the radioactive inventories, we have developed a calculation scheme which includes a 3D mapping of the neutron flux, the calculation of the radiological inventories of the structures of interest, and finally the validation of the results. The validation needs samples to propose calculation/measurement ratios. Unfortunately before the final shut down, the internal and vessel samplings are not possible. To anticipate the decommissioning of the current French nuclear fleet, this paper shows how the samples of the vessels fluence monitoring program can be used to validate the calculated radiological inventories. Using state-of-the-art simulations (i.e. 3D geometric model, 3D neutron sources, 3D neutron propagation, operational fuel loading coupled with effective power distributions) we calculated the radiological inventories of some vessel fluence monitoring program samples. The comparisons between calculated and measured results were done on 'standard chemical elements'. To qualify a chemical element as 'standard', many criteria must be satisfied such as a high concentration level, a low uncertainty about concentration, activation into an expanded cross section range, production of radionuclides having significant half-lives and finally no difficulties measuring the radionuclides produced. The retained 'standard' is Fe which produces, under neutrons flux, Fe-55. The comparisons show that the calculations slightly overestimate the measurements. (authors)

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Implementation of a Dose-based Compliance System for WCS - 19178

Waste Control Specialists LLC (WCS) operates a low-level radioactive waste (LLRW) disposal facility in Andrews, Texas. The site includes a compact waste facility (CWF) that began receiving waste in 2012, a federal waste facility (FWF) that started receiving waste in 2013, as well as a Resource Conservation and Recovery Act (RCRA) landfill and a byproduct facility. The current site license uses a complex system of concentration-based investigation levels and action levels (ILs and ALs) coupled with analytical decision levels (ADLs) that, when exceeded, require specific steps to be taken. These concentration-based ILs and ALs are media specific (i.e. air, soil, water), radionuclide specific, location specific, and disposal facility specific. This results in thousands of individual ILs, ALs, and ADLs that need to be managed and evaluated routinely in order to demonstrate compliance. Further, under the current system, each exceedance of an IL and AL can trigger comparisons to numerous additional isotopic ILs per sample, which is cumbersome, error prone, and costly. This paper describes implementation of a dose-based compliance system that has been developed to replace the existing system. The dose-based compliance system is implemented in RACER{sup C}, a cloud-based software developed by Risk Assessment Corporation (RAC). This system maintains all the analytical results related to the sampling and analysis conducted as part of the Radiological Environmental Monitoring Program (REMP) together with the geo-spatial data allowing instantaneous trending and analysis of the data. Further, the system contains the information needed to compare the analytical results to the new media-specific screening levels that have been developed, and the parameters and routines to compute doses using prescribed exposure scenarios and dose coefficients for compliance evaluation. Once measurement data are entered into RACER, the routines for continuous screening of air, soil, groundwater, and dosimeter data are triggered, and any sample result failing the screening step or exceeding the dose IL/AL is identified and flagged automatically for further review or action, as appropriate. Because RACER is cloud-based, the data, screening, and dose calculations can be accessed remotely at any time, providing a timely and efficient method for identifying any possible releases from the site to the environment as well as determining the potential dose consequences associated with a release. Furthermore, the system is accessible by the regulator providing transparency and ensuring they remain fully informed in an efficient manner. (authors)

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3D Gamma Source Mapping and Intervention Analysis - 19243

3D gamma source mapping and intervention analysis, through Transco Products, Inc.'s RadVision3D{sup R}, uses the N-Visage Scanner{sup TM} by Createc combining laser scanning, optical imaging, and CZT (Cadmium Zinc Telluride) technologies to capture plant geometry, images, and gamma radiation data. By capturing multiple scans in an area of interest a full 3D analysis can be performed using N-Visage Fusion{sup TM} software by Createc which develops a 3D model showing radioactive sources in the environment and allowing various interventions, such as shielding or source removal, to be modeled virtually. The output of a RadVision3D{sup R} project is a scaled virtual environment that the user can 'walk through' on a PC for training and work planning activities. Included in the viewer are dose planes for the as-scanned conditions as well as for each intervention, showing the dose rate at any point in the room. A virtual dosimeter is built into the viewer to allow users to be fully immersed in the environment in which they will be working, without being exposed to actual radiation or other hazardous conditions. This technology can help save dose at operating nuclear power plants when used for planning large work scopes in high radiation areas and is valuable as a characterization tool for decommissioning facilities. Adopters of 3D gamma source mapping and intervention analysis save time, money, and dose by evaluating options well in advance of the performance of any work, and optimizing interventions using accurate modelling techniques to plan work evolutions. (author)

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Initial Assessment of Cover Degradation Features at the Mexican Hat, Utah, UMTRCA Disposal Site - 19556

The Mexican Hat, Utah, Uranium Mill Tailings Radiation Control Act (UMTRCA) Title I Disposal Site is located on the Navajo Reservation in southeast Utah. The US Nuclear Regulatory Commission licensed the site to the US Department of Energy Office of Legacy Management (LM) for custody and long-term care. LM manages long-term surveillance and maintenance activities at the site with the principal goal of protecting human health and the environment. The disposal cell was designed to encapsulate low-level radioactive mill tailings and other residual radioactive materials (RRM) in a way that minimizes the need for active maintenance and limits radon gas emanation and precipitation infiltration. The disposal cell has a multicomponent cover, consisting of a 60 cm thick (24 inch), low-permeability, bentonite-amended radon barrier, overlain by a 15 cm thick (6 inch) sandy gravel bedding/filter layer and a 30 cm thick (12 inch) riprap erosion-protection layer. Under UMTRCA, designs intended to control and contain RRM shall be effective for up to 1000 years, to the extent reasonably achievable and, in any case, for at least 200 years. In 2016, multiple subtle depressions were identified on the rock cover along the toe and lower portions of the northeast side slope of the disposal cell. Due to concerns regarding potential impacts to disposal cell performance and erosion resistance, evaluations of the depressions and cell cover design and construction were initiated. The evaluations included reviews of the disposal cell as-built drawings and supporting design calculations for the rock cover components. Also, in 2017, a weather monitoring station was installed at the site to collect continuous site-specific meteorological data, and repeatable ground-based light imaging, detection, and ranging (lidar) topographical and aerial photogrammetry surveys were implemented to monitor for potential changes in the surface depression features. The evaluations also included visual inspections of the depressions, and in 2018, small-area manual excavations of the rock cover components (test pits) were performed to observe the conditions of the cover components, scan for radioactivity, and observe evidence of erosion on the surface of the radon barrier material. Voids and incisions were discovered within the radon barrier on the north and northeast side slopes of the disposal cell. Visual observations at test pits indicate that the bedding/filter material is highly segregated and may not be in conformance with the disposal cell engineering and construction design specifications. Post-construction development of a weak to strongly cemented material has also been observed immediately below the base of the bedding layer in test pits with observed radon barrier degradation. A series of radiological surveys have been performed at the site, and radiological readings have not exceeded natural background conditions in the vicinity of the site. Thus, the site remains protective of human health and the environment. Implementation of continuous radiological monitoring at the site will be initiated in fall 2018 through the deployment of radon cups and thermoluminescent dosimeters to obtain data that provides supporting evidence that the disposal cell remains protective of human health and the environment. Evaluations to determine the cause(s) of the depression features and associated radon barrier erosion are ongoing. Possible mechanisms of cover degradation identified thus far include segregated bedding material that would allow for higher precipitation runoff velocities, resulting in erosion of the radon barrier; post-construction cementation of radon barrier or aeolian material that could negatively affect the performance of the radon barrier; cation exchange leading to the development of cementation; and aeolian deposition affecting precipitation runoff. Moreover, geotechnical sampling and testing is planned to verify spatial cover conditions relative to design specifications. The resulting information will be used to identify possible causes for the surface depressions and associated radon barrier degradation, gain insight on potential long-term performance implications along the side slopes of the disposal cell, and identify potential corrective actions. (authors)

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Gamma Imaging and Mapping Advancements

The SRNL developed GrayQb{sup TM} gamma mapping system has been successfully deployed in field situations. Currently, to get the image from the GrayQb{sup TM} the internal Phosphor Storage Plate (PSP) used to capture radiation images must be recovered and scanned by a ScanX Scanner. Upgrades are being implemented which will enable the GrayQB{sup TM} to read the PSP using a camera and red LEDs then transmit results to a remote location. This will greatly reduce personnel interaction, increasing safety as well as eliminating the need for the ScanX. Upgrades have been based off of the MiniMax, a Los Alamos National Laboratory developed PSP reading device constructed with a Nikon DSLR and a red LED flash to obtain the images from the PSP. The electronics in the upgraded GrayQb{sup TM} need to be both functional and environmentally rugged. A PC/104 was chosen for its wider operational temperature range and its physical durability. The Sony α7 ii and the Mightex are the candidate cameras for the upgrades based on test results. PSPs were exposed to gamma radiation sources at SRS's Health Physics Instrumentation Calibration Laboratory (HPICL). PSPs were tested with both Am-241 and Cs-137. Linear intensity increased with dose verifying UV image simulations. Data collected enabled the PSP intensity to be referenced to a total dose. Further work includes design and implementation of a 3D printed housing for the new camera system. The housing will include the camera, light flash, PSP holders, tungsten dual pinhole, PC/104, dosimeter, and a battery or tethering option. Once the housing is finalized further testing at the HPICL facility is planned for early August. During this testing, the final housing design will capture both Am-241 and Cs-137 images.

3D PRINTING↗

Analysis of Exposure during Transportation of Waste to the Nevada National Security Site (NNSS) - 20445

Safety is a priority for the U.S. Department of Energy (DOE) Environmental Management (EM) Nevada Program. This commitment to safety is integrated into requirements and work procedures at DOE sites across the U.S. that generate low-level radioactive waste, mixed low-level radioactive waste, and classified waste that is transported to the Nevada National Security Site (NNSS) for permanent disposal. Generators of this waste are responsible for ensuring it is packaged and transported in a safe and compliant manner. These generators and their contracted commercial carriers must comply with U.S. Department of Transportation (DOT) regulations; the Nevada National Security Site Waste Acceptance Criteria (NNSSWAC); and other applicable federal, state, and local regulations and requirements. This includes packaging and shipping the waste to meet DOT regulatory radiation dose limits to ensure public safety during transportation. NNSS waste generators have a solid safety record for complying with these stringent regulations as demonstrated by the fact that no shipments exceeding DOT dose rate limits were received at the NNSS Area 5 Radioactive Waste Management Complex (RWMC) during FY 2014 through FY 2018. A 2005 study conducted by the Desert Research Institute validated shipments to the NNSS comply with DOT radiation dose limits. In response to recent Nevada stakeholder requests for an updated study, an analysis was conducted to verify and provide evidence that the public continues to be safe from exposure to radioactive waste shipment to the NNSS. Radiation exposure from radioactive waste shipments in transit to the NNSS was evaluated. Three studies were performed: 1. Confirm compliance of waste shipments to the DOT radiation limits using dose rate surveys taken at the generator site and at the disposal site. 2. Estimate the dose to the public from waste shipments using the dosimetry results for disposal site personnel by comparing time of exposure for various individuals/scenarios. 3. Estimate the truck driver dose using the receipt dose rate surveys and time of exposure, and from dosimetry results. Study 1 confirmed compliance with the DOT dose rate limits for a sample of waste shipments (123 of 1,038) received during fiscal year (FY) 2017. Study 2 showed that the average annual radiation equivalent dose for disposal site personnel during FY 2017 was approximately 6.7% [0.415 mSv (41.5 millirem)] of the annual average dose that a person living in the U.S. receives from all sources [6.2 mSv (620 mrem)]. Maximum dose to a member of the public, a person resting/sleeping in an adjacent truck at a rest area to a waste shipment, was 0.0166 mSv (1.66 mrem), which is less than the dose received from a person taking a round trip from the east coast to the west coast of the continental U.S. on an airplane [0.07 mSv (7 mrem) per round trip]. Study 3 showed that the truck driver who made the most shipments of radioactive waste to the NNSS, who drove the most hours (estimated time of exposure 2,520 hours), during FY 2017 had a total dose of 0.15 mSv (15 mrem), which was obtained from their personal dosimeter. The annual dose recorded for disposal site personnel, the dose estimates for the public, and the truck driver dose were all a small percentage of the average radiation dose a person receives from all sources (e.g., background and medical radiation). At these levels, risk should only be described qualitatively. Radiation exposure from radioactive waste shipments to the NNSS were shown to be compliant with the DOT dose rate limits, safe, and very low (i.e., within background levels). (authors)

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