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CsRbNa2 crystallizes in the orthorhombic Immm space group. The structure is one-dimensional and consists of two CsRbNa2 ribbons oriented in the (0, 1, 0) direction. Cs is bonded in a linear geometry to two equivalent Na atoms. Both Cs–Na bond lengths are 4.15 Å. Rb is bonded in a linear geometry to two equivalent Na atoms. Both Rb–Na bond lengths are 4.04 Å. Na is bonded in a linear geometry to one Cs and one Rb atom.
Cs2RbNa crystallizes in the orthorhombic Immm space group. The structure is one-dimensional and consists of two Cs2RbNa ribbons oriented in the (0, 1, 0) direction. Cs is bonded in a linear geometry to one Rb and one Na atom. The Cs–Rb bond length is 4.89 Å. The Cs–Na bond length is 4.15 Å. Rb is bonded in a linear geometry to two equivalent Cs atoms. Na is bonded in a linear geometry to two equivalent Cs atoms.