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Results for “Charge-exchange reactions”

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At least 19 records
All sourcesNASA NTRSDOE OSTI
NASA NTRS1991

Momentum transfer in relativistic heavy ion charge-exchange reactions

Relativistic heavy ion charge-exchange reactions yield fragments (Delta-Z = + 1) whose longitudinal momentum distributions are downshifted by larger values than those associated with the remaining fragments (Delta-Z = 1, -2,...). Kinematics alone cannot account for the observed downshifts; therefore, an additional contribution from collision dynamics must be included. In this work, an optical model description of collision momentum transfer is used to estimate the additional dynamical momentum downshift. Good agreement between theoretical estimates and experimental data is obtained.

Townsend, L. W.↗
NASA NTRS1993

Energy-loss cross sections for inclusive charge-exchange reactions at intermediate energies

Charge-exchange reactions for scattering to the continuum are considered in a high-energy multiple scattering model. Calculations for (p,n) and (He-3,H-3) reactions are made and compared with experimental results for C-12, O-16, and Al-27 targets. Coherent effects are shown to lead to an important role for inelastic multiple scattering terms when light projectiles are considered.

Cucinotta, Francis A.↗
NASA NTRS1986

Delta excitations and shell-model information in heavy-ion, charge-exchange reactions

We calculate total cross sections for coherent pion production using localized plane-wave approximations for the shell-structure of valence nucleons that are excited to delta particles in the intermediate state in the (12C, 12B) and (12C, 12N) charge-exchange, heavy-ion reactions. We find comparable agreement to projectile downshift data for 12C(12C, 12B)12N. Then we improve the formalism by replacing the localized plane wave bound states with harmonic oscillator states which are imbedded in a multipole expansion approach and calculate pion differential cross sections to test for the sensitivity of the spectra to the single-particle mass parameter.

NASA Program Space Medicine↗
NASA NTRS1981

Parasitic current losses due to solar electric propulsion generated plasmas

Solar electric propulsion is a leading candidate for many upcoming space missions. Under many circumstances plasma produced by charge-exchange reactions within the ion beam dominates the ambient environment near the spacecraft. The calculations presented here contain a predictive hydrodynamic model for the charge-exchange plasma expansion, and a fully three-dimensional model for the structure of the plasma sheath around the solar array wing. Results of calculations for several configurations and voltage levels indicate that with kilovolt biases power losses of approximately 10 percent or more are likely, even with only one engine in operation, and that ameliorative measures should focus on the inboard portion of the solar arrays.

Katz, I.↗
NASA NTRS1991

Theoretical study of the bonding of Nb(2+) to CH2, C2H2, and C2H4

The bonding of Nb(2+) with CH2, C2H2, and C2H4 is studied by using electronic structure calculations that include high levels of electron correlation. The binding energy for NbCH2(2+) is in good agreement with the lower bound determined from the reaction with CH4 but is significantly smaller than the value determined from the binding energy and ionization potential of NbCH2(+). The calculations and a new interpretation of the experiment indicate that the larger value is in error primarily because the ionization potential of NbCH2(+) determined from bracketing charge-exchange reactions is too small. The computed binding energy of NbC2H2(2+) is in good agreement with experiment. The calculations show that the bonding is predominantly covalent in character for both NbCH2(2+) and NbC2H2(2+), whereas for NbC2H4(2+) the electronic states that are predominantly ionic and covalent are nearly degenerate. The trend in binding energies, CH2 greater than C2H2 greater than C2H4, is consistent with the energy required to prepare the ligands for bonding.

Bauschlicher, Charles W., Jr.↗
NASA NTRS1972

Oxygen and hydrogen ion densities above Millstone Hill.

Measurements of the vertical flux of oxygen ions, when combined with simultaneous measurements of electron density and of electron and ion temperatures, present a unique opportunity to examine conditions in the topside ionosphere. The measured fluxes and densities may be used directly to evaluate terms in the O+ continuity equation without requiring any assumptions to be made about neutral winds, electric fields, or the ambipolar diffusion coefficient. From observations at Millstone Hill we have, in this way, derived the rate of loss of O+ in the charge-exchange reaction with hydrogen, the rate of photoionization of atomic oxygen, and the rate of loss of O+ in reactions with N2 and O2. In combination with laboratory and theoretical results, these rates can be interpreted to yield number densities of the corresponding neutral species. When the measured fluxes are examined for consistency with measured density gradients and temperature profiles, we find clear evidence of wind-induced or electrodynamic vertical drifts larger than 60 m/sec.

Schunk, R. W.↗
NASA NTRS1977

Interstellar ultraviolet absorption lines and galactic X-ray sources

X-ray photoionization can create zones of highly ionized trace elements in the interstellar gas around a galactic X-ray source. Ultraviolet absorption lines due to the resulting ionic column densities may be observable and may provide information on the environment and age of the X-ray source. The calculated column densities are sensitive to the rates of charge-exchange reactions.

Mccray, R.↗
NASA NTRS1983

Escape and ionization of atomic oxygen from Io

Model calculations of the neutral O cloud of Io, based on atom-electron-impact excitation and ionization processes in the plasma torus, are presented. The model is quantitatively anchored to the 6300-A O I emission intensity observations of Brown (1981), and uses a plasma temperature and density structure based on Voyager 1 and 2 and EUV data. Parameters predicted by the model include satellite emission flux = 1.5 x 10 to the 9th/sq cm sec, ion-loading rate = 6.2 x 10 to the 26th ions/sec, O mass-loading rate = 16.6 kg/sec, and O ion-energy input rate = 2.7 x 10 to the 10th W. The spatial morphologies of the parameters are shown. Rough estimates obtained by accounting for a neutral S cloud and plasma-torus charge-exchange reactions include O source flux = 1.2 x 10 to the 10th/sq cm sec, ion-loading rate = 4.0 x 10 to the 27th ions/sec, ion-diffusive-loss time = 200 days, plasma mass-loading rate = 150 kg/sec, satellite mass-loss rate = 270 kg/sec, and maximum ion-energy input = 4 x 10 to the 11th W.

Smyth, W. H.↗
NASA NTRS1993

Characterization of in-flight performance of ion propulsion systems

In-flight measurements of ion propulsion performance, ground test calibrations, and diagnostic performance measurements were reviewed. It was found that accelerometers provided the most accurate in-flight thrust measurements compared with four other methods that were surveyed. An experiment has also demonstrated that pre-flight alignment of the thrust vector was sufficiently accurate so that gimbal adjustments and use of attitude control thrusters were not required to counter disturbance torques caused by thrust vector misalignment. The effects of facility background pressure, facility enhanced charge-exchange reactions, and contamination on ground-based performance measurements are also discussed. Vacuum facility pressures for inert-gas ion thruster life tests and flight qualification tests will have to be less than 2 mPa to ensure accurate performance measurements.

Sovey, James S.↗
NASA NTRS1993

Characterization of in-flight performance of ion propulsion systems

In-flight measurements of ion propulsion performance, ground test calibrations, and diagnostic performance measurements were reviewed. It was found that accelerometers provided the most accurate in-flight thrust measurements compared with four other methods that were surveyed. An experiment has also demonstrated that pre-flight alignment of the thrust vector was sufficiently accurate so that gimbal adjustments and use of attitude control thrusters were not required to counter disturbance torques caused by thrust vector misalignment. The effects of facility background pressure, facility enhanced charge-exchange reactions, and contamination on ground-based performance measurements are also discussed. Vacuum facility pressures for inert-gas ion thruster life tests and flight qualification tests will have to be less than 2 mPa to ensure accurate performance measurements.

Sovey, James S.↗
NASA NTRS1976

Abundances of simple oxygen-bearing molecules and ions in interstellar clouds

The abundances of simple oxygen-bearing interstellar molecules in warm (T at least 40 K), diffuse, and moderately thick clouds are calculated on the basis of binary gas-phase reactions. The most important reactions are ion-molecule, charge-exchange, and dissociative-recombination reactions, as suggested mainly by earlier workers. The progenitor of these molecules in diffuse clouds is the cosmic-ray-produced H(+) ion, working through the charge-exchange reaction with O. The ionization of H(+) and He(+) is also discussed. Dissociative charge exchange of He(+) with H2 is an important source of H(+) in regions of large fractional abundance of H2, as well as an important destruction mechanism for He(+) even for small f (at least 0.1). The calculated molecular abundances are consistent with some of the available observational information.

Glassgold, A. E.↗
NASA NTRS1982

Charge exchange in the Io torus and exosphere

Charge-exchange cross sections and their velocity dependence have been estimated for the most important reactions in the Io torus and exosphere. The methods used for calculating the cross sections are given and discussed in some detail. For symmetric-resonant single and double charge exchange, the cross sections are slowly varying functions of velocity. For inelastic charge-exchange collisions, the transition probabilities into a given final state can depend critically on velocity. Models are described which can be used to estimate both the most rapid charge-exchange processes and those states which play an important role. Calculated cross sections are used to obtain reaction rates as a function of radial position, demonstrating the importance of charge exchange in the inner torus. Charge-exchange reactions of torus ions with molecular species in Io's exosphere may yield a net supply of neutrals and plasma to the torus.

Johnson, R. E.↗
NASA NTRS1972

Metallic ions in the equatorial ionosphere

Four positive ion composition measurements of the equatorial E region made at Thumba, India, are presented. During the day, the major ions between 90 and 125 km are NO(+) and O2(+). A metallic ion layer centered at 92 km is observed, and found to contain Mg(+), Fe(+), Ca(+), K(+), Al(+), and Na(+) ions. The layer is explained in terms of a similarly shaped latitude distribution of neutral atoms which are photoionized and charge-exchanged with NO(+) and O2(+). Three body reactions form molecular metallic ions which are rapidly lost by dissociative ion-electron recombination. Nighttime observations show downward drifting of the metallic ion layer caused by equatorial dynamo effects. These ions react and form neutral metals which exchange charges with NO(+) and O2(+) to produce an observed depletion of those ions within the metallic ion region.

Aikin, A. C.↗
NASA NTRS1972

Molecular ions in the F2 layer.

Data on ion concentrations at heights of 400-500 km, obtained by the OGO VI satellite, suggest that the O(+) and molecular ion concentrations are sometimes anticorrelated. To assist in explaining this phenomenon, a table of the chemical reactions most likely to control the molecular ion concentrations is drawn up, and its validity tested with the aid of data from rocket-borne mass spectrometers at heights of 220-400 km. The anticorrelation of O(+) and NO(+) ions by day is thought to be due to the importance of a reaction between N2(+) ions and O atoms; the main source of N2(+) above 300 km is probably charge-exchange between N2 and O(+), the latter being produced by photoionization. However, at night another source of NO(+) ions is required, which may be N(+) ions that are either stored in the magnetosphere or are produced from He(+) and N2.

Rishbeth, H.↗
NASA NTRS1994

Formation of Na-containing molecular ions at Io

Fast sodium atoms, which appear to be associated with the motion of the magnetic 'field lines' downstream from Io (Schneider et al. 1991), are thought to be produced by dissociation of NaX(+) in Io's plasma torus. It was suggested that these molecular ions are formed near Io's exobase by electron-impact ionization and picked up be the corotating filed lines (Wilson and Schneider 1994). Because electron cooling processes dominate electron-impact ionization in Io's corona, two reactions are suggested here as sources of NaX(+) and, hence, as the ultimate sources of the observed fast Na. First, the charge-exchange cross sections for forming NaX(+) are shown to be large for plasma torus ions (O(+), S(+), O(2+), S(3+)) colliding with NaX molecules in Io's corona. Sputtering from the surface (Chrisey et al. 1988) and rapid transport to the exobase is a potential source of NaX, where X is O,S, Na, or a molecular species such as NaS or O2. Second ions of the more abundant molecules (e.g., SO(+), SO2(+), O2(+), and S2(+)) can react efficiently with atomic Na in Io's corona to form NaX(+). Here cross sections are estimated for these two processes, as well as for charge exchange in O(+) and S(+) on Na collisions.

Johnson, R. E.↗
NASA NTRS1983

A deficiency of O III in the Io plasma torus

Evidence for a deficiency of O III ions in the Io plasma torus is reported and implications of this deficiency for the physical processes controlling the plasma are considered. Observations of the O III 5007-A as well as Cl III and S III emissions from the Io plasma torus were made by a ground-based echelle spectrograph and intensified Reticon detector in February and May, 1981. The O III observations allow an upper limit of 4/cu cm to be placed on torus O III abundance, which is inconsistent with expectations for a low density plasma controlled by electron collisions. The inclusion of ion-ion and ion-atom charge exchange reactions and a depleted high energy electron component in the model is found to suppress O III levels, however observed limiting values are only achieved if it is assumed that the O III is kinetically hot. In addition, the charge-exchange model developed is inconsistent with previous observations of the kinetics of the S II-S III system. The present observations also establish upper limits of 2 R on 5518-A and 5538-A Cl III emission, and an emission rate of 58 + or - 40 R for the S III 6312-A line in the hot torus.

Brown, R. A.↗