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All sourcesNASA NTRSDOE OSTI
DOE OSTI2016

Nuclear Data Sheets for A = 79

Nuclear spectroscopic information for known nuclides of mass number 79 (Ni,Cu,Zn,Ga,Ge,As,Se,Br,Kr,Rb, Sr,Y,Zr) has been evaluated and presented together with adopted energies, Jπ, and decay modes of levels in these nuclei. No data are yet available for excited states in {sup 79}Ni, {sup 79}Cu and {sup 79}Zr. The half–life of {sup 79}Se, a nuclide of importance in reactor–irradiated fuel composition has been measured by several independent groups and reported in a number of publications after 1995, and seems to be converging to a narrow margin of experimental values. These measurements were likely prompted by a recommendation made in the 1993 update of A = 79 nuclides (1993Si28), that since a 1949PaZZ report, there had been no measurement until 1993, and that based on simulation studies by 1993HeZW, the value listed in 1949PaZZ, and cited in all data tables and charts for 44 years, was quite likely in error, being too low by a factor of 10. According to conclusions in recent papers such as 2014Do20, there is still room for improvement in the measurement of this half–life, and further experiments are expected. This evaluation supersedes earlier Nuclear Data Sheets for A = 79 (2002Si13,1993Si28, 1982Si21,1975Ur03).

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2016

Immunotoxicological and neurotoxicological profile of health effects following subacute exposure to geogenic dust from sand dunes at the Nellis Dunes Recreation Area, Las Vegas, NV

Exposure to geogenic particulate matter (PM) comprised of mineral particles has been linked to human health effects. However, very little data exist on health effects associated with geogenic dust exposure in natural settings. Therefore, we characterized particulate matter size, metal chemistry, and health effects of dust collected from the Nellis Dunes Recreation Area (NDRA), a popular off-road vehicle area located near Las Vegas, NV. Adult female B6C3F1 mice were exposed to several concentrations of mineral dust collected from active and vegetated sand dunes in NDRA. Dust samples (median diameter: 4.4 μm) were suspended in phosphate-buffered saline and delivered at concentrations ranging from 0.01 to 100 mg dust/kg body weight by oropharyngeal aspiration. ICP-MS analyses of total dissolution of the dust resulted in aluminum (55,090 μg/g), vanadium (70 μg/g), chromium (33 μg/g), manganese (511 μg/g), iron (21,600 μg/g), cobalt (9.4 μg/g), copper (69 μg/g), zinc (79 μg/g), arsenic (62 μg/g), strontium (620 μg/g), cesium (13 μg/g), lead 25 μg/g) and uranium (4.7 μg/g). Arsenic was present only as As(V). Mice received four exposures, once/week over 28-days to mimic a month of weekend exposures. Descriptive and functional assays to assess immunotoxicity and neurotoxicity were performed 24 h after the final exposure. The primary observation was that 0.1 to 100 mg/kg of this sand dune derived dust dose-responsively reduced antigen-specific IgM antibody responses, suggesting that dust from this area of NDRA may present a potential health risk. - Graphical abstract: During periods of heavy wind erosion, dense dust clouds of locally emitted geogenic dust enrobe the central Nellis Dune Recreation Area dunes. - Highlights: • Toxicological effects were characterized specific to geogenic dust exposure from a recreational sand dune site in Nevada. • The geogenic dust is a mixture of many metals and crystalline silica. • Exposure to geogenic dust dose-responsively decreased IgM antibody responses in a mouse model.

60 APPLIED LIFE SCIENCES↗
DOE OSTI2013

A new method for imaging nuclear threats using cosmic ray muons

Muon tomography is a technique that uses cosmic ray muons to generate three-dimensional images of volumes using information contained in the Coulomb scattering of the muons. Advantages of this technique are the ability of cosmic rays to penetrate significant overburden and the absence of any additional dose delivered to subjects under study beyond the natural cosmic ray flux. Disadvantages include the relatively long exposure times and poor position resolution and complex algorithms needed for reconstruction. Furthermore, we demonstrate a new method for obtaining improved position resolution and statistical precision for objects with spherical symmetry.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2015

Surface purity control during XMASS detector refurbishment

The XMASS project aims at detecting dark matter, pp and {sup 7}Be solar neutrinos, and neutrino less double beta decay using large volume of pure liquid xenon. The first physics target of the XMASS project is to detect dark matter with 835 kg liquid xenon. After the commissioning runs, XMASS detector was refurbished to minimize the background contribution mainly from PMT sealing material and we restarted data taking in November 2013. We report how we control surface purity, especially how we prevent radon daughter accumulation on the detector copper surface, during XMASS detector refurbishment. The result and future plan of XMASS are also reported.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2016

THE EXTREME ULTRAVIOLET SPECTRUM OF HIGHLY CHARGED COPPER IONS

This paper reports the laboratory measurements of extreme ultraviolet spectra of highly charged copper ions. In this work, 82 lines from Cu xv to Cu xxiii in the 160–360 Å wavelength range are identified as the transitions of the 2p{sup 2}3p–2p{sup 2}3d, 2p{sup 4}3s–2p{sup 4}3p, 2p{sup 4}3p–2p{sup 4}3d, 2p{sup 5}3s–2p{sup 5}3p, 2p{sup 5}3s–2p{sup 5}3p, 3s3p–3p{sup 2}, 3s{sup 2}3p{sup 3}-3s3p{sup 4}, 3s{sup 2}3p–3s3p{sup 2}, 3s{sup 2}3p{sup 3}–3s3p{sup 4}, and 2p{sup 4} ({sup 3}P)3s–2p{sup 4} ({sup 3}P) 3p, in which 40 spectral lines have been newly and accurately measured. Their identification is based on comparisons with available experimental and theoretical values and the calculations with Cowan codes.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2016

A STUDY OF THE ELEMENTS COPPER THROUGH URANIUM IN SIRIUS A: CONTRIBUTIONS FROM STIS AND GROUND-BASED SPECTRA

We determine abundances or upper limits for all of the 55 stable elements from copper to uranium for the A1 Vm star Sirius. The purpose of the study is to assemble the most complete picture of elemental abundances with the hope of revealing the chemical history of the brightest star in the sky, apart from the Sun. We also explore the relationship of this hot metallic-line (Am) star to its cooler congeners, as well as the hotter, weakly- or non-magnetic Mercury-manganese (HgMn) stars. Our primary observational material consists of Hubble Space Telescope ( HST ) spectra taken with the Space Telescope Imaging Spectrograph in the ASTRAL project. We have also used archival material from the COPERNICUS satellite, and from the HST Goddard High-Resolution Spectrograph, as well as ground-based spectra from Furenlid, Westin, Kurucz, Wahlgren, and their coworkers, ESO spectra from the UVESPOP project, and NARVAL spectra retrieved from PolarBase. Our analysis has been primarily by spectral synthesis, and in this work we have had the great advantage of extensive atomic data unavailable to earlier workers. We find most abundances as well as upper limits range from 10 to 100 times above solar values. We see no indication of the huge abundance excesses of 1000 or more that occur among many chemically peculiar stars of the upper main sequence. The picture of Sirius as a hot Am star is reinforced.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2014

New detections of arsenic, selenium, and other heavy elements in two metal-poor stars

We use the Space Telescope Imaging Spectrograph on board the Hubble Space Telescope to obtain new high-quality spectra covering the 1900 ≤λ ≤ 2360 Å wavelength range for two metal-poor stars, HD 108317 and HD 128279. We derive abundances of Cu II, Zn II, As I, Se I, Mo II, and Cd II, which have not been detected previously in either star. Abundances derived for Ge I, Te I, Os II, and Pt I confirm those derived from lines at longer wavelengths. We also derive upper limits from the non-detection of W II, Hg II, Pb II, and Bi I. The mean [As/Fe] ratio derived from these two stars and five others in the literature is unchanged over the metallicity range –2.8 < [Fe/H] <–0.6, ([As/Fe]) = +0.28 ± 0.14 (σ = 0.36 dex). The mean [Se/Fe] ratio derived from these two stars and six others in the literature is also constant, ([Se/Fe]) = +0.16 ± 0.09 (σ = 0.26 dex). The As and Se abundances are enhanced relative to a simple extrapolation of the iron-peak abundances to higher masses, suggesting that this mass region (75 ≤A ≤ 82) may be the point at which a different nucleosynthetic mechanism begins to dominate the quasi-equilibrium α-rich freezeout of the iron peak. ([Cu II/Cu I]) = +0.56 ± 0.23 in HD 108317 and HD 128279, and we infer that lines of Cu I may not be formed in local thermodynamic equilibrium in these stars. The [Zn/Fe], [Mo/Fe], [Cd/Fe], and [Os/Fe] ratios are also derived from neutral and ionized species, and each ratio pair agrees within the mutual uncertainties, which range from 0.15 to 0.52 dex.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2018

Description of Differential Cross Sections for {sup 63}Cu + p Nuclear Reactions Induced by High-Energy Cosmic-Ray Protons

The results of calculation of {sup 63}Cu + p differential cross sections at incident-proton energies between 10 and 200 MeV and a comparative analysis of these results are presented as a continuation of the earlier work of our group on developing methods for calculating the contribution of nuclear reactions to radiative effects arising in the onboard spacecraft electronics under the action of high-energy cosmic-ray protons on {sup 63}Cu nuclei (generation of single-event upsets) and as a supplement to the earlier calculations performed on the basis of the TАLYS code in order to determine elastic- and inelastic-scattering cross sections and charge, mass, and energy distributions of recoil nuclei (heavy products of the {sup 63}Cu + p nuclear reaction). The influence of various mechanisms of the angular distributions of particles emitted in the {sup 63}Cu + p nuclear reaction is also discussed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2015

Non-LTE analysis of neutral copper in late-type metal-poor stars

We investigated the copper abundances of 64 late-type stars in the Galactic disk and halo with effective temperatures from 5400 to 6700 K and [Fe/H] from −1.88 to −0.17. For the first time, the copper abundances are derived using both local thermodynamic equilibrium (LTE) and non-local thermodynamic equilibrium (non-LTE) calculations. High-resolution (R>40,000), high signal-to-noise ratio (S/N>100) spectra from the FOCES spectrograph are used. The atmospheric models are calculated based on the MAFAGS opacity sampling code. All the abundances are derived using spectrum synthesis methods. Our results indicate that the non-LTE effects of copper are important for metal-poor stars, showing a departure of ∼0.17 dex at a metallicity of ∼−1.5. We also find that the copper abundances derived from non-LTE calculations are enhanced compared with those from LTE. The enhancements show clear dependence on the metallicity, which gradually increases with decreasing [Fe/H] for our program stars, leading to a flatter distribution of [Cu/Fe] with [Fe/H] than previous work. There is a hint that the thick- and thin-disk stars have different behaviors in [Cu/Fe], and bending of the disk stars may exist.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2014

New probe of M1 and E1 strengths in GDR regions

The M1 strengths (or level density of 1{sup +} states) are of importance for estimation of interaction strengths between neutrinos and nuclei for the study of the supernova neutrino-process. In 1957, Agodi predicted theoretically angular distribution of neutrons emitted from states excited via dipole transitions with linearly polarized gamma-ray beam at the polar angle of θ=90° should be followed by a simple function, a + b cos(2φ), where φ, is azimuthal angel. However, this theoretical prediction has not been verified over the wide mass region except for light nuclei as deuteron. We have measured neutron angular distributions with (polarized gamma, n) reactions on Au, Nal, and Cu. We have verified the Agodi's prediction for the first time over the wide mass region. This suggests that (polarized gamma, n) reactions may be useful tools to study M1 strengths in giant resonance regions.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2014

Statistical equilibrium of copper in the solar atmosphere

Non-local thermodynamic equilibrium (NLTE) line formation for neutral copper in the one-dimensional solar atmospheres is presented for the atomic model, including 96 terms of Cu I and the ground state of Cu II. The accurate oscillator strengths for all the line transitions in model atom and photoionization cross sections were calculated using the R-matrix method in the Russell-Saunders coupling scheme. The main NLTE mechanism for Cu I is the ultraviolet overionization. We find that NLTE leads to systematically depleted total absorption in the Cu I lines and, accordingly, positive abundance corrections. Inelastic collisions with neutral hydrogen atoms produce minor effects on the statistical equilibrium of Cu I in the solar atmosphere. For the solar Cu I lines, the departures from LTE are found to be small, the mean NLTE abundance correction of ∼0.01 dex. It was found that the six low-excitation lines, with excitation energy of the lower level E {sub exc} ≤ 1.64 eV, give a 0.14 dex lower mean solar abundance compared to that from the six E {sub exc} > 3.7 eV lines, when applying experimental gf-values of Kock and Richter. Without the two strong resonance transitions, the solar mean NLTE abundance from 10 lines of Cu I is log ε{sub ☉}(Cu) = 4.19 ± 0.10, which is consistent within the error bars with the meteoritic value 4.25 ± 0.05 of Lodders et al. The discrepancy between E {sub exc} = 1.39-1.64 eV and E {sub exc} > 3.7 eV lines can be removed when the calculated gf-values are adopted and a mean solar abundance of log ε{sub ☉}(Cu) = 4.24 ± 0.08 is derived.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2015

EXPLORING ANTICORRELATIONS AND LIGHT ELEMENT VARIATIONS IN NORTHERN GLOBULAR CLUSTERS OBSERVED BY THE APOGEE SURVEY

We investigate the light-element behavior of red giant stars in northern globular clusters (GCs) observed by the SDSS-III Apache Point Observatory Galactic Evolution Experiment. We derive abundances of 9 elements (Fe, C, N, O, Mg, Al, Si, Ca, and Ti) for 428 red giant stars in 10 GCs. The intrinsic abundance range relative to measurement errors is examined, and the well-known C–N and Mg–Al anticorrelations are explored using an extreme-deconvolution code for the first time in a consistent way. We find that Mg and Al drive the population membership in most clusters, except in M107 and M71, the two most metal-rich clusters in our study, where the grouping is most sensitive to N. We also find a diversity in the abundance distributions, with some clusters exhibiting clear abundance bimodalities (for example M3 and M53) while others show extended distributions. The spread of Al abundances increases significantly as cluster average metallicity decreases as previously found by other works, which we take as evidence that low metallicity, intermediate mass AGB polluters were more common in the more metal-poor clusters. The statistically significant correlation of [Al/Fe] with [Si/Fe] in M15 suggests that {sup 28}Si leakage has occurred in this cluster. We also present C, N, and O abundances for stars cooler than 4500 K and examine the behavior of A(C+N+O) in each cluster as a function of temperature and [Al/Fe]. The scatter of A(C+N+O) is close to its estimated uncertainty in all clusters and independent of stellar temperature. A(C+N+O) exhibits small correlations and anticorrelations with [Al/Fe] in M3 and M13, but we cannot be certain about these relations given the size of our abundance uncertainties. Star-to-star variations of α-element (Si, Ca, Ti) abundances are comparable to our estimated errors in all clusters.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2018

An Analysis of Frenkel Defects and Backgrounds Modeling for SuperCDMS Dark Matter Searches

Years of astrophysical observations suggest that dark matter comprises more than $\sim$ 80 % of all matter in the universe. Particle physics theories favor a weakly-interacting particle that could be directly detected in terrestrial experiments. The Super Cryogenic Dark Matter Search (SuperCDMS) Collaboration operates world-leading experiments to directly detect dark matter interacting with ordinary matter. The SuperCDMS Soudan experiment searched for weakly interacting massive particles (WIMPs) via their elastic-scattering interactions with nuclei in low-temperature germanium detectors. During the operation of the SuperCDMS Soudan experiment, $^{210}$Pb sources were installed to study background rejection of the Ge detectors. Data from these sources were used to investigate energy loss associated with Frenkel defect formation in germanium crystals at mK temperatures. The spectrum of $^{206}$Pb nuclear recoils was examined near its expected 103 keV endpoint energy to extract the first experimentally determined average displacement threshold energy of 19.7 $\pm$ 0.5 (stat) $\pm$ 0.1 (syst) eV for germanium. This has implications for the sensitivity of future germanium-based dark matter searches including the SuperCDMS SNOLAB experiment. The SuperCDMS SNOLAB experiment will employ germanium and silicon detectors to improve current WIMP-search results by at least one order of magnitude for masses $\leq$ 10 GeV/c$^2$. This will require substantial shielding against cosmogenic and radiogenic backgrounds. The SuperCDMS SNOLAB passive shield will be permanent for the duration of the experiment so extensive simulations were undertaken to optimize the shield design. This resulted in a design of an outer layer of 60 cm of water, a middle layer of 20 cm of lead, and 30 cm of polyethylene which limits the background rate to that required for the primary physics goals of the experiments. The experiment will begin operations in 2020 and care must be taken during the construction phase to limit exposure to the $\pm$ 135 Bq/m$^3$ radon activity in the laboratory. The daughter products of $^{222}$Rn can attach to nearby surfaces leaving long-lived $^{210}$Pb in place for the duration of the experiment. For non-line-of-sight surfaces of the polyethylene shield, the maximum allowable $^{210}$Pb activity is 10,000 nBq/cm$^2$. A study was conducted to experimentally determine the contamination rate of polyethylene and copper by exposing samples for 83 days at SNOLAB. From the resulting surface activities, obtained from high-sensitivity measurements of alpha emissivity using the XIA UltraLo-1800 spectrometer, the average $^{210}$Pb plate-out rate was determined to be 249 and 423 atoms/day/cm$^2$ for polyethylene and copper, respectively. A time-dependent model of alpha activity was

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2013

NUCLEOSYNTHESIS IN THE OUTFLOWS ASSOCIATED WITH ACCRETION DISKS OF TYPE II COLLAPSARS

We investigate nucleosynthesis inside the outflows from gamma-ray burst (GRB) accretion disks formed by the Type II collapsars. In these collapsars, massive stars undergo core collapse to form a proto-neutron star initially, and a mild supernova (SN) explosion is driven. The SN ejecta lack momentum, and subsequently this newly formed neutron star gets transformed to a stellar mass black hole via massive fallback. The hydrodynamics and the nucleosynthesis in these accretion disks have been studied extensively in the past. Several heavy elements are synthesized in the disk, and much of these heavy elements are ejected from the disk via winds and outflows. We study nucleosynthesis in the outflows launched from these disks by using an adiabatic, spherically expanding outflow model, to understand which of these elements thus synthesized in the disk survive in the outflow. While studying this, we find that many new elements like isotopes of titanium, copper, zinc, etc., are present in the outflows. {sup 56}Ni is abundantly synthesized in most of the cases in the outflow, which implies that the outflows from these disks in a majority of cases will lead to an observable SN explosion. It is mainly present when outflow is considered from the He-rich, {sup 56}Ni/{sup 54}Fe-rich zones of the disks. However, outflow from the Si-rich zone of the disk remains rich in silicon. Although emission lines of many of these heavy elements have been observed in the X-ray afterglows of several GRBs by Chandra, BeppoSAX, XMM-Newton, etc., Swift seems to have not yet detected these lines.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2012

TWO EXTRASOLAR ASTEROIDS WITH LOW VOLATILE-ELEMENT MASS FRACTIONS

Using ultraviolet spectra obtained with the Cosmic Origins Spectrograph on the Hubble Space Telescope, we extend our previous ground-based optical determinations of the composition of the extrasolar asteroids accreted onto two white dwarfs, GD 40 and G241-6. Combining optical and ultraviolet spectra of these stars with He-dominated atmospheres, 13 and 12 polluting elements are confidently detected in GD 40 and G241-6, respectively. For the material accreted onto GD 40, the volatile elements C and S are deficient by more than a factor of 10 and N by at least a factor of 5 compared to their mass fractions in primitive CI chondrites and approach what is inferred for bulk Earth. A similar pattern is found for G241-6 except that S is undepleted. We have also newly detected or placed meaningful upper limits for the amount of Cl, Al, P, Ni, and Cu in the accreted matter. Extending results from optical studies, the mass fractions of refractory elements in the accreted parent bodies are similar to what is measured for bulk Earth and chondrites. Thermal processing, perhaps interior to a snow line, appears to be of central importance in determining the elemental compositions of these particular extrasolar asteroids.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2012

SENSITIVITY OF ASTROPHYSICAL REACTION RATES TO NUCLEAR UNCERTAINTIES

Sensitivities of nuclear reaction rates to a variation of nuclear properties are studied. Target nuclei range from proton- to neutron dripline for 10 {<=} Z {<=} 83. Reactions considered are nucleon- and {alpha}-induced reactions mediated by strong interaction. The contribution of reactions occurring on the target ground state to the total stellar rate is also given. General dependencies on various input quantities are discussed. Additionally, sensitivities of laboratory cross-sections of nucleon-, {alpha}-, and {gamma}-induced reactions are shown, allowing us to estimate the impact of cross-section measurements. Finally, recommended procedures to explore and improve reaction rate uncertainties using the present sensitivity data are outlined.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2015

Nanosecond Nd-YAG laser induced plasma emission characteristics in low pressure CO{sub 2} ambient gas for spectrochemical application on Mars

An experimental study is conducted on the possibility and viability of performing spectrochemical analysis of carbon and other elements in trace amount in Mars, in particular, the clean detection of C, which is indispensible for tracking the sign of life in Mars. For this study, a nanosecond Nd-YAG laser is employed to generate plasma emission from a pure copper target in CO{sub 2} ambient gas of reduced pressure simulating the atmospheric condition of Mars. It is shown that the same shock wave excitation mechanism also works this case while exhibiting remarkably long cooling stage. The highest Cu emission intensities induced by 4 mJ laser ablation energy is attained in 600 Pa CO{sub 2} ambient gas. Meanwhile the considerably weaker carbon emission from the CO{sub 2} gas appears relatively featureless over the entire range of pressure variation, posing a serious problem for sensitive trace analysis of C contained in a solid sample. Our time resolved intensity measurement nevertheless reveals earlier appearance of C emission from the CO{sub 2} gas with a limited duration from 50 ns to 400 ns after the laser irradiation, well before the initial appearance of the long lasting C emission from the solid target at about 1 μs, due to the different C-releasing processes from their different host materials. The unwanted C emission from the ambient gas can thus be eliminated from the detected spectrum by a proper time gated detection window. The excellent spectra of carbon, aluminum, calcium, sodium, hydrogen, and oxygen obtained from an agate sample are presented to further demonstrate and verify merit of this special time gated LIBS using CO{sub 2} ambient gas and suggesting its viability for broad ranging in-situ applications in Mars.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗