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At least 19 records
All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Numerical case study of the aerosol–cloud interactions in warm boundary layer clouds over the eastern North Atlantic with an interactive chemistry module

The presence of warm boundary layer stratiform clouds over the eastern North Atlantic (ENA) region is commonly influenced by the Azores High, especially during the summer season. To investigate comprehensive aerosol–cloud interactions, this study employs the Weather Research and Forecasting model coupled with a chemistry component (WRF-Chem), incorporating aerosol chemical components that are relevant to the formation of cloud condensation nuclei (CCN) and accounting for aerosol spatiotemporal variation. This study focuses on aerosol indirect effects, particularly the long-range transport of aerosols, in the ENA region under three different weather regimes: a ridge with a surface high-pressure system, a post-trough with a surface high-pressure system, and a weak trough. The WRF-Chem simulations conducted at a near-large-eddy scale offer valuable insights into the model's performance, especially in terms of its ability to use high spatial resolution to capture mesoscale cloud features across various weather regimes. Our result shows that introducing 5 times more aerosols to either non-precipitating or precipitating clouds significantly increases ambient CCN numbers, resulting in, to varying degrees, higher liquid water path (LWP) values. The substantial aerosol–cloud interaction especially occurs in the precipitating clouds and demonstrates the susceptibility of the LWP to changes in CCN under different regimes. Conversely, thin, non-rain clouds at the edges of a cloud system are prone to evaporation, exhibiting an aerosol drying effect. The aerosols released during this process transition back to the accumulation mode, facilitating future activation. This dynamic behavior is not adequately represented in prescribed-aerosol simulations.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1978

Radio observations of interstellar CN toward diffuse clouds, dark clouds, black clouds, and circumstellar clouds

Emission at 113 GHz from the CN molecule has been searched for in a large number of interstellar regions, primarily dark dust clouds. Lines have been detected in four dark clouds, the first time CN has been observed in this type of object. Comparative CO observations were also performed. The CN/CO abundance ratio varies from cloud to cloud, even among objects which are apparently otherwise similar. This variation suggests that the chemistry of dark clouds may be time-dependent. A previously reported detection of CN emission from a diffuse cloud was not confirmed. Several black clouds and circumstellar clouds were reobserved to obtain better line parameters and to serve as comparative interstellar chemical systems.

Allen, M.↗
DOE OSTI2023

The Role of Cloud–Cloud Interactions in the Life Cycle of Shallow Cumulus Clouds

Some of the climate research puzzles relate to a limited understanding of the critical factors governing the life cycle of cumulus clouds. These factors force the initiation and the various mixing processes during cloud life cycles. To shed some light into these processes, we tracked the life cycle of thousands of individual shallow cumulus clouds in a large-eddy simulation during the Holistic Interactions of Shallow Clouds, Aerosols, and Land-Ecosystems field campaign in the U.S. southern Great Plains. Concurrent evolution of clouds is tracked and their respective neighboring clouds are examined. Results show that the clouds initially smaller than neighboring clouds can grow larger than the neighboring clouds by a factor of 2 within 20% of their lifetime. Two groups of the tracked clouds with growing and decaying neighboring clouds, respectively, show distinct characteristics in their life cycles. Clouds with growing neighboring clouds form above regions with larger surface heterogeneity, whereas clouds with decaying neighboring clouds are associated with less heterogeneous surfaces. Also, those with decaying neighboring clouds experience larger instability and a more humid boundary layer, indicating evaporation below the cloud base is likely occurring before those clouds are formed. Larger instability leads to higher vertical velocity and convergence within the cloud, which causes stronger surrounding downdrafts and water vapor removal in the surrounding area. The latter appears to be the reason for the decaying neighboring clouds. Finally, understanding those processes provide insights into how cloud–cloud interactions modulate the evolution of cloud population and into how this evolution can be represented in future cumulus parameterizations.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

The Effects of Shallow Cumulus Cloud Shape on Interactions Among Clouds and Mixing With Near-Cloud Environments

Cloud lifecycles are influenced by interactions among clouds and mixing with cloud-free environments. Cloud shapes dictate the length of cloud boundaries, which affects these interactions. This study uses a large eddy simulation to examine the relationships between the shallow cumulus cloud shapes, processes at their boundaries, and lifecycles. To characterize the shape of clouds, two metrics are newly defined: one reflects the overall horizontal cloud shape, and the other defines the cloud edge irregularity. Simulated clouds experience increased irregularity, but little changes in aspect ratio. Irregularity-driven cloud perimeter growth strongly indicates cloud splitting, with a more pronounced effect than aspect ratio-driven perimeter growth. Smaller cloud-shell gradients of properties across cloud boundaries are associated with more irregular clouds, suggesting enhanced mixing of clouds with the cloud-free environment. These findings indicate that the shallow cumulus evolution is partly driven by the irregularity of the cloud edge through lateral mixing and cloud splitting.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS2007

Statistical Analyses of Satellite Cloud Object Data from CERES: Comparison with Cloud-Resolving Model Simulations of Tropical Convective Clouds - Part III

The present study evaluates the ability of a cloud-resolving model (CRM) to simulate the physical properties of tropical deep convective cloud objects identified from a Clouds and the Earth s Radiant Energy System (CERES) data product. The emphasis of this study is the comparisons among the small-, medium- and large-size categories of cloud objects observed during March 1998 and between the large-size categories of cloud objects observed during March 1998 (strong El Ni o) and March 2000 (weak La Ni a). Results from the CRM simulations are analyzed in a way that is consistent with the CERES retrieval algorithm and they are averaged to match the scale of the CERES satellite footprints. Cloud physical properties are analyzed in terms of their summary histograms for each category. It is found that there is a general agreement in the overall shapes of all cloud physical properties between the simulated and observed distributions. Each cloud physical property produced by the CRM also exhibits different degrees of disagreement with observations over different ranges of the property. The simulated cloud tops are generally too high and cloud top temperatures are too low except for the large-size category of March 1998. The probability densities of the simulated top-of-the-atmosphere (TOA) albedos for all four categories are underestimated for high albedos, while those of cloud optical depth are overestimated at its lowest bin. These disagreements are mainly related to uncertainties in the cloud microphysics parameterization and inputs such as cloud ice effective size to the radiation calculation. Summary histograms of cloud optical depth and TOA albedo from the CRM simulations of the large-size category of cloud objects do not differ significantly between the March 1998 and 2000 periods, consistent with the CERES observations. However, the CRM is unable to reproduce the significant differences in the observed cloud top height while it overestimates the differences in the observed outgoing longwave radiation and cloud top temperature between the two periods. Comparisons between the CRM results and the observations for most parameters in March 1998 consistently show that both the simulations and observations have larger differences between the large- and small-size categories than between the large- and medium-size, or between the medium- and small-size categories. However, the simulated cloud properties do not change as much with size as observed. These disagreements are likely related to the spatial averaging of the forcing data and the mismatch in time and in space between the numerical weather prediction model from which the forcing data are produced and the CERES observed cloud systems.

Luo, Yali↗
DOE OSTI2025

Microphysics regimes due to haze–cloud interactions: cloud oscillation and cloud collapse

Abstract. It is known that aqueous haze particles can be activated into cloud droplets in a supersaturated environment. However, haze–cloud interactions have not been fully explored, partly because haze particles are not represented in most cloud-resolving models. Here, we conduct a series of large-eddy simulations (LESs) of a cloud in a convection chamber using a haze-capable Eulerian-based bin microphysics scheme to explore haze–cloud interactions over a wide range of aerosol injection rates. Results show that the cloud is in a slow microphysics regime at low aerosol injection rates, where the cloud responds slowly to an environmental change and droplet deactivation is negligible. The cloud is in a fast microphysics regime at moderate aerosol injection rates, where the cloud responds quickly to an environmental change and haze–cloud interactions are important. More interestingly, two more microphysics regimes are observed at high aerosol injection rates due to haze–cloud interactions. Cloud oscillation is driven by the oscillation of the mean supersaturation around the critical supersaturation of aerosol due to haze–cloud interactions. Cloud collapse happens under weaker forcing of supersaturation where the chamber transfers cloud droplets to haze particles efficiently, leading to a significant decrease (collapse) in cloud droplet number concentration. One special case of cloud collapse is the haze-only regime. It occurs at extremely high aerosol injection rates, where droplet activation is inhibited, and the sedimentation of haze particles is balanced by the aerosol injection rate. Our results suggest that haze particles and their interactions with cloud droplets should be considered, especially in polluted conditions.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRSDate not supplied

Cloud-Type Mean Cloud Properties and Associated Cloud Radiative Effects in the Tropical “Chimney” Zones Using 20 Years High-Resolution CERES Satellite Data

It has been well known that convection tends to be more intense over land than over ocean and continental convection generally contains wider cores that are protected from entrainment than their oceanic counterparts. How does this difference in convective intensity impact the rest of cloud types and associated cloud radiative effects (CREs)? We select five regions in the tropical “chimney” zones, with two regions over land (Africa and Amazon) and three regions over ocean (eastern and western Pacific, and Atlantic) to understand the differences in the cloud-type mean cloud properties and associated CREs using 20-years high-resolution (2x2 km2) CERES satellite data. The cloud types are based upon the ISCCP classification using the joint cloud-top pressure and cloud optical depth distribution. These five regions are compared to the entire tropics (25°S to 25°N). First, we compare the frequencies of occurrence of cloud types among the regions. Compared to the entire tropics, the “chimney” zones are cloudier, particularly, for cloud types with moderate cloud optical depths in the middle and upper troposphere. Except for the eastern Pacific region, the low-level cloud types are less abundant over land (due to higher boundary layers) and ocean (due to weaker lower-tropospheric subsidence). Over Africa, upper-level clouds are scarcer, due perhaps to weak production of convective anvils related to the drier atmosphere. Second, liquid water path (LWP) and ice water path (IWP) are compared among the regions. Compared to the entire tropics, mean LWPs for moderate cloud optical depths are higher for oceanic regions but lower for Africa while they are slightly lower in the lower troposphere but slightly higher in the middle troposphere for Amazon. Not surprisingly, mean IWPs are higher over land than over ocean, which is directly related to the difference in convective intensity. That is, the explanations to this result are the relatively weak convective intensity over the eastern Pacific and the abundance of anvil clouds over the western Pacific. Both reduce the mean IWPs. The CRE results are still being analyzed because the totally-clear grids (1° x 1°) of the CERES data product should be removed before taking a regional mean of clear-sky fluxes, which cause the wrong signs of CREs for a few cloud types.

cloud radiative effects↗
DOE OSTI2025

Technical note: Recommendations for diagnosing cloud feedbacks and rapid cloud adjustments using cloud radiative kernels

Abstract. The cloud radiative kernel method is a popular approach to quantify cloud feedbacks and rapid cloud adjustments to increased CO2 concentrations and to partition contributions from changes in cloud amount, altitude, and optical depth. However, because this method relies on cloud property histograms derived from passive satellite sensors or produced by passive satellite simulators in models, changes in obscuration of lower-level clouds by upper-level clouds can cause apparent low-cloud feedbacks and adjustments, even in the absence of changes in lower-level cloud properties. Here, we provide a methodology for properly diagnosing the impact of changing obscuration on cloud feedbacks and adjustments and quantify these effects across climate models. Averaged globally and across global climate models, properly accounting for obscuration leads to weaker positive feedbacks from lower-level clouds and stronger positive feedbacks from upper-level clouds while simultaneously removing a mostly artificial anti-correlation between them. Given that the methodology for diagnosing cloud feedbacks and adjustments using cloud radiative kernels has evolved over several papers, and obscuration effects have only occasionally been considered in recent papers, this paper serves to establish recommended best practices and to provide a corresponding code base for community use.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1987

Formation of giant molecular clouds in global spiral structures: The role of orbital dynamics and cloud-cloud collisions

The different roles played by orbital dynamics and dissipative cloud-cloud collisions in the formation of giant molecular clouds (GMCs) in a global spiral structure are investigated. The interstellar medium (ISM) is simulated by a system of particles, representing clouds, which orbit in a spiral-perturbed, galactic gravitational field. The overall magnitude and width of the global cloud density distribution in spiral arms is very similar in the collisional and collisionless simulations. The results suggest that the assumed number density and size distribution of clouds and the details of individual cloud-cloud collisions have relatively little effect on these features. Dissipative cloud-cloud collisions play an important steadying role for the cloud system's global spiral structure. Dissipative cloud-cloud collisions also damp the relative velocity dispersion of clouds in massive associations and thereby aid in the effective assembling of GMC-like complexes.

Roberts, W. W., Jr.↗
DOE OSTI2023

Earth System Model Aerosol–Cloud Diagnostics (ESMAC Diags) package, version 2: assessing aerosols, clouds, and aerosol–cloud interactions via field campaign and long-term observations

Abstract. Poor representations of aerosols, clouds, and aerosol–cloud interactions (ACIs) in Earth system models (ESMs) have long been the largest uncertainties in predicting global climate change. Huge efforts have been made to improve the representation of these processes in ESMs, and the key to these efforts is the evaluation of ESM simulations with observations. Most well-established ESM diagnostics packages focus on the climatological features; however, they lack process-level understanding and representations of aerosols, clouds, and ACIs. In this study, we developed the Earth System Model Aerosol–Cloud Diagnostics (ESMAC Diags) package to facilitate the routine evaluation of aerosols, clouds, and ACIs simulated the Energy Exascale Earth System Model (E3SM) from the US Department of Energy (DOE). This paper documents its version 2 functionality (ESMAC Diags v2), which has substantial updates compared with version 1 (Tang et al., 2022a). The simulated aerosol and cloud properties have been extensively compared with in situ and remote-sensing measurements from aircraft, ship, surface, and satellite platforms in ESMAC Diags v2. It currently includes six field campaigns and two permanent sites covering four geographical regions: the eastern North Atlantic, the central US, the northeastern Pacific, and the Southern Ocean. These regions produce frequent liquid- or mixed-phase clouds, with extensive measurements available from the DOE Atmospheric Radiation Measurement user facility and other agencies. ESMAC Diags v2 generates various types of single-variable and multivariable diagnostics, including percentiles, histograms, joint histograms, and heatmaps, to evaluate the model representation of aerosols, clouds, and ACIs. Select examples highlighting the capabilities of ESMAC Diags are shown using E3SM version 2 (E3SMv2). In general, E3SMv2 can reasonably reproduce many observed aerosol and cloud properties, with biases in some variables such as aerosol particle and cloud droplet sizes and number concentrations. The coupling of aerosol and cloud number concentrations may be too strong in E3SMv2, possibly indicating a bias in processes that control aerosol activation. Furthermore, the liquid water path response to a perturbed cloud droplet number concentration behaves differently in E3SMv2 and observations, which warrants further study to improve the cloud microphysics parameterizations in E3SMv2.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1993

Low cloud investigations for project FIRE: Island studies of cloud properties, surface radiation, and boundary layer dynamics. A simulation of the reflectivity over a stratocumulus cloud deck by the Monte Carlo method

The radiation field over a broken stratocumulus cloud deck is simulated by the Monte Carlo method. We conducted four experiments to investigate the main factor for the observed shortwave reflectively over the FIRE flight 2 leg 5, in which reflectivity decreases almost linearly from the cloud center to cloud edge while the cloud top height and the brightness temperature remain almost constant through out the clouds. From our results, the geometry effect, however, did not contribute significantly to what has been observed. We found that the variation of the volume extinction coefficient as a function of its relative position in the cloud affects the reflectivity efficiently. Additional check of the brightness temperature of each experiment also confirms this conclusion. The cloud microphysical data showed some interesting features. We found that the cloud droplet spectrum is nearly log-normal distributed when the clouds were solid. However, whether the shift of cloud droplet spectrum toward the larger end is not certain. The decrease of number density from cloud center to cloud edges seems to have more significant effects on the optical properties.

Ackerman, Thomas P.↗
NASA NTRS2005

Comparison of Monthly Mean Cloud Fraction and Cloud Optical depth Determined from Surface Cloud Radar, TOVS, AVHRR, and MODIS over Barrow, Alaska

A one year comparison is made of mean monthly values of cloud fraction and cloud optical depth over Barrow, Alaska (71 deg 19.378 min North, 156 deg 36.934 min West) between 35 GHz radar-based retrievals, the TOVS Pathfinder Path-P product, the AVHRR APP-X product, and a MODIS based cloud retrieval product from the CERES-Team. The data sets represent largely disparate spatial and temporal scales, however, in this paper, the focus is to provide a preliminary analysis of how the mean monthly values derived from these different data sets compare, and determine how they can best be used separately, and in combination to provide reliable estimates of long-term trends of changing cloud properties. The radar and satellite data sets described here incorporate Arctic specific modifications that account for cloud detection challenges specific to the Arctic environment. The year 2000 was chosen for this initial comparison because the cloud radar data was particularly continuous and reliable that year, and all of the satellite retrievals of interest were also available for the year 2000. Cloud fraction was chosen as a comparison variable as accurate detection of cloud is the primary product that is necessary for any other cloud property retrievals. Cloud optical depth was additionally selected as it is likely the single cloud property that is most closely correlated to cloud influences on surface radiation budgets.

Uttal, Taneil↗
DOE OSTI2023

Validation of the Cloud_CCI (Cloud Climate Change Initiative) cloud products in the Arctic

The role of clouds in the Arctic radiation budget is not well understood. Ground-based and airborne measurements provide valuable data to test and improve our understanding. However, the ground-based measurements are intrinsically sparse, and the airborne observations are snapshots in time and space. Passive remote sensing measurements from satellite sensors offer high spatial coverage and an evolving time series, having lengths potentially of decades. However, detecting clouds by passive satellite remote sensing sensors is challenging over the Arctic because of the brightness of snow and ice in the ultraviolet and visible spectral regions and because of the small brightness temperature contrast to the surface. Consequently, the quality of the resulting cloud data products needs to be assessed quantitatively. In this study, we validate the cloud data products retrieved from the Advanced Very High Resolution Radiometer (AVHRR) post meridiem (PM) data from the polar-orbiting NOAA-19 satellite and compare them with those derived from the ground-based instruments during the sunlit months. The AVHRR cloud data products by the European Space Agency (ESA) Cloud Climate Change Initiative (Cloud_CCI) project uses the observations in the visible and IR bands to determine cloud properties. The ground-based measurements from four high-latitude sites have been selected for this investigation: Hyytiälä (61.84°N, 24.29°E), North Slope of Alaska (NSA; 71.32°N, 156.61°W), Ny-Ålesund (Ny-Å; 78.92°N, 11.93°E), and Summit (72.59°N, 38.42°W). The liquid water path (LWP) ground-based data are retrieved from microwave radiometers, while the cloud top height (CTH) has been determined from the integrated lidar–radar measurements. The quality of the satellite products, cloud mask and cloud optical depth (COD), has been assessed using data from NSA, whereas LWP and CTH have been investigated over Hyytiälä, NSA, Ny-Å, and Summit.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS2000

Comparison of Cirrus Cloud Models: A Project of the GEWEX Cloud System Study (GCSS) Working Group on Cirrus Cloud Systems

The GEWEX Cloud System Study (GCSS, GEWEX is the Global Energy and Water Cycle Experiment) is a community activity aiming to promote development of improved cloud parameterizations for application in the large-scale general circulation models (GCMs) used for climate research and for numerical weather prediction. The GCSS strategy is founded upon the use of cloud-system models (CSMs). These are "process" models with sufficient spatial and temporal resolution to represent individual cloud elements, but spanning a wide range of space and time scales to enable statistical analysis of simulated cloud systems. GCSS also employs single-column versions of the parametric cloud models (SCMs) used in GCMs. GCSS has working groups on boundary-layer clouds, cirrus clouds, extratropical layer cloud systems, precipitating deep convective cloud systems, and polar clouds.

Starr, David O'C.↗
NASA NTRS2000

Comparison of Cirrus Cloud Models: A Project of the GEWEX Cloud System Study (GCSS) Working Group on Cirrus Cloud Systems

The GEWEX Cloud System Study (GCSS, GEWEX is the Global Energy and Water Cycle Experiment) is a community activity aiming to promote development of improved cloud parameterizations for application in the large-scale general circulation models (GCMs) used for climate research and for numerical weather prediction (Browning et al, 1994). The GCSS strategy is founded upon the use of cloud-system models (CSMs). These are "process" models with sufficient spatial and temporal resolution to represent individual cloud elements, but spanning a wide range of space and time scales to enable statistical analysis of simulated cloud systems. GCSS also employs single-column versions of the parametric cloud models (SCMs) used in GCMs. GCSS has working groups on boundary-layer clouds, cirrus clouds, extratropical layer cloud systems, precipitating deep convective cloud systems, and polar clouds.

Starr, David OC.↗
DOE OSTI2025

Causal Directions Matter: How Environmental Factors Drive Convective Cloud Detrainment Heights

This study investigates how environmental factors influence the level of maximum detrainment (LMD) in deep convective clouds. Through a novel application of the Linear Non‐Gaussian Acyclic Model (LiNGAM), we discover causal structures between environmental variables and LMD, observed at six tropical sites operated by the Atmospheric Radiation Measurement (ARM) user facility. LiNGAM effectively identifies causal directions among variables of interest, revealing robust relationships such as those among the lifting condensation level (LCL), level of free convection (LFC), and convective inhibition (CIN), aligning with prior knowledge. Relative humidity is shown to directly influence LMD; however, this relationship exhibits strong nonlinearity and becomes difficult to detect when the contrast between oceanic and continental environments is excluded from the analysis. This study highlights the importance of establishing causal relationships before performing statistical inference.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1987

A method for remote sensing the emissivity, fractional cloud cover and cloud top temperature of high-level, thin clouds

A methodology for retrieving the emissivity, cloud cover and cloud top temperature of high-level, thin clouds is developed and described. In the thermal infrared windows, the outgoing radiances from the earth's atmosphere contain information about cloud emissivity and cloud top temperature. This information is clearly demonstrated in the brightness temperature difference curves of two window channels. For the purpose of illustration, two window channels centered at 810 and 930 cm are chosen to construct the brightness temperature difference curves for a range of cloud top temperatures. These curves vary for different cloud top temperatures, and along each of these curves the emissivity changes. The brightness temperature difference method is used in a simulation study to demonstrate the feasibility of retrieving the cloud top temperature and emissivity by the utilization of measurements in two window channels. As expected, a perfect retrieval is found if perfect measurements and ideal atmospheric conditions are assumed. If a random error, which has a normal distribution with a mean of zero and standard deviation of + or - 0.5 C, is imposed to the measurements, a reasonable retrieval is found for emissivity greater than 0.3. The algorithm has been applied to a limited amount of HIRS2 data, which has 3.7, 3.98 and 11 micron channels. The cloud top temperature, emissivity and cloud cover are determined by using these channels.

Wu, Man-Li C.↗
NASA NTRS2006

The Influence of Aerosols on the Shortwave Cloud Radiative Forcing from North Pacific Oceanic Clouds: Results from the Cloud Indirect Forcing Experiment (CIFEX)

Aerosols over the Northeastern Pacific Ocean enhance the cloud drop number concentration and reduce the drop size for marine stratocumulus and cumulus clouds. These microphysical effects result in brighter clouds, as evidenced by a combination of aircraft and satellite observations. In-situ measurements from the Cloud Indirect Forcing Experiment (CIFEX) indicate that the mean cloud drop number concentration in low clouds over the polluted marine boundary layer is greater by 53/cu cm compared to clean clouds, and the mean cloud drop effective radius is smaller by 4 microns. We link these in-situ measurements of cloud modification by aerosols, for the first time, with collocated satellite broadband radiative flux observations from the Clouds and the Earth's Radiant Energy System (CERES) to show that these microphysical effects of aerosols enhance the top-of-atmosphere cooling by -9.9+/-4.3 W/sq m for overcast conditions.

Wilcox, Eric M.↗