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At least 19 records

Measurement of absolute E2 transition strengths in {sup 176}W: Signatures for a rapid shape change

The X(5) symmetry describes nuclei at the critical point of the shape phase transition from axially deformed rotor nuclei to spherical vibrators. {sup 150}Nd, {sup 152}Sm, and {sup 154}Gd were the first nuclei where the predicted characteristics of the X(5) symmetry were observed. Later it was shown that also {sup 176,178,180}Os can be successfully described with the X(5) symmetry.In the close vicinity of shape phase transitions one expects strongly changing nuclear shapes. In the X(5) region around A = 150 this was observed for nuclei with different neutron numbers, whereas in the X(5) region around A = 180 this is to be expected for different proton numbers. The aim of the work presented here is the confirmation of a rapid shape change for nuclei close to {sup 178}Os. Besides the knowledge on the level scheme of the nuclei of interest, especially absolute E2 transition strengths are crucial for the interpretation of nuclear structure. Prolate deformation is expected for {sup 176}W. Thus we performed a recoil distance Doppler shift (RDDS) measurement on {sup 176}W to measure E2 transition strengths from level lifetimes. The experiment was performed at the Cologne FN TANDEM accelerator with the Cologne coincidence plunger with the reaction {sup 169}Dy({sup 16}O,4n){sup 176}W and a beam energy of 80 MeV. We will present our experimental results and relate them to data on the neighboring nuclei {sup 178}Os and {sup 182}Pt. The results will be discussed in the framework of nuclear shape transitions in this mass region and compared to calculations with both the Interacting Boson Model (IBM) and the GCM.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Natural Radioactivity of Boron Added Clay Samples

Clay, consisting fine-grained minerals, is an interesting materials and can be used in a variety of different fields especially in dermatology application. Using clay such a field it is important to measure its natural radioactivity. Thus the purpose of this study is to measure {sup 226}Ra, {sup 232}Th and {sup 40}K concentration in clay samples enriched with boron. Three different types of clay samples were prepared where boron is used in different rate. The measurements have been determined using a gamma-ray spectrometry consists of a 3''x3'' NaI(Tl) detector. From the measured activity the radium equivalent activities (Ra{sub eq}), external hazard index (H{sub ex}), absorbed dose rate in air (D) and annual effective dose (AED) have also been obtained.

54 ENVIRONMENTAL SCIENCES↗

Possible excited deformed rotational bands in {sup 82}Ge

Excited states of neutron-rich nucleus {sup 82}Ge were studied from the spontaneous fission of {sup 252}Cf. Eleven new transitions and seven new levels in {sup 82}Ge were identified by using X(Dy)-{gamma}-{gamma} and {gamma}-{gamma}-{gamma} triple coincidences. Possible excited deformed rotational bands are observed, for the first time, in this nuclear region. Coexistence of the spherical ground and deformed excited shapes is proposed in {sup 82}Ge. These deformed rotational bands can be formed by two-particle, two-hole excitations with the 0{sup +} pairing energy states of the {nu}9/2[404]{sup -2} x 1/2[431]{sup 2} configuration across the N=50 closed shell.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Absolute neutrino mass measurements

The neutrino mass plays an important role in particle physics, astrophysics and cosmology. In recent years the detection of neutrino flavour oscillations proved that neutrinos carry mass. However, oscillation experiments are only sensitive to the mass-squared difference of the mass eigenvalues. In contrast to cosmological observations and neutrino-less double beta decay (0v2{beta}) searches, single {beta}-decay experiments provide a direct, model-independent way to determine the absolute neutrino mass by measuring the energy spectrum of decay electrons at the endpoint region with high accuracy.Currently the best kinematic upper limits on the neutrino mass of 2.2eV have been set by two experiments in Mainz and Troitsk, using tritium as beta emitter. The next generation tritium {beta}-experiment KATRIN is currently under construction in Karlsruhe/Germany by an international collaboration. KATRIN intends to improve the sensitivity by one order of magnitude to 0.2eV. The investigation of a second isotope ({sup 137}Rh) is being pursued by the international MARE collaboration using micro-calorimeters to measure the beta spectrum. The technology needed to reach 0.2eV sensitivity is still in the R and D phase. This paper reviews the present status of neutrino-mass measurements with cosmological data, 0v2{beta} decay and single {beta}-decay.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

The Concentrations of {sup 40}K, {sup 226}Ra and {sup 232}Th in Soil Sample in Osmaniye (Turkey)

The {sup 40}K, {sup 226}Ra and {sup 232}Th concentration is due to the magmatic structure of the earth and it can be varied from place to place. Osmaniye is located in the Eastern side of Mediteranean Region. It holds the climatic characteristics of the same region and arises with Middle Taurus Mountains from west to North and with Amonos Mounations in East and West-east parts and is situated between 35 deg. .52'-36 deg. .42' east longitudes and 36 deg. .57'-37 deg. .45' north latitudes. In this study, the natural radioactivity concentrations {sup 40}K, {sup 226}Ra and {sup 232}Th in some soil samples collected in Osmaniye have been investigated. The measurements have been performed using 3x3{sup ''} NaI(Tl) detector system.

54 ENVIRONMENTAL SCIENCES↗

{beta}-decay study of {sup 150}Er, {sup 152}Yb, and {sup 156}Yb: Candidates for a monoenergetic neutrino beam facility

The {beta} decays of {sup 150}Er, {sup 152}Yb, and {sup 156}Yb nuclei are investigated using the total absorption spectroscopy technique. These nuclei can be considered possible candidates for forming the beam of a monoenergetic neutrino beam facility based on the electron capture (EC) decay of radioactive nuclei. Our measurements confirm that for the cases studied the EC decay proceeds mainly to a single state in the daughter nucleus.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Onset of collectivity in Neutron-Rich iron isotopes: Toward a new island of inversion?

The lifetimes of the first excited 2{sup +} states in {sup 62}Fe and {sup 64}Fe have been measured for the first time using the recoil-distance Doppler shift technique, at GANIL. A {sup 238}U beam of 6.5 AMeV impinged on {sup 64}Ni target, and the target like products were slowed down by a degrader foil positioned at micrometer distance downstream of the target and identified in the VAMOS spectrometer on an event-by-event basis. The lifetimes were then determined from the intensities of the degraded and fully Doppler shifted components of the 2{sup +}{yields}0{sup +} transition detected in EXOGAM detectors positioned at backward angles.The resulting lifetimes show a steep increase of the B(E2) values of the first excited 2{sup +} state from {sup 62}Fe to {sup 64}Fe. A comparison with shell model calculations shows that the onset of collectivity is related to the occupation of neutron intruder orbitals. The large B(E2) value for {sup 64}Fe is only reproduced if the valence space includes both the neutron g{sub 9/2} and d{sub 5/2} orbitals. The transition from spherical {sup 68}Ni to more proton-deficient N 40 isotones has some similarity with the island of inversion around {sup 32}Mg. The developing quadrupole collectivity can in both cases be related to the occupation of neutron intruder orbitals which are at the same time quasi-SU(3) partners: (f{sub 7/2}, p{sub 3/2}) for {sup 32}Mg and (g{sub 9/2}, d{sub 5/2}) for the neutron-rich Fe.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Gyromagnetic factors in {sup 144-150}Nd

The U(5) to SU(3) evolution of the nuclear structure in the even {sup 144-156}Nd isotopes has been investigated in the framework of the interacting boson approximation (IBA-2) model, taking into account the effect of the partial Z=64 subshell closure on the structure of the states of a collective nature. The analysis, which led to a satisfactory description of excitation energy patterns, quadrupole moments, and decay properties of the states (even when important M1 components were present in the transitions), is extended to the available data on g factors, in {sup 144-150}Nd. Their values are reasonably reproduced by the calculations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Data Validation Package May 2015, Groundwater Sampling at the Shoal, Nevada, Site

The U.S. Department of Energy Office of Legacy Management conducted annual sampling at the Shoal, Nevada, Site (Shoal) in May 2015. Groundwater samples were collected from wells MV-1, MV-2, MV-3, MV-4, MV-5, H-3, HC-1, HC-2d, HC-3, HC-4, HC-5, HC-6, HC-7, HC-8, and HS-1. Sampling was conducted as specified in the Sampling and Analysis Plan for US. Department of Energy Office of Legacy Management Sites (LMS/PRO/S04351, continually updated, http://energy.gov/lm/downloads/sampling-and-analysis-plan-us-department-energy­ office-legacy-management-sites). Monitoring wells MV-1, MV-2, MV-3, MV-4, MV-5, HC-2d, HC-4, HC-5, HC-7, HC-8, and HS-1 were purged prior to sampling using dedicated submersible pumps. At least one well casing volume was removed, and field parameters (temperature, pH, and specific conductance) were allowed to stabilize before samples were collected. Samples were collected from wells H-3, HC-1, HC-3, and HC-6 using a depth-specific bailer because these wells are not completed with dedicated submersible pumps. Samples were submitted under Requisition Index Number (RIN) 15057042 to ALS Laboratory Group in Fort Collins, Colorado, for the determination of bromide, gross alpha, gross beta, tritium, uranium isotopes, and total uranium (by mass); and under RIN 15057043 to the University of Arizona for the determination of carbon-14 and iodine-129. A duplicate sample from location MV-2 was included with RIN 15057042. The laboratory results from the 2015 sampling event are consistent with those of previous years with the exception of sample results from well HC-4. This well continues to be the only well with tritium concentrations above the laboratory’s minimum detectable concentration which is attributed to the wells proximity to the nuclear detonation. The tritium concentration (731 picocuries per liter [pCi/L]) is consistent with past results and is below the U.S. Environmental Protection Agency's (EPA) maximum contaminant level (MCL) of 20,000 pCi/L. However, concentrations of gross alpha, uranium, and carbon-14 all increased in the sample from well HC-4 during this sampling event. Concentrations of gross alpha and uranium have been above the EPA MCLs in this well since 2012 and the highest concentrations of gross alpha (60.6 pCi/L) and uranium (110 micrograms per liter) were detected during this sampling event. Refer to the time-concentration plots included with this report. Also see the 2015 Groundwater Monitoring Report Project Shoal Area: Subsurface Corrective Action Unit 447 for additional information on the 2015 sampling results.

54 ENVIRONMENTAL SCIENCES↗

Uptake of chloride and carbonate ions by calcium monosulfoaluminate hydrate

Decommissioning of old nuclear reactors may produce waste streams containing chlorides and carbonates, including radioactive {sup 36}Cl{sup -} and {sup 14}CO{sub 3}{sup 2-}. Their insolubilization by calcium monosulfoaluminate hydrate was investigated. Carbonates were readily depleted from the solution, giving at thermodynamic equilibrium monocarboaluminate, monocarboaluminate + calcite, or calcite only, depending on the initial ratio between the anion and calcium monosulfoaluminate hydrate. Chloride ions reacted more slowly and were precipitated as Kuzel's salt, Kuzel's and Friedel's salts, or Friedel's salt only. Rietveld refinement of X-Ray powder diffraction patterns was successfully used to quantify the phase distributions, which were compared to thermodynamic calculations. Moreover, analysing the lattice parameters of Kuzel's salt as a function of its chloride content showed the occurrence of a restricted solid solution towards the sulfate side with general formula 3CaO{center_dot}Al{sub 2}O{sub 3}{center_dot}xCaCl{sub 2}{center_dot}(1 - x)CaSO{sub 4}{center_dot}(12 - 2x){center_dot}H{sub 2}O (0.36 {<=} x {<=} 0.50).

36 MATERIALS SCIENCE↗

Nuclear Data Sheets for A = 27

Evaluated spectroscopic data and level schemes from radioactive decay and nuclear reaction studies are presented for {sup 27}F, {sup 27}Ne, {sup 27}Na, {sup 27}Mg, {sup 27}Al, {sup 27}Si, {sup 27}P, and {sup 27}S. This evaluation for A=27 supersedes the earlier evaluation by P.M. Endt (1998En04 and 1990En08).

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Nuclear Data Sheets for A = 44

The experimental data are evaluated for known nuclides of mass number A=44 (Si,P,S,Cl,Ar,K,Ca,Sc,Ti,V, Cr,Mn). Detailed evaluated level properties and related information are presented, including adopted values of level and {gamma}-ray energies, decay data (energies, intensities and placement of radiations), and other spectroscopic data. This work supersedes earlier full evaluations of A=44 published by 1999Ca45 and 1990En08 (also 1998En04 update). No excited states are known in {sup 44}Si, {sup 44}P, {sup 44}Cr, {sup 44}Mn. Only one excited state is known in 44V and its Isobaric Analog State (IAS) has been observed but with the level energy not known. Information for {sup 44}S, {sup 44}Cl and {sup 44}Ar is limited and their radioactive decay schemes seem incomplete in view of large Q values and known excitations much below than allowed by Q values. The {sup 44}Ca, {sup 44}Sc and {sup 44}Ti nuclides remain as the most extensively studied from many different reactions and decays.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Mapping quadrupole collectivity in the Cd isotopes: The breakdown of harmonic vibrational motion

The stable Cd isotopes have long been used as paradigms for spherical vibrational motion. Extensive investigations with in-beam {gamma} spectroscopy have resulted in very-well-established level schemes, including many lifetimes or lifetime limits. A programme has been initiated to complement these studies with very-high-statistics {beta} decay using the 8{pi} spectrometer at the TRIUMF radioactive beam facility. The decays of {sup 112}In and {sup 112}Ag have been studied with an emphasis on the observation of, or the placement of stringent limits on, low-energy branches between potential multi-phonon levels. A lack of suitable 0{sup +} or 2{sup +} three-phonon candidates has been revealed. Further, the sum of the B(E2) strength from spin 0{sup +} and 2{sup +} states up to 3 MeV in excitation energy to the assigned two-phonon levels falls far short of the harmonic-vibrational expectations. This lack of strength points to the failing of collective models based on vibrational phonon structures.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Cadmium mass measurements between the neutron shell closures at N = 50 and 82

The mass values of the neutron-deficient cadmium isotopes {sup 99-109}Cd and of the neutron-rich isotopes {sup 114,120,122-124,126,128}Cd have been measured using ISOLTRAP. The behavior of the separation energies of the cadmium isotopes from N = 50 to 82 is discussed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Simulations of Bunch Merging in a Beta Beam Decay Ring

To further study neutrino oscillation properties a Beta Beam facility has been proposed. Beta decaying ions with high kinetic energy are stored in a storage ring (''Decay Ring'') with straight sections to create pure focused (anti) electron neutrino beams. However to reach high sensitivity to neutrino oscillation parameters in the experiment the bunched beam intensity and duty cycle in the DR have to be optimized. The first CERN-based scenario, using {sup 6}He and {sup 18}Ne as neutrino sources, has been studied using a bunch merging RF scheme. Two RF cavities at different frequencies are used to capture newly injected bunches and then merge them into the stored bunches. It was shown that this scheme could satisfy the requirements on intensity and duty cycle set by the experiment. This merging scheme has now been revised with new simulation software providing new results for {sup 6}He and {sup 18}Ne. Furthermore bunch merging has been studied for the second CERN-based scenario using {sup 8}Li and {sup 8}B.

43 PARTICLE ACCELERATORS↗

Exploring leptonic CP violation with a Li/B {beta}-beam from CERN to Gran Sasso

We have considered a {beta}-beam setup which tries to leverage at most existing European facilities to boost high-Q ions aiming at a far detector located at L = 732 km in the Gran Sasso Underground Laboratory. The average neutrino energy obtained from {sup 8}Li and {sup 8}B ions boosted at {gamma}-tilde100 is in the range eV - GeV, high enough to use a large iron detector of the MINOS type. We perform, then, a study of the neutrino and antineutrino fluxes needed to observe CP violation and to establish the neutrino mass hierarchy in a significant part of the parameter space.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Counting the number of correlated pairs in a nucleus

We suggest that the number of correlated nucleon pairs in an arbitrary nucleus can be estimated by counting the number of proton-neutron, proton-proton, and neutron-neutron pairs residing in a relative S state. We present numerical calculations of those amounts for the nuclei {sup 4}He, {sup 9}Be, {sup 12}C, {sup 27}Al, {sup 40}Ca, {sup 48}Ca, {sup 56}Fe, {sup 63}Cu, {sup 108}Ag, and {sup 197}Au. The results are used to predict the values of the ratios of the per-nucleon electron-nucleus inelastic scattering cross section to the deuteron in the kinematic regime where correlations dominate.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Charge radii of neon isotopes across the sd neutron shell

We report on the changes in mean square charge radii of unstable neon nuclei relative to the stable {sup 20}Ne, based on the measurement of optical isotope shifts. The studies were carried out using collinear laser spectroscopy on a fast beam of neutral neon atoms. High sensitivity on short-lived isotopes was achieved thanks to nonoptical detection based on optical pumping and state-selective collisional ionization, which was complemented by an accurate determination of the beam kinetic energy. The new results provide information on the structural changes in the sequence of neon isotopes all across the neutron sd shell, ranging from the proton drip line nucleus and halo candidate {sup 17}Ne up to the neutron-rich {sup 28}Ne in the vicinity of the ''island of inversion.'' Within this range the charge radius is smallest for {sup 24}Ne with N=14 corresponding to the closure of the neutron d{sub 5/2} shell, while it increases toward both neutron shell closures, N=8 and N=20. The general trend of the charge radii correlates well with the deformation effects which are known to be large for several neon isotopes. In the neutron-deficient isotopes, structural changes arise from the onset of proton-halo formation for {sup 17}Ne, shell closure in {sup 18}Ne, and clustering effects in {sup 20,21}Ne. On the neutron-rich side the transition to the island of inversion plays an important role, with the radii in the upper part of the sd shell confirming the weakening of the N=20 magic number. The results add new information to the radii systematics of light nuclei where data are scarce because of the small contribution of nuclear-size effects to the isotope shifts which are dominated by the finite-mass effect.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗