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Diagnosing the DARHT Electron Beam-Target Interaction and Hydrodynamic Expansion [Dissertation]

Quantitative electron beam-target interaction studies on the Dual-Axis Radiographic Hydrodynamic Test (DARHT) electron linear induction accelerators have only been performed recently. This includes characterization of the temperature, density, pressure, extent, and expansion velocity of the plasma plume. The results presented in this dissertation present a detailed and unified overview of the accelerator systems, target heating physics, beam transport, and diagnostic tools. Additional information includes calibration sources, radiation hydrodynamics, spectroscopic-quality radiation transport modeling, experimental measurements, and analyses of electron beam driven aluminum experiments. The first set of spatially and temporally resolved spectroscopic measurements of electron beam driven aluminum are presented. Contamination quantification analyses are used to understand the origin of the strong Na-I 3p-3s lines that are observed in absorption within the aluminum plasma continuum. These results inform the creation of the first spectroscopic-quality radiation transport model that links several atomic physics codes to interpret the conditions from which the Na-I lines originate. A good agreement is found between the surface analysis results and the model which confirms the concentration of the sodium present within the aluminum alloy foil material. It also demonstrates, for the first time on electron beam-driven target experiments, the ability to interpret plasma conditions from measured absorption lines. In a second experimental campaign which focuses on pure aluminum, the Al-I 3p-4s and 3p3d doublets are both measured in emission. A detailed analysis of the Al-I 3p-4s doublet reveals that the lines undergo moderate self-absorption. A simple model of the self-absorption effect is successfully used to match measured spectra at various temperature/density/plasma scale length combinations. These measurements led to the realization of the minimum density that can be resolved by the spectrometers for the Al-I 3p-4s lines due to the large slit width required to observe a signal on aluminum. These measurements also demonstrate the sensitivity of visible and long wave UV spectroscopy to minor changes in both temperature and density. The simple self-absorption model will be useful for analysis of other beam-target interaction experiments with spectra exhibiting either self-absorption or full self-reversal. Substantial headway has been made on the modeling front by linking together several codes needed to model both the energy deposition, hydrodynamic motion, and atomic kinetics to produce synthetic spectral calculations that are compared with experimental measurements. There exists ample space for improvement, especially with benchmarking the hydrodynamics codes and equation-of-state tables with experimental measurements. The X-ray diagnostics required to make these new measurements along with the simulation capabilities required to interpret the results are under development and will be the subject of future studies.

43 PARTICLE ACCELERATORS↗

Materials Data on YAl by Materials Project

YAl crystallizes in the orthorhombic Cmcm space group. The structure is three-dimensional. Y is bonded in a 7-coordinate geometry to seven equivalent Al atoms. There are a spread of Y–Al bond distances ranging from 3.09–3.24 Å. Al is bonded in a 9-coordinate geometry to seven equivalent Y and two equivalent Al atoms. Both Al–Al bond lengths are 2.76 Å.

36 MATERIALS SCIENCE↗

Materials Data on YAl by Materials Project

YAl is Tetraauricupride structured and crystallizes in the cubic Pm-3m space group. The structure is three-dimensional. Y is bonded in a body-centered cubic geometry to eight equivalent Al atoms. All Y–Al bond lengths are 3.12 Å. Al is bonded in a body-centered cubic geometry to eight equivalent Y atoms.

36 MATERIALS SCIENCE↗

Materials Data on Y2Al by Materials Project

AlY2 is Cotunnite structured and crystallizes in the orthorhombic Pnma space group. The structure is three-dimensional. there are two inequivalent Y sites. In the first Y site, Y is bonded in a 5-coordinate geometry to five equivalent Al atoms. There are a spread of Y–Al bond distances ranging from 3.07–3.47 Å. In the second Y site, Y is bonded in a 3-coordinate geometry to five equivalent Al atoms. There are a spread of Y–Al bond distances ranging from 3.16–3.57 Å. Al is bonded in a 10-coordinate geometry to ten Y atoms.

36 MATERIALS SCIENCE↗

Materials Data on YAl3 by Materials Project

Al3Y crystallizes in the hexagonal P6_3/mmc space group. The structure is zero-dimensional and consists of two Al3Y clusters. Y is bonded in a trigonal planar geometry to three equivalent Al atoms. All Y–Al bond lengths are 2.95 Å. Al is bonded in a distorted single-bond geometry to one Y atom.

36 MATERIALS SCIENCE↗

Materials Data on Y3Al2 by Materials Project

Y3Al2 crystallizes in the tetragonal P4_2/mnm space group. The structure is three-dimensional. there are three inequivalent Y sites. In the first Y site, Y is bonded in a distorted square co-planar geometry to four equivalent Al atoms. All Y–Al bond lengths are 3.32 Å. In the second Y site, Y is bonded in a 6-coordinate geometry to six equivalent Al atoms. There are four shorter (3.11 Å) and two longer (3.13 Å) Y–Al bond lengths. In the third Y site, Y is bonded in a 6-coordinate geometry to six equivalent Al atoms. There are two shorter (3.07 Å) and four longer (3.23 Å) Y–Al bond lengths. Al is bonded in a 10-coordinate geometry to eight Y and two equivalent Al atoms. There are one shorter (2.77 Å) and one longer (3.02 Å) Al–Al bond lengths.

36 MATERIALS SCIENCE↗

Materials Data on YAl2 by Materials Project

Al2Y is Cubic Laves structured and crystallizes in the cubic Fd-3m space group. The structure is three-dimensional. Y is bonded in a 12-coordinate geometry to four equivalent Y and twelve equivalent Al atoms. All Y–Y bond lengths are 3.41 Å. All Y–Al bond lengths are 3.27 Å. Al is bonded to six equivalent Y and six equivalent Al atoms to form a mixture of edge, face, and corner-sharing AlY6Al6 cuboctahedra. All Al–Al bond lengths are 2.79 Å.

36 MATERIALS SCIENCE↗

Materials Data on YAl3 by Materials Project

Al3Y crystallizes in the trigonal R-3m space group. The structure is three-dimensional. there are two inequivalent Y sites. In the first Y site, Y is bonded to twelve Al atoms to form a mixture of corner and face-sharing YAl12 cuboctahedra. There are a spread of Y–Al bond distances ranging from 3.03–3.11 Å. In the second Y site, Y is bonded to twelve Al atoms to form a mixture of corner and face-sharing YAl12 cuboctahedra. There are six shorter (3.08 Å) and six longer (3.10 Å) Y–Al bond lengths. There are two inequivalent Al sites. In the first Al site, Al is bonded in a 10-coordinate geometry to four Y and six Al atoms. There are a spread of Al–Al bond distances ranging from 2.72–2.89 Å. In the second Al site, Al is bonded in a 12-coordinate geometry to four Y and eight Al atoms. All Al–Al bond lengths are 3.10 Å.

36 MATERIALS SCIENCE↗

Materials Data on Y3Al by Materials Project

Y3Al is Uranium Silicide structured and crystallizes in the cubic Pm-3m space group. The structure is three-dimensional. Y is bonded to eight equivalent Y and four equivalent Al atoms to form YY8Al4 cuboctahedra that share corners with twelve equivalent YY8Al4 cuboctahedra, edges with eight equivalent AlY12 cuboctahedra, edges with sixteen equivalent YY8Al4 cuboctahedra, faces with four equivalent AlY12 cuboctahedra, and faces with fourteen equivalent YY8Al4 cuboctahedra. All Y–Y bond lengths are 3.38 Å. All Y–Al bond lengths are 3.38 Å. Al is bonded to twelve equivalent Y atoms to form AlY12 cuboctahedra that share corners with twelve equivalent AlY12 cuboctahedra, edges with twenty-four equivalent YY8Al4 cuboctahedra, faces with six equivalent AlY12 cuboctahedra, and faces with twelve equivalent YY8Al4 cuboctahedra.

36 MATERIALS SCIENCE↗

Materials Data on AlI3 by Materials Project

AlI3 crystallizes in the monoclinic P2_1/c space group. The structure is zero-dimensional and consists of two ac1mi10q molecules. Al3+ is bonded to four I1- atoms to form edge-sharing AlI4 tetrahedra. There are a spread of Al–I bond distances ranging from 2.49–2.68 Å. There are three inequivalent I1- sites. In the first I1- site, I1- is bonded in a single-bond geometry to one Al3+ atom. In the second I1- site, I1- is bonded in a single-bond geometry to one Al3+ atom. In the third I1- site, I1- is bonded in an L-shaped geometry to two equivalent Al3+ atoms.

36 MATERIALS SCIENCE↗

Materials Data on YAl3 by Materials Project

Al3Y crystallizes in the hexagonal P6_3/mmc space group. The structure is three-dimensional. Y is bonded to twelve equivalent Al atoms to form a mixture of distorted face and corner-sharing YAl12 cuboctahedra. There are six shorter (3.08 Å) and six longer (3.14 Å) Y–Al bond lengths. Al is bonded in a 10-coordinate geometry to four equivalent Y and six equivalent Al atoms. There are two shorter (2.76 Å) and four longer (2.81 Å) Al–Al bond lengths.

36 MATERIALS SCIENCE↗

Materials Data on Y4Al by Materials Project

Y4Al is Iron carbide-like structured and crystallizes in the cubic Fd-3m space group. The structure is zero-dimensional and consists of eight Y4Al clusters. Y is bonded in a single-bond geometry to one Al atom. The Y–Al bond length is 2.77 Å. Al is bonded in a tetrahedral geometry to four equivalent Y atoms.

36 MATERIALS SCIENCE↗