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Ca2AgTl crystallizes in the orthorhombic Immm space group. The structure is one-dimensional and consists of two Ca2AgTl ribbons oriented in the (1, 0, 0) direction. Ca is bonded in a linear geometry to one Ag and one Tl atom. The Ca–Ag bond length is 2.99 Å. The Ca–Tl bond length is 3.25 Å. Ag is bonded in a linear geometry to two equivalent Ca atoms. Tl is bonded in a linear geometry to two equivalent Ca atoms.
CaAg2Tl crystallizes in the orthorhombic Immm space group. The structure is one-dimensional and consists of two CaAg2Tl ribbons oriented in the (1, 0, 0) direction. Ca is bonded in a linear geometry to two equivalent Ag atoms. Both Ca–Ag bond lengths are 2.92 Å. Ag is bonded in a linear geometry to one Ca and one Tl atom. The Ag–Tl bond length is 2.92 Å. Tl is bonded in a linear geometry to two equivalent Ag atoms.