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All sourcesNASA NTRSDOE OSTI
DOE OSTI2018

Study of Reconstructed 39 Ar Beta Decays at the MicroBooNE Detector

In atmospheric argon, 39 Ar beta decays occur at a rate of roughly one Becquerel per kilogram; as a result, large liquid argon time projection chambers (LArTPCs) see plentiful amounts of these decays in each event readout window. These 39 Ar beta decays can provide a variety of different uses in LArTPC experiments. They allow for the study of reconstructing point-like ionization charge deposition in the detector, which is relevant for the reconstruction of supernova neutrino interactions. The point-like topology and well-known energy spectrum of 39 Ar beta decays also provides a unique handle for calibrations. Presented here is the first study of reconstructing 39 Ar beta decays in the MicroBooNE LArTPC. The spectrum of reconstructed electron energies from 39 Ar beta decays, measured using raw TPC waveforms, is found to have a similar end point as the predicted distribution. Additionally, the signal shapes of reconstructed 39 Ar beta decay candidates are used to validate the collection plane wire field response.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2019

Cosmogenic production of 39 Ar and 37 Ar in argon

We have experimentally determined the production rate of 39 Ar and 37 Ar from cosmic ray neutron interactions in argon at sea level. Understanding these production rates is important for argon-based dark matter experiments that plan to utilize argon extracted from deep underground because it is imperative to know what the ingrowth of 39 Ar will be during the production, transport, and storage of the underground argon. These measurements also allow for the prediction of 39 Ar and 37 Ar concentrations in the atmosphere which can be used to determine the presence of other sources of these isotopes. Through controlled irradiation with a neutron beam that mimics the cosmic ray neutron spectrum, followed by direct counting of 39 Ar and 37 Ar decays with sensitive ultralow background proportional counters, we determined that the production rate from cosmic ray neutrons at sea level is expected to be (759 ± 128) atoms / (k Ar day) for 39 Ar, and (51.0 ± 7.4) atoms / (kg Ar day) for 37 Ar . We also performed a survey of the alternate production mechanisms based on the state of knowledge of the associated cross sections to obtain a total sea-level cosmic ray production rate of (1048 ± 133) atoms / (kg Ar day) for 39 Ar, (56.7 ± 7.5) atoms / (kg Ar day) for 37 Ar in underground argon, and (92 ± 13) atoms / (kg Ar day) for 37 Ar in atmospheric argon.

20 ≤ A ≤ 3839 ≤ A ≤ 58↗
DOE OSTI2018

Nuclear Data Sheets for A=39☆

Experimental nuclear structure data from various reactions and decays have been evaluated for all known nuclides of mass 39 (Mg, Al, Si, P, S, Cl, Ar, K, Ca, Sc, Ti). Detailed evaluated nuclear structure information is presented for each reaction and decay and the best values combining all available data are recommended for level energies, half-lives, γ-ray energies and intensities, decay properties (energies, intensities and placement of radiations), and other spectroscopic data. The {sup 39}K, {sup 39}Ca and {sup 39}Ar are the most extensively studied nuclides; no excited states are known in {sup 39}Mg and {sup 39}Ti. This work supersedes the earlier full evaluation of A=39 by B. Singh and J. Cameron (2006Si02).

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2017

Air and radon pathways screenings methodologies for the next revision of the E-area PA

The strategic plan for the next E-Area Low-Level Waste Facility Performance Assessment includes recommended changes to the screening criteria used to reduce the number of radioisotopes that are to be considered in the air and radon pathways incorporated into the GoldSim® atmospheric release model (ARM). For the air pathway, a revised screening methodology was developed based on refinement of previous E-Area PA screening approaches and consideration of the strategic plan recommendations. The revised methodology has three sequential screening steps for each radioisotope: (1) volatility test using the Periodic Table of the Elements, (2) stability test based on half-life, and (3) stability test based on volatility as measured by the Henry’s Law constant for the assumed dominant gaseous species or vapor pressure in the case of tritiated water. Of the 1252 radioisotopes listed in the International Commission on Radiological Protection Publication 107, only the 10 that satisfied all three steps of the revised screening methodology will be included in the ARM. They are: Ar-37, Ar-39, Ar-42, C-14, H-3, Hg-194, Hg-203, Kr-81, Kr-85, and Xe-127. For the radon pathway, a revised screening methodology was developed that also has three sequential steps: (1) identify all decay chains that terminate at Rn-222, (2) screen out parents that decay through U-238 because of its 4.5-billion-year primordial half-life, and (3) eliminate remaining parents whose half-life is shorter than one day. Of the 86 possible decay chains leading to Rn-222, six decay chains consist of 15 unique radioisotopes that will be incorporated into the ARM. The 15 radioisotopes are: U-238, Th-234, Pa-234m, Pu-238, U-234, Th-230, Ra-226, Cf-246, Cm-242, Am-242m, Am-242, Np-238, Np-234, Pa-230, and Rn-222.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
DOE OSTI2015

Liquid xenon purification, de-radonation (and de-kryptonation)

Liquid xenon detectors are at the forefront of rare event physics, including searches for neutrino-less double beta decay and WIMP dark matter. The xenon for these experiments needs to be purified from chemical impurities such as electronegative atoms and molecules, which absorb ionization electrons, and VUV (178 nm) scintillation light-absorbing chemical species. In addition, superb purification from radioactive impurities is required. Particularly challenging are radioactive noble isotopes ({sup 85}Kr,{sup 39,42}Ar,{sup 220,222}Rn). Radon is a particularly universal problem, due to the extended decay sequence of its daughters and its ubiquitous presence in detector materials. Purification and de-radonation of liquid xenon are addressed with particular focus on the experience gained with the EXO-200 neutrino-less double beta decay detector.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2013

Calibration of an ultra-low-background proportional counter for measuring {sup 37}Ar

An ultra-low-background proportional counter design has been developed at Pacific Northwest National Laboratory (PNNL) using clean materials, primarily electro-chemically-purified copper. This detector, along with an ultra-low-background counting system (ULBCS), was developed to complement a new shallow underground laboratory (30 meters water-equivalent) at PNNL. The ULBCS design includes passive neutron and gamma shielding, along with an active cosmic-veto system. This system provides a capability for making ultra-sensitive measurements to support applications like age-dating soil hydrocarbons with {sup 14}C/{sup 3}H, age-dating of groundwater with {sup 39}Ar, and soil-gas assay for {sup 37}Ar to support On-Site Inspection (OSI). On-Site Inspection is a key component of the verification regime for the Comprehensive Nuclear-Test-Ban Treaty (CTBT). Measurements of radionuclides created by an underground nuclear explosion are valuable signatures of a Treaty violation. For OSI, the 35-day half-life of {sup 37}Ar, produced from neutron interactions with calcium in soil, provides both high specific activity and sufficient time for inspection before decay limits sensitivity. This work describes the calibration techniques and analysis methods developed to enable quantitative measurements of {sup 37}Ar samples over a broad range of proportional counter operating pressures. These efforts, along with parallel work in progress on gas chemistry separation, are expected to provide a significant new capability for {sup 37}Ar soil gas background studies.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2016

The DarkSide awakens

Here, the DarkSide program at LNGS aims to perform background-free WIMP searches using two phase liquid argon time projection chambers, with the ultimate goal of covering all parameters down to the so-called neutrino floor. One of the distinct features of the program is the use of underground argon with has a reduced content of the radioactive 39 Ar compared to atmospheric argon. The DarkSide Collaboration is currently operating the DarkSide-50 experiment, the first such WIMP detector using underground argon. Operations with underground argon indicate a suppression of 39 Ar by a factor (1.4 ± 0.2) × 10 3 relative to atmospheric argon. The new results obtained with DarkSide-50 and the plans for the next steps of the DarkSide program, the 20t fiducial mass DarkSide-20k detector and the 200 t fiducial Argo, are reviewed in this proceedings.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2022

Evaluation of cosmogenic production of 39 Ar and 42 Ar for rare-event physics using underground argon

Underground argon (UAr) with lower cosmogenic activities of 39 Ar and 42 Ar has been planned as a detector in detecting scintillation light and charge collection using time projection chambers for dark matter searches and as a veto detector in suppressing backgrounds for neutrinoless double beta decay (0$vββ$ ) experiments. Long-lived radioactive isotopes, 39 Ar and 42 Ar, can also be produced on the surface when UAr is pumped out from a deep well. Understanding the production of long-lived isotopes in Ar is important for utilizing UAr for dark matter and 0$vββ$ experiments in terms of its production, transportation, and storage. Ar exposure to cosmic rays at sea-level is simulated using Geant4 for a given cosmic ray muon, neutron, and proton energy spectrum. Here we report the simulated cosmogenic production rates of 39 Ar, 42 Ar, and other long-lived isotopes at sea-level from fast neutrons, high energy muons, and high energy protons. Total production rates of 938.53/kg Ar day and 5.81 × 10 -3 /kg Ar day for 39 Ar and 42 Ar are found from our simulation. Utilizing these production rates, we set a time limit of 954 days constrained by the production of 39 Ar for UAr to be on the surface before it compromises the sensitivity for a dark matter experiment. Similarly, a time limit of 1702 days constrained by the production of 42 Ar is found for a 0$vββ$ experiment.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2023

Study of cosmogenic activation above ground for the DarkSide-20k experiment

The activation of materials due to exposure to cosmic rays may become an important background source for experiments investigating rare event phenomena. DarkSide-20k, currently under construction at the Laboratori Nazionali del Gran Sasso, is a direct detection experiment for galactic dark matter particles, using a two-phase liquid-argon Time Projection Chamber (TPC) filled with 49.7 tonnes (active mass) of Underground Argon (UAr) depleted in 39 Ar. Despite the outstanding capability of discriminating γ / β background in argon TPCs, this background must be considered because of induced dead time or accidental coincidences mimicking dark-matter signals and it is relevant for low-threshold electron-counting measurements. Here, the cosmogenic activity of relevant long-lived radioisotopes induced in the experiment has been estimated to set requirements and procedures during preparation of the experiment and to check that it is not dominant over primordial radioactivity; particular attention has been paid to the activation of the 120 t of UAr used in DarkSide-20k. Expected exposures above ground and production rates, either measured or calculated, have been considered in detail. From the simulated counting rates in the detector due to cosmogenic isotopes, it is concluded that activation in copper and stainless steel is not problematic. The activity of 39 Ar induced during extraction, purification and transport on surface is evaluated to be 2.8% of the activity measured in UAr by DarkSide-50 experiment, which used the same underground source, and thus considered acceptable. Other isotopes in the UAr such as 37 Ar and 3 H are shown not to be relevant due to short half-life and assumed purification methods.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2017

The DarkSide experiment: Present status and future

Here, DarkSide is a multi-stage program devoted to direct searches of Dark Matter particles with detectors based on double phase liquid Argon Time Projection Chamber. The DarkSide-50 setup is running underground at the Laboratori Nazionali del Gran Sasso. First it was operated with Atmospheric Argon and during that run (1422 ± 67) kg×d of truly background-free exposure has been accumulated. Obtained data made it possible to set a 90% C.L. upper limit on the WIMP-nucleon cross section of 6.1 × 10 –44 cm 2 (for a WIMP mass of 100 GeV/c 2 ). Presently the detector is filled with Underground Argon, which is depleted in 39 Ar by a factor of (1.4 ± 0.2)×10 3 with respect to Atmospheric Argon. Acquired so far (2616 ± 43) kg×d (71 live days) in combination with the data from the Atmospheric Argon run give us the 90% C.L. upper limit on the WIMP-nucleon spin-independent cross section of 2.0×10 –44 cm 2 for a WIMP mass of 100 GeV/c 2 . Up to date this is the best limit obtained with an argon target.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2025

Structurally Driven Selective Adsorption of Hydrocarbons by Metal Substitution in Isostructural Rare-Earth Metal–Organic Frameworks

The design and realization of highly selective nanoporous materials are necessary to target critical separations across industries. By leveraging pore size, pore shape, and linker functionalization, the design of nanoporous solid adsorbents will enable the rapid production of energy efficient separation materials for high-value gas mixtures. This study uses a combination of modeling, synthesis, and gas adsorption testing to investigate a new class of small-pore isostructural rare-earth (RE) 2,5-dihydroxyterephthalic acid (DOBDC) metal–organic frameworks (MOFs) (RE: Pr-, Gd-, Er-, Yb; DOBDC = 2,5-dihydroxyterephthalic acid) and their adsorption selectivity for acetylene/ethylene mixtures. Density functional theory simulations identified that selective binding of acetylene over ethylene in the Gd-, Er-, and Yb-DOBDC MOFs was due to hydrogen-bonding between acetylene and the linker hydroxyl. Adsorption experiments validated the computational results by identifying mechanisms that control the acetylene/ethylene adsorption selectivity and high acetylene adsorption. Furthermore, dynamic column breakthrough experiments with the Gd-DOBDC MOF validated the simulations and indicated that ethylene can be separated from acetylene in a mixture containing 1 vol % acetylene and 39 vol % ethylene (balance argon). In conclusion, the results highlight the complexity of gas binding in functional porous materials and how combining modeling and experiment enables a fundamental understanding of gas–framework interactions that can be leveraged for the design of future separation materials.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2018

Electroluminescence pulse shape and electron diffusion in liquid argon measured in a dual-phase TPC

Here, we report the measurement of the longitudinal diffusion constant in liquid argon with the DarkSide-50 dual-phase time projection chamber. The measurement is performed at drift electric fields of 100 V/cm, 150 V/cm, and 200 V/cm using high statistics $^{39}$Ar decays from atmospheric argon. We derive an expression to describe the pulse shape of the electroluminescence signal (S2) in dual-phase TPCs. The derived S2 pulse shape is fit to events from the uppermost portion of the TPC in order to characterize the radial dependence of the signal. The results are provided as inputs to the measurement of the longitudinal diffusion constant DL, which we find to be (4.12 $\pm$ 0.04) cm$^2$/s for a selection of 140keV electron recoil events in 200V/cm drift field and 2.8kV/cm extraction field. To study the systematics of our measurement we examine datasets of varying event energy, field strength, and detector volume yielding a weighted average value for the diffusion constant of (4.09 $\pm$ 0.09) cm$^2$ /s. The measured longitudinal diffusion constant is observed to have an energy dependence, and within the studied energy range the result is systematically lower than other results in the literature.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2017

Simulation of argon response and light detection in the DarkSide-50 dual phase TPC

A Geant4-based Monte Carlo package named G4DS has been developed to simulate the response of DarkSide-50, an experiment operating since 2013 at LNGS, designed to detect WIMP interactions in liquid argon. In the process of WIMP searches, DarkSide-50 has achieved two fundamental milestones: the rejection of electron recoil background with a power of ~10 7 , using the pulse shape discrimination technique, and the measurement of the residual 39 Ar contamination in underground argon, ~3 orders of magnitude lower with respect to atmospheric argon. These results rely on the accurate simulation of the detector response to the liquid argon scintillation, its ionization, and electron-ion recombination processes. This work provides a complete overview of the DarkSide Monte Carlo and of its performance, with a particular focus on PARIS, the custom-made liquid argon response model.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗