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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 19 records
All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

Demonstrating the β-Ga 2 O 3 Schottky diodes for alpha radiation detection

Schottky barrier diodes were fabricated on (001) monoclinic β-Ga 2 O 3 wafers with low doped epitaxial layers of 7.0 × 10 15 cm −3 . Circular Ni Schottky contacts with area 2 mm 2 were deposited by electron beam evaporation. Devices were characterized electrically by performing forward and reverse current-voltage sweeps with a range of −100 V–2 V, as well as capacitance-voltage sweeps to −30 V. The breakdown voltage was also determined to be −180 V for the devices. Experiments measuring the electrical response from incident X-ray radiation was performed. A response time to X-ray radiation of less than 1 s was recorded and a decay time of approximately 2 s after removing X-ray source, which primarily attribute to X-ray switching on and off time. Energy spectra of alpha particles from a 0.9 μCi 241 Am button source was collected at various voltage biases using devices with the lowest measured leakage current while reverse biased. The total count rate was observed to increase linearly with increasing device bias. In conclusion, the peak channel number was observed to increase with increasing bias with the best resolution of 9.5% at −100 V reverse bias.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2025

Scintillation light detection in polycrystalline diamond using single photon detectors

Here, this study investigates the scintillation properties of polycrystalline diamond for particle detection applications, particularly in neutron and alpha radiation environments. Polycrystalline diamonds provide a cost-effective alternative to monocrystalline diamonds while retaining essential detection properties. Photoluminescence measurements were performed to analyze emission spectra, revealing distinct characteristics based on impurity content and crystallinity. Scintillation responses were assessed using Silicon Photomultipliers (SiPMs), demonstrating the capability of polycrystalline diamond powders to respond to alpha irradiation, albeit with reduced resolution compared to traditional scintillators. A prototype neutron detector was developed by combining diamond powder with neutron-sensitive 6 LiF, and its performance was evaluated through experimental testing and Geant4 simulations. The findings indicate that polycrystalline diamond-based detectors can achieve significant detection efficiency while remaining insensitive to gamma radiation, offering potential for portable neutron detection applications.

47 OTHER INSTRUMENTATION↗
DOE OSTI2025

Hints of primordial magnetic fields at recombination and implications for the Hubble tension

Primordial Magnetic Fields (PMFs), long studied as relics of the early Universe, accelerate recombination and have been proposed as a way to relieve the Hubble tension. However, previous studies relied on simplified toy models. Here, in this study, we use recent evaluations of recombination with PMFs, incorporating full magnetohydrodynamic (MHD) simulations and detailed Lyman-alpha radiative transfer, to test PMF-enhanced recombination (bΛCDM) against observational data from the cosmic microwave background (CMB), baryon acoustic oscillations (BAO), and Type Ia supernovae (SN). Focusing on non-helical PMFs with a Batchelor spectrum, we find a preference for presentday total field strengths of approximately 5-10 pico-Gauss. Depending on the dataset combination, this preference ranges from mild (∼ 1.8σ with Planck + DESI) to moderate (∼ 3σ with Planck + DESI + SH0ES-calibrated SN) significance. The bΛCDM has Planck + DESI χ 2 values equal to or better than ΛCDM while predicting a higher Hubble constant. Future high-resolution CMB temperature and polarization measurements will be crucial for confirming or further constraining PMFs at recombination. Field strengths of 5-10 pico-Gauss align closely with those required for cluster magnetic fields to originate entirely from primordial sources, without the need for additional dynamo amplification.

Jedamzik, Karsten [Centre National de la Recherche↗
DOE OSTI2026

Radiative corrections to superallowed beta decays at $\mathcal{O}\left({\alpha}^2Z\right)$

We compute $\mathcal{O}\left({\alpha}^2Z\right)$ radiative corrections to superallowed β decays with a heavy-particle effective field theory that systematically describes the interactions of low-energy ultrasoft photons with nuclei. We calculate two-loop virtual and one-loop real-virtual amplitudes by reducing the Feynman integrals to a set of master integrals, which we solve analytically using a variety of techniques. These techniques can be applied to other phenomenologically interesting observables. The ultrasoft corrections can then be combined with contributions arising from the exchange of potential photons to obtain the complete $\mathcal{O}\left({\alpha}^2Z\right)$ correction to the decay rate, with resummation of large logarithms of the electron energy times the nuclear radius. We find that $\mathcal{O}\left({\alpha}^2Z\right)$ ultrasoft loops induce a relative correction to the decay rate that ranges from 0.7 ∙ 10 −3 in the decay of 10 C to 3.6 ∙ 10 −3 in the decay of 54 Co, and will thus impact the extraction of V ud at the permille level. We show that the inclusion of these corrections reduces the residual renormalization scale dependence of the decay rate to a negligible level, making missing ultrasoft perturbative corrections a subdominant source of theoretical uncertainty.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2026

Effects of He-Ion Radiation on Solid-State Uranyl Nitrate Compounds under Dry and Hydrated Atmospheric Conditions

Radioactive decay of uranium (U) and its related daughter/fission products emit ionizing radiation, including γ (γ) rays and α (α) particles, that result in the formation of radical species and induce chemical reactivity in materials. While radioactivity is inherent to the chemistry of U there are limited studies that detail changes at an atomistic level. Here, this work describes the He-ion radiolysis of four solid-state U(VI) species: [UO 2 (NO 3 ) 2 ]·3(H 2 O) and M[UO 2 (NO 3 ) 3 ] (M = K + , Rb + , Cs + ). These materials were irradiated under different conditions (i.e. closed, open – Ar gas, or open – H 2 O-saturated Ar gas) to further evaluate the impact of water radiolysis on the chemical modification of these materials. Pre- and post-irradiation analyses were conducted using EPR, Raman, and ATR-IR spectroscopy on materials irradiated to 0, 5, 10, and 25 MGy. The results indicated the presence of nitrate radical (NO 3 • ) formation in all solid-state materials with similarities to those observed in γ-radiation studies. Irradiation of [UO 2 (NO 3 ) 2 ]·3(H 2 O) did not show evidence of reactive oxygen species bound to the U(VI) cation under inert conditions; however, surface reactivity was observed for samples irradiated in the H 2 O-saturated environment. Similar chemical changes were observed in the uranyl trinitrato compounds irradiated in the presence of H 2 O vapor and there were observed differences in the reactivity depending on the identity of the alkali cation.

38 - RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCL↗
DOE OSTI2024

Understanding Radiotropism in Filamentous Fungi

Melanized species of filamentous fungi isolated from high radiation environments have been reported to exhibit radiotropism, defined as the directed growth toward a source of ionizing radiation. Inconsistencies in the experimental approaches and results have impeded our understanding of the key factors involved in radiotropism. In the present study, we assessed radiotropism in four isolates of fungi: Aspergillus niger, A. calidoustus JC-1043, Paecilomyces variotii SNL-1, and P. variotii IMV-00236. Of these fungi, only P. variotii IMV-00236 had been previously reported to exhibit radiotropic behavior. Plates of each fungus were placed in equivalent proximity to a 137 Cs source, with a primary gamma emission of 662 keV, and differences in the rate and direction of mycelia growth were measured over a seven-day period. Significant differences were not observed in the rate or direction of growth of the different fungi based on exposure to gamma radiation, which suggested a lack of measurable radiotropism in these experiments. Additional studies varying parameters such gamma emission rates and energies, as well as other types of ionizing radiation (e.g., alpha and beta particles, neutrons) are necessary to gain further insights to the factors critical to the expression of radiotropic behavior in filamentous fungi.

59 BASIC BIOLOGICAL SCIENCES↗
DOE OSTI2025

Real-time gross actinide monitoring in extreme (10 6 :1) beta-gamma background fluid streams using mini-ATMFDs

Real-time, trace alpha activity monitoring in extreme mixed radiation fields is a well-known challenge in fission product-rich streams containing mixtures of beta-gamma-alpha radiation-emitting isotopes, arising due to the extreme 10 6 :1 ratio of background beta-gamma vs. alpha radiation activity levels. This paper presents results from a novel approach to addressing this challenge, based on Tensioned Metastable Fluid Detector (TMFD) sensing technology. An acoustically driven technique was developed and tested at Purdue University (using dissolved Rn-Po and U-chain alpha emitters), and validated (with dissolved Pu) at Savannah River National Laboratory for real-time monitoring of alpha activity in the 100–10,000 dpm/mL range.

Environmental Monitoring↗
DOE OSTI2025

Prediction of Alpha-Particle-Immune Gate-All-Around Field-Effect Transistors (GAA-FET) Based SRAM Design

Alpha particles are known to be a major source of particles creating soft errors in semiconductor devices, such as content flipping in Static Random-Access Memory (SRAM). Recent advancements in transistor nodes have led to the introduction of Gate-All-Around Field Effect Transistors (GAA-FETs), which have better gate control, thus better electrostatics. Moreover, the introduction of bottom dielectric isolation (BDI) eliminates substrate leakage and thus is expected to enhance its radiation hardness. It is thus important to explore if one can design an SRAM that is completely radiation-hard to alpha particles. In this paper, using 3D Technology Computer-Aided-Design (TCAD) simulations, we show that it is possible to design an SRAM using GAA-FET technology so that it is immune to single alpha particle radiation error. In other words, with the design, there will be no single-event upset (SEU) due to alpha particles. We first use ab initio calculations in PHITS to show that there is a maximum linear energy transfer (LET), LET max , for the alpha particle in Si and Si x Ge 1-x . Based on that, by de signing a sub-7nm GAA-FET-based SRAM with BDI, we show that the SRAM does not flip even if the particle strike is in the worst-case scenario for LET > LET max .

42 ENGINEERING↗
DOE OSTI2025

Charge collection efficiency of diamond and silicon sensors irradiated with alpha particles

To evaluate the viability of using semiconductors as sensor materials in a detector for the Associated Particle Imaging technique, the radiation hardness of silicon and diamond diodes to alpha particles has been assessed. Here, the detector lifetimes for both silicon and diamond sensors were measured under the prolonged exposure to alpha particles emitted by an 241 Am source. The silicon detector was exposed to alpha radiation for approximately two months, reaching an accumulated fluence of ~ 1.5 x 10 12 α cm –2 . Additionally, by using a high purity single-crystal diamond with coplanar electrodes operating with full charge collection, the diamond detector response was measured over approximately ten months reaching an accumulated fluence of over 6 x 10 12 α cm –2 cm.

47 OTHER INSTRUMENTATION↗
DOE OSTI2024

Informing solar blind radioluminescence imaging through a calibrated spectrum

While direct radiation detection methods offer great insight into the origin of ionizing particles and photons, their use to locate contaminated areas or concealed radioactive sources can lead to undue exposure of personnel and equipment to ionizing radiation or the potential for contamination. These same sources induce ultraviolet (UV) optical photon fluorescence in air – a process referred to as radioluminescence – that may be imaged from low dose regions over larger attenuation lengths than ionizing radiation. However, most optical detection methods are limited to low lighting conditions to image the more abundant ultraviolet-A (UV-A) photons. To extend this capability to room light or daytime conditions, the solar blind region (Ultraviolet-C (UV-C), <280 nm) can be tapped. Though the emission yield of UV-C photons is roughly two orders of magnitude lower than that in the UV-A regime, the UV-C offers dramatic improvements in signal-to-noise ratios under bright lighting conditions due to decreased background interferences. The yield of specific UV-C lines, if present in the literature at all, varies widely, which has a large impact in modeling and analyzing standoff UV-C measurement scenarios. Thus, we have captured improved radioluminescence spectra over 250–400 nm and identified observed emission peaks in ambient air. Many of the UV-C photons produced by ionizing radiation excitation result from high-energy, molecular nitrogen Gaydon-Herman transitions which have had limited study to date for this application. Relating these findings to published UV-A yields, we estimate emissions between 0.15–0.19 photons/MeV over 250–280 nm. Additionally, we also use a commercial corona-discharge imaging camera to demonstrate outdoor UV-C radiation mapping of alpha and gamma emitters from 50 and 75 m standoffs, respectively. The imaged “counts” are compared to optically modelled values and show the same trend over distance.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2026

Online Alpha Monitoring of High Cs-137 Hanford and SRS High Level Waste with Tensioned Metastable Fluid Detectors

The Department of Energy’s Hanford and Savannah River Sites maintain millions of gallons of caustic supernate and salt high activity waste in their high-level waste (HLW) tank farm inventories. The Savannah River Site is currently treating this waste with a calixarene-based solvent extraction of Cs-137 to reduce these inventories. Hanford is employing an at-tank crystalline silico titanate (CST) based solid phase extraction methodology to reduce their liquid HLW inventories. Due to the high solubility of Cs-137 and the relative insolubility of the actinides in these caustic waste forms, the beta to alpha radioactivity ratio can often exceed six orders of magnitude in the feed solutions to these treatment processes. This unique characteristic leads to significant technical challenges in making rapid gross alpha measurements in the presence of the overwhelming beta, gamma, as well as dissolved sodium salt in these HLW matrices. Conventional radioanalytical techniques, such as liquid scintillation analysis or gas flow proportional counting require significant radiochemistry preparation prior to the radiometric measurements for gross alpha activity. These required pretreatments render these technologies untenable for rapid quantification of gross alpha activity that could be required to support on or at-line measurements ensuring a waste stream will meet regulatory requirements. The radiation measurement properties of Tensioned Metastable Fluid Detectors (TMFDs) have been studied by Purdue University’s Taleyarkhan research group for well over a decade. Fluids tensioned to the appropriate degree will rupture when struck by radiation, resulting in a measurable cavitation event. The negative pressure generating this tension can be adjusted by centrifugal rotation or by acoustic means in such a way that these cavitation events can be generated from alpha radiation but will not be generated by beta or gamma radiation. Purdue University and the Savannah River National Laboratory are currently collaborating to develop a gamma/beta blind, spectroscopic alpha measurement system based on the Tensioned Metastable Fluid Detector technology to provide a potential solution for performing rapid gross alpha measurements on these high gamma/beta sample matrices. Measurements using the Indirect Drive Acoustically Tensioned Metastable Fluid Detectors developed as part of this collaboration were performed with an alpha emitting radionuclide. Successful determination of gross alpha activity was observed, indicating a potential pathway for rapid gross alpha measurements in remote-handled shielded cells or in process situations requiring online alpha monitoring. Measurements using this system have been conducted on high beta activity solutions, demonstrating the beta blind capability of this system. Measurements are currently underway to test the system’s capability to measure gross alpha activity on Savannah River Site high level waste high Cs-137 samples that have been measured by the SRNL radiochemistry team. This work was supported by the DOE EM Technology Development program.

DiPrete, David [Savannah River National Laboratory↗
DOE OSTI2026

Investigation of the 244 Pu ⁢( 48 Ca,𝑥⁢𝑛) 292−𝑥 Fl reaction with the LBNL SHREC detector: Investigation of decay chains of isotopes of flerovium (𝑍=114)

The 244 Pu ⁢( 48 Ca,𝑥⁢𝑛)⁢ 292−𝑥 Fl reaction was investigated at Lawrence Berkeley National Laboratory’s 88 Inch Cyclotron using the Berkeley Gas-filled Separator (BGS), the newly installed Superheavy Recoil detector, along with an upgraded digital electronics and data acquisition system. Seven decay chains were observed starting with an evaporation residue, followed by a single 𝛼 decay and a spontaneous fission. The decay characteristics of these seven decay chains led to an assignment to 288 Fl , the product of the 4⁢𝑛 reaction channel. Two additional chains were (tentatively) assigned to the decay of the 3⁢𝑛 exit channel, 289 Fl . Cross sections for the 4⁢𝑛 and 3⁢𝑛 exit channels were 𝜎 prod =6.7⁢($^{36}_{25}$) pb and 𝜎 prod =1.6⁢($^{22}_{11}$) pb, respectively. Another decay chain, tentatively assigned to the 5⁢𝑛 exit channel through the 48 Ca + 244 Pu reaction or the 3⁢𝑛 exit channel of the 48 Ca + 242 Pu reaction, was also detected. Detailed information regarding the observed decay chains and their nuclear structure aspects is discussed, along with the performance of the BGS and the new detection system.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2026

Non-Equilibrium Actinide Radiation Chemistry and the Nuclear Fuel Cycle

Actinides are inherently unstable elements that frequently coexist with other radioisotopes, generating intense ionizing radiation fields that drive the formation of non equilibrium oxidation states. These transient species exert a profound mechanistic influence on the radiation response of actinide containing systems due to their unique redox chemistry. Despite their importance, they remain poorly understood, yet such insight is essential for advancing actinide science and accurately predicting radiation driven behavior. Actinide separations—critical for nuclear energy technologies, strategic deterrence, space exploration, and nuclear medicine—depend on precise control of actinide oxidation states to recover targeted elements from complex matrices such as used nuclear fuel. However, during these processes, actinides, their coordination complexes, and the separation media are all exposed to intense, multicomponent (alpha, beta, gamma, etc.) radiation fields that can alter process efficiency, selectivity, and chemical stability. Understanding, controlling, and mitigating radiation induced reactions is therefore key to innovating and optimizing next generation separation technologies. This seminar will provide an overview of the nuclear fuel cycle and non equilibrium actinide radiation chemistry in the context of recovering actinides from used nuclear fuel, with a particular emphasis on direct dissolution–based reprocessing strategies. We will explore time resolved electron pulse radiolysis and alpha and gamma dose accumulation studies, integrated with multiscale computational modeling, to elucidate the molecular level roles of radiation driven, non equilibrium actinide species in process performance and in the radiolytic stability of organic ligands used for actinide recovery. These insights offer new pathways for designing advanced separation methods and next generation solvent systems, with broad implications for the future of the nuclear fuel cycle.

37 - INORGANIC, ORGANIC, PHYSICAL AND ANALYTICAL C↗
DOE OSTI2024

Low-alpha Operation of the Iota Storage Ring

Operation with ultra-low momentum-compaction factor (alpha) is a desirable capability for many storage rings and synchrotron radiation sources. For example, low-alpha lattices are commonly used to produce picosecond bunches for the generation of coherent THz radiation and are the basis of a number of conceptual designs for EUV generation via steady-state microbunching (SSMB). Achieving ultra-low alpha requires not only a high-level of stability in the linear optics but also flexible control of higher-order compaction terms. Operation with lower momentum-compaction lattices has recently been investigated at the IOTA storage ring at Fermilab. A procedure for lowering the ring compaction using the linear optics along with compensations from the higher-order magnets was developed with the aid of a model, and an experimental technique for measuring the momentum compaction was developed. The lowest momentum compaction achieved during the available run-time was $3.4\times10^{-4}$, around 15 times lower than previously operated. These feasibility studies ensure an improved experimental understanding of the IOTA optics and potentially will enable new research programs at the facility.

43 PARTICLE ACCELERATORS↗
DOE OSTI2026

Non-Equilibrium Actinide Radiation Chemistry and the Nuclear Fuel Cycle

Invited John and Naomi Fackler Lectureship in Chemistry and English seminar at Valparaiso University, IN, USA. Actinides are inherently unstable elements that frequently coexist with other radioisotopes, generating intense ionizing radiation fields that drive the formation of non-equilibrium oxidation states. These transient species exert a profound mechanistic influence on the radiation response of actinide-containing systems due to their unique redox chemistry. Despite their importance, they remain poorly understood, yet such insight is essential for advancing actinide science and accurately predicting radiation-driven behavior. Actinide separations—critical for nuclear energy technologies, strategic deterrence, space exploration, and nuclear medicine—depend on precise control of actinide oxidation states to recover targeted elements from complex matrices such as used nuclear fuel. However, during these processes, actinides, their coordination complexes, and the separation media are all exposed to intense, multicomponent (alpha, beta, gamma, etc.) radiation fields that can alter process efficiency, selectivity, and chemical stability. Understanding, controlling, and mitigating radiation-induced reactions is therefore key to innovating and optimizing next-generation separation technologies. This seminar will provide an overview of the nuclear fuel cycle and non-equilibrium actinide radiation chemistry in the context of recovering actinides from used nuclear fuel, with a particular emphasis on direct-dissolution–based reprocessing strategies. We will explore time-resolved electron pulse radiolysis and gamma dose accumulation studies to elucidate the molecular-level roles of radiation-driven, non-equilibrium actinide species in process performance and in the radiolytic stability of organic ligands used for actinide recovery. These insights offer new pathways for designing advanced separation methods and next-generation solvent systems, with broad implications for the future of the nuclear fuel cycle.

37 - INORGANIC, ORGANIC, PHYSICAL AND ANALYTICAL C↗
DOE OSTI2024

First look at neutron emission shape characteristics of ignition hotspots at the National Ignition Facility (invited)

The nuclear imaging system has been capturing neutron images of inertial confinement fusion (ICF) driven implosions for over a decade at the National Ignition Facility. This imaging system has evolved from one to three nearly orthogonal lines-of-sight, allowing for the study of three-dimensional shape characteristics of ignition shots. Limited-view tomography algorithms help visualize the burning hotspot in 3D and assess neutron source geometry using Legendre mode parameters. With its neutron, gamma-ray, and x-ray image reconstruction capabilities, NIS has provided critical insight into mechanisms that have limited implosion performance, such as fill tube diameter for ignition-type targets. This comprehensive diagnostic suite opens a window into the shape characteristics of ignition shots and how symmetry affects ICF implosion performance. In more recent ignition shots, neutron yields have visibly increased. Analyzing the shape and size of the reconstructed neutron source has shown an expansion of the burn volume, which is indicative of more efficient alpha heating during the implosion process.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2024

Diagnosing up-scattered deuterium–tritium fusion neutrons produced in burning plasmas at the National Ignition Facility (invited)

In the push to higher performance fusion plasmas, two critical quantities to diagnose are α-heat deposition that can improve and impurities mixed into the plasma that can limit performance. In high-density, highly collisional inertial confinement fusion burning plasmas, there is a significant probability that deuterium–tritium (DT) fusion products, 14.1 MeV neutrons and 3.5 MeV α-particles, will collide with and deposit energy onto (“up-scatter”) surrounding deuterium and tritium fuel ions. These up-scattered D and T ions can then undergo fusion while in-flight and produce an up-scattered neutron (15–30 MeV). These reaction-in-flight (RIF) neutrons can then be uniquely identified in the measured neutron energy spectrum. Further, the magnitude, shape, and relative size of this spectral feature can inform models of stopping-power in the DT plasma and hence is directly proportional to α-heat deposition. In addition, the RIF spectrum can be related to mix into the burning fuel, particularly relevant for high-Z shell and other emerging National Ignition Facility platforms. The neutron time-of-flight diagnostic upgrades needed to obtain this small signal, ~10 –5 times the primary DT neutron peak, will be discussed. Results from several gain > 1 implosions will be shown and compared to previous RIF spectra. Finally, comparisons of experimental data to a simplified computational model will be made.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗