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At least 19 records

Advances and challenges in cryo ptychography at the Advanced Photon Source

Ptychography has emerged as a nondestructive tool to quantitatively study extended samples at a high spatial resolution. In this manuscript, we report on recent developments from our team. We have combined cryo ptychography and fluorescence microscopy to provide simultaneous views of ultrastructure and elemental composition, we have developed multi-GPU parallel computation to speed up ptychographic reconstructions, and we have implemented fly-scan ptychography to allow for faster data acquisition. We conclude with a discussion of future challenges in high-resolution 3D ptychography.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Progress on an energy recovery linac upgrade to the Advanced Photon Source

The Advanced Photon Source (APS) is a third-generation storage-ring-based x-ray source that has been operating for more than 13 years and is enjoying a long period of stable, reliable operation. However, major accelerator upgrades are being investigated in order to maintain scientific relevance into the future. One very promising possibility is the use of an energy recovery linac (ERL). In this option, APS would transition from a source based on a stored electron beam to one based on a continuously generated high-brightness electron beam from a linac. Such a source promises dramatically improved brightness and transverse coherence compared to third-generation storage rings. We present a new design for an ERL upgrade that incorporates very long insertion devices. We show that operation at high electron beam energy provides the promise of extremely high brightness for hard x-rays. We also show results of the first start-to-end simulations of an ERL-based x-ray source.

43 PARTICLE ACCELERATORS↗

Multi-objective direct optimization of dynamic acceptance and lifetime for potential upgrades of the Advanced Photon Source.

The Advanced Photon Source (APS) is a 7 GeV storage ring light source that has been in operation for well over a decade. In the near future, the ring may be upgraded, including changes to the lattice such as provision of several long straight sections (LSS). Because APS beamlines are nearly fully built out, we have limited freedom to place LSSs in a symmetric fashion. Arbitrarily-placed LSSs will drastically reduce the symmetry of the optics and would typically be considered unworkable. We apply a recently-developed multi-objective direct optimization technique that relies on particle tracking to compute the dynamic aperture and Touschek lifetime. We show that this technique is able to tune sextupole strengths and select the working point in such a way as to recover the dynamic and momentum acceptances. We also show the results of experimental tests of lattices developed using these techniques.

43 PARTICLE ACCELERATORS↗

Status of the Short-Pulse X-ray Project at the Advanced Photon Source

The Advanced Photon Source Upgrade (APS-U) Project at Argonne will include generation of short-pulse x-rays based on Zholents deflecting cavity scheme. We have chosen superconducting (SC) cavities in order to have a continuous train of crabbed bunches and flexibility of operating modes. In collaboration with Jefferson Laboratory, we are prototyping and testing a number of single-cell deflecting cavities and associated auxiliary systems with promising initial results. In collaboration with Lawrence Berkeley National Laboratory, we are working to develop state-of-the-art timing, synchronization, and differential rf phase stability systems that are required for SPX. Collaboration with Advanced Computations Department at Stanford Linear Accelerator Center is looking into simulations of complex, multi-cavity geometries with lower- and higher-order modes waveguide dampers using ACE3P. This contribution provides the current R&D status of the SPX project.

43 PARTICLE ACCELERATORS↗

Measurements of source emittance and beam coherence properties of the upgraded Advanced Photon Source

The Advanced Photon Source (APS) has been upgraded with a multi-bend achromat lattice, achieving significantly reduced electron beam emittance and enhanced X-ray coherence. Precise characterization of these properties is essential for optimizing beamline performance and enabling new experiments that take full advantage of the upgraded source. We report on measurements of source size and transverse coherence properties using grating interferometry at two beamlines: the APS 3-ID-B undulator beamline and the 1-BM-B bending magnet beamline. The results confirm the world-record horizontal emittance of the upgraded APS below 30 pm rad and validate the theoretical design parameters. We further investigate the impact of optical aberrations and mechanical vibrations at the 12-ID-C beamline on coherence preservation. These measurements establish a benchmark for future beamline enhancements and demonstrate the effectiveness of grating interferometry for high-precision beam characterization. Our findings provide critical insights into synchrotron beam dynamics, coherence degradation mechanisms, and strategies for optimizing beamline X-ray optics at next-generation light sources.

Advanced Photon Source↗

MAGNET DESIGNS FOR THE MULTI-BEND ACHROMAT LATTICE AT THE ADVANCED PHOTON SOURCE

The Advanced Photon Source (APS) is currently investigating replacing the existing two-bend 7 GeV lattice with a 6 GeV seven-bend achromat magnet lattice in order to achieve a low electron beam emittance [1]. This new lattice requires 1320 magnets, of which there are nine types. These include high strength quadrupoles (gradient up to ~97 T/m), sextupoles with second derivative of field up to ~7000 T/m2, longitudinal gradient dipoles with field ratio of up to 5, and transverse gradient dipoles with gradients of ~50 T/m and central field of ~0.6 T. These field requirements and the limited space available pose several design challenges. This paper presents a summary of magnet designs for the various magnet types developed through a collaboration of APS with FNAL and BNL.

Jaski, M.↗

Dynamic Exploding Foil Initiator Imaging at the Advanced Photon Source

Recent advances in diagnostics coupled with synchrotron sources have allowed the in-situ investigation of exploding foil initiators (EFI) during flight. Herein, we present the first images of EFIs during flight utilizing x-ray phase contrast imaging at the Advanced Photon Source (APS) located in Argonne National Laboratory. These images have provided the DOE/DoD community with unprecedented images resolving details on the micron scale of the flyer formation, plasma instabilities and in-flight characteristics along with the subsequent interaction with high explosives on the nanosecond time scale. Phase contrast imaging has allowed the ability to make dynamic measurements on the length and time scale necessary to resolve initiator function and provide insight to key design parameters. These efforts have also probed the fundamental physics at “burst” to better understand what burst means in a physical sense, rather than the traditional understanding of burst as a peak in voltage and increase in resistance. This fundamental understanding has led to increased knowledge on the mechanisms of burst and has allowed us to improve our predictive capability through magnetohydrodnamic modeling. This manuscript presents results from several EFI designs along with a look to the future for upcoming work.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

High-energy diffraction microscopy at the advanced photon source

The status of the High Energy Diffraction Microscopy (HEDM) program at the 1-ID beam line of the Advanced Photon Source is reported. HEDM applies high energy synchrotron radiation for the grain and sub-grain scale structural and mechanical characterization of polycrystalline bulk materials in situ during thermomechanical loading. Case studies demonstrate the mapping of grain boundary topology, the evaluation of stress tensors of individual grains during tensile deformation and comparison to a finite element modeling simulation, and the characterization of evolving dislocation structure. Complementary information is obtained by post mortem electron microscopy on the same sample volume previously investigated by HEDM.

43 PARTICLE ACCELERATORS↗

Conceptual design of front ends for the advanced photon source multi-bend achromats upgrade

The proposed Advanced Photon Source (APS) upgrade from a double-bend achromats (DBA) to multi-bend achromats (MBA) lattice with ring energy change from 7 GeV to 6 GeV and beam current from 100 mA to 200 mA poses new challenges for front ends. All front ends must be upgraded to fulfill the following requirements: 1) handle the high heat load from two insertion devices in either inline or canted configuration, 2) include a clearing magnet in the front end to deflect and dump any electrons in case the electrons escape from the storage ring during swap-out injection with the safety shutters open, 3) incorporate the next generation x-ray beam position monitors (XBPMs) into the front end to meet the new stringent beam stability requirements. This paper presents the evaluation of the existing APS front ends and standardizes the insertion device (ID) front ends into two types: one for the single beam and one for the canted beams. The conceptual design of high heat load front end (HHLFE) and canted undulator front end (CUFE) for APS MBA upgrade is presented.

43 PARTICLE ACCELERATORS↗

Spatially Resolved Elemental Analysis, Spectroscopy and Diffraction at the GSECARS Sector at the Advanced Photon Source

X‐ray microprobes (XRM) coupled with high‐brightness synchrotron X‐ray facilities are powerful tools for environmental biogeochemistry research. One such instrument, the XRM at the Geo Soil Enviro Center for Advanced Radiation Sources Sector 13 at the Advanced Photon Source (APS; Argonne National Laboratory, Lemont, IL) was recently improved as part of a canted undulator geometry upgrade of the insertion device port, effectively doubling the available undulator beam time and extending the operating energy of the branch supporting the XRM down to the sulfur K edge (2.3 keV). Capabilities include rapid, high‐resolution, elemental imaging including fluorescence microtomography, microscale X‐ray absorption fine structure spectroscopy including sulfur K edge capability, and microscale X‐ray diffraction. These capabilities are advantageous for (i) two‐dimensional elemental mapping of relatively large samples at high resolution, with the dwell times typically limited only by the count times needed to obtain usable counting statistics for low concentration elements, (ii) three‐dimensional imaging of internal elemental distributions in fragile hydrated specimens, such as biological tissues, avoiding the need for physical slicing, (iii) spatially resolved speciation determinations of contaminants in environmental materials, and (iv) identification of contaminant host phases. In this paper, we describe the XRM instrumentation, techniques, applications demonstrating these capabilities, and prospects for further improvements associated with the proposed upgrade of the APS. Core Ideas X‐ray microprobes are powerful tools for environmental biogeochemistry. Upgraded GSECARS XRM operates down to the sulfur K edge. Capabilities: spatially resolved elemental analysis, spectroscopy, and diffraction. Advanced Photon Source upgrade will further advance XRM capabilities.

Sutton, Stephen R.↗

Status of the Short-Pulse X-ray Project (SPX) at the Advanced Photon Source (APS)

The Advanced Photon Source Upgrade project (APS-U) at Argonne includes implementation of Zholents’* deflecting cavity scheme for production of short x-ray pulses. This is a joint project between Argonne National Laboratory, Thomas Jefferson National Laboratory, and Lawrence Berkeley National Laboratory. This paper describes performance characteristics of the proposed source and technical issues related to its realization. Ensuring stable APS storage ring operation requires reducing quality factors of these modes by many orders of magnitude. These challenges reduce to those of the design of a single-cell SC cavity that can achieve the desired operating deflecting fields while providing needed damping of all these modes. The project team is currently prototyping and testing several promising designs for single-cell cavities with the goal of deciding on a winning design in the near future. Here

43 PARTICLE ACCELERATORS↗

Tolerance analyses of a quadrupole magnet for advanced photon source upgrade

Given physics requirements, the mechanical fabrication and assembly tolerances for storage ring magnets can be calculated using analytical methods [1, 2]. However, this method is not easy for complicated magnet designs [1]. In this paper, a novel method is proposed to determine fabrication and assembly tolerances consistent with physics requirements, through a combination of magnetic and mechanical tolerance analyses. In this study, finite element analysis using OPERA is conducted to estimate the effect of fabrication and assembly errors on the magnetic field of a quadrupole magnet and to determine the allowable tolerances to achieve the specified magnetic performances. Based on the study, allowable fabrication and assembly tolerances for the quadrupole assembly are specified for the mechanical design of the quadrupole magnet. Next, to achieve the required assembly level tolerances, mechanical tolerance stackup analyses using a 3D tolerance analysis package are carried out to determine the part and subassembly level fabrication tolerances. This method can be used to determine the tolerances for design of other individual magnets and of magnet strings.

43 PARTICLE ACCELERATORS↗

Field Quality from Tolerance Stack-up In R&D Quadrupoles for the Advanced Photon Source Upgrade

The Advanced Photon Source (APS) at Argonne National Laboratory (ANL) is considering upgrading the current double-bend, 7-GeV, 3rd generation storage ring to a 6-GeV, 4th generation storage ring with a Multibend Achromat (MBA) lattice. In this study, a novel method is proposed to determine fabrication and assembly tolerances through a combination of magnetic and mechanical tolerance analyses. Mechanical tolerance stackup analyses using Teamcenter Variation Analysis are carried out to determine the part and assembly level fabrication tolerances. Finite element analyses using OPERA are conducted to estimate the effect of fabrication and assembly errors on the magnetic field of a quadrupole magnet and to determine the allowable tolerances to achieve the desired magnetic performance. Finally, results of measurements in R&D quadrupole prototypes are compared with the analysis results.

Quadrupole, Field quality, tolerance, Finite Eleme↗

Beam Characterization and Coherent Optical Transition Radiation Studies at the Advanced Photon Source Linac

The Advanced Photon Source facility includes a 450-MeV S-band linac with the option for injection from a photocathode (PC) rf gun. A diode-pumped, twice-frequency doubled Nd:glass regen laser (263 nm) is used with the Cu PC to generate the ele ctron beams. Characterization of these beams and studies of the microbunching instability following beam compression in the four-dipole magnetic chicane are described. A suite of diagnostics is employed including a three-screen emittance section, a FIR co herent transition radiation autocorrelator, electron spectrometers, and an optical diagnostics end station. An energy chirp impressed on the beam is used to compress the 1-2 ps, rms bunch as it passes through the chicane. With compression, bunch lengths o f 170-200 fs, rms at 450 pC are measured, and coherent optical transition radiation (COTR) due to the microbunching instability is observed. Mitigation techniques of the COTR in the beam profile diagnostics are demonstrated both spectrally and temporally. At 100 pC without compression normalized transverse emittances of 1.8 and 2.7 microns are observed in the x and y planes, in reasonable agreement with initial ASTRA simulations.

43 PARTICLE ACCELERATORS↗

GeoSoilEnviroCARS (Sector 13) at the Advanced Photon Source: a comprehensive synchrotron radiation facility for Earth science research at ambient and extreme conditions

GeoSoilEnviroCARS (GSECARS) is a comprehensive analytical laboratory for Earth and environmental science research using X-ray beams from the Advanced Photon Source, Argonne National Laboratory. State-of-the-art instruments are available for (1) high-pressure/high- or low-temperature diffraction, total scattering, and spectroscopy (Brillouin, Raman, and VIS-IR) using the laser heated diamond anvil cell (DAC); (2) high-pressure/high-temperature diffraction, scattering, and imaging as well as acoustic emission (AE) and ultrasonics using the large-volume press (LVP); (3) powder, single crystal, and surface/interface diffraction; (4) X-ray absorption fine structure spectroscopy; (5) X-ray fluorescence microprobe analysis; and (6) microtomography. As shown here, experiments are facilitated by senior level staff who collaborate on all aspects of the analytical work including experiment design, sample preparation, data collection, data interpretation, and publication preparation. Both technical and scientific synergies occur as a result of the intimate association of the various techniques and scientists experienced in the applications of synchrotron radiation to Earth, environmental, and planetary science problems. The facility includes state-of-the-art instrumentation designed and built in-house, including custom X-ray optics, online and offline laser-based systems, specialized sample environments and positioning systems, as well as pixel-array and multi-crystal energy dispersive X-ray detectors, which are available to be shared among the experimental stations.

36 MATERIALS SCIENCE↗

Progress on the development of the next generation x-ray beam position monitors at the advanced photon source

Accurate and stable x-ray beam position monitors (XBPMs) are key elements in obtaining the desired user beam stability in the Advanced Photon Source (APS). The next generation XBPMs for high heat load front ends (HHL FEs) have been designed to meet these requirements by utilizing Cu K-edge x-ray fluorescence (XRF) from a pair of copper absorbers and have been installed at the front ends (FEs) of the APS. Commissioning data showed a significant performance improvement over the existing photoemission-based XBPMs. While a similar design concept can be applied for the canted undulator front ends, where two undulator beams are separated by 1.0-mrad, the lower beam power (< 10 kW) per undulator allows us to explore lower-cost solutions based on Compton scattering from the diamond blades placed edge-on to the x-ray beam. A prototype of the Compton scattering XBPM system was installed at 24-ID-A in May 2015. In this report, the design and test results for XRF-based XBPM and Compton scattering based XBPM are presented. Ongoing research related to the development of the next generation XBPMs on thermal contact resistance of a joint between two solid bodies is also discussed.

43 PARTICLE ACCELERATORS↗