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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 1,765 records · Page 98
All sourcesNASA NTRSDOE OSTI
DOE OSTI2019

Significant Phonon Drag Enables High Power Factor in the AlGaN/GaN Two-Dimensional Electron Gas

In typical thermoelectric energy harvesters and sensors, the Seebeck effect is caused by diffusion of electrons or holes in a temperature gradient. However, the Seebeck effect can also have a phonon drag component, due to momentum exchange between charge carriers and lattice phonons, which is more difficult to quantify. In this work, we present the first study of phonon drag in the AlGaN/GaN two-dimensional electron gas (2DEG). We find that phonon drag does not contribute significantly to the thermoelectric behavior of devices with ~100 nm GaN thickness, which suppresses the phonon mean free path. Yet, when the thickness is increased to ~1.2 μm, up to 32% (88%) of the Seebeck coefficient at 300 K (50 K) can be attributed to the drag component. In turn, the phonon drag enables state-of-the-art thermoelectric power factor in the thicker GaN film, up to ~40 mW m –1 K –2 at 50 K. By measuring the thermal conductivity of these AlGaN/GaN films, we show that the magnitude of the phonon drag can increase even when the thermal conductivity decreases. Decoupling of thermal conductivity and Seebeck coefficient could enable important advancements in thermoelectric power conversion with devices based on 2DEGs.

2D electron gas (2DEG)↗
DOE OSTI2019

Spectroscopic Comparison of Thermal Transport at Organic–Inorganic and Organic-Hybrid Interfaces Using CsPbBr 3 and FAPbBr 3 (FA = Formamidinium) Perovskite Nanocrystals

Thermal transport across interfaces depends on the matching of vibrational structure at the interface. This work examines the transfer of thermal excitation from an organic ligand coating to either all-inorganic cesium lead tribromide (CsPbBr 3 ) nanocrystals or hybrid organic-inorganic formamidinium lead tribromide (FAPbBr 3 ) nano crystals using selective infrared optical excitation. Here, these two semiconductors are directly compared because they (or similar semiconductors) are currently envisioned as strong candidates in many optoelectronic technologies and they differ due to the presence of an organic or inorganic cation, which introduces substantial differences in the phonon density of states in otherwise quite similar semiconductors. Infrared excitation of C-H vibrations of surface-bound ligands generates a temperature gradient between the organic ligand shell and nanocrystal core, which results in heat flow, measured by probing changes of the semiconductor band gap. Heat transfer to both perovskite compositions of comparable sizes is similar (25-30 ps), due to fast intramolecular vibrational relaxation and similar matching of low-energy phonons with the organic ligand, but FAPbBr 3 samples show a slow bleaching kinetic on the order of 1 ns. This slow, heat-induced change in the semiconductor band gap is attributed not to interfacial heat transfer but instead to thermal equilibration between the organic and inorganic sublattices of FAPbBr 3 . Ab initio molecular dynamics simulations support the hypothesis that low-energy inorganic sublattice phonon modes are populated initially in the heat transfer process, with a slow thermal population of the higher-energy phonon modes associated primarily with the organic cation. Slow thermal equilibration of FAPbBr 3 is likely to substantially impact the time-dependent response of optoelectronic devices that heat the semiconductor active layer and provide further evidence that the poor bulk thermal transport of hybrid perovskite materials extends to microscopic thermal processes.

77 NANOSCIENCE AND NANOTECHNOLOGY↗
DOE OSTI2020

High-Quality SnSe 2 Single Crystals: Electronic and Thermoelectric Properties

In this work, high-quality SnSe 2 single crystals were successfully synthesized using a temperature gradient method. N-type characteristics and strong anisotropic transport properties of SnSe 2 single crystals were exhibited between the ab plane and the c-axis. At 673 K, the power factor (PF) value along the ab plane is 3.43 μW cm -1 K -2 , while it is 0.92 μW cm -1 K -2 along the c-axis. The ratio between thermal conductivities along the ab plane (κ ab ) and c-axis (κ c ) is on the order of 7.6 at 300 K, while this value is about 5.6 at 673 K. The thermoelectric figure of merit (ZT) in the c-axis (0.15) is higher than that (0.1) along the ab plane, according to the ultralow out-of-plane thermal conductivity. The electronic band structure results, which were examined by angle-resolved photoemission spectroscopy (ARPES) predicted the potential of improving the thermoelectric performance of SnSe 2 single crystals by electron doping.

36 MATERIALS SCIENCE↗
DOE OSTI2021

Suspended Membrane Evaporators Integrating Environmental and Solar Evaporation for Oily Wastewater Purification

Solar-driven evaporation is promising in oily wastewater treatment, in particular for emulsions, but conventional evaporators suffer from pore blocking by residual oil or contamination by volatile oil compounds in the condensed water. In the current research, we develop a suspended membrane evaporator integrating solar evaporation with oil-in-water emulsion separation. The heating and evaporating interface is separated from the rejecting interface to avoid oil escape and improve heat management. A temperature gradient forms on the membrane surface that can promote evaporation performance by combining both solar and environmental evaporation. Such an evaporator achieves a maximum evaporation rate of 1.645 kg/(m 2 ·h) as well as an apparent evaporation efficiency of 111.9%. Moreover, the superhydrophilic and superoleophobic membrane shows excellent oil repellence and emulsion rejection, which can achieve an oil removal efficiency above 98.8% in oil-in-water emulsion separation, and high evaporation rate recovery in cycling tests. Furthermore, a scaled-up membrane evaporator array produces ~8 kg/(m 2 ·d) of clean water from oily wastewater in outdoor experiments, further demonstrating the strong purification performance of this evaporator in oily wastewater treatment.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2024

Recycling of Post-Consumer Waste Polystyrene Using Commercial Plastic Additives

Photothermal conversion can promote plastic depolymerization (chemical recycling to a monomer) through light-to-heat conversion. The highly localized temperature gradient near the photothermal agent surface allows selective heating with spatial control not observed with bulk pyrolysis. However, identifying and incorporating practical photothermal agents into plastics for end-of-life depolymerization have not been realized. Interestingly, plastics containing carbon black as a pigment present an ideal opportunity for photothermal conversion recycling. Herein, we use visible light to depolymerize polystyrene plastics into styrene monomers by using the dye in commercial black plastics. A model system is evaluated by synthesizing polystyrene–carbon black composites and depolymerizing under white LED light irradiation, producing styrene monomer in up to 60% yield. Excitingly, unmodified postconsumer black polystyrene samples are successfully depolymerized to a styrene monomer without adding catalysts or solvents. Using focused solar irradiation, yields up to 80% are observed in just 5 min. Furthermore, combining multiple types of polystyrene plastics with a small percentage of black polystyrene plastic enables full depolymerization of the mixture. This simple method leverages existing plastic additives to actualize a closed-loop economy of all-colored plastics.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2012

Generalized Two-Dimensional Perturbation Correlation Infrared Spectroscopy reveals Mechanisms for the Development of Surface Charge and Recalcitrance in Plant-derived Biochars

Fundamental knowledge of how biochars develop surface-charge and resistance to environmental degradation (or recalcitrance) is crucial to their production for customized applications or, understanding their functions in the environment. Two-dimensional perturbation-based correlation infrared spectroscopy (2D-PCIS) was used to study the biochar formation process in three taxonomically-different plant biomass, under oxygen-limited conditions along a heat-treatment-temperature gradient (HTT; 200-650 oC). Results from 2D-PCIS pointed to the systematic, HTT-induced defragmenting of lignocellulose H-bonding network, and demethylenation/demethylation, oxidation or dehydroxylation/dehydrogenation of lignocellulose fragments as the primary reactions controlling biochar properties along the HTT gradient. The cleavage of OH O-type H-bonds, oxidation of free primary hydroxyls (HTT≤500 oC), and their subsequent dehydrogenation/dehydroxylation (HTT>500 oC) controlled surface charge on the biochars; while the dehydrogenation of methylene groups, which yielded increasingly condensed structures (R-CH2-R →R=CH-R →R=C=R), controlled biochar recalcitrance. Variations in biochar properties across plant biomass type were attributable to taxa-specific transformations. For example, apparent inefficiencies in the cleavage of wood-specific H-bonds, and their subsequent oxidation to carboxyls, lead to lower surface charge in wood biochars (compared to grass biochars). Both non-taxa and taxa-specific transformations highlighted by 2D-PCIS could have significant implications for biochar functioning in fire-impacted or biochar-amended systems.

Harvey, Omar R↗
DOE OSTI2024

A Mechanism-Based Reaction–Diffusion Model for Accelerated Discovery of Thermoset Resins Frontally Polymerized by Olefin Metathesis

Frontal ring-opening metathesis polymerization (FROMP) involves a self-perpetuating exothermic reaction, which enables the rapid and energy-efficient manufacturing of thermoset polymers and composites. Current state-of-the-art reaction–diffusion FROMP models rely on a phenomenological description of the olefin metathesis kinetics, limiting their ability to model the governing thermo-chemical FROMP processes. Furthermore, the existing models are unable to predict the variations in FROMP kinetics with changes in the resin composition and as a result are of limited utility toward accelerated discovery of new resin formulations. In this work, we formulate a chemically meaningful model grounded in the established mechanism of ring-opening metathesis polymerization (ROMP). Our study aims to validate the hypothesis that the ROMP mechanism, applicable to monomer-initiator solutions below 100 °C, remains valid under the nonideal conditions encountered in FROMP, including ambient to >200 °C temperatures, sharp temperature gradients, and neat monomer environments. Through extensive simulations, we demonstrate that our mechanism-based model accurately predicts the FROMP behavior across various resin compositions, including polymerization front velocities and thermal characteristics (e.g., T max ). Additionally, we introduce a semi-inverse workflow that predicts FROMP behavior from a single experimental data point. Notably, the physiochemical parameters utilized in our model can be obtained through DFT calculations and minimal experiments, highlighting the model’s potential for rapid screening of new FROMP chemistries in pursuit of thermoset polymers with superior thermo-chemo-mechanical properties.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2012

Fast and Slow Responses of the South Asian Monsoon System to Anthropogenic Aerosols

Using a global climate model with fully predictive aerosol life cycle, we investigate the fast and slow responses of the South Asian monsoon system to anthropogenic aerosol forcing. Our results show that the feedbacks associated with sea surface temperature (SST) change caused by aerosols play a more important role than the aerosol's direct impact on radiation, clouds and land surface (rapid adjustments) in shaping the total equilibrium climate response of the monsoon system to aerosol forcing. Inhomogeneous SST cooling caused by anthropogenic aerosols eventually reduces the meridional tropospheric temperature gradient and the easterly shear of zonal winds over the region, slowing down the local Hadley cell circulation, decreasing the northward moisture transport, and causing a reduction in precipitation over South Asia. Although total responses in precipitation are closer to the slow responses in general, the fast component dominates over land areas north of 25°N. Our results also show an east-west asymmetry in the fast responses to anthropogenic aerosols causing increases in precipitation west of 80°E but decreases east of it.

aerosols↗
DOE OSTI2019

Intensification of the Pre-Meiyu Rainband in the Late 21st Century

Increased atmospheric moisture content and changing land-ocean thermal contrasts are usually implicated in the East Asian summer rainfall response to global warming. We highlight an additional influence whereby increased meridional stationary eddy circulation downstream of the Tibetan Plateau drives a stronger moisture flux convergence over southeastern China, intensifying the early summer rainband. This effect occurs robustly across the Community Earth System Model large ensemble Representative Control Pathway 8.5 simulations, and only for its pre-Meiyu stage (mid-May through late June). The westerly jet impinging on the Plateau is also enhanced, suggesting an orographic influence on the westerlies as the root cause. The increased westerlies result from warmer tropical tropospheric temperatures that enhance the meridional temperature gradient at the latitudes of the Plateau. Finally, our results highlight the potential role of the westerlies in altering the East Asian early summer monsoon rainfall in the late 21st century.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2019

Effects of Model Resolution, Physics, and Coupling on Southern Hemisphere Storm Tracks in CESM1.3

Two high–resolution versions of a Coupled Earth System Model (CESM1.3: 0.25° atmosphere, 1° ocean; CESM1.1: 0.25° atmosphere, 0.1° ocean) are compared to the standard resolution CESM1.1 and CESM1.3 (1° atmosphere, 1° ocean). The CESM1.3 versions are documented, and the consequences of model resolution, air–sea coupling, and physics in the atmospheric models are studied with regard to storm tracks in the Southern Hemisphere as represented by 850–hPa eddy kinetic energy. Increasing the resolution from 1° to 0.25° in the atmosphere (same physics) coupled to the 1° ocean intensifies the strength of the storm tracks closer to observations. The 0.25° atmosphere with the older CESM1.1 physics coupled to the 0.1° ocean has fewer low clouds, warmer Southern Ocean sea surface temperatures, a weaker meridional temperature gradient, and a degraded storm track simulation compared to the 0.25° atmosphere with CESM1.3 physics coupled to the 1° ocean. Furthermore, deficient physics in the atmospheric model can negate the gains attained by higher resolution in atmosphere and ocean.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

Seasonally Modulated Stratospheric Aerosol Geoengineering Alters the Climate Outcomes

Abstract By reflecting some incoming solar radiation, stratospheric aerosol intervention using SO 2 would reduce global mean temperature. Previous research has shown that multiple injection latitudes can be used to maintain not only global mean temperature, but also interhemispheric and equator‐to‐pole temperature gradients. However, the regional climate response depends not only on where the SO 2 is injected, but also on when. We show here that even with these same objectives and same choices of latitudes, injecting in only one season instead of continuously throughout the year results in significant differences in regional climate, for instance in the magnitude of precipitation changes over India. The differential outcomes highlight the potential for underlying trade‐offs, with different choices regarding deployment leading to a different distribution of benefits or harms. This aspect of climate engineering should be considered in developing governance and emphasizes the need for a deeper understanding of the mechanisms underlying the regional responses.

Visioni, Daniele↗
DOE OSTI2020

Impacts of Latent Energy and Snow Fall Speed on a Wintertime Midlatitude Cyclone

This study aimed to understand the impacts of latent energy as well as snow fall speeds on precipitation properties and synoptic-scale storm characteristics of a wintertime midlatitude cyclone. Simulations of a potent winter storm that impacted the Rocky Mountains and northern Great Plains of the United States in February 2017 were performed using the Weather Research and Forecasting model with latent heating or cooling from individual microphysical processes systematically turned off and fall speeds adjusted by ±50%. Results indicated substantial impacts on the microphysical characteristics of the simulated storm to fall speed, cooling from sublimation, and warming from deposition. The impacts of cooling and warming were manifested as differences in accumulated snowfall. Increased (decreased) fall speeds led to smaller (larger) ice crystals and total mass, resulting in offsetting effects on the precipitation flux, and thus minimal impacts on snowfall and large-scale characteristics of the storm. Warming and cooling associated with deposition and sublimation, respectively, impacted the synoptic-scale dynamics, whereby removing warming from deposition resulted in an increased meridional temperature gradient near the jet stream, thus increasing the jet strength and causing it to be more westerly with less curvature aloft. This in turn limited upper-level divergence, creating a weaker surface low and shifting the precipitation shield southward. The opposite occurred with the removal of latent cooling due to sublimation. This study highlights the potential importance of latent energy associated with ice sublimation and deposition and fall speeds in the larger-scale characteristics of winter storms.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2021

An Overview of Atmospheric Features Over the Western North Atlantic Ocean and North American East Coast—Part 2: Circulation, Boundary Layer, and Clouds

The Western North Atlantic Ocean (WNAO) is a complex land-ocean-atmosphere system that experiences a wide range of atmospheric phenomena, which in turn drive unique aerosol transport pathways, cloud morphologies, and boundary layer variability. This work, Part 2 of a 2-part paper series, provides an overview of the atmospheric circulation, boundary layer variability, three-dimensional cloud structure, and precipitation over the WNAO; the companion paper (Part 1) focused on chemical characterization of aerosol, gas, and wet deposition. Seasonal changes in the circulation and sea surface temperature explain a clear transition in cloud morphologies from small shallow cumulus clouds, convective clouds, and tropical storms in summer, to stratus/stratocumulus and multi-layer cloud systems associated with winter storms. Synoptic variability in cloud fields is estimated using satellite-based weather states, and the role of postfrontal conditions (cold-air outbreaks) in the development of stratiform clouds is further analyzed. Precipitation is persistent over the ocean, with a regional peak over the Gulf Stream path, where offshore sea surface temperature gradients are large and surface fluxes reach a regional peak. Satellite data show a clear annual cycle in cloud droplet number concentration along the coast in winter, and minima in summer, suggesting a marked annual cycle in aerosol-cloud interactions. The performance of four climate models are assessed against satellite cloud retrievals. The models qualitatively reproduce the annual cycle in cloud cover and liquid water path, but with large discrepancies across models, especially in the extra-tropics. The paper concludes with a summary of outstanding issues and recommendations for future work.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

The Role of Coupled Feedbacks in the Decadal Variability of the Southern Hemisphere Eddy-Driven Jet

The Southern Hemisphere summertime eddy-driven jet and storm tracks have shifted poleward over the recent few decades. In previous studies, explanations have mainly stressed the influence of external forcing in driving this trend. Here we examine the role of internal tropical SST variability in controlling the austral summer jet’s poleward migration, with a focus on interdecadal time scales. The role of external forcing and internal variability are isolated by using a hierarchy of Community Earth System Model version 1 (CESM1) simulations, including the pre-industrial control, large ensemble, and pacemaker runs. Model simulations suggest that in the early twenty-first century, both external forcing and internal tropical Pacific SST variability are important in driving a positive southern annular mode (SAM) phase and a poleward migration of the eddy-driven jet. Additionally, Tropical Pacific SST variability, associated with the negative phase of the interdecadal Pacific oscillation (IPO), acts to shift the jet poleward over the southern Indian and southwestern Pacific Oceans and intensify the jet in the southeastern Pacific basin, while external forcing drives a significant poleward jet shift in the South Atlantic basin. In response to both external forcing and decadal Pacific SST variability, the transient eddy momentum flux convergence belt in the middle latitudes experiences a poleward migration due to the enhanced meridional temperature gradient, leading to a zonally symmetric southward migration of the eddy-driven jet. This mechanism distinguishes the influence of the IPO on the midlatitude circulation from the dynamical impact of ENSO, with the latter mainly promoting the subtropical wave-breaking critical latitude poleward and pushing the midlatitude jet to higher latitudes.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2022

Westward-Propagating Moisture Mode Over the Tropical Western Hemisphere

A westward-propagating Rossby-like wave signal is found to explain a large fraction of the intraseasonal variance in cloud brightness over the Western Hemisphere. A series of diagnostic criteria suggest that this wave is a moisture mode: its moisture anomalies dominate the distribution of moist static energy (MSE) and are in phase with the precipitation anomalies; and the thermodynamic equation obeys the weak temperature gradient approximation. Further, the wave propagates westward due to zonal moisture advection by the mean flow and is maintained by radiative heating and meridional moisture advection. These properties compare favorably with the westward propagating Rossby mode in an equatorial beta-plane model with prognostic moisture, mean meridional moisture gradient, and mean zonal wind. These results underscore the importance of water vapor in the dynamics of slowly evolving tropical systems, and the limitations of dry shallow water theory that rely on a “reduced equivalent depth” to represent moist dynamics.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

Convective Vortices and Dust Devils Detected and Characterized by Mars 2020

Abstract We characterize vortex and dust devils (DDs) at Jezero from pressure and winds obtained with the Mars Environmental Dynamics Analyzer (MEDA) instrument on Mars 2020 over 415 Martian days (sols) ( Ls = 6°–213°). Vortices are abundant (4.9 per sol with pressure drops >0.5 Pa correcting from gaps in coverage) and they peak at noon. At least one in every five vortices carries dust, and 75% of all vortices with Δ p > 2.0 Pa are dusty. Seasonal variability was small but DDs were abundant during a dust storm ( Ls = 152°–156°). Vortices are more frequent and intense over terrains with lower thermal inertia favoring high daytime surface‐to‐air temperature gradients. We fit measurements of winds and pressure during DD encounters to models of vortices. We obtain vortex diameters that range from 5 to 135 m with a mean of 20 m, and from the frequency of close encounters we estimate a DD activity of 2.0–3.0 DDs km −2 sol −1 . A comparison of MEDA observations with a Large Eddy Simulation of Jezero at Ls = 45° produces a similar result. Three 100‐m size DDs passed within 30 m of the rover from what we estimate that the activity of DDs with diameters >100 m is 0.1 DDs km −2 sol −1 , implying that dust lifting is dominated by the largest vortices in Jezero. At least one vortex had a central pressure drop of 9.0 Pa and internal winds of 25 ms −1 . The MEDA wind sensors were partially damaged during two DD encounters whose characteristics we elaborate in detail.

Hueso, R.↗
DOE OSTI2022

Near‐Surface Hydrology and Soil Properties Drive Heterogeneity in Permafrost Distribution, Vegetation Dynamics, and Carbon Cycling in a Sub‐Arctic Watershed

Abstract Discontinuous permafrost environments exhibit strong spatial heterogeneity at scales too small to be driven by weather forcing or captured by Earth System Models. Here we analyze effects of observed spatial heterogeneity in soil and vegetation properties, hydrology, and thermal dynamics on ecosystem carbon dynamics in a watershed on the Seward Peninsula in Alaska. We apply a Morris global sensitivity analysis to a process‐rich, successfully tested terrestrial ecosystem model (TEM), ecosys , varying soil properties, boundary conditions, and weather forcing. We show that landscape heterogeneity strongly impacts soil temperatures and vegetation composition. Snow depth, O‐horizon thickness, and near‐surface water content, which vary at scales of O(m), control the soil thermal regime more than an air temperature gradient corresponding to a 140 km north–south distance. High shrub productivity is simulated only in talik (perennially unfrozen) soils with high nitrogen availability. Through these effects on plant and permafrost dynamics, landscape heterogeneity impacts ecosystem productivity. Simulations with near‐surface taliks have higher microbial respiration (by 78.0 gC m −2 yr −1 ) and higher net primary productivity (by 104.9 gC m −2 yr −1 ) compared to runs with near‐surface permafrost, and simulations with high shrub productivity have outlying values of net carbon uptake. We explored the prediction uncertainty associated with ignoring observed landscape heterogeneity, and found that watershed net carbon uptake is 60% larger when heterogeneity is accounted for. Our results highlight the complexity inherent in discontinuous permafrost environments and demonstrate that missing representation of subgrid heterogeneity in TEMs could bias predictions of high‐latitude carbon budget.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

Making a Superbolt: Reconciling Observations of the Optically Brightest Lightning on Earth From Different Satellites

We previously documented geographic distributions of the optically brightest lightning on Earth—known as “superbolts”—using two space-based instruments: the photodiode detector (PDD) on the Fast On-orbit Recording of Transient Events (FORTE) satellite and the Geostationary Lightning Mapper (GLM) on NOAA's Geostationary Operational Environmental Satellites. In this study, we further examine the superbolts identified by the PDD and GLM to reconcile the differences between their geographic distributions. We find that both the physical extent of the parent flash and the development speed of its leaders are important for making a superbolt. The oceanic PDD superbolts tend to occur early in flashes that rapidly expand laterally into long horizontal “megaflashes.” The top GLM superbolts occur over land at later times in particularly large megaflashes. These land-based flashes grow more slowly until they extend over multiple hundreds of kilometers. The FORTE PDD missed these delayed superbolts due to limitations in its triggering. Coincident Tropical Rainfall Measuring Mission measurements show that the warm season megaflash superbolts detected by Lightning Imaging Sensor/GLM and wintertime oceanic superbolts observed by the PDD occur in otherwise similar thunderstorm environments. Both are marked by: low storm heights (<10 km), widespread precipitation near the surface, small infrared brightness temperature gradients, and low flash rates. We suggest that the vertically compact, stratiform nature of these clouds provides favorable conditions for superbolt production.

54 ENVIRONMENTAL SCIENCES↗