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At least 1,765 records · Page 98
All sourcesNASA NTRSDOE OSTI
DOE OSTI2018

Quantum tricritical point in the temperature-pressure-magnetic field phase diagram of CeTiGe 3

We report the temperature-pressure-magnetic eld phase diagram of the ferromagnetic Kondolattice CeTiGe 3 determined by means of electrical resistivity measurements. Measurements up to ~5.8GPa reveal a rich phase diagram with multiple phase transitions. At ambient pressure, CeTiGe 3 orders ferromagnetically at T C =14 K. Application of pressure suppresses T C , but a pressure induced ferromagnetic quantum criticality is avoided by the appearance of two new successive transitions for p>4.1GPa that are probably antiferromagnetic in nature. These two transitions are suppressed under pressure, with the lower temperature phase being fully suppressed above 5.3GPa. The critical pressures for the presumed quantum phase transitions are p1≅4.1GPa and p2≅5.3GPa. Above 4.1GPa, application of magnetic eld shows a tricritical point evolving into a wing structure phase with a quantum tricritical point at 2.8T at 5.4GPa, where the rst order antiferromagneticferromagnetic transition changes into the second order antiferromagnetic-ferromagnetic transition.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2019

Anisotropic magnetic entropy change in Cr 2 X 2 Te 6 ( X = Si and Ge )

Intrinsic, two-dimensional (2D) ferromagnetic semiconductors are an important class of materials for spintronics applications. Cr 2 X 2 Te 6 ( X = Si and Ge ) semiconductors show 2D Ising-like ferromagnetism, which is preserved in few-layer devices. The maximum magnetic entropy change associated with the critical properties around the ferromagnetic transition for Cr 2 Si 2 Te 6 - ΔS$max\atop{M}$ ~ 5.05 J kg -1 K -1 is much larger than - ΔS$max\atop{M}$ ~ 2.64 J kg -1 K -1 for Cr 2 Ge 2 Te 6 with an out-of-plane field change of 5 T. The rescaled - ΔS M (T,H) curves collapse onto a universal curve independent of temperature and field for both materials. Here, this indicates similar critical behavior and 2D Ising magnetism, confirming the magnetocrystalline anisotropy that could preserve the long-range ferromagnetism in a few layers of Cr 2 X 2 Te 6 .

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2020

Evolution of noncollinear magnetism in magnetocaloric MnPtGa

MnPtGa crystallizes in the hexagonal Ni 2 In structure type in space group P6 3 /mmc and has been reported to display a ferromagnetic Curie temperature near 220K. Here we find a transition near T c = 236 K to a ferromagnetic state, albeit with a reduced moment from what is expected for collinear ordering. The peak magnetocaloric entropy change was determined to be ΔS M = –1.9 J kg –1 K –1 for an applied magnetic field of H = 5 T at the ferromagnetic ordering temperature. Magnetostructural coupling manifests as a change in the slope of the thermal expansion coefficients of the c lattice parameter near T c , with a negative spontaneous volume magnetostriction; ω = –300 ppm at 190K. In this work, neutron powder diffraction studies of the magnetic ground state reveal an evolution in complexity as temperature decreases: from a ferromagnet, to a canted antiferromagnet, to the eventual formation of a spin-density-wave state at low temperatures.

36 MATERIALS SCIENCE↗
DOE OSTI2018

Optical manipulation of magnetic vortices visualized in situ by Lorentz electron microscopy

By understanding the fundamental dynamics of topological vortex and antivortex naturally formed in microscale/nanoscale ferromagnetic building blocks under external perturbations is crucial to magnetic vortex–based information processing and spintronic devices. All previous studies have focused on magnetic vortex–core switching via external magnetic fields, spin-polarized currents, or spin waves, which have largely prohibited the investigation of novel spin configurations that could emerge from the ground states in ferromagnetic disks and their underlying dynamics. We report in situ visualization of femtosecond laser quenching–induced magnetic vortex changes in various symmetric ferromagnetic Permalloy disks by using Lorentz phase imaging of four-dimensional electron microscopy that enables in situ laser excitation. Besides the switching of magnetic vortex chirality and polarity, we observed with distinct occurrence frequencies a plenitude of complex magnetic structures that have never been observed by magnetic field– or current-assisted switching. These complex magnetic structures consist of a number of newly created topological magnetic defects (vortex and antivortex) strictly conserving the topological winding number, demonstrating the direct impact of topological invariants on magnetization dynamics in ferromagnetic disks. Their spin configurations show mirror or rotation symmetry due to the geometrical confinement of the disks. Combined micromagnetic simulations with the experimental observations reveal the underlying magnetization dynamics and formation mechanism of the optical quenching–induced complex magnetic structures. Their distinct occurrence rates are pertinent to their formation-growth energetics and pinning effects at the disk edge. On the basis of these findings, we propose a paradigm of optical quenching–assisted fast switching of vortex cores for the control of magnetic vortex–based information recording and spintronic devices.

4D electron microscopy↗
DOE OSTI2019

Magnetization switching using topological surface states

Topological surface states (TSSs) in a topological insulator are expected to be able to produce a spin-orbit torque that can switch a neighboring ferromagnet. This effect may be absent if the ferromagnet is conductive because it can completely suppress the TSSs, but it should be present if the ferromagnet is insulating. This study reports TSS-induced switching in a bilayer consisting of a topological insulator Bi 2 Se 3 and an insulating ferromagnet BaFe 12 O 19 . A charge current in Bi 2 Se 3 can switch the magnetization in BaFe 12 O 19 up and down. When the magnetization is switched by a field, a current in Bi 2 Se 3 can reduce the switching field by ~4000 Oe. The switching efficiency at 3 K is 300 times higher than at room temperature; it is ~30 times higher than in Pt/BaFe 12 O 19 . These strong effects originate from the presence of more pronounced TSSs at low temperatures due to enhanced surface conductivity and reduced bulk conductivity.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2019

Exchange Bias Training Effect in GdBaCo{sub 2}O{sub 5.5} Cobaltite

The nature of the training effect in exchange bias compounds, which consists in a decrease in the exchange bias field H{sub EB} under magnetic field cycling, is clarified. It is shown that the training effect in GdBaCo{sub 2}O{sub 5 + δ} cobaltite with δ ≈ 0.5 is caused by a decrease in magnetization. Depending on time, magnetization M(t) decreases sharply after the first cycle and slowly in subsequent N cycles. A direct relationship (proportionality) is established between the decrease in the magnetization M(t) of ferromagnetic particles and the change of the field H{sub EB}(t). It is assumed that the cooling of a sample in a magnetic field gives rise to small (single-domain) and large ferromagnetic clusters in an antiferromagnetic environment. The sharp decrease in M(t) and H{sub EB}(t) and the deviation of the function H{sub EB}(N) from the well-known power-law relation ΔH{sub EB} ∝ N{sup –1/2} with N > 1 is explained by the transformation of large ferromagnetic clusters into a multidomain state under magnetic field cycling. The results are consistent with the phenomenological model of Meiklejohn and Bean, which predicts a linear dependence of the exchange bias on the ferromagnetic magnetization of a ferromagnet/antiferromagnet structure.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2013

Room-Temperature Multiferroic Hexagonal LuFeO3

We observed the coexistence of ferroelectricity and weak ferromagnetism at room temperature in the hexagonal phase of LuFeO3 stabilized by epitaxial thin film growth. While the ferroelectricity in hexagonal LuFeO3 can be understood as arising from its polar structure, the observation of weak ferromagnetism at room temperature is remarkable considering the frustrated triangular spin structure. An explanation of the room temperature weak ferromagnetism is proposed in terms of a subtle lattice distortion revealed by the structural characterization. The combination of ferroelectricity and weak ferromagnetism in epitaxial films at room temperature offers great potential for the application of this novel multiferroic material in next generation devices.

Cheng, Xuemei↗
DOE OSTI2013

Magnetism and phase transitions in LaCoO3

Neutron scattering and magnetometry measurements have been used to study phase transitions in LaCoO3 (LCO). For H 100 Oe, evidence for a ferromagnetic (FM) transition is observed at Tc 87 K. For 1 kOe H 60 kOe, no transition is apparent. For all H, Curie Weiss analysis shows predominantly antiferromagnetic (AFM) interactions for T > Tc, but the lack of long-range AFM order indicates magnetic frustration. We argue that the weak ferromagnetism in bulk LCO is induced by lattice strain, as is the case with thin films and nanoparticles. The lattice strain is present at the bulk surfaces and at the interfaces between the LCO and a trace cobalt oxide phase. The ferromagnetic ordering in the LCO bulk is strongly affected by the Co O Co angle ( ), in agreement with recent band calculations which predict that ferromagnetic long-range order can only take place above a critical value, C. Consistent with recent thin film estimations, we find C D 162:8. For > C, we observe power-law behavior in the structural parameters. decreases with T until the critical temperature, To 37 K; below To the rate of change becomes very small. For T < To, FM order appears to be confined to regions close to the surfaces, likely due to the lattice strain keeping the local Co O Co angle above C.

Belanger, David P↗
DOE OSTI2014

Wireless sensor for detecting explosive material

Disclosed is a sensor for detecting explosive devices. The sensor includes a ferromagnetic metal and a molecular recognition reagent coupled to the ferromagnetic metal. The molecular recognition reagent is operable to expand upon absorption of vapor from an explosive material such that the molecular recognition reagent changes a tensile stress upon the ferromagnetic metal. The explosive device is detected based on changes in the magnetic switching characteristics of the ferromagnetic metal caused by the tensile stress.

45 MILITARY TECHNOLOGY, WEAPONRY, AND NATIONAL DEF↗
DOE OSTI2014

Magnetism in nanoparticle LaCoO3

Neutron scattering and magnetometry measurements have been used to study phase transitions in LaCoO3 (LCO). For H <= 100 Oe, evidence for a ferromagnetic (FM) transition is observed at T-c approximate to 87 K. For 1 kOe <= H <= 60 kOe, no transition is apparent. For all H, Curie-Weiss analysis shows predominantly antiferromagnetic (AFM) interactions for T > T-c, but the lack of long-range AFM order indicates magnetic frustration. We argue that the weak ferromagnetism in bulk LCO is induced by lattice strain, as is the case with thin films and nanoparticles. The lattice strain is present at the bulk surfaces and at the interfaces between the LCO and a trace cobalt oxide phase. The ferromagnetic ordering in the LCO bulk is strongly affected by the Co-O-Co angle (gamma), in agreement with recent band calculations which predict that ferromagnetic long-range order can only take place above a critical value, gamma C. Consistent with recent thin film estimations, we find gamma C = 162.8 degrees. For gamma > gamma C, we observe power-law behavior in the structural parameters. gamma decreases with T until the critical temperature, T-o approximate to 37 K; below T-o the rate of change becomes very small. For T < T-o, FM order appears to be confined to regions close to the surfaces, likely due to the lattice strain keeping the local Co-O-Co angle above gamma C.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2016

Wireless sensor

Disclosed is a sensor for detecting a target material. The sensor includes a ferromagnetic metal and a molecular recognition reagent coupled to the ferromagnetic metal. The molecular recognition reagent is operable to expand upon exposure to vapor or liquid from the target material such that the molecular recognition reagent changes a tensile stress upon the ferromagnetic metal. The target material is detected based on changes in the magnetic switching characteristics of the ferromagnetic metal caused by the changes in the tensile stress.

36 MATERIALS SCIENCE↗
DOE OSTI2016

Wireless radiation sensor

Disclosed is a sensor for detecting radiation. The sensor includes a ferromagnetic metal and a radiation sensitive material coupled to the ferromagnetic metal. The radiation sensitive material is operable to change a tensile stress of the ferromagnetic metal upon exposure to radiation. The radiation is detected based on changes in the magnetic switching characteristics of the ferromagnetic metal caused by the changes in the tensile stress.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2017

Self-Assembled Layered Supercell Structure of Bi2AlMnO6 with Strong Room-Temperature Multiferroic Properties.

Room-temperature (RT) multiferroics, possessing ferroelectricity and ferromagnetism simultaneously at RT, hold great promise in miniaturized devices including sensors, actuators, transducers, and multi-state memories. In this work, we report a novel 2D layered RT multiferroic system with self-assembled layered supercell structure consisting of two mismatch-layered sub-lattices of [Bi 3 O 3+δ ] and [MO 2 ] 1.84 (M=Al/Mn, simply named as BAMO), i.e., alternative layered stacking of two mutually incommensurate sublattices made of a three-layer-thick Bi-O slab and a one-layer-thick Al/Mn-O octahedra slab along the out-of-plane direction. Strong room-temperature multiferroic responses, e.g., ferromagnetic and ferroelectric properties, have been demonstrated and attributed to the highly anisotropic 2D nature of the non-ferromagnetic and ferromagnetic sublattices which are highly mismatched. The work demonstrates an alternative design approach for new 2D layered oxide materials that hold promises as single-phase multiferroics, 2D oxides with tunable bandgaps, and beyond.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Nanodevice, method of making the same, and method of using the same

A nanodevice provides for electric-field control of magnon-QSD interactions. The nanodevice includes a ferroelectric substrate, a ferromagnetic material disposed over the ferroelectric substrate, and a nanodiamond including an ensemble of nitrogen-vacancy (NV) spins, each NV magnetically interfacing with the ferromagnetic material. An electric field is measured by applying a voltage across the ferroelectric substrate and the ferromagnetic material, changing a magnon excitation spectrum of the ferromagnetic material with respect to an electron spin resonance frequency of the ensemble of NV spins, and measuring a relaxation rate of the ensemble of NV spins.

Shalaev, Vladimir M.↗
DOE OSTI2011

Soft magnetism and microwave magnetic properties of Fe-Co-Hf films deposited by composition gradient sputtering

A composition gradient sputtering method was employed to deposit a series of (Fe{sub x}Co{sub 1-x}){sub 1-y}Hf{sub y} alloy films with different Fe/Co atomic ratios and Hf-doping. At Fe/Co = 70/30, the magnetically annealed (Fe{sub 0.7}Co{sub 0.3}){sub 1-y}Hf{sub y} films with y = 0.087-0.124 showed a very high uniaxial anisotropy and an ultrahigh ferromagnetic resonance frequency over 7 GHz after the films were annealed at 350 deg. C, while at Fe/Co 50/50, the as-deposited (Fe{sub 0.5}Co{sub 0.5}){sub 1-y}Hf{sub y} films with y 0.074-0.168 showed an excellent in-plane uniaxial anisotropy and high ferromagnetic resonance frequency over 3 GHz. These Fe-Co-Hf films deposited by the composition gradient sputtering method exhibited ahigh saturation magnetization of 1.8 - 2.2 T, a large uniaxial anisotropy field of 200 - 500 Oe, and a high ferromagnetic resonance frequency over 7 GHz, which provides great opportunities for integrated magnetic devices.

36 MATERIALS SCIENCE↗
DOE OSTI2011

Structural, optical and magnetic properties of polycrystalline BaTi{sub 1-x}Fe{sub x}O{sub 3} ceramics

Polycrystalline BaTi{sub 1-x}Fe{sub x}O{sub 3} ceramics have been prepared by conventional solid-state reaction. Their structural, optical and magnetic properties are then studied by means of x-ray diffraction (XRD), Raman scattering (RS) and absorption spectrometers, and a physical properties measurement system. Detailed analyses of XRD patterns and RS spectra reveal the phase separation of the tetragonal-hexagonal structure at a threshold concentration of x = 0.005. The increase in the Fe-doping content (x) leads to development of the hexagonal phase. Magnetic measurements prove that many BaTi{sub 1-x}Fe{sub x}O{sub 3} samples exhibit the room-temperature ferromagnetic order, excepting the samples with x = 0.02-0.06. The ferromagnetism depends strongly on concentration of Fe impurities. The nature of this ferromagnetism is discussed by means of the results of structural analyses and optical absorption spectra.

36 MATERIALS SCIENCE↗
DOE OSTI2013

The local structure, magnetic, and transport properties of Cr-doped In{sub 2}O{sub 3} films

Cr-doped In{sub 2}O{sub 3} films were deposited on Si (100) substrates by RF-magnetron sputtering technique. The local structure, magnetic, and transport properties of films are investigated by X-ray diffraction, X-ray photoelectron spectroscopy, X-ray absorption fine structure, Hall effect, R-T, and magnetic measurements. Structural analysis clearly indicates that Cr ions substitute for In{sup 3+} sites of the In{sub 2}O{sub 3} lattice in the valence of +2 states and Cr-related secondary phases or clusters as the source of ferromagnetism is safely ruled out. The films with low Cr concentration show a crossover from semiconducting to metallic transport behavior, whereas only semiconducting behavior is observed in high Cr concentration films. The transport property of all films is governed by Mott variable range hopping behavior, suggesting that the carriers are strongly localized. Magnetic characterizations show that the saturated magnetization of films increases first, and then decreases with Cr doping, while carrier concentration n{sub c} decreases monotonically, implying that the ferromagnetism is not directly induced by the mediated carriers. It can be concluded the ferromagnetism of films is intrinsic and originates from electrons bound in defect states associated with oxygen vacancies.

36 MATERIALS SCIENCE↗
DOE OSTI2014

Kinetic arrest induced antiferromagnetic order in hexagonal FeMnP{sub 0.75}Si{sub 0.25} alloy

The magnetic state of the FeMnP{sub 0.75}Si{sub 0.25} alloy was investigated by first principles calculations. The coexistence of ferromagnetic and antiferromagnetic phases in FeMnP{sub 0.75}Si{sub 0.25} with the same hexagonal crystal structure was revealed. It was found that kinetic arrest during the transition from the high temperature disordered paramagnetic phase to the low temperature ordered ferromagnetic phase results in the intermediate metastable and partially disordered antiferromagnetic phase. We propose that the ratio of the ferromagnetic and antiferromagnetic phases in the FeMnP{sub 0.75}Si{sub 0.25} sample can be tuned by adjusting the kinetic process of atomic diffusion. The investigations suggest that careful control of the kinetic diffusion process provides another tuning parameter to design candidate magnetocaloric materials.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗