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Development of safety requirements for HTGRs design - 18467

The safety requirements for the design of High Temperature Gas-cooled Reactors (HTGRs), which is analogous to the IAEA specific safety requirements (SSR) for Light Water Reactor (LWR) design (IAEA SSR-2/1), has been developed by the research committee established in the Atomic Energy Society of Japan so as to incorporate the HTGR safety features demonstrated by High Temperature Engineering Test Reactor (HTTR), lessons learned from the accident of Fukushima Daiichi Nuclear Power Station and requirements for the coupling of the hydrogen production plants with nuclear plant. The safety design approach was determined to establish a high level of safety design standards by utilizing inherent safety features of HTGRs. The safety requirements is then developed using the objectives provisions tree methodology based on the safety design approach. The requirements for a structural integrity of fuel during accident conditions, for a confinement structure instead of a leak-tight pressure resistance containment vessel, for a passive residual heat removal from outside of reactor pressure vessel, etc., which are significantly different from those of LWR, are stated in the developed safety requirements. This paper describes overview of the proposed HTGR specific safety requirements. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Passive techniques for long-term reactor cooling

In a pressurized water reactor (PWR), emergency core cooling (ECC) responds to depressurization due to a vessel penetration break at the top of the pressure vessel by draining water from a body of water through an injection line into the pressure vessel. A barrier operates concurrently with the ECC to suppress flow of liquid water from the pressure vessel out the vessel penetration break. The barrier may comprise one or more of: (1) an injection line extension passing through the central riser to drain water into the central riser; (2) openings in a lower portion of a central riser to shunt some upward flow from the central riser into a lower portion of the downcomer annulus; and (3) a surge line providing fluid communication between a pressurizer volume at the top of the pressure vessel and the remainder of the pressure vessel which directs water outboard toward the downcomer annulus.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Passive techniques for long-term reactor cooling

In a pressurized water reactor (PWR), emergency core cooling (ECC) responds to depressurization due to a vessel penetration break at the top of the pressure vessel by draining water from a body of water through an injection line into the pressure vessel. A barrier operates concurrently with the ECC to suppress flow of liquid water from the pressure vessel out the vessel penetration break. The barrier may comprise one or more of: (1) an injection line extension passing through the central riser to drain water into the central riser; (2) openings in a lower portion of a central riser to shunt some upward flow from the central riser into a lower portion of the downcomer annulus; and (3) a surge line providing fluid communication between a pressurizer volume at the top of the pressure vessel and the remainder of the pressure vessel which directs water outboard toward the downcomer annulus.

Malloy, III, John D.↗

Mass separation of deuterium and helium with conventional quadrupole mass spectrometer by using varied ionization energy

Deuterium pressure in deuterium-helium mixture gas is successfully measured by a common quadrupole mass spectrometer (model: RGA200) with a resolution of ∼0.5 atomic mass unit (AMU), by using varied ionization energy together with new developed software and dedicated calibration for RGA200. The new software is developed by using MATLAB with the new functions: electron energy (EE) scanning, deuterium partial pressure measurement, and automatic data saving. RGA200 with new software is calibrated in pure deuterium and pure helium 1.0 × 10{sup −6}–5.0 × 10{sup −2} Pa, and the relation between pressure and ion current of AMU4 under EE = 25 eV and EE = 70 eV is obtained. From the calibration result and RGA200 scanning with varied ionization energy in deuterium and helium mixture gas, both deuterium partial pressures (P{sub D{sub 2}}) and helium partial pressure (P{sub He}) could be obtained. The result shows that deuterium partial pressure could be measured if P{sub D{sub 2}} > 10{sup −6} Pa (limited by ultimate pressure of calibration vessel), and helium pressure could be measured only if P{sub He}/P{sub D{sub 2}} > 0.45, and the measurement error is evaluated as 15%. This method is successfully employed in EAST 2015 summer campaign to monitor deuterium outgassing/desorption during helium discharge cleaning.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Ductile fracture of cylindrical vessels containing a large flaw

The fracture process in pressurized cylindrical vessels containing a relatively large flaw is considered. The flaw is assumed to be a part-through or through meridional crack. The flaw geometry, the yield behavior of the material, and the internal pressure are assumed to be such that in the neighborhood of the flaw the cylinder wall undergoes large-scale plastic deformations. Thus, the problem falls outside the range of applicability of conventional brittle fracture theories. To study the problem, plasticity considerations are introduced into the shell theory through the assumptions of fully-yielded net ligaments using a plastic strip model. Then a ductile fracture criterion is developed which is based on the concept of net ligament plastic instability. A limited verification is attempted by comparing the theoretical predictions with some existing experimental results.

Erdogan, F.↗

A high-pressure flow through test vessel for neutron imaging and neutron diffraction-based strain measurement of geological materials

Neutron scattering and neutron imaging have emerged as powerful methods for experimentally investigating material deformation and fluid flow in the interior of otherwise inaccessible or opaque structures. This paper describes the design and provides example uses of a pressure cell developed for investigating such behaviors within geological materials. The cell can accommodate cylindrical samples with diameters up to 38.1 mm and lengths up to 154 mm. Additionally, ports in the cell and a pressure isolating sleeve around the sample allow the independent application of confining pressure up to 69 MPa and axial pressure up to 34.5 MPa. Furthermore, two material versions of the cell have been manufactured and used to date. An aluminum version is typically used for temperatures below 40 °C, because of its relative transparency to neutrons, while a titanium version, which is comparatively more neutron attenuating, is used for experiments requiring triaxial pressurization under conditions up to 350 °C. The pressure cells were commissioned at the VULCAN engineering diffractometer at the Oak Ridge National Laboratory (ORNL), Spallation Neutron Source, and have since been used at the ORNL high flux isotope reactor CG1-D imaging beamline, National Institute of Standard and Technology (NIST) BT-2, and NIST NG6 imaging beamlines.

47 OTHER INSTRUMENTATION↗

First lithium experiments in HIDRA and evidence of helium retention during quasi-steady-state stellarator plasma operations

Recent experiments in Hybrid Illinois Device for Research and Applications (HIDRA) have had operational discharges between t discharge = 60 and 1000 s using electron cyclotron resonant heating (ECRH) of the plasma. This means that quasi-steady-state plasma discharges reach conditions to study long-pulse plasma material interactions (PMIs). The newly commissioned HIDRA-Material Analysis Test-stand PMI diagnostic is used to place a drop of lithium onto a heated tungsten surface, transfer the sample in-vacuo and expose it in a helium plasma. Helium is of interest as there is an open question to whether lithium will be able to remove helium ash in real fusion devices. The introduction of the W-Li sample in HIDRA resulted in evaporation of lithium into the helium plasma during a 600 s pulse and caused a reduction of over 90% in neutral pressure during the discharge. It was also observed that the plasma density and temperature increased by over 2.5 times. Using spectroscopy and a helium collisional radiative model, the peak temperature and density of the helium plasma can be monitored during the discharge. During lithium evaporation, as significant lithium ionization occurs, there is a 85% drop in the HIDRA vessel neutral pressure, despite a constant flow rate of He gas. This reduction in neutral pressure is supported by spectroscopy data with corresponding reductions in He I line intensities (587 nm, 667 nm, 706 nm, and 728 nm), as well as those of other impurities. At one point in the discharge a lithium plasma is created, as indicated by an increase in Li + emission and a complete reduction in He + emission, but the electron density jumps from ne = 3 × 10 18 m –3 to over ne = 8 × 10 18 m –3 while the core temperature stays relatively constant between Te = 16 eV and 20 eV. Once lithium has completely evaporated from the sample and the majority of the ionized lithium has diffused from the plasma to the vessel walls, pressure and spectroscopy data paired with He collisional radiative model calculations shows a re-establishment of a helium plasma in a low recycling regime. In this regime, the density drops down to ne = 2 × 10 18 m –3 and the electron temperature increases from T e = 20 eV to over T e = 50 eV indicating an increase in helium heating efficiency. This is also indicated by the He+ emission re-establishing and having a higher intensity. Here, we show the results from the first lithium campaign in HIDRA. In the presence of lithium, and in particular when lithium ions are present, the helium disappears from the plasma via an as of yet unknown complex relationship that needs to be further studied. The most likely explanation is that the lithium ions are distributed around the vessel and able to trap helium to the surface turning HIDRA into a large gettering surface. These results have potential implications on future plasma facing component design using liquid lithium for impurity and recycling control using limiters and divertors.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Supercritical cryo-compressed hydrogen storage for fuel cell electric buses

Liquid hydrogen (LH 2 ) truck delivery and storage at dispensing sites is likely to play an important role in an emerging H 2 infrastructure. Here, we analyzed the performance of single phase, supercritical, on-board cryo-compressed hydrogen storage (CcH 2 ) with commercially-available LH 2 pump enabled single-flow refueling for application to fuel cell electric buses (FCEB). We conducted finite-element stress analyses of Type 3 CcH 2 tanks using ABAQUS for carbon fiber requirement and Fe-Safe for fatigue life. The results from these analyses indicate that, from the standpoint of weight, volume and cost, 2-mm 316 stainless steel liner is preferred to aluminium 6061 alloy in meeting the required 15,000 charge-discharge cycles for 350–700 bar storage pressures. Compared to the Type 3, 350 bar, ambient-temperature H 2 storage systems in current demonstration FCEBs, 500-bar CcH 2 storage system is projected to achieve 91% improvement in gravimetric capacity, 175% improvement in volumetric capacity, 46% reduction in carbon fiber composite mass, and 21% lower system cost, while exceeding >7 day loss-free dormancy with initially 85%-full H 2 tank.

08 HYDROGEN↗

Effects of high-pressure hydrogen on storage vessel materials

Tensile tests on welded plates of three grades of steel indicate an appreciable decrease of tensile strength and ductility of notched specimens and a decrease in ductility of unnotched samples. Surface cracking, evident in unnotched specimens, is conducive to breakdown in tensile strength and ductility.

Chandler, W. T.↗

Evaluating methods to reduce duration of near-threshold fatigue crack growth rate measurements for low-alloy steels in hydrogen gas

Measurement of the near-threshold fatigue crack growth rate (da/dN) vs. stress-intensity factor range (∆K) relationship in hydrogen gas is essential for maximizing the calculated design fatigue life of high-pressure hydrogen storage vessels. However, such measurements are rarely performed, since the low cyclic loading frequencies applied in standard practice lead to prohibitively protracted test durations. The objective of this study was to demonstrate two means for reducing test durations when measuring near-threshold da/dN vs. ΔK relationships under decreasing ΔK for low-alloy pressure vessel steels in hydrogen gas: 1) imposing steeper K-gradients relative to the recommended limits in standards such as ASTM E647, and 2) increasing cyclic loading frequency relative to typical values applied during fatigue crack growth testing of low-alloy steels in hydrogen gas. Recognizing that steeper K-gradients could amplify loading-history effects, test methods employing this approach were designed to mitigate such effects by either maintaining constant K max or gradually increasing the K-gradient as the threshold was approached. Although the varying K-gradient method was vulnerable to loading-history effects in the form of plasticity-induced crack closure, particularly at lower stress ratio (R) and higher starting K max values, these effects could be compensated by applying the adjusted compliance ratio (ACR) method. Here, it was demonstrated that steeper K-gradients in concert with increased cyclic loading frequency reduced the duration of near-threshold fatigue crack growth tests in hydrogen gas by more than 99% relative to standard practices.

Fatigue threshold↗

Initial development of a high temperature life prediction method directly accounting for variability in material properties

This report presents the initial development of a life prediction method that accounts for the variability of the material properties in Grade 91 steel. We account for material variability by both fitting a variable 3-parameter Weibull distribution to the rupture data of the material and by quantifying the effect that the creep deformation properties have on stresses via a Monte Carlo approach. To ensure a reasonable time frame when applying Monte Carlo to the creep stress, we propose a methodology that models the material as an extremely viscous Stokes flow with a non-Newtonian viscosity, therefore solving the problem in a single step. We use the final probabilistic model for structural failure developed in this document to evaluate a Flat Head Vessel designed with the Section III, Division 5 ASME Boiler Pressure and Vessel Code rules with a 100,000h design life and assess its probability of premature failure.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Analysis of N-16 concentration in primary cooling system of AP1000 power reactor

Nitrogen-16 (N-16) is one of the radiation safety parameter on the primary reactor system. The activation product, N-16, is the predominant contributor to the activity in the reactor coolant system during reactor operation. N-16 is activation product derived from activation of O-16 with fast neutron based on {sup 16}O(n,p){sup 16}N reaction. Thus study is needed and it performs to determine N-16 concentration in reactor coolant (primary coolant) in supporting radiation safety. One of the way is using analytical methode based on activation and redecay princip to obtain N-16 concentration. The analysis was performed on the configuration basis and operational of Westinghouse AP1000 power reactor in several monitoring points at coolant reactor system. The results of the calculation of N-16 concentration at the core outlet, reactor vessel outlet, pressurizer line, inlet and outlet of steam generators, primary pumps, reactor vessels inlet and core inlet are: 281, 257, 255, 250, 145, 142, 129 and 112 µCi/gram respectively. The results of analysis compared with AP1000 design control document as standard values. The verification showed very high accuracy comparation between analytical results and standard values.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

HSLA-100 Forging Contract Vendor Post-Award Meeting [Slides]

LANL utilizes thick-walled, spherical vessels for numerous basic science, materials, and system performance experiments. These pressure retaining vessels are designed and fabricated to meet the intent of ASM E B&PV Section VIII, Division 3 and Code Case 2564. LANL has successfully contracted past production of component parts (nozzle and cover forgings, plate production and head forming) and overall vessel construction (welding, inspection, hydrostatic testing) utilizing HSLA-100 steel. As current vessel inventories approach design lifetimes, we are once again embarking upon a series of fabrication contracts to produce replacement components and vessel assemblies to ensure continued experiment cadence at LANL. We anticipate releasing additional future vessel production contracts as experimental demands at LANL continue to increase

36 MATERIALS SCIENCE↗

Electrochemical compressor refrigeration appartus with integral leak detection system

An electrochemical compressor system, such as an electrochemical refrigeration system includes a sealed vessel that reduces leak issues related to the electrochemical cell. The sealed vessel may be molded or formed from a polymer or a composite polymer having reinforcing materials, such as fibers therein. The sealed vessel may be plated with metal to reduce gas permeation through the wall of the vessel and to accommodate and improve the attachment of conduits, including metal conduits thereto. A metal conduit may be brazed onto a vessel and the brazing material may be selected for polymer to metal joining and for reduced contamination potential of the system. The electrochemical compressor system incorporates a leak sensor configured at least partially within the sealed rigid vessel that measures the pressure within the vessel.

Bahar, Bamdad↗

Development of thermal transit flow measurement for small modular reactors - 140

Safe, reliable, and efficient operation of nuclear reactors requires timely and accurate measurement of primary coolant parameters such as temperature, flow, pressure, and level. These measurements may be challenging in small modular reactors (SMRs) with integral vessel design. For SMRs with the integral design, sensors may be located in confined spaces or embedded within pressure vessels. The absence of primary coolant loops is another fundamental design attribute that will affect the location of sensors, sensor interfaces, and types of sensors suited for process parameter measurements. Further, the number and location of pressure vessel penetrations may be constrained compared to traditional nuclear power plants (NPPs). As a result, conventional NPP temperature, flow, pressure, and level sensors may not be appropriate for use in SMRs. This paper addresses the development of new sensor technology for hybrid temperature, flow, and level measurement. The authors demonstrate the alternative use of resistance temperature detectors (RTDs) where cross-correlation of process temperature variations between RTDs is used to calculate process flow velocity. The new sensor and measurement technology will also incorporate RTD response time and self-heating characteristics to provide flow and level measurement in accident conditions. This capability would simplify reactor design and enable optimal placement of reactor pressure vessel penetrations leading to increased operational reliability and safety. The cross-correlation of temperature signals and adaptation for flow measurement in a laboratory setting is presented here. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Biphasic production of 2,4,6-triamino-1,3,5-trinitrobenzene (TATB)

Production of 2,4,6-triamino-1,3,5-trinitrobenzene (TATB) through a safer, less harmful process while yielding a superior product is disclosed. The biphasic production process may include mixing a solution of 1,3,5-trichloro-2,4,6-trinitrobenzene (TCTNB) and a surfactant into a solvent in a sealed, heated vessel such that TATB is formed in a mixture. The biphasic production process may also include pressurizing the vessel with gaseous ammonia such that aqueous TATB is formed and separating the TATB from the mixture.

Leonard, Philip↗