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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 1,747 records · Page 97
All sourcesNASA NTRSDOE OSTI
NASA NTRS1987

Atmospheric correction of NS-001 data and extraction of multiple angle reflectance data sets

The percentage of incident solar flux reflected by a surface is a quantity of considerable interest in remote sensing studies. To calculate reflectance from remotely sensed radiance data some estimate of incident flux is needed. Since simultaneous ground-based radiometric measurements are often not available for observations by aircraft or satellite sensors, a procedure based on modeling atmospheric transmittance and scattering was developed. The primary application is to an aircraft data set collected with the NASA C-130 over the Superior National Forest, Minnesota. Atmospherically corrected multiple angle reflectance data sets and reflectance images are generated for areas of natural forest vegetation. These data and the technique may be useful for studies of the interactions of light with forested canopies.

Strebel, D. E.↗
NASA NTRS1982

Radar backscattering from a rough rotating triaxial ellipsoid with applications to the geodesy of small asteroids

Radar geodesy of the asteroid 433 Eros was reported by Jurgens and Goldstein (1976). Their measurements were based on the spectral properties of a rough rotating triaxial ellipsoid. This paper presents the theory by which theoretical spectra based on a backscattering model of the form of the nth power of the cosine of theta, or any reasonable backscattering model, can be computed. Some general properties of these spectra are demonstrated, and simple measurements of the apparent radar cross section, center frequency, and effective bandwidth as a function of time are shown to be useful in determining the sizes of the semi-major axes, the exponent n in the scattering model, the backscatter efficiency of the surface material, the rotation period, and the declination of the observer above or below the rotation equator. Some of these parameters are correlated, and multiple estimation may be difficult unless the observations span a period sufficiently long so as to present a wide range of declinations of the observer. However, the departure from a spherical shape aids in separating the scattering properties from the target dimensions and facilitates the simultaneous estimation of all free parameters.

Jurgens, R. F.↗
NASA NTRS1995

Program Classifies Multiple-Frequency Polarimetric SAR Data

POLMAP computer program classifies multifrequency, polarimetric synthetic-aperture-radar (SAR) data into homogeneous classes of radar back-scatter. Software implements maximum-a-posteriori classification scheme. Performs by use of simulated-annealing procedure, takes much longer to compute than ICM solution, but it maximizes posteriori distribution of classes for whole scene. Input statistics of image classes must be created by some independent means, and supplied as input to POLMAP. Used as input to image processing application program. Written in FORTRAN 77.

Rignot, Eric↗
DOE OSTI2023

5ω Optical Thomson Scattering Report

The 5ω Optical Thomson Scattering system on the National Ignition Facility (NIF) is a diagnostic designed to measure temporally and spatially resolved plasma conditions in Inertial Confinement Fusion (ICF) Hohlraums. The system was proposed in 2014 and a phased approach to implementation was developed. In phase one the collection system was designed, built, and fielded on the NIF to be used for 3ω Thomson scattering measurements and background measurements near 211 nm (5ω. The initial commissioning experiment for the collection system was completed in Oct. 2016. Commissioning of the collection system continued through 2017 and the system is now fielded for a range of user experiments and regularly produces publication quality data. A dedicated 5ω probe laser was designed and built to allow Thomson scattering measurements in the presence of 2 MJ of 3ω drive energy. Due to scattered light (spectral reflections, laser-plasma instabilities, and unconverted drive energy) from the 3w drive lasers typical wavelengths (2ω and 4ω) fielded at other laser facilities like the Nova Laser Facility and the Omega Laser Facility were unable to meeting the signal to background requirements in design studies. A 10 Joule 5ω probe was proposed as a solution that met requirements. This 10 Joule laser was more energetic than previously fielded 5w lasers by 2-3 orders of magnitude. As part of a risk reduction plan, phase two of the project was to develop a 1 Joule, 5ω laser to demonstrate conversion efficiency >20% from 1ω to 5ω and make initial Thomson scattering measurements in the first few nanoseconds of an ICF laser pulse. Initial tests of the 5w conversion were completed at the Laboratory for Laser Energetics (LLE) and produced record 5ω energies. Based on these results from LLE, a 1 Joule, 5w laser system was designed for the NIF in 2018 and commissioning began in 2019. Commissioning of the 5ω laser system continued through 2023 and was eventually paused in Q1 of FY24 due to completing resource constraints. Commissioning of the 5w laser system proved incredibly challenging. Multiple issues were identified during commissioning and resolved, but issues remain. Currently there is not a clear understanding of why 5ω scattered has not been detected on the OTS collection system. Based on offline measurements, calculations, and preshot measurements the system appears to meet all requirements. Potential target physics issues have been investigated and do not appear to be an issue. The current hypothesis is that there is an error in one or more aspects of the offline testing not translating to expected performance when the system is fielded on the NIF. Additional full system testing in-situ utilizing the complete OTS system and NIF target chamber center time is needed to further test potential failure modes.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2024

Advanced Characterization of Solid-State Battery Materials Using Neutron Scattering Techniques

Advanced batteries require advanced characterization techniques, and neutron scattering is one of the most powerful experimental methods available for studying next-generation battery materials. Neutron scattering offers a non-destructive method to probe the complex structural and chemical processes occurring in batteries during operation in truly in situ/in operando measurements with a high sensitivity to battery-relevant elements such as lithium. Neutrons have energies comparable to the energies of excitations in materials and wavelengths comparable to atomic distances in the solid state, thus giving access to study structural and dynamical properties of materials on an atomic scale. In this review, a broad overview of selected neutron scattering techniques is presented to illustrate how neutron scattering can be used to gain invaluable information of solid-state battery materials, with a focus on in situ/in operando methods. These techniques span multiple decades of length and time scales to uncover the complex processes taking place fundamentally on the atomic scale and to determine how these processes impact the macroscale properties and performance of functional battery systems. This review serves the solid-state battery research community by examining how the unique capabilities of neutron scattering can be applied to answer critical and unresolved questions of materials research in this field. A thorough and broad perspective is provided with numerous practical examples showing these techniques in action for battery research.

25 ENERGY STORAGE↗
DOE OSTI2017

Robust X-ray angular correlations for the study of meso-structures

As self-assembling nanomaterials become more sophisticated, it is becoming increasingly important to measure the structural order of finite-sized assemblies of nano-objects. These mesoscale clusters represent an acute challenge to conventional structural probes, owing to the range of implicated size scales (10 nm to several micrometres), the weak scattering signal and the dynamic nature of meso-clusters in native solution environments. The high X-ray flux and coherence of modern synchrotrons present an opportunity to extract structural information from these challenging systems, but conventional ensemble X-ray scattering averages out crucial information about local particle configurations. Conversely, a single meso-cluster scatters too weakly to recover the full diffraction pattern. Using X-ray angular cross-correlation analysis, it is possible to combine multiple noisy measurements to obtain robust structural information. This paper explores the key theoretical limits and experimental challenges that constrain the application of these methods to probing structural order in real nanomaterials. A metric is presented to quantify the signal-to-noise ratio of angular correlations, and it is used to identify several experimental artifacts that arise. In particular, it is found that background scattering, data masking and inter-cluster interference profoundly affect the quality of correlation analyses. A robust workflow is demonstrated for mitigating these effects and extracting reliable angular correlations from realistic experimental data.

77 NANOSCIENCE AND NANOTECHNOLOGY↗
DOE OSTI2021

High Thermoelectric Performance through Crystal Symmetry Enhancement in Triply Doped Diamondoid Compound Cu 2 SnSe 3

The presence of high crystallographic symmetry and nanoscale defects are favorable for thermoelectrics. With proper electronic structures, a highly symmetric crystal tends to possess multiple carrier channels and promote electrical conductivity without sacrificing Seebeck coefficient. In addition, nanoscale defects can effectively scatter acoustic phonons to suppress thermal conductivity. Here, we report that the triple doping of Cu 2 SnSe 3 leads to a high ZT value of 1.6 at 823 K for Cu 1.85 Ag 0.15 (Sn 0.88 Ga 0.1 Na 0.02 )Se 3 , and a decent average ZT (ZT ave ) value of 0.7 is also achieved for Cu 1.85 Ag 0.15 (Sn 0.93 Mg 0.06 Na 0.01 )Se 3 from 475 to 823 K. Our study reveals: (1) Ag doping on Cu sites generates numerous point defects and greatly decreases lattice thermal conductivity. (2) Doping Mg or Ga converts the monoclinic Cu 2 SnSe 3 into a cubic structure. This symmetry enhancing leads to increase in the effective mass from 0.8 m e to 2.6 m e (m e , free electron mass) and the power factor from 4.3 μW/cm –1 K –2 for Cu 2 SnSe 3 to 11.6 μW/cm –1 K –2 . (3) Na doping creates dense dislocation arrays and nanoprecipitates, which strengthens the phonon scattering. (4) Pair distribution function analysis shows localized symmetry breakdwon in the cubic Cu 1.85 Ag 0.15 (Sn 0.88 Ga 0.1 Na 0.02 )Se 3 . Furthermore, the present work provides a standpoint to design promising thermoelectric materials by synergistically manipulating crystal symmetry and nanoscale defects.

36 MATERIALS SCIENCE↗
DOE OSTI2017

Broadband surface-enhanced coherent anti-Stokes Raman spectroscopy with high spectral resolution

Both the surface-enhanced Raman spectroscopy (SERS) and coherent anti-Stokes Raman spectroscopy (CARS) are widely used methods in the bio-sensing field for improving the intensity of Raman scattering process. By combining the mechanisms of CARS (coherence and nonlinear process) and SERS (plasmon resonance), a multiplicative enhancement can be achieved through surface-enhanced CARS (SECARS). Besides sensitivity, high specificity with wide spectral bandwidth is also preferred for bio-sensing techniques but not well developed in SECARS setups reported in the literature. A broadband SECARS setup with high sensitivity and high spectral resolution is presented. Rhodamine 6G dye molecules and several biomolecules are used as the model system to benchmark the functionality of the SECARS system in terms of its sensitivity, the lowest detectable concentration, and the spectral resolution. Our setup rendered single-molecule sensitivity with spectral resolution of <35 cm -1 . More than 10 2 times stronger signal-to-noise ratio compared with that of SERS is observed with the detection limit being 10 -9 m. Different from the SECARS systems in the literature, our setup employs a unique graphene-Au pyramids hybrid platform. The graphene in this structure provides additional SERS enhancement and a bio-compatible surface. Finally, this powerful technique could be instrumental in furthering the understanding of various chemical and biological processes.

42 ENGINEERING↗
DOE OSTI2014

CHANDRA DETECTION OF A NEW DIFFUSE X-RAY COMPONENT FROM THE GLOBULAR CLUSTER 47 TUCANAE

In re-analyzing the archival Chandra data of the globular cluster 47 Tucanae, we have detected a new diffuse X-ray emission feature within the half-mass radius of the cluster. The spectrum of the diffuse emission can be described by a power-law model plus a plasma component with photon index Γ ∼ 1.0 and plasma temperature kT ∼ 0.2 keV. While the thermal component is apparently uniform, the non-thermal contribution falls off exponentially from the core. The observed properties could possibly be explained in the context of multiple shocks resulting from the collisions among the stellar wind in the cluster and the inverse Compton scattering between the pulsar wind and the relic photons.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2025

Unraveling the Origin of Glassy Thermal Transport in Medium-Entropy Semiconductors: From Nanoscale Phase Segregation to Atomic-Scale Lattice Distortion

Thermoelectric (TE) materials can directly and reversibly convert heat into electricity, offering a promising pathway for reshaping the global energy landscape. The performance of thermoelectric materials is evaluated using the figure of merit, zT = S 2 σT/κ, which can be optimized by improving Seebeck coefficient (S) and electrical conductivity (σ) while suppressing the thermal conductivity (κ) at the operating temperature (T). Here, we introduce a medium-entropy metal chalcogenide that exhibits phonon-glass electron-crystal behavior. The conventional perspective hypothesizes that the suppression of thermal transport arises solely from disordered atomic occupation, which enhances alloy scattering mechanisms for phonon transport. However, emerging evidence suggests the presence of structural and chemical inhomogeneity at multiple length scales in entropy-engineered materials, a phenomenon that has rarely been investigated in detail.

Liu, Yukun [Northwestern Univ]↗
DOE OSTI2022

Feature Extraction for Pipeline Defects Inspection Based Upon Distributed Acoustic Fiber Optic Sensing Data

Fiber-optic distributed acoustic sensing (DAS) is becoming an increasingly important tool for real-time monitoring of energy and civil infrastructure structural health such as pipelines. We present a systematic theoretical study of the potential for DAS to be directly coupled with guided ultrasonic waves typically used in conventional acoustic non-destructive evaluation (NDE) methods for real-time pipeline health monitoring. We are referring to this innovative new NDE technique as ultrasonic guided wave and optical fiber sensor fusion. In the practical application of DAS coupled with guided ultrasonic waves, the structural design of (1) the specific guided waves excited, (2) the physical installation of the acoustic transducers and the fiber optic sensors, and (3) the functional performance specifications (gauge length, sensitivity, Etc.) of fiber optic DAS have an important influence on overall capabilities of the monitoring system. Meanwhile, physics-based analysis of acoustic waves is still a challenge due to the complex nature of the Lamb wave when it propagates, scatters, and disperses in the presence of structural defects. In this work, we simulate carbon steel pipes relevant for oil and gas pipeline applications with diameters of approximately 6-12” and wall thickness of 0.5” as the objects to be monitored. By establishing and implementing these capabilities, we seek to pursue an in-depth study on structural parameter optimization of DAS network, measurement range, and signal processing with an ultimate goal of increasing the sensitivity and efficacy of DAS to defect identification for various modes of corrosion expected in practice. To study the characteristics of scattered acoustic waves and performance of DAS for defect identification, we simulated the response of DAS for multiple pipe structures, defect types, and DAS sensor network configuration using finite element software Ansys, then the properties of signal response are extracted to construct defect-sensitive features. The raw data simulated, and the associated features extracted can ultimately be utilized as annotated training data to benchmark various designs for DAS applications, guided acoustic excitation sources, and learning model parameters to enhance early detection of potentially problematic defects.

Pipeline Defects Inspection, Fiber-optic sensors, ↗
DOE OSTI2016

Azimuthal distributions in unpolarized SIDIS

We present studies of multiplicities and the cosf, and cos2f moments, in charged pion production in semi-inclusive deep inelastic scattering (SIDIS). The data set used was the E1-f run from the CEBAF Large Acceptance Spectrometer (CLAS) at Jefferson Lab which ran in 2003. The run used a 5.498 GeV longitudinally polarized electron beam and an unpolarized liquid hydrogen target. Two pion channels (\pi+ and \pi-) were studied over a broad kinematical range (x = 0.1-0.6, Q2 = 1.0-4.5 GeV2, z = 0.0-1.0, PT^2 = 0.0-1.0 GeV^2, and -180 < \phi_h < 180). These measurements give insights into the transverse momentum dependence of parton distribution functions (PDFs) describing the dynamics of quarks and gluons inside of the proton.

Avakian, Harut↗
DOE OSTI2016

Si K EDGE STRUCTURE AND VARIABILITY IN GALACTIC X-RAY BINARIES

We survey the Si K edge structure in various absorbed Galactic low-mass X-ray binaries (LMXBs) to study states of silicon in the inter- and circum-stellar medium. The bulk of these LMXBs lie toward the Galactic bulge region and all have column densities above 10{sup 22} cm{sup −2}. The observations were performed using the Chandra High Energy Transmission Grating Spectrometer. The Si K edge in all sources appears at an energy value of 1844 ± 0.001 eV. The edge exhibits significant substructure that can be described by a near edge absorption feature at 1849 ± 0.002 eV and a far edge absorption feature at 1865 ± 0.002 eV. Both of these absorption features appear variable with equivalent widths up to several mÅ. We can describe the edge structure using several components: multiple edge functions, near edge absorption excesses from silicates in dust form, signatures from X-ray scattering optical depths, and a variable warm absorber from ionized atomic silicon. The measured optical depths of the edges indicate much higher values than expected from atomic silicon cross sections and interstellar medium abundances, and they appear consistent with predictions from silicate X-ray absorption and scattering. A comparison with models also indicates a preference for larger dust grain sizes. In many cases, we identify Si xiii resonance absorption and determine ionization parameters between log ξ = 1.8 and 2.8 and turbulent velocities between 300 and 1000 km s{sup −1}. This places the warm absorber in close vicinity of the X-ray binaries. In some data, we observe a weak edge at 1.840 keV, potentially from a lesser contribution of neutral atomic silicon.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2018

Formation and evolution of Tar Balls from Northwestern US wildfires

Biomass burning is a major source of light-absorbing black and brown carbonaceous particles. Brown carbon is a poorly characterized mixture that includes tar balls (TBs), a type of carbonaceous particle apparently unique to biomass burning. Here we describe the first atmospheric observations of the formation and evolution of TBs from forest fires. Aerosol particles were collected on TEM grids during aircraft transects at various downwind distances from the Colockum Tarp wildland fire. TB mass fractions, derived from TEM and in-situ measurements, increased from < 1 % near the fire to 31–45 % downwind, with little change in TB diameter. Single-scattering albedo determined from scattering and absorption measurements increased slightly with downwind distance. Similar TEM and SSA results were observed sampling multiple wildfires. Mie calculations are consistent with weak light absorbance by TBs (m = 1.56–0.02i) but not consistent with order-of-magnitude stronger absorption observed in different settings. The field-derived TB mass fractions reported here indicate that this particle type should be accounted for in biomass-burn emission inventories.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1991

Scattering-induced optical polarization in thick accretion disks

A general formalism for calculating the linear polarization induced by scattering within the central funnel of a thick accretion disk is presented, and it is shown that multiple photon reflections off the funnel walls can produce polarization values of up to about 10 percent, with the polarization position angle aligned parallel to the disk symmetry axis. It is suggested that this process is responsible for the observed optical polarization levels in X-ray-selected BL Lac objects (XBLs), which generally show linear polarization percentages P less than about 10 percent. According to this interpretation, XBLs with high optical polarization are viewed at an angle of less than about 60 deg to the funnel axis and their projected polarization vectors should be preferentially aligned with the associated radio jets. The possible relevance of this model to Seyfer 1 galaxies and quasars is also discussed.

Kartje, John F.↗
NASA NTRS1992

Non-linear effects of QED multiple-photon processes on cyclotron spectra

The relativistic magnetic resonant multiple-photon processes are discussed up to order alpha(f)exp 2, in particular two-photon scattering and two-photon emission. The latter also contributes to the opacity and photon production, although more weakly than the scattering. These processes are nonlinear in the radiation field, and therefore the transfer depends sensitively on the cross sections. We show model spectra including three cyclotron harmonics for the accreting pulsar Her X-1 and the gamma-ray burster GB880205. The lines are highly polarized, and their depth is sensitive to the polarization treatment.

Meszaros, P.↗
NASA NTRS2000

Rayleigh Scattering Diagnostic for Simultaneous Measurements of Dynamic Density and Velocity

A flow diagnostic technique based on the molecular Rayleigh scattering of laser light is used to obtain dynamic density and velocity data in turbulent flows. The technique is based on analyzing the Rayleigh scattered light with a Fabry-Perot interferometer and recording information about the interference pattern with a multiple anode photomultiplier tube (PMT). An artificial neural network is used to process the signals from the PMT to recover the velocity time history, which is then used to calculate the velocity power spectrum. The technique is illustrated using simulated data. The results of an experiment to measure the velocity power spectrum in a low speed (100 rn/sec) flow are also presented.

Seasholtz, Richard G.↗