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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

Performance of a phonon-mediated kinetic inductance detector at the NEXUS cryogenic facility

Microcalorimeters that leverage microwave kinetic inductance detectors to read out phonon signals in the particle-absorbing target, referred to as kinetic inductance phonon-mediated (KIPM) detectors, offer an attractive detector architecture to probe dark matter (DM) down to the fermionic thermal relic mass limit. A prototype KIPM detector featuring a single aluminum resonator patterned onto a 1-gram silicon substrate was operated in the Northwestern EXerimental Underground Site (NEXUS) low-background facility at Fermilab for characterization and evaluation of this detector architecture’s efficacy for a DM search. An energy calibration was performed by exposing the bare substrate to a pulsed source of 470-nm photons, resulting in a baseline resolution on the energy absorbed by the phonon sensor of 2.1 ± 0.2 eV, a factor of two better than the current state of the art, enabled by quasiparticle lifetimes extending up to 6.5 ms. However, due to the subpercent phonon collection efficiency, the resolution on energy deposited in the substrate is limited to σ E = 318 ± 29 eV. We further model both the signal pulse shape as a function of device temperature to extract quasiparticle lifetimes, and the observed noise spectra.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2017

Antineutrino Monitoring of Spent Nuclear Fuel

Military and civilian applications of nuclear energy have left a significant amount of spent nuclear fuel over the past 70 years. Currently, in many countries worldwide, the use of nuclear energy is on the rise. Therefore, the management of highly radioactive nuclear waste is a pressing issue. In this work, we explore antineutrino detectors as a tool for monitoring and safeguarding nuclear-waste material. We compute the flux and spectrum of antineutrinos emitted by spent nuclear fuel elements as a function of time, and we illustrate the usefulness of antineutrino detectors in several benchmark scenarios. In particular, we demonstrate how a measurement of the antineutrino flux can help to reverify the contents of a dry storage cask in case the monitoring chain by conventional means gets disrupted. We then comment on the usefulness of antineutrino detectors at long-term storage facilities such as Yucca mountain. Finally, we put forward antineutrino detection as a tool in locating underground “hot spots” in contaminated areas such as the Hanford site in Washington state.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2017

Shock equation of state of LiH 6 to 1.1 TPa

Using laser-generated shock waves, we have measured pressure, density, and temperature of LiH on the principal Hugoniot between 260 and 1100 GPa (2.6–11 Mbar) and on a second-shock Hugoniot up to 1400 GPa to near fivefold compression, extending the maximum pressure reached in non-nuclear experiments by a factor of two. Here, we observe the onset of metal-like reflectivity consistent with temperature-induced ionization of the Li 2s electron, and no sign of additional changes in ionization up to the maximum pressure. Our measurements are in good agreement with gas gun, Z-machine, and underground test data and are accurately described by quantum molecular dynamics simulations. The results confirm the validity of equation of state models built on an average-atom description of the electron-thermal contribution to the free energy and a density-dependent Grüneisen parameter to describe shock response of LiH over this pressure range.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2019

Search for neutrinoless double- β decay in Ge 76 with 26 kg yr of exposure from the Majorana Demonstrator

The MAJORANA Collaboration is operating an array of high purity Ge detectors to search for the neutrinoless double-beta decay of $^{76}$Ge. The MAJORANA DEMONSTRATOR consists of 44.1 kg of Ge detectors (29.7 kg enriched to 88% in $^{76}$Ge) split between two modules constructed from ultra-clean materials. Both modules are contained in a low-background shield at the Sanford Underground Research Facility in Lead, South Dakota. We present updated results on the search for neutrinoless double-beta decay in $^{76}$Ge with $26.0\pm0.5$ kg-yr of enriched exposure. With the DEMONSTRATOR's unprecedented energy resolution of 2.53 keV FWHM at $Q_{\beta\beta}$, we observe one event in the region of interest with 0.65 events expected from the estimated background, resulting in a lower limit on the $^{76}$Ge neutrinoless double-beta decay half-life of $2.7\times10^{25}$ yr (90% CL) with a median sensitivity of $4.8\times10^{25}$ yr (90% CL). Depending on the matrix elements used, a 90% CL upper limit on the effective Majorana neutrino mass in the range of 200-433 meV is obtained. The measured background in the low-background configurations is $11.9\pm2.0$ counts/(FWHM t yr).

59 ≤ A ≤ 89↗
DOE OSTI2021

Projected sensitivity of the LUX-ZEPLIN experiment to the two-neutrino and neutrinoless double $\beta$ decays of $^{134}$Xe

The projected sensitivity of the LUX-ZEPLIN (LZ) experiment to two-neutrino and neutrinoless double beta decay of 134 Xe is presented. LZ is a 10-tonne xenon time projection chamber optimized for the detection of dark matter particles, that is expected to start operating in 2021 at Sanford Underground Research Facility, USA. Its large mass of natural xenon provides an exceptional opportunity to search for the double beta decay of 134 Xe, for which xenon detectors enriched in 136 Xe are less effective. For the two-neutrino decay mode, LZ is predicted to exclude values of the half-life up to 1.7 x 10 24 years at 90% confidence level (CL), and has a three-sigma observation potential of 8.7 x 10 23 years, approaching the predictions of nuclear models. For the neutrinoless decay mode LZ, is projected to exclude values of the half-life up to 7.3 x 10 24 years at 90% CL.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2022

Signatures of muonic activation in the Majorana Demonstrator

Experiments searching for very rare processes such as neutrinoless double-beta decay require a detailed understanding of all sources of background. Signals from radioactive impurities present in construction and detector materials can be suppressed using a number of well-understood techniques. Background from in situ cosmogenic interactions can be reduced by siting an experiment deep underground. However, the next generation of such experiments have unprecedented sensitivity goals of 10 28 years half-life with background rates of 10 -5 cts/(keV kg yr) in the region of interest. To achieve these goals, the remaining cosmogenic background must be well understood. In the work presented here, Majorana Demonstrator data are used to search for decay signatures of metastable germanium isotopes. Contributions to the region of interest in energy and time are estimated using simulations and compared to Demonstrator data. Correlated time-delayed signals are used to identify decay signatures of isotopes produced in the germanium detectors. A good agreement between expected and measured rate is found and different simulation frameworks are used to estimate the uncertainties of the predictions. The simulation campaign is then extended to characterize the background for the LEGEND experiment, a proposed tonne-scale effort searching for neutrinoless double-beta decay in 76 Ge .

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

Constraints on partial half-lives of 136 Ce and 138 Ce double electron captures

The γ-ray emissions from a radiopure cerium-bromide crystal with a mass of 4381 g were measured for a total of 497.4 d by means of high-resolution γ-ray spectrometry in the HADES underground laboratory at a depth of 500 m.w.e. A search for 0/2νϵϵ and 0/2νϵβ + double beta decay transitions of 136 Ce and 13 8Ce was performed using Bayesian analysis techniques. No signals were observed for a total of 35 investigated decay modes. 90% credibility limits were set in the order of 10 18 -10 19 yr. Existing constraints from a cerium oxide powder measurement were tested with a different cerium compound and half-life limits could be improved for most of the decay modes. The most likely accessible decay mode of the 136 Ce 2νϵϵ transition into the $0_{1}^{+}$ state of 136 Ba results in a new best 90% credibility limit of 5.0×10 18 yr.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

Search for neutrinoless β-plus-EC decay of 120 Te with CUORE

The Cryogenic Underground Observatory for Rare Events (CUORE) is a large-scale cryogenic experiment searching for neutrinoless double-beta decay (0νββ) in 130 Te. The CUORE detector is made of natural tellurium, providing the possibility of rare event searches on isotopes other than 130 Te. In this work we describe a search for neutrinoless positron-emitting electron capture (β + EC ) decay in 120 Te with a total TeO 2 exposure of 355.7 kg yr, corresponding to 0.2405 kg yr of 120 Te. Albeit 0νββ with two final-state electrons represents the most promising channel, the emission of a positron and two 511-keV γ 's make 0νβ + EC decay signature extremely clear. To fully exploit the potential offered by the detector modularity we include events with different topology and perform a simultaneous fit of five selected signal signatures. Using blinded data we extract a median exclusion sensitivity of 3.4 × 10 22 yr at 90% credibility interval (C.I.). After unblinding we find no evidence of 0νβ + EC signal and set a 90% C.I. Bayesian lower limit of 2.9 × 10 22 yr on 120 Te half-life. This result improves by an order of magnitude the existing limit from the combined analysis of CUORE-0 and Cuoricino.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗
DOE OSTI2018

First limit on neutrinoless quadruple β decay of Nd 150 to the 0 1 + state of Gd 150

Observation of lepton number violation via detection of neutrinoless double β decay requires that the neutrino be a Majorana particle. If the neutrino is a Dirac particle, a potential lepton-number violating process is neutrinoless quadruple β decay. Only a few nuclei can undergo neutrinoless quadruple β decay; one of these nuclei is 150 Nd. This study yields the first half-life limit of the neutrinoless quadruple β decay to the excited $0$ $^{+}_{1}$ state of 150 Gd. Here, we searched for neutrinoless quadruple β decay events to excited final states of 150 Gd by detecting the deexcitation γ rays of the daughter nucleus in coincidence. These γ rays have energies of 569.031 and 638.050 keV, and are emitted in coincidence through a $0$ $^{+}_{1}$ → $2$ $^{+}_{1}$ → $0$ $^{+}_{gs}$ transition. The enriched Nd 2 O 3 sample consisted of 40.33 ± 0.02 g 150 Nd and was observed for 642.8 days at the Kimballton Underground Research Facility. A half-life limit for the decay to the $0$ $^{+}_{1}$ state of 150 Gd was found to be T 1/2 > 1.76 × 10 20 years (90% CL). We report the first search for this decay to excited final states. Though the predicted half-life of this decay is many orders of magnitudes larger, constraining this value experimentally is vital to check for potential enhancements to the decay rate.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2019

Multisite event discrimination for the majorana demonstrator

The MAJORANA DEMONSTRATOR is searching for neutrinoless double-beta decay($0\nu\beta\beta$) in 76 Ge using arrays of point-contact germanium detectors operating at the Sanford Underground Research Facility. Background results in the $0\nu\beta\beta$ region of interest from data taken during construction, commissioning, and the start of full operations have been recently published. A pulse shape analysis cut applied to achieve this result, named AvsE , is described in this paper. This cut is developed to remove events whose waveforms are typical of multi-site energy deposits while retaining (90 ± 3.5)% of single-site events. This pulse shape discrimination is based on the relationship between the maximum current and energy, and tuned using 228 Th calibration source data. In conclusion, the efficiency uncertainty accounts for variation across detectors, energy, and time, as well as for the position distribution difference between calibration and $0\nu\beta\beta$ events, established using simulations.

59 ≤ A ≤ 89↗
DOE OSTI2019

Dark Matter Search Results from the Complete Exposure of the PICO-60 C$_3$F$_8$ Bubble Chamber

Final results are reported from operation of the PICO-60 C3F8 dark matter detector, a bubble chamber filled with 52 kg of C3F8 located in the SNOLAB underground laboratory. The chamber was operated at thermodynamic thresholds as low as 1.2 keV without loss of stability. A new blind 1404-kg-day exposure at 2.45 keV threshold was acquired with approximately the same expected total background rate as the previous 1167-kg-day exposure at 3.3 keV. This increased exposure is enabled in part by a new optical tracking analysis to better identify events near detector walls, permitting a larger fiducial volume. These results set the most stringent direct-detection constraint to date on the weakly interacting massive particle (WIMP)-proton spin-dependent cross section at 3.2×10-41 cm2 for a 25 GeV WIMP, improving on previous PICO results for 3–5 GeV WIMPs by an order of magnitude.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2019

Electromagnetic backgrounds and potassium-42 activity in the DEAP-3600 dark matter detector

The DEAP-3600 experiment is searching for weakly interacting massive particles dark matter with a 3.3 × 10 3 kg single phase liquid argon (LAr) target, located 2.1 km underground at SNOLAB. The experimental signature of dark matter interactions is kilo electron volt–scale 40 Ar nuclear recoils producing 128 nm LAr scintillation photons observed by photomultiplier tubes. The largest backgrounds in DEAP-3600 are electronic recoils (ERs) induced by β and γ rays originating from internal and external radioactivity in the detector material. A background model of the ER interactions in DEAP-3600 was developed and is described in this work. The model is based on several components which are expected from radioisotopes in the LAr, from ex situ material assay measurements, and from dedicated independent in situ analyses. This prior information is used in a Bayesian fit of the ER components to a 247.2 d dataset to model the radioactivity in the surrounding detector materials. Pulse-shape discrimination separates ER and NR events. However, detailed knowledge of the ER background and activity of detector components sets valuable constraints on NR backgrounds including neutrons and alphas. In addition, the activity of 42 Ar in LAr in DEAP-3600 is determined by measuring the daughter decay of 42 K. Finally, this cosmogenically activated trace isotope is a relevant background at higher energies for other rare event searches using atmospheric argon, e.g., DarkSide-20k, GERDA, or LEGEND. The specific activity of 42 Ar in the atmosphere is found to be 40.4 ± 5.9 μ Bq/kg of argon.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2020

Neutrino interaction classification with a convolutional neural network in the DUNE far detector

The Deep Underground Neutrino Experiment is a next-generation neutrino oscillation experiment that aims to measure $CP$-violation in the neutrino sector as part of a wider physics program. A deep learning approach based on a convolutional neural network has been developed to provide highly efficient and pure selections of electron neutrino and muon neutrino charged-current interactions. The electron neutrino (antineutrino) selection efficiency peaks at 90% (94%) and exceeds 85% (90%) for reconstructed neutrino energies between 2-5 GeV. The muon neutrino (antineutrino) event selection is found to have a maximum efficiency of 96% (97%) and exceeds 90% (95%) efficiency for reconstructed neutrino energies above 2 GeV. When considering all electron neutrino and antineutrino interactions as signal, a selection purity of 90% is achieved. These event selections are critical to maximize the sensitivity of the experiment to $CP$-violating effects.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2020

Discrimination of electronic recoils from nuclear recoils in two-phase xenon time projection chambers

We present a comprehensive analysis of electronic recoil vs. nuclear recoil discrimination in liquid/gas xenon time projection chambers, using calibration data from the 2013 and 2014-16 runs of the Large Underground Xenon (LUX) experiment. We observe strong charge-to-light discrimination enhancement with increased event energy. For events with S1 = 120 detected photons, i.e. equivalent to a nuclear recoil energy of ~100 keV, we observe an electronic recoil background acceptance of <10 –5 at a nuclear recoil signal acceptance of 50%. We also observe modest electric field dependence of the discrimination power, which peaks at a field of around 300 V/cm over the range of fields explored in this study (50-500 V/cm). In the WIMP search region of S1 = 1-80 phd, the minimum electronic recoil leakage we observe is (7.3 ± 0.6) 10 –4 , which is obtained for a drift field of 240-290 V/cm. Pulse shape discrimination is utilized to improve our results, and we find that, at low energies and low fields, there is an additional reduction in background leakage by a factor of up to 3. We develop an empirical model for recombination fluctuations which, when used alongside the Noble Element Scintillation Technique (NEST) simulation package, correctly reproduces the skewness of the electronic recoil data. We use this updated simulation to study the width of the electronic recoil band, finding that its dominant contribution comes from electron-ion recombination fluctuations, followed in magnitude of contribution by fluctuations in the S1 signal, fluctuations in the S2 signal, and fluctuations in the total number of quanta produced for a given energy deposition.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2020

Light new physics in XENON1T

We examine the recently-reported low-energy electron recoil spectrum observed at the XENON1T underground dark matter direct detection experiment, in the context of new interactions with solar neutrinos. In particular we show that scalar and vector mediators with masses $\lesssim 50$ keV coupled to leptons could already leave a visible signature in the XENON1T experiment, similar to the observed peak below 7 keV. This signals that dark matter detectors are already competing with neutrino scattering experiments such as GEMMA, CHARM-II and Borexino. If these results from XENON1T are interpreted as a new signal of such physics, the parameters which fit the excess face challenges from astrophysics which seem very difficult to overcome. If they are rather viewed as a constraint on new couplings, they herald the start of an era of novel precise probes of physics beyond the standard model with dark matter detectors.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2021

Effective field theory analysis of the first LUX dark matter search

The Large Underground Xenon (LUX) dark matter search was a 250-kg active mass dual-phase time projection chamber that operated by detecting light and ionization signals from particles incident on a xenon target. In December 2015, LUX reported a minimum 90% upper C.L. of 6 x 10 -46 cm 2 on the spin-independent WIMP-nucleon elastic scattering cross section based on a 1.4 x 10 4 kg ∙ day exposure in its first science run. Tension between experiments and the absence of a definitive positive detection suggest it would be prudent to search for WIMPs outside the standard spin-independent/spin-dependent paradigm. Recent theoretical work has identified a complete basis of 14 independent effective field theory (EFT) operators to describe WIMP-nucleon interactions. In addition to spin-independent and spin-dependent nuclear responses, these operators can produce novel responses such as angular-momentum-dependent and spin-orbit couplings. Here we report on a search for all 14 of these EFT couplings with data from LUX's first science run. Limits are placed on each coupling as a function of WIMP mass.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2022

Fast and flexible analysis of direct dark matter search data with machine learning

We present the results from combining machine learning with the profile likelihood fit procedure, using data from the Large Underground Xenon (LUX) dark matter experiment. This approach demonstrates reduction in computation time by a factor of 30 when compared with the previous approach, without loss of performance on real data. We establish its flexibility to capture non-linear correlations between variables (such as smearing in light and charge signals due to position variation) by achieving equal performance using pulse areas with and without position-corrections applied. Its efficiency and scalability furthermore enables searching for dark matter using additional variables without significant computational burden. We demonstrate this by including a light signal pulse shape variable alongside more traditional inputs such as light and charge signal strengths. Furthermore, this technique can be exploited by future dark matter experiments to make use of additional information, reduce computational resources needed for signal searches and simulations, and make inclusion of physical nuisance parameters in fits tractable.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗