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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 1,729 records · Page 96
All sourcesNASA NTRSDOE OSTI
DOE OSTI2019

Probing single-unit-cell resolved electronic structure modulations in oxide superlattices with standing-wave photoemission

Control of structural coupling at complex-oxide interfaces is a powerful platform for creating ultrathin layers with electronic and magnetic properties unattainable in the bulk. Yet, with the capability to design and control the electronic structure of such buried layers and interfaces at a unit-cell level, a new challenge emerges to be able to probe these engineered emergent phenomena with depth-dependent atomic resolution as well as element- and orbital selectivity. In this work, we utilize a combination of core-level and valence-band soft x-ray standing-wave photoemission spectroscopy, in conjunction with scanning transmission electron microscopy, to probe the depth-dependent and single-unit-cell resolved electronic structure of an isovalent manganite superlattice [Eu 0.7 Sr 0.3 MnO 3 /La 0.7 Sr 0.3 MnO 3 ]×15 wherein the electronic-structural properties are intentionally modulated with depth via engineered oxygen octahedra rotations/tilts and A-site displacements. Our unit-cell resolved measurements reveal significant transformations in the local chemical and electronic valence-band states, which are consistent with the layer-resolved first-principles theoretical calculations, hence opening the door for future depth-resolved studies of a wide variety of heteroengineered material systems.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2020

Concurrent probing of electron-lattice dephasing induced by photoexcitation in 1 T -TaSeTe using ultrafast electron diffraction

It has been technically challenging to concurrently probe the electrons and the lattices in materials during nonequilibrium processes, allowing their correlations to be determined. Here, in a single set of ultrafast electron diffraction patterns taken on the charge-density-wave (CDW) material 1T-TaSeTe, we discover a temporal shift in the diffraction intensity measurements as a function of scattering angle. With the help of dynamic models and theoretical calculations, we show that the ultrafast electrons probe both the valence-electron and lattice dynamic processes, resulting in the temporal shift measurements. Our results demonstrate unambiguously that the CDW is not merely a result of the periodic lattice deformation ever present in 1T-TaSeTe but has significant electronic origin. This method demonstrates an approach for studying many quantum effects that arise from electron-lattice dephasing in molecules and crystals for next-generation devices.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2021

Probing the effect of magnetic field on charge order in the quasi-two-dimensional Mott insulator κ - (ET) 2 Hg(SCN) 2 Cl

Molecular-based quasi-two-dimensional charge-ordered Mott insulators can possess both spin S = 1/2 and an electric dipole degree of freedom residing on each (BEDT - TTF) 2 lattice site. There exists a theoretical proposal for a magnetoelectric effect in such a material, which can manifest itself as a sensitivity of charge distribution on (BEDT - TTF) 2 dimers to the magnetic field. Here in this work, we used Raman scattering spectroscopy in the magnetic field up to 31 T applied perpendicular to the two-dimensional triangular lattice planes to probe a magnetoelectric effect in $\kappa$ - (ET) 2 H g (SCN) 2 Cl. This is a model compound, which shows charge order and antiferromagnetic correlations at temperatures below 30 K. We discuss possible reasons for the absence of an observable magnetoelectric effect in the probed temperature and magnetic field ranges.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Antiferromagnetic real-space configuration probed by dichroism in scattered x-ray beams with orbital angular momentum

X-ray beams with orbital angular momentum (OAM) are a promising tool for x-ray characterization techniques. Beams with OAM have a helicity - an azimuthally varying phase - which leads to a gradient of the light field. New material properties can be probed by utilizing the helicity of an OAM beam. Here, we demonstrate a dichroic effect in resonant diffraction from an artificial antiferromagnet with a topological defect. We found that the scattered OAM beam has circular dichroism at the antiferromagnetic Bragg peak whose sign is coupled to its helicity, which reveals the real-space configuration of the antiferromagnetic ground state. Thermal cycling of the artificial antiferromagnet can change the ground state, as indicated by reversal of the sign of circular dichroism. This result is one of the first demonstrations of a soft x-ray spectroscopy characterization technique utilizing the OAM of x rays. In conclusion, this helicity-dependent circular dichroism exemplifies the potential to utilize OAM beams to probe matter in a way that is inaccessible using currently available x-ray techniques.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2023

Weak-coupling theory of neutron scattering as a probe of altermagnetism

Inelastic neutron scattering provides a powerful probe of the magnetic excitations of quantum magnets. Altermagnets have recently emerged as a new class of magnets with vanishing net magnetization characteristic of antiferromagnets and with a spin-split electronic structure typical of ferromagnets. Here we introduce a minimal Hubbard model with two-sublattice orthorhombic anisotropy as a framework to study altermagnetism. Using unrestricted Hartree-Fock calculations, we find an altermagnetic state for this model that evolves from a metallic state to an insulating state with increasing Hubbard-U Coulomb repulsion. We then examine the inelastic neutron scattering response in these states using random-phase approximation calculations of the dynamic spin susceptibility χ"(q,ω). We find that the magnetic excitation spectrum depends on its chirality for q along certain directions in reciprocal space, an observation that may be used in inelastic neutron scattering experiments as a probe of altermagnetism.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2016

Aberrated electron probes for magnetic spectroscopy with atomic resolution: Theory and practical aspects

It was recently proposed that electron magnetic circular dichroism (EMCD) can be measured in scanning transmission electron microscopy (STEM) with atomic resolution by tuning the phase distribution of a electron beam. Here, we describe the theoretical and practical aspects for the detection of out-of-plane and in-plane magnetization utilizing atomic size electron probes. Here we present the calculated optimized astigmatic probes and discuss how to achieve them experimentally.

47 OTHER INSTRUMENTATION↗
DOE OSTI2016

Optical spectroscopy and ultrafast pump-probe studies on the heavy-fermion compound CePt 2 In 7

We report optical spectroscopy and ultrafast pump-probe measurements on the antiferromagnetic heavy-fermion compound CePt 2 In 7 , a member showing stronger two dimensionality than other compounds in the CeIn 3 -derived heavy-fermion family. Here, we identify clear and typical hybridization spectral structures at low temperature from the two different spectroscopy probes. But, the strength and related energy scale of the hybridization are much weaker and smaller than that in the superconducting compounds CeCoIn 5 and CeIrIn 5 . The features are more similar to observations on the antiferromagnetic compounds CeIn 3 and CeRhIn 5 in the same family. Our results clearly indicate that the Kondo interaction and hybridizations exist in the antiferromagnetic compounds but with weaker strength.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2016

Probing inter- and intrachain Zhang-Rice excitons in Li 2 CuO 2 and determining their binding energy

Cuprate materials, such as those hosting high-temperature superconductivity, represent a famous class of materials where the correlations between the strongly entangled charges and spins produce complex phase diagrams. Several years ago, the Zhang-Rice singlet was proposed as a natural quasiparticle in hole-doped cuprates. The occurrence and binding energy of this quasiparticle, consisting of a pair of bound holes with antiparallel spins on the same CuO 4 plaquette, depends on the local electronic interactions, which are fundamental quantities for understanding the physics of the cuprates. Here, we employ state-of-the-art resonant inelastic x-ray scattering (RIXS) to probe the correlated physics of the CuO 4 plaquettes in the quasi-one-dimensional chain cuprate Li 2 CuO 2 . By tuning the incoming photon energy to the O K edge, we populate bound states related to the Zhang-Rice quasiparticles in the RIXS process. Both intra- and interchain Zhang-Rice singlets are observed and their occurrence is shown to depend on the nearest-neighbor spin-spin correlations, which are readily probed in this experiment. Finally, we also extract the binding energy of the Zhang-Rice singlet and identify the Zhang-Rice triplet excitation in the RIXS spectra.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2016

Directly probing spin dynamics in insulating antiferromagnets using ultrashort terahertz pulses

We investigate spin dynamics in the antiferromagnetic (AFM) multiferroic TbMnO3 using opticalpump, terahertz (THz)-probe spectroscopy. Photoexcitation results in a broadband THz transmission change, with an onset time of 25 ps at 6 K that becomes faster at higher temperatures. We attribute this time constant to spin-lattice thermalization. The excellent agreement between our measurements and previous ultrafast resonant x-ray diffraction measurements on the same material confirms that our THz pulse directly probes spin order. We suggest that this could be the case in general for insulating AFM materials, if the origin of the static absorption in the THz spectral range is magnetic.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2018

Sb 121 , 123 nuclear quadrupole resonance as a microscopic probe in the Te-doped correlated semimetal FeSb 2 : Emergence of electronic Griffith phase, magnetism, and metallic behavior

121,123 Sb nuclear quadrupole resonance (NQR) was applied to Fe(Sb 1-x Te x ) 2 in the low doping regime (x = 0 , 0.01, and 0.05) as a microscopic zero field probe to study the evolution of 3d magnetism and the emergence of metallic behavior. Whereas the NQR spectra itself reflects the degree of local disorder via the width of the individual NQR lines, the spin lattice relaxation rate (SLRR) 1/T 1 (T) probes the fluctuations at the Sb site. The fluctuations originate either from conduction electrons or from magnetic moments. In contrast to the semimetal FeSb 2 with a clear signature of the charge and spin gap formation in 1/T 1 (T)T[~exp/(Δk B T)] , the 1% Te-doped system exhibits almost metallic conductivity and the SLRR nicely confirms that the gap is almost filled. A weak divergence of the SLRR coefficient 1/T 1 (T)T ~ T -n ~ T -0.2 points towards the presence of electronic correlations towards low temperatures. This is supported by the electronic specific heat coefficient γ = (C el /T) showing a power-law divergence γ (T) ~ T -m ~ (1/T 1 T) 1/2 ~ T -n/2 ~ C el /T which is expected in the renormalized Landau Fermi liquid theory for correlated electrons. In contrast to that the 5% Te-doped sample exhibits a much larger divergence in the SLRR coefficient showing 1/T 1 (T)T ~ T -0.72 . According to the specific heat divergence a power law with n = 2 m = 0.56 is expected for the SLRR. This dissimilarity originates from admixed critical magnetic fluctuations in the vicinity of antiferromagnetic long range order with 1/T 1 (T)T ~ T -3/4 behavior. Furthermore Te-doped FeSb 2 as a disordered paramagnetic metal might be a platform for the electronic Griffith phase scenario. NQR evidences a substantial asymmetric broadening of the 121,123 Sb NQR spectrum for the 5% sample. Lastly, this has a predominant electronic origin in agreement with the electronic Griffith phase and stems probably from an enhanced Sb-Te bond polarization and electronic density shift towards the Te atom inside Sb-Te dumbbell.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2018

Probing short-range magnetic order in a geometrically frustrated magnet by means of the spin Seebeck effect

The spin Seebeck effect (SSE) is a phenomenon where a spin current is generated from thermal excitations in magnetic materials. It is believed that magnetic long-range order (LRO) is not required for SSE, while short-ranged order (SRO) plays an important role. However, a definitive experimental demonstration of the connection between the SSE and SRO has been missing. Here, we show that the SSE is able to probe a specific SRO in a model geometrically frustrated magnet Gd 3 Ga 5 O 12 (GGG). A field-induced SRO in GGG is detected by the SSE in the temperature range 2-5 K. The origin of the SRO is verified by comparing the SSE data directly to existing neutron scattering measurements at much lower temperatures (T < 0.9 K), where field-induced LRO exists. Our theoretical calculations of the magnetic structure further confirm the anisotropic field dependence of the SRO in GGG. Furthermore, these findings establish that the SSE can serve as an effective probe of SRO in geometrically frustrated magnets.

36 MATERIALS SCIENCE↗
DOE OSTI2023

SMEFT probes in future precision DIS experiments

We analyze the potential of future high-energy deep-inelastic scattering (DIS) experiments to probe new physics within the framework of the Standard Model effective field theory (SMEFT). We perform a detailed study of SMEFT probes at a future Large Hadron-electron Collider (LHeC) and a Future Circular lepton-hadron Collider (FCC-eh) machine, and extend previous simulations of the potential of an electron-ion collider (EIC) to include 𝑍-boson vertex corrections. Precision 𝑍-pole constraints on vertex corrections suffer from numerous degeneracies in the Wilson-coefficient parameter space. We find that both the LHeC and the FCC-eh can help remove these degeneracies present in the existing global fits of precision 𝑍-pole observables and LHC data. The FCC-eh and LHeC will in many cases improve upon the existing precision electroweak bounds on the SMEFT parameter space. This highlights the important role of precision DIS measurements for new physics studies.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2015

Probing strong electroweak symmetry breaking dynamics through quantum interferometry at the LHC

Here, we present a new probe of strongly coupled electroweak symmetry breaking at the 14 TeV LHC by measuring a phase shift in the event distribution of the decay azimuthal angles in massive gauge boson scattering. One generically expects a large phase shift in the longitudinal gauge boson scattering amplitude due to the presence of broad resonances. This phase shift is observable as an interference effect between the strongly interacting longitudinal modes and the transverse modes of the gauge bosons. We find that even very broad resonances of masses up to 900 GeV can be probed at 3σ significance with a 3000 fb -1 run of the LHC by using this technique. We also present the estimated reach for a future 50 TeV proton-proton collider.

43 PARTICLE ACCELERATORS↗
DOE OSTI2017

Deep inelastic scattering as a probe of entanglement

Using nonlinear evolution equations of QCD, we compute the von Neumann entropy of the system of partons resolved by deep inelastic scattering at a given Bjorken x and momentum transfer q 2 = - Q 2 . We interpret the result as the entropy of entanglement between the spatial region probed by deep inelastic scattering and the rest of the proton. At small x the relation between the entanglement entropy S ( x ) and the parton distribution x G ( x ) becomes very simple: S ( x ) = ln [ x G ( x ) ] . In this small x , large rapidity Y regime, all partonic microstates have equal probabilities—the proton is composed by an exponentially large number exp ( Δ Y ) of microstates that occur with equal and exponentially small probabilities exp ( - Δ Y ) , where Δ is defined by x G ( x ) ~ 1 / x Δ . For this equipartitioned state, the entanglement entropy is maximal—so at small x , deep inelastic scattering probes a maximally entangled state. Here, we propose the entanglement entropy as an observable that can be studied in deep inelastic scattering. This will then require event-by-event measurements of hadronic final states, and would allow to study the transformation of entanglement entropy into the Boltzmann one. We estimate that the proton is represented by the maximally entangled state at x ≤ 10 -3 ; this kinematic region will be amenable to studies at the Electron Ion Collider.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2017

Resonant di-Higgs boson production in the b b ¯ W W channel: Probing the electroweak phase transition at the LHC

Here, we analyze the prospects for resonant di-Higgs production searches at the LHC in the $b\bar{b}$W + W - (W + →ℓ + ν ℓ , W - →ℓ - $\bar{v}$ ℓ ) channel, as a probe of the nature of the electroweak phase transition in Higgs portal extensions of the Standard Model. In order to maximize the sensitivity in this final state, we develop a new algorithm for the reconstruction of the $b\bar{b}$W + W - invariant mass in the presence of neutrinos from the W decays, building from a technique developed for the reconstruction of resonances decaying to τ + τ - pairs. We show that resonant di-Higgs production in the $b\bar{b}$W + W - channel could be a competitive probe of the electroweak phase transition already with the data sets to be collected by the CMS and ATLAS experiments in run 2 of the LHC. The increase in sensitivity with larger amounts of data accumulated during the high-luminosity LHC phase can be sufficient to enable a potential discovery of the resonant di-Higgs production in this channel.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2017

Probing new spin-independent interactions through precision spectroscopy in atoms with few electrons

The very high precision of current measurements and theory predictions of spectral lines in few-electron atoms allows us to efficiently probe the existence of exotic forces between electrons, neutrons and protons. We investigate here the sensitivity to new spin-independent interactions in transition frequencies (and their isotopic shifts) of hydrogen, helium and some heliumlike ions. We find that present data probe new regions of the force-carrier couplings to electrons and neutrons around the MeV mass range. We also find that, below few keV, the sensitivity to the electron coupling in precision spectroscopy of helium and positronium is comparable to that of the anomalous magnetic moment of the electron. Finally, we interpret our results in the dark-photon model where a new gauge boson is kinetically mixed with the photon. There, we show that helium transitions, combined with the anomalous magnetic moment of the electron, provide the strongest indirect bound from laboratory experiments above 100 keV.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2018

Bottom-quark fusion processes at the LHC for probing Z ' models and B -meson decay anomalies

We investigate models of a heavy neutral gauge boson Z' coupling mostly to third generation quarks and second generation leptons. In this scenario, bottom quarks arising from gluon splitting can fuse into Z' allowing the LHC to probe it. In the generic framework presented, anomalies in B -meson decays reported by the LHCb experiment imply a flavor-violating b s coupling of the featured Z ' constraining the lowest possible production cross section. A novel approach searching for a Z ' (→ μ μ) in association with at least one bottom-tagged jet can probe regions of model parameter space existing analyses are not sensitive to.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2018

Temperature Measurement by a Nanoscale Electron Probe Using Energy Gain and Loss Spectroscopy

Heat dissipation in integrated nanoscale devices is a major issue that requires the development of nanoscale temperature probes. Here, we report the implementation of a method that combines electron energy gain and loss spectroscopy to provide a direct measurement of the local temperature in the nanoenvironment. Loss and gain peaks corresponding to an optical-phonon mode in boron nitride were measured from room temperature to ~ 1600 K. Both loss and gain peaks exhibit a shift towards lower energies as the sample is heated up. First-principles calculations of the temperature-induced phonon frequency shifts provide insights into the origin of this effect and confirm the experimental data. The experiments and theory presented here open the doors to the study of anharmonic effects in materials by directly probing phonons in the electron microscope.

36 MATERIALS SCIENCE↗