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At least 1,729 records · Page 96
All sourcesNASA NTRSDOE OSTI
DOE OSTI2015

Discontinuous non-equilibrium phase transition in a threshold Schloegl model for autocatalysis: Generic two-phase coexistence and metastability

Threshold versions of Schloegl’s model on a lattice, which involve autocatalytic creation and spontaneous annihilation of particles, can provide a simple prototype for discontinuous non-equilibrium phase transitions. These models are equivalent to so-called threshold contact processes. A discontinuous transition between populated and vacuum states can occur selecting a threshold of N ≥ 2 for the minimum number, N, of neighboring particles enabling autocatalytic creation at an empty site. Fundamental open questions remain given the lack of a thermodynamic framework for analysis. For a square lattice with N = 2, we show that phase coexistence occurs not at a unique value but for a finite range of particle annihilation rate (the natural control parameter). This generic two-phase coexistence also persists when perturbing the model to allow spontaneous particle creation. Such behavior contrasts both the Gibbs phase rule for thermodynamic systems and also previous analysis for this model. We find metastability near the transition corresponding to a non-zero effective line tension, also contrasting previously suggested critical behavior. Mean-field type analysis, extended to treat spatially heterogeneous states, further elucidates model behavior.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2016

High-precision measurement of magnetic penetration depth in superconducting films

We report that the magnetic penetration depth (λ) in thin superconducting films is usually measured by the mutual inductance technique. The accuracy of this method has been limited by uncertainties in the geometry of the solenoids and in the film position and thickness, by parasitic coupling between the coils, etc. Here, we present several improvements in the apparatus and the method. To ensure the precise thickness of the superconducting layer, we engineer the films at atomic level using atomic-layer-by-layer molecular beam epitaxy. In this way, we also eliminate secondary-phase precipitates, grain boundaries, and pinholes that are common with other deposition methods and that artificially increase the field transmission and thus the apparent λ. For better reproducibility, the thermal stability of our closed-cycle cryocooler used to control the temperature of the mutual inductance measurement has been significantly improved by inserting a custom-built thermal conductivity damper. Next, to minimize the uncertainties in the geometry, we fused a pair of small yet precisely wound coils into a single sapphire block machined to a high precision. Lastly, the sample is spring-loaded to exactly the same position with respect to the solenoids. Altogether, we can measure the absolute value of λ with the accuracy better than ±1%.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2018

Origins of low-symmetry phases in asymmetric diblock copolymer melts

Cooling disordered compositionally asymmetric diblock copolymers leads to the formation of nearly spherical particles, each containing hundreds of molecules, which crystallize upon cooling below the order–disorder transition temperature (T ODT ). Self-consistent field theory (SCFT) reveals that dispersity in the block degrees of polymerization stabilizes various Frank–Kasper phases, including the C14 and C15 Laves phases, which have been accessed experimentally in low-molar-mass poly(isoprene)-b-poly(lactide) (PI-PLA) diblock copolymers using thermal processing strategies. Heating and cooling a specimen containing 15% PLA above and below the TODT from the body-centered cubic (BCC) or C14 states regenerates the same crystalline order established at lower temperatures. This memory effect is also demonstrated with a specimen containing 20% PLA, which recrystallizes to either C15 or hexagonally ordered cylinders (HEX C ) upon heating and cooling. The process-path–dependent formation of crystalline order shapes the number of particles per unit volume, n/V, which is retained in the highly structured disordered liquid as revealed by small-angle X-ray scattering (SAXS) experiments. We hypothesize that symmetry breaking during crystallization is governed by the particle number density imprinted in the liquid during ordering at lower temperature, and this metastable liquid is kinetically constrained from equilibrating due to prohibitively large free energy barriers for micelle fusion and fission. Ordering at fixed n/V is enabled by facile chain exchange, which redistributes mass as required to meet the multiple particle sizes and packing associated with specific low-symmetry Frank–Kasper phases. Lastly, this discovery exposes universal concepts related to order and disorder in self-assembled soft materials.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2020

Skyrmion–skyrmion interaction in a magnetic film

Interaction of two skyrmions stabilized by the ferromagnetic exchange, Dzyaloshinskii–Moriya interaction (DMI), and external magnetic field has been studied numerically on a 2D lattice of size large compared to the separation, d, between the skyrmions. We show that two skyrmions of the same chirality (determined by the symmetry of the crystal) repel. In accordance with earlier analytical results, their long-range pair interaction falls out with the separation as exp(-d/δ H ), where δ H is the magnetic screening length, independent of the DMI. The prefactor in this expression depends on the DMI that drives the repulsion. The latter results in the spiral motion of the two skyrmions around each other, with the separation between them growing logarithmically with time. When two skyrmions of the total topological charge Q = 2 are pushed close to each other, the discreteness of the atomic lattice makes them collapse into one skyrmion of charge Q = 1 below a critical separation. Experiment is proposed that would allow one to measure the interaction between two skyrmions by holding them in positions with two magnetic tips. Our findings should be of value for designing topologically protected magnetic memory based upon skyrmions.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2019

Performance of layer wound epoxy-impregnated coils made from a multifilamentary cable of exfoliated YBCO

The performance and reliability of magnets made from second generation (2G), exfoliated, YBCO conductors are highly improved by use of narrow, stacked, multifilamentary cable instead of a single wide tape. This work reports on tests of five mini-coils wound from 2.4 mm wide ExoCable™, which is comprised of eight, stacked, exfoliated, YBCO filaments. The filaments are coupled electrically through a re-flow process, which results in enhanced electrical connectivity between the adjacent layers. The coils were tested at 77 K (up to 500 A) in liquid nitrogen and at 22 K (up to 700 A) in a conduction-cooled mode. The cable carries 500 A critical current at 77 K. A six-layer coil wound from 10.5 m of the cable, the largest coil created in the study, demonstrates a critical current of 280 A at 77 K at 0.4 T magnetic field on the winding. The coils were fully impregnated with Stycast 1266 and Henkel W19 low-viscosity epoxies. Repeated thermal cycling, to 77 and 22 K, does not degrade the coil's performance. The cable AC loss and the coil winding magnetization are compared with the traditional 2G wide tape pancake geometry at 77 K. We observe a five times reduction of the winding magnetization when the 12 mm tape is replaced by a 2.4 mm cable, which is explained by the smaller magnetic moment of the cable winding. The field hysteresis profiles recorded at 22 and 77 K are presented to demonstrate the effect of the operation temperature on the winding magnetization. A finite element analysis of the winding magnetization shows a good agreement between the experimentally measured trapped field value, and the critical state model prediction. Finally, we discuss the stability of an ExoCable™ coil in a conduction-cooled operation.

2G cables↗
DOE OSTI2025

Dependence of ion-cyclotron range of frequencies instabilities on species mix and fast-ion distribution: II. Time evolution

Dedicated DIII-D experiments studied instabilities below the ion cyclotron frequency f ci and at cyclotron harmonics by injecting thirteen different neutral beam populations into plasmas with different thermal compositions of H and D at five different values of toroidal field. The resulting database of 2529 conditions is described in Part 1: Stability. This paper focuses on the temporal evolution. For some beam geometries, the ion cyclotron emission (ICE) is much stronger at the beginning of injection, suggesting the importance of ‘bump-on-tail’ energy drive. Sawtooth crashes cause the emission to cease for some beam types and emission bands, but the opposite effect occurs for others. When unstable, for virtually all conditions and frequency bands, the emission bursts in a cycle reminiscent of predator-prey oscillations. Evidence for nonlinear interaction between ICE harmonics is observed. Strongly unstable modes typically appear within 1 ms from the start of beam injection and often decay within 0.1 ms when the beam turns off, but both the initial rise and final decay of the mode power exhibit a wide variety of behavior.

electromagnetic ion cyclotron instabilities↗
DOE OSTI2016

Bubble and skyrmion crystals in frustrated magnets with easy-axis anisotropy

We clarify the conditions for the emergence of multiple-Q structures out of lattice and easy-axis spin anisotropy in frustrated magnets. By considering magnets whose exchange interaction has multiple global minima in momentum space, we find that both types of anisotropy stabilize triple-Q orderings. Moderate anisotropy leads to a magnetic field-induced skyrmion crystal, which evolves into a bubble crystal for increasing spatial and spin anisotropy. Finally, the bubble crystal exhibits a quasi-continuous (devil’s staircase) temperature dependent ordering wave-vector, characteristic of the competition between frustrated exchange and strong easy-axis anisotropy.

36 MATERIALS SCIENCE↗
DOE OSTI2017

Switching dynamics of the spin density wave in superconducting CeCoIn 5

The ordering wave vector Q of a spin density wave (SDW), stabilized within the superconducting state of CeCoIn 5 in a high magnetic field, has been shown to be hypersensitive to the direction of the field. Q can be switched from a nodal direction of the d-wave superconducting order parameter to a perpendicular node by rotating the in-plane magnetic field through the antinodal direction within a fraction of a degree. In this paper, we address the dynamics of the switching of Q. We use a free-energy functional based on the magnetization density, which describes the condensation of magnetic fluctuations of nodal quasiparticles, and show that the switching process includes closing of the SDW gap at one Q and then reopening the SDW gap at another Q perpendicular to the first one. The magnetic field couples to Q through the spin-orbit interaction. Our calculations show that the width of the hysteretic region of switching depends linearly on the deviation of magnetic field from the critical field associated with the SDW transition, consistent with our thermal conductivity measurements. Finally, the agreement between theory and experiment supports our scenario of the hypersensitivity of the Q phase on the direction of magnetic field, as well as the magnon condensation as the origin of the SDW phase in CeCoIn 5 .

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2019

Realization of ordered magnetic skyrmions in thin films at ambient conditions

Magnetic skyrmions have captivated physicists due to their topological nature and novel physical properties. In addition, skyrmions hold significant promise for future information technologies. A key barrier to realizing skyrmion-based devices has been stabilizing these spin structures under ambient conditions. In this paper, we demonstrate that the tunable magnetic properties of amorphous Fe/Gd mulitlayers enable the formation of skyrmion lattices which are stable over a large temperature and magnetic field parameter space, including room temperature and zero magnetic field. These skyrmions, having a hybrid nature displaying both Bloch-type and Néel-type characteristics, are stabilized by dipolar interactions rather than Dzyaloshinskii-Moriya interactions, typically considered a requirement for the generation of skyrmions. Small angle neutron scattering (SANS) was used in combination with soft x-ray microscopy to provide a unique, multiscale probe of the local and long-range order of these structures. The hexagonal lattice seen in SANS results from the hybrid skyrmion picture obtained with micromagnetic simulations. Furthermore, these results identify a pathway to engineer controllable skyrmion phases in thin film geometries which are stable at ambient conditions.

36 MATERIALS SCIENCE↗
DOE OSTI2026

Er Al :Al 2 ⁢O 3 for telecom-band photonics: Electronic structure and optical properties

Er-doped Al 2 ⁢O 3 is a promising host for telecom-band integrated photonics. Here, in this study, we combine ab initio calculations with a symmetry-resolved analysis to elucidate substitutional Er on the Al site (Er Al ) in 𝛼−Al 2 ⁢O 3 . First-principles relaxations confirm the structural stability of Er Al . We then use the local trigonal crystal-field symmetry to classify the Er-derived impurity levels by irreducible representations and to derive polarization-resolved electric-dipole selection rules, explicitly identifying the symmetry-allowed 𝑓−𝑑 hybridization channels. Kubo-Greenwood absorption spectra computed from Kohn-Sham states quantitatively corroborate these symmetry predictions. Furthermore, we connect the calculated intra-4⁢𝑓 line strengths to Judd-Ofelt theory, clarifying the role of 4⁢𝑓−5⁢𝑑 admixture in enabling optical activity. Notably, we predict a characteristic absorption near 1.47 µ⁢m (telecom band), relevant for on-chip amplification and emission. To our knowledge, a symmetry-resolved first-principles treatment of Er:Al 2 ⁢O 3 with an explicit Judd-Ofelt interpretation has not been reported, providing a transferable framework for tailoring rare-earth dopants in wide-band-gap oxides for integrated photonics. Our results for the optical spectra are in good agreement with experimental data. The resulting symmetry-based selection rules translate directly to polarization-dependent coupling in Al 2 ⁢O 3 integrated photonic waveguides and resonators, enabling device-level design of TE/TM-mode interaction with Er emitters in the 1.5-µ⁢m telecom band.

Er-doped Al2O3↗
DOE OSTI2025

Design and Analysis of Short Period 2G-HTS Undulators

Recent advancements in second-generation high-temperature superconducting (2G-HTS) materials have opened new possibilities for superconducting undulator (SCU) technology, particularly in achieving shorter periods and higher magnetic fields. Here, this paper presents the design and analysis of a short-period, as small as 10 mm, 2G-HTS undulator, focusing on magnetic performance, mechanical force minimization, and quench protection. A force-balanced coil pack design is introduced to significantly reduce mechanical stresses on the conductors, eliminating the need for heavy support structures. Rapid prototyping techniques such as3D printing is employed to refine the design for scalability and manufacturability. Correction schemes for end-field effects are developed using a combination of 2G-HTS tapes and NbTi conductors to optimize field integrals. Simulation results demonstrated that optimized magnetic performance and enhanced mechanical stability, positioning 2G-HTS undulators as promising candidates for storage ring and free-electron based light sources.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2017

On the Evolution From Micrometer-Scale Inhomogeneity to Global Overheated Structure During the Intense Joule Heating of a z-Pinch Rod

Ultrafast optical microscopy of metal z-pinch rods pulsed with megaampere current is contributing new data and critical insight into what provides the fundamental seed for the magneto-Rayleigh-Taylor (MRT) instability. A two-frame near infrared/visible intensified-charge-coupled device gated imager with 2-ns temporal resolution and 3-μm spatial resolution captured emissions from the nonuniformly Joule heated surfaces of ultrasmooth aluminum (Al) rods. Nonuniform surface emissions are consistently first observed from discrete, 10-μm scale, subelectronvolt spots. Aluminum 6061 alloy, with micrometer-scale nonmetallic resistive inclusions, forms several times more spots than 99.999% pure Al 5N; 5-10 ns later, azimuthally stretched elliptical spots and distinct strata (40-100 μm wide by 10 μm tall) are observed on Al 6061, but not on Al 5N. In such overheat strata, aligned parallel to the magnetic field, we find that they are highly effective seeds for MRT instability growth. Our data give credence to the hypothesis that early nonuniform Joule heating, such as the electrothermal instability, may provide the dominant seed for MRT.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2014

SU-E-T-220: Investigation of Intrafraction Changes to Photon Beam Profiles

Purpose: Treatment Planning Systems model beam profiles to be static and independent of gantry angle. This work investigates how beam profiles change over time, with varying gantry angle. Methods: 200 cGy was delivered to ICProfiler (Sun Nuclear) on 2 Elekta Synergys and 1 Varian 21EX linacs at 8 gantry angles and 1 clockwise arc. Measurements were recorded 8 times per second. To investigate the initial portion of the beams, single-shot and multi-control-point beams were measured. The differences in beam profiles were analyzed as well as the length of time for the beam to stabilize. Symmetry was calculated 5cm from the central axis at 100cm SSD. Field sizes ranged from 30×30 cm{sup 2} to 40×40 cm{sup 2}. Results: The beam profiles changed over time and were dependent on gantry angle. The composite profile for each beam met 1% tolerance described in TG-142. It took up to 14.7, 3.7 and 11.3 cGy for the two Elektas and Varian respectively to satisfy the tolerance. All linacs had the most flat, symmetric, and stable beam profile with the gantry at 0 degrees, where the symmetry was 100.5%±0.55, 101.0%±0.52 and 101.1%±0.44 respectively. The symmetry was 100.7%±1.06, 101.1%±1.05 and 101.2%±0.64 at the gantry angle with the biggest discrepancy (90, 180 and 180 degrees respectively). Symmetry was better in the X direction for the Elektas and the Y for the Varian. Fluctuations in beam profiles corresponded to changes in dose rate. Conclusion: Flatness and symmetry changed over time and with gantry angle. Because Treatment Planning Systems do not account for these changes, it may be necessary to limit certain beams from clinical use, for example, beams with low MU. It may also be necessary to add additional QA procedures beyond those suggested in TG-142 to account for these changes.

07 ISOTOPE AND RADIATION SOURCES↗
DOE OSTI2018

Assessing the Strategic Effects of Artificial Intelligence (Workshop Summary)

On September 20-21, the Center for Global Security Research (CGSR) at Lawrence Livermore National Laboratory (LLNL), in collaboration with Technology for Global Security (Tech4GS), hosted a workshop to examine the implications of advances in artificial intelligence (AI) on international security and strategic stability. Participating policymakers, scholars, technical experts, and representatives of various private sector organizations addressed the central question of whether the United States government should consider adjusting its approach to nuclear deterrence and strategic stability in light of the wide range of developments in the AI field. The workshop examined the potential risks and opportunities presented by military applications of AI and assessed which of these require consideration in the near term—and which might be exaggerated. This report is a summary of workshop discussion. The views reported here are the personal views of individual participants and should not be attributed to the organizers, the National Nuclear Security Administration, the Department of Energy, or the United States government.

99 GENERAL AND MISCELLANEOUS↗
DOE OSTI2020

High Fidelity Simulations of a Methane-Oxygen Rotating Detonation Rocket Engine

The rotating detonation combustor (RDC) is an important realization of pressure gain combustion for practical applications. The RDC system is characterized by a highly unsteady flow field, with multiple reflected pressure waves following the strong detonations and the existence of partially-burnt gases entrained within the detonation annulus during the injector recovery process. While experimental efforts have provided macroscopic properties of an RDC with a given fuel-oxidizer mixture and geometry, limited optical access and reduced lifespan of flow-field diagnostic equipment constrain understanding of the mechanisms that lend to wave stability, controllability, and sustainability. To this end, high-fidelity numerical simulations of the Air Force Research Laboratory (AFRL) methane-oxygen rotating detonation rocket engine (RDRE) are performed to provide detailed insight into the detonation physics and anomalous behavior within the combustor. The results highlight the merit of high-fidelity numerical studies in analyzing the combustion processes and injector dynamics of a complex combustion system. The simulations capture the general wave behavior observed within the experimental studies. Three different operating conditions, with varying global equivalence ratio and system mass flow rate, are considered: (1) baseline configuration, (2) high equivalence ratio, and (3) high mass flow rate. The high mass flow rate case results in increased detonation wave strength whereas the high equivalence ratio results in increased deflagrative heat release. The high equivalence ratio case results in chaotic behavior with two pairs of counter-rotating detonation waves, whereas a single pair of co-rotating waves is observed in the baseline and high mass flow rate cases. Further, parasitic combustion of the reactant mixture ahead of the detonation wave diminishes its strength and reduces propagation speed to approximately 50-60\% of the Chapman-Jouguet (CJ) condition. In this work, a detailed analysis of the detonation wave behavior, injector dynamics, and the statistics of combustion parameters are presented.

Prakash, Supraj↗
DOE OSTI2020

Chemical and Structural Changes in Corn Stover After Ensiling: Influence on Bioconversion

Production of biofuels, bioproducts, and bioenergy requires a well-characterized, stable, and reasonably uniform biomass supply and well-established supply chains for shipping biomass from farm fields to biorefineries, while achieving year-round production targets. Preserving and stabilizing biomass feedstock during storage is a necessity for cost-effective and sustainable biofuel production. Ensiling is a common storage method used to preserve and even improve forage quality; however, the impact of ensiling on biomass physical and chemical properties that influence bioconversion processes has been variable. Our objective in this work was to determine the effects of ensiling on lignocellulosic feedstock physicochemical properties and how that influences bioconversion requirements. We observed statistically significant decreases (p < 0.05) in the content of two major structural carbohydrates (glucan and xylan) of 5 and 8%, respectively, between the ensiled and non-ensiled materials. We were unable to detect differences in sugar yields from structural carbohydrates after pretreatment and enzymatic hydrolysis of the ensiled materials compared to non-ensiled controls. Based on this work, we conclude that ensiling the corn stover did not change the bioconversion requirements compared to the control samples and incurred losses of structural carbohydrates. At the light microscopy level, ensiled corn stover exhibited little structural change or relocation of cell wall components as detected by immunocytochemistry. However, more subtle structural changes were revealed by electron microscopy, as ensiled cell walls exhibit ultrastructural characteristics such as wall delimitation intermediate between non-ensiled and dilute-acid-pretreated cell walls. These findings suggest that alternative methods of conversion, such as deacetylation and mechanical refining, could take advantage of lamellar defects and may be more effective than dilute acid or hot water pretreatment for biomass conversion of ensiled materials.

09 BIOMASS FUELS↗
DOE OSTI2017

The Fate of Close-in Planets: Tidal or Magnetic Migration?

Planets in close-in orbits interact magnetically and tidally with their host stars. These interactions lead to a net torque that makes close-in planets migrate inward or outward depending on their orbital distance. We systematically compare the strength of magnetic and tidal torques for typical observed star–planet systems (T-Tauri and hot Jupiter, M-dwarf and Earth-like planet, K star and hot Jupiter) based on state-of-the-art scaling laws. We find that depending on the characteristics of the system, tidal or magnetic effects can dominate. For very close-in planets, we find that both torques can make a planet migrate on a timescale as small as 10–100 thousands of years. Both effects thus have to be taken into account when predicting the evolution of compact systems.

79 ASTRONOMY AND ASTROPHYSICS↗