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All sourcesNASA NTRSDOE OSTI
NASA NTRS1996

Computational Modeling of Multi-Phase/Multi-Species Flows with Applications to Liquid Rocket Engines

Accurate prediction of all physical phenomena in a combustion chamber is essential for better understanding of the system performance. Atomization, evaporation, combustion, chemical kinetics, and turbulence are those processes of great importance that need to be well understood. Processes involving the liquid phase in a combustion chamber will be further complicated under supercritical conditions. More advanced and accurate numerical techniques are required to extend our understanding of the above phenomena. A computer program for multi-species/multi-phase flow was developed for NASA/MSFC in 1992. This code, called Liquid Thrust Chamber Performance (LTCP) program takes an Eulerian- Eulerian approach and is based on the Total Variation Diminishing (TVD) technique with Lax-Friedrichs upwind method. Under the NASA/ASEE SFFP the LTCP code was used to predict the performance characteristics of several engines that were of particular interest to NASA. This code was also successful in a combustion detonation study. Converting the program to the PC platform was accomplished which extends usability and makes it available to a wider range of users. The Eulerian formulation of the liquid phase provides a suitable model that can be extended to include combustion modeling under supercritical conditions. The results have been compared against the ones of other codes and available measured data. The algorithm proved to be robust and efficient for problems with stiff source terms.

Navaz, Homayun K.↗
NASA NTRS1999

Inversion of Gravity Fields From the Spacecraft Orbital Data Using an Adjoint Operator Approach

In perturbation approximation, the forward problem of orbital dynamics (equations with initial conditions) is linear with respect to variations of coordinates and/or velocities of the spacecraft and to corresponding variations of the gravity field in the models used. The linear operator adjoint to the linear operator of such forward problem turns out to be instrumental in inversion of differences between observed and predicted coordinates/velocities in terms of the updates of harmonics in the initial gravity field model. Based on this approach, the solution of resulting adjoint problem of orbital dynamics can be used to directly evaluate the matrix of partial derivatives of observable differences with respect to the gravity field harmonics. General discussion of the adjoint problem of orbital dynamics is given and an example of a mathematical formalism for the practical retrieval algorithm is presented.

Ustinov, E. A.↗
NASA NTRS2011

NPP VIIRS Geometric Performance Status

Visible Infrared Imager Radiometer Suite (VIIRS) instrument on-board the National Polar-orbiting Operational Environmental Satellite System (NPOESS) Preparatory Project (NPP) satellite is scheduled for launch in October, 2011. It is to provide satellite measured radiance/reflectance data for both weather and climate applications. Along with radiometric calibration, geometric characterization and calibration of Sensor Data Records (SDRs) are crucial to the VIIRS Environmental Data Record (EDR) algorithms and products which are used in numerical weather prediction (NWP). The instrument geometric performance includes: 1) sensor (detector) spatial response, parameterized by the dynamic field of view (DFOV) in the scan direction and instantaneous FOV (IFOV) in the track direction, modulation transfer function (MTF) for the 17 moderate resolution bands (M-bands), and horizontal spatial resolution (HSR) for the five imagery bands (I-bands); 2) matrices of band-to-band co-registration (BBR) from the corresponding detectors in all band pairs; and 3) pointing knowledge and stability characteristics that includes scan plane tilt, scan rate and scan start position variations, and thermally induced variations in pointing with respect to orbital position. They have been calibrated and characterized through ground testing under ambient and thermal vacuum conditions, numerical modeling and analysis. This paper summarizes the results, which are in general compliance with specifications, along with anomaly investigations, and describes paths forward for characterizing on-orbit BBR and spatial response, and for improving instrument on-orbit performance in pointing and geolocation.

Lin, Guoqing↗
DOE OSTI2021

Adaptive Variational Quantum Imaginary Time Evolution Approach for Ground State Preparation

Abstract An adaptive variational quantum imaginary time evolution (AVQITE) approach is introduced that yields efficient representations of ground states for interacting Hamiltonians on near‐term quantum computers. It is based on McLachlan's variational principle applied to imaginary time evolution of variational wave functions. The variational parameters evolve deterministically according to equations of motions that minimize the difference to the exact imaginary time evolution, which is quantified by the McLachlan distance. Rather than working with a fixed variational ansatz, where the McLachlan distance is constrained by the quality of the ansatz, the AVQITE method iteratively expands the ansatz along the dynamical path to keep the McLachlan distance below a chosen threshold. This ensures the state is able to follow the quantum imaginary time evolution path in the system Hilbert space rather than in a restricted variational manifold set by a predefined fixed ansatz. AVQITE is used to prepare ground states of H 4 , H 2 O, and BeH 2 molecules, where it yields compact variational ansätze and ground state energies within chemical accuracy. Polynomial scaling of circuit depth with system size is shown through a set of AVQITE calculations of quantum spin models. Finally, quantum Lanczos calculations are demonstrated alongside AVQITE without additional quantum resource costs.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2025

Estimation of cutting tool wear using an elastomeric tactile sensor

Machining performance of cutting tools and part quality are affected by the geometric condition of the cutting edge, which is influenced by thermomechanical loads experienced during the process. Tool condition monitoring (TCM) systems provide insight for timely replacement of cutting tools. However, existing TCM systems are expensive and require specialized equipment or sensors, hindering widespread adoption. A novel TCM system is developed herein using an elastomeric tactile sensor. Sensor images of the cutting edge are used to quantify wear using two distinct algorithms. In the first algorithm, the unworn and worn edges are identified based on Canny edge detect. In the second, the unworn edge is identified using edge detection while the region of wear is identified using a relative intensity method. In both cases, the maximum wear width is calculated based on an experimentally determined pixel to-physical distance scale. The TCM system is first used to estimate flank wear on a solid carbide helical end mill before evaluating its robustness by employing it to estimate insert wear of an indexable helical end mill. Measurements are also performed manually using an optical microscope and a high-resolution focus variation microscope for verification. The novel technique estimates flank wear in the solid carbide tool with a high accuracy of 98%. Larger discrepancies are observed for the inserts, however, with overlapping uncertainties. In conclusion, the technique shows promise in adaptability, automation, and closed loop control of machine tools.

Machining↗
DOE OSTI2025

Adaptive PID Gain Scheduling Control for Hydropower Turbine Using Neural CDE and Stochastic Distribution Shaping

This paper introduces a gain-scheduling PID controller design strategy for hydroturbine frequency control mode. This scheme first uses real data to learn the nonlinear dynamics of the hydroturbine using neural controlled differential equations and then perturbs the obtained nonlinear system at different equilibrium points, based on which a static output feedback adaptive dynamic programming algorithm is then used to optimize the PID gains for each equilibrium point. Moreover, a continuous-time version of stochastic distribution control is proposed to further fine-tune the optimized PID gains. Finally, the controller is obtained by implementing linear interpolation between the optimized PID control gains. The simulation results show that the proposed gain-scheduling PID controller can control a larger range of operation points compared with the given fixed PID controller and the baseline method. Compared with the given fixed PID controller, the proposed gain-scheduling PID controller can regulate hydroturbine frequency against disturbances induced by power-load variation with over 50% less overshoot for some operation points.

13 HYDRO ENERGY↗
DOE OSTI2024

Performance Comparison of Machine Learning Models for Ultrasonic Nondestructive Evaluation of Alkali-Silica Reaction in Concrete

Alkali-silica reaction (ASR) causes concrete degradation, leading to cracking, rebar corrosion, and reduced structural integrity, which raises safety concerns. Ultrasonic nondestructive evaluation (NDE) effectively assesses concrete properties and monitors ASR progression. However, its deployment and analysis require specialized expertise and subjective interpretation. As computational power increases, artificial intelligence (AI) and machine learning (ML) algorithms are increasingly being used to automate NDE data analysis across various industries for AI-assisted automation. Regulatory agencies are adapting to this technological shift, prompting a need to evaluate current ML technologies’ capabilities and limitations in assessing concrete material properties and damage. This report presents a comparative analysis of four ML regression models for predicting concrete material damage induced by ASR expansion using long-term ultrasonic data monitoring. The models investigated include linear regression (LR), support vector regression (SVR), shallow neural networks (NN), and deep neural networks (DNN). LR, SVR, and shallow NN models use features extracted from ultrasonic signals, whereas the DNN model processes time-domain ultrasonic signals and frequency spectra directly. The study systematically compared the models’ performance from various perspectives, including model input, prediction performance, and generalization ability. The findings indicate significant variability in model performance, with some ML algorithms achieving very high or very low prediction accuracy depending on the preprocessing and feature engineering (extraction and selection) applied. Key insights include the observation that shallow ML models (LR, SVR, and shallow NNs) require meticulous preprocessing and feature extraction to achieve high accuracy. In contrast, the DNN model, although it bypasses the need for feature engineering, necessitates extensive preprocessing to mitigate noise and computational demands. The SVR model emerged as the top performer among the shallow models, and the DNN model exhibited superior performance on specific datasets but struggled with generalization across specimens from different batches. Additionally, the SVR model is sensitive to temperature variations, whereas the DNN model is robust in this regard. Using recurrent neural networks is recommended for future ASR expansion prediction studies. Recurrent neural networks’ inherent ability to capture temporal dependencies and long-term patterns makes them well suited for analyzing sequential ultrasonic monitoring data. Overall, the results and conclusions of this study could provide insights into the capabilities and effectiveness of ML when applied to ultrasonic NDE data and help identify best practices for using ML for ultrasonic NDE of concrete material properties.

36 MATERIALS SCIENCE↗
NASA NTRS1988

Water vapor profiling using microwave radiometry

Water vapor is one of the most important constituents in the Earth's atmosphere. Its spatial and temporal variations affect a wide spectrum of meteorological phenomena ranging from the formation of clouds to the development of severe storms. The passive microwave technique offers an excellent means for water vapor measurements. It can provide both day and night coverage under most cloud conditions. Two water vapor absorption features, at 22 and 183 GHz, were explored in the past years. The line strengths of these features differ by nearly two orders of magnitude. As a consequence, the techniques and the final products of water vapor measurements are also quite different. The research effort in the past few years was to improve and extend the retrieval algorithm to the measurements of water vapor profiles under cloudy conditions. In addition, the retrieval of total precipitable water using 183 GHz measurements, but in a manner analogous to the use of 22 GHz measurements, to increase measurement sensitivity for atmospheres of very low moisture content was also explored.

Wang, J. R.↗
NASA NTRS1995

Interaction of the terrestrial and atmospheric hydrological cycles in the context of the North American southwest summer monsoon

Work under this grant has used information on precipitation and water vapor fluxes in the area of the Mexican Monsoon to analyze the regional precipitation climatology, to understand the nature of water vapor transport during the monsoon using model and observational data, and to analyze the ability of the TRMM remote sensing algorithm to characterize precipitation. An algorithm for estimating daily surface rain volumes from hourly GOES infrared images was developed and compared to radar data. Estimates were usually within a factor of two, but different linear relations between satellite reflectances and rainfall rate were obtained for each day, storm type and storm development stage. This result suggests that using TRMM sensors to calibrate other satellite IR will need to be a complex process taking into account all three of the above factors. Another study, this one of the space-time variability of the Mexican Monsoon, indicate that TRMM will have a difficult time, over the course of its expected three year lifetime, identifying the diurnal cycle of precipitation over monsoon region. Even when considering monthly rainfalls, projected satellite estimates of August rainfall show a root mean square error of 38 percent. A related examination of spatial variability of mean monthly rainfall using a novel method for removing the effects of elevation from gridded gauge data, show wide variation from a satellite-based rainfall estimates for the same time and space resolution. One issue addressed by our research, relating to the basic character of the monsoon circulation, is the determination of the source region for moisture. The monthly maps produced from our study of monsoon variability show the presence of two rainfall maxima in the analysis normalized to sea level, one in south-central Arizona associated with the Mexican monsoon maximum and one in southeastern New Mexico associated with the Gulf of Mexico. From the point of view of vertically-integrated fluxes and flux divergence of water vapor from ECMWF data, most moisture at upper levels arrives from the Gulf of Mexico, while low level moisture comes from the northern Gulf of California. Composites of ECMWF analyses for wet and dry periods (classified by rain gauge data) show that both regimes show low level moisture arriving from northern and central Gulf of California. Above 700 MB, moisture comes from both source regions and the Sierra Madre Occidental. During wet periods a longer fetch through the moist air mass above western Mexico results in a greater moisture flux into the Sonoran Desert region, while there is less moisture from the Gulf of Mexico both above and below 700 mb. Work on the grant subcontract at the University of Colorado concentrated on the development of a technique useful to TRMM combining visible, infrared and passive microwave data for measuring precipitation. Two established techniques using either visible or infrared data applied over the US Southwest correlated with gauges at the 0.58 to 0.70 level. The application of some established passive microwave techniques were less successful for a variety of reason, including problems in both the gauge and satellite data quality, sampling problems and weaknesses inherent in the algorithms themselves. A more promising solution for accurate rainfall estimation was explored using visible and infrared data to perform a cloud classification, which when combined with information about the background (e.g. Iand/ocean), was used to select the most appropriate microwave algorithm from a suite of possibilities.

Dickinson, Robert E.↗
NASA NTRS2018

Modeling Key Predictors of Airport Runway Configurations Using Learning Algorithms

Advanced traffic flow management automation will need accurate predictions of airport runway configurations. Terminal area weather and traffic demand are generally considered to be the most significant factors in predicting runway configuration. Weather information is forecasted across multiple features, including wind direction, wind speed, gusts, cloud ceilings, visibility, temperature, and precipitation, among many others. We use machine learning techniques on historical weather and runway data to determine weather features that correlate well with runway configurations. We analyze the predictive capability of weather features using different learning models trained on data from four major U.S. airports: Atlanta (ATL), Washington – Dulles (IAD), New York – Kennedy (JFK), and San Francisco (SFO). Wind direction alone is strongly correlated with runway configurations above all other examined factors, as expected. This correlation is the most significant component of the ~80% prediction accuracy in selecting between the two most frequently used runway configurations. However, individual airports show variations on how well the runway configuration decisions correlate with wind direction. While wind direction was identified as the most significant indicator of configuration decisions in ATL, IAD, and JFK, it did not emerge as such at SFO. Traffic demand was not found to be a strong factor in predicting runway configurations at any of the airports analyzed. In rare instances, when high demand cannot be accommodated within the current configuration, temporary changes are likely to be attributable to demand. However, these occurrences are so limited in number that their overall effect is not sufficient to consider traffic demand as a major indicator of runway configuration at the airports analyzed.

Bilimoria, Karl D.↗
NASA NTRS1990

Comparison of satellite based cloud retrieval methods for cirrus and stratocumulus

One difficulty in using satellite remote sensing data is the spatial variability of cloud properties on scales smaller than most meteorological satellite fields of view (approx. 4 to 8 km). The variation is examined of satellite derived cloud cover as a function of the satellite sensor spatial resolution for seven cloud cover retrieval methods: (1) Reflectance threshold; (2) Temperature threshold; (3) ISCCP; (4) HBTM (Hybrid Bispectral Threshold Method); (5) NCLE; (6) Spatial coherence; and (7) Functional Box Counting. The first two methods are simple single spectral thresholds which specify a satellite pixel as cloud filled if the measured reflectance is greater than the threshold, or if the measured equivalent blackbody temperature is less than the threshold. The next three methods are bispectral, using one visible wavelength window channel and one thermal infrared wavelength window. The final two algorithms rely on the spatial variability within the cloud field to determine cloud cover. Spatial coherence assumes only that the cloud field occurs in a single layer and that the clouds are optically thick in the infrared window. LANDSAT Thematic Mapper (TM) data is used to test the spatial resolution dependence of the cloud algorithms. The ISCCP bispectral threshold applied to the full resolution data is used as the reference or truth cloud cover, after which the retrieval methods are applied to the spatial resolutions. Studies of the fraction of pixels in the scene at cloud edge, and of the profile of reflectance and temperature near cloud edges indicate an uncertainty in the reference cloud fraction of 1 to 5 percent.

Parker, Lindsay↗
NASA NTRS2012

Spatial and Temporal Distribution of Clouds Observed by MODIS Onboard the Terra and Aqua Satellites

The Moderate Resolution Imaging Spectroradiometer (MODIS) was developed by NASA and launched aboard the Terra spacecraft on December 18, 1999 and Aqua spacecraft on May 4, 2002. A comprehensive set of remote sensing algorithms for the retrieval of cloud physical and optical properties have enabled over twelve years of continuous observations of cloud properties from Terra and over nine years from Aqua. The archived products from these algorithms include 1 km pixel-level (Level-2) and global gridded Level-3 products. In addition to an extensive cloud mask, products include cloud-top properties (temperature, pressure, effective emissivity), cloud thermodynamic phase, cloud optical and microphysical parameters (optical thickness, effective particle radius, water path), as well as derived statistics. Results include the latitudinal distribution of cloud optical and radiative properties for both liquid water and ice clouds, as well as latitudinal distributions of cloud top pressure and cloud top temperature. MODIS finds the cloud fraction, as derived by the cloud mask, is nearly identical during the day and night, with only modest diurnal variation. Globally, the cloud fraction derived by the MODIS cloud mask is approx.67%, with somewhat more clouds over land during the afternoon and less clouds over ocean in the afternoon, with very little difference in global cloud cover between Terra and Aqua. Overall, cloud fraction over land is approx.55%, with a distinctive seasonal cycle, whereas the ocean cloudiness is much higher, around 72%, with much reduced seasonal variation. Cloud top pressure and temperature have distinct spatial and temporal patterns, and clearly reflect our understanding of the global cloud distribution. High clouds are especially prevalent over the northern hemisphere continents between 30 and 50 . Aqua and Terra have comparable zonal cloud top pressures, with Aqua having somewhat higher clouds (cloud top pressures lower by 100 hPa) over land due to afternoon deep convection. The coldest cloud tops (colder than 230 K) generally occur over Antarctica and the high clouds in the tropics (ITCZ and the deep convective clouds over the western tropical Pacific and Indian sub-continent).

King, Michael D.↗
NASA NTRS2018

The Next-Generation Goddard Convective-Stratiform Heating Algorithm: New Tropical and Warm-Season Retrievals for GPM

The Goddard convective-stratiform heating (CSH) algorithm, used to estimate cloud heating in support of the Tropical Rainfall Measuring Mission (TRMM), is upgraded in support of the Global Precipitation Measurement (GPM) mission. The algorithm's lookup tables (LUTs) are revised using new and additional cloud-resolving model (CRM) simulations from the Goddard Cumulus Ensemble (GCE) model, producing smoother heating patterns that span a wider range of intensities because of the increased sampling and finer GPM product grid. Low-level stratiform cooling rates are reduced in the land LUTs for a given rain intensity because of the rain evaporation correction in the new four-class ice (4ICE) scheme. Additional criteria, namely, echo-top heights and low-level reflectivity gradients, are tested for the selection of heating profiles. Those resulting LUTs show greater and more precise variation in their depth of heating as well as a tendency for stronger cooling and heating rates when low-level dBZ values decrease toward the surface. Comparisons versus TRMM for a 3-month period show much more low-level heating in the GPM retrievals because of increased detection of shallow convection, while upper-level heating patterns remain similar. The use of echo tops and low-level reflectivity gradients greatly reduces midlevel heating from ~2 to 5 km in the mean GPM heating profile, resulting in a more top-heavy profile like TRMM versus a more bottom-heavy profile with much more midlevel heating. Integrated latent heating rates are much better balanced versus surface rainfall for the GPM retrievals using the additional selection criteria with an overall bias of +4.3%.

Lang, Stephen E.↗
DOE OSTI2025

Quantum Algorithm for Linear Non-unitary Dynamics with Near-Optimal Dependence on All Parameters

We introduce a family of identities that express general linear non-unitary evolution operators as a linear combination of unitary evolution operators, each solving a Hamiltonian simulation problem. This formulation can exponentially enhance the accuracy of the recently introduced linear combination of Hamiltonian simulation (LCHS) method [An, Liu, and Lin, Physical Review Letters, 2023]. For the first time, this approach enables quantum algorithms to solve linear differential equations with both optimal state preparation cost and near-optimal scaling in matrix queries on all parameters.

Applied Dynamical Systems↗
NASA NTRS1993

Three dimensional modeling of cirrus during the 1991 FIRE IFO 2: Detailed process study

A three-dimensional model of cirrus cloud formation and evolution, including microphysical, dynamical, and radiative processes, was used to simulate cirrus observed in the FIRE Phase 2 Cirrus field program (13 Nov. - 7 Dec. 1991). Sulfate aerosols, solution drops, ice crystals, and water vapor are all treated as interactive elements in the model. Ice crystal size distributions are fully resolved based on calculations of homogeneous freezing of solution drops, growth by water vapor deposition, evaporation, aggregation, and vertical transport. Visible and infrared radiative fluxes, and radiative heating rates are calculated using the two-stream algorithm described by Toon et al. Wind velocities, diffusion coefficients, and temperatures were taken from the MAPS analyses and the MM4 mesoscale model simulations. Within the model, moisture is transported and converted to liquid or vapor by the microphysical processes. The simulated cloud bulk and microphysical properties are shown in detail for the Nov. 26 and Dec. 5 case studies. Comparisons with lidar, radar, and in situ data are used to determine how well the simulations reproduced the observed cirrus. The roles played by various processes in the model are described in detail. The potential modes of nucleation are evaluated, and the importance of small-scale variations in temperature and humidity are discussed. The importance of competing ice crystal growth mechanisms (water vapor deposition and aggregation) are evaluated based on model simulations. Finally, the importance of ice crystal shape for crystal growth and vertical transport of ice are discussed.

Jensen, Eric J.↗
NASA NTRS2003

Regional Variability in Convection and Rain Retrievals from the TRMM Microwave Imager (TMI)

Precipitation Radar (PR) on board the TRMM satellite shows that the average height of 30 dBz in convective rain areas of the tropics varies significantly from one region to the other. When the convection is weak this height is shallow and when convection is strong this height extends deeper into the troposphere. The brightness temperature (Tb) measured by the microwave radiometer by itself does not reflect this nature of convection satisfactorily. Radiative transfer simulations of Tbs reveal that this could be due to the variations in the vertical distribution of optically active water and ice hydrometeors and their density, shape, and size. These variations are not coupled uniquely to the strength of the convective updrafts, and as a result the Tbs do not reflect properly the convective strength indicated by PR. Because of this deficiency in the Tbs the rain rate deduced from them differs from that of PR. For this reason, to improve the estimation of rain rate we have developed an empirical method. In this method a parameter based on the areal extent of the Tbs that exceed a certain magnitude is included along with the Tbs. Rain rate deduced with this approach is better correlated with that of PR when compared to the current Version 5 operational algorithm. The percentage of rain volume as a function of rain rate, for a given region of 5deg lat. X 5deg long. over a period of three months, deduced from this method, is also in better agreement with that of the PR.

Prabhakara, C.↗
NASA NTRS2004

Hydrodynamic Modeling of Oxidizer-Rich Staged Combustion Injector Flow

The main objective of this work is to determine the unsteady hydrodynamic characteristics of coaxial swirl atomizers of interest in oxidizer-rich staged combustion (ORSC) liquid rocket engines. To this end, the pseudo-density (homogeneous flow) treatment combined with the Marker-and-Cell (MAC) numerical algorithm has been used to develop an axisymmetric with swirl, two-phase, unsteady model. The numerical model is capable of assessing the time-dependent orifice exit conditions and internal mixing for arbitrary fuel and oxidizer gas injection conditions. Parametric studies have been conducted to determine the effect of geometry, gas properties, and liquid properties on the exit massflow rate and velocity. It has been found that the frequency at which the liquid film oscillates increases as the density ratio and thickness increase, decreases as film thickness and liquid swirl velocity increase, and is unaffected by the mixing length. Additionally, it has been determined that the variation in the massflow rate increases as the liquid swirl velocity and liquid film thickness increase, and decreases as the density ratio, collar thickness, and mixing length increase.

Canino, J. V.↗
NASA NTRS2022

Inferring iron-oxide species content in atmospheric mineral dust from DSCOVR EPIC observations

The iron-oxide content of dust in the atmosphere and most notably its apportionment between hematite (α-Fe2O3) and goethite (α-FeOOH) are key determinants in quantifying dust’s light absorption, its top of atmosphere UV radiances used for dust monitoring, and ultimately shortwave dust direct radiative effects (DRE). Hematite and goethite column mass concentrations and iron-oxide mass fractions of total dust mass concentration were retrieved from the DeepSpace Climate Observatory (DSCOVR) Earth Polychromatic Imaging Camera (EPIC) measurements in the ultraviolet–visible (UV–Vis) channels. The retrievals were performed for dust-identified aerosol plumes over land using aerosol optical depth (AOD) and spectral imaginary refractive index provided by the Multi-Angle Implementation of Atmospheric Correction (MAIAC) algorithm over six continental regions (North America, North Africa, West Asia, Central Asia, EastAsia, and Australia). The dust particles are represented as an internal mixture of non-absorbing host and absorbing hematite and goethite. We use the Maxwell–Garnett effective medium approximation with carefully selected complex refractive indices of hematite and goethite that produce mass fractions of iron oxides species consistent with in situ values found in the literature to derive the hematite and goethite volumetric/mass concentrations from MAIAC EPIC products. We compared the retrieved hematite and goethite concentrations with in situ dust aerosol mineralogical content measurements, as well as with published data. Our data display variations within the published range of hematite, goethite, and iron-oxide mass fractions for pure mineral dust cases. A specific analysis is presented for 15 sites over the main dust source regions. Sites in the central Sahara, Sahel, and Middle East exhibit a greater temporal variability of iron oxides relative to other sites. Niger site(13.52°N, 2.63°E) is dominated by goethite over Harmattan season with median of ~2 weight percentage (wt.%) of iron-oxide. Saudi Arabia site (27.49°N, 41.98°E) over Middle East also exhibited surge of goethite content with the beginning of Shamal season. The Sahel dust is richer in iron-oxide than Saharan and northern China dust except in Summer. The Bodélé Depression area shows a distinctively lower iron-oxide concentration (~1 wt.%) throughout the year. Finally, we show that EPIC data allow to constrain the hematite refractive index. Specifically, we select 5 out of 13 different number of hematite refractive indices widely variable in published laboratory studies by constraining the iron-oxide mass ratio to the known measured values. Provided climatology of hematite and goethite mass fractions across main dust regions of the Earth will be useful for dust shortwave DRE studies and climate modeling.

Sujung Go↗