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DOE OSTI2025

Experimental study of high-energy single-pulse nanosecond discharges in pin-to-pin configuration

Single-pulse pin-to-pin nanosecond pulsed discharges in ambient air (gap distances of 3–7 mm) were investigated at high pulse energies (∼20–30 mJ deposited energy per 11 ns full width at half maximum pulse). A Michelson interferometry setup (532 nm continuous-wave laser) was employed to record time-resolved interferograms of the discharge, enabling spatially resolved calculation of the electron number density. An intensified charge-coupled device camera was used to capture the spatiotemporal evolution of the discharge (streamer formation and spark channel development), and Coherent Anti-Stokes Raman Spectroscopy (CARS) was used to measure post-discharge N 2 vibrational temperatures. Discharge current and voltage were monitored with a back-current shunt. The discharge was initiated with simultaneous cathode-directed and anode-directed streamers that bridge the gap within ∼1 ns and form a luminous, filamentary plasma channel immediately after breakdown. Laser interferometry measurements showed peak electron number densities of the order of 10 1 7–10 18 cm −3 , occurring about 15–20 ns after pulse arrival at the discharge gap. Shorter gap discharges yielded higher peak electron densities, consistent with the higher energy density in the smaller gaps. Spatially, the electron density was highest near the electrodes and decreased toward the midgap region, with 5 and 7 mm gaps exhibiting a pronounced drop in the central channel. CARS indicated initial vibrational temperatures of approximately 4000–6000 K in the spark core of ∼50 ns after the discharge onset, decaying on a ∼500 ns timescale as the plasma cooled and recombined.

Coherent anti-Stokes Raman spectroscopy↗

DOE OSTI2023

Delocalized polaron and Burstein-Moss shift induced by Li in α–V 2 O 5 : A DFT + DMFT study

For this work, we performed density functional theory (DFT)+U and dynamical mean field theory (DMFT) calculations with a continuous-time quantum Monte Carlo impurity solver to investigate the electronic properties of V 2 O 5 and Li x V 2 O 5 (x = 0.125 and 0.25). Pristine V 2 O 5 is a charge-transfer insulator with strong O p–V d hybridization, and it exhibits a large band gap (E gap ) as well as a nonzero conduction-band (CB) gap.We show that the band gap, the number of d electrons of vanadium, N d , and the CB gap for V 2 O 5 obtained from our DMFT calculations are in excellent agreement with the experimental values. While the DFT +U approach replicates the experimental band gap, it overestimates the value of N d and underestimates the CB gap. In the presence of low Li doping, the electronic properties of V 2 O 5 are mainly driven by a polaronic mechanism, and electron spin resonance and electron nuclear double resonance spectroscopies observed the coexistence of free and bound polarons. Notably, our DMFT results identify both polaron types, with the bound polaron being energetically preferred, while the DFT +U method only predicts the free polaron. Our DMFT analysis also reveals that increased Li doping leads to electron filling in the conduction band, shifting the Fermi level. This result is consistent with the observed Burstein-Moss shift upon enhanced Li doping, and we thus demonstrate that the DFT + DMFT approach can be used for an accurate and realistic description of strongly correlated materials.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2024

Multigap nodeless superconductivity in the topological semimetal PdTe

Recently, PdTe was identified as a spin-orbit-coupled topological Dirac semimetal and was claimed to exhibit both bulk-nodal and surface-nodeless superconducting gaps. Here we report on ultra-low-temperature thermal-conductivity measurements on PdTe single crystals with T c = 4.5 K to investigate its superconducting gap structure. It is found that the residual linear term κ 0 /T is negligible in zero magnetic field. Furthermore, the field dependence of κ 0 ⁡(H)/T exhibits an S-shaped curve. These results suggest that PdTe has multiple nodeless superconducting gaps, which is at odds with the claimed bulk-nodal gap. The reason for the discrepancy is likely that previous angle-resolved photoemission spectroscopy measurements were only performed down to 2 K and cannot observe the smaller nodeless gap. As a result, the fully gapped superconducting state in PdTe is compatible with it being a topological superconductor candidate.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2020

Isolating p- and n-Doped Fingers With Intrinsic Poly-Si in Passivated Interdigitated Back Contact Silicon Solar Cells

Polycrystalline silicon on silicon oxide (poly-Si/SiO x ) passivating contacts enable ultra high efficiency interdigitated back contact silicon solar cells. To prevent shunt between n- and p-type doped fingers, an insulating region is required between them. We evaluate the use of intrinsic poly Si for this isolation region. Interdigitated fingers were formed by plasma deposition of doped hydrogenated amorphous silicon through mechanically aligned shadow masks, on top of a full-area intrinsic amorphous silicon layer. High temperature annealing then crystallized the a-Si:H to poly Si and drove in the dopants. Two mechanisms were identified which cause contamination of the intrinsic poly Si gap during processing. During deposition of doped fingers, we show using secondary ion mass spectrometry and conductivity measurements that the intrinsic gap becomes contaminated by doped a-Si:H tails several nanometers thick to concentrations of ~10 20 cm -3 . Another source of contamination occurs during high-temperature annealing, where dopants desorb from doped regions and readsorb onto intrinsic a Si:H. Both pathways reduce the resistivity of the intrinsic gap from ~10 5 Ω·cm to ~10 -1 Ω·cm. We show that plasma etching of the a-Si:H surface before crystallizing with a capping layer can eliminate the contamination of the intrinsic poly-Si, maintaining a resistivity of ~10 5 Ω·cm. Lastly, this demonstrates masked plasma deposition as a dopant patterning method for Si solar cells.

14 SOLAR ENERGY↗

DOE OSTI2025

Participation in and Assessment of the Second DNCSH Public Workshop

The DOE/NRC Criticality Safety for Commercial-Scale HALEU Fuel Cycle and Transportation (DNCSH) project was established through the Inflation Reduction Act of 2022 (H.R. 5376) to support the US Nuclear Regulatory Commission (NRC) and industry in addressing critical experiment validation gaps that impede the licensing basis and regulatory approval of high-assay low-enriched uranium (HALEU) operations. An initial public workshop was held in February 2024 to address HALEU transportation validation gaps. The resulting call for proposals was released in April and resulted in funding for the execution and/or evaluation of 16 critical experiments. A second public workshop was held in August 2025 to address facility and operational validation gaps, precluding a second call for proposals. A list of attendees is provided in APPENDIX A, Table A-1. A total of 319 participants joined the meeting, which was hosted online via Microsoft Teams as well as in person. The slides from the meeting were uploaded online to the NRC’s Agencywide Documents Access and Management System (ADAMS). The meeting agenda is provided in Table 1-1. In preparation for the meeting, a study was performed to examine expected fissile forms for the fuel cycles of various fuel types at different stages of production and the apparent validation gaps. The resulting report, titled “Benchmark Gap Assessment for the Manufacturing of High-Assay Low-Enriched Uranium Fuels,” provided the foundation for the discussions that took place during the workshop. The discussions and the validation gaps in the report were used to develop the second call for proposals. The present report presents the feedback received before, during, and after the second workshop. All the data presented are based on voluntarily self-reported identification, opinions from workshop participants, and survey responses and are assumed to be as accurate as practically reasonable. The discussions during the workshop and the subsequent survey responses were intended to direct attention to industry-specific areas of interest and to collect feedback on the work performed to date by the DNCSH project.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

DOE OSTI2020

Retention of Long-period Gas Giant Planets: Type II Migration Revisited

During their formation, emerging protoplanets tidally interact with their natal disks. Proto–gas giant planets, with Hill radii larger than the disk thickness, open gaps and quench gas flow in the vicinity of their orbits. It is usually assumed that their type II migration is coupled to the viscous evolution of the disk. Although this hypothesis provides an explanation for the origin of close-in planets, it also encounters a predicament on the retention of long-period orbits for most gas giant planets. Moreover, numerical simulations indicate that the planets' migrations are not solely determined by the viscous diffusion of their natal disk. In this work, we carry out a series of hydrodynamic simulations combined with analytic studies to examine the transition between different paradigms of type II migration. We find a range of planetary mass for which gas continues to flow through a severely depleted gap so that the surface density distribution in the disk region beyond the gap is maintained in a quasi-steady state. The associated gap profile modifies the location of corotation and Lindblad resonances. In the proximity of the planet's orbit, high-order Lindblad and corotation torque are weakened by the gas depletion in the gap, while low-order Lindblad torques near the gap walls preserve their magnitude. Consequently, the intrinsic surface density distribution of the disk delicately determines both the pace and direction of the planets' type II migration. We show that this effect might stall the inward migration of giant planets and preserve them in disk regions where the surface density is steep.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2020

Heterogeneous Machine Learning on High Performance Computing for End to End Driving of Autonomous Vehicles

Current artificial intelligence techniques for end to end driving of autonomous vehicles typically rely on a single form of learning or training processes along with a corresponding dataset or simulation environment. Relatively speaking, success has been shown for a variety of learning modalities in which it can be shown that the machine can successfully “drive” a vehicle. However, the realm of real-world driving extends significantly beyond the realm of limited test environments for machine training. This creates an enormous gap in capability between these two realms. With their superior neural network structures and learning capabilities, humans can be easily trained within a short period of time to proceed from limited test environments to real world driving. For machines though, this gap is guarded by at least two challenges: 1) machine learning techniques remain brittle and unable to generalize to a wide range of scenarios, and 2) effective training data that enhances generalization and generates the desired driving behavior. Further, each challenge can be computationally intensive on its own thereby exasperating the gap. Moreover, is has not yet been shown that a single form of learning or training is capable of addressing a large range of scenarios. As a result, solving the first challenge does not inherently solve the second and vice versa. The work described here discusses an approach to address the first challenge that would also provide a foundation for solving the second. Our approach utilizes a combination of conditional imitation learning with a static dataset, reinforcement learning with a simulation environment, and high-performance computing to train a neural network. As a result, this reduces the “time to solution” from to the existing techniques for autonomous driving and provides an extensible framework to address the second key challenge.

autonomous vehicles↗

NASA NTRS1978

Arc-jet test and analysis of Orbiter TPS inter-tile heating in high pressure gradient flow

During entry of the Space Shuttle Orbiter, the convective heating within inter-tile gaps of the Thermal Protection System (TPS) material produces elevated tile sidewall temperatures in regions of high surface pressure gradient. Arc-jet tests have been conducted recently to obtain a measure of the gap heating down the TPS tile sidewalls at test conditions representative of Orbiter flight environments. The object of this paper is to present the gap heating correlations that were developed from a thermal analysis for 3-D curved and flat TPS tile segments. Predictions of gap sidewall temperature were obtained within 30 F of test data on both Wing Glove and Double Wedge models. Derived heating ratios were obtained for a range of test conditions (pressure, pressure gradient, enthalpy, boundary layer thickness, gap width, surface temperature, etc.). The results of the study, which showed that heating ratios varied with the pressure gradient times the square root of the surface pressure, are being used to provide an assessment of gap filler requirements on Orbiter forward fuselage/chine and wing glove regions.

Rochelle, W. C.↗

NASA NTRS1980

A numerical study of the NOL large-scale test

The large-scale gap test was modeled numerically using the reactive hydrodynamics code 2DE with forest fire burn rates. The model gives good agreement between calculated and experimental critical gap values. The calibration of peak pressure in the gap versus gap length is obtained from these calculations, and is in good agreement with the published experiment curve. The two dimensional nature of the gap test is evident from the curvature of the shock wave in the gap and test sample, and from the observed distance of run to detonation in the test samples.

Bowan, A. L.↗

NASA NTRS1988

VLA telemetry performance with concatenated coding for Voyager at Neptune

Current plans for supporting the Voyager encounter at Neptune include the arraying of the Deep Space Network (DSN) antennas at Goldstone, California, with the National Radio Astronomy Observatory's Very Large Array (VLA) in New Mexico. Not designed as a communications antenna, the VLA signal transmission facility suffers a disadvantage in that the received signal is subjected to a gap or blackout period of approximately 1.6 msec once every 5/96 sec control cycle. Previous analyses showed that the VLA data gaps could cause disastrous performance degradation in a VLA stand-alone system and modest degradation when the VLA is arrayed equally with Goldstone. New analysis indicates that the earlier predictions for concatenated code performance were overly pessimistic for most combinations of system parameters, including those of Voyager-VLA. The periodicity of the VLA gap cycle tends to guarantee that all Reed-Solomon codewords will receive an average share of erroneous symbols from the gaps. However, large deterministic fluctuations in the number of gapped symbols from codeword to codeword may occur for certain combinations of code parameters, gap cycle parameters, and data rates. Several mechanisms for causing these fluctuations are identified and analyzed. Even though graceful degradation is predicted for the Voyager-VLA parameters, catastrophic degradation greater than 2 dB can occur for a VLA stand-alone system at certain non-Voyager data rates inside the range of the actual Voyager rates. Thus, it is imperative that all of the Voyager-VLA parameters be very accurately known and precisely controlled.

Dolinar, S. J., Jr.↗

NASA NTRS1991

Tail venting for enhanced yaw damping at spinning conditions

An investigation was conducted in the NASA Langley 20-ft Vertical Spin Tunnel to determine the spin and spin-recovery characteristics of a 1/11-scale model of a low-wing general aviation airplane with a horizontal tail modified with variable-size gaps to allow ventilation of the vertical stabilizer and rudder. Erect spins at symmetric loadings were tested with varying gap sizes on either or both sides of the horizontal tail. The model results indicate that the basic airplane (with no gaps) exhibits a fast, flat spin from which no recoveries can be obtained. The airplane with the modified tail has either a fast, flat spin from which no recoveries or poor recoveries may be made, or a slower, steeper spin from which fair to excellent recoveries may be obtained, depending on the size and orientation of the tail gaps. The major contribution to spin recovery was from the gap on the leeward side of the tail. Gap widths of 15-25 percent of the tail semispan were needed to produce satisfactory recovery from the flat spin.

Stough, H. P., III↗

NASA NTRS1992

Evidence for unseen companions around T Tauri stars

The observed spectral energy distributions of HK Tau, T Tau, and R Y Tau exhibit shallow (but significant) dips at mid-infrared wavelengths. This behavior can be explained by the existence of discrete gaps in their circumstellar disks since, if the temperature in the disks decreases monotonically outward, a gap would result in a range of "missing" temperatures. The gap centers for the three objects occur at radial distances of 0.5, 1.4, and 1.6 AU, respectively, while the corresponding ratios of outer to inner radii of the gaps are 6:1, 7:1, and 15:1, respectively. Larger mid-infrared dips are observed for SU Aur and GM Aur and are interpreted as correspondingly larger gaps, with almost complete clearing of the inner region of the disk in the latter case. The gaps in all cases are consistent with the tidal effects of either companion stars or planets.

Marsh, Kenneth A.↗

NASA NTRS1993

Radial spline assembly for antifriction bearings

An outer race carrier is constructed for receiving an outer race of an antifriction bearing assembly. The carrier in turn is slidably fitted in an opening of a support wall to accommodate slight axial movements of a shaft. A plurality of longitudinal splines on the carrier are disposed to be fitted into matching slots in the opening. A deadband gap is provided between sides of the splines and slots, with a radial gap at ends of the splines and slots and a gap between the splines and slots sized larger than the deadband gap. With this construction, operational distortions (slope) of the support wall are accommodated by the larger radial gaps while the deadband gaps maintain a relatively high springrate of the housing. Additionally, side loads applied to the shaft are distributed between sides of the splines and slots, distributing such loads over a larger surface area than a race carrier of the prior art.

Moore, Jerry H.↗

NASA NTRS1993

Thermally activated retainer means utilizing shape memory alloy

A retainer member suitable for retaining a gap filler placed in gaps between adjacent tile members is presented. One edge of the retainer member may be attached to the gap filler and another edge may be provided with a plurality of tab members which in an intermediate position do not interfere with placement or removal of the gap filler between tile members. The retainer member may be fabricated from a shape memory alloy which when heated to a specified memory temperature will thermally activate the tab members to predetermined memory positions engaging the tile members to retain the gap filler in the gap. This invention has particular application to the thermal tiles on space vehicles such as the Space Shuttle Orbiter.

Grimaldi, Margaret E.↗

NASA NTRS1996

Calculation of tip clearance effects in a transonic compressor rotor

The flow through the tip clearance region of a transonic compressor rotor (NASA rotor 37) was computed and compared to aerodynamic probe and laser anemometer data. Tip clearance effects were modeled both by gridding the clearance gap and by using a simple periodicity model across the ungridded gap. The simple model was run with both the full gap height, and with half the gap height to simulate a vena-contracta effect. Comparisons between computed and measured performance maps and downstream profiles were used to validate the models and to assess the effects of gap height on the simple clearance model. Recommendations were made concerning the use of the simple clearance model. Detailed comparisons were made between the gridded clearance gap solution and the laser anemometer data near the tip at two operating points. The computer results agreed fairly well with the data but overpredicted the extent of the casing separation and underpredicted the wake decay rate. The computations were then used to describe the interaction of the tip vortex, the passage shock, and the casing boundary layer.

Chima, R. V.↗

NASA NTRS1995

Recent Developments in Quantum-Well Infrared Photodetectors

Intrinsic infrared (IR) detectors in the long wavelength range (8-20 Am) are based on an optically excited interband transition, which promotes an electron across the band gap (E(sub g)) from the valence band to the conduction band as shown. These photoelectrons can be collected efficiently, thereby producing a photocurrent in the external circuit. Since the incoming photon has to promote an electron from the valence band to the conduction band, the energy of the photon (h(sub upsilon)) must be higher than the E(sub g) of the photosensitive material. Therefore, the spectral response of the detectors can be controlled by controlling the E(sub g) of the photosensitive material. Examples for such materials are Hg(1-x), Cd(x), Te, and Pb(1-x), Sn(x), Te, in which the energy gap can be controlled by varying x. This means detection of very-long-wavelength IR radiation up to 20 microns requires small band gaps down to 62 meV. It is well known that these low band gap materials, characterized by weak bonding and low melting points, are more difficult to grow and process than large-band gap semiconductors such as GaAs. These difficulties motivate the exploration of utilizing the intersub-band transitions in multiquantum well (MQW) structures made of more refractory large-band gap semiconductors. The idea of using MQW structures to detect IR radiation can be explained by using the basic principles of quantum mechanics. The quantum well is equivalent to the well-known particle in a box problem in quantum mechanics, which can be solved by the time independent Schroudiner equation.

Gunapala, S. D.↗

NASA NTRS1998

Calculation of Tip Clearance Effects in a Transonic Compressor Rotor

The flow through the tip clearance region of a transonic compressor rotor (NASA rotor 37) was computed and compared to aerodynamic probe and laser anemometer data. Tip clearance effects were modeled both by gridding the clearance gap and by using a simple periodicity model across the ungridded gap. The simple model was run with both the full gap height, and with half the gap height to simulate a vena-contracta effect. Comparisons between computed and measured performance maps and downstream profiles were used to validate the models and to assess the effects of gap height on the simple clearance model. Recommendations were made concern- ing the use of the simple clearance model Detailed comparisons were made between the gridded clearance gap solution and the laser anemometer data near the tip at two operating points. The computed results agreed fairly well with the data but overpredicted the extent of the casing separation and underpredicted the wake decay rate. The computations were then used to describe the interaction of the tip vortex, the passage shock, and the casing boundary layer.

Chima, R. V.↗

NASA NTRS2008

Photocatalytic Coatings for Exploration and Spaceport Design

This project developed self-cleaning photocatalytic coatings that remove contamination without human intervention. The coatings chemically remove organic contaminants and leave no residue. The photocatalyst will not negatively affect other coating properties, especially corrosion resistance. Titanium dioxide, TiO2, is an extremely popular photocatalyst because of its chemical stability, nontoxicity, and low cost. TiO2 is commonly used in the photocatalytic oxidation of organic matter or pollutants in the gas and liquid phases. However, TiO2 does have some drawbacks. It has limited light absorption because of its large band-gap and suffers from a photonic efficiency of less than 10 percent for organic degradation. Dopants can lower the band-gap and improve efficiency. Since the photocatalytically active form of TiO2 is a nanocrystalline powder, it can be difficult to make a robust coating with enough catalyst loading to be effective. Photocatalysts become active when certain light energy is absorbed. When photons with an energy greater than the band-gap, Eg, (wavelengths shorter than 400 nm) impinge upon the surface of the TiO2, an electron-hole pair is formed. The electron-hole pair oxidizes adsorbed substances either directly or via reactive intermediates that form on the surface, such as hydroxyl radicals (OH) or superoxide ions (O2-). Several factors can influence the band-gap energy of TiO2, two of which are crystal structure and impurities. TiO2 exists as three crystal structures brookite, anatase, and rutile that can be controlled via heat treatment. Anatase is the most photocatalytically active crystal form of TiO2. Doping TiO2 with impurities can alter its band-gap energy, as well as its effectiveness as a catalyst. Depending on their size, dopant atoms can occupy either the substitutional or interstitial lattice positions. Atoms that are relatively large will assume the interstitial positions and create a much greater energy disturbance in the crystal than will smaller atoms that take on the substitutional positions. This energy disturbance narrows the band-gap and thus allows photons with longer wavelengths and smaller energies (such as those in the visible-light spectrum) to create electron-hole pairs. Raman spectroscopy was performed for the purpose of determining the crystal structure and the degree of crystallinity of the TiO2 particles. Reflectance measurements indicated the wavelengths of light absorbed by the different catalysts.

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