Engineering Papers⌕ Search

SEARCH · Engineering Papers

Results for “Diffuse Scattering”

Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

Quote a phrase for an exact phrase match. Source license links do not imply unrestricted reuse.

At least 1,711 records · Page 95
All sourcesNASA NTRSDOE OSTI
DOE OSTI2012

GLOBAL PROPERTIES OF M31'S STELLAR HALO FROM THE SPLASH SURVEY. I. SURFACE BRIGHTNESS PROFILE

We present the surface brightness profile of M31's stellar halo out to a projected radius of 175 kpc. The surface brightness estimates are based on confirmed samples of M31 red giant branch stars derived from Keck/DEIMOS spectroscopic observations. A set of empirical spectroscopic and photometric M31 membership diagnostics is used to identify and reject foreground and background contaminants. This enables us to trace the stellar halo of M31 to larger projected distances and fainter surface brightnesses than previous photometric studies. The surface brightness profile of M31's halo follows a power law with index -2.2 {+-} 0.2 and extends to a projected distance of at least {approx}175 kpc ({approx}2/3 of M31's virial radius), with no evidence of a downward break at large radii. The best-fit elliptical isophotes have b/a = 0.94 with the major axis of the halo aligned along the minor axis of M31's disk, consistent with a prolate halo, although the data are also consistent with M31's halo having spherical symmetry. The fact that tidal debris features are kinematically cold is used to identify substructure in the spectroscopic fields out to projected radii of 90 kpc and investigate the effect of this substructure on the surface brightness profile. The scatter in the surface brightness profile is reduced when kinematically identified tidal debris features in M31 are statistically subtracted; the remaining profile indicates that a comparatively diffuse stellar component to M31's stellar halo exists to large distances. Beyond 90 kpc, kinematically cold tidal debris features cannot be identified due to small number statistics; nevertheless, the significant field-to-field variation in surface brightness beyond 90 kpc suggests that the outermost region of M31's halo is also comprised to a significant degree of stars stripped from accreted objects.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2016

TIME-DEPENDENT ELECTRON ACCELERATION IN BLAZAR TRANSIENTS: X-RAY TIME LAGS AND SPECTRAL FORMATION

Electromagnetic radiation from blazar jets often displays strong variability, extending from radio to γ -ray frequencies. In a few cases, this variability has been characterized using Fourier time lags, such as those detected in the X-rays from Mrk 421 using Beppo SAX. The lack of a theoretical framework to interpret the data has motivated us to develop a new model for the formation of the X-ray spectrum and the time lags in blazar jets based on a transport equation including terms describing stochastic Fermi acceleration, synchrotron losses, shock acceleration, adiabatic expansion, and spatial diffusion. We derive the exact solution for the Fourier transform of the electron distribution and use it to compute the Fourier transform of the synchrotron radiation spectrum and the associated X-ray time lags. The same theoretical framework is also used to compute the peak flare X-ray spectrum, assuming that a steady-state electron distribution is achieved during the peak of the flare. The model parameters are constrained by comparing the theoretical predictions with the observational data for Mrk 421. The resulting integrated model yields, for the first time, a complete first-principles physical explanation for both the formation of the observed time lags and the shape of the peak flare X-ray spectrum. It also yields direct estimates of the strength of the shock and the stochastic magnetohydrodynamical wave acceleration components in the Mrk 421 jet.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2024

Validating a microphysical prognostic stratospheric aerosol implementation in E3SMv2 using observations after the Mount Pinatubo eruption

Abstract. This paper describes the addition of a stratospheric prognostic aerosol (SPA) capability – developed with the goal of accurately simulating sulfate aerosol formation and evolution in the stratosphere – in the Department of Energy (DOE) Energy Exascale Earth System Model, version 2 (E3SMv2). The implementation includes changes to the four-mode Modal Aerosol Module microphysics in the stratosphere to allow for larger particle growth and more accurate stratospheric aerosol lifetime following the Pinatubo eruption. E3SMv2-SPA reasonably reproduces stratospheric aerosol lifetime, burden, aerosol optical depth, and top-of-atmosphere flux when compared to remote sensing observations. E3SMv2-SPA also has close agreement with the interactive chemistry–climate model CESM2-WACCM (Community Earth System Model version 2–Whole Atmosphere Community Climate Model) – which has a more complete chemical treatment – and the observationally constrained, prescribed volcanic aerosol treatment in E3SMv2. Global stratospheric aerosol size distributions identify the nucleation and growth of sulfate aerosol from volcanically injected SO2 from both major and minor volcanic eruptions from 1991 to 1993. The modeled aerosol effective radius is consistently lower than satellite and in situ measurements (max differences of ∼ 30 %). Comparisons with in situ size distribution samples indicate that this simulated underestimation in both E3SMv2-SPA and CESM2-WACCM is due to overly small accumulation and coarse-mode aerosols 6–18 months post-eruption, with E3SMv2-SPA simulating ∼ 50 % of the coarse-mode geometric mean diameters of observations 11 months post-eruption. Effective radii from the models and observations are used to calculate offline scattering and absorption efficiencies to explore the implications of smaller simulated aerosol size for the Pinatubo climate impacts. Scattering efficiencies at wavelengths of peak solar irradiance (∼ 0.5 µm) are 10 %–80 % higher for daily samples in models relative to observations through 1993, suggesting higher diffuse radiation at the surface and a larger cooling effect in the models due to the smaller simulated aerosol; absorption efficiencies at the peak wavelengths of outgoing terrestrial radiation (∼ 10 µm) are 15 %–40 % lower for daily samples in models relative to observations, suggesting an underestimation in stratospheric heating in the models due to the smaller simulated aerosol. These potential biases are based on aerosol size alone and do not take into account differences in the aerosol number. The overall agreement of E3SMv2-SPA with observations and its similar performance to the well-validated CESM2-WACCM makes E3SMv2-SPA a viable alternative to simulating climate impacts from stratospheric sulfate aerosols.

Brown, Hunter York (ORCID:0000000218147874)↗
NASA NTRS1977

Observations of neutral composition and related ionospheric variations during a magnetic storm in February 1974

The neutral-atmosphere composition experiment on Atmosphere Explorer C measured N2, O, Ar, and He densities during a magnetic storm at altitudes down to about 160 km. At latitudes above 45 deg N, N2 and Ar densities generally increase during the storm, while He and O densities decrease. Below 45 deg N all densities tend to increase during the storm. The density increases at perigee indicate that density- or temperature-profile changes are taking place below 160 km. The return to prestorm conditions is very slow, demonstrating the integrating effect of the atmospheric response. A recent theoretical model incorporating thermospheric circulation and diffusion effects reproduces the longitudinally averaged data, including latitude trends and the asymmetry about the storm maximum. Comparison with the mass-spectrometer and incoherent-scatter empirical model shows qualitative agreement with latitude trends but not with storm asymmetry, while the earlier J71 model based on total mass density is not in agreement with observed latitudinal trends. A close correlation is found between in situ O/N2 measurements and in situ and ground-based ionosonde measurements of electron density.

Hedin, A. E.↗
NASA NTRS1989

Atmospheric correction of high resolution land surface images

Algorithms to correct for atmospheric-scattering effects in high-spatial resolution land-surface images require the ability to perform rapid and accurate computations of the top-of-atmosphere diffuse radiance field for arbitrarily general surface reflectance distributions (which may be both heterogeneous and non-Lambertian) and atmospheric models. Using three-dimensional radiative transfer (3DRT) theory algorithms are being developed. The methodology used to perform the 3DRT calculations is described. It is shown how these calculations are used to perform atmospheric corrections, and the sensitivity of the retrieved surface reflectances to atmospheric structural parameters is illustrated.

Diner, D. J.↗
NASA NTRS1993

Ignition and combustion characteristics of metallized propellants

Experimental and analytical investigations focusing on secondary atomization and ignition characteristics of aluminum/liquid hydrocarbon slurry propellants were conducted. Experimental efforts included the application of a laser-based, two-color, forward-scatter technique to simultaneously measure free-flying slurry droplet diameters and velocities for droplet diameters in the range of 10-200 microns. A multi-diffusion flame burner was used to create a high-temperature environment into which a dilute stream of slurry droplets could be introduced. Narrowband measurements of radiant emission were used to determine if ignition of the aluminum in the slurry droplet had occurred. Models of slurry droplet shell formation were applied to aluminum/liquid hydrocarbon propellants and used to ascertain the effects of solids loading and ultimate particle size on the minimum droplet diameter that will permit secondary atomization. For a 60 weight-percent Al slurry, the limiting critical diameter was predicted to be 34.7 microns which is somewhat greater than the 20-25 micron limiting diameters determined in the experiments. A previously developed model of aluminum ignition in a slurry droplet was applied to the present experiments and found to predict ignition times in reasonable agreement with experimental measurements. A model was also developed that predicts the mechanical stress in the droplet shell and a parametric study was conducted. A one-dimensional model of a slurry-fueled rocket combustion chamber was developed. This model includes the processes of liquid hydrocarbon burnout, secondary atomization, aluminum ignition, and aluminum combustion. Also included is a model for radiant heat transfer from the hot aluminum oxide particles to the chamber walls. Exercising this model shows that only a modest amount of secondary atomization is required to reduce residence times for aluminum burnout, and thereby maintain relatively short chamber lengths. The model also predicts radiant heat transfer losses to the walls to be only approximately 3 percent of the fuel energy supplied. Additional work is required to determine the effects of secondary atomization on two-phase losses in the nozzle.

Turns, Stephen R.↗
NASA NTRS1993

Access to Japanese aerospace-related scientific and technical information: The NASA Aerospace Database

With Japan's growing R&D strength in aerospace-related fields, it is increasingly important for U.S. researchers to be aware of Japanese advances. However, several factors make it difficult to do so. After reviewing the diffusion of aerospace STI in Japan, four factors which make it difficult for U.S. researchers to gather this information are discussed: language, the human network, information scatter, and document acquisition. NASA activities to alleviate these difficulties are described, beginning with a general overview of the NASA STI Program. The effects of the new National Level Agreement between NASA and NASDA are discussed.

Hoetker, Glenn P.↗
NASA NTRS1996

A New Generation Fiber Optic Probe: Characterization of Biological Fluids, Protein Crystals and Ophthalmic Diseases

A new fiber optic probe developed for determining transport properties of sub-micron particles in fluids experiments in a microgravity environment has been applied to characterize particulate dispersions/suspensions in various challenging environments which have been hitherto impossible. The probe positioned in front of a sample delivers a low power light (few nW - 3mW) from a laser and guides the light which is back scattered by the suspended particles through a receiving optical fiber to a photo detector and to a digital correlator. The probe provides rapid determination of macromolecular diffusivities and their respective size distributions. It has been applied to characterize various biological fluids, protein crystals, and ophthalmic diseases.

Ansari, Rafat R.↗
NASA NTRS2001

Turbulent Flame Processes Via Diffusion Flame-Vortex Ring Interactions

Flame-vortex interactions are canonical configurations that can be used to study the underlying processes occurring in turbulent reacting flows. This configuration contains many of the fundamental aspects of the coupling between fluid dynamics and combustion that could be investigated with more controllable conditions than are possible under direct investigations of turbulent flames. Diffusion flame-vortex ring interaction contains many of the fundamental elements of flow, transport, combustion, and soot processes found in turbulent diffusion flames. Some of these elements include concentrated vorticity, entrainment and mixing, strain and nonequilibrium phenomena, diffusion and differential diffusion, partial premixing and diluent effects, soot formation and oxidation, and heat release effects. Such simplified flowfield allows the complex processes to be examined more closely and yet preserving the physical processes present in turbulent reacting flows. Furthermore, experimental results from the study of flame-vortex interactions are useful for the validation of numerical simulations and more importantly to deepen our understanding of the fundamental processes present in reacting flows. Experimental and numerical results obtained under microgravity conditions of the diffusion flame-vortex ring interaction are summarized in this paper. Results are obtained using techniques that include Flame Luminosity Imaging (FLI), Laser Soot-Mie Scattering (LSMS), Computational Fluid Dynamics and Combustion (CFDC), and Diode Laser Spectroscopy/Iterative Temperature with Assumed Chemistry (DLS/ITAC).

Dahm, Werner J. A.↗
NASA NTRS2010

Simultaneous Retrieval of Aerosol and Surface Optical Properties from Combined Airborne- and Ground-Based Direct and Diffuse Radiometric Measurements

This paper presents a new method for simultaneously retrieving aerosol and surface reflectance properties from combined airborne and ground-based direct and diffuse radiometric measurements. The method is based on the standard Aerosol Robotic Network (AERONET) method for retrieving aerosol size distribution, complex index of refraction, and single scattering albedo, but modified to retrieve aerosol properties in two layers, below and above the aircraft, and parameters on surface optical properties from combined datasets (Cloud Absorption Radiometer (CAR) and AERONET data). A key advantage of this method is the inversion of all available spectral and angular data at the same time, while accounting for the influence of noise in the inversion procedure using statistical optimization. The wide spectral (0.34-2.30 m) and angular range (180 ) of the CAR instrument, combined with observations from an AERONET sunphotometer, provide sufficient measurement constraints for characterizing aerosol and surface properties with minimal assumptions. The robustness of the method was tested on observations made during four different field campaigns: (a) the Southern African Regional Science Initiative 2000 over Mongu, Zambia, (b) the Intercontinental Transport Experiment-Phase B over Mexico City, Mexico (c) Cloud and Land Surface Interaction Campaign over the Atmospheric Radiation Measurement (ARM) Central Facility, Oklahoma, USA, and (d) the Arctic Research of the Composition of the Troposphere from Aircraft and Satellites (ARCTAS) over Elson Lagoon in Barrow, Alaska, USA. The four areas are dominated by different surface characteristics and aerosol types, and therefore provide good test cases for the new inversion method.

Gatebe, C. K.↗
DOE OSTI2016

TWO-DIMENSIONAL CORE-COLLAPSE SUPERNOVA SIMULATIONS WITH THE ISOTROPIC DIFFUSION SOURCE APPROXIMATION FOR NEUTRINO TRANSPORT

The neutrino mechanism of core-collapse supernova is investigated via non-relativistic, two-dimensional (2D), neutrino radiation–hydrodynamic simulations. For the transport of electron flavor neutrinos, we use the interaction rates defined by Bruenn and the isotropic diffusion source approximation (IDSA) scheme, which decomposes the transported particles into trapped-particle and streaming-particle components. Heavy neutrinos are described by a leakage scheme. Unlike the “ray-by-ray” approach in some other multidimensional supernova models, we use cylindrical coordinates and solve the trapped-particle component in multiple dimensions, improving the proto-neutron star resolution and the neutrino transport in angular and temporal directions. We provide an IDSA verification by performing one-dimensional (1D) and 2D simulations with 15 and 20 M{sub ⊙} progenitors from Woosley et al. and discuss the difference between our IDSA results and those existing in the literature. Additionally, we perform Newtonian 1D and 2D simulations from prebounce core collapse to several hundred milliseconds postbounce with 11, 15, 21, and 27 M{sub ⊙} progenitors from Woosley et al. with the HS(DD2) equation of state. General-relativistic effects are neglected. We obtain robust explosions with diagnostic energies E{sub dia} ≳ 0.1–0.5 B (1 B ≡ 10{sup 51} erg) for all considered 2D models within approximately 100–300 ms after bounce and find that explosions are mostly dominated by the neutrino-driven convection, although standing accretion shock instabilities are observed as well. We also find that the level of electron deleptonization during collapse dramatically affects the postbounce evolution, e.g., the neglect of neutrino–electron scattering during collapse will lead to a stronger explosion.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2019

fPINNs: Fractional Physics-Informed Neural Networks

Physics-informed neural networks (PINNs), introduced, are effective in solving integer-order partial differential equations (PDEs) based on scattered and noisy data. PINNs employ standard feedforward neural networks (NNs) with the PDEs explicitly encoded into the NN using automatic differentiation, while the sum of the mean-squared PDE residuals and the mean-squared error in initial-boundary conditions is minimized with respect to the NN parameters. Here we extend PINNs to fractional PINNs (fPINNs) to solve space-time fractional advection-diffusion equations (fractional ADEs), and we study systematically their convergence, hence explaining both fPINNs and PINNs for the first time. Specifically, we demonstrate their accuracy and effectiveness in solving multidimensional forward and inverse problems with forcing terms whose values are only known at randomly scattered spatio-temporal coordinates (black-box (BB) forcing terms). A novel element of the fPINNs is the hybrid approach that we introduce for constructing the residual in the loss function using both automatic differentiation for the integer-order operators and numerical discretization for the fractional operators. This approach bypasses the difficulties stemming from the fact that automatic differentiation is not applicable to fractional operators because the standard chain rule in integer calculus is not valid in fractional calculus. To discretize the fractional operators, we employ the Grünwald--Letnikov (GL) formula in one-dimensional fractional ADEs and the vector GL formula in conjunction with the directional fractional Laplacian in two- and three-dimensional fractional ADEs. We first consider the one-dimensional fractional Poisson equation and compare the convergence of the fPINNs against the finite difference method (FDM). We present the solution convergence using both the mean L 2 error as well as the standard deviation due to sensitivity to NN parameter initializations. Using different GL formulas we observe first-, second-, and third-order convergence rates for small size training sets but the error saturates for larger training sets. We explain these results by analyzing the four sources of numerical errors due to discretization, sampling, NN approximation, and optimization. The total error decays monotonically (below 10 –5 for a third-order GL formula) but it saturates beyond that point due to the optimization error. We also analyze the relative balance between discretization and sampling errors and observe that the sampling size and the number of discretization points (auxiliary points) should be comparable to achieve the highest accuracy. As we increase the depth of the NN up to certain value, the mean error decreases and the standard deviation increases, whereas the width has essentially no effect unless its value is either too small or too large. We next consider time-dependent fractional ADEs and compare white-box (WB) and BB forcing. We observe that for the WB forcing, our results are similar to the aforementioned cases; however, for the BB forcing fPINNs outperform FDM. Subsequently, we consider multidimensional time-, space-, and space-time-fractional ADEs using the directional fractional Laplacian and we observe relative errors of 10 –3 ~ 10 –4 . Lastly, we solve several inverse problems in one, two, and three dimensions to identify the fractional orders, diffusion coefficients, and transport velocities and obtain accurate results given proper initializations even in the presence of significant noise.

97 MATHEMATICS AND COMPUTING↗
DOE OSTI2021

Scattering by whistler-mode waves during a quiet period perturbed by substorm activity

We study the dynamics of radiation belt electrons during a 10-day quiet period perturbed by substorm activity and preceding a high-speed stream (HSS), aiming at a global description of the radiation belts in L-shell, L in [2, 6], and energy [0.1, 10] MeV. We combine Van Allen Probes observations and Fokker-Planck numerical simulations of pitch-angle diffusion. The Fokker-Planck model uses event-driven pitch angle diffusion coefficients from whistler-mode waves, built from the wave properties and the ambient plasma density measurements from the Van Allen Probes. We first find this event has some similar characteristics to regular quiet times previously studied; a widely extended plasmasphere within which we observe strong and varying whistler-mode waves. These ambient conditions lead to strong pitch-angle scattering, which contributes to the creation of a wide slot region as well as a significant decay of the outer radiation belts, which are observed and qualitatively well simulated. In addition, we find the substorm activity causes short duration (within ± 4h) decay of the plasma density and a lowering amplitude of the whistler-mode waves within the plasmasphere, both causing opposite effects in terms of pitch angle diffusion. This leads to a diminution of pitch-angle diffusion at the time of the main substorm activity. Conversely, whistler-mode waves become enhanced in the time periods between the substorm injections. All effects cumulated, we find an enhancement of pitch angle diffusion by whistler-mode waves above L~4.7 during the 10-day period. This directly relates to the combination of quietness and substorm activity which allows pitch angle diffusing of up to 1 MeV electrons in the outer belt. Relativistic electrons of 1–2 MeV remain trapped in the outer belt, from L~4.7 to L~5.2, forming, in both the observations and the simulations, a distinct pocket of remnant electrons.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2017

X-Ray Studies of the Extended TeV Gamma-Ray Source VER J2019+368

This article reports the results of X-ray studies of the extended TeV γ-ray source VER J2019+368. Suzaku observations conducted to examine properties of the X-ray pulsar wind nebula (PWN) around PSR J2021+3651 revealed that the western region of the X-ray PWN has a source extent of 15{sup ′}×10{sup ′} with the major axis oriented to that of the TeV emission. The PWN-west spectrum was closely fitted by a power law for absorption at N(H)=(8.2{sub −1.1}{sup +1.3})×10{sup 21} cm{sup −2} and a photon index of Γ=2.05±0.12, with no obvious change in the index within the X-ray PWN. The measured X-ray absorption indicates that the distance to the source is much less than the 10 kpc inferred by radio data. Aside from the PWN, no extended emission was observed around PSR J2021+3651 even by Suzaku. Archival data from the XMM-Newton were also analyzed to complement the Suzaku observations, indicating that the eastern region of the X-ray PWN has a similar spectrum (N(H)=(7.5±0.9)×10{sup 21} cm{sup −2} and Γ=2.03±0.10) and source extent up to at least 12{sup ′} along the major axis. The lack of significant change in the photon index and the source extent in X-ray are used to constrain the advection velocity or the diffusion coefficient for accelerated X-ray-producing electrons. A mean magnetic field of ∼3 μG is required to account for the measured X-ray spectrum and reported TeV γ-ray spectrum. A model calculation of synchrotron radiation and inverse Compton scattering was able to explain ∼80% of the reported TeV flux, indicating that the X-ray PWN is a major contributor of VER J2019+368.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2025

Detection of atomic oxygen and its electronic coherence decays using time-resolved ultrafast coherent Raman scattering

We report the detection of atomic oxygen and quantitative measurements of its electronic Raman coherence decays in flames and low-temperature plasmas using time-resolved hybrid femtosecond/picosecond coherent anti-Stokes Raman scattering (CARS). Atomic oxygen was detected using the Raman transitions between the spin–orbit coupled triplet ground states. Atomic oxygen was generated in an H 2 /O 2 /Ar diffusion flame and an O 2 /Ar pulsed plasma discharge. Single exponential decays were observed for the O( 3 P 2 )–O( 3 P 1 ) Raman transition at 158.3 cm −1 and the O( 3 P 2 )–O( 3 P 0 ) Raman transition at 227 cm −1 . From the decay measurements, the atomic O Raman linewidths were obtained from 25 to 150 Torr in non-equilibrium plasma and at 760 Torr in a flame. Enhanced signal-to-noise ratios (SNRs) of atomic oxygen and atomic to molecular oxygen signal contrasts were obtained by taking advantage of electronic triplet coherence beating. Enhancement of up to seven times in the atomic O SNR was observed. Furthermore, we also found that the dephasing rates of O 2 (v = 0–3, N = 37) were similar, which provides evidence for the assumption that vibrational excitation does not influence the dephasing of diatomic molecular rotational CARS transitions.

Atomic and molecular spectroscopy↗
DOE OSTI2021

Realization of a high luminosity muon beam at the Jefferson Lab

The proton is the major component of the visible matter of our universe, so being able to determine its fundamental properties, such as its charge radius, is of vital importance. In recent years, several experiments have been performed for the accurate measurement of the proton radius with different experimental techniques. The main and most common are based on two different techniques: ep scattering and Lamb shift spectroscopy of regular hydrogen atoms. The latter can also be performed on muonic hydrogen atoms with a significant improvement in accuracy. Recent measurements that use this method have highlighted a discrepancy between the results obtained with the diffusion of electrons and those obtained with the spectroscopic technique leading to the so-called ?proton radius puzzle?. The explanation of why this difference between the measured values exists is still a matter of discussion. The last attempt to address the puzzle was the PRad Experiment. It was performed with a unique experimental setup that gave the scientists an excellent control on the systematic errors that are usually present in electron-proton scattering experiments. This has significantly increased the precision of the measurement, bringing it in the same area as the spectroscopic ones done on muonic hydrogen atoms, which are considered the most precise. However, to solve the puzzle once and for all, even more precise electron scattering measurements are needed. Alternatively, new methods can be used, such as eg. muon-proton scattering at low transferred momenta in order to lower the systematic errors that comes with the measurement. This thesis tries to address this problem by studying the set up of an intense muon beam at the Jefferson Laboratory (JLab) that can be used to carry out a high-precision m ? p scattering experiment. Using Montecarlo simulations I studied the muon production resulting from the interaction of the primary electron beam with the beam-dump at JLab Hall-A. The simulations were performed using the FLUKA package via the FLAIR graphical interface. In this study, I modified an existing geometry (built for the ?Beam Dump eXperiment?) and performed several studies in order to optimize the muon beam parameters. In order to estimate the beam intensity, I studied the muon generation and transportation through the concrete bunker surrounding the Hall-A beam-dump. Detailed studies on muon attenuation and dispersion at different depth allowed me to track the beam profile in space and momentum as a function of the distance from the beam-dump. Last, but not least, I studied a possible tagging system for the muon beam. The tagging system will allow us to know with good precision (O(1=1000)) the energy of each muon of the beam. Based on the results obtained, I created an event generator that incorporates the detailed description of the muon beam (energy, position, emittance) useful to define and optimize the experimental setup for a future measurement of the proton radius at the JLab.

Fulci, Antonino↗
DOE OSTI2014

Dynamics of Block Copolymer Nanocomposites

A detailed study of the dynamics of cadmium sulfide nanoparticles suspended in polystyrene homopolymer matrices was carried out using X-ray photon correlation spectroscopy for temperatures between 120 and 180 °C. For low molecular weight polystyrene homopolymers, the observed dynamics show a crossover from diffusive to hyper-diffusive behavior with decreasing temperatures. For higher molecular weight polystyrene, the nanoparticle dynamics appear hyper-diffusive at all temperatures studied. The relaxation time and characteristic velocity determined from the measured hyper-diffusive dynamics reveal that the activation energy and underlying forces determined are on the order of 2.14 × 10 -19 J and 87 pN, respectively. We also carried out a detailed X-ray scattering study of the static and dynamic behavior of a styrene– isoprene diblock copolymer melt with a styrene volume fraction of 0.3468. At 115 and 120 °C, we observe splitting of the principal Bragg peak, which we attribute to phase coexistence of hexagonal cylindrical and cubic double- gyroid structure. In the disordered phase, above 130 °C, we have characterized the dynamics of composition fluctuations via X-ray photon correlation spectroscopy. Near the peak of the static structure factor, these fluctuations show stretched-exponential relaxations, characterized by a stretching exponent of about 0.36 for a range of temperatures immediately above the MST. The corresponding characteristic relaxation times vary exponentially with temperature, changing by a factor of 2 for each 2 °C change in temperature. At low wavevectors, the measured relaxations are diffusive with relaxation times that change by a factor of 2 for each 8 °C change in temperature.

36 MATERIALS SCIENCE↗
DOE OSTI2025

Microstructurally informed synchrotron x-ray analysis revealing helium defect transitions in ultrafine grained tungsten

The formation of insoluble gaseous defects in materials due to nuclear transmutation or ion implantation involves the diffusion of impurity atoms to form atomic defect clusters that coalesce into bubbles or cavities and ultimately degrade the material properties. Transmission electron microscopy (TEM) is limited in its ability to resolve sub-nanometer gas clusters whereas X-ray diffraction (XRD) provides information pertaining to local atomic changes. Here, in this study, helium (He) implanted ultrafine grained tungsten is explored through a multimodal defect characterization campaign combining TEM-informed Small Angle X-ray Scattering (SAXS) analysis, XRD lattice parameter measurements, and nanoscale He cluster quantification from a region of reciprocal space accessible via Wide Angle X-ray Scattering (WAXS). Moderate elevated temperature implantations are shown to produce high concentrations of sub-nanoscale He clusters and small, homogeneously distributed cavities, which collectively are linked to lattice expansion and further substantiated through complementary atomistic simulations. Increased implantation temperatures encourage the diffusion of these defects to the grain boundaries (GBs), leading to lattice relaxation and the growth of large GB cavities manifesting as bimodal size distributions in the SAXS analysis. Overall, our results demonstrate the utility of multimodal synchrotron X-ray analysis in bridging the gap between microscale He cavity quantification and atomic-scale defect analysis.

36 MATERIALS SCIENCE↗