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At least 1,693 records · Page 94
All sourcesNASA NTRSDOE OSTI
DOE OSTI2015

Push or Pull? Proton Responsive Ligand Effects in Rhenium Tricarbonyl CO 2 Reduction Catalysts

Proton responsive ligands offer control of catalytic reactions through modulation of pH-dependent properties, second coordination sphere stabilization of transition states, or by providing a local proton source for multi-proton, multi-electron reactions. Two fac -[ReI(α-diimine)(CO)₃Cl] complexes with α-diimine = 4,4'- (or 6,6'-) dihydroxy-2,2'-bipyridine (4DHBP and 6DHBP) have been prepared and analyzed as electrocatalysts for reduction of carbon dioxide. Consecutive electrochemical reduction of these complexes yields species identical to those obtained by chemical deprotonation. An energetically feasible mechanism for reductive deprotonation is proposed in which the bpy anion is protonated followed by loss of H₂ and 2H⁺. Cyclic voltammetry reveals a two-electron, three-wave system owing to competing EEC and ECE pathways. The chemical step of the ECE pathway might be attributed to the reductive deprotonation. but cannot be distinguished from chloride dissociation. The rate obtained by digital simulation is approximately 8 s⁻¹. Under CO₂, these competing reactions generate a two-slope catalytic waveform with onset potential of –1.65 V vs Ag/AgCl. Reduction of CO₂ to CO by the [ReI (4DHBP–2H⁺)(CO)₃]⁻ suggests the interaction of CO₂ with the deprotonated species or a third reduction followed by catalysis. Conversely, the reduced form of [Re(6DHBP)(CO)₃Cl] converts CO₂ to CO with a single turnover.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2018

Subsurface Structure of Long Valley Caldera Imaged With Seismic Scattering and Intrinsic Attenuation

Here we image seismic intrinsic (Q i -1 ) and scattering (Q s -1 ) attenuations in Long Valley Caldera, California, by analyzing more than 1,700 vertical component waveforms from local earthquakes. Observed energy envelopes are fit to the diffusion model and seismic attenuation images are produced using two-dimensional space weighting functions. Low intrinsic and low scattering attenuation anomalies in the center south of the caldera correspond to the location of an earthquake swarm in 2014. We identify high intrinsic and high scattering attenuation anomalies in the fluid-rich western and eastern areas of the caldera. From a comparison with other geophysical images (magnetotellurics and seismic tomography) we attribute these anomalies to a hydrothermal system (high attenuation). Average to high attenuation values are also observed at the adjacent Mammoth Mountain (southwest of the caldera) and may also have a hydrothermal origin. High intrinsic attenuation at low frequencies to the west of the Hartley Springs Fault may be produced by the magmatic system that produced the Inyo Craters. Finally, seismic attenuation imaging provides insights into subsurface structures that are complementary to velocity and conductivity images.

58 GEOSCIENCES↗
DOE OSTI2018

Relocation of Light and Moderate-Magnitude ( M 4-6) Seismicity Along the Central Mid-Atlantic

In this study, we estimate precise relative epicentroid locations of earthquakes along the Mid-Atlantic Ridge (MAR) between 12°N and 19°N using intermediate-period Rayleigh and Love wave cross-correlation measurements. We relocate 152 earthquakes with magnitudes ranging between 4.0 and 6.0 and when possible use P waveform modeling to estimate centroid depths. We compare surface-wave locations to locations in the U.S. Geological Survey, Global Centroid Moment Tensor, and Pacific Marine Environmental Laboratory hydroacoustic catalogs (Smith et al., 2002, https://doi.org/10.1029/2001GL013912) and demonstrate that surface-wave based relative location techniques provide significant improvement on precision. Our analyses shift locations to more tectonically consistent alignments that correlate strongly with bathymetric features. Relocations along the Fifteen-Twenty and Marathon Fracture Zones (FZs) move to within a few kilometers of the transform bathymetry. Events along ridge segments scatter over a distance of about 10–20 km perpendicular to the local plate boundary and most ridge-segment seismicity clusters spatially. North of the Fifteen-Twenty FZ, ridge events along several segments locate preferentially in the North American Plate, suggesting recent asymmetric seismic strain release and perhaps asymmetric spreading. Along the ridge between 13°N and 14°N, moderate-magnitude seismic strain release concentrates in an area with two active oceanic core complexes (OCC) along the western rift boundary, but the largest events along this segment appear to occur along the eastern boundary rift valley faults and represent deformation opposite the OCC detachment surface processes. Finally, precise moderate-magnitude earthquake epicentroid locations for events that occurred over the last few decades complement the results of temporary seismometer deployments that have imaged microseismic activity along the MAR.

58 GEOSCIENCES↗
DOE OSTI2018

Detecting lightning infrasound using a high-altitude balloon

Acoustic waves with a wide range of frequencies are generated by lightning strokes during thunderstorms, including infrasonic waves (0.1 to 20 Hz). The source mechanism for these low frequency acoustic waves is still debated and studies have so far been limited to ground–based instruments. Here we report the first confirmed detection of lightning generated infrasound with acoustic instruments suspended at stratospheric altitudes using a free–flying balloon. We observe high–amplitude signals generated by lightning strokes located within 100 km of the balloon as it flew over the Tasman Sea on 17 May 2016. The signals share many characteristics with waveforms recorded previously by ground–based instruments near thunderstorms. The ability to measure lightning activity with high–altitude infrasound instruments has demonstrated the potential for using these platforms to image the full acoustic wavefield in the atmosphere. In conclusion, it validates the use of these platforms for recording and characterizing infrasonic sources located beyond the detection range of ground–based instruments.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2019

The Potential of DAS in Teleseismic Studies: Insights From the Goldstone Experiment

Distributed acoustic sensing (DAS) is a recently developed technique that has demonstrated its utility in the oil and gas industry. Here we demonstrate the potential of DAS in teleseismic studies using the Goldstone OpticaL Fiber Seismic experiment in Goldstone, California. By analyzing teleseismic waveforms from the 10 January 2018 M7.5 Honduras earthquake recorded on ~5,000 DAS channels and the nearby broadband station GSC, we first compute receiver functions for DAS channels using the vertical-component GSC velocity as an approximation for the incident source wavelet. The Moho P -to- s conversions are clearly visible on DAS receiver functions. Here, we then derive meter-scale arrival time measurements along the entire 20-km-long array. We are also able to measure path-averaged Rayleigh wave group velocity and local Rayleigh wave phase velocity. The latter, however, has large uncertainties. Our study suggests that DAS will likely play an important role in many fields of passive seismology in the near future.

58 GEOSCIENCES↗
DOE OSTI2018

Properties of Intense Field-Aligned Lower-Band Chorus Waves: Implications for Nonlinear Wave-Particle Interactions: INTENSE FIELD-ALIGNED CHORUS WAVE-PACKETS

Resonant interactions between electrons and chorus waves are responsible for a wide range of phenomena in near-Earth space (e.g., diffuse aurora and acceleration of > 1 MeV electrons). Although quasi-linear diffusion is believed to be the primary paradigm for describing such interactions, an increasing number of investigations suggest that nonlinear effects are also important in controlling the rapid dynamics of electrons. However, present models of nonlinear wave-particle interactions, which have been successfully used to describe individual short-term events, are not directly applicable for a statistical evaluation of nonlinear effects and the long-term dynamics of the outer radiation belt, because they lack information on the properties of intense (nonlinearly resonating with electrons) chorus waves. In this paper, we use the Time History of Events and Macroscale Interactions during Substorms and Van Allen Probes data sets of field-aligned chorus waveforms to study two key characteristics of these waves: effective amplitude Β w (nonlinear interaction can occur when Β w >2) and wave packet length β (the number of wave periods within it). While as many as 10–15% of chorus wave packets are sufficiently intense (Β w >2–3) to interact nonlinearly with relativistic electrons, most of them are short (β < 10) reducing the efficacy of such interactions. Revised models of nonlinear interactions are thus needed to account for the long-term effects of these common, intense but short chorus wave packets. We also discuss the dependence of Β w , β on location (MLT and L-shell) and on the properties of the suprathermal electron population.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2020

Probing Slow Earthquakes With Deep Learning

Abstract Slow earthquakes may trigger failure on neighboring locked faults that are stressed sufficiently to break, and slow slip patterns may evolve before a nearby great earthquake. However, even in the clearest cases such as Cascadia, slow earthquakes and associated tremor have only been observed in intermittent and discrete bursts. By training a convolutional neural network to detect known tremor on a single seismic station in Cascadia, we isolate and identify tremor and slip preceding and following known larger slow events. The deep neural network can be used for the detection of quasi‐continuous tremor, providing a proxy that quantifies the slow slip rate. Furthermore, the model trained in Cascadia recognizes tremor in other subduction zones and also along the San Andreas Fault at Parkfield, suggesting a universality of waveform characteristics and source processes, as posited from experiments and theory.

58 GEOSCIENCES↗
DOE OSTI2019

Modeling Frequency–Independent Q Viscoacoustic Wave Propagation in Heterogeneous Media

Quantifying the attenuation of seismic waves propagating in the Earth interior is critical to study the subsurface structure. Previous studies have proposed fractional anelastic wave equations to model the frequency–independent Q seismic wave propagation. Such wave equations involve fractional derivatives that pose computational challenges for the numerical schemes in terms of accuracy and efficiency when dealing with heterogeneous Earth media. To tackle these challenges, here we derive a new viscoacoustic wave equation, where the power terms of the fractional Laplacian operators are spatially independent, thus accurate and efficient methods (e.g., the Fourier pseudospectral method) can be adopted. Our derivation enables the resultant equation to capture both amplitude and phase signatures of the anelastic wave propagation by matching the complex wave numbers for all the frequencies of interest. We verify the derivation by comparing the dispersion curves of both the attenuation factor and the phase velocity produced by the new wave equation with their theoretical values as well as the Pierre Shale in situ measurements. Following that, we use a synthetic attenuating gas chimney model to demonstrate the attenuation effects on seismic waveforms and then construct the Q–compensated reverse time migration to undo these effects for seismic image enhancement. Finally, we find that our forward modeling results can characterize the spatiotemporal attenuation effects revealed in the Frio–II CO2 injection time–lapse seismic monitoring data. Here, we expect this proposed equation to be useful to quantify the attenuation in seismic data to push the resolution limits of seismic imaging and inversion.

25 ENERGY STORAGE↗
DOE OSTI2020

A Retrospective of Findings From the FORTE Satellite Mission

We revisit the findings from the FORTE satellite program (1997–2004), which collected optical imaging of lightning as well as optical and radio frequency time series waveforms globally from low-earth-orbit. These include surveys of the earth's radio frequency anthropogenic noise environment; earth surface reflectivity at radio frequencies; a scheme for classifying lightning discharge types on the basis of their very high frequency time domain power envelope; insights into the polarization and radiation pattern characteristics of different lightning types, with implications for the underlying discharge processes; and estimates of cloud optical properties based on the statistics of scattered light. Most significantly, FORTE was uniquely suited to capture large samples of data from the rare discharge known as “narrow bipolar events,” enabling detailed examination of their basic characteristics and confirming that they appear to result from fundamentally distinct physical processes compared to other lightning. In particular, despite representing huge charge transfer they evidently produce little-to-no light output.

47 OTHER INSTRUMENTATION↗
DOE OSTI2021

Dynamic Earthquake Triggering in Southern California in High Resolution: Intensity, Time Decay, and Regional Variability

Abstract Earthquake triggering by seismic waves has been recognized as a phenomenon for nearly 30 years. However, our ability to study dynamic triggering has been limited by our ability to capture the triggering stresses accurately and record the resultant earthquakes. Here we use full waveforms from a dense seismic network and a modern, high‐resolution seismic catalog to measure triggering in Southern California from 2008 to 2017 based on interevent time ratios. We find that the fractional seismicity rate change, which we term triggering intensity or triggerability, as a function of peak strain change for the period of ∼20 s due to distant earthquakes is monotonically increasing and compatible with earlier measurements made with a disjoint data set from 1984 to 2008. A triggering strain of 1 microstrain is equivalent to the local productivity generated by an M 1.8 earthquakes. This result implies that a prediction of seismicity rate changes can be made based on recorded ground shaking using the same formalism as currently used for aftershock prediction. For a teleseismic event, this small level of triggering occurs throughout the region and thus aggregates to a regional effect. We find that the triggering rate decays after the triggerer follows an Omori‐Utsu law, but at a much slower rate than a typical aftershock sequence. The slow decay rate suggests that an ancillary process such as creep or fluid flow must be part of dynamic triggering. The prevalence of triggering in areas of creep or fluid involvement reinforces this inference. A triggering cascade of secondary earthquakes is insufficient to explain the data.

Miyazawa, Masatoshi↗
DOE OSTI2020

Machine-Learning-Based Analysis of the Guy-Greenbrier, Arkansas Earthquakes: A Tale of Two Sequences

Here, we revisited the June 2010 to October 2011 Guy-Greenbrier earthquake sequence in central Arkansas using PhaseNet, a deep neural network trained to pick P and S arrival times. We applied PhaseNet to continuous waveform data and used phase association and hypocenter relocation to locate nearly 90,000 events. Our catalog suggests that the sequence consists of two adjacent earthquake sequences on the same fault and that the second sequence may be associated with the wastewater disposal well to the west of the Guy-Greenbrier Fault, rather than the wells to the north and the east that were previously implicated. We find that each sequence is composed of many small clusters that exhibit diffusion along the fault at shorter timescales. Our study demonstrates that machine-learning-based earthquake catalog development is now feasible and will yield new insights into earthquake behavior.

58 GEOSCIENCES↗
DOE OSTI2020

The Spatiotemporal Evolution of Granular Microslip Precursors to Laboratory Earthquakes

Laboratory earthquake experiments provide important observational constraints for our understanding of earthquake physics. Here we leverage continuous waveform data from a network of piezoceramic sensors to study the spatial and temporal evolution of microslip activity during a shear experiment with synthetic fault gouge. We combine machine learning techniques with ray theoretical seismology to detect, associate, and locate tens of thousands of microslip events within the gouge layer. Microslip activity is concentrated near the center of the system but is highly variable in space and time. While microslip activity rate increases as failure approaches, the spatiotemporal evolution can differ substantially between stick-slip cycles. These results illustrate that even within a single, well-constrained laboratory experiment, the dynamics of earthquake nucleation can be highly complex.

58 GEOSCIENCES↗
DOE OSTI2021

Unusual Seismic Signals in the Sevier Desert, Utah Possibly Related to the Black Rock Volcanic Field

Abstract On September 12, 2018 and April 14, 2019 shallow (<2.5 km from the surface, <1 km relative to sea level) earthquakes ( M w 4.0 and 4.1, respectively) struck a relatively aseismic area in south‐central Utah, within the Black Rock Desert volcanic field. Seismic waveforms are dominated by long‐period energy, no clear direct S‐wave arrivals, and signal durations of ∼100 s. Using co‐seismic interferograms, we detect clear and distinguishable surface deformation confirming the shallowness of the two mainshocks, while full moment tensor solutions rule out an isotropic source, such as an explosion or collapse. For the April 2019 sequence, we build an earthquake catalog using a dense temporary geophone array. The enhanced earthquake catalog shows a rapidly decaying aftershock sequence, with 85% of aftershocks occurring during the first three hours. Combining these observations, we argue that these earthquake sequences are related to the Black Rock Desert volcanic field.

Mesimeri, Maria↗
DOE OSTI2021

Combined Optical and Radio-Frequency Perspectives on a Hybrid Cloud-To-Ground Lightning Flash Observed by the FORTE Satellite

In this work, we use the coincident optical and radio-frequency (RF) measurements taken by the Fast On-orbit Recording of Transient Events (FORTE) satellite to shed light on common optical signatures recorded by NASA and NOAA lightning imagers during Cloud-to-Ground (CG) lightning. We build flash cluster data for FORTE using the same techniques as the NASA/NOAA instruments to document the optical/RF evolution of an oceanic hybrid -CG flash. The flash began with strong Very High Frequency (VHF)-band emission from a Narrow Bipolar Event (NBE) that initiated a period of normal bilevel intracloud (IC) activity in two vertical layers (8 and 12 km) that lasted for 490 ms. VHF waveforms show step leader activity ahead of the return stroke. All impulsive VHF sources after the stroke come from the lower (8 km) layer. K-changes are noted following the return stroke, but no subsequent strokes are detected. The optical flash began 136 ms after the NBE RF pulse. Twenty-two of the 33 optical groups were dim and occurred during the in-cloud phase of the flash. This activity included both isolated pulses and sustained periods of illumination over tens of milliseconds. Initial cloud pulses accounted for 23% of the total optical radiance from the flash. Illumination during the return stroke contributed 58% of the total radiance, and the K-changes and cloud pulses after the stroke supplied the remaining 19%. These results highlight the benefit of having RF alongside optical lightning measurements for clarifying signatures in the optical data and providing information on their physical origins.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Combined Optical and Radio-Frequency Measurements of a Lightning Megaflash by the FORTE Satellite

The optical and VHF instrumentation on the Fast On-Orbit Recording of Transient Events (FORTE) satellite is used to document the combined phenomenology evolution of a lightning “megaflash” – mesoscale lightning that propagates laterally over exceptional distances. We identify a FORTE flash whose maximum extent was 82 km and inferred length over multiple distinct branches exceeded 100 km. This flash lasted 1.2 s and produced 250 optical and 591 RF events. We find that the channel development mapped by FORTE’s pixelated lightning imager (LLS) occurred at a typical speed of 2.6x10 5 m s -1 and was accompanied by sustained periods of VHF emission that could individually exceed 100 ms in duration. The impulsive IC events generated by the flash indicate that this development occurred at altitudes between 3 and 8 km. Four +CG strokes were identified in the VHF waveform data that are responsible for two of the three highly-radiant LLS groups (two of the +CGs were not as optically bright as the others). These strokes occurred at different locations throughout the flash footprint with the most distant strokes separated by approximately 50 km. These space-based observations match previous observations of megaflashes as well as ground-based measurements of negative leader development during “spider” lightning, suggesting that FORTE is sensing the same phenomena.

Peterson, Michael Jay↗
DOE OSTI2021

Infrasound From a Buried Chemical Explosion Recorded on a Balloon in the Lower Stratosphere

Abstract Infrasound waveforms generated by natural and anthropogenic phenomena contain important clues about the size and nature of the event. We show that sensors on balloons in the lower stratosphere can record faithful representations of the near‐source acoustic wave field at unprecedented range. The acoustic signature of a buried chemical explosion recorded at a range of 56 km and an altitude of 21.8 km was nearly identical to that recorded on the ground 0.5 km from the epicenter, but absent on a ground sensor located 46 km away. Our results demonstrate that balloon‐borne infrasound techniques greatly increase the range at which well‐preserved acoustic representations of near‐source physics can be acquired, and that their propagation is simple to model. Our work has implications for monitoring remote regions of the earth for explosions, volcanic eruptions, and other phenomena. It also supports the prospect of balloon‐based infrasound seismology on Venus.

Bowman, Daniel C.↗
DOE OSTI2022

Strong Upper-Plate Heterogeneity at the Hikurangi Subduction Margin (North Island, New Zealand) Imaged by Adjoint Tomography

We use earthquake-based adjoint tomography to invert for three-dimensional structure of the North Island, New Zealand, and the adjacent Hikurangi subduction zone. The study area, having a shallow depth to the plate interface below the North Island, offers a rare opportunity for imaging material properties at an active subduction zone using land-based measurements. Starting from an initial model derived using ray tomography, we perform iterative model updates using spectral element and adjoint simulations to fit waveforms with periods ranging from 4–30 s. We perform 28 model updates using an L-BFGS optimization algorithm, improving data fit and introducing P- and S-wave velocity changes of up to ±30%. Resolution analysis using point spread functions show that our measurements are most sensitive to heterogeneities in the upper 30 km. The most striking velocity changes coincide with areas related to the active Hikurangi subduction zone. Lateral velocity structures in the upper 5 km correlate well with New Zealand geology. Here, the inversion reveals increased along-strike heterogeneity on the margin. In Cook Strait we observe a low-velocity zone interpreted as deep sedimentary basins. In the central North Island, low-velocity anomalies are linked to surface geology, and we relate velocity structures at depth to crustal magmatic activity below the Taupō Volcanic Zone.

58 GEOSCIENCES↗