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At least 1,693 records · Page 94
All sourcesNASA NTRSDOE OSTI
DOE OSTI2022

On the mechanisms of ion adsorption to aqueous interfaces: air-water vs. oil-water

The adsorption of ions to water-hydrophobe interfaces influences a wide range of phenomena, including chemical reaction rates, ion transport across biological membranes, and electrochemical and many catalytic processes; hence, developing a detailed understanding of the behavior of ions at water-hydrophobe interfaces is of central interest. Here, we characterize the adsorption of the chaotropic thiocyanate anion (SCN − ) to two prototypical liquid hydrophobic surfaces, water-toluene and water-decane, by surface-sensitive nonlinear spectroscopy and compare the results against our previous studies of SCN − adsorption to the air-water interface. For these systems, we observe no spectral shift in the charge transfer to solvent spectrum of SCN − , and the Gibb’s free energies of adsorption for these three different interfaces all agree within error. We employed molecular dynamics simulations to develop a molecular-level understanding of the adsorption mechanism and found that the adsorption for SCN − to both water-toluene and water-decane interfaces is driven by an increase in entropy, with very little enthalpic contribution. This is a qualitatively different mechanism than reported for SCN − adsorption to the air-water and graphene-water interfaces, wherein a favorable enthalpy change was the main driving force, against an unfavorable entropy change.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
NASA NTRS1989

Interacting masers and the extreme brightness of astrophysical water masers

Extreme surface brightnesses have long been reported for water masers which are well beyond what is found in self-consistent, theoretical investigations of these masers. The transport of maser radiation is calculated when two masers, having the properties inferred for the numerous weaker masers and separated by distances characteristic of the molecular cloud, are aligned to within the angular spread of the beam of maser radiation. The beam size is reduced and brightness temperatures similar to the highest observed values are readily produced. This enhanced beaming reduces the number of photons required from each maser feature to a level that can be understood within available pumping scenarios. The large number of weaker masers that have been identified in the most luminous galactic cloud of water masers (the W49 region) makes it especially plausible that alignments occur and produce the very bright masers in this region.

Deguchi, Shuji↗
NASA NTRS2017

Design and characterization of a low cost CubeSat multi-band optical receiver to map water ice on the lunar surface for the Lunar Flashlight mission

Lunar Flashlight is an innovative NASA CubeSat mission dedicated to mapping water ice in the permanently shadowed regions of the Moon, which may act as cold traps for volatiles. To this end, a multi-band reflectometer will be sent to orbit the Moon. This instrument consists of an optical receiver aligned with four lasers, each of which emits sequentially at a different wavelength in the near-infrared between 1 μm and 2 μm. The receiver measures the laser light reflected from the lunar surface; continuum/absorption band ratios are then analyzed to quantify water ice in the illuminated spot. Here, we present the current state of the optical receiver design. To optimize the optical signal-to-noise ratio, we have designed the receiver so as to maximize the laser signal collected, while minimizing the stray light reaching the detector from solar-illuminated areas of the lunar surface outside the field-of-view, taking into account the complex lunar topography. Characterization plans are also discussed. This highly mass- and volume-constrained mission will demonstrate several firsts, including being one of the first CubeSats performing science measurements beyond low Earth orbit.

Sellar, Glenn R.↗
NASA NTRS1970

The dynamics of oceanic fronts. Part 1: The Gulf Stream

The establishment and maintenance of the mean hydrographic properties of large scale density fronts in the upper ocean is considered. The dynamics is studied by posing an initial value problem starting with a near surface discharge of buoyant water with a prescribed density deficit into an ambient stationary fluid of uniform density. The full time dependent diffusion and Navier-Stokes equations for a constant Coriolis parameter are used in this study. Scaling analysis reveals three independent length scales of the problem, namely a radius of deformation or inertial length scale, Lo, a buoyance length scale, ho, and a diffusive length scale, hv. Two basic dimensionless parameters are then formed from these length scales, the thermal (or more precisely, the densimetric) Rossby number, Ro = Lo/ho and the Ekman number, E = hv/ho. The governing equations are then suitably scaled and the resulting normalized equations are shown to depend on E alone for problems of oceanic interest. Under this scaling, the solutions are similar for all Ro. It is also shown that 1/Ro is a measure of the frontal slope. The governing equations are solved numerically and the scaling analysis is confirmed. The solution indicates that an equilibrium state is established. The front can then be rendered stationary by a barotropic current from a larger scale along-front pressure gradient. In that quasisteady state, and for small values of E, the main thermocline and the inclined isopycnics forming the front have evolved, together with the along-front jet. Conservation of potential vorticity is also obtained in the light water pool. The surface jet exhibits anticyclonic shear in the light water pool and cyclonic shear across the front.

Kao, T. W.↗
NASA NTRS1999

Extratropical Influence of Sea Surface Temperature and Wind on Water Recycling Rate Over Oceans and Coastal Lands

Water vapor and precipitation are two important parameters confining the hydrological cycle in the atmosphere and over the ocean surface. In the extratropical areas, due to variations of midlatitude storm tracks and subtropical jetstreams, water vapor and precipitation have large variability. Recently, a concept of water recycling rate defined previously by Chahine et al. (GEWEX NEWS, August, 1997) has drawn increasing attention. The recycling rate of moisture is calculated as the ratio of precipitation to total precipitable water (its inverse is the water residence time). In this paper, using multi-sensor spacebased measurements we will study the role of sea surface temperature and ocean surface wind in determining the water recycling rate over oceans and coastal lands. Response of water recycling rate in midlatitudes to the El Nino event will also be discussed. Sea surface temperature data are derived from satellite observations from the Advanced Very High Resolution Radiometer (AVHRR) blended with in situ measurements, available for the period 1982-1998. Global sea surface wind observations are obtained from spaceborne scatterometers aboard on the European Remote-Sensing Satellite (ERS1 and 2), available for the period 1991-1998. Global total precipitable water provided by the NASA Water Vapor Project (NVAP) is available for the period 1988-1995. Global monthly mean precipitation provided by the Global Precipitation Climatology Project (GPCP) is available for the period 1987-1998.

Hu, Hua↗
NASA NTRS1986

Experimental evidence for modifying the current physical model for ice accretion on aircraft surfaces

Closeup movies, still photographs, and other experimental data suggest that the current physical model for ice accretion needs significant modification. At aircraft airspeeds there was no flow of liquid over the surface of the ice after a short initial flow, even at barely subfreezing temperatures. Instead, there were very large stationary drops on the ice surface that lose water from their bottoms by freezing and replenish their liquid by catching the microscopic cloud droplets. This observation disagrees with the existing physical model, which assumes there is a thin liquid film continuously flowing over the ice surface. With no such flow, the freezing-fraction concept of the model fails when a mass balance is performed on the surface water. Rime ice does, as the model predicts, form when the air temperature is low enough to cause the cloud droplets to freeze almost immediately on impact. However, the characteristic shapes of horn-glaze ice or rime ice are primarily caused by the ice shape affecting the airflow locally and consequently the droplet catch and the resulting ice shape. Ice roughness greatly increases the heat transfer coefficient, stops the movement of drops along the surface, and may also affect the airflow initially and thereby the droplet catch. At high subreezing temperatures the initial flow and shedding of surface drops have a large effect on the ice shape. At the incipient freezing limit, no ice forms.

Olsen, W.↗
DOE OSTI2023

Global impacts of vegetation clumping on regulating land surface heat fluxes

The clumping index (CI) quantifies the non-random distribution of vegetation across space, which regulates the canopy radiative transfer processes and land surface carbon, water, and energy cycles. However, its impact on global surface energy budget, particularly sensible heat fluxes and surface temperature, is not well understood. Additionally, while there have been studies showing significant seasonal variations in CI, the impacts of these variations on surface energy fluxes remain unclear. In this study, we incorporated satellite-derived spatially and temporally explicit CI data into the Community Land Model version 5 (CLM5) to evaluate the effects of CI on global land energy fluxes. Our results showed that including CI increased the global mean sensible heat flux dissipated from ground by 3.9 W m -2 (~18%), while decreasing the global mean vegetation sensible heat flux by 4.9 W m -2 (~65%), resulting in a total sensible heat decrease of 1.0 W m -2 (~3%). In contrast, CI increased the global mean latent heat flux by 0.8 W m -2 (~2%), primarily due to increased evapotranspiration (up to 11 W m -2 ) in tropical regions. We also found considerable impacts of seasonal variations in CI, particularly on sensible heat fluxes from ground and vegetation in evergreen needleleaf forests and deciduous needleleaf forests. Using constant CI rather than considering seasonal variations resulted in significant overestimation and underestimation of the sensible heat fluxes from vegetation and ground, respectively, in boreal summer. In conclusion, these changes in surface energy fluxes caused by CI and its seasonal variations led to up to 1.7 and 0.5 K differences in simulated mean ground temperature. These findings highlight the importance of including CI and considering its seasonal variations in modeling land surface energy fluxes.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1990

The nature of low-albedo asteroids from 3-micron multi-color photometry

The present broadband and narrowband 1.2-3.5 micron spectrophotometry of 16 low-albedo asteroids encompasses C-, F-, P-, D-, and T-class asteroids, and has been used in an effort to identify low-temperature minerals on their surfaces. Attention has been given to the identification of water of hydration. While G-class asteroids have water-rich surfaces, and I asteroids possess some hydrated silicates, not all class Cs do. Finally, the P-, F-, and T-class asteroids do not seem to possess hydrated-silicate surfaces.

Lebofsky, Larry A.↗
NASA NTRS1996

Retrieval of Surface Snow Grain Size and Melt Water from AVIRIS Spectra

The Earth's energy balance and hydrology are affected by the distribution and characteristics of snow cover on the surface. Snow grain size and snow melt influence surface albedo and hydrology. A model of snow reflectance that depends on both grain size and surface melt water was developed to derive these parameters from remote spectral measurements. This reflectance model is based on a discrete ordinate radiative transfer approach that uses Mie calculations of snow optical properties, which are based on the complex refractive index of ice and water. This snow model was linked to an atmospheric radiative transfer code and a nonlinear least squares fitting algorithm. The resulting combined algorithm was applied to an AVIRIS snow data set acquired over Mammoth Mountain, California. Maps of grain size and surface snow melt were generated that are consistent with the expected ranges and distributions for conditions at the site.

Green Robert O.↗
NASA NTRS2001

Tropical Ocean Evaporation/SST Sensitivity and It's Link to Water and Energy Budget Variations During ENSO

The continuing debate over feedback mechanisms governing tropical sea surface temperatures (SSTs) and tropical climate in general has highlighted the diversity of potential checks and balances within the climate system. Competing feedbacks due to changes in surface evaporation, water vapor, and cloud long- and shortwave radiative properties each may serve critical roles in stabilizing or destabilizing the climate system. It is also intriguing that even those climate variations having origins internal to the climate system - changes in ocean heat transport for example, apparently require complementary equilibrating effects by changes in atmospheric energy fluxes. Perhaps the best observational evidence of this is the relatively invariant nature of tropically averaged net radiation exiting the top-of-atmosphere (TOA) as measured by broadband satellite sensors over the past two decades. Thus, analyzing how these feedback mechanisms are operating within the context of current interannual variability may offer considerable insight for anticipating future climate change. In this paper we focus primarily on interannual variations of ocean evaporative fluxes and their significance for coupled water and energy cycles within the tropical climate system. In particular, we use both the da Silva estimates of surface fluxes (based on the Comprehensive Ocean Atmosphere Data Set, COADS) and numerical simulations from several global climate models to examine evaporation sensitivity to perturbations in SST associated with warm and cold ENSO events. The specific questions we address are as follows: (1) What recurring patterns of surface wind and humidity anomalies are present during ENSO and how do they combine to yield systematic evaporation anomalies?, (2) What is the resulting tropical ocean mean evaporation-SST sensitivity associated with this climate perturbation?, and (3) What role does this evaporation play in tropical heat and water balance over tropical oceanic regions? We use the da Silva ocean flux data to identify composite structure of departures of latent heat flux from climatology. We also show how these patterns arise out of associated wind and humidity anomaly distributions. Our preliminary work shows that evaporation sensitivity estimates from the da Silva / COADS data, computed for the tropical oceans (30 degrees N/S) are in the neighborhood of 5 to 6 W/square m K. Model estimates are also quite close to this figure. This rate is only slightly less than a rate corresponding to constant relative humidity; however, substantial regional departures from constant relative humidity are present. These patterns are robust and we relate the associated wind and humidity fluctuations noted in previous investigations to the derived evaporation anomalies. Finally, these results are interpreted with other data from the Earth radiation Budget Experiment (ERBE), Global Precipitation Climatology Project (GPCP) and NASA's Surface Radiation Budget (SRB) data set to characterize the tropical energetics of ENSO-related climate variability.

Robertson, Franklin R.↗
NASA NTRS1984

Quaternary North Atlantic Surface Paleoceanography in Regions of Potential Deep-water Formation

At the time scale of the Quaternary climate cycles, the sites of formation of North Atlantic Deep Water are not known. The interglacial extreme is presumably exemplified by the modern regions; the Norwegian, Greenland and Labrador Seas. During the major glacial-age coolings in the North Atlantic, the sites may have shifted well to the south, perhaps as far as the limit of the polar front at 40 to 50 N. Still other sites may have been important during intermediate climatic conditions. Because of the close coupling of high-latitude surface waters to North Atlantic Deep Water in the modern ocean, the history of sea-surface temperature (SST) oscillations across the high-latitude North Atlantic is relevant to an understanding of deep-water formation on the longer time scales.

Ruddiman, W. F.↗
NASA NTRS1987

Remote sensing of snow

The snow parameters affecting sensor responses at different wavelengths are discussed. The effects of snow depth and background radiation on gamma ray sensors and of crystal size, contaminants, snow depth, liquid water, and surface roughness on visible and near-infrared sensors are considered. The influence of temperature, crystal size, and liquid water on thermal infrared sensors and of liquid water, crystal size, water equivalent depth, stratification, snow surface roughness, density, temperature, and soil condition on microwave sensors are addressed.

Foster, J. L.↗
DOE OSTI2025

Computational Modeling of Water Infiltration From Ditches Into Roadway Embankments

Ditches are built along roadways to convey the stormwater runoff. They collect the runoff from the pavement and adjacent drainage areas. Water can move freely in a ditch away from the road surface, thus making it safer for the vehicular traffic. South Carolina DOT expressed interest in studying infiltration of water from ditches into roadway embankments. As part of the current design criteria, it is recommended that the road subgrades be 1.0 foot above the design event water surface elevation in the ditch. The distance between the water surface and bottom of the subbase is referred to as “freeboard”. The purpose of this requirement is to lower the risk of pavement damage by moving the flow away from the pavement, containing the captured flow, and conveying flow received from adjacent properties to outfalls. With changes in roadway design standards, larger shoulders and flatter cross-slopes have moved ditches further away from the pavement and the subbase. These changes could allow for a lower freeboard standard without reducing safety margins due to the increased lateral distance from the subbase to the ditch. The objective of this study is to evaluate whether the current SCDOT criterion requiring the roadway subgrade to be 1 ft above the design-event ditch water surface can be relaxed under selected geometric and soil conditions, particularly where larger shoulder widths and flatter side slopes increase horizontal separation between ditch water and pavement structure.

42 ENGINEERING↗
NASA NTRS2023

Virus Infection of Phytoplankton Increases Average Molar Mass and Reduces Hygroscopicity of Aerosolized Organic Matter

Viral infection of phytoplankton is a pervasive mechanism of cell death and bloom termination, which leads to the production of dissolved and colloidal organic matter that can be aerosolized into the atmosphere. Earth-observing satellites can track the growth and death of phytoplankton blooms on weekly time scales but the impact of viral infection on the cloud forming potential of associated aerosols is largely unknown. Here, we determine the influence of viral-derived organic matter, purified viruses, and marine hydrogels on the cloud condensation nuclei activity of their aerosolized solutions, compared to organic exudates from healthy phytoplankton. Dissolved organic material derived from exponentially growing and infected cells of well-characterized eukaryotic phytoplankton host-virus systems, including viruses from diatoms, coccolithophores and chlorophytes, was concentrated, desalted, and nebulized to form aerosol particles composed of primarily of organic matter. Aerosols from infected phytoplankton cultures resulted in an increase in critical activation diameter and average molar mass in three out of five combinations evaluated, along with a decrease in organic kappa (hygroscopicity) compared to healthy cultures and seawater controls. The infected samples also displayed evidence of increased surface tension depression at realistic cloud water vapor supersaturations. Amending the samples with xanthan gum to simulate marine hydrogels increased variability in organic kappa and surface tension in aerosols with high organic to salt ratios. Our findings suggest that the pulses of increased dissolved organic matter associated with viral infection in surface waters may increase the molar mass of dissolved organic compounds relative to surface waters occupied by healthy phytoplankton or low phytoplankton biomass.

Atmospheric science↗
DOE OSTI2024

Greenhouse gas and dissolved oxygen production and consumption rates associated with Regier et al. (2023)

Tidal inundation along the coastal terrestrial-aquatic interface controls soil and sediment biogeochemistry and gas dynamics. Although a rich literature exist on studies of the influence of tidal waters on the biogeochemistry of coastal ecosystem soils, few studies have experimentally addressed the reverse question: How do soils (or sediments) from different coastal ecosystems influence the biogeochemistry of the tidal waters that inundate them? We conducted short-term microcosm laboratory experiments where seawater was amended with sediments and soils collected across regional gradients of inundation exposure (i.e., frequently to rarely inundated) and measured changes in dissolved oxygen and greenhouse gas concentrations to calculate gas consumption or production rates occurring during seawater exposure to terrestrial materials. This data package contains dissolved oxygen and greenhouse gas data collected during incubation of soils and sediments collected at 18 sites, which were used in the publication Regier et al. (2023) entitled “Coastal inundation regime moderates the short-term effects of sediment and soil additions on seawater oxygen and greenhouse gas dynamics: a microcosm experiment” which is published in Frontiers in Marine Science (DOI: https://doi.org/10.3389/fmars.2023.1308590).---Acknowledging EXCHANGE: General Support and Data Product UseWe ask that users of EXCHANGE data add the following acknowledgement when publishing data in scholarly articles and data repositories:"This research is based on work supported by COMPASS-FME, a multi-institutional project supported by the U.S. Department of Energy, Office of Science, Biological and Environmental Research as part of the Environmental System Science Program."

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2025

Model data for a watershed-scale study in the Portage River Basin (OH) examining the effects of subsurface drainage on the hydrologic response of an agricultural watershed.

This study builds on Rathore et al. (2024, WRR) and investigates the role of artificial tile-drainage on various aspects of watershed hydrological response, with a particular focus on peakflow. The model-data for the original modeling-focused paper (Rathore et al., 2024, WRR) is archived at Rathore et al. (2024, ESS-DIVE). Hence, this model-data archive provides scripts that are specific to this study that includes model updates, processing and analysis scripts. For details and models files of original model, readers are referred to Rathore et al. (2024, ESS-DIVE). The key difference between the model configuration in this study and Rathore et al. (2024, WRR) is that the tile drains are applied to the entire domain, to study the impact of tile-drains on different aspects of hydrological response. Additional scenario considering intensified precipitation after a dry period was also simulated. The Watershed Workflow package is implemented in Python3. The Jupyter notebooks can be executed through multiple open-source tools, for example, Anaconda Jupyter Lab, VS Studio Code, etc. Other data files include CSV and HDF5 files, which can be read through Python scripts.

54 ENVIRONMENTAL SCIENCES↗