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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 1,693 records · Page 94
All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

Direct electron beam patterning of electro-optically active PEDOT:PSS

The optical and electronic tunability of the conductive polymer poly(3,4-ethylenedioxythiophene):poly(styrene sulfonate) (PEDOT:PSS) has enabled emerging applications as diverse as bioelectronics, flexible electronics, and micro- and nano-photonics. High-resolution spatial patterning of PEDOT:PSS opens up opportunities for novel active devices in a range of fields. However, typical lithographic processes require tedious indirect patterning and dry etch processes, while solution-processing methods such as ink-jet printing have limited spatial resolution. Here, we report a method for direct write nano-patterning of commercially available PEDOT:PSS through electron-beam induced solubility modulation. The written structures are water stable and maintain the conductivity as well as electrochemical and optical properties of PEDOT:PSS, highlighting the broad utility of our method. We demonstrate the potential of our strategy by preparing prototypical nano-wire structures with feature sizes down to 250 nm, an order of magnitude finer than previously reported direct write methods, opening the possibility of writing chip-scale microelectronic and optical devices. We finally use the high-resolution writing capabilities to fabricate electrically-switchable optical diffraction gratings. We show active switching in this archetypal system with >95 % contrast at CMOS-compatible voltages of +2 V and -3 V, offering a route towards highly-miniaturized dynamic optoelectronic devices.

42 ENGINEERING↗
NASA NTRS1994

The X-ray selected cataclysmic variables H0459 + 246 and H0857 - 242

We report the discovery of two cataclysmic variables located with the assistance of X-ray positions from the HEAO 1 Modulation Collimator and the Large-Area Sky Survey. Each case is distinguished by evidence of two periodic modulations that appear to represent the orbital period and the spin period of the white dwarf, respectively. The first case, H0459 + 246, has been observed optically during faint states (V approximately 16), in which there are spectral features of both an accretion disk and a K star. The light curves in the V and I bands are consistent with ellipsoidal variations in the secondary stars with a binary period of 9.952 hr. X-ray observations with EXOSAT reveal a strong pulsation with a period approximately 62 minutes. This result confirms an 'intermediate polar' classification for H0459 + 246. The pulsation is observed at 63.2 minutes in the optical I band. The long orbital period opens the possibility that H0459 + 246 is a relatively young intermediate polar that might evolve into a polar. The second case, H0857--242, shows radial velocity modulations at 1.78 hr along with photometric variations at a period approximately 49 minutes. The latter are observed only during the decay phase of dwarf nova outbursts (13 less than V less than 17), which apparently recur frequently. Given the lack of X-ray monitoring observations and the absence of proof that the 49 minute periodicity is coherent over long time-scales, we regard H0857--242 as a candidate intermediate polar. Photographic records from th e Harvard Observatory Plate Library further reveal superoutbursts for H0857--242 (V approximately 11). A bright X-ray source that is both an intermediate polar and a continually cycling dwarf nova may provide an effective means of measuring the time delay for the arrival of accreting matter at the white dwarf surface, relative to the onset of optical brightening.

Remillard, R. A.↗
NASA NTRS2010

Fiber-Coupled Planar Light-Wave Circuit for Seed Laser Control in High Spectral Resolution Lidar Systems

Precise laser remote sensing of aerosol extinction and backscatter in the atmosphere requires a high-power, pulsed, frequency doubled Nd:YAG laser that is wavelength- stabilized to a narrow absorption line such as found in iodine vapor. One method for precise wavelength control is to injection seed the Nd:YAG laser with a low-power CW laser that is stabilized by frequency converting a fraction of the beam to 532 nm, and to actively frequency-lock it to an iodine vapor absorption line. While the feasibility of this approach has been demonstrated using bulk optics in NASA Langley s Airborne High Spectral Resolution Lidar (HSRL) program, an ideal, lower cost solution is to develop an all-waveguide, frequency-locked seed laser in a compact, robust package that will withstand the temperature, shock, and vibration levels associated with airborne and space-based remote sensing platforms. A key technology leading to this miniaturization is the integration of an efficient waveguide frequency doubling element, and a low-voltage phase modulation element into a single, monolithic, planar light-wave circuit (PLC). The PLC concept advances NASA's future lidar systems due to its compact, efficient and reliable design, thus enabling use on small aircraft and satellites. The immediate application for this technology is targeted for NASA Langley's HSRL system for aerosol and cloud characterization. This Phase I effort proposes the development of a potassium titanyl phosphate (KTP) waveguide phase modulator for future integration into a PLC. For this innovation, the proposed device is the integration of a waveguide-based frequency doubler and phase modulator in a single, fiber pigtail device that will be capable of efficient second harmonic generation of 1,064-nm light and subsequent phase modulation of the 532 nm light at 250 MHz, providing a properly spectrally formatted beam for HSRL s seed laser locking system. Fabrication of the integrated PLC chip for NASA Langley, planned for the Phase II effort, will require full integration and optimization of the waveguide components (SHG waveguide, splitters, and phase modulator) onto a single, monolithic device. The PLC will greatly reduce the size and weight, improve electrical- to-optical efficiency, and significantly reduce the cost of NASA Langley s current stabilized HSRL seed laser system built around a commercial off-the-shelf seed laser that is free-space coupled to a bulk doubler and bulk phase modulator.

Cook, Anthony↗
DOE OSTI2022

Remote surface optical phonon scattering in ferroelectric Ba 0.6 Sr 0.4 TiO 3 gated graphene

We report the effect of remote surface optical (RSO) phonon scattering on carrier mobility in monolayer graphene gated by ferroelectric oxide. We fabricate monolayer graphene transistors back-gated by epitaxial (001) Ba 0.6 Sr 0.4 TiO 3 films, with field effect mobility up to 23 000 cm 2 V –1 s –1 achieved. Switching ferroelectric polarization induces nonvolatile modulation of resistance and quantum Hall effect in graphene at low temperatures. Ellipsometry spectroscopy studies reveal four pairs of optical phonon modes in Ba 0.6 Sr 0.4 TiO 3 , from which we extract RSO phonon frequencies. The temperature dependence of resistivity in graphene can be well accounted for by considering the scattering from the intrinsic longitudinal acoustic phonon and the RSO phonon, with the latter dominated by the mode at 35.8 meV. Furthermore, our study reveals the room temperature mobility limit of ferroelectric-gated graphene transistors imposed by RSO phonon scattering.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Frequency combs in optically injected terahertz ring quantum cascade lasers

Quantum cascade lasers (QCLs) have emerged as promising candidates for generating chip-scale frequency combs in mid-infrared and terahertz wavelengths. In this work, we demonstrate frequency comb formation in ring terahertz QCLs using the injection of light from a distributed feedback (DFB) laser. The DFB design frequency is chosen to match the modes of the ring cavity (near 3.3 THz), and light from the DFB is injected into the ring QCL via a bus waveguide. By controlling the power and frequency of the optical injection, we show that combs can be selectively formed and controlled in the ring cavity. Numerical modeling suggests that this comb is primarily frequency-modulated in character, with the injection serving to trigger comb formation. We also show that the ring can be used as a filter to control the output of the DFB QCL, potentially being of interest in terahertz photonic integrated circuits. Our work demonstrates that waveguide couplers are a compelling approach for injecting and extracting radiation from ring terahertz combs and offer exciting possibilities for the generation of new comb states in terahertz, such as frequency-modulated waves, solitons, and more.

47 OTHER INSTRUMENTATION↗
DOE OSTI2020

Development of a position–velocity–time-modulated two-dimensional ion beam figuring system for synchrotron x-ray mirror fabrication

With the rapid evolution of synchrotron x-ray sources, the demand for high-quality precision x-ray mirrors has greatly increased. Single nanometer shape accuracy is required to keep imaging capabilities at the diffraction limit. Ion beam figuring (IBF) has been used frequently for ultra-precision finishing of mirrors, but achieving the ultimate accuracy depends on three important points: careful alignment, accurate dwell time calculation and implementation, and accurate optical metrology. The Optical Metrology Group at National Synchrotron Light Source II has designed and built a position–velocity–time-modulated two-dimensional IBF system (PVT-IBF) with three novel characteristics: (1) a beam footprint on the mirror was used as a reference to align the coordinate systems between the metrology and the IBF hardware; (2) the robust iterative Fourier transform-based dwell time algorithm proposed by our group was applied to obtain an accurate dwell time map; and (3) the dwell time was then transformed to velocities and implemented with the PVT motion scheme. In this study, the technical aspects of the PVT-IBF systems are described in detail, followed by an experimental demonstration of the figuring results. In our first experiment, the 2D RMS in a 50mm×5mm clear aperture was reduced from 3.4 to 1.1 nm after one IBF run. In our second experiment, due to a 5 mm pinhole installed in front of the source, the 2D RMS in a 50mm×5mm clear aperture was reduced from 39.1 to 1.9 nm after three IBF runs, demonstrating that our PVT-IBF solution is an effective and deterministic figuring process.

47 OTHER INSTRUMENTATION↗
NASA NTRS1981

Simultaneous X-ray and optical observations of an Ursae Majoris during a low state

In November 1975, AN UMa was detected as a soft X-ray source with a 0.1-0.4 keV flux which was modulated with the orbital cycle. In order to investigate further this orbital dependence and to correlate it with existing photometric and spectroscopic observations to aid in determining the geometry of the system, simultaneous X-ray and optical observations were made throughout several cycles of AN UMa. The system was in a low optical state during the observations. The X-ray observations were made with the Imaging Proportional Counter on the Einstein Observatory, yielding measurements over an available energy range of 0.1-4 keV. Attention is given to total X-ray flux, the X-ray light curve, optical and infrared data, and model implications.

Szkody, P.↗
DOE OSTI2020

W-band system-on-chip electron cyclotron emission imaging system on DIII-D

Monolithic, millimeter wave “system-on-chip” (SoC) technology has been employed in heterodyne receiver integrated circuit radiometers in a newly developed Electron Cyclotron Emission Imaging (ECEI) system on the DIII-D tokamak for 2D electron temperature profile and fluctuation evolution diagnostics. Here, a prototype module operating in E-band (72-80 GHz) was first employed in a 2 x 10 element array that demonstrated significant improvements over the previous quasi-optical Schottky diode mixer arrays during the 2018 operational campaign of the DIII-D tokamak. For compatibility with International Thermonuclear Experimental Reactor (ITER) relevant scenarios on DIII-D, the SoC ECEI system was upgraded with 20 horn-waveguide receiver modules. Each individual module contains a University of California at Davis designed W-band (75 -110 GHz) receiver die that integrates a broadband low noise amplifier (LNA), a double balanced down-converting mixer, and a x4 multiplier on the local oscillator (LO) chain. A x2 multiplier and two IF amplifiers are packaged and selected to further boost the signal strength as well as downconvert the signal frequency. The upgraded W-band array exhibits > 30 dB additional gain and 20x improvement in noise temperature comparing with the previous Schottky diode radio frequency (RF) mixer input systems; an internal 8 times multiplier chain is used to bring down the LO frequency below 12 GHz, thereby obviating the need for a large aperture for quasi-optical LO coupling and replacing it with coaxial connectors. The horn-waveguide shielding housing avoids out-of-band noise interference on each individual module. The upgraded ECEI system plays an important role for absolute electron temperature evolution and fluctuation measurements for edge and core region transport physics studies.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2023

PV encapsulant formulations and stress test conditions influence dominant degradation mechanisms

Polyethylene-based poly(ethylene-co-vinyl acetate) (EVA), polyolefin elastomer (POE), and thermoplastic polyolefin (TPO) are common polymer candidates for photovoltaic (PV) module encapsulants. The choice of encapsulant must be carefully considered in novel module designs, such as bifacial glass/glass laminates, to limit performance degradation through loss of optical transmittance, mechanical integrity, and corrosion - as well as potential-induced degradation. Encapsulant quality and resilience against environmental stressors are readily influenced by the additives in the encapsulant formulation. Here, we show that, the changes in optical transmittance after UV aging result from the discoloration caused by interactions between additives, and optical scattering from changes in the polymer crystal structure. We observed competing cross-linking and chain scission mechanisms, with their kinetics influenced by the presence of oxygen and elevated temperatures. Increasing chamber temperatures from 55 °C to 85 °C during the UV stress test amplified encapsulant discoloration and promoted polymer cross-linking, causing severe, irreversible damage that remains to be proven field relevant. Damp heat aging was found to be insufficient to produce significant encapsulant degradation; however, combining stress tests sequentially allowed detection of further degradation beyond the limitations of the damp heat test alone. Appropriate degradation screening methods are necessary to uncover potential encapsulant weaknesses.

14 SOLAR ENERGY↗
DOE OSTI2022

Understanding the Effect of Lead Iodide Excess on the Performance of Methylammonium Lead Iodide Perovskite Solar Cells

The presence of unreacted lead iodide in organic-inorganic lead halide perovskite solar cells is widely correlated with an increase in power conversion efficiency. We investigate the mechanism for this increase by identifying the role of surfaces and interfaces present between methylammonium lead iodide perovskite films and excess lead iodide. We show how type I and II band alignments arising under different conditions result in either passivation of surface defects or hole injection. Through first-principles simulations of solid-solid interfaces, we find that lead iodide captures holes from methylammonium lead iodide and modulates the formation of defects in the perovskite, affecting recombination. Using surface-sensitive optical spectroscopy techniques, such as transient reflectance and time-resolved photoluminescence, we show how excess lead iodide affects the diffusion and surface recombination velocity of charge carriers in methylammonium lead iodide films. Our coupled experimental and theoretical results elucidate the role of excess lead iodide in perovskite solar cells.

14 SOLAR ENERGY↗
DOE OSTI2022

Voltage-controlled reversible modulation of colloidal quantum dot thin film photoluminescence

Active modulation of quantum dot thin film photoluminescence (PL) has been far-reaching potential applications in biomedical and optoelectronic systems, but challenges remain in achieving large PL modulation depth and fast temporal response. Here, we report an efficient voltage-controlled optical down-converter by optically exciting a colloidal quantum dot thin film within a quantum dot light-emitting diode under reverse bias. Utilizing field-induced luminescence quenching, we show that a large electric field can strongly modify carrier dynamics in this nanostructured device, resulting in stable and reversible photoluminescence quenching. The device exhibits photoluminescence reduction of up to 99.5%, corresponding to a contrast ratio of 200:1 under the applied electric field of 3 MV cm -1 with a 300 ns response time. Using excitation wavelength dependent and transient PL spectroscopy, we further show that the high degree of quenching is achieved by a synergistic interplay of quantum-confined Stark effect and field-induced exciton dissociation.

42 ENGINEERING↗
DOE OSTI2020

100 Gbps Radiation Tolerant Optical Transceiver (Final Technical Report)

The overall technical objective in phase I for the Surface Emitting Laser-Electro-Absorption Modulator (EAM) was to demonstrate feasibility of this approach by designing and building the laser-EAM chips, optimizing the fabrication process for the Laser/EAM in a series of 3 fabrication runs, irradiating Laser/EAM chips from each run and DC testing of the chips post radiation. 100 Gbps/channel testing would be done at the end of the phase II program before and after radiation. The overall technical objective for the driver circuit was to demonstrate the radiation tolerance of a circuit using the same technology as the driver, and to design the appropriate driver circuit.

43 PARTICLE ACCELERATORS↗
NASA NTRS1972

Coherent Optical Processing of Phased Array Radar Data

Interfacing a coherent optical processor, which utilizes an electron-beam addressed, potassium dideuterium phosphate (KDP) crystal modulator, with a linear phased array is studied. An abbreviated development of typical radar signals from a linear array is included. A plan for formating the spatial modulator with linear array signals is presented. The theoretical expectations which include target angle and Doppler are derived. A simulated set of M signals which are typical of a linear array of M elements was devised. This set of signals was used to modulate the wave front of collimated laser light via the KDP crystal according to the format presented.

Rogers, J. W.↗
NASA NTRS1980

Advanced very high resolution radiometer, Mod 2 engineering report

The Advanced High Resolution Radiometer, Mod 2 (AVHRR/2) is a modification of the original AVHRR (AVHRR/1) to expand the number of channels from four to five and provide additional sensing in the infrared region. A comparison of the spectral regions employed in the two instruments is given. Three of the channels are the same on both instruments. The difference in instruments is in the long wave IR region where a single channel was replaced by two channels. The modification from AVHRR/1 to AVHRR/2 was done with a minimum of changes. The areas of change are highlighted and the modifications by module are summarized. It is seen that the primary changes are in the relay optics and in the cooler. In this development program only two models are involved. The first model, the Optical Test Model was constructed and tested to prove the performance and structural integrity of the optical system and the modified cooler. The second model constructed is the Protoflight. Only the areas of the AVHRR/2 which were modified from the AVHRR/1 design are discussed.

Source record↗
NASA NTRS1983

Precise Measurement of Effective Focal Length

Computerized instrument measures effective focal lengths to 0.01 percent accuracy. Laser interferometers measure mirror angle and stage coordinate y in instrument for accurate measurment of focal properties of optical systems. Operates under computer control to measure effective focal length, focal surface shape, modulation transfer function, and astigmatism.

Wise, T. D.↗
NASA NTRS1983

Two hundred passage three-way valve: Fraction collector

This paper describes the design and operation of a fraction collector used to direct flow of separated biological materials from 197 capillary tubes to either a collection tray or to a waste tank. This mechanism uses a 28-volt dc gear motor driving twin cams to force 197 needles through a self-sealing silicone rubber septum, where they inject the material in 197 separate pockets in a collection tray. The position of the collector tray is sensed by two optical limit switches. The time sequences are controlled automatically by an electronics control monitoring module.

Keffer, J. L.↗
NASA NTRS1983

Experiments with optical instruments

Photography was used to document known defects of the periscopic instrument used to check spacecrews in the descent module of the Soyuz T-4. The screen of the altitude control unit was also photographed and revealed glare in the central field of vision. A light filter was installed in the peripheral window to observe the Sun and horizon of the Earth. Checking attitude control by means of polaroids enabled a 5 further advance (500 km) into the zone of shadow. The attitude control unit was used to check the orbital orientation with respect to the vertical during the night segment of flight. A lens screen was used for the emission glow of the atmosphere at an altitude of about 100 km. Docking of the Soyuz T-4 was observed by means of an onboard display, a television camera, and a sighting device. From a distance of about 5 km, the space station could be seen as a bright dot in the sighting device. Docking occurred in shadow.

Savinykh, V.↗