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DOE OSTI2025

Nanoscale Free-Electron Lasing (Final Technical Report)

Optical control of electron dynamics and energy structure can be leveraged for tailoring classical and quantum light sources. Previous work was primarily limited to Transmission Electron Microscopes (TEMs). Our work under this program sought to enable full time and energy control of electrons in SEMs for exploring the physics of attosecond electron dynamics and light generation at the nanoscale. The motivation behind this work was to understand these fundamental processes important to free-electron lasing at the nanoscale using sub-relativistic electrons.

42 ENGINEERING↗

DOE OSTI2022

Fiber-optic diagnostic system for future accelerator magnets

The next generation high energy physics accelerators will require magnetic fields at ~20 T. HTS coils will be an essential component of future accelerator magnets and several efforts are currently dedicated on designing 20 T HTS- LTS hybrid magnets. Among the existing challenges, there is the lack of a robust quench detection system for hybrid magnet technology. Another big challenge is represented by the high number of training quenches required by Nb3Sn magnets to reach performance level. In this framework it is important to find a tool that allow local real-time monitoring of magnet strain and temperature. In this paper, we propose the use of fiber optics sensors for diagnostic and quench detection in future accelerator superconducting magnets. Discrete and distributed fiber optic sensors have demonstrated to be a promising tool. The goal is to instrument hundreds of accelerator superconducting magnets and to move beyond the proof-of-concept level. Significant developments are still needed. Here, we are going to present the most recent results and discuss the most urgent technical developments in order to make those sensors a robust and reliable diagnostic tool for accelerator superconducting magnets over the next 10 year. We foresee that discrete fiber sensors will be a stable diagnostic probe for superconducting magnets over the next 3 to 5 years. More R&D work will be necessary for distributed fibers. The most urgent needs are the increase of sample rate and sensitivity. Close collaboration with vendors will be necessary to improve mechanical properties and fabrication processes in order to produce hundreds of meters of fiber and instrument a large number of accelerator superconducting magnets. Those R&D efforts will last up to 10 years with a founding level that spans between 5-10 M$.

43 PARTICLE ACCELERATORS↗

NASA NTRS2005

Atom Skimmers and Atom Lasers Utilizing Them

Atom skimmers are devices that act as low-pass velocity filters for atoms in thermal atomic beams. An atom skimmer operating in conjunction with a suitable thermal atomic-beam source (e.g., an oven in which cesium is heated) can serve as a source of slow atoms for a magneto-optical trap or other apparatus in an atomic-physics experiment. Phenomena that are studied in such apparatuses include Bose-Einstein condensation of atomic gases, spectra of trapped atoms, and collisions of slowly moving atoms. An atom skimmer includes a curved, low-thermal-conduction tube that leads from the outlet of a thermal atomic-beam source to the inlet of a magneto-optical trap or other device in which the selected low-velocity atoms are to be used. Permanent rare-earth magnets are placed around the tube in a yoke of high-magnetic-permeability material to establish a quadrupole or octupole magnetic field leading from the source to the trap. The atoms are attracted to the locus of minimum magnetic-field intensity in the middle of the tube, and the gradient of the magnetic field provides centripetal force that guides the atoms around the curve along the axis of the tube. The threshold velocity for guiding is dictated by the gradient of the magnetic field and the radius of curvature of the tube. Atoms moving at lesser velocities are successfully guided; faster atoms strike the tube wall and are lost from the beam.

Hulet, Randall↗

DOE OSTI2021

Terahertz emission spectroscopy of ultrafast exciton shift current in the noncentrosymmetric semiconductor CdS

The charge-neutral exciton has been predicted to carry genuine photocurrent due to the geometric Berry phase of the electronic bands, if the inversion symmetry in a crystal is broken. Here we detect such exciton shift current in a prototypical polar semiconductor CdS by using terahertz emission spectroscopy. A distinct peak emerges in the photocurrent spectra at the energy of the exciton resonance, which is demonstrated to result from the distinct displacements of electrons and holes in real space within the excitons to produce a finite transient charge current at subpicosecond time scale. Our findings elucidate the Berry phase physics of the charge-neutral photoexcitations and also shed light on the novel energy harvesting mechanism by exciton generation.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2023

Non-Fermi Liquids from Kinetic Constraints in Tilted Optical Lattices

Here we study Fermi-Hubbard models with kinetically constrained dynamics that conserves both total particle number and total center of mass, a situation that arises when interacting fermions are placed in strongly tilted optical lattices. Through a combination of analytics and numerics, we show how the kinetic constraints stabilize an exotic non-Fermi liquid phase described by fermions coupled to a gapless bosonic field, which in several respects mimics a dynamical gauge field. This offers a novel route towards the study of non-Fermi liquid phases in the precision environments afforded by ultracold atom platforms.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2022

A wide-field micro-computed tomography detector: micron resolution at half-centimetre scale

Ideal three-dimensional imaging of complex samples made up of micron-scale structures extending over mm to cm, such as biological tissues, requires both wide field of view and high resolution. For existing optics and detectors used for micro-CT (computed tomography) imaging, sub-micron pixel resolution can only be achieved for fields of view of <2 mm. This article presents a unique detector system with a 6 mm field-of-view image circle and 0.5 µm pixel size that can be used in micro-CT units utilizing both synchrotron and commercial X-ray sources. A resolution-test pattern with linear microstructures and whole adult Daphnia magna were imaged at beamline 8.3.2 of the Berkeley Advanced Light Source. Volumes of 10000 × 10000 × 7096 isotropic 0.5 µm voxels were reconstructed over a 5.0 mm × 3.5 mm field of view. Measurements in the projection domain confirmed a 0.90 µm measured spatial resolution that is largely Nyquist-limited. This unprecedented combination of field of view and resolution dramatically reduces the need for sectional scans and computational stitching for large samples, ultimately offering the means to elucidate changes in tissue and cellular morphology in the context of larger, whole, intact model organisms and specimens. This system is also anticipated to benefit micro-CT imaging in materials science, microelectronics, agricultural science and biomedical engineering.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

NASA NTRS1989

A physical model for predicting bidirectional reflectances over bare soil

While most previous attempts to retrieve soil surface optical property characteristics have proceeded through a fitting of empirical functions to the data, an optimization technique is presently applied to a physically-based surface reflectance model developed for the study of planetary surfaces. This inversion procedure is shown to allow the direct estimation of the single-scattering coefficient, two parameters describing the 'hot spot' phenomenon, and two parameters describing the scattering phase function. A comparison of inversion technique results with both synthetic data and actual observations shows the model to be capable of predicting the observed bidirectional reflectances as well as directional-hemispherical reflectances; it can also build the complete radiance field over the upward hemisphere.

Pinty, Bernard↗

DOE OSTI2024

Four Channel Time Multiplexed Photonic Doppler Velocimetry using an Optical Switch

Photonic Doppler Velocimetry (PDV) is a diagnostic commonly used in shock physics and dynamic compression experiments to reliably get velocity information from experiments. In PDV systems, a common method of reducing experimental cost is to use time and frequency multiplexing to increase the number of PDV probes. With time multiplexing, interference between probes is a frequent problem. In this report, we look at using a high-speed optical switch to reduce this interference, including measuring the amount of interference generated to determine if it has the potential to affect experiments and integrating a time multiplexing system into an experiment. We find that, when applied to PDV systems, there is approximately (-23.4 ± 0.9) dB of interference measured in the short time Fourier transform between switch inputs. When an optical switch based time multiplexing system was integrated into a dynamic compression experiment, the system was able to successfully combine the signals from four different PDV probes onto a single optical cable without unacceptable levels of interference in the spectrogram. An optical switch based time multiplexing system appears to be a promising method for reducing the cost of fielding larger numbers of PDV probes in an experiment.

47 OTHER INSTRUMENTATION↗

DOE OSTI2024

Analog optical signal transmission for HEP experiments

A critical element in all high-energy physics experiments is the signal transmission from the active elements to the data acquisition system. It is especially challenging in large volume detectors based on noble liquids that are extensively being used for dark matter and neutrino detection.The topic of this contribution is the optical signal transmission of the signals acquired with silicon photomultipliers, which is able to satisfy many stringent experimental requirements. It is RF-noise immune and operates in cryogenic liquids and in high-electric fields.This transmission system is based on commercially available electronics components and customized Fabry-Perot laser diodes.I will talk about encountered challenges, breakthrough, and advances from the original concept of this system up to final validation tests, demonstrating progressive developments.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

NASA NTRS1993

Infrared coronal emission lines and the possibility of their maser emission in Seyfert nuclei

Energetic emitting regions have traditionally been studied via x-ray, UV and optical emission lines of highly ionized intermediate mass elements. Such lines are often referred to as 'coronal lines' since the ions, when produced by collisional ionization, reach maximum abundance at electron temperatures of approx. 10(exp 5) - 10(exp 6) K typical of the sun's upper atmosphere. However, optical and UV coronal lines are also observed in a wide variety of Galactic and extragalactic sources including the Galactic interstellar medium, nova shells, supernova remnants, galaxies and QSOs. Infrared coronal lines are providing a new window for observation of energetic emitting regions in heavily dust obscured sources such as infrared bright merging galaxies and Seyfert nuclei and new opportunities for model constraints on physical conditions in these sources. Unlike their UV and optical counterparts, infrared coronal lines can be primary coolants of collisionally ionized plasmas with 10(exp 4) less than T(sub e)(K) less than 10(exp 6) which produce little or no optical or shorter wavelength coronal line emission. In addition, they provide a means to probe heavily dust obscured emitting regions which are often inaccessible to optical or UV line studies. In this poster, we provide results from new model calculations to support upcoming Infrared Space Observatory (ISO) and current ground-based observing programs involving infrared coronal emission lines in AGN. We present a complete list of infrared (lambda greater than 1 micron) lines due to transitions within the ground configurations 2s(2)2p(k) and 3s(2)3p(k) (k = 1 to 5) or the first excited configurations 2s2p and 3s3p of highly ionized (x greater than or equal to 100 eV) astrophysically abundant (n(X)/n(H) greater than or equal to 10(exp -6)) elements. Included are approximately 74 lines in ions of O, Ne, Na, Mg, Al, Si, S, Ar, Ca, Fe, and Ni spanning a wavelength range of approximately 1 - 280 microns. We present new results from detailed balance calculations, new critical densities for collisional de-excitation, intrinsic photon rates, branching ratios, and excitation temperatures for the majority of the compiled transitions. The temperature and density parameter space for dominant cooling via infrared coronal lines is presented, and the relationship of infrared to optical coronal lines is discussed.

Greenhouse, Matthew A.↗

DOE OSTI2025

Perspectives of active Si photonics devices for data communication and optical sensing

Si photonics has made rapid progress in research and commercialization in the past two decades. While it started with electronic–photonic integration on Si to overcome the interconnect bottleneck in data communications, Si photonics has now greatly expanded into optical sensing, light detection and ranging (LiDAR), optical computing, and microwave/RF photonics applications. From an applied physics point of view, this perspective discusses novel materials and integration schemes of active Si photonics devices for a broad range of applications in data communications, spectrally extended complementary metal–oxide–semiconductor (CMOS) image sensing, as well as 3D imaging for LiDAR systems. We also present a brief outlook of future synergy between Si photonic integrated circuits and Si CMOS image sensors toward ultrahigh capacity optical I/O, ultrafast imaging systems, and ultrahigh sensitivity lab-on-chip molecular biosensing.

electronic band structure↗

DOE OSTI2025

EM Physics

Geant4 provides a comprehensive set of electromagnetic (EM) processes and models for electron/positron, gamma and long-lived charged particles, spanning energies from 100 eV to 100 TeV. Covering diverse energy regions often requires multiple models, which can be constructed using pre-packaged or user-defined EM physics constructors. Geant4 also supports detailed low-energy EM physics through models like Livermore, Penelope, and ICRU73, offering extensive data for elements across a wide energy range (250 eV–100 GeV). Application domains include space, medical, and radiobiology simulations. Additionally, Geant4 provides robust options for simulating complex optical photon production and transportation processes, enhancing its versatility in physics research and applications.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

NASA NTRS1996

HAC: Band Gap, Photoluminescence, and Optical/Near-Infrared Absorption

We report results of laboratory measurements which illustrate the wide range of physical properties found among hydrogenated amorphous carbon (HAC) solids. Within this range, HAC can match quantitatively the astronomical phenomena ascribed to carbonaceous coatings on interstellar grains. We find the optical band gap of HAC to be well correlated with other physical properties of HAC of astronomical interest, and conclude that interstellar HAC must be fairly hydrogen-rich with a band gap of E(sub g) is approx. greater than 2.0 eV.

Witt, Adolf N.↗

NASA NTRS1990

Microwave and optical lunar transponders

The scientific areas which used data from the Lunar Laser Ranging Experiment, collected from measurements to the Apollo 11, 14, and 15 and Lunakhod 2, include lunar science (i.e., studies of variations in the lunar angular orientation from that for uniform rotation, lunar tidal displacements, and the lunar mass distribution), geodynamics, astrometry, and gravitational physics. This paper argues that the placement of microwave and optical transponders on the moon would improve the accuracy of laser range measurements by nearly two orders of magnitude and would simplify the measurements. The K-band microwave transponders would be operated at the lunar base and at two remote sites on the moon surface, yielding much improved lunar libration and tidal displacement measurements. A two-wavelength laser transponder also would be operated at the lunar base, allowing accurate tropospheric propagation corrections to be made. This would introduce major improvements in measurements of the lunar orbit and of the earth's rotation, and in tests of general relativity.

Bender, P. L.↗

DOE OSTI2022

Liquid Crystal‐Based Detection of Antigens with ELISA Sensitivity

Abstract A highly sensitive label‐free liquid crystal (LC)‐based technique is presented for detecting Immunoglobulin G (IgG) antigens used to uncover viral infections. The effectiveness, sensitivity, and selectivity of this detection method is demonstrated with goat IgG antigen at concentrations as low as 100 pg ml −1 , which is comparable to the sensitivity of the current enzyme‐linked immunosorbent assay (ELISA). The sensor is fabricated by decorating a transmission electron microscopy grid immobilized glass surfaces with antibodies; the target antigen is detected by a liquid crystal suspended onto the grid. This is different from previous methods where the antigen is detected either at the LC‐aqueous interface or in an LC sandwich cell with an antibody/antigen‐decorated substrate. This new approach has advantages such as easy sample preparation, higher sensitivity, and better storage capabilities. Binding the target antigen to the antibody results in a reorientation of the LC director that is detected optically. In addition to demonstrating the sensitivity, the physical principle of the detection is also discussed. This technique may apply to detect virtually any antigen of interest.

36 MATERIALS SCIENCE↗

DOE OSTI2024

Bulk reconstruction and non-isometry in the backwards-forwards holographic black hole map

The backwards-forwards map, introduced as a generalization of the non-isometric holographic maps of the black hole interior of Akers, Engelhardt, Harlow, Penington, and Vardhan to include non-trivial dynamics in the effective description, has two possible formulations differing in when the post-selection is performed. While these two forms are equivalent on the set of dynamically generated states — states formed from unitary time evolution acting on well-defined initial configurations of infalling matter — they differ on the generic set of states necessary to describe the apparent world of the infalling observer. We show that while both versions successfully reproduce the Page curve, the version involving post-selection as the final step, dubbed the backwards-forwards-post-selection (BFP) map, has the desirable properties of being non-isometric but isometric on average and providing state-dependent reconstruction of bulk operators, while the other version does not. Thus the BFP map is a suitable non-isometric code describing the black hole interior including interior interactions.

3-D Image Reconstruction↗

DOE OSTI2023

Anomalous hydrodynamics effective actions from holography

We derive an effective action for charged plasmas with an anomalous (abelian) global current charge current using holography. The holographic description is captured by the dynamics of an Einstein-Maxwell-Chern-Simons theory in an asymptotically AdS spacetime. The ’t Hooft anomaly contribution, which is encoded in the Chern-Simons term, contributes at the Gaussian order in the effective action only in the momentum diffusion sector, where it leads to chiral shear waves. However, as we demonstrate, beyond the Gaussian order, there is non-trivial imprint of the parity-violating anomaly term in sound and charge diffusion dynamics as well.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2021

Theoretical predictive screening of noble-metal-containing M 3 AuC 2 (M = Ti, V, and Cr) MAX phases

Using first-principles density functional theory (DFT), the ground state physical properties of the newly synthesized noble-metal-containing Ti 3 AuC 2 MAX phase have been investigated. The effect of transition-element Ti replacement (V and Cr) on physical properties, including structural, elastic, electronic, thermal, and optical are presented. The optimized lattice parameters of Ti 3 AuC 2 MAX phase are in good agreement with the experimental values and decrease when we replace Ti with V and then Cr. The magnetic properties of M 3 AuC 2 are predicted by using generalized gradient approximation (GGA) incorporating onsite electron correlation parameter (Hubbard U parameter) within DFT. Out of three studied MAX phases, V 3 AuC 2 and Cr 3 AuC 2 phases exhibit magnetism. The thermodynamical stability of M 3 AuC 2 (M = Ti, V, and Cr) phases is discussed by the formation enthalpy with respect to their most competing phases. The electronic structure reveals that these phases have metallic nature and are electrically anisotropic. The M-element replacement has an effect on the bonding properties of M 3 AuC 2 . The bonding between M-C is in the order of Cr 3 AuC 2 > V 3 AuC 2 > Ti 3 AuC 2 according to their peak positions and heights of density of states in the occupied site, which is also confirmed from the charge density distribution. The elastic properties indicate that M 3 AuC 2 phases are ductile, machinable, less stiff, and better resistant to thermal shock and are elastically anisotropic. To understand the properties of M 3 AuC 2 for the extreme environment, we employed a quasi-harmonic Debye model at the pressure and temperature range of 0–50 GPa and 0–1600 K, respectively. Additionally, we evaluated thermal conductivity and melting temperature to further understand the potential of these MAX phases in coating applications at elevated temperature. In relation to optical properties, these MAX phases have a reasonable absorption coefficient in the visible as well as in the ultra-violet regions. The reflectivity of M 3 AuC 2 phases is polarization dependent and of 45 % against the visible region, which reveals its potential as coating material to minimize solar heating.

312 MAX phases↗