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At least 1,675 records · Page 93
All sourcesNASA NTRSDOE OSTI
NASA NTRS1998

GCM Simulations of Cirrus Clouds and Cloud Feedbacks

Cirrus clouds are a particularly uncertain component of general circulation model (GCM simulations of long-term climate change for a variety of reasons: (1) They encompass a wide range of optical thicknesses and altitudes, from thin tropopause cirrus to thick anvil cirrus that descend to the freezing level, and thus can exert both positive and negative forcing and feedback on the climate; (2) The dynamical processes that create them are poorly resolved in climate GCMs and different in the tropics and midlatitudes; (3) Predictions of their formation and microphysical properties depend on the accuracy of dynamical transports of small concentrations of water vapor to and within the upper troposphere; (4) The relative humidity conditions at which they form depends on the nature and concentration of nucleating particles and is poorly understood; (5) They are more difficult to observe than other cloud types, and hence their parameterization is more loosely constrained by available data. We will illustrate the potential sensitivity of the perturbed climate to uncertainties in cirrus cloud formulation. We will also examine the processes that form cirrus in climate models and discuss the accuracy with which climate GCMs represent these processes. We will also discuss ways in which GCM grid-scale parameterizations might be derived from cloud-scale observations. Finally, we will emphasize the types of global observations needed to constrain parameterizations of cirrus in climate GCMs.

DelGenio, Anthony D.↗
NASA NTRS1997

X-ray Variability in M87

We present evidence for X-ray variability from the core and from knot A in the M87 jet based on data from two observations with the Einstein Observatory High Resolution Imager (HRI) and three observations with the ROSAT HRI. The core intensity showed a 16 per cent increase in 17 months (1979-80); a 12 per cent increase in the 3 years 1992 to 1995; and a 17 per cent drop in the last half of 1995. The intensity of knot A appears to have decreased by 16 per cent between 1992 June and 1995 December. Although the core variability is consistent with general expectations for AGN, the changes in knot A provide constraints on the X-ray emission process and geometry. Thus we predict that the X-ray morphology of knot A will differ significantly from the radio and optical structure.

Harris, D. E.↗
NASA NTRS2001

The Bermuda Bio-Optics Program (BBOP)

The Bermuda Bio-Optics Project (BBOP) is a collaborative effort between the Institute for Computational Earth System Science (ICESS) at the University of California at Santa Barbara (UCSB) and the Bermuda Biological Station for Research (BBSR). This research program is designed to characterize light availability and utilization in the Sargasso Sea, and to provide an optical link by which biogeochemical observations may be used to evaluate bio-optical models for pigment concentration, primary production, and sinking particle fluxes from satellite-based ocean color sensors. The BBOP time-series was initiated in 1992, and is carried out in conjunction with the US JGOFS Bermuda Atlantic Time-series Study (BATS) at the Bermuda Biological Station for Research. The BATS program itself has been observing biogeochemical processes (primary productivity, particle flux at and elemental cycles) in the mesotrophic waters of the Sargasso Sea since 1988. Closely affiliated with BBOP and BATS is a separate NASA-funded study of the spatial variability of biogeochemical processes in the Sargasso Sea using high-resolution Advanced Very High Resolution Radiometer (AVHRR) and Sea-Viewing Wide Field-of-view Sensor (SeaWiFS) data collected at Bermuda. The collaboration between BATS and BBOP measurements has resulted in a unique data set that addresses not only the SIMBIOS goals but also the broader issues of important factors controlling the carbon cycle.

Siegel, David A.↗
NASA NTRS2007

Space Flight Requirements for Fiber Optic Components; Qualification Testing and Lessons Learned

"Qualification" of fiber optic components holds a very different meaning than it did ten years ago. In the past, qualification meant extensive prolonged testing and screening that led to a programmatic method of reliability assurance. For space flight programs today, the combination of using higher performance commercial technology, with shorter development schedules and tighter mission budgets makes long term testing and reliability characterization unfeasible. In many cases space flight missions will be using technology within years of its development and an example of this is fiber laser technology. Although the technology itself is not a new product the components that comprise a fiber laser system change frequently as processes and packaging changes occur. Once a process or the materials for manufacturing a component change, even the data that existed on its predecessor can no longer provide assurance on the newer version. In order to assure reliability during a space flight mission, the component engineer must understand the requirements of the space flight environment as well as the physics of failure of the components themselves. This can be incorporated into an efficient and effective testing plan that "qualifies" a component to specific criteria defined by the program given the mission requirements and the component limitations. This requires interaction at the very initial stages of design between the system design engineer, mechanical engineer, subsystem engineer and the component hardware engineer. Although this is the desired interaction what typically occurs is that the subsystem engineer asks the components or development engineers to meet difficult requirements without knowledge of the current industry situation or the lack of qualification data. This is then passed on to the vendor who can provide little help with such a harsh set of requirements due to high cost of testing for space flight environments. This presentation is designed to guide the engineers of design, development and components, and vendors of commercial components with how to make an efficient and effective qualification test plan with some basic generic information about many space flight requirements. Issues related to the ~ physics of failure, acceptance criteria and lessons learned will also be discussed to assist with understanding how to approach a space flight mission in an ever changing commercial photonics industry.

Ott, Melanie N.↗
NASA NTRS2015

Deploying the NASA Meter Class Autonomous Telescope (MCAT) on Ascension Island

NASA has successfully constructed the 1.3m Meter Class Autonomous Telescope (MCAT) facility on Ascension Island in the South Atlantic Ocean. MCAT is an optical telescope designed specifically to collect ground-based data for the statistical characterization of orbital debris ranging from Low Earth Orbit (LEO) through Middle Earth Orbits (MEO) and beyond to Geo Transfer and Geosynchronous Orbits (GTO/GEO). The location of Ascension Island has two distinct advantages. First, the near-equatorial location fills a significant longitudinal gap in the Ground-based Electro-Optical Deep Space Surveillance (GEODSS) network of telescopes, and second, it allows access to objects in Low Inclination Low-Earth Orbits (LILO). The MCAT facility will be controlled by a sophisticated software suite that operates the dome and telescope, assesses sky and weather conditions, conducts all necessary calibrations, defines an observing strategy (as dictated by weather, sky conditions and the observing plan for the night), and carries out the observations. It then reduces the collected data via four primary observing modes ranging from tracking previously cataloged objects to conducting general surveys for detecting uncorrelated debris. Nightly observing plans, as well as the resulting text file of reduced data, will be transferred to and from Ascension, respectively, via a satellite connection. Post-processing occurs at NASA Johnson Space Center. Construction began in September, 2014 with dome and telescope installation occurring in April through early June, 2015. First light was achieved in June, 2015. Acceptance testing, full commissioning, and calibration of this soon-to-be fully autonomous system commenced in summer 2015. The initial characterization of the system from these tests is presented herein.

Lederer, S. M.↗
NASA NTRS1990

Acousto-optic signature analysis for inspection of the orbiter thermal protection tile bonds

The goal of this research is to develop a viable NDE technique for the inspection of orbiter thermal protection system (TPS) tile bonds. Phase 2, discussed here, concentrated on developing an empirical understanding of the bonded and unbonded vibration signatures of acreage tiles. Controlled experiments in the laboratory have provided useful information on the dynamic response of TPS tiles. It has been shown that several signatures are common to all the pedigree tiles. This degree of consistency in the tile-SIP (strain isolation pad) dynamic response proves that an unbond can be detected for a known tile and establish the basis for extending the analysis capability to arbitrary tiles for which there are no historical data. The field tests of the noncontacting laser acoustic sensor system, conducted at the Kennedy Space Center (KSC), investigated the vibrational environment of the Orbiter Processing Facility (OPF) and its effect on the measurement and analysis techniques being developed. The data collected showed that for orbiter locations, such as the body flap and elevon, the data analysis scheme, and/or the sensor, will require modification to accommodate the ambient motion. Several methods were identified for accomplishing this, and a solution is seen as readily achievable. It was established that the tile response was similar to that observed in the laboratory. Of most importance, however, is that the field environment will not affect the physics of the dynamic response that is related to bond condition. All of this information is fundamental to any future design and development of a prototype system.

Rodriguez, Julio G.↗
NASA NTRS2006

A Coupled GCM-Cloud Resolving Modeling System, and A Regional Scale Model to Study Precipitation Processes

Recent GEWEX Cloud System Study (GCSS) model comparison projects have indicated that cloud-resolving models (CRMs) agree with observations better than traditional single-column models in simulating various types of clouds and cloud systems from different geographic locations. Current and future NASA satellite programs can provide cloud, precipitation, aerosol and other data at very fine spatial and temporal scales. It requires a coupled global circulation model (GCM) and cloud-scale model (termed a super-parameterization or multi-scale modeling framework, MMF) to use these satellite data to improve the understanding of the physical processes that are responsible for the variation in global and regional climate and hydrological systems. The use of a GCM will enable global coverage, and the use of a CRM will allow for better and more sophisticated physical parameterization. NASA satellite and field campaign cloud related datasets can provide initial conditions as well as validation for both the MMF and CRMs. The Goddard MMF is based on the 2D Goddard Cumulus Ensemble (GCE) model and the Goddard finite volume general circulation model (fvGCM), and it has started production runs with two years results (1998 and 1999). Also, at Goddard, we have implemented several Goddard microphysical schemes (21CE, several 31CE), Goddard radiation (including explicitly calculated cloud optical properties), and Goddard Land Information (LIS, that includes the CLM and NOAH land surface models) into a next generation regional scale model, WRF. In this talk, I will present: (1) A brief review on GCE model and its applications on precipitation processes (microphysical and land processes), (2) The Goddard MMF and the major difference between two existing MMFs (CSU MMF and Goddard MMF), and preliminary results (the comparison with traditional GCMs), and (3) A discussion on the Goddard WRF version (its developments and applications).

Tao, Wei-Kuo↗
NASA NTRS2007

A Coupled GCM-Cloud Resolving Modeling System, and a Regional Scale Model to Study Precipitation Processes

Recent GEWEX Cloud System Study (GCSS) model comparison projects have indicated that cloud-resolving models (CRMs) agree with observations better than traditional single-column models in simulating various types of clouds and cloud systems from different geographic locations. Current and future NASA satellite programs can provide cloud, precipitation, aerosol and other data at very fine spatial and temporal scales. It requires a coupled global circulation model (GCM) and cloud-scale model (termed a superparameterization or multi-scale modeling framework, MMF) to use these satellite data to improve the understanding of the physical processes that are responsible for the variation in global and regional climate and hydrological systems. The use of a GCM will enable global coverage, and the use of a CRM will allow for better and more sophisticated physical parameterization. NASA satellite and field campaign cloud related datasets can provide initial conditions as well as validation for both the MMF and CRMs. The Goddard MMF is based on the 2D Goddard Cumulus Ensemble (GCE) model and the Goddard finite volume general circulation model (fvGCM), and it has started production runs with two years results (1998 and 1999). Also, at Goddard, we have implemented several Goddard microphysical schemes (2ICE, several 31CE), Goddard radiation (including explicitly calculated cloud optical properties), and Goddard Land Information (LIS, that includes the CLM and NOAH land surface models) into a next generatio11 regional scale model, WRF. In this talk, I will present: (1) A brief review on GCE model and its applications on precipitation processes (microphysical and land processes), (2) The Goddard MMF and the major difference between two existing MMFs (CSU MMF and Goddard MMF), and preliminary results (the comparison with traditional GCMs), and (3) A discussion on the Goddard WRF version (its developments and applications).

Tao, Wei-Kuo↗
NASA NTRS2014

Limb Correction of RGB Composite Imagery for Improved Interpretation

RGB (Red‐Green‐Blue) imagery, created by integrating several spectral channels into one composite image, is currently used by the operational weather community to aid in quick, real‐time analysis of atmospheric processes. However, the limb effect - a result of an increasing optical path length of the absorbing atmosphere between the satellite and the earth as scan angle increases - interferes with the qualitative interpretation of RGB composites at large scan angles. It also makes the comparison of similar products from multiple satellite sensors difficult. Recent work has indicated that correcting for the limb effect in the basic channel imagery using simple statistical relationships greatly improves the utility of the derived RGB imagery. However, it is hypothesized that the limb correction coefficients vary with respect to latitude, season, cloud cover, and surface albedo. This poster will highlight an improved approach to the limb correction of RGB imagery using varying coefficients. The Joint Center for Satellite and Data Assimilation (JCSDA) Community Radiative Transfer Model (CRTM) was used to simulate top of atmosphere brightness temperatures at varying scan angles for infrared channels corresponding to the Aqua and Terra Moderate Resolution Imaging Spectroradiometer (MODIS), Suomi NPP Visible Infrared Imaging Radiometer Suite (VIIRS), and Meteosat‐10 Spinning Enhanced Visible and Infrared Imager (SEVIRI) sensors. A subset of European Center for Medium‐Range Weather Forecasts (ECMWF) temperature, specific humidity, and ozone mixing ratio profiles from March 2013 through February 2014 were used as input to the CRTM. The simulated brightness temperatures were used to determine the best fit slope of the linear relationship between the natural log of the cosine of the scan angle and the difference of the simulated brightness temperature at nadir and on the limb. The correction coefficients were then analyzed for variability with respect to latitude, season, cloud cover, and surface type and used to produce improved limb corrected imagery. Applications of the results will be presented.

Elmer, Nicholas↗
NASA NTRS2019

Multi-Band Atmospheric Correction Algorithm for Ocean Color Retrievals

NASA's current Atmospheric Correction (AC) algorithm for ocean color utilizes two bands and their ratio in the Near Infrared (NIR) to estimate aerosol reflectance and aerosol type. The algorithm then extrapolates the spectral dependence of aerosol reflectance to the visible wavelengths based on modeled spectral dependence of the identified aerosol type. Future advanced ocean color sensors, such as the Ocean Color Instrument (OCI) that will be carried on the Plankton, Aerosol, Cloud, and ocean Ecosystem (PACE) satellite, will be capable of measuring the hyperspectral radiance from 340 to 890 nm at 5-nm spectral resolution and at 7 discrete Short-wave Infrared (SWIR) channels: 940, 1038,1250, 1378, 1615, 2130, and 2260 nm. To optimally employ this unprecedented instrument capability, we propose an improved AC algorithm that utilizes all atmospheric-window channels in the NIR to SWIR spectral range to reduce the uncertainty in the AC process. A theoretical uncertainty analysis of this, namely Multi-Band AC (MBAC), indicates that the algorithm can reduce the uncertainty in remote sensing reflectance (Rrs) retrievals of the ocean caused by sensor random noise. Furthermore, in optically complex waters, where the NIR signal is affected by contributions from highly-reflective turbid waters, the MBAC algorithm can be adaptively weighted to the strongly-absorbing SWIR channels to enable improved ocean color retrievals in coastal waters. We provide here a description of the algorithm and demonstrate the improved performance in ocean color retrievals, relative to the current NASA standard AC algorithm, through comparison with field measurements and assessment of propagated uncertainties in applying the MBAC algorithm to MODIS and simulated PACE OCI data.

PACE↗
NASA NTRSDate not supplied

The International Space Station Lightning Imaging Sensor: Performance, Applications, and Cross-Platform Science

The Lightning Imaging Sensor (LIS), an optically based lightning detector developed at NASA Marshall Space Flight Center, was launched to the International Space Station (ISS) in February 2017, detecting optical signatures of lightning with storm-scale horizontal resolution (4-km) during both day and night. ISS LIS data are available 1 March 2017 to present. Millisecond timing allows detailed intercalibration and validation with other spaceborne and ground-based lightning sensors. Initial comparisons with those other sensors suggest flash detection efficiency around 60% (diurnal variability of 51-75%), false alarm rate under 5%, timing accuracy better than 2 ms, and horizontal location accuracy around 3 km. The spatially uniform flash detection capability of ISS LIS from low-Earth orbit allows assessment of spatially varying flash detection efficiency for other sensors and networks, particularly the Geostationary Lightning Mappers (GLMs). ISS LIS provides research data suitable for investigations of lightning physics, climatology, thunderstorm processes, and atmospheric composition, as well as realtime lightning data for operational forecasting and aviation weather interests. ISS LIS enables enrichment and extension of the long-term global climatology of lightning from space, and is the only recent platform that extends the global record to higher latitudes (± 55°). The global spatial distribution of lightning from ISS LIS is broadly similar to previous datasets, with globally averaged seasonal/annual flash rates (3-year average: ~44 s) about 5-10% lower. This difference is likely due to reduced flash detection efficiency that will be mitigated in future ISS LIS data processing, as well as the shorter ISS LIS period of record. The expected land/ocean contrast in the diurnal variability of global lightning is also observed. The near-realtime ISS LIS data make the instrument important to operational weather forecasting and related applications, including public safety. Finally, ISS LIS is demonstrating utility as part (or potential part) of cross-platform studies examining a diverse array of topics, including lightning physics, thunderstorm processes, convective precipitation, and atmospheric composition.

Timothy Lang↗
NASA NTRS1988

Development of a high-speed H-alpha camera system for the observation of rapid fluctuations in solar flares

A solid-state digital camera was developed for obtaining H alpha images of solar flares with 0.1 s time resolution. Beginning in the summer of 1988, this system will be operated in conjunction with SMM's hard X-ray burst spectrometer (HXRBS). Important electron time-of-flight effects that are crucial for determining the flare energy release processes should be detectable with these combined H alpha and hard X-ray observations. Charge-injection device (CID) cameras provide 128 x 128 pixel images simultaneously in the H alpha blue wing, line center, and red wing, or other wavelength of interest. The data recording system employs a microprocessor-controlled, electronic interface between each camera and a digital processor board that encodes the data into a serial bitstream for continuous recording by a standard video cassette recorder. Only a small fraction of the data will be permanently archived through utilization of a direct memory access interface onto a VAX-750 computer. In addition to correlations with hard X-ray data, observations from the high speed H alpha camera will also be correlated and optical and microwave data and data from future MAX 1991 campaigns. Whether the recorded optical flashes are simultaneous with X-ray peaks to within 0.1 s, are delayed by tenths of seconds or are even undetectable, the results will have implications on the validity of both thermal and nonthermal models of hard X-ray production.

Kiplinger, Alan L.↗
NASA NTRS2007

Optical Measurements in a Combustor Using a 9-Point Swirl-Venturi Fuel Injector

This paper highlights the use of two-dimensional data to characterize a multipoint swirl-venturi injector. The injector is based on a NASA-conceived lean direct injection concept. Using a variety of advanced optical diagnostic techniques, we examine the flows resultant from multipoint, lean-direct injectors that have nine injection sites arranged in a 3 x 3 grid. The measurements are made within an optically-accessible, jet-A-fueled, 76-mm by 76-mm flame tube combustor. Combustion species mapping and velocity measurements are obtained using planar laser-induced fluorescence of OH and fuel, planar laser scatter of liquid fuel, chemiluminescence from CH*, NO*, and OH*, and particle image velocimetry of seeded air (non-fueled). These measurements are used to study fuel injection, mixedness, and combustion processes and are part of a database of measurements that will be used for validating computational combustion models.

Hicks, Yolanda R.↗
NASA NTRS2021

Three-Dimensional Measurement of the Crater Formation During Plume–Surface Interactions Using Stereo-Photogrammetry

The present investigation focused on adapting and validating stereo-photogrammetry for obtaining 3-D, time-resolved, non-intrusive, full-domain measurements of crater evolution during the plume-surface interaction (PSI) process. An atmospheric experimental facility was designed and constructed to facilitate the development of the stereo-photogrammetry technique for PSI applications. Stereo-photogrammetry was then used to measure the dynamic crater evolution process at nozzle heights of 25, 40, 55, and 70 nozzle diameters above the sand simulant bed. From the stereo-photogrammetry data, time-resolved 3-D reconstructions of the crater geometry were generated, and crater depth, radius, and volume time histories were extracted. Crater depth was observed to grow logarithmically for the two highest nozzle heights, and the depth growth rate for the lower two nozzle heights was more rapid. Crater volume growth was well characterized by a power law fit. The slope of the collapsed crater post nozzle flow was found to increase with nozzle height, along with the final crater volume. The results show that stereo-photogrammetry can be used to successfully measure the crater geometry in cases where optical access to the crater is not completely degraded by ejected particles.

DC Stubbs↗
NASA NTRSDate not supplied

Open Source Application of Fusing Aerosol Products from GEO and LEO Satellites

Retrieving aerosol optical depths (AODs) from sun-synchronous polar orbiting (aka low earth orbit, LEO) satellites, such as MODISs, and VIIRSs, OMI, TROPOMI, etc, has become well-established as a tool for extracting information on particulate matter (PM) and related processes in the atmosphere. However, with recently launched geostationary satellites (GEO), such as GOES-16/17/18, and Himawari-8/9, and Meteosat Third Generation (MTG) they provide a much higher temporal resolution (order of 10 minutes), typically an image once or more per hour during daylight compared to LEO once per day. By combining these observations, we may be able to characterize the diurnal cycle of global AOD at the local, regional and global scale. While the science community is still exploring the new data from GEO observations, we have been thinking about how to properly combine/merge/fuse those data considering differences in their spatial and temporal resolutions. However, this poses a “Big Data” challenge. The big data challenge is not just about data storage, but also about data discoverability, and accessibility, and even more, about data migration/mirroring in the cloud-computing environment. This paper is merely showing some of the efforts and approaches we have attempted in fusing six satellites’ Level 2 aerosol data (three are from GEO (GOES-16/17 and Himawari-8), and the other three are from LEO (TERRA/MODIS, AQUA/MODIS, SNPP-VIIRS) from Dark Target (DT) aerosol retrieval algorithm. Having the on-demand capability of fusing remote sensing products onto the desired temporal and spatial domain enables researchers and application practitioners to better manipulate and work with satellite and sensor data. It is our hopeWe hope that by making such an open-source package, and the accompanying functionality, the scientific community will be granted easier access to aerosol data processing resources. The MEaSUREs Program (Making Earth System Data Records for Use in Research Environments) expands our understanding of the Earth's current system through atmospheric and surface measurements. In an effort to aid the scientific research component and improve open source methods, this project developed Python code for fusing six satellite Level 2 aerosol data (three are from geostationary satellites (GEO), and the other three are from low earth orbital satellites (LEO)) from Dark Target Aerosol Retrieval Algorithm.

Jennifer Wei↗
NASA NTRS1993

Design and specification of a centralized manufacturing data management and scheduling system

As was revealed in a previous study, the Materials and Processes Laboratory's Productivity Enhancement Complex (PEC) has a number of automated production areas/cells that are not effectively integrated, limiting the ability of users to readily share data. The recent decision to utilize the PEC for the fabrication of flight hardware has focused new attention on the problem and brought to light the need for an integrated data management and scheduling system. This report addresses this need by developing preliminary designs specifications for a centralized manufacturing data management and scheduling system for managing flight hardware fabrication in the PEC. This prototype system will be developed under the auspices of the Integrated Engineering Environment (IEE) Oversight team and the IEE Committee. At their recommendation the system specifications were based on the fabrication requirements of the AXAF-S Optical Bench.

Farrington, Phillip A.↗
NASA NTRS1995

Ocean observations with EOS/MODIS: Algorithm development and post launch studies

Several significant accomplishments were made during the present reporting period. (1) Initial simulations to understand the applicability of the MODerate Resolution Imaging Spectrometer (MODIS) 1380 nm band for removing the effects of stratospheric aerosols and thin cirrus clouds were completed using a model for an aged volcanic aerosol. The results suggest that very simple procedures requiring no a priori knowledge of the optical properties of the stratospheric aerosol may be as effective as complex procedures requiring full knowledge of the aerosol properties, except the concentration which is estimated from the reflectance at 1380 nm. The limitations of this conclusion will be examined in the next reporting period; (2) The lookup tables employed in the implementation of the atmospheric correction algorithm have been modified in several ways intended to improve the accuracy and/or speed of processing. These have been delivered to R. Evans for implementation into the MODIS prototype processing algorithm for testing; (3) A method was developed for removal of the effects of the O2 'A' absorption band from SeaWiFS band 7 (745-785 nm). This is important in that SeaWiFS imagery will be used as a test data set for the MODIS atmospheric correction algorithm over the oceans; and (4) Construction of a radiometer, and associated deployment boom, for studying the spectral reflectance of oceanic whitecaps at sea was completed. The system was successfully tested on a cruise off Hawaii on which whitecaps were plentiful during October-November. This data set is now under analysis.

Gordon, Howard R.↗
NASA NTRS2004

Microgravity Studies of Liquid-Liquid Phase Transitions in Alumina-Yttria Melts

The scientific objective of this research is to increase the fundamental knowledge base for liquid- phase processing of technologically important oxide materials. The experimental objective is to define conditions and hardware requirements for microgravity flight experiments to test and expand the experimental hypotheses that: 1. Liquid phase transitions can occur in undercooled melts by a diffusionless process. 2. Onset of the liquid phase transition is accompanied by a large change in the temperature dependence of melt viscosity. Experiments on undercooled YAG (Y3A15012)- and rare earth oxide aluminate composition liquids demonstrated a large departure from an Arrhenian temperature dependence of viscosity. Liquid YAG is nearly inviscid at its 2240 K melting point. Glass fibers were pulled from melts undercooled by ca. 600 K indicating that the viscosity is on the order of 100 Pans (1000 Poise) at 1600 K. This value of viscosity is 500 times greater than that obtained by extrapolation of data for temperatures above the melting point of YAG. These results show that the liquids are extremely fragile and that the onset of the highly non-Arrhenian viscosity-temperature relationship occurs at a temperature considerably below the equilibrium melting point of the solid phases. Further results on undercooled alumina-yttria melts containing 23-42 mole % yttrium oxide indicate that a congruent liquid-liquid phase transition occurs in the undercooled liquids. The rates of transition are inconsistent with a diffusion-limited process. This research is directed to investigation of the scientifically interesting phenomena of polyamorphism and fragility in undercooled rare earth oxide aluminum oxide liquids. The results bear on the technologically important problem of producing high value rare earth-based optical materials.

Guynes, Buddy↗