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DOE OSTI2023

Quantitative investigation of sooting dynamics in droplet combustion using an automated image analysis algorithm

This paper reports an image analysis approach using a newly-developed open-source program to extract quantitative measurements of soot volume fraction (SVF) from digital video images of burning n-heptane droplets. The automated program developed in this work can analyze images of fixed and untethered droplets to quantify sooting dynamics. The images analyzed in the program were taken from experiments carried out in the Multi-user Droplet Combustion Apparatus (MDCA) onboard the International Space Station (ISS). In these experiments, video imaging of burning droplets was obtained using backlighting by a laser diode with a wavelength of 653 nm. Here, the light was collimated before it passed through the droplet and soot-containing region, after which the light was then attenuated and projected onto the camera’s sensors. This technique facilitates the measurements of SVF based on the principles of the full field light extinction method (FFLEM). The measurements provide quantitative data that reveal the sooting dynamics of liquid fuels during droplet combustion processes. The analyses of a soot-attenuating image (ISS n-heptane, untethered droplet) at an instant during the burning show that the SVF distribution has a peak at the soot shell location. It then decreases due to soot oxidation when the location is further away from the burning droplet. Regarding temporal effects on the maximum SVF (SVF max ), results show that SVF max first increases after the burning is initiated until a peak value is reached, after which SVF max decreases. The SVF max values identified in this study for n-heptane are quantitatively consistent with previously reported values for fiber-supported droplets and are reached relatively early in the burning history. n-Heptane images are also analyzed to show the effects of initial droplet sizes on the maximum soot volume fraction. Results show that SVF max decreases with increasing initial droplet size, which is consistent with visual observations of less soot formed and dimmer flame brightness as Do increases.

42 ENGINEERING↗

DOE OSTI2023

Global fire modelling and control attributions based on the ensemble machine learning and satellite observations

Contemporary fire dynamics is one of the most complex and least understood land surface phenomena. Global fire controls related to climate, vegetation, and anthropogenic activity are usually intertwined, and difficult to disentangle in a quantitative way. Here, we leveraged an ensemble of five machine learning (ML) models and multiple satellite-based observations to conduct global fire modeling for three fire metrics (burned area, fire number, and fire size), and quantified driving mechanisms underlying annual fire changes in a spatially resolved manner for the period 2003–2019. Ensemble learning is a meta-approach that combines multiple ML predictions to improve accuracy, robustness, and generalization performance. We found that the optimized ensemble ML well reproduced annual dynamics of global burned area (R 2 = 0.90, P < 0.001), total fire numbers (R 2 = 0.86, P < 0.001), and averaged fire size (R 2 = 0.70, P < 0.001). Additionally, the ensemble ML captured key spatial patterns of multi-year mean magnitudes, annual variabilities, anomalies, and trends for different fire metrics. Our ML-based fire attributions further highlighted the dominant role of enhanced anthropogenic activity in reducing global burned area (–1.9 Mha/yr, P < 0.01), followed by climate control (–1.3 Mha/yr, P < 0.01) and insignificant positive vegetation control (0.4 Mha/yr, P = 0.60). Spatially, climate dominated a much larger burned area (53.7%) than human (23.4%) or vegetation control (22.9%); however, the counteracting effects from regional wetting and drying trends weakened the net climate impacts on global burned area. The fire number and fire size exhibited similar spatial control patterns with burned area; globally, however, fire number tended to be more affected by climate while fire size more influenced by human activities. Overall, our study confirmed the feasibility and efficiency of ensemble ML in global fire modeling and subsequent control attributions, providing a better understanding of contemporary fire regimes and contributing to robust fire projections in a changing environment.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2012

Kinetics of small single particle combustion of zirconium alloy

We present quantitative kinetic information regarding small, 1-10 {mu}m in diameter, single particle combustion of Zr-rich metal alloy foils subjected to either mechanical impacts or laser-ablation. The lights from combustion of metal fragments were recorded on a high-speed camera. The particle size was determined by the motion analysis of individual particle trajectory based on an aerodynamic drag law and further verified by the microstructure and chemical composition analysis of recovered post-burn particles. The measured particle sizes show a log-normal distribution centered at around 3.1 {mu}m in diameter, and the composition of recovered particles is that of fully oxidized ZrO{sub 2}. The temperature evolution of each particle along the space/time-trajectory is determined based on the thermal emission from combustion using a single-color photographic spectro-pyrometry. The result indicates that the particle has reached the maximum combustion temperature of 4000 K, well beyond the melting temperature of ZrO{sub 2}, and undergone the solidification of molten ZrO{sub 2} during the cooling stage. It also shows that the maximum combustion temperature decreases linearly with increasing the particle diameter, following the correlation t aD{sup 1.5-1.8} between the burn time (t) and the particle diameter (D). Combining the particle size, the burn time, and the particle temperature, both temperature and mass burn rates are obtained as a function of particle size. As the particle size increases, the temperature burn rate decreases, whereas the mass burn rate goes in the opposite direction.

36 MATERIALS SCIENCE↗

DOE OSTI2012

The neutron imaging diagnostic at NIF (invited)

A neutron imaging diagnostic has recently been commissioned at the National Ignition Facility (NIF). This new system is an important diagnostic tool for inertial fusion studies at the NIF for measuring the size and shape of the burning DT plasma during the ignition stage of Inertial Confinement Fusion (ICF) implosions. The imaging technique utilizes a pinhole neutron aperture, placed between the neutron source and a neutron detector. The detection system measures the two dimensional distribution of neutrons passing through the pinhole. This diagnostic has been designed to collect two images at two times. The long flight path for this diagnostic, 28 m, results in a chromatic separation of the neutrons, allowing the independently timed images to measure the source distribution for two neutron energies. Typically the first image measures the distribution of the 14 MeV neutrons and the second image of the 6-12 MeV neutrons. The combination of these two images has provided data on the size and shape of the burning plasma within the compressed capsule, as well as a measure of the quantity and spatial distribution of the cold fuel surrounding this core.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

DOE OSTI2024

Soil microbiome feedbacks during disturbance-driven forest ecosystem conversion

Abstract Disturbances cause rapid changes to forests, with different disturbance types and severities creating unique ecosystem trajectories that can impact the underlying soil microbiome. Pile burning—the combustion of logging residue on the forest floor—is a common fuel reduction practice that can have impacts on forest soils analogous to those following high-severity wildfire. Further, pile burning following clear-cut harvesting can create persistent openings dominated by nonwoody plants surrounded by dense regenerating conifer forest. A paired 60-year chronosequence of burn scar openings and surrounding regenerating forest after clear-cut harvesting provides a unique opportunity to assess whether belowground microbial processes mirror aboveground vegetation during disturbance-induced ecosystem shifts. Soil ectomycorrhizal fungal diversity was reduced the first decade after pile burning, which could explain poor tree seedling establishment and subsequent persistence of herbaceous species within the openings. Fine-scale changes in the soil microbiome mirrored aboveground shifts in vegetation, with short-term changes to microbial carbon cycling functions resembling a postfire microbiome (e.g. enrichment of aromatic degradation genes) and respiration in burn scars decoupled from substrate quantity and quality. Broadly, however, soil microbiome composition and function within burn scar soils converged with that of the surrounding regenerating forest six decades after the disturbances, indicating potential microbial resilience that was disconnected from aboveground vegetation shifts. This work begins to unravel the belowground microbial processes that underlie disturbance-induced ecosystem changes, which are increasing in frequency tied to climate change.

Nelson, Amelia R.↗

DOE OSTI2024

Case study of UAS ignition of prescribed fire in a mixedwood on the William B. Bankhead National Forest, Alabama

Abstract Background For at least four decades, practitioners have recognized advantages of aerial versus ground ignition for maximizing the effectiveness of prescribed fires. For example, larger areas can be ignited in less time, or ignition energy may be variously targeted over an area in accordance with the uneven distribution of fuels. The maturation of wireless communication, geopositioning systems, and unmanned aerial systems (UAS) has enhanced those advantages, and UAS approaches also provide further advantages relative to helicopter ignitions, such as reduced risk to human safety, lower operating costs, and higher operational flexibility. In a long running study at the Bankhead National Forest in northcentral Alabama, prescribed fire has been used for nearly 20 years. Most of the burns have been hand-ignited via drip torches, while some have been aerially ignited via helicopter. In March 2022, for the first time, a UAS was used to ignite prescribed fires across a landscape that included a long-term research stand. This field note relates comparisons of both fire behavior and fuel consumption metrics for the UAS-ignited burn versus previous burns on the same stand, and versus burns of other research stands in the same year. Results The UAS-ignited prescribed fire experienced burn effects similar to those from ground-ignited prescribed fires on the same stand in previous years, as well as those from ground-ignited prescribed fires on other stands in the same year. Conclusion This post hoc analysis suggests that UAS ignition approaches may be sufficient for achieving prescribed burn goals, thereby enabling practitioners to realize the advantages offered by that ignition mode.

Environmental Sciences & Ecology↗

DOE OSTI2012

Alternative Fuel for Portland Cement Processing

The production of cement involves a combination of numerous raw materials, strictly monitored system processes, and temperatures on the order of 1500 °C. Immense quantities of fuel are required for the production of cement. Traditionally, energy from fossil fuels was solely relied upon for the production of cement. The overarching project objective is to evaluate the use of alternative fuels to lessen the dependence on non-renewable resources to produce portland cement. The key objective of using alternative fuels is to continue to produce high-quality cement while decreasing the use of non-renewable fuels and minimizing the impact on the environment. Burn characteristics and thermodynamic parameters were evaluated with a laboratory burn simulator under conditions that mimic those in the preheater where the fuels are brought into a cement plant. A drop-tube furnace and visualization method were developed that show potential for evaluating time- and space-resolved temperature distributions for fuel solid particles and liquid droplets undergoing combustion in various combustion atmospheres. Downdraft gasification has been explored as a means to extract chemical energy from poultry litter while limiting the throughput of potentially deleterious components with regards to use in firing a cement kiln. Results have shown that the clinkering is temperature independent, at least within the controllable temperature range. Limestone also had only a slight effect on the fusion when used to coat the pellets. However, limestone addition did display some promise in regards to chlorine capture, as ash analyses showed chlorine concentrations of more than four times greater in the limestone infused ash as compared to raw poultry litter. A reliable and convenient sampling procedure was developed to estimate the combustion quality of broiler litter that is the best compromise between convenience and reliability by means of statistical analysis. Multi-day trial burns were conducted at a full-scale cement plant with alternative fuels to examine their compatibility with the cement production process. Construction and demolition waste, woodchips, and soybean seeds were used as alternative fuels at a full-scale cement production facility. These fuels were co-fired with coal and waste plastics. The alternative fuels used in this trial accounted for 5 to 16 % of the total energy consumed during these burns. The overall performance of the portland cement produced during the various trial burns performed for practical purposes very similar to the cement produced during the control burn. The cement plant was successful in implementing alternative fuels to produce a consistent, high-quality product that increased cement performance while reducing the environmental footprint of the plant. The utilization of construction and demolition waste, woodchips and soybean seeds proved to be viable replacements for traditional fuels. The future use of these fuels depends on local availability, associated costs, and compatibility with a facility's production process.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗

DOE OSTI2015

Status of Readiness to Receive and Store Sister Rods from the R&D Project

While low burn-up fuel [that characterized as having a burn-up of less than 45 gigawatt days per metric ton uranium (GWD/MTU)] has been stored for nearly three decades, the storage of high burn-up used fuels is more recent. The DOE has funded a High Burn-Up (HBU) Confirmatory Data Project to confirm the behavior of used high burn-up fuel under prototypic conditions. The Electric Power Research Institute (EPRI) is leading a project team to develop and implement the Test Plan to collect this data from a UNF dry storage system containing high burn-up fuel. As part of that project, 25 “sister” fuel rods have been selected, removed from assemblies, and placed in a fuel container ready for shipment to a national laboratory. This report documents that status of readiness to receive the fuel if that fuel were to be sent to Idaho National Laboratory (INL).

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

DOE OSTI2016

Hybrid fs/ps CARS for Sooting and Particle-laden Flames [PowerPoint]

We report the application of ultrafast rotational coherent anti-Stokes Raman scattering (CARS) for temperature and relative oxygen concentration measurements in the plume emanating from a burning aluminized ammonium perchlorate propellant strand. Combustion of these metal-based propellants is a particularly hostile environment for laserbased diagnostics, with intense background luminosity, scattering and beam obstruction from hot metal particles that can be as large as several hundred microns in diameter. CARS spectra that were previously obtained using nanosecond pulsed lasers in an aluminumparticle- seeded flame are examined and are determined to be severely impacted by nonresonant background, presumably as a result of the plasma formed by particulateenhanced laser-induced breakdown. Introduction of fs/ps laser pulses enables CARS detection at reduced pulse energies, decreasing the likelihood of breakdown, while simultaneously providing time-gated elimination of any nonresonant background interference. Temperature probability densities and temperature/oxygen correlations were constructed from ensembles of several thousand single-laser-shot measurements from the fs/ps rotational CARS measurement volume positioned within 3 mm or less of the burning propellant surface. Preliminary results in canonical flames are presented using a hybrid fs/ps vibrational CARS system to demonstrate our progress towards acquiring vibrational CARS measurements for more accurate temperatures in the very high temperature propellant burns.

47 OTHER INSTRUMENTATION↗

DOE OSTI2017

PTF1 J082340.04+081936.5: a hot subdwarf B star with a low-mass white dwarf companion in an 87-minute orbit

We present the discovery of the hot subdwarf B star (sdB) binary PTF1 J082340.04+081936.5. The system has an orbital period of P{sub orb} = 87.49668(1) minutes (0.060761584(10) days), making it the second-most compact sdB binary known. The light curve shows ellipsoidal variations. Under the assumption that the sdB primary is synchronized with the orbit, we find a mass of M{sub sdB}=0.45{sub −0.07}{sup +0.09} M{sub ⊙}, a companion white dwarf mass of M{sub WD}=0.46{sub −0.09}{sup +0.12} M{sub ⊙}, and a mass ratio of q=((M{sub WD})/(M{sub sdB}))=1.03{sub −0.08}{sup +0.10}. The future evolution was calculated using the MESA stellar evolution code. Adopting a canonical sdB mass of M{sub sdB}=0.47 M{sub ⊙}, we find that the sdB still burns helium at the time it will fill its Roche lobe if the orbital period was less than 106 minutes at the exit from the last common envelope (CE) phase. For longer CE exit periods, the sdB will have stopped burning helium and turned into a C/O white dwarf at the time of contact. Comparing the spectroscopically derived logg and T{sub eff} with our MESA models, we find that an sdB model with a hydrogen envelope mass of 5×10{sup −4} M{sub ⊙} matches the measurements at a post-CE age of 94 Myr, corresponding to a post-CE orbital period of 109 minutes, which is close to the limit to start accretion while the sdB is still burning helium.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2025

ELM2.1-XGBfire1.0: improving wildfire prediction by integrating a machine learning fire model in a land surface model

Wildfires have shown increasing trends in both frequency and severity across the contiguous United States (CONUS). However, process-based fire models have difficulties in accurately simulating the burned area over the CONUS due to a simplification of the physical process and cannot capture the interplay among fire, ignition, climate, and human activities. The deficiency of burned area simulation deteriorates the description of fire impact on energy balance, water budget, and carbon fluxes in the Earth system models (ESMs). Alternatively, fire models based on machine learning (ML), which capture statistical relationships between the burned area and environmental factors, have shown promising burned area predictions and corresponding fire impact simulation. We develop a hybrid framework (ELM2.1-XGBFire1.0) that integrates an eXtreme Gradient Boosting (XGBoost) wildfire model with the Energy Exascale Earth System Model (E3SM) land model (ELM) version 2.1. A Fortran–C–Python deep learning bridge is adapted to support online communication between ELM and the ML fire model. Specifically, the burned area predicted by the ML-based wildfire model is directly passed to ELM to adjust the carbon pool and vegetation dynamics after disturbance, which are then used as predictors in the ML-based fire model in the next time step. Evaluated against the historical burned area from Global Fire Emissions Database 5 from 2001–2019, the ELM2.1-XGBFire1.0 outperforms process-based fire models in terms of spatial distribution and seasonal variations. The ELM2.1-XGBFire1.0 has proven to be a new tool for studying vegetation–fire interactions and, more importantly, enables seamless exploration of climate–fire feedback, working as an active component of E3SM.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS1975

Feasibility of an advanced thrust termination assembly for a solid propellant rocket motor

A total of 68 quench tests were conducted in a vented bomb assembly (VBA). Designed to simulate full-scale motor operating conditions, this laboratory apparatus uses a 2-inch-diameter, end-burning propellant charge and an insulated disc of consolidated hydrated aluminum sulfate along with the explosive charge necessary to disperse the salt and inject it onto the burning surface. The VBA was constructed to permit variation of motor design parameters of interest; i.e., weight of salt per unit burning surface area, weight of explosive per unit weight of salt, distance from salt surface to burning surface, incidence angle of salt injection, chamber pressure, and burn time. Completely satisfactory salt quenching, without re-ignition, occurred in only two VBA tests. These were accomplished with a quench charge ratio (QCR) of 0.023 lb salt per square inch of burning surface at dispersing charge ratios (DCR) of 13 and 28 lb of salt per lb of explosive. Candidate materials for insulating salt charges from the rocket combustion environment were evaluated in firings of 5-inch-diameter, uncured end-burner motors. A pressed, alumina ceramic fiber material was selected for further evaluation and use in the final demonstration motor.

Source record↗

NASA NTRS1976

Monitoring the extent and occurence of fire in the different veld types of South Africa with particular reference to it's ecological role

The author has identified the following significant results. Imagery showed the highest amount of burned area to be in the western, southern, and eastern Transvaal and in one scene of the Transkei coast region. The percentage of burned area per image in all instances exceeded 1.4% reaching a maximum of 8.24% equivalent to 121,758 ha out of 1,476,540 ha of one image in the eastern Transvaal lowveld. There was a consistent increase in the amount of burnt area on images from July through to the end of October. From October onwards, there was a decrease in burned area so that during December there was none or very little burning evident. Four scenes comprising nine images showed burning according to the twelve veld types. Considerable variation was evident in the burning between different veld types: between 10 and 19% of the mixed, sourish-mixed, and sour bushveld types was burnt, but in other veld types the percentage of burnt area was less than 1%.

Edwards, D.↗

NASA NTRS1979

Particle size and velocity measurement in flames by laser anemometer

Simultaneous droplet size and velocity measurements by a particle counting Laser Doppler Anemometer (LDA) in kerosene fuel sprays under burning and non-burning conditions are presented. Particle sizes are derived from pulse height analysis of the mean LDA signals and velocities are simultaneously determined by measuring Doppler shift frequencies. The measurements show that droplet velocity is a function of droplet diameter for burning and non-burning conditions, and spatially averaged size distributions are derived from velocity data. A comparison of results obtained under burning and non-burning conditions show changes in size distribution due to preferential vaporization of small droplets, acceleration due to thermal expansion of gases, and corresponding changes in droplet momentum.

Chigier, N. A.↗

NASA NTRS1984

Annihilation of angular momentum drift during spinning-up and thrusting maneuvers of rigid bodies

A very simple, yet accurate, heuristic solution for the spiral path of the angular momentum vector during spin-up and spin-down maneuvers of rigid body spacecraft is presented. A two-burn scheme is proposed consisting of a burn, a coast, and a second burn of the spin thruster. The appropriate burn times are found by a transcendental equation similar to Kepler's equation. Numerical results verify the accuracy of the burn, coast, and burn times given by closed form expressions. The scheme can also be applied to the problem of axial thrusting during constant spin.

Longuski, J. M.↗

NASA NTRS1987

Combustion of velcro in low gravity

An experimental program was conducted to investigate the low gravity burning characteristics on nylon and Nomex Velcro fastening tapes in an atmosphere of 30-percent oxygen, 70-percent nitrogen at a 70-kPa pressure. The tests were conducted using the NASA Lewis Research Center Zero Gravity Facility. The test results, as documented by high-speed cameras, indicate that both nylon and Nomex burn in low gravity for the full 5.18 sec test time but that Nomex burns less vigorously than nylon. Nylon melts as it burns, whereas Nomex forms a solid char. Nylon also sputters burning droplets as it burns. Thus, from these limited tests, it appears that Nomex Velcro is less hazardous than nylon Velcro for spacecraft applications. The results also show that residual gas velocities, and by analogy spacecraft air circulation, can enhance the low-gravity combustion.

Olson, Sandra L.↗

NASA NTRS1994

Theory and computation of optimal low- and medium-thrust transfers

This report presents two numerical methods considered for the computation of fuel-optimal, low-thrust orbit transfers in large numbers of burns. The origins of these methods are observations made with the extremal solutions of transfers in small numbers of burns; there seems to exist a trend such that the longer the time allowed to perform an optimal transfer the less fuel that is used. These longer transfers are obviously of interest since they require a motor of low thrust; however, we also find a trend that the longer the time allowed to perform the optimal transfer the more burns are required to satisfy optimality. Unfortunately, this usually increases the difficulty of computation. Both of the methods described use small-numbered burn solutions to determine solutions in large numbers of burns. One method is a homotopy method that corrects for problems that arise when a solution requires a new burn or coast arc for optimality. The other method is to simply patch together long transfers from smaller ones. An orbit correction problem is solved to develop this method. This method may also lead to a good guidance law for transfer orbits with long transfer times.

Chuang, C.-H.↗

NASA NTRS1996

RSRM Chamber Pressure Oscillations: Transit Time Models and Unsteady CFD

Space Shuttle solid rocket motor low frequency internal pressure oscillations have been observed since early testing. The same type of oscillations also are present in the redesigned solid rocket motor (RSRM). The oscillations, which occur during RSRM burn, are predominantly at the first three motor cavity longitudinal acoustic mode frequencies. Broadband flow and combustion noise provide the energy to excite these modes at low levels throughout motor burn, however, at certain times during burn the fluctuating pressure amplitude increases significantly. The increased fluctuations at these times suggests an additional excitation mechanism. The RSRM has inhibitors on the propellant forward facing surface of each motor segment. The inhibitors are in a slot at the segment field joints to prevent burning at that surface. The aft facing segment surface at a field joint slot burns and forms a cavity of time varying size. Initially the inhibitor is recessed in the field joint cavity. As propellant burns away the inhibitor begins to protrude into the bore flow. Two mechanisms (transit time models) that are considered potential pressure oscillation excitations are cavity-edge tones, and inhibitor hole-tones. Estimates of frequency variation with time of longitudinal acoustic modes, cavity edge-tones, and hole-tones compare favorably with frequencies measured during motor hot firing. It is believed that the highest oscillation amplitudes occur when vortex shedding frequencies coincide with motor longitudinal acoustic modes. A time accurate computational fluid dynamic (CFD) analysis was made to replicate the observations from motor firings and to observe the transit time mechanisms in detail. FDNS is the flow solver used to detail the time varying aspects of the flow. The fluid is approximated as a single-phase ideal gas. The CFD model was an axisymmetric representation of the RSRM at 80 seconds into burn.Deformation of the inhibitors by the internal flow was determined through an iterative structural and CFD analysis. The analysis domain ended just upstream of the nozzle throat. This is an acoustic boundary condition that caused the motor to behave as a closed-open organ pipe. This differs from the RSRM which behaves like a closed-closed organ pipe. The unsteady CFD solution shows RSRM chamber pressure oscillations predominately at the longitudinal acoustic mode frequencies of a closed-open organ pipe. Vortex shedding in the joint cavities and at the inhibitors contribute disturbances to the flow at the second longitudinal acoustic mode frequency. Further studies are planned using an analysis domain that extends downstream of the nozzle throat.

Nesman, Tom↗