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DOE OSTI2026

A Relief Zone Architecture for Enhanced Durability of Ultrathin Membranes in Electrochemical Conversion Devices

Premature cell failures in electrochemical conversion systems often result when membrane electrode assemblies (MEAs) are prepared with ultra-thin (= 15 micrometer-thick) polymer electrolyte membranes (PEMs). These high-performance PEMs are susceptible to mechanical degradation from stress concentrations arising from component and device-level integration. Herein, a relief zone was developed to mitigate mechanical degradation by alleviating excess and non-uniform compression across the active area. Relief zones, created through the ablation of carbonaceous diffusion material achieves a seamless adaptation across a range of MEA dimensions and electrochemical applications without need for costly hardware modifications. This concept was demonstrated using fuel cells as a case study. Accelerated stress test (AST) validations yielded a 6-fold improvement for MEAs prepared with relief zones (i.e., lifetime approximately 1500 h) compared to those fabricated using conventional edge-protection techniques, showcasing the utility of this technique in decoupling integration and device-level engineering effects from intrinsic material limitations for durable electrochemical devices.

14 SOLAR ENERGY↗

DOE OSTI2022

Physics constrained learning for data-driven inverse modeling from sparse observations

Deep neural networks (DNN) have been used to model nonlinear relations between physical quantities. Those DNNs are embedded in physical systems described by partial differential equations (PDE) and trained by minimizing a loss function that measures the discrepancy between predictions and observations in some chosen norm. This loss function often includes the PDE constraints as a penalty term when only sparse observations are available. As a result, the PDE is only satisfied approximately by the solution. However, the penalty term typically slows down the convergence of the optimizer for stiff problems. We present a new approach that trains the embedded DNNs while numerically satisfying the PDE constraints. We develop an algorithm that enables differentiating both explicit and implicit numerical solvers in reverse-mode automatic differentiation. This allows the gradients of the DNNs and the PDE solvers to be computed in a unified framework. We demonstrate that our approach enjoys faster convergence and better stability in relatively stiff problems compared to the penalty method. Furthermore, our approach allows for the potential to solve and accelerate a wide range of data-driven inverse modeling, where the physical constraints are described by PDEs and need to be satisfied accurately.

97 MATHEMATICS AND COMPUTING↗

DOE OSTI2026

From Cell to System: Accelerated hpc Simulations of BESS Aging under Frequency Regulation and Arbitrage use cases

Lithium-ion battery energy storage systems (BESS) packs have emerged as a leading solution for grid-scale energy storage, enhancing resiliency and balancing load fluctuations. Yet, experimental characterization of large-format LIB packs-particularly to assess performance and degradation over hundreds of cycles - demands substantial hardware investment and multi-year testing campaigns. In this work, we couple a hierarchical, physics-based modeling framework agnostic to electrode chemistries with high-performance computing to accelerate systems level evaluation by upto two orders of magnitude. Building on the open-source liionpack platform, we implement cell, module, and pack-scale electrochemical models enriched with mechanistic aging mechanisms and deploy them on an HPC cluster to simulate 150−200kWh systems over 500 - 1,000 cycles with in days. We subject these virtual B ESS to both constant-current cycling and realistic grid service profiles spanning frequency regulation, ramp-rate support, and energy arbitrage-and quantify the resulting degradation patterns. Our results reveal that localized cell aging can induce substantial nonuniformity at module and pack levels, with service-specific cycling protocols driving distinct aging modes. This rapid, multiscale modeling approach provides a powerful design-space exploration tool for optimizing electrical architecture, control strategies, and operational schedules to prolong pack lifetime and lower total cost of ownership.

Ayalasomayajula, Surya [ORNL] (ORCID:0009000860788↗

DOE OSTI2024

Neutrino Program at Fermilab - Enhancing Proton Beam Power and Accelerator Infrastructure

The upcoming long baseline neutrino experiments aim to enhance proton beam power to multi-MW scale and utilize large-scale detectors to address the challenge of limited event statistics. The DUNE experiment at LBNF will test the three neutrino flavor paradigm and directly search for CP violation by studying oscillation signatures in the high intensity $\nu_{\mu}$ (anti-$\nu_{\mu}$) beam to $\nu_e$ (anti-$\nu_e$) measured over a long baseline.\par Higher beam power and improved accelerator up-time will enhance neutrino flux for the neutrino program by increasing the number of protons on target. LBNF/DUNE, as well as PIP-II upgrade and Accelerator Complex Evolution (ACE) plan, play a vital role in this effort. The scientific potential of ACE plan extends beyond neutrino physics, encompassing endeavors such as the Muon Collider, Charged Lepton Flavor Violation (CLFV), Dark Sectors, and exploration of neutrinos beyond DUNE. In the era of higher-power accelerator operation, research in target materials and beam instrumentation is crucial for optimizing design modifications. This abstract discusses Fermilab ACE, the science opportunities it provides, and how Fermilab is pushing the limits of proton beam power and accelerator infrastructure. By tackling neutrino beam challenges and exploring research and development ideas, we are advancing our understanding of fundamental particles and their interactions.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

NASA NTRS2020

Development and Comparison of an Artificial Gravity Concept for Human Spaceflight

Artificial Gravity (AG) for a long-duration space journey has been theorized since the dawn of human spaceflight. The purpose of this project is to begin bringing those concepts into real-life. The goal and primary study for this project is to research and understand the physics behind making a rotating centrifuge and the human limitations that may contribute to the design. The research first started with finding the physics equations we can use to calculate the rotational speed required for a certain gravity or the required radius for the centrifuge structure, this equation is a(sub c) = v2/r = w(sub c)2 r, where v is linear velocity, r is the radius of the structure, and is the rotational speed. Next, it is important to understand AG may be worthwhile because of the negative health effects of microgravity. The research then leads to finding human limitations in a rotating structure. The main limitation of a human living in this habitat is the Coriolis effect, which causes discomfort and motion sickness in the subject inside the structure, this causes the three semicircular fluid canals in your head that sense balance and motion. Finally, we use that knowledge to best hypothesize and propose the radius size for the structure that would negate the Coriolis effect, and using that we can calculate the appropriate rotational speed to get the desired gravity level, for example: 1 g or 9.81 m/s2 of acceleration. Overall this research can encourage increase knowledge in understanding AG, the physics and human limitation in a rotating centrifuge on future NASA long-duration Missions and Goals. This research can be a reference to future design proposals for long-duration exploration missions and colonization of planets or moons.

Cody L Beard↗

DOE OSTI2023

Magnetic Measurements and Alignment Results of LQXFA/B Cold Mass Assemblies at Fermilab

MQXFA production series quadrupole magnets are being built for the Hi-Lumi (HL) LHC upgrade by the U.S. Accelerator Upgrade Project (US-HL-LHC AUP). These magnets are being placed in pairs, as a cold mass, within cryostats at Fermilab, and are being tested to assess alignment and magnetic performance at Fermilab's horizontal test stand facility. The ~10 m - long assembly must meet stringent specifications for quadrupole strength and harmonic field integrals determination, magnetic axis position, and for magnet variations in positioning and local field profile. Here this paper describes the results of the magnetic and alignment measurements which characterize the first LQXFA/B assembly.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

NASA NTRS2023

Energetic Proton Acceleration By EMIC Waves in Io’s Footprint Tail

In this study, we present a survey of energetic proton observations associated with Io’s footprint tail (FPT) and compare their signatures with in situ measurements of the plasma waves and lower-energy electron environments. We find further supporting evidence that proton acceleration in Io’s FPT is likely a consequence of wave–particle interactions via electromagnetic ion cyclotron waves that are generated by precipitating electrons into Jupiter’s ionosphere. This idea was originally proposed by Clark et al. (2020) and Sulaiman et al. (2020) based on NASA’s Juno mission likely transiting Io’s Main Alfvén Wing (MAW) during its twelfth orbit (i.e., PJ12). Additionally, the analysis of > 50 keV protons presented here highlights important observational details about the Io–Jupiter interaction as follows: 1) proton acceleration in Io’s FPT is a persistent feature and the energy flux carried by the protons is highest at smaller Io-Alfvén tail distances; 2) energetic protons exhibit positive correlations with both plasma waves and <100 keV/Q electrons; 3) during a small number of Io FPT crossings, the protons display finer spatial/temporal structure reminiscent of the electron observations reported by Szalay et al. (2018); and 4) the proton pitch angle distributions are characterized by two types: conic distributions in or near Io’s MAW and isotropic elsewhere.

space physics↗

DOE OSTI2022

Computationally Accelerated Discovery of High Entropy Pyrochlore Oxides

High entropy ceramics provide enhanced flexibility for tailoring a wide range of physical properties, emerging from the diverse chemical and configurational degrees of freedom. Expanding upon the endeavors of recently synthesized high entropy ceramics in rock salt, fluorite, spinel, and perovskite structures, we explore the relative feasibility of formation of high entropy pyrochlore oxides, A 2 B 2 O 7 , with multication occupancy of the B-site, estimated from first-principles-based thermodynamic descriptors. Subsequently, we used Monte Carlo simulations to estimate the phase composition, oxygen vacancy concentration, and local ionic segregation as a function of temperature and oxygen partial pressure. In synergy with the theoretical calculations, we have investigated the synthesis of several multicomponent oxides with a pyrochlore composition, related to our computational investigations, resulting in four phase pure and one 97.4% pure high entropy pyrochlore oxides. Ultimately, our approach allows us to evaluate potential impurity phases, ionic disorder, and oxygen vacancy concentration in response to the experimental variables, thereby making realistic predictions that can direct and accelerate experimental synthesis of novel multicomponent ceramics.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2024

New μ forces from ν μ sources

Accelerator-based experiments reliant on charged pion and kaon decays to produce muon-neutrino beams also deliver an associated powerful flux of muons. Therefore, these experiments can additionally be sensitive to light new particles that preferentially couple to muons and decay to visible final states on macroscopic length scales. Such particles are produced through rare 3-body meson decays in the decay pipe or via muon scattering in the beam dump, and decay in a downstream detector. To demonstrate the potential of this search strategy, we recast existing MiniBooNE and MicroBooNE studies of neutral pion production in neutrino-induced neutral-current scattering ( ν μ N → ν μ N π 0 , π 0 → γ γ ) to place limits on light ( < 2 m μ ) muon-philic scalar particles that decay to diphotons through loops of virtual muons. While much of this parameter space has already been excluded by E137, we also project that SBND can be sensitive to unexplored parameter space for these models, and provide a road map for future neutrino experiments to perform dedicated searches for muon-philic forces. Published by the American Physical Society 2024

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2022

Searches for New Particles, Dark Matter, and Gravitational Waves with SRF Cavities

This is a Snowmass white paper on the utility of existing and future superconducting cavities to probe fundamental physics. Superconducting radio frequency (SRF) cavity technology has seen tremendous progress in the past decades, as a tool for accelerator science. With advances spear-headed by the SQMS center at Fermilab, they are now being brought to the quantum regime becoming a tool in quantum science thanks to the high degree of coherence. The same high quality factor can be leveraged in the search for new physics, including searches for new particles, dark matter, including the QCD axion, and gravitational waves. We survey some of the physics opportunities and the required directions of R&D. Given the already demonstrated integration of SRF cavities in large accelerator systems, this R&D may enable larger scale searches by dedicated experiments.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2023

Controls at the Fermilab PIP-II Superconducting Linac

PIP-II is an 800 MeV superconducting RF linac under development at Fermilab. As the new first stage in our accelerator chain, it will deliver high-power beam to multiple experiments simultaneously and thus drive Fermilab’s particle physics program for years to come. In a pivot for Fermilab, controls for PIP-II are based on EPICS instead of ACNET, the legacy control system for accelerators at the lab. This paper discusses the status of the EPICS controls work for PIP-II. We describe the EPICS tools selected for our system and the experience of operators new to EPICS. We introduce our continuous integration / continuous development environment. We also describe some efforts at cooperation between EPICS and ACNET, or efforts to move towards a unified interface that can apply to both control systems.

43 PARTICLE ACCELERATORS↗

DOE OSTI2024

Neutrino Program at Fermilab - Enhancing Proton Beam Power and Accelerator Infrastructure

The upcoming long baseline neutrino experiments aim to enhance proton beam power to multi-MW scale and utilize large-scale detectors to address the challenge of limited event statistics. The DUNE experiment at LBNF will test the three-neutrino flavor paradigm and directly search for CP violation by studying oscillation signatures in the high intensity (anti-) beam to (anti-) measured over a long baseline. Higher beam power and improved accelerator up-time will enhance neutrino flux for the neutrino program by increasing the number of protons on target. LBNF/DUNE, as well as PIP-II upgrade and Accelerator Complex Evolution (ACE) plan, play a vital role in this effort. The scientific potential of ACE plan extends beyond neutrino physics, encompassing endeavors such as the Muon Collider, Charged Lepton Flavor Violation (CLFV), Dark Sectors, and exploration of neutrinos beyond DUNE.\par In the era of higher-power accelerator operation, research in target materials and beam instrumentation is crucial for optimizing design modifications. This abstract discusses Fermilab ACE, the science opportunities it provides, and how Fermilab is pushing the limits of proton beam power and accelerator infrastructure. By tackling neutrino beam challenges and exploring research and development ideas, we are advancing our understanding of fundamental particles and their interactions.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2022

Nonideal Fields Solve the Injection Problem in Relativistic Reconnection

Magnetic reconnection in relativistic plasmas is well established as a fast and efficient particle accelerator, capable of explaining the most dramatic astrophysical flares. With particle-in-cell simulations, we demonstrate the importance of nonideal fields for the early stages (“injection”) of particle acceleration. Most of the particles ending up with high energies (near or above the mean magnetic energy per particle) must have passed through nonideal regions where the assumptions of ideal magnetohydrodynamics are broken (i.e., regions with E > B or nonzero E ∥ = E ∙ B/B), whereas most of the particles that do not experience nonideal fields end up with Lorentz factors of order unity. So, injection by nonideal fields is a necessary prerequisite for further acceleration. Our results have important implications for the origin of nonthermal particles in high-energy astrophysical sources.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

NASA NTRS1987

Microphysics of the auroral acceleration region of other regions of the magnetosphere

Electric field and plasma measurements pertinent to the microphysics of the auroral acceleration region are reviewed. Observations in other regions of the magnetosphere, which appear to involve similar physical processes, are summarized in order to emphasize the requirement on Cluster instrumentation for wide dynamic range, high time resolution, time domain field, and particle measurements. It is suggested that the microphysics of current driven instabilities in the auroral acceleration region is duplicated in the high latitude boundary of the plasma sheet and that the macroscale structure of the tail is determined by this microphysics.

Mozer, F. S.↗

NASA NTRS1994

Prediction of solar flares for the Space Exploration Initiative

The 21st century is likely to see the start of the manned exploration and settlement of the inner solar system. NASA's plans for this endeavor are focused upon the Space Exploration Initiative which calls for a return to the Moon, to stay, followed by manned missions to Mars. To execute these missions safely provides solar physics with both a challenge and an opportunity. As the past solar maximum has clearly demonstrated, the Sun, through the solar flare process, is capable of generating and accelerating to high energies large fluxes of protons whose cumulative dose to unprotected astronauts can be fatal. It will be the responsibility of solar physicists to develop an accurate physical description of the mechanisms of flare energy storage and release, and of particle acceleration and propagation through interplanetary space upon which to base a sound method of flare and energetic particle prediction.

Davis, John M.↗

DOE OSTI2026

Biasing from galaxy trough and peak profiles with the DES Y3 redMaGiC galaxies and the weak lensing mass map

We measure the correspondence between the distribution of galaxies and matter around troughs and peaks in the projected galaxy density, by comparing redMaGiC galaxies (0.15 < z < 0.65) to weak lensing mass maps from the Dark Energy Survey (DES) Y3 data release. We obtain stacked profiles, as a function of angle θ, of the galaxy density contrast δ g and the weak lensing convergence κ, in the vicinity of these identified troughs and peaks, referred to as ‘void’ and ‘cluster’ superstructures. The ratio of the profiles depend mildly on θ, indicating good consistency between the profile shapes. We model the amplitude of this ratio using a function $F(\boldsymbol{\eta }, \theta )$ that depends on cosmological parameters $\boldsymbol{\eta }$, scaled by the galaxy bias. We construct templates of $F(\boldsymbol{\eta }, \theta )$ using a suite of N-body (‘Gower Street’) simulations forward-modelled with DES Y3-like noise and systematics. We discuss and quantify the caveats of using a linear bias model to create galaxy maps from the simulation dark matter shells. We measure the galaxy bias in three lens tomographic bins (near to far): $2.32^{+0.86}_{-0.27}, 2.18^{+0.86}_{-0.23}, 1.86^{+0.82}_{-0.23}$ for voids, and $2.46^{+0.73}_{-0.27}, 3.55^{+0.96}_{-0.55}, 4.27^{+0.36}_{-1.14}$ for clusters, assuming the best-fit Planck cosmology. Similar values with ∼0.1σ shifts are obtained assuming the mean DES Y3 cosmology. The biases from troughs and peaks are broadly consistent, although a larger bias is derived for peaks, which is also larger than those measured from the DES Y3 3 × 2-point analysis. This method shows an interesting avenue for measuring field-level bias that can be applied to future lensing surveys.

cosmology: observations↗

DOE OSTI2025

Review of Neutron Yield from (α, n) Reactions: Data, Methods, and Prospects

Understanding the radiogenic neutron production rate through the (α, n) reaction is crucial in many areas of physics, including dark matter searches, neutrino studies, and nuclear astrophysics. In addition to its relevance for fundamental research, the (α, n) reaction also plays a significant role in nuclear energy technologies, for example by contributing to neutron production in subcritical systems using UO2, as well as in applications such as medical physics. This review examines the current state of (α, n) yield calculations and neutron spectra, describes the computational tools used for their estimation, and discusses the available cross-section data. We discuss the uncertainties affecting (α, n) yield estimations and propose a strategy to enhance their accuracy. Furthermore, this paper discusses and emphasizes the need for new measurements of (α, n) cross-sections for a variety of relevant materials. Such measurements are essential for improving neutron flux predictions, which are crucial for reducing uncertainties in sensitivity estimates for next-generation physics experiments operating in the keV—MeV range.

(α, n)reactions↗

DOE OSTI2022

Controlled Injection of Electrons for Improved Performance of Laser-Wakefield Acceleration

Our lab performed a series of experiments on controlled injection of LWFA with two extreme laser pulses: one laser pulse was used to drive LWFA. In contrast, the other precisely controls the injection of electrons into the wakefield plasma wave. We have demonstrated an efficient reduction of electron beam emittance by optical injection and novel spatio-temporal manipulation of the electron beam by the extreme laser-plasma waves. Moreover, the optical injection process involves unprecedented new physics, which will benefit studies in astrophysics, inertial confinement fusion, laser-driven x-ray light sources, and ultrafast science. We further improved the performance of LWFA by a better understanding and control of the extreme laser-plasma wave dynamics for optical injection. Three novel mechanisms were identified in the optical injection process: (1) collision of two laser pulses, (2) collision of a laser pulse with a wakefield plasma wave, and (3) collision of two laser wakefields. All three methods improved electron-beam energy spread, emittance, stability, and reproducibility. First, we identified, compared, and independently controlled these different injection mechanisms by controlling the polarization of the injector laser pulse. Second, we manipulated the spatiotemporal splitting of LWFA electron beams to reduce their emittance. Third, we applied the same laser-plasma-wave dynamics and the same experimental setup for improved performance of ion acceleration, which has also been predicted by the recent simulations.

43 PARTICLE ACCELERATORS↗