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NASA NTRS2003

Measurement and Modeling of Vertically Resolved Aerosol Optical Properties and Radiative Fluxes Over the ARM SGP Site

In order to meet one of its goals - to relate observations of radiative fluxes and radiances to the atmospheric composition - the Department of Energy's Atmospheric Radiation Measurement (ARM) program has pursued measurements and modeling activities that attempt to determine how aerosols impact atmospheric radiative transfer, both directly and indirectly. However, significant discrepancies between aerosol properties measured in situ or remotely remain. One of the objectives of the Aerosol Intensive Operational Period (TOP) conducted by ARM in May 2003 at the ARM Southern Great Plains (SGP) site in north central Oklahoma was to examine and hopefully reduce these differences. The IOP involved airborne measurements from two airplanes over the heavily instrumented SGP site. We give an overview of airborne results obtained aboard the Center for Interdisciplinary Remotely-Piloted Aircraft Studies (CIRPAS) Twin Otter aircraft. The Twin Otter performed 16 research flights over the SGP site. The aircraft carried instrumentation to perform in-situ measurements of aerosol absorption, scattering, extinction and particle size. This included such novel techniques as the photoacoustic and cavity ring-down methods for in-situ absorption (675 nm) and extinction (675 and 1550 nm) and a new multiwavelength, filter-based absorption photometer (467, 530, 660 nm). A newly developed instrument measured cloud condensation nucleus concentration (CCN) concentrations at two supersaturation levels. Aerosol optical depth and extinction (354-2139 nm) were measured with the NASA Ames Airborne Tracking 14-channel sunphotometer. Furthermore, up-and downwelling solar (broadband and spectral) and infrared radiation were measured using seven individual radiometers. Three up-looking radiometers werer mounted on a newly developed stabilized platform, keeping the instruments level up to aircraft pitch and roll angles of approximately 10(exp 0). This resulted in unprecedented continuous vertical profiles of radiative fluxes, which we will compare to modeled fluxes using the aforementioned data as input.

Schmid, B.↗
NASA NTRS2003

Space Borne Cloud and Aerosol Measurements by the Geoscience Laser Altimeter System: Initial Results

In January 2003 the Geoscience Laser Altimeter System (GLAS) was successfully launched into orbit. Beginning in March 2003 GLAS will provide global coverage lidar measurement of the height distribution of clouds and aerosol in the atmosphere for up to five years. The characteristic and value of the unique data will be presented. The instrument is a basic backscatter lidar that operates at two wavelengths, 532 and 1064 nm. The mission data products for atmospheric observations include the calibrated, observed, attenuated backscatter cross section for cloud and aerosol; height detection for multiple cloud layers; planetary boundary layer height; cirrus and aerosol optical depth and the height distribution of aerosol and cloud scattering cross section profiles. The data is expected to significantly enhance knowledge in several areas of atmospheric science, in particular the distribution, transport and influence of atmospheric aerosol and thin clouds. Measurements of the coverage and height of polar and cirrus cloud should be significantly more accurate than previous global observations. In March and April 2003, airborne and ground based data verification experiments will be carried out. Initial results from the verification experiments and the first several months of operation will be presented.

Spinhirne, James D.↗
NASA NTRS2004

Spatial and Temporal Distribution of Tropospheric Clouds and Aerosols Observed by MODIS Onboard the Terra and Aqua Satellites

Remote sensing of cloud and aerosol optical properties is routinely obtained using the Moderate Resolution Imaging Spectroradiometer (MODIS) onboard the Terra and Aqua satellites. Techniques that are being used to enhance our ability to characterize the global distribution of cloud and aerosol properties include well-calibrated multispectral radiometers that rely on visible, near-infrared, and thermal infrared channels. The availability of thermal channels to aid in cloud screening for aerosol properties is an important additional piece of information that has not always been incorporated into sensor designs. In this paper, we describe the radiative properties of clouds as currently determined from satellites (cloud fraction, optical thickness, cloud top pressure, and cloud effective radius), and highlight the global and regional cloud microphysical properties currently available for assessing climate variability and forcing. These include the latitudinal distribution of cloud optical and radiative properties of both liquid water and ice clouds, as well as joint histograms of cloud optical thickness and effective radius for selected geographical locations around the world. In addition, we will illustrate the radiative and microphysical properties of aerosol particles that are currently available from space-based observations, and show selected cases in which aerosol particles are observed to modify the cloud optical properties.

King, Michael D.↗
NASA NTRS2004

Clouds Aerosols Internal Affaires: Increasing Cloud Fraction and Enhancing the Convection

Clouds developing in a polluted environment have more numerous, smaller cloud droplets that can increase the cloud lifetime and liquid water content. Such changes in the cloud droplet properties may suppress low precipitation allowing development of a stronger convection and higher freezing level. Delaying the washout of the cloud water (and aerosol), and the stronger convection will result in higher clouds with longer life time and larger anvils. We show these effects by using large statistics of the new, 1km resolution data from MODIS on the Terra satellite. We isolate the aerosol effects from meteorology by regression and showing that aerosol microphysical effects increases cloud fraction by average of 30 presents for all cloud types and increases convective cloud top pressure by average of 35mb. We analyze the aerosol cloud interaction separately for high pressure trade wind cloud systems and separately for deep convective cloud systems. The resultant aerosol radiative effect on climate for the high pressure cloud system is: -10 to -13 W/sq m at the top of the atmosphere (TOA) and -11 to -14 W/sq m at the surface. For deeper convective clouds the forcing is: -4 to -5 W/sq m at the TOA and -6 to -7 W/sq m at the surface.

Koren, Ilan↗
NASA NTRS2003

Chemical and Physical Properties of Bulk Aerosols within Four Sectors Observed during TRACE-P

Chemical and physical aerosol data collected on the DC-8 during TRACE-P were grouped into four sectors based on back trajectories. The four sectors represent long-range transport from the west (WSW), regional circulation over the western Pacific and Southeast Asia (SE Asia), polluted transport from Northern Asia with substantial sea salt at low altitudes (NNW) and a substantial amount of dust (Channel). WSW has generally low mixing ratios at both middle and high altitudes, with the bulk of the aerosol mass due to non-sea-salt water-soluble inorganic species. Low altitude SE Asia also has low mean mixing ratios in general, with the majority of the aerosol mass comprised of non-sea-salts, however, soot is also relatively important m this region. "w had the highest mean sea salt mixing ratios, with the aerosol mass at low altitudes (a km) evenly divided between sea salts, mm-sea-salts, and dust. The highest mean mixing ratios of water-soluble ions and soot were observed at the lowest altitudes (a km) in the Channel sector. The bulk of the aerosol mass exported from Asia emanates h m Channel at both low and midaltitudes, due to the prevalence of dust compared to other sectors. Number densities show enhanced fine particles for Channel and NNW, while their volume distributions are enhanced due to sea salt and dust Low-altitude Channel exhibits the highest condensation nuclei ((34) number densities along with enhanced scattering coefficients, compared to the other sectors. At midaltitudes (2-7 km), low mean CN number densities coupled with a high proportion of nonvolatile particles (265%) observed in polluted sectors (Channel and NNW) are attributed to wet scavenging which removes hygroscopic CN particles. Low single scatter albedo m SE Asia reflects enhanced soot

Jordan, C. E.↗
NASA NTRS2005

How well can we Measure the Vertical Profile of Tropospheric Aerosol Extinction?

The recent Department of Energy Atmospheric Radiation Measurement (ARM) Aerosol Intensive Operations Period (MOP, May 2003) yielded one of the best measurement sets obtained to-date to assess our ability to measure the vertical profile of ambient aerosol extinction sigma(sub ep)(lambda) in the lower troposphere. During one month, a heavily instrumented aircraft with well characterized aerosol sampling ability carrying well proven and new aerosol instrumentation, devoted most of the 60 available flight hours to flying vertical profiles over the heavily instrumented ARM Southern Great Plains (SGP) Climate Research Facility (CRF). This allowed us to compare vertical extinction profiles obtained from 6 different instuments: airborne Sun photometer (AATS-14), airborne nephelometer/absorption photometer, airborne cavity ring-down system, ground-based Raman lidar and 2 ground-based elastic backscatter lidars. We find the in-situ measured sigma(sub ep)(lambda) to be lower than the AATS-14 derived values. Bias differences are 0.002 - 0.004 K/m equivalent to 12-17% in the visible, or 45% in the near-infrared. On the other hand, we find that with respect to AATS-14, the lidar sigma(sub ep)(lambda) are higher. An unnoticed loss of sensitivity of the Raman lidar had occurred leading up to AIOP and we expect better agreement from the recently restored system looking at the collective results from 6 field campaigns conducted since 1996, airborne in situ measurements of sigma(sub ep)(lambda) tend to be biased slightly low (17% at visible wavelengths) when compared to airborne Sun photometer sigma(sub ep)(lambda). On the other hand, sigma(sub ep)(lambda) values derived from lidars tend to have no or positive biases. From the bias differences we conclude that the typical systematic error associated with measuring the tropospheric vertical profile of the ambient aerosol extinction with current state of-the art instrumentation is 15-20% at visible wavelengths and potentially larger in the UV and near-infrared.

Schmid, Beat↗
NASA NTRS2003

Coordinated Airborne, Spaceborne and Ground-based Measurements of Massive Thick Aerosol Layers during the Dry Season in Southern Africa

During the dry season airborne campaign of the Southern African Regional Science Initiative (SAFARI 2000), coordinated observations were made of massive thick aerosol layers. These layers were often dominated by aerosols from biomass burning. We report on airborne Sun photometer measurements of aerosol optical depth (lambda = 0.354- 1.557 microns), columnar water vapor, and vertical profiles of aerosol extinction and water vapor density that were obtained aboard the University of Washington's Convair-580 research aircraft. We compare these with ground-based AERONET Sun/sky radiometer results, with ground based lidar data (MPL-Net), and with measurements from a downward pointing lidar aboard the high-flying NASA ER-2 aircraft. Finally, we show comparisons between aerosol optical depths fiom the Sun photometer and those retrieved over land and over water using four spaceborne sensors (TOMS, MODIS, MISR, and ATSR-2).

Schmid, B.↗
NASA NTRS2006

Comparisons of global aerosol simulations from GOCART and GMI-UMich

Global aerosol mass and optical thickness (AOT) simulated by two aerosol models (GOCART and GMI-UMich) are evaluated and the strengths and shortcomings of the model approaches are investigated. These two offline CTM models are driven by the same meteorological fields (NASA GEOS-4), use the same dynamic transport algorithm, and have the same spatial resolution. However, they differ partially in emission, dry/wet deposition, and chemistry. The simulated aerosol masses are evaluated by the surface long-term measurements and short-term field campaigns (ACE-Asia and TRACE-P). AOT are calculated using modeled aerosol mass but externally mixed for GOCART and partially internally mixed for GMI-Mich. These AOT are evaluated using satellite observations from MODIS and MISR and ground measurements from AERONET. Our work demonstrates that there are significant differences in simulated aerosol mass and AOT by the two approaches. Further investigation will be performed to evaluate each mechanism which induces the differences quantitatively by implementing GOCART-like emission, deposition, and chemistry into GMI framework.

Bian, Huisheng↗
NASA NTRS2005

Height Distribution Between Cloud and Aerosol Layers from the GLAS Spaceborne Lidar in the Indian Ocean Region

The Geoscience Laser Altimeter System (GLAS), a nadir pointing lidar on the Ice Cloud and land Elevation Satellite (ICESat) launched in 2003, now provides important new global measurements of the relationship between the height distribution of cloud and aerosol layers. GLAS data have the capability to detect, locate, and distinguish between cloud and aerosol layers in the atmosphere up to 40 km altitude. The data product algorithm tests the product of the maximum attenuated backscatter coefficient b'(r) and the vertical gradient of b'(r) within a layer against a predetermined threshold. An initial case result for the critical Indian Ocean region is presented. From the results the relative height distribution between collocated aerosol and cloud shows extensive regions where cloud formation is well within dense aerosol scattering layers at the surface. Citation: Hart, W. D., J. D. Spinhime, S. P. Palm, and D. L. Hlavka (2005), Height distribution between cloud and aerosol layers from the GLAS spaceborne lidar in the Indian Ocean region,

Hart, William D.↗
NASA NTRS2006

Intercontinental Transport of Aerosols: Implication for Regional Air Quality

Aerosol particles, also known as PM2.5 (particle diameter less than 2.5 microns) and PM10 (particle diameter less than 10 microns), is one of the key atmospheric components that determine ambient air quality. Current US air quality standards for PM10 (particles with diameter < 10 microns) and PM2.5 (particles with diameter 2.5 microns) are 50 pg/cu m and 15 pg/cu m, respectively. While local and regional emission sources are the main cause of air pollution problems, aerosols can be transported on a hemispheric or global scale. In this study, we use the Goddard Chemistry Aerosol Radiation and Transport (GOCART) model to quantify contributions of long-range transport vs. local/regional pollution sources and from natural vs. anthropogenic sources to PM concentrations different regions. In particular, we estimate the hemispheric impact of anthropogenic sulfate aerosols and dust from major source areas on other regions in the world. The GOCART model results are compared with satellite remote sensing and ground-based network measurements of aerosol optical depth and concentrations.

Chin, Mian↗
NASA NTRS2006

Spatial and Temporal Distribution of Tropospheric Clouds and Aerosols Observed by MODIS Onboard the Terra and Aqua Satellites

Remote sensing of cloud and aerosol optical properties is routinely obtained using the Moderate Resolution Imaging Spectroradiometer (MODIS) onboard the Terra and Aqua satellites. Instruments that are being used to enhance our ability to characterize the global distribution of cloud and aerosol properties include well-calibrated multispectral radiometers that measure in the visible, near-infrared, and thermal infrared. The availability of thermal channels to enhance detection of cloud when estimating aerosol properties is an important improvement. In this paper, we describe the radiative properties of clouds as currently determined from satellites (cloud fraction, optical thickness, cloud top pressure, and cloud particle effective radius) and highlight the global/regional cloud microphysical properties currently available for assessing climate variability and forcing. These include the latitudinal distribution of cloud optical and radiative properties of both liquid water and ice clouds, as well as joint histograms of cloud optical thickness and effective particle radius for selected geographical locations around the world. In addition, we will illustrate the radiative and microphysical properties of aerosol particles (in cloud free regions) that are currently available from space-based observations, and show the latitudinal distribution of aerosol optical properties over both land and ocean surfaces.

King, Michael D.↗
NASA NTRS2007

Aerosol Radiative Effects on Deep Convective Clouds and Associated Radiative Forcing

The aerosol radiative effects (ARE) on the deep convective clouds are investigated by using a spectral-bin cloud-resolving model (CRM) coupled with a radiation scheme and an explicit land surface model. The sensitivity of cloud properties and the associated radiative forcing to aerosol single-scattering albedo (SSA) are examined. The ARE on cloud properties is pronounced for mid-visible SSA of 0.85. Relative to the case excluding the ARE, cloud fraction and optical depth decrease by about 18% and 20%, respectively. Cloud droplet and ice particle number concentrations, liquid water path (LWP), ice water path (IWP), and droplet size decrease significantly when the ARE is introduced. The ARE causes a surface cooling of about 0.35 K and significantly high heating rates in the lower troposphere (about 0.6K/day higher at 2 km), both of which lead to a more stable atmosphere and hence weaker convection. The weaker convection and the more desiccation of cloud layers explain the less cloudiness, lower cloud optical depth, LWP and IWP, smaller droplet size, and less precipitation. The daytime-mean direct forcing induced by black carbon is about 2.2 W/sq m at the top of atmosphere (TOA) and -17.4 W/sq m at the surface for SSA of 0.85. The semi-direct forcing is positive, about 10 and 11.2 W/sq m at the TOA and surface, respectively. Both the TOA and surface total radiative forcing values are strongly negative for the deep convective clouds, attributed mostly to aerosol indirect forcing. Aerosol direct and semi-direct effects are very sensitive to SSA. Because the positive semi-direct forcing compensates the negative direct forcing at the surface, the surface temperature and heat fluxes decrease less significantly with the increase of aerosol absorption (decreasing SSA). The cloud fraction, optical depth, convective strength, and precipitation decrease with the increase of absorption, resulting from a more stable and dryer atmosphere due to enhanced surface cooling and atmospheric heating.

Fan, J.↗
NASA NTRS2005

Optical Characterization of Metallic Aerosols

Airborne metallic particulates from industry and urban sources are highly conducting aerosols. The characterization of these pollutant particles is important for environment monitoring and protection. Because these metallic particulates are highly reflective, their effect on local weather or regional radiation budget may also need to be studied. In this work, light scattering characteristics of these metallic aerosols are studied using exact solutions on perfectly conducting spherical and cylindrical particles. It is found that for perfectly conducting spheres and cylinders, when scattering angle is larger than approx. 90 deg. the linear polarization degree of the scattered light is very close to zero. This light scattering characteristics of perfectly conducting particles is significantly different from that of other aerosols. When these perfectly conducting particles are immersed in an absorbing medium, this light scattering characteristics does not show significant change. Therefore, measuring the linear polarization of scattered lights at backward scattering angles can detect and distinguish metallic particulates from other aerosols. This result provides a great potential of metallic aerosol detection and monitoring for environmental protection.

Sun, Wenbo↗
NASA NTRS2006

How Well do State-of-the-Art Techniques Measuring the Vertical Profile of Tropospheric Aerosol Extinction Compare?

The recent Department of Energy Atmospheric Radiation Measurement (ARM) Aerosol Intensive Operations Period (AIOP, May 2003) yielded one of the best measurement sets obtained to date to assess our ability to measure the vertical profile of ambient aerosol extinction sigma(ep)(lambda) in the lower troposphere. During one month, a heavily instrumented aircraft with well-characterized aerosol sampling ability carrying well-proven and new aerosol instrumentation devoted most of the 60 available flight hours to flying vertical profiles over the heavily instrumented ARM Southern Great Plains (SGP) Climate Research Facility (CRF). This allowed us to compare vertical extinction profiles obtained from six different instruments: airborne Sun photometer (AATS-14), airborne nephelometer/absorption photometer, airborne cavity ring-down system, groundbased Raman lidar, and two ground-based elastic backscatter lidars. We find the in situ measured sigma(ep)(lambda) to be lower than the AATS-14 derived values. Bias differences are 0.002-0.004 Km!1 equivalent to 13-17% in the visible, or 45% in the near-infrared. On the other hand, we find that with respect to AATS-14, the lidar sigma(ep)(lambda) are higher: Bias differences are 0.004 Km(-1) (13%) and 0.007 Km(-1) (24%) for the two elastic backscatter lidars (MPLNET and MPLARM, lambda = 523 nm) and 0.029 Km(-1) (54%) for the Raman lidar (lambda = 355 nm). An unnoticed loss of sensitivity of the Raman lidar had occurred leading up to AIOP, and we expect better agreement from the recently restored system. Looking at the collective results from six field campaigns conducted since 1996, airborne in situ measurements of sigma(ep)(lambda) tend to be biased slightly low (17% at visible wavelengths) when compared to airborne Sun photometer sigma(ep)(lambda). On the other hand, sigma(ep)(lambda) values derived from lidars tend to have no or positive biases. From the bias differences we conclude that the typical systematic error associated with measuring the tropospheric vertical profile of the ambient aerosol extinction with current state-of-the-art instrumentation is 15-20% at visible wavelengths and potentially larger in the UV and near-infrared.

Schmid, B.↗
NASA NTRS2008

SAGE II Measurements of Stratospheric Aerosol Properties at Non-Volcanic Levels

Since 2000, stratospheric aerosol levels have been relatively stable and at the lowest levels observed in the historical record. Given the challenges of making satellite measurements of aerosol properties at these levels, we have performed a study of the sensitivity of the product to the major components of the processing algorithm used in the production of SAGE II aerosol extinction measurements and the retrieval process that produces the operational surface area density (SAD) product. We find that the aerosol extinction measurements, particularly at 1020 nm, remain robust and reliable at the observed aerosol levels. On the other hand, during background periods, the SAD operational product has an uncertainty of at least a factor of 2 during due to the lack of sensitivity to particles with radii less than 100 nm.

Thomason, Larry W.↗
NASA NTRS2007

Continental Scale Aerosol Optical Properties Over East Asia as Measured by Aeronet and Comparison to Satellite and Modeled Results

The AERONET program has operated in E. Asia since 1995 providing time continuous and time averaged ground-based column-integrated aerosol optical properties in a variety of aerosol regimes In the last four years the distribution has greatly increased in Siberia, China, SE Asia and India in particular. Commensurate with that, significant improvement in data processing algorithms (Version 2.0) and access to ancillary data products through the WWW have become available to the scientific community. At this writing the following distribution represents E and S. Asia: 5 sites operate in Siberia (2 years), 1 in Mongolia (9 years), 3 in Korea (3 to 6 years), 3 in Japan (2 to 7 years), China 11 (6 to 0 years), Taiwan 4 (7 to 2 yrs), Viet Nam 2 (4 years), Thailand 2 to 5 (4 years), and Singapore 1 (4 months), India 1 to 3 (7 to 1 years), Pakistan 2 (1 year), and UAE 3 (3 years). An analysis of the aerosol optical depth at 500 nm using annual average quality assured AERONET data (pre 2006) was used to estimate the mean annual aerosol loading by continent, sub continent and ocean. The individual site data were assumed representative of regional aerosol loading and aggregated to the sub-continental, continental and oceanic areas and presented. This analysis will be updated with more recent data with particular emphasis on seasonal results for Asia and the addition of single scattering albedo retrievals. The ground based results will be compared to MODIS collection 5 results and model estimates for E. Asia using the AERONET Synergy Tool.

Holben, B. N.↗
NASA NTRS2007

Version 2.0 AERONET Dust Aerosol properties, Constraints and Application to Asian Dust Observations

In November 2006, AERONET released Version 2 of the Dubovik and King sky radiance and optical depth inversion. Reanalysis of the entire AERONET database revealed marked differences in aerosol properties in arid and semi arid regions with dust dominated aerosols. The change will be illustrated through sensitivity analysis and examples from the UAE2 (United Arab Emirates Unified Aerosol Experiment) field campaign. Properties of dust dominated aerosols will be presented from regional AERONET sites in China showing variations in dust aerosol properties. The constraints and limitations of the AERONET inversion will be presented that will facilitate analysis by the user community of these data.

Holben, Brent↗
NASA NTRS2008

The Global Aerosol System As Viewed By MODIS Today

The MODerate resolution Imaging Spectroradiometer (MODIS) aerosol algorithms have been working steadily since early 2000 to transform the MODIS-measured spectral solar reflectance from the Earth's surface and atmosphere into a variety of aerosol products. In this lecture I will proceed through a survey of these products, answering the following questions as I proceed. What are the products? How do they compare with ground truth? How do we use these products to describe the global aerosol system? Are aerosols increasing or decreasing? How do aerosols affect climate and clouds?

Remer, Lorraine↗