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At least 1,639 records · Page 91
All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

Spatially-resolved soot evolution and statistics in high-pressure diesel spray flames using two-color pyrometry

Previous studies of diesel spray flames have focused on details of the sooting behavior mainly during the quasi-steady period, but few have considered the spatially-resolved transient evolution in combination with injection-to-injection variations. In this study, a 500-injection data set is utilized to investigate the temporal evolution of a spray flame during auto-ignition, the premixed burn phase, and the quasi-steady period. Spatially-resolved OH* chemiluminescence data provide ignition delay times and reaction zone locations. Two-color pyrom-etry with a vastly improved optical system is used to quantify spatially-resolved soot evolution and its statistical variations. The ambient thermodynamic con-ditions are slightly below those in modern diesel engines, resulting in longer lift-off lengths and lower overall soot production. Spatially, soot formation in the lift-off region is small, but appreciable soot forms in the jet core and jet head regions, while it oxidizes gradually on the jet periphery. Total soot mass profiles indicate that regions with larger local soot mass take longer to form, but are the first to oxidize. Probability distributions of soot mass in localized regions indicate that a few injections with high soot mass bias the average soot mass data towards higher values. Altogether, results show good agreement with previous studies employing different diagnostic techniques while providing statistical details of transient and localized soot behavior in high pressure diesel spray flames in support of the related modeling efforts.

09 BIOMASS FUELS↗
DOE OSTI2025

Expanding the homogeneity range of UFe 2 : Formation of Laves phase UFe 2 +Ni

Uranium-based intermetallic Laves phases (UM 2 ) provide valuable insight into the interplay of 5f orbital hybridization and magnetic properties. However, ferromagnetism in these compounds is rare. UFe 2 is a cubic C15 Laves phase with greatest Curie temperature (T C ) of all such compounds, at 162 K. In this study, we report the synthesis and characterization of a novel U-based Laves phase, UFe 2 +Ni, effectively forcing excess Ni in to the UFe 2 structure. UFe 2 +Ni crystallizes in the cubic C15 Laves phase, appearing to deviate from the typical UM 2 formula and exhibiting a significantly extended homogeneity range. Annealing this material leads to an increased ferromagnetic transition temperature, between 35 and 155 K, and decreased lattice parameter with higher annealing temperatures. This variation is attributed to changes in Fe and Ni solubility with annealing temperature. In conclusion, our findings highlight the potential for tuning magnetic properties in U-based Laves phases through compositional and thermal modifications, expanding the understanding of magnetically ordered intermetallics.

Annealing effects↗
DOE OSTI2022

A general framework for gravitational charges and holographic renormalization

We develop a general framework for constructing charges associated with diffeomorphisms in gravitational theories using covariant phase space techniques. This framework encompasses both localized charges associated with space–time subregions, as well as global conserved charges of the full space–time. Expressions for the charges include contributions from the boundary and corner terms in the subregion action, and are rendered unambiguous by appealing to the variational principle for the subregion, which selects a preferred form of the symplectic flux through the boundaries. The Poisson brackets of the charges on the subregion phase space are shown to reproduce the bracket of Barnich and Troessaert for open subsystems, thereby giving a novel derivation of this bracket from first principles. In the context of asymptotic boundaries, we show that the procedure of holographic renormalization can be always applied to obtain finite charges and fluxes once suitable counterterms have been found to ensure a finite action. This enables the study of larger asymptotic symmetry groups by loosening the boundary conditions imposed at infinity. We further present an algorithm for explicitly computing the counterterms that renormalize the action and symplectic potential, and, as an application of our framework, demonstrate that it reproduces known expressions for the charges of the generalized Bondi–Metzner–Sachs algebra.

Physics↗
DOE OSTI2021

Study of the Effect of Reflections on High-Power, 110-GHz Pulsed Gyrotron Operation

The effect of reflection is studied experimentally and theoretically on a high-power 110-GHz gyrotron operating in the TE 22,6 mode in 3 μs pulses at 96 kV, 40 A. The experimental setup allows variation of the reflected power from 0 to 33% over a range of gyrotron operating conditions. The phase of the reflection is varied by translating the reflector along the axis. Operating at a higher efficiency point, at 4.40 T with 940kW of output power, reflected power exceeding 11% causes a switch from operation in the TE 22,6 to simultaneous operation in the TE 22,6 and TE 21,6 modes with a large decrease of the total gyrotron output power. This switching effect is in good agreement with simulations using the MAGY code. Operating at a more stable point, 4.44 T with 580kW of output power, when the reflection is increased, the output power remains in the TE 22,6 mode but it decreases monotonically with increasing reflection, dropping to 200kW at 33% reflection. Furthermore, at a reflection above 22%, a power modulation at 25 to 30MHz is observed, independent of the phase of the reflected wave. Such a modulated signal may be useful in spectroscopic and other applications.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2021

Topological approach to electron correlations at fractional quantum Hall effect

Highlights: • Braids in 2D electron systems in magnetic field acquire a cyclotron metrics. • Commensurability of 2D braids with Wigner crystal of electrons leads to FQHE. • Homotopy invariants define the hierarchy of FQHE universal in all 2D Hall systems. • Composite fermions illustrate multiloop braids in the simplest homotopy case. • Correlations in FQHE reveal long-range quantum entanglement of all electrons. The classification of homotopy invariants in interacting multi-electron 2D systems at quantizing magnetic fields is presented, explaining the topologically protected correlations occurring at integer and fractional quantum Hall effects. The long-range quantum entanglement is essential for homotopy correlated phases in contrast to the binary entanglement for conventional phases with local order parameters. The classification of homotopy long-range correlated phases induced by the Coulomb interaction of electrons has been derived in terms of homotopy invariants, which are universal and robust against local disorder and single-particle crystal field, as illustrated by experimental observations in various materials with different microscopic structure, like GaAs 2DES, graphene monolayer and bilayer and in Chern topological insulators. The homotopy phases are demonstrated to be topologically protected and immune to single-particle perturbations, temperature chaos and variation of the electron interaction strength. The nonzero repulsive interaction between electrons is shown, however, to be essential for the definition of the homotopy invariants, which disappear in gaseous systems.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2025

Remote sensing of Pu in uranyl nitrate crystals using reflectance spectroscopy and chemometrics

Remote quantification of Pu(VI) (0–5 mol%) co-crystallized with U in uranyl nitrate hexahydrate (UNH) crystals was achieved in a glove box using reflectance spectroscopy coupled with chemometric modeling. Reflectance spectra were also acquired for Pu(IV) and Np(VI) (0–5 mol%) crystallized with UNH; revealing spectral features consistent with their solution-phase analogs. Principal component analysis revealed Pu(IV/VI) and Np(VI) concentrations as the primary source of variation in the data, informing the development of a supervised partial least squares regression model for Pu(VI). The resulting calibration demonstrated robust performance, with replicate root mean square errors near 10% and quantifiable limits near 0.2 mol% Pu(VI) relative to U. The Pu(VI) remained stable in the crystalline UNH matrix for at least one week with minimal reduction to Pu(IV). Notably, Pu(VI) and Np(VI) incorporation in UNH quenched U(VI) fluorescence while Pu(IV) did not. This study presents a noninvasive, spectroscopic approach for solid-state Pu quantification, with direct implications for material accountability and nuclear nonproliferation monitoring.

Sadergaski, Luke R. [Oak Ridge National Laboratory↗
DOE OSTI2020

Machine learning for nonintrusive model order reduction of the parametric inviscid transonic flow past an airfoil

Fluid flow in the transonic regime finds relevance in aerospace engineering, particularly in the design of commercial air transportation vehicles. Computational fluid dynamics models of transonic flow for aerospace applications are computationally expensive to solve because of the high degrees of freedom as well as the coupled nature of the conservation laws. While these issues pose a bottleneck for the use of such models in aerospace design, computational costs can be significantly minimized by constructing special, structure-preserving surrogate models called reduced-order models. In this work, we propose a machine learning method to construct reduced-order models via deep neural networks and we demonstrate its ability to preserve accuracy with a significantly lower computational cost. In addition, our machine learning methodology is physics-informed and constrained through the utilization of an interpretable encoding by way of proper orthogonal decomposition. Application to the inviscid transonic flow past the RAE2822 airfoil under varying freestream Mach numbers and angles of attack, as well as airfoil shape parameters with a deforming mesh, shows that the proposed approach adapts to high-dimensional parameter variation well. Notably, the proposed framework precludes the knowledge of numerical operators utilized in the data generation phase, thereby demonstrating its potential utility in the fast exploration of design space for diverse engineering applications. Comparison against a projection-based nonintrusive model order reduction method demonstrates that the proposed approach produces comparable accuracy and yet is orders of magnitude computationally cheap to evaluate, despite being agnostic to the physics of the problem.

97 MATHEMATICS AND COMPUTING↗
DOE OSTI2021

Chemical pumps and flexible sheets spontaneously form self-regulating oscillators in solution

The synchronization of self-oscillating systems is vital to various biological functions, from the coordinated contraction of heart muscle to the self-organization of slime molds. Through modeling, we design bioinspired materials systems that spontaneously form shape-changing self-oscillators, which communicate to synchronize both their temporal and spatial behavior. Here, catalytic reactions at the bottom of a fluid-filled chamber and on mobile, flexible sheets generate the energy to “pump” the surrounding fluid, which also transports the immersed sheets. The sheets exert a force on the fluid that modifies the flow, which in turn affects the shape and movement of the flexible sheets. This feedback enables a single coated (active) and even an uncoated (passive) sheet to undergo self-oscillation, displaying different oscillatory modes with increases in the catalytic reaction rate. Two sheets (active or passive) introduce excluded volume, steric interactions. This distinctive combination of the hydrodynamic, fluid–structure, and steric interactions causes the sheets to form coupled oscillators, whose motion is synchronized in time and space. We develop a heuristic model that rationalizes this behavior. These coupled self-oscillators exhibit rich and tunable phase dynamics, which depends on the sheets’ initial placement, coverage by catalyst and relative size. Moreover, through variations in the reactant concentration, the system can switch between the different oscillatory modes. This breadth of dynamic behavior expands the functionality of the coupled oscillators, enabling soft robots to display a variety of self-sustained, self-regulating moves.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2023

CMIP6 skill at predicting interannual to multi-decadal summer monsoon precipitation variability

Monsoons affect the economy, agriculture, and human health of two thirds of the world’s population. Therefore, predicting variations in monsoon precipitation is societally important. We explore the ability of climate models from the sixth phase of the Climate Model Intercomparison Project to predict summer monsoon precipitation variability by using hindcasts from the Decadal Climate Prediction Project (Component A). The multi-model ensemble-mean shows significant skill at predicting summer monsoon precipitation from one year to 6–9 years ahead. However, this skill is dependent on the model, monsoon domain, and lead-time. In general, the skill of the multi-model ensemble-mean prediction is low in year 1 but increases for longer-lead times and is largely consistent with externally forced changes. The best captured region is northern Africa for the 2–5 and 6–9 year forecast lead times. In contrast, there is no significant skill using the ensemble-mean over East and South Asia and, furthermore, there is significant spread in skill among models for these domains. By sub-sampling the ensemble we show that the difference in skill between models is tied to the simulation of the externally forced response over East and South Asia, with models with a more skilful forced response capable of better predictions. A further contribution is from skilful prediction of Pacific Ocean temperatures for the South Asian summer monsoon at longer lead-times. Therefore, these results indicate that predictions of the East and South Asian monsoons could be significantly improved.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

Process Intensification by One-Step, Plasma-Assisted Catalytic Synthesis of Liquid Chemicals from Light Hydrocarbons

In this project, we present a plasma-assisted, catalytic process that can handle variations in production rates and gas compositions of producing wells and reliably converts the hydrocarbons to gas phase olefins, high molecular weight alkanes, and liquid chemicals. The low-temperature plasma serves as a reactive chemical environment that activates and converts the light hydrocarbons to these valuable products. We present results from the integration of a catalyst into the low-temperature plasma zone to improve reaction efficiency and product selectivity. We show that the gas composition, bulk gas temperature, and input power of the plasma, with and without catalysts, influence the production rates of liquids from natural gas feeds.

03 NATURAL GAS↗
NASA NTRS1972

Numerical analysis method for linear induction machines.

A numerical analysis method has been developed for linear induction machines such as liquid metal MHD pumps and generators and linear motors. Arbitrary phase currents or voltages can be specified and the moving conductor can have arbitrary velocity and conductivity variations from point to point. The moving conductor is divided into a mesh and coefficients are calculated for the voltage induced at each mesh point by unit current at every other mesh point. Combining the coefficients with the mesh resistances yields a set of simultaneous equations which are solved for the unknown currents.

Elliott, D. G.↗
NASA NTRS1972

The phase discrepancy between temperature and density in the thermosphere

The observations of thermospheric densities by satellite drag analysis and the thermospheric temperatures by back scatter radar measurements show a phase difference. The dependence of this phase difference on various factors is briefly reviewed. It is shown that by choosing certain boundary conditions at 120 km the observations of both temperature and densities become consistent. The possible range of boundary conditions is analysed. Furthermore it is shown that the phase discrepancy is largely due to the higher harmonic components of both the temperature and the density variation in the thermosphere.

Blum, P. W.↗
NASA NTRS1973

Latitude measures of Jupiter in the 0.89 micron methane band

Jupiter has been photographed by the Lunar and Planetary Laboratory in the 0.89 micron methane band since October 1968. A photometric evaluation of these photographs has not yet been carried out, but a visual study of this collection and a comparison with the color records has been made. This comparison, together with diameter and latitude measures of the methane records, shows that the albedos and latitudes of most features shown in 0.89 micron vary with time and the albedos and latitudes of most features shown in 0.89 micron vary with time and that there is no simple correlation between the visual color and/or intensity of a feature and its intensity in the methane band. The latitudes of the Red Spot and South Tropical Zone have remained unchanged, while those of the Equatorial Zone, North Tropical Zone, and South Polar Hood have changed. Measures of images taken near opposition show the polar diameter to be within 0.5% of the American Ephemeris Value, but the equatorial diameter as 1.3% smaller. Measures near quadrature suggest a phase defect 3.5 times greater in value than the American Ephemeris value. The large phase defect and bright South Polar Hood contribute to the circular appearance of Jupiter in methane. Latitude variations of the North edge of the South Polar Hood support the 1964 Munch and Younkin hypothesis that this feature is composed of frozen methane.

Minton, R. B.↗
NASA NTRS1973

Partial pressures of oxygen, phosphorus and fluorine in some lunar lavas

Lunar sample 14310 is a feldspar-rich basalt which shows no evidence of shock deformation or recrystallization. Pyroxenes include Mg-rich orthopyroxene, pigeonite and augite; pyroxferroite occurs in the interstitial residuum. Plagioclase feldspars are zoned from An(96) to An(67), and variations in feldspar compositions do not necessarily indicate loss of Na during eruption of the lava. Opaque phases include ilmenite, ulvospinel, metallic iron, troilite, and schreibersite. Both whitlockite and apatite are present, and the interstitial residua contain baddeleyite, tranquillityite and barium-rich sanidine. Theoretical calculations provide estimates of partial pressures of oxygen, phosphorus, and fluorine in lunar magmas. In general, partial pressures of oxygen are restricted by the limiting assemblages of iron-wuestite and ilmenite-iron-rutile; phosphorus partial pressures are higher in lunar magmas than in terrestrial lavas. The occurrence of whitlockite indicates significantly lower fugacities of fluorine in lunar magmas than in terrestrial magmas.

Nash, W. P.↗
NASA NTRS1973

PLZT block data composers operated in differential phase mode

The use of PLZT ceramics with the 7/65/35 composition in block data composer (BDC) input devices for holographic memory systems has previously been described for operation in the strain biased, scattering, and edge effect modes. A new and promising mode of BDC operation is the differential phase mode in which each element of a matrix array BDC acts as a phase modulator. The phase modulation results from a phase difference in the optical path length between the electrically poled and depoled states of the PLZT. It is shown that a PLZT BDC can be used as a matrix-type phase modulator to record and process digital data by the differential phase mode in a holographic recording/processing system with readout contrast ratios of between 10:1 and 15:1. The differential phase mode has the advantages that strain bias is not required and that the thickness and strain variations in the PLZT are cancelled out.

Drake, M. D.↗
NASA NTRS1976

The observation program for the GSFC cosmic X-ray spectroscopy experiment

The cosmic X-ray spectroscopy experiment on OSO-8 will observe seven X-ray binary sources in its first six months of operation. If possible, each of these sources will be observed for one or more binary orbits so that the X-ray spectrum of each object can be observed through all phases of its orbit. For the two pulsing binaries, Her X-1 and Cen X-3, spectral variations over the pulse period will be studied. Simultaneous radio observations of Cyg X-1 and Cyg X-3 will search for any correlation between radio and X-ray emission. During the first year of operation, the detectors will observe over 50% of the known X-ray sources.

Becker, R. H.↗
NASA NTRS1976

Latitudinal changes of composition in the disturbed thermosphere from Esro 4 measurements

Densities of N2, O, Ar, and He at a height of 280 km, obtained from gas analyzer measurements aboard Esro-4, were analyzed to establish a global pattern for variations that are associated with geomagnetically induced disturbances. It is shown that during longer periods of sustained geomagnetic activity, thermospheric temperature increases with geomagnetic latitude, reaching a maximum in the region of the magnetic pole, while during short-lived magnetic storms, the maximum temperature may be reached in the auroral zones. The observed variations of composition in middle and high latitudes can be explained by assuming that temperature variations are accompanied by variations in the height of the homopause. In the equatorial region the four gases studied vary in phase with similar amplitudes during a magnetic storm, indicating a density wave proceeding from higher latitudes.

Jacchia, L. G.↗