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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 1,639 records · Page 91
All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

Anomalous thermal effect in Zr Te 5 observed via photothermal measurements

In this study, we explore the magneto-thermoelectric power (MTP) of $ZrTe$ 5 , a canonical Dirac semimetal, through a novel photothermal technique. Unlike conventional thermoelectric studies that rely on on-chip heaters and are limited by fabrication processes, especially for stress-sensitive materials, our approach utilizes photothermal effects to induce temperature gradients. Our experiments, applying a magnetic field approximately parallel and transverse to the photocurrent detection direction, reveal that the photothermal method efficiently and reliably extracts both diagonal and off-diagonal components of the thermoelectric coefficient of $ZrTe$ 5 . Here, we observe that the longitudinal MTP reproduces features previously reported in thermal transport studies, while the photoinduced transverse MTP confirms the anomalous Nernst effect. This photothermal measurement technique opens new avenues for investigating transport properties in a wide range of quantum materials, both in 3D and 2D systems.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2020

Confinement, reduced entanglement, and spin-glass order in a random quantum spin-ice model

In this work, we study an effective spin model derived perturbatively from a random transverse-field Ising model on the pyrochlore lattice. The model consists of spin configurations on the pyrochlore lattice, restricted to the spin-ice subspace, with spins interacting with random Ising exchange couplings as well as ring exchanges along the hexagons of the lattice. This model is studied by exact diagonalization up to N=64 site systems. Furthermore, we calculate spin-glass correlation functions and local entanglement entropy S T between spins in a single tetrahedron and the rest of the system. We find that the model undergoes two phase transitions. At weak randomness the model is in a quantum spin-ice phase where S T =ln 6. Increasing randomness, at low transverse fields, first leads to a frozen phase, with long-range spin-glass order and S T =ln 2 corresponding to the Cat states associated with Ising order. Further increase in randomness leads to a random resonating-hexagon phase with a frozen backbone of spins and a broad distribution of entanglement entropies. The implications of these studies for non-Kramers rare-earth pyrochlores are discussed.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2020

Effective theory of superconductivity in strongly coupled amorphous materials

A theory of phonon-mediated superconductivity in strong-coupling amorphous materials is developed based on an effective description of structural disorder and its effect on the vibrational spectrum. The theory accounts for the diffusivelike transport of vibrational excitations due to disorder-induced scattering within the Eliashberg theory of strong-coupling superconductivity. The theory provides a good analytical description of the Eliashberg function $α^2F(ω)$ in comparison with experiments and allows one to disentangle the effects of transverse and longitudinal excitations on the Eliashberg function. In particular, it shows that the transverse excitations play a crucial role in driving an increase or excess in the Eliashberg function at low energy, which is related to the boson peak phenomenon in vibrational spectra of glasses. This low-energy excess, on the one hand, drives an enhancement of the electron-phonon coupling but at the same time reduces the characteristic energy scale $ω_{\text{log}}$ in the Allen-Dynes formula. As a consequence, the nonmonotonicity of $T_c$ as a function of alloying (disorder) in Pb-based systems can be rationalized. Further, the case of Al-based systems, where disorder increases $T_c$ from the start, is also analyzed. General material-design principles for enhancing $T_c$ in amorphous superconductors are presented.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2021

Prediction and observation of intermodulation sidebands from anharmonic phonons in NaBr

A quantum Langevin model, like models from optomechanics, was developed for phonons. It predicts intermodulation phonon sidebands (IPSs) in anharmonic crystals. Ab initio calculations of anharmonic phonons in rock-salt NaBr showed these spectral features as many-body effects. Modern inelastic neutron scattering measurements on a crystal of NaBr at 300 K revealed diffuse intensity at high phonon energy from a predicted upper IPS. The transverse optical (TO) part of the new features originates from phonon intermodulation between the transverse acoustic (TA) and TO phonons. The longitudinal optical spectral features originate from three-phonon coupling between the TA modes and the TO lattice modes. The partner lower IPS proves to be an intrinsic localized mode. Interactions with the thermal bath broaden and redistribute the spectral weight of the IPS pair. These sidebands are a probe of the anharmonicity and quantum noise of phonons in NaBr and suggest novel interactions between photons and phonons.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2021

Dynamics of Spin Polarization in Tilted Polariton Rings

We have observed the effect of pseudomagnetic field originating from the polaritonic analog of spin-orbit coupling [transverse electric and transverse magnetic (TE-TM) splitting] on a polariton condensate in a ring-shaped microcavity. The effect gives rise to a stable four-leaf pattern around the ring as seen from the linear polarization measurements of the condensate photoluminescence. This pattern is found to originate from the interplay of the cavity potential, energy relaxation, and TE-TM splitting in the ring. Our observations are compared to the dissipative one-dimensional spinor Gross-Pitaevskii equation with the TE-TM splitting energy, which shows good qualitative agreement.

CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS↗
DOE OSTI2021

Topological Nernst effect, anomalous Nernst effect, and anomalous thermal Hall effect in the Dirac semimetal Fe 3 Sn 2

Topological semimetals have been a focal point of research in recent years. One of the salient characters of topological semimetals is the anomalous Hall effect arising from the nontrivial momentum-space Berry phase. In contrast, anomalous transverse thermoelectric coefficient and thermal Hall effect are much less explored up to date. In this paper, we report thermoelectric and thermal transport properties of Fe 3 Sn 2 , a prototypical Dirac semimetal. We find that Fe 3 Sn 2 exhibits large topological Nernst effect which is associated with the non-zero spin chirality of the skyrmion bubble phase. Furthermore, Fe 3 Sn 2 shows prominent anomalous thermal Hall effect and anomalous Nernst effect with features similar to the anomalous Hall effect. The anomalous Nernst signal is about 2.1 μV/K at room temperature, which is comparable to the largest value reported thus far. These results highlight the synergic effects of Berry phase in both real space and momentum space of Fe 3 Sn 2 , and this study demonstrates an effective strategy of investigating topological materials by measuring their transverse thermal and thermoelectric responses.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2021

Z 2 topological order and first-order quantum phase transitions in systems with combinatorial gauge symmetry

We study a generalization of the two-dimensional transverse-field Ising model, combining both ferromagnetic and antiferromagnetic two-body interactions, that hosts exact global and local Z 2 gauge symmetries. Using exact diagonalization and stochastic series expansion quantum Monte Carlo methods, we confirm the existence of the topological phase in line with previous theoretical predictions. Our simulation results show that the transition between the confined topological phase and the deconfined paramagnetic phase is of first order, in contrast to the conventional Z 2 lattice gauge model in which the transition maps onto that of the standard Ising model and is continuous. We further generalize the model by replacing the transverse field on the gauge spins with a ferromagnetic X X interaction while keeping the local gauge symmetry intact. We find that the Z 2 topological phase remains stable, while the paramagnetic phase is replaced by a ferromagnetic phase. The topological-ferromagnetic quantum phase transition is also of first order. For both models, we discuss the low-energy spinon and vison excitations of the topological phase and their avoided level crossings associated with the first-order quantum phase transitions.

2-dimensional systems↗
DOE OSTI2022

Anomalous Nernst and Seebeck coefficients in epitaxial thin film Co 2 MnAl x Si 1 - x and Co 2 FeAl

Here we have measured the Seebeck and anomalous Nernst coefficients and corresponding transverse and longitudinal thermoelectric conductivities from 2 to 400 K in thin film (thickness t ~10 nm) Co 2 MnAl x Si 1-x (0 ≤ x ≤ 1) and Co 2 FeAl grown by molecular beam epitaxy (MBE). A large (-14 A m -1 K -1 at 300 K) anomalous component of the transverse thermoelectric conductivity is observed in Co 2 MnAl, especially as contrasted to Co 2 MnSi (0.28 A m -1 K -1 at 300 K). This enhancement is likely due to Weyl points close to the Fermi level of Co 2 MnAl which disappear as x decreases.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Topological Nernst and topological thermal Hall effect in rare-earth kagome ScMn 6 Sn 6

Thermal and thermoelectric measurements are known as powerful tools to uncover the physical properties of quantum materials due to their sensitivity towards the scattering and chirality of heat carriers. We use these techniques to confirm the presence of momentum and real-space topology in ScMn 6 Sn 6 . There is an unconventional dramatic increase in the Seebeck coefficient on entering the transverse conical spiral (TCS) state below $T$ = 200 K, suggesting an unusual scattering of heat carriers. In addition, the observed anomalous thermal Hall effect and the anomalous Nernst effect indicate nonzero Berry curvature in k space. Furthermore, we identify a significant topological contribution to the thermal Hall and Nernst signals in the TCS phase revealing the impacts of real-space Berry curvature. We discuss the presence of the topological thermal Hall effect and topological Nernst effect in the diverse HfFe 6 Ge 6 family. In conclusion, this study illustrates the importance of transverse thermal and thermoelectric measurements to investigate the origin of topological transport in the noncoplanar magnetic phases in this family of kagome metals.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2023

Slowly decaying zero mode in a weakly nonintegrable boundary impurity model

The transverse field Ising model (TFIM) on the half-infinite chain possesses an edge zero mode. This work considers an impurity model: TFIM perturbed by a boundary integrability-breaking interaction. For sufficiently large transverse field, but in the ordered phase of the TFIM, the zero mode is observed to decay. The decay is qualitatively different from zero modes where the integrability-breaking interactions are nonzero all along the chain. It is shown that for the impurity model, the zero mode decays by relaxing to a nonlocal quasiconserved operator, the latter being exactly conserved when the opposite edge of the chain has no noncommuting perturbations so as to ensure perfect degeneracy of the spectrum. In the thermodynamic limit, the quasiconserved operator vanishes, and a regime is identified where the decay of the zero mode obeys Fermi's golden rule. Furthermore, a toy model for the decay is constructed in Krylov space and it is highlighted how Fermi's golden rule may be recovered from this toy model.

1-dimensional systems↗
DOE OSTI2024

Gallery of soft modes: Theory and experiment at a ferromagnetic quantum phase transition

We examine the low-energy excitations in the vicinity of the quantum critical point in LiHoF4, a physical realization of the Transverse Field Ising Model, focusing on the long-range fluctuations which soften to zero energy at the ferromagnetic quantum phase transition. Microwave spectroscopy in tunable loop-gap resonator structures identifies and characterizes the electronuclear soft mode and higher-energy electronuclear states as a function of frequency and magnetic fields applied transverse and parallel to the Ising axis. These are understood in the context of a theoretical model of a soft electronuclear mode that interacts with soft photons as well as soft phonons. We identify competing infrared divergences at the quantum critical point, coming from the photons and the electronuclear soft mode. It is an incomplete cancellation of these divergences that leads to the muted but distinct signatures observed in the experiments. The application of a longitudinal magnetic field gaps the soft mode. As a result, measurements well away from the quantum critical point reveal a set of "Walker'' modes associated with ferromagnetic domain dynamics.

Dipolar interaction↗
DOE OSTI2024

Universal model of Floquet operator Krylov space

It is shown that the stroboscopic time evolution under a Floquet unitary, in any spatial dimension, and of any Hermitian operator, can be mapped to an operator Krylov space, which is identical to that generated by the edge operator of the noninteracting Floquet transverse-field Ising model (TFIM) in one-spatial dimension, and with inhomogeneous Ising and transverse field couplings. The latter has four topological phases reflected by the absence (topologically trivial) or presence (topologically nontrivial) of edge modes at 0 and/or π quasienergies. It is shown that the Floquet dynamics share certain universal features characterized by how the Krylov parameters vary in the topological phase diagram of the Floquet TFIM with homogeneous couplings. Furthermore, these results are highlighted through examples, all chosen for numerical convenience to be in one spatial dimension: nonintegrable Floquet spin 1/2 chains and Floquet Z 3 clock model where the latter hosts period-tripled edge modes.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2024

Quantum embedding study of strain- and electric-field-induced Stark effects on the NV - center in diamond

The NV - color center in diamond has been demonstrated as a powerful nanosensor for quantum metrology due to the sensitivity of its optical and spin properties to external electric, magnetic, and strain fields. In view of these applications, we use quantum embedding to derive a many-body description of strain- and electric-field-induced Stark effects on the NV - center. Here, we quantify how strain longitudinal to the axis of NV - shifts the excited states in energy, while strain with a component transverse to the NV - axis splits the degeneracies of the 3 E and 1 E states. The largest effects are for the optically relevant 3 E manifold, which splits into E x and E y with transverse strain. From these responses we extract strain susceptibilities for the E x/y states within the quasilinear regime. Additionally, we study the many-body dipole matrix elements of the NV - and find a permanent dipole 1.6 D at zero strain, which is somewhat smaller than that obtained from recent density functional theory calculations. We also determine the transition dipole between the E x and E y and how it evolves with strain.

47 OTHER INSTRUMENTATION↗
DOE OSTI2020

Nuclear modification of leading hadrons and jets within a virtuality ordered parton shower

In this work, the event generator based on the higher-twist energy loss formalism—Modular All Twist Transverse-scattering Elastic-drag and Radiation (M ATTER )—is further developed and coupled to a hydrodynamic model for studying jet modification in relativistic nuclear collisions. The probability of parton splitting is calculated using the Sudakov form factor that is constructed by a combination of vacuum and medium-induced splitting functions; and the full parton showers are simulated, including both energy-momentum and space-time evolutions of all jet partons. With the assumption that partons below a virtual scale of 1 GeV is absorbed by the medium, this framework is able to provide a reasonable description of the nuclear modification of both leading hadrons and jets at high transverse momentum at the BNL Relativistic Heavy Ion Collider and the CERN Large Hadron Collider.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Bulk properties of the system formed in Au + Au collisions at s N N = 14.5 GeV at the BNL STAR detector

We report systematic measurements of bulk properties of the system created in Au+Au collisions at √ S NN = 14.5 GeV recorded by the STAR detector at the Relativistic Heavy Ion Collider (RHIC). The transverse momentum spectra of π ± , K ± and p(p¯) are studied at mid-rapidity (|y| < 0.1) for nine centrality intervals. The centrality, transverse momentum (p T ), and pseudorapidity (η) 3 dependence of inclusive charged particle elliptic flow (v 2 ), and rapidity-odd charged particles directed flow (v 1 ) results near mid-rapidity are also presented. These measurements are compared with the published results from Au+Au collisions at other energies, and from Pb+Pb collisions at √ S NN =2.76 TeV. The results at √ S NN = 14.5 GeV show similar behavior as established at other energies and fit well in the energy dependence trend. Furthermore, these results are important as the 14.5 GeV energy fills the gap in μ B, which is of the order of 100 MeV, between √ S NN =11.5 and 19.6 GeV. Comparisons of the data with UrQMD and AMPT models show poor agreement in general.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2021

Prehydrodynamic evolution and its signatures in final-state heavy-ion observables

We investigate the effects of prehydrodynamic evolution on final-state observables in heavy-ion collisions using state-of-the art event simulations coupled to different prehydrodynamic scenarios, which include the recently developed effective kinetic transport theory evolution model KøMPøST. Differential flow observables are found to be mostly insensitive to the details of prehydrodynamic evolution. The main effect we observe is in the p T spectra, particularly the mean transverse momentum. However, at least part of this effect is a consequence of the underlying conformal invariance assumption currently present in such approaches, which is known to be violated in the temperature regime probed in heavy-ion collisions. This assumption of early time conformal invariance leads to an artificially large out-of-equilibrium bulk pressure when switching from (conformal) prehydrodynamic evolution to hydrodynamics (using the nonconformal QCD equation of state), which in turn increases the transverse momentum. Our study indicates that a consistent treatment of prehydrodynamic evolution in heavy-ion collisions requires the use of nonconformal models of early time dynamics.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Cumulants and correlation functions of net-proton, proton, and antiproton multiplicity distributions in Au+Au collisions at energies available at the BNL Relativistic Heavy Ion Collider

Here, we report a systematic measurement of cumulants, C n , for net-proton, proton, and antiproton multiplicity distributions, and correlation functions, κ n , for proton and antiproton multiplicity distributions up to the fourth order in Au+Au collisions at $\sqrt{s_{NN}}$ = 7.7, 11.5, 14.5, 19.6, 27, 39, 54.4, 62.4, and 200 GeV. The C n and κ n are presented as a function of collision energy, centrality and kinematic acceptance in rapidity, y, and transverse momentum, p T . The data were taken during the first phase of the Beam Energy Scan (BES) program (2010–2017) at the BNL Relativistic Heavy Ion Collider (RHIC) facility. The measurements are carried out at midrapidity (|y| < 0.5) and transverse momentum 0.4 < p T < 2.0 GeV/c, using the STAR detector at RHIC. We observe a nonmonotonic energy dependence ($\sqrt{s_{NN}}$ = 7.7–62.4 GeV) of the net-proton C 4 /C 2 with the significance of 3.1σ for the 0–5% central Au+Au collisions. This is consistent with the expectations of critical fluctuations in a QCD-inspired model. Thermal and transport model calculations show a monotonic variation with $\sqrt{s_{NN}}$. For the multiparticle correlation functions, we observe significant negative values for a two-particle correlation function, κ 2 , of protons and antiprotons, which are mainly due to the effects of baryon number conservation. Furthermore, it is found that the four-particle correlation function, κ 4 , of protons plays a role in determining the energy dependence of proton C 4 /C 1 below 19.6 GeV, which cannot be understood by the effect of baryon number conservation.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Imprints of high-momentum nucleons in nuclei on hard photons from heavy-ion collisions near the Fermi energy

The short-range correlation (SRC) induced by the tensor force in the isosinglet neutron-proton interaction channel leads to a high-momentum tail (HMT) in the single-nucleon momentum distributions n(k) in nuclei. Owing to the remaining uncertainties about the tensor force, the shape of the nucleon HMT may be significantly different from the dilute interacting Fermi gas model prediction n(k) ~ 1/k 4 similar to the HMT in cold atoms near the unitary limit. Within an isospin- and momentum-dependent Boltzmann-Uehling-Uhlenbeck transport model incorporating approximately the nucleon HMT, we investigate hard photon emissions in 14 N + 12 C and 48 Ca + 124 Sn reactions at beam energies around the Fermi energy. Imprints of different shapes of the HMT on the energy spectrum, angular distribution and transverse momentum spectrum of hard photons are studied. Furthermore, while the angular distribution does not carry any information about the shape of the nucleon HMT, the energy spectra and especially the mid-rapidity transverse momentum spectra of hard photons are found to bare strong imprints of the shapes of nucleon HMTs in the two colliding nuclei.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗