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At least 1,639 records · Page 91

Gas Dynamics, Characterization, and Calibration of Fast Flow Flight Cascade Impactor Quartz Crystal Microbalances (QCM) for Aerosol Measurements

During recent high altitude flights, we have tested the aerosol section of the fast flow flight cascade impactor quartz crystal microbalance (QCM) on loan to Howard University from NASA. The aerosol mass collected during these flights was disappointingly small. Increasing the flow through the QCM did not correct the problem. It was clear that the instrument was not being operated under proper conditions for aerosol collect ion primarily because the gas dynamics is not well understood. A laboratory study was therefore undertaken using two different fast flow QCM's in an attempt to establish the gas flow characteristics of the aerosol sections and its effect on particle collection, Some tests were made at low temperatures but most of the work reported here was carried out at room temperature. The QCM is a cascade type impactor originally designed by May (1945) and later modified by Anderson (1966) and Mercer et al (1970) for chemical gas analysis. The QCM has been used extensively for collecting and sizing stratospheric aerosol particles. In this paper all flow rates are given or corrected and referred to in terms of air at STP. All of the flow meters were kept at STP. Although there have been several calibration and evaluation studies of moderate flow cascade impactors of less than or equal to 1 L/rein., there is little experimental information on the gas flow characteristics for fast flow rates greater than 1 L/rein.

Grant, J.R.↗

What we can Learn About Aerosols from EOS-MISR Multi-Angle Remote Sensing Observations

Multiangle, multispectral remote sensing observations, such as those anticipated from the Earth Observing System (EOS) Multiangle Imaging SpectroRadiometer (MISR), promise to significantly improve our ability to constrain aerosol properties from space. Recent advances in modeling the Earth's climate have brought us to a point where the contributions made by aerosols to the global radiation budget noticeably affect the results. Knowledge of both aerosol optical depth and the microphysical properties of particles is needed to adequately model aerosol effects. This talk explores the ability of multiangle, multi-spectral remote sensing observations anticipated from the EOS MISR instrument, to retrieve aerosol optical depth and information about mixes of particle types, globally, at 17.6 km spatial resolution. The instrument is scheduled for launch into a 10:30 AM, sun-synchronous polar orbit in 1999.

Kahn, Ralph↗

Remote Sensing of Aerosol Backscatter and Earth Surface Targets By Use of An Airborne Focused Continuous Wave CO2 Doppler Lidar Over Western North America

Airborne lidar systems are used to determine wind velocity and to measure aerosol or cloud backscatter variability. Atmospheric aerosols, being affected by local and regional sources, show tremendous variability. Continuous wave (cw) lidar can obtain detailed aerosol loading with unprecedented high resolution (3 sec) and sensitivity (1 mg/cubic meter) as was done during the 1995 NASA Multi-center Airborne Coherent Atmospheric Wind Sensor (MACAWS) mission over western North America and the Pacific Ocean. Backscatter variability was measured at a 9.1 micron wavelength cw focused CO2 Doppler lidar for approximately 52 flight hours, covering an equivalent horizontal distance of approximately 30,000 km in the troposphere. Some quasi-vertical backscatter profiles were also obtained during various ascents and descents at altitudes that ranged from approximately 0.1 to 12 km. Similarities and differences for aerosol loading over land and ocean were observed. Mid-tropospheric aerosol backscatter background mode was approximately 6 x 10(exp -11)/ms/r, consistent with previous lidar datasets. While these atmospheric measurements were made, the lidar also retrieved a distinct backscatter signal from the Earth's surface from the unfocused part of the focused cw lidar beam during aircraft rolls. Atmospheric backscatter can be highly variable both spatially and temporally, whereas, Earth-surface backscatter is relatively much less variant and can be quite predictable. Therefore, routine atmospheric backscatter measurements by an airborne lidar also give Earth surface backscatter which can allow for investigating the Earth terrain. In the case where the Earth's surface backscatter is coming from a well-known and fairly uniform region, then it can potentially offer lidar calibration opportunities during flight. These Earth surface measurements over varying Californian terrain during the mission were compared with laboratory backscatter measurements using the same lidar of various Earth surfaces giving good agreement, suggesting that the lidar efficiency, and thus a lidar calibration factor for detection, can be estimated fairly well using Earth's surface signal.

Jarzembski, Maurice A.↗

Global Distribution and Sources of Volatile and Nonvolatile Aerosol In the Remote Troposphere

Airborne measurements of aerosol (Condensation Nuclei, CN) and selected trace gases made in the areas of the North Atlantic Ocean during SONEX (October/November 1997), and the south tropical Pacific Ocean during PEM-Tropics A (September/October 1996) and PEM-Tropics B (March/April 1999) have been analyzed. Emphasis is on the interpretations of variations in the number densities of the fine (>17 nm) and ultrafine (>8 nm) CN in the upper troposphere (8-12 km). These data suggest that large number densities of highly volatile CN (10(exp 4)-10(exp 5)/cu cm) are present in the clean upper troposphere with highest values over the tropical1subtropical region. Through marine convection and long-distance horizontal transport, volatile CN originating from the tropical/subtropical regions can frequently impact the abundance of aerosol in the middle and upper troposphere at mid to high latitudes. Nonvolatile aerosol particles behave in a manner similar to tracers of combustion (CO) and photochemical pollution (PAN), implying a source from continental pollution of industrial or biomass burning origin. In the upper troposphere, we find that volatile and nonvolatile partials number densities are inversely correlated. An aerosol microphysical model is used to suggest that coagulation of fine volatile particles with fewer larger nonvolatile particles provides one possible mechanism for this relationship. It appears that nonvolatile particles, of principally anthropogenic origin,provide a highly efficient removal process for the fine volatile aerosol.

Singh, Hanwant B.↗

Properties of Stratospheric Aerosol Estimated from HALOE Data

Extinction coefficients for stratospheric aerosols at 8 HALOE (HALogen Occultation Experiment) wavelengths are determined by comparing transmittances data for two adjacent solar occultation measurements, where one limb path is loaded with aerosols but the other path is free of aerosols. These extinction coefficients are used to infer the aerosol properties such as composition and size distribution parameters. Mie theory has been used to calculate the extinction coefficients, and a nonlinear least square method is applied to determine the aerosol properties. Sixteen cases are selected for the retrieval in southern hemisphere at latitudes from 21 to 48 deg S for the period of 29 Mar - 31 May 1992. Retrieved size width ranges from 1.1 to 1.5 and radius ranges from 0.25 to 0.45 micrometers. These size parameters are within the ranges of in situ measurements at Laramie, Wyoming. Retrieved weight percent of H2SO4 is larger than the equilibrium value by about 5 to approximately 10 weight percent, similar to the results for northern hemisphere at latitudes 20 to 55 deg N for the period from Nov 1991 to Feb. 1992.

Lee, Kwang-Mog↗

Effect of Aerosols on Cloud Field with Satellite-Derived Data and GCM Simulation

Numerical experiment was performed using an general circulation model (GCM) including aerosol indirect effect into water cloud and the simulated global distribution of cloud droplet radii was compared with the global distribution of cloud effective radii retrieved from Advanced Very High Resolution Radiometer (AVHRR). Comparisons of GCM calculation with AVHRR retrieval showed that our GCM generally can simulate the global characteristics of cloud droplet radii such as a land-sea contrast associated with difference of aerosol abundance and coastal region feature due to aerosol injection from adjacent continental area. AVHRR retrieval and GCM simulation, however, are turned out to show disagreement over tropical region. AVHRR retrieval may tend to overestimate droplet radii due to the contamination of signal by drizzles and ice particles, whereas our GCM does not treat aerosol indirect effect in deep convective clouds predominant over tropics. Over equatorial central Pacific, where satellite retrieval may suffer from statistical biases, satellite retrieval and GCM simulation are also found to be different. Keywords: aerosol indirect effect

Suzuki, Kentaroh↗

Measurements of the Vertical Structure of Aerosols and Clouds Over the Ocean Using Micro-Pulse LIDAR Systems

The determination of the vertical distribution of aerosols and clouds over the ocean is needed for accurate retrievals of ocean color from satellites observations. The presence of absorbing aerosol layers, especially at altitudes above the boundary layer, has been shown to influence the calculation of ocean color. Also, satellite data must be correctly screened for the presence of clouds, particularly cirrus, in order to measure ocean color. One instrument capable of providing this information is a lidar, which uses pulses of laser light to profile the vertical distribution of aerosol and cloud layers in the atmosphere. However, lidar systems prior to the 1990s were large, expensive, and not eye-safe which made them unsuitable for cruise deployments. During the 1990s the first small, autonomous, and eye-safe lidar system became available: the micro-pulse lidar, or MPL. The MPL is a compact and eye-safe lidar system capable of determining the range of aerosols and clouds by firing a short pulse of laser light (523 nm) and measuring the time-of-flight from pulse transmission to reception of a returned signal. The returned signal is a function of time, converted into range using the speed of light, and is proportional to the amount of light backscattered by atmospheric molecules (Rayleigh scattering), aerosols, and clouds. The MPL achieves ANSI eye-safe standards by sending laser pulses at low energy (micro-J) and expanding the beam to 20.32 cm in diameter. A fast pulse-repetition-frequency (2500 Hz) is used to achieve a good signal-to-noise, despite the low output energy. The MPL has a small field-of-view (< 100 micro-rad) and signals received with the instrument do not contain multiple scattering effects. The MPL has been used successfully at a number of long-term sites and also in several field experiments around the world.

Welton, Ellsworth J.↗

Center for Aerosol Research (AEROCENTER)

The newly established Center for Aerosol Research (AEROCENTER) located at the NASA/Goddard Space Flight Center in Greenbelt MD is dedicated to fostering interdisciplinary research in all aspects of aerosol science. AEROCENTER will be an incubator for innovative new analysis of existing data and ideas for new space missions. The plan is to tap and harvest ideas from a broad international and interdisciplinary science community and to incorporate these ideas into NASA's aerosol research effort for understanding and predicting the aerosol effect on climate and the environment. In order to achieve this goal the center aims to host several established and developing scientists for a period of 3-6 months each year. AEROCENTER will also develop a new technical infrastructure that will integrate the present aerosol research activities and data resources of GSFC/Greenbelt and GSFC/GISS, increase efficiency in the use of NASA remote sensing data, and increase the involvement of a larger national and international scientific community. The center aims to institutionalize and extend the present knowledge base within NASA into a national resource for the education and research communities.

Kleidman, Richard↗

Physical and Optical/Radiative Characteristics of Aerosol and Cloud Particles in Tropical Cirrus: Importance in Radiation Balance

Whether cirrus clouds heat or cool the Earth-atmosphere system depends on the relative importance of the cloud shortwave albedo effect and the cloud thermal greenhouse effect. Both are determined by the distribution of ice condensate with cloud particle size. The microphysics instrument package flown aboard the NASA DC-8 in TOGA/COARE included an ice crystal replicator, a 2D Greyscale Cloud Particle Probe and a Forward Scattering Spectrometer Aerosol Probe. In combination, the electro-optical instruments permitted particle size measurements between 0.5 micrometer and 2.6 millimeter diameter. Ice crystal replicas were used to validate signals from the electrooptical instruments. Both optical and scanning electron microscopy were utilized to analyze aerosol and ice particle replicas between 0.1 micrometer and several 100 micrometer diameter. In first approximation, the combined aerosol-cloud particle spectrum in several clouds followed a power law N alpha D(sup -2.5). Thus, large cloud particles carried most of the condensate mass, while small cloud and aerosol particles determined the surface area. The mechanism of formation of small particles is growth of (hygroscopic, possibly ocean-derived) aerosol particles along the Kohler curves. The concentration of small particles is higher and less variable in space and time, and their tropospheric residence time is longer, than those of large cloud particles because of lower sedimentation velocities. Small particles shift effective cloud particle radii to sizes much smaller than the mean diameter of the cloud particles. This causes an increase in shortwave reflectivity and IR emissivity, and a decrease in transmissivity. Occasionally, the cloud reflectivity increased with altitude (decreasing temperature) stronger than did cloud emissivity, yielding enhanced radiative cooling at higher altitudes. Thus, cirrus produced by deep convection in the tropics may be critical in controlling processes whereby energy from warm tropical oceans is injected to different levels in the atmosphere to subsequently influence not only tropical but mid-latitude climate.

Pueschel, R. F.↗

Airborne Lidar Measurements of Aerosol Optical Properties During SAFARI-2000

The Cloud Physics Lidar (CPL) operated onboard the NASA ER-2 high altitude aircraft during the SAFARI-2000 field campaign. The CPL provided high spatial resolution measurements of aerosol optical properties at both 1064 nm and 532 nm. We present here results of planetary boundary layer (PBL) aerosol optical depth analysis and profiles of aerosol extinction. Variation of optical depth and extinction are examined as a function of regional location. The wide-scale aerosol mapping obtained by the CPL is a unique data set that will aid in future studies of aerosol transport. Comparisons between the airborne CPL and ground-based MicroPulse Lidar Network (MPL-Net) sites are shown to have good agreement.

McGill, M. J.↗

Coordinated Airborne, Spaceborne, and Ground-Based Measurements of Massive, Thick Aerosol Layers During the Dry Season in Southern Africa

During the dry-season airborne campaign of the Southern African Regional Science Initiative (SAFARI 2000), unique coordinated observations were made of massive, thick aerosol layers. These layers were often dominated by aerosols from biomass burning. We report on airborne Sunphotometer measurements of aerosol optical depth (lambda=354-1558 nm), columnar water vapor, and vertical profiles of aerosol extinction and water vapor density that were obtained aboard the University of Washington's Convair-580 research aircraft. We compare these with ground-based AERONET Sun/sky radiometer results, with ground based lidar data MPL-Net), and with measurements from a downward-pointing lidar aboard the high-flying NASA ER-2 aircraft. Finally, we show comparisons between aerosol optical depths from the Sunphotometer and those retrieved over land and over water using four spaceborne sensors (TOMS (Total Ozone Mapping Spectrometer), MODIS (Moderate Resolution Imaging Spectrometer), MISR (Multiangle Imaging Spectroradiometer) and ATSR-2 (Along Track Scanning Radiometer)).

Schmid, B.↗

Airborne Sunphotometer Measurements of Aerosol Optical Depth and Columnar Water Vapor During the Puerto Rico Dust Experiment, and Comparison with Land, Aircraft, and Satellite Measurements

Analyses of aerosol optical depth (AOD) and columnar water vapor (CWV) measurements obtained with the six-channel NASA Ames Airborne Tracking Sunphotometer (AATS-6) mounted on a twin-engine aircraft during the summer 2000 Puerto Rico Dust Experiment are presented. In general, aerosol extinction values calculated from AATS-6 AOD measurements acquired during aircraft profiles up to 5 km ASL reproduce the vertical structure measured by coincident aircraft in-situ measurements of total aerosol number and surface area concentration. Calculations show that the spectral dependence of AOD was small (mean Angstrom wavelength exponents of approximately 0.20) within three atmospheric layers defined as the total column beneath the top of each aircraft profile, the region beneath the trade wind inversion, and the region within the Saharan Air Layer (SAL) above the trade inversion. This spectral behavior is consistent with attenuation of incoming solar radiation by large dust particles or by dust plus sea salt. Values of CWV calculated from profile measurements by AATS-6 at 941.9 nm and from aircraft in-situ measurements by a chilled mirror dewpoint hygrometer agree to within approximately 4% (0.13 g/sq cm). AATS-6 AOD values measured on the ground at Roosevelt Roads Naval Air Station and during low altitude aircraft runs over the adjacent Cabras Island aerosol/radiation ground site agree to within 0.004 to 0.030 with coincident data obtained with an AERONET Sun/sky Cimel radiometer located at Cabras Island. For the same observation times, AERONET retrievals of CWV exceed AATS-6 values by a mean of 0.74 g/sq cm (approximately 21 %) for the 2.9-3.9 g/sq cm measured by AATS-6. Comparison of AATS-6 aerosol extinction values obtained during four aircraft ascents over Cabras Island with corresponding values calculated from coincident aerosol backscatter measurements by a ground-based micro-pulse lidar (MPL-Net) located at Cabras yields a similar vertical structure above the trade inversion. Finally, AATS-6 AOD values measured during low altitude aircraft traverses over the ocean are compared with corresponding AOD values retrieved over water from upwelling radiance measurements by the MODIS, TOMS, and GOES-8 Imager satellite sensors, with mixed results. These exercises highlight the need for continued satellite sensor comparison/validation studies to improve satellite AOD retrieval algorithms, and the usefulness of airborne sunphotometer measurements in the validation process.

Livingston, John M.↗

Airborne DIAL Ozone and Aerosol Trends Observed at High Latitudes Over North America from February to May 2000

Ozone (O3) and aerosol scattering ratio profiles were obtained from airborne lidar measurements on thirty-eight aircraft flights over seven aircraft deployments covering the latitudes of 40 deg.-85 deg.N between 4 February and 23 May 2000 as part of the TOPSE (Tropospheric Ozone Production about the Spring Equinox) field experiment. The remote and in situ O3 measurements were used together to produce a vertically-continuous O3 profile from near the surface to above the tropopause. Ozone, aerosol, and potential vorticity (PV) distributions were used together to identify the presence of pollution plumes and stratospheric intrusions. The number of observed pollution plumes was found to increase into the spring along with a significant increase in aerosol loading. Ozone was found to increase in the middle free troposphere (4-6 km) at high latitudes (60 deg.-85 deg. N) by an average of 4.3 ppbv/mo from about 55 ppbv in early February to over 72 ppbv in mid-May. The average aerosol scattering ratios in the same region increased at an average rate of 0.37/mo from about 0.35 to over 1.7. Ozone and aerosol scattering were highly correlated over entire field experiment. Based on the above results and the observed aircraft in-situ measurements, it was estimated that stratospherically-derived O3 accounted for less than 20% of the observed increase in mid tropospheric O3 at high latitudes. The primary cause of the observed O3 increase was found to be the photochemical production of O3 in pollution plumes.

Hair, Jonathan W.↗

Evaluation of the MODIS Retrievals of Dust Aerosol over the Ocean during PRIDE

The Puerto Rico Dust Experiment (PRIDE) took place in Roosevelt Roads, Puerto Rico from June 26 to July 24,2000 to study the radiative and physical properties of African dust aerosol transported into the region. PRIDE had the unique distinction of being the first major field experiment to allow direct comparison of aerosol retrievals from the MODerate Imaging Spectro-radiometer (MODIS) with sunphotometer and in-situ aerosol measurements. Over the ocean, the MODIS algorithm retrieves aerosol optical depth (AOD) as well as information about the aerosols size distribution. During PRIDE, MODIS derived AODs in the red wavelengths (0.66 micrometers) compare closely with AODs measured from sunphotometers, but, are too large at blue and green wavelengths (0.47 and 0.55 micrometers) and too small in the infrared (0.87 micrometers). This discrepancy of spectral slope results in particle size distributions retrieved by MODIS that are small compared to in-situ measurements, and smaller still when compared to sunphotometer sky radiance inversions. The differences in size distributions are, at least in part, associated with MODIS simplification of dust as spherical particles. Analysis of this PRIDE data set is a first step towards derivation of realistic non-spherical models for future MODIS retrievals.

Levy, Robert C.↗

Boundary Layer Aerosol Composition over Sierra Nevada Mountains using 9.11- and 10.59-micron CW Lidars and Modeled Backscatter from Size Distribution Data

An inversion technique has been developed to determine volume fractions of an atmospheric aerosol composed primarily of ammonium sulfate and ammonium nitrate and water combined with fixed concentration of elemental and organic carbon. It is based on measured aerosol backscatter obtained with 9.11 - and 10.59-micron wavelength continuous wave CO2 lidars and modeled backscatter from aerosol size distribution data. The technique is demonstrated during a flight of the NASA DC-8 aircraft over the Sierra Nevada Mountain Range, California on 19 September, 1995. Volume fraction of each component and effective complex refractive index of the composite particle were determined assuming an internally mixed composite aerosol model. The volume fractions were also used to re-compute aerosol backscatter, providing good agreement with the lidar-measured data. The robustness of the technique for determining volume fractions was extended with a comparison of calculated 2.1,-micron backscatter from size distribution data with the measured lidar data converted to 2.1,-micron backscatter using an earlier derived algorithm, verifying the algorithm as well as the backscatter calculations.

Cutten, D. R.↗

Longwave Radiative Forcing of Saharan Dust Aerosols Estimated from MODIS, MISR and CERES Observations on Terra

Using observations from the Multi-angle Imaging Spectroradiometer (MISR), the Moderate Resolution Imaging Spectroradiometer (MODIS), and the Clouds and the Earth's Radiant Energy System (CERES) instruments onboard the Terra satellite; we present a new technique for studying longwave (LW) radiative forcing of dust aerosols over the Saharan desert for cloud-free conditions. The monthly-mean LW forcing for September 2000 is 7 W/sq m and the LW forcing efficiency' (LW(sub eff)) is 15 W/sq m. Using radiative transfer calculations, we also show that the vertical distribution of aerosols and water vapor are critical to the understanding of dust aerosol forcing. Using well calibrated, spatially and temporally collocated data sets, we have combined the strengths of three sensors from the same satellite to quantify the LW radiative forcing, and show that dust aerosols have a "warming" effect over the Saharan desert that will counteract the shortwave "cooling effect" of aerosols.

Zhang, Jiang-Long↗

Airborne Sun Photometer Measurements of Aerosol Optical Depth during SOLVE II: Comparison with SAGE III and POAM III Measurements

The 14-channel NASA Ames Airborne Tracking Sunphotometer (AATS-14) was operated aboard the NASA DC-8 during the Second SAGE III Ozone Loss and Validation Experiment (SOLVE II) and obtained successful measurements during the sunlit segments of eight science flights. These included six flights out of Kiruna, Sweden, one flight out of NASA Dryden Flight Research Center (DFRC), and the Kiruna-DFRC return transit flight. Values of spectral aerosol optical depth (AOD), columnar ozone and columnar water vapor have been derived from the AATS-14 measurements. In this paper, we focus on AATS-14 AOD data. In particular, we compare AATS-14 AOD spectra with temporally and spatially near-coincident measurements by the Stratospheric Aerosol and Gas Experiment III (SAGE III) and the Polar Ozone and Aerosol Measurement III (POAM III) satellite sensors. We examine the effect on retrieved AOD of uncertainties in relative optical airmass (the ratio of AOD along the instrument-to-sun slant path to that along the vertical path) at large solar zenith angles. Airmass uncertainties result fiom uncertainties in requisite assumed vertical profiles of aerosol extinction due to inhomogeneity along the viewing path or simply to lack of available data. We also compare AATS-14 slant path solar transmission measurements with coincident measurements acquired from the DC-8 by the NASA Langley Research Center Gas and Aerosol Measurement Sensor (GAMS).

Russell, P.↗

Observations of Dust Using the NASA Geoscience Laser Altimeter System (GLAS): New New Measurements of Aerosol Vertical Distribution From Space

On January 12, 2003 NASA launched the first satellite-based lidar, the Geoscience Laser -Altimeter System (GLAS), onboard the ICESat spacecraft. The GLAS atmospheric measurements introduce a fundamentally new and important tool for understanding the atmosphere and climate. In the past, aerosols have only been studied from space using images gathered by passive sensors. Analysis of this passive data has lead to an improved understanding of aerosol properties, spatial distribution, and their effect on the earth's climate. However, these images do not show the aerosol's vertical distribution. As a result, a key piece of information has been missing. The measurements now obtained by GLAS will provide information on the vertical distribution of aerosols and clouds, and improve our ability to study their transport processes and aerosol-cloud interactions. Here we show an overview of GLAS, provide an update of its current status, and present initial observations of dust profiles. In particular, a strategy of characterizing the height profile of dust plumes over source regions will be presented.

Welton, Ellsworth↗