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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 1,621 records · Page 90
All sourcesNASA NTRSDOE OSTI
DOE OSTI2015

A new look at the position operator in quantum theory

The postulate that coordinate and momentum representations are related to each other by the Fourier transform has been accepted from the beginning of quantum theory by analogy with classical electrodynamics. As a consequence, an inevitable effect in standard theory is the wave packet spreading (WPS) of the photon coordinate wave function in directions perpendicular to the photon momentum. This leads to the following paradoxes: if the major part of photons emitted by stars are in wave packet states (what is the most probable scenario) then we should see not separate stars but only an almost continuous background from all stars; no anisotropy of the CMB radiation should be observable; data on gamma-ray bursts, signals from directional radio antennas (in particular, in experiments on Shapiro delay) and signals from pulsars show no signs of WPS. In addition, a problem arises why there are no signs of WPS for protons in the LHC ring. We argue that the above postulate is based neither on strong theoretical arguments nor on experimental data and propose a new consistent definition of the position operator. Then WPS in directions perpendicular to the particle momentum is absent and the paradoxes are resolved. Different components of the new position operator do not commute with each other and, as a consequence, there is no wave function in coordinate representation. Implications of the results for entanglement, quantum locality and the problem of time in quantum theory are discussed.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2017

Subminiature emitters based on a single (111) In(Ga)As quantum dot and hybrid microcavity

The results of numerical modeling and investigation of a hybrid microcavity based on a semiconductor Bragg reflector and a microlens selectively positioned above a single (111) In(Ga)As quantum dot are presented. Emitters based on the hybrid microcavity demonstrate the effective pumping of a single quantum dot and high emission output efficiency. The microcavity design can be used to implement emitters of polarization- entangled photon pairs based on single semiconductor quantum dots.

36 MATERIALS SCIENCE↗
DOE OSTI2018

The Pulsed Excitation in Two-Qubit Systems

The temporal dynamics of absorption of a single-photon pulse by two qubits interacting with a microwave field of a one-dimensional waveguide have been studied. The theory, which allows one to use arbitrary shapes of the input single-photon wave packet as an initial condition, as well as investigate the excitation dynamics of each qubit, has been developed. The numerical calculation is performed for the packet of a Gaussian shape, at different parameters of frequency detuning and duration of the input pulse. The excitation dynamics of both identical and nonidentical qubits have been studied. It has been specifically shown that it is possible to form symmetric and antisymmetric entangled states for identical qubits.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2022

Random Quantum Circuits

Quantum circuits—built from local unitary gates and local measurements—are a new playground for quantum many-body physics and a tractable setting to explore universal collective phenomena far from equilibrium. These models have shed light on longstanding questions about thermalization and chaos, and on the underlying universal dynamics of quantum information and entanglement. In addition, such models generate new sets of questions and give rise to phenomena with no traditional analog, such as dynamical phase transitions in quantum systems that are monitored by an external observer. Quantum circuit dynamics is also topical in view of experimental progress in building digital quantum simulators that allow control of precisely these ingredients. Randomness in the circuit elements allows a high level of theoretical control, with a key theme being mappings between real-time quantum dynamics and effective classical lattice models or dynamical processes. Many of the universal phenomena that can be identified in this tractable setting apply to much wider classes of more structured many-body dynamics.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2016

Quantum Coherence and Random Fields at Mesoscopic Scales

We seek to explore and exploit model, disordered and geometrically frustrated magnets where coherent spin clusters stably detach themselves from their surroundings, leading to extreme sensitivity to finite frequency excitations and the ability to encode information. Global changes in either the spin concentration or the quantum tunneling probability via the application of an external magnetic field can tune the relative weights of quantum entanglement and random field effects on the mesoscopic scale. These same parameters can be harnessed to manipulate domain wall dynamics in the ferromagnetic state, with technological possibilities for magnetic information storage. Finally, extensions from quantum ferromagnets to antiferromagnets promise new insights into the physics of quantum fluctuations and effective dimensional reduction. A combination of ac susceptometry, dc magnetometry, noise measurements, hole burning, non-linear Fano experiments, and neutron diffraction as functions of temperature, magnetic field, frequency, excitation amplitude, dipole concentration, and disorder address issues of stability, overlap, coherence, and control. We have been especially interested in probing the evolution of the local order in the progression from spin liquid to spin glass to long-range-ordered magnet.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2023

Tunneling between Multiple Histories as a Solution to the Information Loss Paradox

The information loss paradox associated with black hole Hawking evaporation is an unresolved problem in modern theoretical physics. In a recent brief essay, we revisited the evolution of the black hole entanglement entropy via the Euclidean path integral (EPI) of the quantum state and allow for the branching of semi-classical histories along the Lorentzian evolution. We posited that there exist at least two histories that contribute to EPI, where one is an information-losing history, while the other is an information-preserving one. At early times, the former dominates EPI, while at the late times, the latter becomes dominant. By doing so, we recovered the essence of the Page curve, and thus, the unitarity, albeit with the turning point, i.e., the Page time, much shifted toward the late time. In this full-length paper, we fill in the details of our arguments and calculations to strengthen our notion. One implication of this modified Page curve is that the entropy bound may thus be violated. We comment on the similarity and difference between our approach and that of the replica wormholes and the islands’ conjectures.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2016

Analysis of flows inside quiescent prominences as captured by Hinode/solar optical telescope

Developing an understanding of how magnetic fields can become entangled in a prominence is important for predicting a possible eruption. This work investigates the kinetic energy and vorticity associated with plasma motion residing inside quiescent prominences (QPs). These plasma flow characteristics can be utilized to improve our understanding of how the prominence maintains a stable magnetic field configuration. Three different contrast-enhanced solar prominence observations from Hinode/Solar Optical Telescope were used to construct velocity maps—in the plane of the sky—via a Fourier local correlation tracking program. The resulting velocities were then used to perform the first-ever analysis of the two-dimensional kinetic energy and enstrophy spectra of a prominence. Enstrophy is introduced here as a means of quantifying the vorticity that has been observed in many QPs. The kinetic energy power spectral density (PSD) produced indices ranging from −1.00 to −1.60. There was a consistent anisotropy in the kinetic energy spectrum of all three prominences examined. Examination of the intensity PSD reveals that a different scaling relationship exists between the observed prominence structure and velocity maps. All of the prominences exhibited an inertial range of at least 0.8⩽k⩽2.0 rads Mm{sup −1}. Quasi-periodic oscillations were also detected in the centroid of the velocity distributions for one prominence. Additionally, a lower limit was placed on the kinetic energy density (ϵ ∼ 0.22–7.04 km{sup 2} s{sup −2}) and enstrophy density (ω ∼ 1.43–13.69 × 10{sup −16} s{sup −2}) associated with each prominence.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2017

Effects of Magnetic and Kinetic Helicities on the Growth of Magnetic Fields in Laminar and Turbulent Flows by Helical Fourier Decomposition

We present a numerical and analytical study of incompressible homogeneous conducting fluids using a helical Fourier representation. We analytically study both small- and large-scale dynamo properties, as well as the inverse cascade of magnetic helicity, in the most general minimal subset of interacting velocity and magnetic fields on a closed Fourier triad. We mainly focus on the dependency of magnetic field growth as a function of the distribution of kinetic and magnetic helicities among the three interacting wavenumbers. By combining direct numerical simulations of the full magnetohydrodynamics equations with the helical Fourier decomposition, we numerically confirm that in the kinematic dynamo regime the system develops a large-scale magnetic helicity with opposite sign compared to the small-scale kinetic helicity, a sort of triad-by-triad α -effect in Fourier space. Concerning the small-scale perturbations, we predict theoretically and confirm numerically that the largest instability is achived for the magnetic component with the same helicity of the flow, in agreement with the Stretch–Twist–Fold mechanism. Vice versa, in the presence of Lorentz feedback on the velocity, we find that the inverse cascade of magnetic helicity is mostly local if magnetic and kinetic helicities have opposite signs, while it is more nonlocal and more intense if they have the same sign, as predicted by the analytical approach. Our analytical and numerical results further demonstrate the potential of the helical Fourier decomposition to elucidate the entangled dynamics of magnetic and kinetic helicities both in fully developed turbulence and in laminar flows.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2017

Evidence for Galaxy Dynamics Tracing Background Cosmology Below the de Sitter Scale of Acceleration

Galaxy dynamics probe weak gravity at accelerations below the de Sitter scale of acceleration a{sub dS}=cH, where c is the velocity of light and H is the Hubble parameter. Low- and high-redshift galaxies hereby offer a novel probe of weak gravity in an evolving cosmology, satisfying H(z)=H{sub 0}√(1+ω{sub m}(6z+12z{sup 2}+12z{sup 3}+6z{sup 4}+(6/5)z{sup 5}))/(1+z) with matter content ω{sub m}=0.2808±0.028 sans tension to H {sub 0} in surveys of the local universe. Galaxy rotation curves show anomalous galaxy dynamics in weak gravity a{sub N}<a{sub dS} across a transition radius r{sub t}=4.7 kpc M{sub 11}{sup 1/2}(H{sub 0}/H){sup (1/2)} in galaxies of mass M=10{sup 11} M{sub ⊙}M{sub 11}, where a {sub N} is the Newtonian acceleration based on baryonic matter content. We identify this behavior with a holographic origin of inertia from entanglement entropy, which introduces a C {sup 0} onset across a{sub N}=a{sub dS} with asymptotic behavior described by a Milgrom parameter satisfying a{sub 0}=ω{sub 0}/2π, where ω{sub 0}=√(1−q)H is a fundamental eigenfrequency of the cosmological horizon. Extending an earlier confrontation with data covering 0.003≲a{sub N}/a{sub dS}≲1 at redshift z∼0 in Lellie et al., the modest anomalous behavior in the Genzel et al. sample at redshifts 0.854⩽z⩽2.282 is found to be mostly due to clustering 0.36≲a{sub N}/a{sub dS}≲1 close to the C {sup 0} onset to weak gravity and an increase of up to 65% in a {sub 0}.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2017

A Three-dimensional Magnetohydrodynamic Simulation of the Formation of Solar Chromospheric Jets with Twisted Magnetic Field Lines

This paper presents a three-dimensional simulation of chromospheric jets with twisted magnetic field lines. Detailed treatments of the photospheric radiative transfer and the equations of state allow us to model realistic thermal convection near the solar surface, which excites various MHD waves and produces chromospheric jets in the simulation. A tall chromospheric jet with a maximum height of 10–11 Mm and lifetime of 8–10 minutes is formed above a strong magnetic field concentration. The magnetic field lines are strongly entangled in the chromosphere, which helps the chromospheric jet to be driven by the Lorentz force. The jet exhibits oscillatory motion as a natural consequence of its generation mechanism. We also find that the produced chromospheric jet forms a cluster with a diameter of several Mm with finer strands. These results imply a close relationship between the simulated jet and solar spicules.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS2003

Linear optics and projective measurements for fun and profit

The technique of projective measurements in linear optics can provide an apparent, efficient nonlinear interaction between photons, which is technically problematic otherwise. We present an application of such a technique to prepare large photon-number path entanglement.

linear↗
DOE OSTI2018

Rainfall From Resolved Rather Than Parameterized Processes Better Represents the Present‐Day and Climate Change Response of Moderate Rates in the Community Atmosphere Model

Abstract Deficiencies in the parameterizations of convection used in global climate models often lead to a distorted representation of the simulated rainfall intensity distribution (i.e., too much rainfall from weak rain rates). While encouraging improvements in high percentile rainfall intensity have been found as the horizontal resolution of the Community Atmosphere Model is increased to ∼25 km, we demonstrate no corresponding improvement in the moderate rain rates that generate the majority of accumulated rainfall. Using a statistical framework designed to emphasize links between precipitation intensity and accumulated rainfall beyond just the frequency distribution, we show that CAM cannot realistically simulate moderate rain rates, and cannot capture their intensification with climate change, even as resolution is increased. However, by separating the parameterized convective and large‐scale resolved contributions to total rainfall, we find that the intensity, geographic pattern, and climate change response of CAM's large‐scale rain rates are more consistent with observations (TRMM 3B42), superparameterization, and theoretical expectations, despite issues with parameterized convection. Increasing CAM's horizontal resolution does improve the representation of total rainfall intensity, but not due to changes in the intensity of large‐scale rain rates, which are surprisingly insensitive to horizontal resolution. Rather, improvements occur through an increase in the relative contribution of the large‐scale component to the total amount of accumulated rainfall. Analysis of sensitivities to convective timescale and entrainment rate confirm the importance of these parameters in the possible development of scale‐aware parameterizations, but also reveal unrecognized trade‐offs from the entanglement of precipitation frequency and total amount.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2016

Soft materials with recoverable shape factors from extreme distortion states

We present elastomeric polysiloxane nanocomposites with elongations of >5000% (more than 3× greater than any previously reported material) with excellent shape recovery. Highly deformable materials are desirable for the fabrication of stretchable implants and microfluidic devices. No crosslinking or domain formation is observed by a variety of analytical techniques, suggesting that their elastomeric behavior is caused by polymer chain entanglements.

36 MATERIALS SCIENCE↗
DOE OSTI2019

Polymers with Side Chain Porosity for Ultrapermeable and Plasticization Resistant Materials for Gas Separations

Polymer membranes with ultrahigh CO 2 permeabilities and high selectivities are needed to address some of the critical separation challenges related to energy and the environment, especially in natural gas purification and postcombustion carbon capture. However, very few solution-processable, linear polymers are known today that access these types of characteristics, and all of the known structures achieve their separation performance through the design of rigid backbone chemistries that concomitantly increase chain stiffness and interchain spacing, thereby resulting in ultramicroporosity in solid-state chain-entangled films. Herein, the separation performance of a porous polymer obtained via ring-opening metathesis polymerization is reported, which possesses a flexible backbone with rigid, fluorinated side chains. This polymer exhibits ultrahigh CO 2 permeability (>21 000 Barrer) and exceptional plasticization resistance (CO 2 plasticization pressure > 51 bar). Compared to traditional polymers of intrinsic microporosity, the rate of physical aging is slower, especially for gases with small effective diameters (i.e., He, H 2 , and O 2 ). Overall, this structural design strategy, coupled with studies on fluorination, demonstrates a generalizable approach to create new polymers with flexible backbones and pore-forming side chains that have unexplored promise for small-molecule separations.

36 MATERIALS SCIENCE↗
DOE OSTI2021

Recent Advances in Functional Materials through Cellulose Nanofiber Templating

Advanced templating techniques have enabled delicate control of both nano- and microscale structures and have helped thrust functional materials into the forefront of society. Cellulose nanomaterials are derived from natural polymers and show promise as a templating source for advanced materials. Use of cellulose nanomaterials in templating combines nanoscale property control with sustainability, an attribute often lacking in other templating techniques. Use of cellulose nanofibers for templating has shown great promise in recent years, but previous reviews on cellulose nanomaterial templating techniques have not provided extensive analysis of cellulose nanofiber templating. Cellulose nanofibers display several unique properties, including mechanical strength, porosity, high water retention, high surface functionality, and an entangled fibrous network, all of which can dictate distinctive aspects in the final templated materials. Many applications exploit the unique aspects of templating with cellulose nanofibers that help control the final properties of the material, including, but not limited to, applications in catalysis, batteries, supercapacitors, electrodes, building materials, biomaterials, and membranes. A detailed analysis on the use of cellulose nanofibers templating is provided, addressing specifically how careful selection of templating mechanisms and methodologies, combined toward goal applications, can be used to directly benefit chosen applications in advanced functional materials.

36 MATERIALS SCIENCE↗
DOE OSTI2021

Ultralow Thermal Conductivity, Multiband Electronic Structure and High Thermoelectric Figure of Merit in TlCuSe

The entanglement of lattice thermal conductivity, electrical conductivity, and Seebeck coefficient complicates the process of optimizing thermoelectric performance in most thermoelectric materials. Semiconductors with ultralow lattice thermal conductivities and high power factors at the same time are scarce but fundamentally interesting and practically important for energy conversion. In this work, an intrinsic p-type semiconductor TlCuSe that has an intrinsically ultralow thermal conductivity (0.25 W m -1 K -1 ), a high power factor (11.6 μ W cm -1 K -2 ), and a high figure of merit, ZT (1.9) at 643 K is described. The weak chemical bonds, originating from the filled antibonding orbitals p-d* within the edge-sharing CuSe 4 tetrahedra and long Tl-Se bonds in the PbClF-type structure, in conjunction with the large atomic mass of Tl lead to an ultralow sound velocity. Strong anharmonicity, coming from Tl + lone-pair electrons, boosts phonon-phonon scattering rates and further suppresses lattice thermal conductivity. The multiband character of the valence band structure contributing to power factor enhancement benefits from the lone-pair electrons of Tl + as well, which modify the orbital character of the valence bands, and pushes the valence band maximum off the Gamma-point, increasing the band degeneracy. The results provide new insight on the rational design of thermoelectric materials.

36 MATERIALS SCIENCE↗
DOE OSTI2022

Machine Learning Guided Synthesis of Flash Graphene

Advances in nanoscience have enabled the synthesis of nanomaterials, such as graphene, from low-value or waste materials through flash Joule heating. Though this capability is promising, the complex and entangled variables that govern nanocrystal formation in the Joule heating process remain poorly understood. In this work, machine learning (ML) models are constructed to explore the factors that drive the transformation of amorphous carbon into graphene nanocrystals during flash Joule heating. An XGBoost regression model of crystallinity achieves an r 2 score of 0.8051 ± 0.054. Feature importance assays and decision trees extracted from these models reveal key considerations in the selection of starting materials and the role of stochastic current fluctuations in flash Joule heating synthesis. Furthermore, partial dependence analyses demonstrate the importance of charge and current density as predictors of crystallinity, implying a progression from reaction-limited to diffusion-limited kinetics as flash Joule heating parameters change. Finally, a practical application of the ML models is shown by using Bayesian meta-learning algorithms to automatically improve bulk crystallinity over many Joule heating reactions. Furthermore, these results illustrate the power of ML as a tool to analyze complex nanomanufacturing processes and enable the synthesis of 2D crystals with desirable properties by flash Joule heating.

01 COAL, LIGNITE, AND PEAT↗