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DOE OSTI2014

Intercomparison of Large-eddy Simulations of Arctic Mixed-phase Clouds: Importance of Ice Size Distribution Assumptions

Large-eddy simulations of mixed-phase Arctic clouds by 11 different models are analyzed with the goal of improving understanding and model representation of processes controlling the evolution of these clouds. In a case based on observations from the Indirect and Semi-Direct Aerosol Campaign (ISDAC), it is found that ice number concentration, Ni, exerts significant influence on the cloud structure. Increasing Ni leads to a substantial reduction in liquid water path (LWP) and potential cloud dissipation, in agreement with earlier studies. By comparing simulations with the same microphysics coupled to different dynamical cores as well as the same dynamics coupled to different microphysics schemes, it is found that the ice water path (IWP) is mainly controlled by ice microphysics, while the inter-model differences in LWP are largely driven by physics and numerics of the dynamical cores. In contrast to previous intercomparisons, all models here use the same ice particle properties (i.e., mass-size, mass-fall speed, and mass-capacitance relationships) and a common radiation parameterization. The constrained setup exposes the importance of ice particle size distributions (PSD) in influencing cloud evolution. A clear separation in LWP and IWP predicted by models with bin and bulk microphysical treatments is documented and attributed primarily to the assumed shape of ice PSD used in bulk schemes. Compared to the bin schemes that explicitly predict the PSD, schemes assuming exponential ice PSD underestimate ice growth by vapor deposition and overestimate mass-weighted fall speed leading to an underprediction of IWP by a factor of two in the considered case.

Arctic↗

NASA NTRS2007

Multi-Layer Arctic Mixed-Phase Clouds Simulated by a Cloud-Resolving Model: Comparison with ARM Observations and Sensitivity Experiments

A cloud-resolving model (CRM) is used to simulate the multiple-layer mixed-phase stratiform (MPS) clouds that occurred during a three-and-a-half day subperiod of the Department of Energy-Atmospheric Radiation Measurement Program s Mixed-Phase Arctic Cloud Experiment (M-PACE). The CRM is implemented with an advanced two-moment microphysics scheme, a state-of-the-art radiative transfer scheme, and a complicated third-order turbulence closure. Concurrent meteorological, aerosol, and ice nucleus measurements are used to initialize the CRM. The CRM is prescribed by time-varying large-scale advective tendencies of temperature and moisture and surface turbulent fluxes of sensible and latent heat. The CRM reproduces the occurrences of the single- and double-layer MPS clouds as revealed by the M-PACE observations. However, the simulated first cloud layer is lower and the second cloud layer thicker compared to observations. The magnitude of the simulated liquid water path agrees with that observed, but its temporal variation is more pronounced than that observed. As in an earlier study of single-layer cloud, the CRM also captures the major characteristics in the vertical distributions and temporal variations of liquid water content (LWC), total ice water content (IWC), droplet number concentration and ice crystal number concentration (nis) as suggested by the aircraft observations. However, the simulated mean values differ significantly from the observed. The magnitude of nis is especially underestimated by one order of magnitude. Sensitivity experiments suggest that the lower cloud layer is closely related to the surface fluxes of sensible and latent heat; the upper cloud layer is probably initialized by the large-scale advective cooling/moistening and maintained through the strong longwave (LW) radiative cooling near the cloud top which enhances the dynamical circulation; artificially turning off all ice-phase microphysical processes results in an increase in LWP by a factor of 3 due to interactions between the excessive LW radiative cooling and extra cloud water; heating caused by phase change of hydrometeors could affect the LWC and cloud top height by partially canceling out the LW radiative cooling. It is further shown that the resolved dynamical circulation appears to contribute more greatly to the evolution of the MPS cloud layers than the parameterized subgrid-scale circulation.

Luo, Yali↗

DOE OSTI2014

Scale dependence of entrainment-mixing mechanisms in cumulus clouds

This work empirically examines the dependence of entrainment-mixing mechanisms on the averaging scale in cumulus clouds using in situ aircraft observations during the Routine Atmospheric Radiation Measurement Aerial Facility Clouds with Low Optical Water Depths Optical Radiative Observations (RACORO) field campaign. A new measure of homogeneous mixing degree is defined that can encompass all types of mixing mechanisms. Analysis of the dependence of the homogenous mixing degree on the averaging scale shows that, on average, the homogenous mixing degree decreases with increasing averaging scales, suggesting that apparent mixing mechanisms gradually approach from homogeneous mixing to extreme inhomogeneous mixing with increasing scales. The scale dependence can be well quantified by an exponential function, providing first attempt at developing a scale-dependent parameterization for the entrainment-mixing mechanism. The influences of three factors on the scale dependence are further examined: droplet-free filament properties (size and fraction), microphysical properties (mean volume radius and liquid water content of cloud droplet size distributions adjacent to droplet-free filaments), and relative humidity of entrained dry air. It is found that the decreasing rate of homogeneous mixing degree with increasing averaging scales becomes larger with larger droplet-free filament size and fraction, larger mean volume radius and liquid water content, or higher relative humidity. The results underscore the necessity and possibility of considering averaging scale in representation of entrainment-mixing processes in atmospheric models.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS2016

Aerosol-Radiation-Cloud Interactions in the South-East Atlantic: Future Suborbital Activities to Address Knowledge Gaps in Satellite and Model Assessments

Southern Africa produces almost a third of the Earth's biomass burning (BB) aerosol particles. Particles lofted into the mid-troposphere are transported westward over the South-East (SE) Atlantic, home to one of the three permanent subtropical stratocumulus (Sc) cloud decks in the world. The SE Atlantic stratocumulus deck interacts with the dense layers of BB aerosols that initially overlay the cloud deck, but later subside and may mix into the clouds. These interactions include adjustments to aerosol-induced solar heating and microphysical effects, and their global representation in climate models remains one of the largest uncertainties in estimates of future climate. Hence, new observations over the SE Atlantic have significant implications for global climate change scenarios. Our understanding of aerosol-cloud interactions in the SE Atlantic is hindered both by the lack of knowledge on aerosol and cloud properties, as well as the lack of knowledge about detailed physical processes involved. Most notably, we are missing knowledge on the absorptive and cloud nucleating properties of aerosols, including their vertical distribution relative to clouds, on the locations and degree of aerosol mixing into clouds, on the processes that govern cloud property adjustments, and on the importance of aerosol effects on clouds relative to co-varying synoptic scale meteorology. We discuss the current knowledge of aerosol and cloud property distributions based on satellite observations and sparse suborbital sampling. Recent efforts to make full use of A-Train aerosol sensor synergies will be highlighted. We describe planned field campaigns in the region to address the existing knowledge gaps. Specifically, we describe the scientific objectives and implementation of the five synergistic, international research activities aimed at providing some of the key aerosol and cloud properties and a process-level understanding of aerosol-cloud interactions over the SE Atlantic: NASA's ORACLES, the UK Met Office's CLARIFY-2016, the DoE's LASIC, NSF's ONFIRE, and CNRS' AEROCLO-SA.

aerosols↗

NASA NTRS2017

Observations of Aerosol-Radiation-Cloud Interactions in the South-East Atlantic: First Results from the ORACLES Deployments in 2016 and 2017

Southern Africa produces almost a third of the Earths biomass burning (BB) aerosol particles. Particles lofted into the mid-troposphere are transported westward over the South-East (SE) Atlantic, home to one of the three permanent subtropical stratocumulus (Sc) cloud decks in the world. The SE Atlantic stratocumulus deck interacts with the dense layers of BB aerosols that initially overlay the cloud deck, but later subside and often mix into the clouds. These interactions include adjustments to aerosol-induced solar heating and microphysical effects, and their global representation in climate models remains one of the largest uncertainties in estimates of future climate. Hence, new observations over the SE Atlantic have significant implications for regional and global climate change predictions.The low-level clouds in the SE Atlantic have limited vertical extent and therefore present favorable conditions for their exploration with remote sensing. On the other hand, the normal coexistence of BB aerosols and Sc clouds in the same scene also presents significant challenges to conventional remote sensing techniques. We describe first results from NASAs airborne ORACLES (ObseRvations of Aerosols Above Clouds and Their IntEractionS) deployments in September 2016 and August 2017. We emphasize the unique role of polarimetric observations by two instruments, the Research Scanning Polarimeter (RSP) and the Airborne Multi-angle SpectroPolarimeter Imager (AirMSPI), and describe how these instruments help address specific ORACLES science objectives. Initial assessments of polarimetric observation accuracy for key cloud and aerosol properties will be presented, in as far as the preliminary nature of measurements permits.

Redemann, Jens↗

DOE OSTI2023

SAIL-Net Raw and Post Corrected POPS Data Fall 2021 - Summer 2023

SAIL-Net is a DOE funded project in the East River Watershed near Crested Butte, Colorado with the goal of advancing our understanding of aerosol-cloud interactions in complex, mountainous regions. Through the deployment of a network of six low cost microphysics nodes in Fall 2021 in the same domain at the SAIL campaign, SAIL-Net provides data on aerosol size distributions, cloud condensation nuclei (CCN), and ice nucleation particles (INP). This network enables the investigation of small-scale variations in complex terrain. Two datasets are provided - one containing raw data and the other containing post-corrected data. The raw dataset provides the raw data recorded from the POPS which were deployed at each of the six sites. These data are organized by site and broken down into daily data files. The six site names used here are: “gothic”, “irwin”, “cbtop”, “cbmid”, “pumphouse”, and “snodgrass”. These data are not cleaned or post-corrected, but some flags have been added. The data are reported at 1 second time resolution. The post-corrected dataset provides the post-corrected and cleaned data recorded from the POPS which were deployed at each of the six sites. This data are also organized by site (same as those found in the raw data) and broken down into daily data files. Unlike the raw POPS data, these data have already been cleaned to remove what we believe are bad values. These data should be ready to use with no cleaning. For a full description of the cleaning and post-correction process, see the readme.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2023

SAIL-Net CloudPuck CCN Data

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS2016

Aerosol-Radiation-Cloud Interactions in the South-East Atlantic: First Results from the ORACLES-2016 Deployment and Plans for Future Activities

Southern Africa produces almost a third of the Earths biomass burning (BB) aerosol particles. Particles lofted into the mid-troposphere are transported westward over the South-East (SE) Atlantic, home to one of the three permanent subtropical stratocumulus (Sc) cloud decks in the world. The SE Atlantic stratocumulus deck interacts with the dense layers of BB aerosols that initially overlay the cloud deck, but later subside and may mix into the clouds. These interactions include adjustments to aerosol-induced solar heating and microphysical effects, and their global representation in climate models remains one of the largest uncertainties in estimates of future climate. Hence, new observations over the SE Atlantic have significant implications for regional and global climate change predictions.Our understanding of aerosol-cloud interactions in the SE Atlantic is severely limited. Most notably, we are missing knowledge on the absorptive and cloud nucleating properties of aerosols, including their vertical distribution relative to clouds, on the locations and degree of aerosol mixing into clouds, on the processes that govern cloud property adjustments, and on the importance of aerosol effects on clouds relative to co-varying synoptic scale meteorology.We describe first results from various synergistic, international research activities aimed at studying aerosol-cloud interactions in the region:NASAs airborne ORACLES (ObseRvations of Aerosols Above Clouds and Their IntEractionS) deployment in AugustSeptember of 2016,the DoEs LASIC (Layered Atlantic Smoke Interactions with Clouds) deployment of the ARM Mobile Facility to Ascension Island (June 2016 October 2017), the ground-based components of CNRS AEROCLO-sA (Aerosols Clouds and Fog over the west coast of southern Africa), and ongoing regional-scale integrative, process-oriented science efforts as part of SEALS-sA (Sea Earth Atmosphere Linkages Study in southern Africa).We expect to describe experimental setups as well as showcase initial aerosol and cloud property distributions. Furthermore, we discuss the implementation of future activities in these programs in coordination with the UK Met Offices CLARIFY (CLoud-Aerosol-Radiation Interactions and Forcing) experiment in 2017.

aerosol↗

DOE OSTI2016

Fingerprints of a riming event on cloud radar Doppler spectra: observations and modeling

In this paper, Radar Doppler spectra measurements are exploited to study a riming event when precipitating ice from a seeder cloud sediment through a supercooled liquid water (SLW) layer. The focus is on the "golden sample" case study for this type of analysis based on observations collected during the deployment of the Atmospheric Radiation Measurement Program's (ARM) mobile facility AMF2 at Hyytiälä, Finland, during the Biogenic Aerosols – Effects on Clouds and Climate (BAECC) field campaign. The presented analysis of the height evolution of the radar Doppler spectra is a state-of-the-art retrieval with profiling cloud radars in SLW layers beyond the traditional use of spectral moments. Dynamical effects are considered by following the particle population evolution along slanted tracks that are caused by horizontal advection of the cloud under wind shear conditions. In the SLW layer, the identified liquid peak is used as an air motion tracer to correct the Doppler spectra for vertical air motion and the ice peak is used to study the radar profiles of rimed particles. A 1-D steady-state bin microphysical model is constrained using the SLW and air motion profiles and cloud top radar observations. The observed radar moment profiles of the rimed snow can be simulated reasonably well by the model, but not without making several assumptions about the ice particle concentration and the relative role of deposition and aggregation. In conclusion, this suggests that in situ observations of key ice properties are needed to complement the profiling radar observations before process-oriented studies can effectively evaluate ice microphysical parameterizations.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS1990

An analysis of lidar observations of polar stratospheric clouds

Lidar observations by Browell et al. (1990) are interpreted using single scattering calculations for nonspherical particles and aerosol microphysical calculations. Many of the lidar observations are consistent with particles containing 10 ppbv of condensed nitric acid vapor and an equivalent mass of water. The lidar observations of these Type 1 clouds identify two subtypes, whose properties are deduced. Type 1b particles are spherical, or nearly spherical, and typically have radii near 0.5 micron; Type 1a particles are not spherical, and have a spherical volume equivalent radius exceeding 1.0 micron. Several factors may cause variations in the size of the particles. The most significant factors are the cooling rate and the degree to which the air parcels cool below the condensation point. Specific examples in which cooling rate and cooling point may have led to variations in particle size are found in the Browell et al. (1990) data set. Condensation of 1 ppmm of water or less is quantitatively sufficient to account for the magnitude of the lidar backscatter observed from water ice clouds. The ice particles are not spherical in shape. The sizes of particles in water ice clouds cannot be determined because they are much larger than the wavelength of the lidar.

Toon, Owen B.↗

NASA NTRS2012

The View from the Top: CALIOP Ice Water Content in the Uppermost Layer of Tropical Cyclones

NASA's CALIPSO satellite carries both the Cloud and Aerosol Lidar with Orthogonal Polarization (CALIOP) and the Imaging Infrared Radiometer (IIR). The lidar is ideally suited to viewing the very top of tropical cyclones, and the IIR provides critical optical and microphysical information. The lidar and the IIR data work together to understand storm clouds since they are perfectly co-located, and big tropical cyclones provide an excellent complex target for comparing the observations. There is a lot of information from these case studies for understanding both the observations and the tropical cyclones, and we are just beginning to scratch the surface of what can be learned. Many tropical cyclone cloud particle measurements are focused on the middle and lower regions of storms, but characterization of cyclone interaction with the lowermost stratosphere at the upper storm boundary may be important for determining the total momentum and moisture transport budget, and perhaps for predicting storm intensity as well. A surprising amount of cloud ice is to be found at the very top of these big storms.

Avery, Melody A.↗

NASA NTRS1995

A Model Simulation of Pinatubo Volcanic Aerosols in the Stratosphere

A one-dimensional, time-dependent model is used to study the chemical, microphysical, and radiative properties of volcanic aerosols produced by the Mount Pinatubo eruption on June 15, 1991. Our model treats gas-phase sulfur photochemistry, gas-to-particle conversion of sulfur, and the microphysics of sulfate aerosols and ash particles under stratospheric conditions. The dilution and diffusion of the volcanic eruption clouds are also accounted for in these conditions. Heteromolecular homogeneous and heterogeneous binary H2SO4/H2O nucleation, acid and water condensational growth, coagulation, and gravitational sedimentation are treated in detail in the model. Simulations suggested that after several weeks, the volcanic cloud was composed mainly of sulfuric acid/water droplets produced in situ from the SO2 emissions. The large amounts of SO2 (around 20 Mt) injected into the stratosphere by the Pinatubo eruption initiated homogeneous nucleation which generated a high concentration of small H2SO4/H2O droplets. These newly formed particles grew rapidly by condensation and coagulation in the first few months and then reach their stabilized sizes with effective radii in a range between 0.3 and 0.5 micron approximately one-half year after the eruption. The predicted volcanic cloud parameters reasonably agree with measurements in term of the vertical distribution and lifetime of the volcanic aerosols, their basic microphysical structures (e.g., size distribution, concentration, mass ratio, and surface area) and radiative properties. The persistent volcanic aerosols can produce significant anomalies in the radiation field, which have important climatic consequences. The large enhancement in aerosol surface area can result in measurable global stratospheric ozone depletion.

Zhao , Jing-xia↗

DOE OSTI2023

TRACER-Uncrewed Aircraft System (TRACER-UAS) Field Campaign Report

Convective processes drive the development of clouds across a variety of scales, thereby playing a central role in governing weather and climate globally. These processes help to set the stage for circulations that redistribute heat and moisture throughout the lower atmosphere, and simultaneously develop storms that supply precipitation to regions that depend on such rain events for supporting a variety of societal needs. At the same time, extreme precipitation events can result in localized flooding of low-lying areas, posing hazards to transportation and regional inhabitants, and potentially damaging structures and infrastructure. As a result, there is an inherent need to better understand the drivers and modulators of clouds and precipitation and leverage such understanding to make projections of how these important systems may evolve with a changing climate. With nearly three billion of Earth’s human inhabitants living within 200 km of a shoreline, development of such understanding is particularly important in coastal regimes. Central drivers of convective cloud development and life cycle in coastal environments include synoptic forcing, local meso- and microscale circulation regimes, microphysical evolution, and aerosol properties. Atmospheric boundary layer (ABL) development and its evolution can help drive the formation and organization of convective clouds, which then impart their own controls through dynamic processes related to latent heating and cooling (including cold-pool formation and propagation), three-dimensional radiative effects, and background environmental conditions (Fan et al. 2016). Such clouds have been contributing to record precipitation events in southeast Texas in recent years, relative to the last several decades of data from regional precipitation gauges (Fagnant et al. 2020). The greater Houston urban area has experienced particularly large increases in the frequency of extreme rainfall events, with enhanced intensity of extreme events (stretching of distribution tails) having potentially significant implications for watershed floodplain planning and mapping in greater Houston and Harris County. While the most extreme precipitation events were associated with tropical cyclones (e.g., Tropical Storm Allison and Hurricane Harvey; Blood 2014, Kao et al. 2019), strong thunderstorms can also deliver large amounts of precipitation over the area over relatively short periods.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS2009

A Multiscale Modeling System: Developments, Applications, and Critical Issues

The foremost challenge in parameterizing convective clouds and cloud systems in large-scale models are the many coupled dynamical and physical processes that interact over a wide range of scales, from microphysical scales to the synoptic and planetary scales. This makes the comprehension and representation of convective clouds and cloud systems one of the most complex scientific problems in Earth science. During the past decade, the Global Energy and Water Cycle Experiment (GEWEX) Cloud System Study (GCSS) has pioneered the use of single-column models (SCMs) and cloud-resolving models (CRMs) for the evaluation of the cloud and radiation parameterizations in general circulation models (GCMs; e.g., GEWEX Cloud System Science Team 1993). These activities have uncovered many systematic biases in the radiation, cloud and convection parameterizations of GCMs and have led to the development of new schemes (e.g., Zhang 2002; Pincus et al, 2003; Zhang and Wu 2003; Wu et al. 2003; Liang and Wu 2005; Wu and Liang 2005, and others). Comparisons between SCMs and CRMs using the same large-scale forcing derived from field campaigns have demonstrated that CRMs are superior to SCMs in the prediction of temperature and moisture tendencies (e.g., Das et al. 1999; Randall et al 2003b; Xie et al. 2005).

Tao, Wei-Kuo↗

DOE OSTI2021

Supersaturation, buoyancy, and deep convection dynamics

Motivated by recent discussions concerning differences of convective dynamics in polluted and pristine environments, the so-called convective invigoration in particular, this paper provides an analysis of factors affecting convective updraft buoyancy, such as the in-cloud supersaturation, condensate and precipitation loading, and entrainment. We use the deep convective period from simulations of daytime convection development over land discussed in our previous publications. An entraining parcel framework is used in the theoretical analysis. We show that for the specific case considered here, finite (positive) supersaturation noticeably reduces pseudo-adiabatic parcel buoyancy and cumulative convective available potential energy (cCAPE) in the lower troposphere. This comes from keeping a small fraction of the water vapor in a supersaturated state and thus reducing the latent heating. Such a lower-tropospheric impact is comparable to the effects of condensate loading and entrainment in the idealized parcel framework. For the entire tropospheric depth, loading and entrainment have a much more significant impact on the total CAPE. For the cloud model results, we compare ensemble simulations applying either a bulk microphysics scheme with saturation adjustment or a more comprehensive double-moment scheme with supersaturation prediction. We compare deep convective updraft velocities, buoyancies, and supersaturations from all ensembles. In agreement with the parcel analysis, the saturation-adjustment scheme provides noticeably stronger updrafts in the lower troposphere. For the simulations predicting supersaturation, there are small differences between pristine and polluted conditions below the freezing level that are difficult to explain by standard analysis of the in-cloud buoyancy components. By applying the piggybacking technique, we show that the lower-tropospheric buoyancy differences between pristine and polluted simulations come from a combination of temperature (i.e., latent heating) and condensate loading differences that work together to make polluted buoyancies and updraft velocities slightly larger when compared to their pristine analogues. Overall, the effects are rather small and contradict previous claims of a significant invigoration of deep convection in polluted environments.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRSDate not supplied

Tropical Convection Through the Lens of the INCUS Mission

The overarching goal of the recently selected NASA INvestigation of Convective UpdraftS (INCUS) mission is to enhance our understanding of why, when and where tropical convective storms form, and why only some of these storms produce extreme weather. Convective storms provide an important pathway for the transport of air and water between Earth’s surface and the upper troposphere. This vertical transport of air and water, often referred to as convective mass flux (CMF), plays a critical role in Earth’s weather and climate system through its impacts on microphysical and precipitation rates, detrainment and upper tropospheric moistening, high cloud feedbacks, and the large-scale circulation. Potential changes to the CMF as a function of the local environment or with changing climates may also have significant implications for severe weather such as flood-producing rainfall, damaging hail and lightning. In spite of the critical role of this vertical transport of water and air, representation of CMF remains a major source of error in weather and climate models, thereby limiting our ability to accurately predict convective storms and their impacts. The tropics-wide observations from INCUS will enhance our understanding of tropical convective storm processes and will provide guidance for representing these processes in numerical models across scales. INCUS is comprised of three SmallSat platforms each carrying a RainCube-heritage Ka-band 7-beam scanning radar. The satellite platforms will be 30 and 90 seconds apart, thus providing three time intervals (30, 90 and 120 seconds) over which observations will be made. INCUS will investigate CMF using a novel time-differenced radar reflectivity profile approach. In addition to the Ka-band radar, a single TEMPEST-D-heritage cross-track-scanning passive microwave radiometer will be housed on the middle SmallSat. The radiometer will provide extensive storm context for the radar observations, as well as observations of the convective anvils. The combination of the radars and radiometer on INCUS will deliver unprecedented three-dimensional views of tropical convective storms. INCUS is the first systematic investigation of the rapidly evolving CMF within tropical convective storms, the observations of which are expected to significantly enhance both our understanding and prediction of storm structure, their dynamics and microphysical processes, and the ways in which these evolve over storm lifetimes. This presentation will highlight the observational capabilities and scientific approach of the INCUS mission.

Susan C. van den Heever↗

NASA NTRS2018

Aerosol-Radiation-Cloud Interactions in the South-East Atlantic: Results from the ORACLES-2016 Deployment and a First Look at ORACLES-2017 and Beyond

Seasonal biomass burning (BB) in Southern Africa during the Southern hemisphere spring produces almost a third of the Earth's BB aerosol particles. These particles are lofted into the mid-troposphere and transported westward over the South-East (SE) Atlantic, where they interact with one of the three semi-permanent subtropical stratocumulus (Sc) cloud decks in the world. These interactions include adjustments to aerosol-induced solar heating and microphysical effects. The representation of these interactions in climate models remains highly uncertain, because of the scarcity of observational constraints on both, the aerosol and cloud properties, and the governing physical processes. The first deployment of the NASA P-3 and ER-2 aircraft in the ORACLES (ObseRvations of Aerosols Above Clouds and Their IntEractionS) project in August/September of 2016 has started to fill this observational gap by providing an unprecedented look at the SE Atlantic cloud-aerosol system. We provide an overview of the first deployment, highlighting aerosol absorptive and cloud-nucleating properties, their vertical distribution relative to clouds, the locations and degree of aerosol mixing into clouds, cloud changes in response to such mixing, and cloud top stability relationships to the aerosol. We also expect to describe preliminary results of the second ORACLES deployment from Sao Tome and Principe in August 2017. We will make an initial assessment of the differences and similarities of the BB plume and cloud properties as observed from a deployment site near the plume's northern edge. We will conclude with an outlook for the third ORACLES deployment in October 2018.

Redemann, Jens↗

DOE OSTI2021

Remote Sensing of Electric Fields Observed Within Winter Precipitation During the 2020 Investigation of Microphysics and Precipitation for Atlantic Coast-Threatening Snowstorms (IMPACTS) Field Campaign

Aircraft electric fields from NASA's Lightning Instrument Package (LIP) were coupled with other airborne and ground-based, and in situ measurements to understand electrification in winter clouds that did not produce lightning. The measurements were made during seven research flights by a NASA ER-2 during the 2020 Investigation of Microphysics and Precipitation for Atlantic Coast-Threatening Snowstorms (IMPACTS) campaign. Observed total electric field magnitudes were as high as 80 V m -1 and variability in the electric field was observed along the flight path of the ER-2, indicating horizontal and/or vertical inhomogeneity in the cloud's electrical structure. X-band airborne radar data indicated 20-dBZ echo tops above 5 km in regions where electrification exceeded 10 V m -1 . In these regions, 85-GHz brightness temperatures (TB) from an airborne radiometer were lower than 265 K, with the lowest T B (~210 K) associated with ice scattering collocated with the strongest electric fields. In situ microphysical measurements from the NASA P-3 aircraft on February 7 indicated that regions near strong electric field contained supercooled water, rimed ice hydrometeors, ice water p- content as high as 1 g m -3 , liquid water content as high as 0.15 g m -3 , and supersaturation as high as 3.5%. Furthermore, these observations support the role of mixed phase microphysics in the generation of electric fields in clouds. In three case studies, ground based S-band polarimetric radar observed depolarization streaks in differential reflectivity near areas where the strongest electrification was observed. This observation reinforces the utility of depolarization streaks to identify areas of electrification prior to lightning occurrence.

54 ENVIRONMENTAL SCIENCES↗