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At least 163 records · Page 9

Four-dimensional emittance measurement at the Spallation Neutron Source

A coasting hadron beam with an elliptical transverse profile, uniform charge density, and small transverse four-dimensional (4D) emittance could improve accelerator performance in several contexts. A phase space painting method to generate such a distribution is being tested in the Spallation Neutron Source (SNS) accumulator ring. A critical component of these efforts is to measure the 4D emittance of the beam during accumulation. The 4D emittance can be reconstructed from measured beam profiles in two ways: in the multi-optics method, the optics between a reconstruction and measurement location are varied; in the fixed-optics method, multiple measurement locations are used without modifying the optics. The fixed-optics method is faster but can lead to large uncertainty in the reconstructed 4D emittance. In this paper, we implement a variant of the multi-optics method using the four available wire-scanners near the SNS target. We also modify the wire-scanner region to reduce the uncertainty of the fixed-optics method. We then demonstrate the usefulness of the fixed-optics method by reconstructing the 4D emittance evolution during accumulation in the SNS ring.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Dynamic systems modeling of the spallation neutron source cryogenic moderator system to optimize transient control and prepare for power upgrades

Through support of the US Department of Energy's Office of Basic Energy Sciences, Oak Ridge National Laboratory has begun applying machine learning methods to improve accelerator and target performance of the Spallation Neutron Source (SNS). These methods are being applied to the control optimization and power upgrade of the SNS Cryogenic Moderator System (CMS). A numerical model of the CMS has been developed to study these optimizations and system modifications using EcosimPro. This paper compares steady-state and transient numerical results with experimental data. Control optimization studies focused on dampening mass flow, temperature, and pressure fluctuations during sudden losses of accelerator beam power. This analysis was conducted by adjusting five proportional-integral-derivative controllers connected to four flow control valves and one heater. Future efforts include power uprate studies focused on increasing the CMS cooling capacity. The current accelerator power is 1.4 MW; the first target station is being upgraded to 2.0 MW as part of the Proton Power Upgrade effort. The CMS cooling capacity is sufficient for 2.0 MW operation.

47 OTHER INSTRUMENTATION↗

First Experiments: New Science Opportunities at the Spallation Neutron Source Second Target Station

Leadership in materials science underpins future technologies in energy, security, and other applications that drive this nation’s economy. Neutron scattering is among the crucial characterization techniques necessary to ensure a world-leading position in materials science for the United States. The Second Target Station (STS) at the Spallation Neutron Source (SNS) will provide transformative new capabilities for the study of a broad range of materials using neutron scattering and will support users in many fields of research—materials science, physics, chemistry, geology, biology, and engineering, among others—and from academia, government laboratories, and industry.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Improved limits on n → n ' transformation from the Spallation Neutron Source

Conversions between neutrons n and dark matter candidate sterile neutrons n' have been proposed as a mechanism for baryon number $\mathscr{B}$ violation. In the case that there is a small mass difference Δ⁢m between the n and the n' states, oscillations can be induced by compensating for Δ⁢m with a magnetic field. A search for such neutron oscillations was performed at the Spallation Neutron Source by looking for anomalous neutron transmission through a strongly absorbing cadmium wafer inside of a 6.6 T magnet. The approach described here saw no regenerated neutrons above background, which provides an improved limit for neutron–sterile neutron transformations for a range of Δ⁢m between 0.1 and 1000 neV.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Nanodiamond Foils for H- Stripping to Support the Spallation Neutron Source (SNS) and Related Applications

Thin diamond foils are needed in many particle accelerator experiments regarding nuclear and atomic physics, as well as in some interdisciplinary research. Particularly, nanodiamond texture is attractive for this purpose as it possesses a unique combination of diamond properties such as high thermal conductivity, mechanical strength and high radiation hardness; therefore, it is a potential material for energetic ion beam stripper foils. At the ORNL Spallation Neutron Source (SNS), the installed set of foils must be able to survive a nominal five-month operation period, without the need for unscheduled costly shutdowns and repairs. Thus, a single nanodiamond foil about the size of a postage stamp is critical to the entire operation of SNS and similar sources in U.S. laboratories and around the world. We are investigating nanocrystalline, polycrystalline and their admixture films fabricated using a hot filament chemical vapor deposition (HFCVD) system for H- stripping to support the SNS at Oak Ridge National Laboratory. Here we discuss optimization of process variables such as substrate temperature, process gas ratio of H2/Ar/CH4, substrate to filament distance, filament temperature, carburization conditions, and filament geometry to achieve high purity diamond foils on patterned silicon substrates with manageable intrinsic and thermal stresses so that they can be released as free standing foils without curling. An in situ laser reflectance interferometry tool (LRI) is used for monitoring the growth characteristics of the diamond thin film materials. The optimization process has yielded free standing foils with no pinholes. The sp3/sp2 bonds are controlled to optimize electrical resistivity to reduce the possibility of surface charging of the foils. The integrated LRI and HFCVD process provides real time information on the growth of films and can quickly illustrate growth features and control over film thickness. The results are discussed in the light of development of nanodiamond foils that will be able to withstand a few MW proton beam and hopefully will be able to be used after possible future upgrades to the SNS to greater than a 3MW beam.

Vispute, R D↗

Development of nanodiamond foils for H- stripping to Support the Spallation Neutron Source (SNS) using hot filament chemical vapor deposition

Thin diamond foils are needed in many particle accelerator experiments regarding nuclear and atomic physics, as well as in some interdisciplinary research. Particularly, nanodiamond texture is attractive for this purpose as it possesses a unique combination of diamond properties such as high thermal conductivity, mechanical strength and high radiation hardness; therefore, it is a potential material for energetic ion beam stripper foils. At the ORNL Spallation Neutron Source (SNS), the installed set of foils must be able to survive a nominal five-month operation period, without the need for unscheduled costly shutdowns and repairs. Thus, a small foil about the size of a postage stamp is critical to the operation of SNS and similar sources in U.S. laboratories and around the world. We are investigating nanocrystalline, polycrystalline and their admixture films fabricated using a hot filament chemical vapor deposition (HFCVD) system for H- stripping to support the SNS at Oak Ridge National Laboratory. Here we discuss optimization of process variables such as substrate temperature, process gas ratio of H2/Ar/CH4, substrate to filament distance, filament temperature, carburization conditions, and filament geometry to achieve high purity diamond foils on patterned silicon substrates with manageable intrinsic and thermal stresses so that they can be released as free standing foils without curling. An in situ laser reflectance interferometry tool (LRI) is used for monitoring the growth characteristics of the diamond thin film materials. The optimization process has yielded free standing foils with no pinholes. The sp3/sp2 bonds are controlled to optimize electrical resistivity to reduce the possibility of surface charging of the foils. The integrated LRI and HFCVD process provides real time information on the growth of films and can quickly illustrate growth features and control film thickness. The results are discussed in the light of development of nanodiamond foils that will be able to withstand a few MW proton beam and hopefully will be able to be used after possible future upgrades to the SNS to greater than a 3MW beam.

Vispute, R D↗

Early-Stage Radiation Safety Analysis for the Spallation Neutron Source Second Target Station Bunker Operations

The Second Target Station project at Oak Ridge National Laboratory will develop a cold neutron source to meet growing experimental needs. This paper describes calculations of the residual dose rates associated with the monolith shield plug and the beamline bunker, two key conventional operations and radiation safety features. While neutron production is active, the instrument hall outside the bunker must be generally accessible with dose rates of less than 0.25 mrem/h. When neutron production is halted, the bunker must be accessible for hands-on maintenance operations. Further, these two requirements form the cause for the assessments reported herein of residual dose rates caused by the monolith shield plug and residual dose rates in the bunker. The monolith shield plug was shown to not produce significant dose rates inside the bunker after a 20-year lifetime, and the residual dose rates inside the bunker for the case of an operating beamline were shown to reasonably allow for hands-on maintenance. These calculations are based on preliminary design models of the relevant systems. Additionally, an example showing the significance of considering neutron supermirror physics in transport calculations that track nuclide production and destruction rates to produce gamma sources for residual dose rate calculations is included. The example shows that if neutron supermirror physics is not considered, dose rate fields may be significantly underpredicted.

61 RADIATION PROTECTION AND DOSIMETRY↗

Characterization of Crystallographic Structures Using Bragg-Edge Neutron Imaging at the Spallation Neutron Source

Over the past decade, wavelength-dependent neutron radiography, also known as Bragg-edge imaging, has been employed as a non-destructive bulk characterization method due to its sensitivity to coherent elastic neutron scattering that is associated with crystalline structures. Several analysis approaches have been developed to quantitatively determine crystalline orientation, lattice strain, and phase distribution. In this study, we report a systematic investigation of the crystal structures of metallic materials (such as selected textureless powder samples and additively manufactured (AM) Inconel 718 samples), using Bragg-edge imaging at the Oak Ridge National Laboratory (ORNL) Spallation Neutron Source (SNS). Firstly, we have implemented a phenomenological Gaussian-based fitting in a Python-based computer called iBeatles. Secondly, we have developed a model-based approach to analyze Bragg-edge transmission spectra, which allows quantitative determination of the crystallographic attributes. Moreover, neutron diffraction measurements were carried out to validate the Bragg-edge analytical methods. These results demonstrate that the microstructural complexity (in this case, texture) plays a key role in determining the crystallographic parameters (lattice constant or interplanar spacing), which implies that the Bragg-edge image analysis methods must be carefully selected based on the material structures.

47 OTHER INSTRUMENTATION↗

Comparison of Measured and Calculated Dose Rates for Ring Injection Dump Exchange at Spallation Neutron Source

According to the accelerator operation plan, the beam-stop and the proton beam window (PBW) assemblies of the existing Ring Injection Dump RID are replaced with fresh assemblies, when they have reached their end-of-life. End of-life is determinate by the stainless-steel beam-stop window having accumulated 10 dpa radiation damage. The exchange process took place during facility maintenance period that started in March 2023. Each of the spent assembles were put into specially designed storage containers temporarily residing near the RID building.The spent beam-stop is predicted to be the part of highest activation that has been removed in Spallation Neutron Source (SNS). The exchange processes require good work planning to minimize radiation exposure to personal. For each exchange step the residual dose rate distribution is calculated and the peak values are identified. This paper gives some examples of calculated vs measured doses during beam-stop assembly exchange.

Popova, Irina I.↗

Spallation Neutron Source Second Target Station Construction Project: Biological Assessment

The Endangered Species Act of 1973 (16 U.S.C. 153 et seq.), as amended (ESA or Act) in section 7(a)(1) directs Federal agencies to conserve and recover listed species and use their authorities in the furtherance of the purposes of the Act by carrying out programs for the conservation of endangered and threatened species so that listing is no longer necessary (50 CFR §402). Furthermore, the Act in section 7(a)(2) directs Federal agencies to consult (referred to as section 7 consultation) with the U.S. Fish and Wildlife Service (USFWS) when their activities “may affect” a listed species or designated critical habitat. This biological assessment (BA) analyzes the potential effects of the proposed Spallation Neutron Source Second Target Station STS construction project on the U. S. Department of Energy Oak Ridge Reservation (ORR) on Federal listed threatened, endangered, proposed, and under consideration for Federal listing bat species, pursuant to section 7(a)(2) of the ESA.

54 ENVIRONMENTAL SCIENCES↗

Analysis of the time-of-flight neutron scattering cross-section data for light water measured at the SEQUOIA spectrometer, Spallation Neutron Source (SNS)

Thermal neutron scattering cross-section data for light water available in the major nuclear data libraries observes significant differences especially at reactor operating temperatures. During the past few years there has been a renewed interest in reviewing the existing thermal scattering models and generating more accurate and reliable thermal scattering cross sections using existing experimental data and in some cases based on Molecular Dynamics (MD) simulations. There is a need for performing new time-of-flight experiments at high temperatures and pressures, to have a better understanding of the physics involved in the scattering process that could help improve the existing TSL data.Lack of experimental thermal scattering data for light water at high temperatures led to a new measurement campaign within the INSIDER project at the Institut de radioprotection et de sûreté nucléaire (IRSN). Double differential scattering cross section for light water have been measured at the SEQUOIA spectrometer based at the Spallation Neutron Source (SNS), Oak Ridge National Laboratory, United States. Several measurements have been carried out at different temperatures and pressures corresponding to liquid light water. Measurements at five different incident neutron energies Ei (8, 60, 160, 280 and 800 meV) have been carried out to help exploring different regions of the frequency spectrum. This paper presents the analysis of the dynamic structure factor and the derived frequency spectrum of light water. The analysis of the experimental data would provide one with better confidence, the behavior of thermal scattering cross sections for light water at high temperatures, knowledge of which is very important for the design of novel reactors as well as existing pressurized water reactors.

Jaiswal, V↗

Recent progress in plasma modelling at INFN-LNS

At Istituto Nazionale di Fisica Nucleare - Laboratori Nazionali del Sud (INFN-LNS), the development of intense ion and proton sources has been supported by a great deal of work on the modelling of microwave generated plasmas for many years. First, a stationary version of the particle-in-cell code was developed for plasma modelling starting from an iterative strategy adopted for the space charge dominated beam transport simulations. Electromagnetic properties of the plasma and full-waves simulations are now affordable for non-homogenous and non-isotropic magnetized plasma via “cold” approximation. The effects of Coulomb collisions on plasma particles dynamics was implemented with the Langevin formalism, instead of simply applying the Spitzer 90° collisions through a Monte Carlo technique. A wide database of different cross sections related to reactions occurring in a hydrogen plasma was implemented. The next step consists of merging such a variety of approaches for retrieving an “as-a-whole” picture of plasma dynamics in ion sources. The preliminary results will be summarized in the paper for a microwave discharge ion source designed for intense and high quality proton beams production, proton source for European Spallation Source project. Even if the realization of a predictive software including the complete processes involved in plasma formation is still rather far, a better comprehension of the source behavior is possible and so the simulations may support the optimization phase.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Plasma emission spectroscopy for operating and developing the Spallation Neutron Source (SNS) H{sup −} ion sources

A RF-driven, Cs-enhanced H{sup −} ion source feeds the SNS accelerator with a high current (typically >50 mA), ∼1.0 ms pulsed beam at 60 Hz. To achieve the persistent high current beam for several weeks long service cycles, each newly installed ion source undergoes a rigorous conditioning and cesiation processes. Plasma conditioning outgases the system and sputter-cleans the ion conversion surfaces. A cesiation process immediately following the plasma conditioning releases Cs to provide coverage on the ion conversion surfaces. The effectiveness of the ion source conditioning and cesiation is monitored with plasma emission spectroscopy using a high-sensitivity optical spectrometer. Plasma emission spectroscopy is also used to provide a means for diagnosing and confirming a failure of the insulating coating of the ion source RF antenna which is immersed in the plasma. Emissions of composition elements of the antenna coating material, Na emission being the most significant, drastically elevate to signal a failure when it happens. Plasma spectra of the developmental ion source with an AlN (aluminum nitrite) chamber and an external RF antenna are also briefly discussed.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Preliminary waste management plan of European spallation

The European Spallation Source (ESS) is the European common effort in designing and building a next generation large-scale user facility for studies of the structure and dynamics of materials. The proposed schematic layout of the ESS facility is based on a linear driver (linac) directing the proton beam (5 MW of 2.5 GeV) of 2.8 ms long pulses with a 20 Hz on a tungsten target where neutrons are produced via spallation reactions. Further the neutrons will be moderated to thermal and sub-thermal energies in a couple of moderators placed around the target. The moderators feed 22 beamlines guiding the neutrons to the scattering instruments, mainly for neutron scattering research, as has been previously mentioned. The objective of this work is to develop a waste management plan for ESS facility. In this respect two important aspects are analyzed. First the present status of the problem is outlined as follow. Estimate types and quantities of waste that the ESS project will generate at different stages: commission, operation, decommissioning were derived using: i) precise Monte Carlo calculations ii) scaling the activity from the operation experience of the existing spallation source installations for waste such it is difficult to predict level of activation or for components of the facility in stage of the preconceptual model. Associated waste treatment/conditioning options and final disposal route were further analyzed in order to define the waste type and packet descriptions in agreement with Swedish regulations and policy. It was found that the compilation of completely new waste type descriptions for qualification of the ESS waste for disposal will be necessary. Particular attention was devoted to 'problematic waste' as Beryllium reflector, C-14 from graphite used as core zone of the beam-dump and collimators or waste arising from the purification systems of both Helium and water cooling circuits. Management of waste on ESS site: collection/segregation systems, characterization system, storage options, is also described. In the second step, the acquired information is used for planning and implementing actions involving all participants (ESS, treatment facility operator, disposal operator, regulatory body and other authorized authorities). (authors)

07 ISOTOPE AND RADIATION SOURCES↗

M-STAR: Magnetism second target advanced reflectometer at the Spallation Neutron Source

M-STAR is a next generation polarized neutron reflectometer with advanced capabilities. A new focusing guide concept is optimized for samples with dimensions down to a millimeter range. A proposed hybrid pulse-skipping chopper will enable experiments at constant geometry at one incident angle in a broad range of wavevector transfer Q up to 0.3 A –1 for specular, off-specular, and GISANS measurements. M-STAR will empower nanoscience and spintronics studies routinely on small samples (~2 × 2 mm 2 ) and of atomic-scale thickness using versatile experimental conditions of magnetic and/or electric fields, light, and temperature applied in situ to novel complex device-like nanosystems with multiple buried interfaces. M-STAR will enable improved grazing incidence diffraction measurements, as a surface-sensitive depth-resolved probe of, e.g., the out-of-plane component of atomic magnetic moments in ferromagnetic, antiferromagnetic, and more complex structures as well as in-plane atomic-scale structures inaccessible with contemporary diffractometry and reflectometry. New horizons will be opened by the development of an option to probe near-surface dynamics with inelastic grazing incidence scattering in the time-of-flight mode. These novel options in combination with ideally matched parameters of the second target station will place M-STAR in the world’s leading position for high resolution polarized reflectometry.

47 OTHER INSTRUMENTATION↗