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At least 163 records · Page 9

CACTI ARM Aerial Facility Measurements of Ice Nucleating Particles

The dataset comprises measures, using Colorado State University's Ice Spectrometer (IS, an immersion freezing device with a range from 0°C down to -26 to -29°C) of atmospheric ice nucleating particle (INP) concentrations taken on the Atmospheric Radiation Measurement (ARM) program Aerial Facilty (AAF) G-1 aircraft. INP measurements on the G-1 were collected from varied altitudes on different flights over the region of the Sierras de Córdoba mountain range of north-central Argentina, centred over ARM's Mobile Facility (AMF-1) near Villa Yacanto, where ground-based INP measures were being taken concurrently. Both studies took place as part of the Cloud, Aerosol, and Complex Terrain Interactions (CACTI) Experiment. A filter sampling system was deployed on the G-1 to collect aerosol particles for post-processing of INPs collected on filters (measuring their immersion freezing ability) once returned to Colorado State University (CSU). Filter holders used were pre-cleaned aluminum in-line units loaded with pre-cleaned and pre-sterilized 47 mm dia. Nuclepore polycarbonate filters (0.2 mm pore size). Filters were drawn for varied times, resulting in varied volumes collected (51 to 1667 SL). Mass flow rate was recorded in real-time so that total sampled volume (at standard temperature and pressure) could be determined. A total of 34 sample filters were collected over the IOP, including 5 blanks. Filters were stored at -20°C freezer prior to frozen return to Colorado State University (CSU). . Processing to obtain spectra of INP number concentration active via the immersion freezing mechanism versus temperature was conducted using CSU's IS instrument (McCluskey et al., 2018). For measurment of INPs, collected aerosol particles were re-suspended in 7 mL of 0.02 µm-filtered deionized water. Aliquots of each suspension, and serial dilutions, were dispensed into trays which were fit into aluminum blocks in the IS. Samples are cooled at 0.33°C min-1 and the freezing temperatures of wells recorded automatically. Cumulative INP concentrations were determined by first calculating the INPs per mL of suspension based on Vali (1971) and then converting to concentration per standard liter of air using the proportion of the total liquid sample dispensed and the air sample volumes. Aliquots of suspensions from selected samples were also heat treated (95°C for 20 min) to denature and deactivate biological INPs, and digested in 10% H2O2 at 95°C under UV-B to remove all organic carbon INPs. McCluskey, C. S., J. Ovadnevaite, M. Rinaldi, J. Atkinson, F. Belosi, D. Ceburnis, S. Marullo, T. C. J. Hill, U. Lohmann, Z. A. Kanji, C. O’Dowd, S. M. Kreidenweis, P. J. DeMott, 2018: Marine and Terrestrial Organic Ice Nucleating Particles in Pristine Marine to Continentally-Influenced Northeast Atlantic Air Masses, Journal of Geophysical Research: Atmospheres, 123, 6196–6212, https://doi.org/10.1029/2017JD028033. Vali, G., 1971: Quantitative evaluation of experimental results on the heterogeneous freezing nucleation of supercooled liquids. J. Atmos. Sci., 28, 402–409.

54 ENVIRONMENTAL SCIENCES↗

MARCUS Ice Nucleating Particle Measurements (revised 7/2020)

These data list ice nucleating particle (INP) number concentrations active in the immersion freezing mode. Aerosol filters were collected during 4 voyages of the Aurora Australis vessel from 02 November 2017 to 22 March 2018, as part of the Measurements of Aerosols, Radiation and Clouds over the Southern Ocean (MARCUS) study. These voyages transected the Southern Ocean from Hobart, Tasmania to four Australian Antarctic Division stations, including three in Antarctica. Collections were made over alternating periods of 24 and 48 hours using open-faced polycarbonate filters that were approximately 18 m MSL, sited near the AOS trailer and other AMF measurements. The volume of air filtered ranged from 19000 to 38000 standard liters per filter sample. Filters were stored and returned frozen to Colorado State University (CSU), where immersion freezing measurements over a range from 0 to -28 degC were made using the CSU Ice Spectrometer (IS). Collected particles from each filter were resuspended in filtered, deionized water, and then dispensed into the IS and cooled to obtain cumulative INP temperature spectra. Aliquots of suspensions from selected samples were also heat treated (95 degC for 20 min) to denature and deactivate biological INPs, and digested in 10% H2O2 at 95 degC under UV-B for 20 min to remove all organic carbon INPs, prior to measurement using the IS.

54 ENVIRONMENTAL SCIENCES↗

AEROICESTUDY-Colorado State University Ice Spectrometer

The dataset comprises measures, using Colorado State University's Ice Spectrometer (IS, an immersion freezing device with a range from 0 °C down to -26 to -29 °C) of atmospheric ice nucleating particle (INP) concentrations taken at ARM's Southern Great Plains (SGP) Site Guest Instrument Facility (GIF), in Lamont, Oklahoma, during the Aerosol-Ice Formation Closure Pilot Study (AEROICESTUDY). A filter sampler was mounted approximately 6 m above ground level atop the GIF rooftop platform. Single-use filter units open to the atmosphere fitted with pre-cleaned and pre-sterilized, 47-mm diameter Nuclepore polycarbonate filters were used. Filters were typically drawn for either a full day period (9AM-5PM CDT) or broken up into morning (9AM-12PM CDT) and afternoon (1PM-5PM CDT) periods. Additionally, 4 overnight filters were taken (6PM-8AM CDT). The volume of air filtered was typically between 3000 and 8000 standard liters for daily samples. After collection, filters were stored at -20 °C until processed. Initial processing to obtain spectra of INP number concentration active via the immersion freezing mechanism versus temperature was conducted using CSU's IS instrument (McCluskey et al., 2018). For measurement of INPs, collected aerosol particles were re-suspended in 8 mL of 0.1 µm-filtered deionized (DI) water. Aliquots of each suspension, and serial dilutions, were dispensed into trays which were fit into aluminum blocks in the IS. Samples were cooled at 0.33 °C per min and the freezing temperatures of wells recorded automatically. Cumulative INP concentrations were determined by first calculating the INPs per mL of suspension based on Vali (1971) and then converting to concentration per standard liter of air using the proportion of the total liquid sample dispensed and the air sample volumes. Two-tailed, 95% confidence intervals for binomial sampling were based on Equation 2 from Agresti and Coull (1998). Aliquots of suspensions from selected samples were also heat treated (95 °C for 20 min) to denature and deactiv

54 ENVIRONMENTAL SCIENCES↗

MOSAiC-Colorado State University Ice Spectrometer

This data set contains atmospheric ice nucleating particle (INP) measurements, using Colorado State University&rsquo;s (CSU) Ice Spectrometer (IS), of filter collections taken at the U.S. DOE ARM AMF2 site onboard the R/V Polarstern P-deck during the Multidisciplinary Drifting Observatory for the Study of Arctic Climate (MOSAiC) field campaign. Samples were collected from October 27, 2019 to September 24, 2020. A filter sampler was mounted approximately 15 m above ground level on a railing in proximity to (and approximately 3 m below) the Aerosol Observation System (AOS) inlet. Single-use filter units open to the atmosphere were pre-cleaned and pre-loaded with 47-mm diameter Nuclepore polycarbonate (0.2 &micro;m pore-diameter) filters. Filters were typically drawn for a three-day period, with an average volume of air filtered of 87,000 standard liters. Total volumes were calculated through recorded daily flow rates using a mass flow meter (TSI). After collection, filters were stored and transported frozen until analysis using CSU&rsquo;s IS instrument (McCluskey et al., 2018). Aerosol particles were first re-suspended in 8 mL of 0.1 &micro;m-filtered deionized (DI) water. Aliquots of each suspension, and corresponding 11-fold dilutions, were dispensed into polymerase chain reaction (PCR) trays and placed into the aluminum blocks of the IS. Samples were cooled at approximately 0.33 &deg;C min -1 and freezing detected optically with corresponding temperatures recorded. Cumulative INP concentrations were determined through calculating the number of INPs per mL of suspension (Vali, 1971) and converting to concentration per standard L of air by accounting for the proportion of liquid used and volume of air collected. All samples were corrected for the number of INPs on the average of four field blanks (cleaned, handled, transported, and analyzed in the same way without air flow). Two-tailed, 95% confidence intervals for binomial sampling are provided (Agresti and Coull, 1998). Select samples were also heat treated (95 &deg;C for 20 min) to denature and deactivate biological INPs present and digested in 10% H 2 O 2 at 95 &deg;C under UV-B for 20 min to remove any organic carbon INPs. Agresti, A, and BA Coull. 1998. "Approximate is better than &ldquo;exact&rdquo; for interval estimation of binomial proportions." American Statistics 52: 119&ndash;126. https://doi.org/10.2307/2685469 McCluskey, CS, J Ovadnevaite, M Rinaldi, J Atkinson, F Belosi, D Ceburnis, &hellip; and PJ DeMott. 2018. "Marine and Terrestrial Organic Ice-Nucleating Particles in Pristine Marine to Continentally Influenced Northeast Atlantic Air Masses." Journal of Geophysical Research: Atmospheres 123 (11): 6196&ndash;6212, https://doi.org/10.1029/2017JD028033 Vali, G. 1971. "Quantitative Evaluation of Experimental Results and the Heterogeneous Freezing Nucleation of Supercooled Liquids." Journal of the Atmospheric Sciences 28: 402-209. https://doi.org/10.1175/1520-0469(1971)028<0402:QEOERA>2.0.CO;2

54 ENVIRONMENTAL SCIENCES↗

ExINP-ENA Ice-Nucleating Particle Concentrations - CRAFT

This data set comprises cumulative ambient ice-nucleating particle (INP) concentrations measured at the U.S. Department of Energy's Atmospheric Radiation Measurement (ARM) Eastern North Atlantic (ENA) observatory on Graciosa Island, Azores (39.0916&deg; N, 28.0257&deg; W). Our INP data were generated using a combination of online instruments, the Portable Ice Nucleation Experiment chamber (PINE), and an offline assay instrument, the West Texas Cryogenic Refrigerator Applied to Freezing Test system (WT-CRAFT), for aerosol particle samples collected on polycarbonate filters (with 0.2-micron diameter pores).

47-mm Nuclepore filter sampler, West Texas Cryogen↗

ExINP-ENA Ice-Nucleating Particle Concentrations - PINE

This data set comprises cumulative ambient ice-nucleating particle (INP) concentrations measured at the U.S. Department of Energy's Atmospheric Radiation Measurement (ARM) Eastern North Atlantic (ENA) observatory on Graciosa Island, Azores (39.0916&deg; N, 28.0257&deg; W). Our INP data were generated using a combination of online instruments, the Portable Ice Nucleation Experiment chamber (PINE), and an offline assay instrument, the West Texas Cryogenic Refrigerator Applied to Freezing Test system (WT-CRAFT), for aerosol particle samples collected on polycarbonate filters (with 0.2-micron diameter pores).

54 ENVIRONMENTAL SCIENCES↗

ExINP NSA Ice Nucleating Particle Concentrations

This data set comprises cumulative ambient ice-nucleating particle (INP) concentrations measured at the National Oceanic and Atmospheric Administration's (NOAA’s) Barrow Atmospheric Baseline Observatory (71.3230° N, 156.6114° W, “BRW” hereafter), next to the Atmospheric Radiation Measurement (ARM) North Slope of Alaska (NSA) site and ~ 6 km northeast of the town of Utqiaġvik. Our INP abundance data were generated using a combination of online instrument, the Portable Ice Nucleation Experiment chamber ver. 3 (PINE-03), and an offline cold stage, the West Texas Cryogenic Refrigerator Applied to Freezing Test system (WT-CRAFT). Our online INP data are all from the Examining the Ice-Nucleating Particles from NSA (ExINP-NSA) campaign conducted from October 19, 2021 to May 24, 2024. The offline INP concentration analysis was performed at West Texas A&M University for aerosol particle samples collected on polycarbonate filters (with 0.2-micron diameter pores). The PINE-03 measurements, as well as sampling activities for offline INP measurements, were conducted using the BRW site. An inset laminar sampling stack was mounted to the instrument platform, allowing PINE-03 to intake particle-laden air. For most of the campaign period, the semi-autonomous PINE-03 chamber was remotely controlled from West Texas A&M University using the LabView interface through the BeyondTrust remote-access console. PINE-03 was set to conduct an immersion freezing expansion experiment (i.e., simulated adiabatic cooling along with RHw at or above 100%). Except during the scheduled maintenance periods, the time resolution of each expansion experiment was approximately 12 minutes. PINE-03 continuously measured INP concentrations during the entire campaign without any substantial breaks. For most of the campaign period, PINE scanned its set-point vessel air temperatures from -14 °C to -31 °C and back to -14 °C about every 120 minutes.

54 ENVIRONMENTAL SCIENCES↗

ExINP NSA Ice Nucleating Particle Concentrations

This data set comprises cumulative ambient ice-nucleating particle (INP) concentrations measured at the National Oceanic and Atmospheric Administration's (NOAA’s) Barrow Atmospheric Baseline Observatory (71.3230° N, 156.6114° W, “BRW” hereafter), next to the Atmospheric Radiation Measurement (ARM) North Slope of Alaska (NSA) site and ~ 6 km northeast of the town of Utqiaġvik. Our INP abundance data were generated using a combination of online instrument, the Portable Ice Nucleation Experiment chamber ver. 3 (PINE-03), and an offline cold stage, the West Texas Cryogenic Refrigerator Applied to Freezing Test system (WT-CRAFT). Our online INP data are all from the Examining the Ice-Nucleating Particles from NSA (ExINP-NSA) campaign conducted from October 19, 2021 to May 24, 2024. The offline INP concentration analysis was performed at West Texas A&M University for aerosol particle samples collected on polycarbonate filters (with 0.2-micron diameter pores). The PINE-03 measurements, as well as sampling activities for offline INP measurements, were conducted using the BRW site. An inset laminar sampling stack was mounted to the instrument platform, allowing PINE-03 to intake particle-laden air. For most of the campaign period, the semi-autonomous PINE-03 chamber was remotely controlled from West Texas A&M University using the LabView interface through the BeyondTrust remote-access console. PINE-03 was set to conduct an immersion freezing expansion experiment (i.e., simulated adiabatic cooling along with RHw at or above 100%). Except during the scheduled maintenance periods, the time resolution of each expansion experiment was approximately 12 minutes. PINE-03 continuously measured INP concentrations during the entire campaign without any substantial breaks. For most of the campaign period, PINE scanned its set-point vessel air temperatures from -14 °C to -31 °C and back to -14 °C about every 120 minutes.

54 ENVIRONMENTAL SCIENCES↗

Hydraulic Conductivity Measurements, Utqiagvik (Barrow), Alaska, 2014

Six individual ice cores were collected from the Barrow Environmental Observatory in Barrow, Alaska, in May of 2013 as part of the Next Generation Ecosystem Experiment (NGEE). Each core was drilled at a different location to varying depths. After drilling, the cores were stored in coolers packed with dry ice and flown to Lawrence Berkeley National Laboratory (LBNL) in Berkeley, CA. 3-dimensional images of the cores were constructed using medical X-ray computed tomography (CT) scanner at 120kV. Hydraulic conductivity samples were extracted from these cores at LBNL Richmond Field Station in Richmond, CA, in February 2014 by cutting 5 to 8 inch segments using a chop saw. Samples were packed individually and stored at -20C freezing temperatures to minimize any changes in structure or loss of ice content prior to analysis. Hydraulic conductivity was determined through falling head tests using a permeameter [ELE International, Model #: K-770B] (Appendix A). Samples were placed in a latex membrane via a membrane stretcher while frozen. Use of a membrane stretcher made the membranes easier to secure and minimized contact with the sample. A clear polycarbonate sleeve, fabricated with a stainless steel ring at the bottom to keep the sleeve from floating, was placed around the sample inside the permeameter to minimize deformation during analysis. The permeameter was filled with water and 1.0 PSI of air was applied for confining pressure during sample defrost. Outflow valves were left open to allow for incremental thawing and samples were left to thaw for approximately 12 hours. After approximately 12 hours of thaw, initial falling head tests were performed. When the flow was significantly too fast or too slow, the analysis was stopped and the burette size was adjusted accordingly (i.e. a larger diameter burette was used for flows that were faster than desired or a smaller diameter burette was used for flows that were slower than desired). Two to four measurements were collected on each sample and collection stopped when the applied head load exceeded 25% change from the original load. Analyses were performed between 2 to 3 times for each sample. The final hydraulic conductivity calculations were computed using methodology of Das et al., 1985.The Next-Generation Ecosystem Experiments: Arctic (NGEE Arctic), was a 15-year research effort (2012-2027) to reduce uncertainty in Earth System Models by developing a predictive understanding of carbon-rich Arctic ecosystems and feedbacks to climate. NGEE Arctic was supported by the Department of Energy's Office of Biological and Environmental Research. The NGEE Arctic project had two field research sites: 1) located within the Arctic polygonal tundra coastal region on the Barrow Environmental Observatory (BEO) and the North Slope near Utqiagvik (Barrow), Alaska and 2) multiple areas on the discontinuous permafrost region of the Seward Peninsula north of Nome, Alaska. Through observations, experiments, and synthesis with existing datasets, NGEE Arctic provided an enhanced knowledge base for multi-scale modeling and contributed to improved process representation at global pan-Arctic scales within the Department of Energy's Earth system Model (the Energy Exascale Earth System Model, or E3SM), and specifically within the E3SM Land Model component (ELM).

54 ENVIRONMENTAL SCIENCES↗

One-piece transparent shell improves design of helmet assembly

One-piece transparent helmet shell made of polycarbonate is equipped with a helmet protection pad, a visor assembly, a communications skull cap, and an emergency oxygen supply. This design offers improvements over previous designs in weight, visual field, comfort and protection.

Jones, R. L.↗

Material Properties Measurements for Selected Materials

Hugoniot equation of state measurements were made on Coconino sandstone, Vacaville basalt, Kaibab limestone, Mono Crater, pumice and Zelux (a polycarbonate resin) for pressures to 2 Mb. A single data point was obtained for fused quartz at 1.6 Mb. In addition to the hugoniot studies, the uniaxial compressive stress behavior of Vacaville basalt and Zelux was investigated at strain rates from about 10(exp -5)/sec to 10(exp 3)/second. The data presented include the stress - strain relations as a function of strain rate for these two materials.

Green, S. J.↗

High Z particle Apollo astronaut dosimetry with plastics

On Apollo missions, the individual astronauts' high Z particle exposure is measured by means of Lexan polycarbonate plastic. These layers form one component of the passive dosimetry packets worn in the constant wear garment. They serve as threshold type, high Z, charged particle track detectors, recording only the very highly ionizing particles. The detectors yield information on the particles' charge, energy, and direction of travel. This data, in turn, is used to obtain the track fluence, the stopping particle density as an integral Z distribution, and the particles' integral LET spectrum. Some of the data gathered on Apollo missions 8-13 is presented.

Benton, E. V.↗

Cosmic ray experiment. Part A: Composition and energy spectra of solar cosmic ray nuclei

The GE experiment consisted of two types of detectors: plastics and glasses located in panel 2 and the lower half of panel 3. In panel 2, the entire exposed detector area of 14.7 by 22.6 cm was composed of 31 sheets of 0.025-cm polycarbonate plastic 9070-112. In panel 3, 39 sheets of 0.02-cm cellulose triacetate with no plasticizer made up the major volume fraction. The lower part of panel 3 contained five types of glass detectors. Particles that entered the array after it was folded were recognized, if they crossed from one sheet to another, by means of a 2-mm relative shift of alternate sheets.

Fleischer, R. L.↗