Engineering Papers⌕ Search

SEARCH · Engineering Papers

Results for “pi: mass”

Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

Quote a phrase for an exact phrase match. Source license links do not imply unrestricted reuse.

At least 163 records · Page 9
All sourcesNASA NTRSDOE OSTI
NASA NTRS1975

Mass transfer in binary X-ray systems

The influence of X-ray heating on gas flows in binary X-ray systems is examined. A simple estimate is obtained for the evaporative wind flux from a stellar atmosphere due to X-ray heating which agrees with numerical calculations by Alme and Wilson (1974) but disagrees with calculations by Arons (1973) and by Basko and Sunyaev (1974) for the Her X-1/HZ Her system. The wind flux is sensitive to the soft X-ray spectrum. The self-excited wind mechanism does not work. Mass transfer in the Hercules system probably occurs by flow of the atmosphere of HZ Her through the gravitational saddle point of the system. The accretion gas stream is probably opaque with atomic density of not less than 10 to the 15th power per cu cm and is confined to a small fraction of 4(pi) steradians. Other binary X-ray systems are briefly discussed.

Mccray, R.↗
DOE OSTI2022

Search for Higgs Portal Scalars and Heavy Neutral Leptons Decaying in the MicroBooNE Detector

This thesis presents a search for Higgs Portal Scalars (HPS) and Heavy Neutral Leptons (HNL) decaying in the MicroBooNE liquid argon time projection chamber (LArTPC). The measurement was performed using data collected in-time with the Neutrino at the Main Injector (NuMI) beam with a total exposure corresponding to $7.01 \times 10^{20}$ protons on target. Mono-energetic HPS and HNL would be produced from kaons decaying at rest in the NuMI hadron absorber, before travelling ${\sim}100$~m to the MicroBooNE detector where they decay. A single selection and search strategy is used to target decays of HPS to $\mu\mu$ pairs and HNL to $\mu\pi$ pairs. The results are expressed as limits, at the $90\%$ confidence level, on the mixing angles that control the rates of production and decay for each new particle. For the HNL model, upper limits are set on the mixing parameter $\mumix$ in the range [$12.9 \times 10^{-8}$, $0.54 \times 10^{-8}$] for HNL with masses in the region $246$--$385$~MeV. % This represents an order of magnitude increase in sensitivity to the previous MicroBooNE HNL result. For the HPS model, limits on the scalar-Higgs mixing angle $\theta^2$ are set, excluding a region with a lower boundary between [$31.3 \times10^{-9}$, $1.09 \times 10^{-9}$] and an upper boundary between [$2.50 \times 10^{-5}$, $5.05 \times 10^{-9}$] for scalars with a mass of $212$--$275$ MeV. These results set the first constraints in this region of parameter space from a dedicated experimental search for HPS.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2023

Structural and spectroscopic characterization of thorium pyrasal complexes

To explore the coordination chemistry of thorium, the most abundant radioactive element on earth, we examine the synthesis and characterization of two Th (IV)-pyrasal complexes, L1 “pyrasal” ((2,2'-((1E,1'E)-(pyrazine-2,3-diylbis(azaneylylidene))bis(methaneylylidene))diphenol), and L2 “naphthylpyrasal” (1,1'-((1E,1'E)-(pyrazine-2,3-diylbis(azaneylylidene))bis(methaneylylidene))bis(naphthalen-2-ol). These complexes demonstrate little or no fluorescence when compared to similar naphthylsalophen thorium complexes previously published. Each complex was synthesized and characterized by IR, NMR (1H), and mass spectrometry. The photometric properties of the complexes were characterized using UV–Vis and fluorescence spectroscopy and their solid-state molecular structures were established by single-crystal X-ray crystallography. The electron-withdrawing effects of the pyrazine ring creates changes in the thorium coordination environment resulting in a secondary solid-state extended structure that minimizes the pi-pi stacking. Further, this subsequently causes an overall decrease in the intensity of fluorescence demonstrated previously in by naphthylsalophen thorium complexes.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2022

Scaling CFB risers: Maintaining microstructure dynamics

Over the years there have been numerous approaches to develop a scaleup methodology for circulating fluidized beds. Many of these past approaches have relied on macroscopic definitions of similitude to define dimensionless groups such as Reynolds number, Froude number, density ratios, and dimensional ratios involving different length scales. These approaches have demonstrated various levels of success, but often fail when used outside the bounds of experimental datasets. The issue with these methods is that they rely on macroscopic similitude with the hopes that those conditions would provide microscopic similitude as it does in single phase systems where the Buckingham Pi techniques have given reasonable success. Two of the main reasons for failure are 1) changing fluidization regimes and 2) changing material properties that result in the material falling into a different Geldart group. Both are certain to change the microstructure (local instantaneous volume solids fraction) and changes to the microstructure affect the interphase transport properties of the reactor system, namely the mass transfer and heat transfer. Here, this work presents a new approach towards scaling based upon maintaining similitude at the microscale. It reviews a novel dimensionless flow regime map developed from analysis of the deterministic chaos parameters and higher order moments to ensure microstructure similitude. The work then examines four cases from the literature to assess the scaling approach used: (1) same particle-different scale risers for Geldart Group B particles, (2) Glicksman scaling of atmospheric circulating fluidized bed combustor, (3) same particle-different scale risers for Geldart Group A particles and (4) Glicksman scaling for pressurized gasification. General findings are that none of the scaling approaches produced directly applicable microstructure similar behavior based upon the chaotic and higher moment analysis. The positive take away is that the approach can define scale conditions that will provide similar microstructure that can be us to predict transport behavior.

42 ENGINEERING↗
NASA NTRS2005

Mapping Galactic 60Fe Synthesis in Cen CIR Region

This included a 1 year no cost time extension. The grant was for research into the origin of radioactive 60Fe, whose detection was a mission goal for INTEGRAL and RHESSI. During the grant period, both missions ultimately discovered gamma-line emission from this long lived radioactivity at precisely the value that had been predicted years before by Timmes and Woosley (ApJ, 449,204 (1995)). Unfortunately, using "revised" stellar models and cross sections Rauscher et a1 (ApJ, 576, 323 (2002)), had meanwhile predicted a much larger value. During the grant period, Dieter Hartmann (PI on the complementary grant at Clemson) and Woosley corresponded on this discrepancy and Hartmann visited Santa Cruz (November 20 - 28,2004). All of the grant funds in NAG513659 paid for the expenses of that visit. Subsequently, partly motivated by conversations with Hartmann and Diehl, Woosley re-investigated the production of 60Fe and 26A1 in massive stars from 12 - 120 solar masses, with an eye towards determining the relevant, uncertain physics. The chief changes in Rauscher et a1 were "new" Hauser Feshbach cross sections for 59,60Fe(ng) and 26Al(np)26Mg. The latter has an experimental evaluation which was actually better represented in the study of Timmes and Woosley. The iron (ng) cross sections are from theory and the Timmes and Woosley values were just as reliable as those from Rauscher. Experiments need to be done to resolve who is right. In addition uncertainties in stellar winds, opacities and the IMF were explored. The bottom line is that the value predicted by Timmes and Woosley could well be the correct one, but the experimental error bar is larger than was realized. At least half of the uncertainty is nuclear cross sections that can, and should be measured in the laboratory.

Woosley, Stanford↗
NASA NTRS2001

Effective Gravitational Temperature in Sedimentation

Particle Image Velocimetry (PIV) is used to study the slow settling motions of spheres in suspensions ranging from dilute to highly concentrated, 0.05 less than phi less than 0.50. During sedimentation, velocity fluctuations are found to be organized into regions of characteristic size L approximately 11 a phi(exp-1/3) and buoyant mass DELTA m given by the rms density fluctuations in a region of size L(sup 3) assuming random statistics with excluded volume effects. A simple model accurately predicts the magnitudes of the velocity fluctuations DELTA V. Finally, we find a new universal relation for particle diffusion during sedimentation that can be written in a Stokes-Einstein type form as D approximately (DELTA mg L)/(6 pi eta L), where the effective temperature DELTA mg L is the gravitational potential energy of density fluctuations.

Segre, Philip N.↗
NASA NTRS1985

Far-infrared emission lines of CO and OH in the Orion-KL molecular shock

Observations of far infrared rotational emission lines which arise in the shocked gas associated with Orion-Kl are presented, including detections of the CO J = 34 yields 33, J = 31 yields 30, J = 26 yields 25, and OH sup 2 PI sub (3/2) J sup P = 7/2(-) yields 5/2(+) emission lines, as well as improved measurements of the CO J = 22 yields 21 and OH sup 2 PI sub (3/2) J = 5/2 yields 3/2 lines. These lines are observed to have velocity widths of Del V approx. 20 to 30 km/sec, somewhat less than either the 2 micro H sub 2 lines or the high velocity plateau component of the millimeter wave CO lines seen in this object. An H sub 2 column density of approx. 3 x 10 to the 21st power, a total mass of approx. 1 solar mass and characteristic temperature and density T approx. 750 K and approx. 2 x 10 to the 6th power per cu cm can be derived from the CO intensities. The density is too low by at least an order of magnitude for the observed infrared H sub 2 and far infrared CO emission to be accounted for by a purely hydrodynamic shock, and support is lent to hydromagnetic shock models. From the present measurements, the relative abundance of CO is estimated to be CO H sub 2 = 1.2 x .0001, corresponding to 20% of the cosmic abundance of C existing in the form of CO. The average relative abundance of OH in the shocked gas is O/H sub 2 or = 5 x 10 to the -7th power. An upper limit to the intensity of the HD J = 1 yields 0 line is used to derive an upper limit of tau or = 3 for the D/H relative abundance in the Orion cloud core.

Watson, D. M.↗
NASA NTRS1985

Far-infrared emission lines of CO and OH in the Orion-KL molecular shock

Observations of far infrared rotational emission lines which arise in the shocked gas associted with Orion-Kl are presented, including detections of the CO J = 34 yields 33, J = 31 yields 30, J = 26 yields 25, and OH sup 2 PI sub (3/2) J sup P = 7/2(-) yields 5/2(+) emission lines, as well as improved measurements of the CO J = 22 yields 21 and OH sup 2 PI sub (3/2) J = 5/2 yields 3/2 lines. These lines are observed to have velocity widths of Del V approx. 20 to 30 km/sec, somewhat less than either the 2 micro H sub 2 lines or the high velocity plateau component of the millimeter wave CO lines seen in this object. An H sub 2 column density of aprox. 3 x 10 to the 21st power, a total mass of approx. 1 solar mass and characteristic temperature and density T approx. 750 K and approx. 2 x 10 to the 6th power per cu cm can be derived from the CO intensities. The density is too low by at least an order of magnitude for the observed infrared H sub 2 and far infrared CO emission to be accounted for by a purely hydrodynamic shock, and support is lent to hydromagnetic shock models. From the present measurements, the relative abundance of CO is estimated to be CO H sub 2 = 1.2 x .0001, corresponding to 20 percent of the cosmic abundance of C existing in the form of CO. The average relative abundance of OH in the shocked gas is O/H sub 2 or = 5 x 10 to the -7th power. An upper limit to the intensity of the HD J - 1 yields 0 line is used to derive an upper limit of tau or = 3 for the D/H relative abundance in the Orion cloud core.

Watson, D. M.↗
NASA NTRS2004

Retrieval and Validation of Cirrus Cloud Properties with the Far-Infrared Sensor for Cirrus (FIRSC) During CRYSTAL-FACE

This grant supported the principal investigator's analysis of data obtained during CRYSTAL-FACE by two submillimeter-wave radiometers: the Far-Infrared Sensor for Cirrus (FIRSC) and the Conical Scanning Submillimeter-wave Imaging Radiometer (CoSSIR). The PI led the overall FIRSC investigation, though Co-I Michael Vanek led the instrument component at NASA Langley. The overall CoSSIR investigation was led by James Wang at NASA Goddard, but the cirrus retrieval and validation was performed at the University of Colorado. The goal of this research was to demonstrate the submillimeter-wave cirrus cloud remote sensing technique, provide retrievals of ice water path (IWP) and median mass particle diameter (D(sub me)), and perform validation of the cirrus retrievals using other CRYSTAL-FACE datasets.

Evans, K. Franklin↗
NASA NTRS2000

Correlations and Gravitational Temperature in Settling Suspensions

Particle Image Velocimetry (PIV) is used to study the slow settling motions of spheres in suspensions ranging from dilute to highly concentrated, 0.05 less than phi less than 0.50. During sedimentation, velocity fluctuations are found to be organized into regions of characteristic size L approximately equal to 11 a phi(exp -1/3) and buoyant mass DELTA m given by the rms density fluctuations in a region of size L(exp 3) assuming random statistics. A simple model incorporating the suspension viscosity and excluded volume effects accurately predicts the magnitudes of the observed velocity fluctuations DELTA V. These lead to a universal relation for particle diffusion that can be written in a Stokes-Einstein type form as D approximately equal to (DELTA m gL)/(6 pi (eta)L).

Segre, Philip N.↗
DOE OSTI2020

Reconstruction and Measurement of $\mathcal{O}$(100) MeV Energy Electromagnetic Activity from $\pi^0 \rightarrow \gamma\gamma$ Decays in the MicroBooNE LArTPC

We present results on the reconstruction of electromagnetic (EM) activity from photons produced in charged current νμ interactions with final state π0s. We employ a fully-automated reconstruction chain capable of identifying EM showers of &calO;(100) MeV energy, relying on a combination of traditional reconstruction techniques together with novel machine-learning approaches. These studies demonstrate good energy resolution, and good agreement between data and simulation, relying on the reconstructed invariant π0 mass and other photon distributions for validation. The reconstruction techniques developed are applied to a selection of νμ + Ar → μ + π0 + X candidate events to demonstrate the potential for calorimetric separation of photons from electrons and reconstruction of π0 kinematics.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2024

Study of η′ → π+π−l+l− decays at BESIII

Abstract With a sample of (10087±44)×10 6 J/ψevents accumulated with the BESIII detector, we analyze the decaysη′→ π + π − l + l − (l=e, μ) via the processJ/ψ → γη′. The branching fractions are measured to be$$ \mathcal{B} $$ B (η′→ π + π − e + e − ) = (2.45±0.02(stat.)±0.08(syst.))×10 −3 and$$ \mathcal{B} $$ B (η′→ π + π − μ + μ − ) = (2.16±0.12(stat.)±0.06(syst.))×10 −5 , and the ratio is$$ \frac{\mathcal{B}\left({\eta}^{\prime}\to {\pi}^{+}{\pi}^{-}{e}^{+}{e}^{-}\right)}{\mathcal{B}\left({\eta}^{\prime}\to {\pi}^{+}{\pi}^{-}{\mu}^{+}{\mu}^{-}\right)}=113.4\pm 0.9\left(\textrm{stat}.\right)\pm 3.7\left(\textrm{syst}.\right) $$ B η ′ → π + π − e + e − B η ′ → π + π − μ + μ − = 113.4 ± 0.9 stat . ± 3.7 syst . . In addition, by combining theη′ →π + π − e + e − andη′ →π + π − μ + μ − decays, the slope parameter of the electromagnetic transition form factor is measured to beb η′ = 1.30 ± 0.19 (GeV/c 2 ) −2 , which is consistent with previous measurements from BESIII and theoretical predictions from the VMD model. The asymmetry in the angle between theπ + π − andl + l − decay planes, which has the potential to reveal theCP-violation originating from an unconventional electric dipole transition, is also investigated. The asymmetry parameters are determined to be$$ {\mathcal{A}}_{CP}\left({\eta}^{\prime}\to {\pi}^{+}{\pi}^{-}{e}^{+}{e}^{-}\right)=\left(-0.21\pm 0.73\left(\textrm{stat}.\right)\pm 0.01\left(\textrm{syst}.\right)\right)\% $$ A CP η ′ → π + π − e + e − = − 0.21 ± 0.73 stat . ± 0.01 syst . % and$$ {\mathcal{A}}_{CP}\left({\eta}^{\prime}\to {\pi}^{+}{\pi}^{-}{\mu}^{+}{\mu}^{-}\right)=\left(0.62\pm 4.71\left(\textrm{stat}.\right)\pm 0.08\left(\textrm{syst}.\right)\right)\% $$ A CP η ′ → π + π − μ + μ − = 0.62 ± 4.71 stat . ± 0.08 syst . % , implying that no evidence ofCP-violation is observed at the present statistics. Finally, an axion-like particle is searched for via the decayη′ →π + π − a, a→e + e − , and upper limits of the branching fractions are presented for the mass assumptions of the axion-like particle in the range of 0−500 MeV/c 2 .

Physics↗
DOE OSTI2020

Search for heavy neutral leptons decaying into muon-pion pairs in the MicroBooNE detector

We present upper limits on the production of heavy neutral leptons (HNLs) decaying to $\mu \pi$ pairs using data collected with the MicroBooNE liquid-argon time projection chamber (TPC) operating at Fermilab. This search is the first of its kind performed in a liquid-argon TPC. We use data collected in 2017 and 2018 corresponding to an exposure of $2.0 \times 10^{20}$ protons on target from the Fermilab Booster Neutrino Beam, which produces mainly muon neutrinos with an average energy of $\approx 800$ MeV. HNLs with higher mass are expected to have a longer time-of-flight to the liquid-argon TPC than Standard Model neutrinos. The data are therefore recorded with a dedicated trigger configured to detect HNL decays that occur after the neutrino spill reaches the detector. We set upper limits at the $90\%$ confidence level on the element $\lvert U_{\mu4}\rvert^2$ of the extended PMNS mixing matrix in the range $\lvert U_{\mu4}\rvert^2<(6.6$-$0.9)\times 10^{-7}$ for Dirac HNLs and $\lvert U_{\mu4}\rvert^2<(4.7$-$0.7)\times 10^{-7}$ for Majorana HNLs, assuming HNL masses between $260$ and $385$ MeV and $\lvert U_{e 4}\rvert^2 = \lvert U_{\tau 4}\rvert^2 = 0$.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
NASA NTRS1990

Reactivity of pi-complexes of Ti, V, and Nb towards dithioacetic acid: Synthesis and structure of novel metal sulfur-containing complexes

In order to use sulfur-containing resources economically and with minimal environmental damage, it is important to understand the desulfurization processes. Hydrodesulfurization, for example, is carried out on the surface of a heterogeneous metal sulfide catalyst. Studies of simple, soluble inorganic systems provide information regarding the structure and reactivity of sulfur-containing compounds with metal complexes. Further, consistent with recent trends in materials chemistry, many model compounds warrant further study as catalyst precursors. The reactivity of low-valent organometallic sandwich pi-complexes toward dithiocarboxylic acids is described. For example, treatment of bisbenzene vanadium with CH3CSSH affords a divanadium tetrakis(dithioacetate) complex. The crystallographically determined V-V bond distance, 2.800(2), is nearly the same as the V-V bond distance in a V(mu-nu squared-S2)2V' unit in the mineral patonite (VS4)n. The stability of the V2S4 core in the dimer is demonstrated by evidence of V2S4(+) in the mass spectrum (70 eV, solid probe) of the vanadium dimer. Several other systems relevant to HDS catalysis are also discussed.

Duraj, Stan A.↗
DOE OSTI2024

First Search for Dark-Trident Processes Using the MicroBooNE Detector

This thesis presents a first search for dark-trident scattering in a neutrino beam using a data set corresponding to $7.2 \times 10^{20}$ protons on target taken with the MicroBooNE detector at Fermilab. Proton interactions in the neutrino target at the Main Injector produce $\pi^0$ and $\eta$ mesons, which could decay into dark matter (DM) particles via a dark photon $A^{\prime}$. A convolutional neural network is trained to identify interactions of the DM particles in the liquid-argon time projection chamber (LArTPC) exploiting its image-like reconstruction capability. In the absence of a DM signal, limits at the $90\%$ confidence level on the squared kinematic mixing parameter $\varepsilon^2$ as a function of the dark-photon mass in the range $10\le M_{A^\prime}\le 400$~MeV are provided. The limits cover previously unconstrained parameter space for the production of fermion or scalar DM particles $\chi$ for two benchmark models with mass ratios $M_{\chi}/M_{A^\prime}=0.6$ and $2$ and for dark fine-structure constants $0.1\le\alpha_D\le 1$.Date of Award1 Aug 2024Original languageEnglishAwarding InstitutionThe University of ManchesterSupervisorStefan Soldner-Rembold (Supervisor) & Justin Evans (Supervisor)

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
NASA NTRS1986

The 10Be contents of SNC meteorites

Several authors have explored the possibility that the Shergottites, Nakhlites, and Chassigny (SNC) came from Mars. The spallogenic gas contents of the SNC meteorites have been used to: constrain the sizes of the SNC's during the last few million years; to establish groupings independent of the geochemical ones; and to estimate the likelihood of certain entries in the catalog of all conceivable passages from Mars to Earth. The particular shielding dependence of Be-10 makes the isotope a good probe of the irradiation conditions experienced by the SNC meteorites. The Be-10 contents of nine members of the group were measured using the technique of accelerator mass spectrometry. The Be-10 contents of Nakhla, Governador Valadares, Chassigny, and probably Lafayette, about 20 dpm/kg, exceed the values expected from irradiation of the surface of a large body. The Be-10 data therfore do not support scenario III of Bogard et al., one in which most of the Be-10 in the SNC meteorites would have formed on the Martian surface; they resemble rather the Be-10 contents found in many ordinary chondrites subjected to 4 Pi exposures. The uncertainties of the Be-10 contents lead to appreciable errors in the Be-10 ages, t(1) = -1/lambda ln(1 Be-10/Be-10). Nonetheless, the Be-10 ages are consistent with the Ne-21 ages calculated assuming conventional, small-body production rates and short terrestrial ages for the finds. It is believed that this concordance strengthens the case for at least 3 different irradiation ages for the SNC meteorites. Given the similar half-thicknesses of the Be-10 and Ne-21 production rates, the ratios of the Be-10 and Ne-21 contents do not appear consistent with common ages for any of the groups. In view of the general agreement between the Be-10 and Ne-21 ages it does not seem useful at this time to construct multiple-stage irradiation histories for the SNC meteorites.

Pal, D. K.↗
NASA NTRS2007

Hydrogen Migration and Vinylidene Pathway for Formation of Methane in the 193 nm Photodissociation of Propene: CH3CH=CH2 and CD3CD=CD2

Photodissociation channels and the final product yields from the 193 nm photolysis of propene-h6 (CH2=CHCH3) and propene-d6 (CD2=CDCD3) have been investigated, employing gas chromatography, mass spectroscopy, and flame ionization (GC/MS/FID) detection methods. The yields of methane as well as butadiene relative to ethane show considerable variations when propene-h6 or propene-d6 are photolyzed. This suggests significant variances in the relative importance of primary photolytic processes and/or secondary radical reactions, occurring subsequent to the photolysis. Theoretical calculations suggest the potential occurrence of an intramolecular dissociation through a mechanism involving vinylidene formation, accompanied by an ethylenic H-migration through the pi-orbitals. This process affects the final yields of methane-h4 versus methane-d4 with respect to other products. The product yields from previous studies of the 193 nm photolysis of methyl vinyl ketone-h6 and -d6 (CH2=CHCOCH3, CD2=CDCOCD3), alternative precursors for generating methyl and vinyl radicals, are compared with the current results for propene.

Zhao, Yi-Lei↗
DOE OSTI2025

Implications of Aerosol Physicochemical Properties Including Ice Nucleation at ARM Mega Sites for Improved Understanding of Microphysical Atmospheric Cloud Processes (Final Technical Report)

Continuous, long-term measurements of atmospheric ice-nucleating particles (INPs) that influence clouds and precipitation were conducted to investigate the abundance and variability of ground-level INPs across the world. Three field campaigns were organized by the DOE Atmospheric Radiation Measurement (ARM) program, including Examining INP from Southern Great Plains (ExINP-SGP, 2019), Examining INP from Eastern North Atlantic (ExINP-ENA, 2020 – 2021), and Examining INP from North Slope of Alaska (ExINP-NSA, 2021 – 2024). Additional small-scale supporting field experiments were performed in 2019 and 2021 to collect airborne particulate matter at SGP for complementary laboratory characterization of the particles’ physical and chemical properties [Aerosol-Ice Formation Closure Pilot Study (AEROICESTUDY), 2019; ExINP-SGP II, 2021]. In these studies, the PI’s team measured INP concentration with both real-time and laboratory measurements in a wide range of freezing temperatures ($T$ from 0 °C to about –30 °C). This project elucidated spatial variability and seasonality in the abundance of immersion mode active INPs across three ARM sites using a single instrument, a Portable Ice Nucleation Experiment (PINE) chamber version 03 (PINE-03 hereafter). Collocated aerosol and meteorological data were analyzed to assess the correlation between ambient INP abundance, air mass origin region, and meteorological variability. Our findings suggest very high freezing efficiency of INPs at the NSA site across the measured temperatures (ice nucleation active surface site density, $n_s(T)$, $\approx 2 \times 10^{8} - 10^{10}$ m -2 for from –16 to –31 °C), which is a factor of 10 – 1000 times greater efficiency as compared to that found in the previous mid-latitude INP measurements in autumn using the same instrument; surprisingly high INP abundance ($\ge 1 \text{ L}^{-1}$ at –25 °C) for the examined temperatures throughout the year that PINE-03 did not measure at other sites; and high INP concentration in spring, possibly related to arctic haze episodes.

58 GEOSCIENCES↗