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DOE OSTI2020

Correlations between thermal history and keyhole porosity in laser powder bed fusion

Additive manufacturing has the potential to revolutionize the production of metallic components as it yields near net shape parts with complex geometries and minimizes waste. At the present day, additively manufactured components face qualification and certification challenges due to the difficulty in controlling defects. This has driven a significant research effort aimed at better understanding and improving processing controls – yielding a plethora of in-situ measurements aimed at correlating defects with material quality metrics of interest. In this work, we develop machine-learning methods to learn correlations between thermal history and subsurface porosity for a variety of print conditions in laser powder bed fusion. Un-normalized surface temperatures (in the form of black-body radiances) are obtained using high-speed infrared imaging and porosity formation is observed in the sample cross-section through synchrotron x-ray imaging. To demonstrate the predictive power of these features, we present four statistical machine-learning models that correlate temperature histories to subsurface porosity formation in laser fused Ti-6Al4V powder.

36 MATERIALS SCIENCE↗

DOE OSTI2021

History and status of spent fuel treatment at the INL Fuel Conditioning Facility

Experimental Breeder Reactor II (EBR-II) had an illustrious operational history from 1964 to 1994 as one of the first sodium-cooled fast reactors to use sodium-bonded metallic driver fuels and blankets. EBR-II was a testbed for fuel development and reactor design principles. Following shutdown, it was decided to use electrometallurgical methods to treat the spent fuel and blanket materials for final disposition. Here, this paper provides a brief history of U.S. liquid metal cooled reactor development with emphasis on EBR-II, and a technical description of the electrometallurgical methods.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

DOE OSTI2024

Cosmogenic surface exposure ( 10 Be) dating of raised beaches in Marguerite bay, Antarctic Peninsula: Implications for relative sea-level history

Understanding the dynamics of ice mass loss in polar regions is crucial for deciphering climate change and Glacio Isostatic Adjustment patterns. This study focuses on Marguerite Bay, located in the south-central Antarctic Peninsula. We dated raised beaches to investigate relative sea-level changes using the cosmogenic surface exposure ( 10 Be) method. Previous studies have provided valuable insights into the region's glacial history, but limitations in dating techniques and age estimates necessitate further investigation. By analysing raised shingle beaches in Gaul Cove of Horseshoe Island and the southern coast of Calmette Bay, this research aims to contribute relative sea-level change history for these areas. In Horseshoe Island's Gaul Cove, raised beaches clustered on prominent steps reveal a 15 m relative sea-level change over the last 3.31 ka. Differently, Calmette Bay exhibits a 36 m relative sea-level fall over the last 7.29 ka. Finally, these findings indicate significant and differential glacial-isostatic adjustments in both regions during the middle and late Holocene. Additionally, our data reveal accelerated sea-level fall periods corresponding to Holocene deglaciation and glacial advance events, indicating the shorelines' relative sea-level change sensitivity to climate change.

58 GEOSCIENCES↗

DOE OSTI2021

The Role of Stratigraphy and Loading History in Generating Complex Compaction Bands in Idealized Field-Scale Settings

The Buckskin Gulch locality in Utah is a landmark example of compaction localization. The outcrop of this locality involves distinct stratigraphic heterogeneity and was exposed to complex loading history. It features multiple sets of deformation bands with different kinematics and orientation. Similar formations were seen in the Valley of Fire, Nevada, and the Orange quarry, France, among other localities. The formation of such complex structures, their propagation mechanisms, and frequency is affected by numerous local and ambient factors whose impacts are not yet fully understood. The simulation of the above-mentioned localities is not feasible because of the limited amount of available information. This work, instead, investigates from a geomechanics standpoint how the interplay among material nonlinearity, outcrop stratigraphy, and loading history interconnects with specific spatiotemporal patterns of compaction band propagation. Our study shows that the system stratigraphy can be responsible for the emergence of coexisting compaction bands with different inclination and kinematics. Specifically, we show that stiffness contrasts induce nonlocal stress changes which may favor the initiation of secondary structures with different compaction localization characteristics. Furthermore, systems of inclined compaction bands induced by burial increase display secondary, noncontemporaneous sets of vertical compaction bands under the effects of postburial shortening. Our results indicate that stages of intermediate burial decrease prior to tectonic shortening can promote the formation of such complex systems. Despite the simplifications involved in our analyses, these findings show how geomechanics computations complement field observations and could provide a mechanics-based validation of site-specific reconstruction hypothesis.

58 GEOSCIENCES↗

DOE OSTI2021

Energy Budget Constraints on the Time History of Aerosol Forcing and Climate Sensitivity

Abstract An observationally constrained time series of historical aerosol effective radiative forcing (ERF) from 1750 to 2019 is developed in this study. We find that the time history of aerosol ERFs diagnosed in CMIP6 models exhibits considerable variation and explore how the time history of aerosol forcing influences the probability distributions of present‐day aerosol forcing and emergent metrics such as climate sensitivity. Using a simple energy balance model, trained on CMIP6 climate models and constrained by observed near‐surface warming and ocean heat uptake, we derive estimates for the historical aerosol forcing. We find 2005–2014 mean aerosol ERF to be −1.1 (−1.8 to −0.5) W m −2 relative to 1750. Assuming recently published historical emissions from fossil fuel and industrial sectors and biomass burning emissions from SSP2‐4.5, aerosol ERF in 2019 is −0.9 (−1.5 to −0.4) W m −2 . There is a modest recovery in aerosol forcing (+0.025 W m −2 decade −1 ) between 1980 and 2014. This analysis also gives a 5%–95% range of equilibrium climate sensitivity of 1.8°C –5.1°C (best estimate 3.1°C) with a transient climate response of 1.2°C –2.6°C (best estimate 1.8°C).

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2021

Precambrian Crystalline Basement Properties From Pressure History Matching and Implications for Induced Seismicity in the US Midcontinent

Injection-induced seismicity across the US midcontinent has almost exclusively occurred in the crystalline basement that underlies the Arbuckle Group aquifer and its equivalents, the primary wastewater disposal zone in this region. However, the properties of the basement are not well known. Newly compiled data, from Class I wells in Kansas, provide a unique record of pressures in the Arbuckle and an opportunity to constrain the reservoir-scale properties of the basement such as permeability, diffusivity, and specific storage. Constraints on these parameters are critical for modeling fluid flow and pressures across the entire Arbuckle-basement system, and are necessary for accurate evaluation and prediction of injection-induced earthquakes. Here, we present a detailed, three-dimensional geological and pressure history-matched numerical model for the Arbuckle and basement, based on data from >400 wells covering a large region in south-central Kansas, where injection-induced seismicity has been concentrated since 2014. Simulations of dynamic data from 319 wells indicate that Arbuckle pressures have increased by 1.1 MPa in high injection rate areas and an overpressure of <0.1 MPa may be the cause of seismicity in the basement. Pressure-history matching also yields the likely range in porosity (0.3%–7%), permeability (0.1–0.7 mD), and diffusivity (0.004–0.07 m2 /s) for the basement. The resulting estimates suggest reservoir-scale properties of the basement are enhanced by faults and fractures. Importantly, the diffusivities determined in this study are lower than estimates derived from Kansas earthquake triggering fronts, and suggest that such seismicity-based techniques may have limitations, particularly where spacetime patterns between injection and seismicity are complex.

58 GEOSCIENCES↗

DOE OSTI2025

The Mystery of Baselevel Controls in the Incision History of the Central Colorado Plateau

Erosion can remain active and changing in landscapes long after tectonic drivers have ceased, potentially due to local-geologic controls, climate changes, or geodynamics. We present new fluvial incision-rate histories and terrain analyses of the Colorado River system through the central Colorado Plateau to understand what has caused the variable erosion across this post-orogenic landscape. Results from new cosmogenic and luminescence dating of fluvial terrace and upland gravel deposits in Glen and Meander Canyons establish incision-rate histories that are marked by an Early-Middle Pleistocene erosion hiatus, followed by ~200 m of rapid incision over the last ~350 kyr. Projection of fluvial topography from above knickzones of the Colorado River drainage system roughly agree with the observed magnitude of recent incision and reflect a common baselevel fall from Pliocene river integration through Grand Canyon, which is still propagating through the drainage. A response-time model indicates that baselevel fall from integration likely took 2–4 Myr to reach the central Colorado Plateau and 100s kyr to travel across the study area, potentially accounting for incision rate changes in the fluvial terrace records of Meander and Glen Canyons. The upstream-migrating incision has likely been partitioned into multiple waves across the landscape due to the local geologic controls of lava damming, salt tectonics, and heterogenous bedrock. As baselevel fall from Pliocene Colorado River integration diffuses upstream, it can only account for perhaps a quarter of the total ~2 km of exhumation in the central Colorado Plateau, demanding an unknown driver for significant erosion in the Pliocene.

58 GEOSCIENCES↗

DOE OSTI2025

Terrestrial atmospheric ion implantation occurred in the nearside lunar regolith during the history of Earth’s dynamo

Light volatile elements in lunar regolith are thought to be a mixture of the solar wind and Earth’s atmosphere, the latter sourced in the absence of geomagnetic field. However, the extent to which both the current and primitive geodynamo influence the transport of terres trial ions still remains unclear, and this uncertainty is further complicated by the enigmatic composition and poorly constrained location of the Eoarchean exosphere. Here we use 3-D MHD numerical simulations with contemporary magnetized and Archean unmagnetized atmospheres to investigate how Earth’s intrinsic magnetic field affects this transfer, aiming to constrain how and when the lunar isotopic signature provides a record of Earth’s pale-oatmosphere. We find that atmospheric transfer is efficient only when the Moon is within Earth’s magnetotail. The non-solar contribution to the lunar soil is best explained by implantation during the long history of the geodynamo with present-day solar wind conditions, rather than any short, putatively unmagnetized epoch of early Archean Earth. This further suggests the history of the terrestrial atmosphere, spanning billions of years, could be preserved in buried lunar soils. Our results indicate that the elemental abundances of Apollo samples are very sensitive to Earth’s hydrodynamic exobase altitude, which, at the time of ion implantation, was never smaller than 190 km.

Atmospheric dynamics↗

DOE OSTI2024

The center for nonlinear studies: A personal history

The Center for Nonlinear Studies (CNLS) was an integral part of my scientific career starting as a Postdoctoral Fellow in 1983 up to my tenure as CNLS Director from 2004 to 2015. As such, I experienced a number of scientific phases of CNLS through almost four decades of foundation, evolution, and transition. Throughout this entire interval, the inspiration and influence of David Campbell guided my way. A proper history of CNLS encompassing all of the many contributors to the CNLS story is beyond my means or purpose here. Instead, I present the history as I experienced it. I emphasize the main scientific accomplishments achieved at CNLS over more than 40 years, but I will also attempt to describe and quantify the attributes that made and continue to make the Center for Nonlinear Studies a special institution of remarkable impact and longevity. Throughout its existence, CNLS owes much to the enduring legacy of David Campbell who laid down the foundations and operating principles that have made it so successful.

Ecke, Robert E. (ORCID:0000000177725876)↗

DOE OSTI2025

Ultra-fast single-crystal CVD diamonds in the particle time-of-flight (PTOF) detector for low yield burn-history measurements on the NIF (invited)

The Particle Time of Flight (PTOF) diagnostic is a chemical vapor deposition diamond-based detector and is the only diagnostic for measuring nuclear bang times of low yield (<1013) shots on the National Ignition Facility. Recently, a comprehensive study of detector impulse responses revealed certain detectors with very fast and consistent impulse responses with a rise time of <50 ps, enabling low yield burn history measurements. At the current standoff of 50 cm, this measurement is possible with fast 14 MeV neutrons from deuterium–tritium (DT) fusion plasmas. PTOF-inferred DT burn width numbers compare well with widths inferred from the gamma reaction history diagnostic on mid-yield (1013–1015) shots, where both systems are capable of making this measurement. These new capabilities could be extended to 2.5 MeV deuterium–deuterium neutrons from D plasmas and to even lower yield by reducing the detector standoff distance to 10 cm; a design for this is also presented.

42 ENGINEERING↗

DOE OSTI2026

The next-generation particle x-ray temporal diagnostic for simultaneous time-resolved measurements of nuclear-burn and x-ray emission histories in support of basic-science and inertial confinement fusion experiments at OMEGA

The next-generation Particle X-ray Temporal Diagnostic (PXTD) has been implemented for simultaneous measurements of x-ray, charged particle, and neutron emission histories from a wide range of inertial confinement fusion and high energy density plasma experiments, demonstrating excellent timing accuracy and greatly improved experimental flexibility. The key changes to the previously fielded system are a redesigned set of thin foil filters in front of the scintillators and individual neutral density filters for each region of the detector. The fully implemented PXTD system can provide unique information about the evolution of ion and electron temperatures in multi-ion and kinetic-physics experiments, proton radiography experiments, and DT experiments executed at the OMEGA facility. The system has 35 ps time resolution and negligible relative timing uncertainty between measured emission history signals. The first use of the upgraded four-channel PXTD system during a set of D 3 He-filled silica-glass implosions on OMEGA captured electron temperatures with a minimum uncertainty of 0.5 keV and resolved both the relative timings and widths of neutron, proton, and x-ray peaks within a single recorded image.

Evans, T. E. [Massachusetts Inst. of Technology (M↗

DOE OSTI2024

Chapter 5: Major Biological Innovations in the History of Life on Earth

All organisms living on Earth descended from a single, common ancestral population of cells, known as LUCA—the last universal common ancestor. Since its emergence, the diversity and complexity of life have increased dramatically. Here this chapter focuses on four key biological innovations throughout Earth's history that had a significant impact on the expansion of phylogenetic diversity, organismal complexity, and ecospace habitation. First is the emergence of the last universal common ancestor, LUCA, which laid the foundation for all life-forms on Earth. Second is the evolution of oxygenic photosynthesis, which resulted in global geochemical and biological transformations. Third is the appearance of a new type of cell—the eukaryotic cell—which led to the origin of a new domain of life and the basis for complex multicellularity. Fourth is the multiple independent origins of multicellularity, resulting in the emergence of a new level of complex individuality. A discussion of these four key events will improve our understanding of the intertwined history of our planet and its inhabitants and better inform the extent to which we can expect life at different degrees of diversity and complexity elsewhere.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2025

Inferring demographic and selective histories from population genomic data using a 2-step approach in species with coding-sparse genomes: an application to human data

Abstract The demographic history of a population, and the distribution of fitness effects (DFE) of newly arising mutations in functional genomic regions, are fundamental factors dictating both genetic variation and evolutionary trajectories. Although both demographic and DFE inference has been performed extensively in humans, these approaches have generally either been limited to simple demographic models involving a single population, or, where a complex population history has been inferred, without accounting for the potentially confounding effects of selection at linked sites. Taking advantage of the coding-sparse nature of the genome, we propose a 2-step approach in which coalescent simulations are first used to infer a complex multi-population demographic model, utilizing large non-functional regions that are likely free from the effects of background selection. We then use forward-in-time simulations to perform DFE inference in functional regions, conditional on the complex demography inferred and utilizing expected background selection effects in the estimation procedure. Throughout, recombination and mutation rate maps were used to account for the underlying empirical rate heterogeneity across the human genome. Importantly, within this framework it is possible to utilize and fit multiple aspects of the data, and this inference scheme represents a generalized approach for such large-scale inference in species with coding-sparse genomes.

Soni, Vivak (ORCID:0000000294969562)↗

DOE OSTI2020

Correlations between triaxial shapes and formation history of dark matter haloes

ABSTRACT The shape of dark matter (DM) haloes plays a critical role in constraining cosmology with upcoming large-scale structure surveys. In this paper, we study the correlations between the triaxial shapes and formation histories in DM haloes in the MultiDark Planck 2 N-body cosmological simulation. We find that halo ellipticity is strongly correlated with halo properties that serve as proxies of halo formation history, such as halo concentration and the normalized peak-centroid offset. These correlations are nearly independent of the halo density peak height. We present a simple model for the correlation between halo ellipticity and concentration using conditional abundance matching, and provide fitting formulae for the multidimensional distributions of triaxial halo shape as a function of halo peak height. We apply our halo shape model to gauge the effects of halo ellipticity and orientation bias on the excess surface mass density profiles in cluster-sized haloes. Our model should be useful for exploring the impact of triaxial halo shape on cosmological constraints in upcoming weak lensing surveys of galaxy clusters.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2021

Size, shade, or shape? The contribution of galaxies of different types to the star formation history of the Universe from SDSS-IV MaNGA

ABSTRACT By fitting stellar populations to the fourth generation of the Sloan Digital Sky Survey (SDSS-IV) Mapping Nearby Galaxies at Apache Point Observatory (MaNGA) survey observations of ∼7000 suitably weighted individual galaxies, we reconstruct the star formation history of the Universe, which we find to be in reasonable agreement with previous studies. Dividing the galaxies by their present-day stellar mass, we demonstrate the downsizing phenomenon, whereby the more massive galaxies hosted the most star formation at earlier times. Further dividing the galaxy sample by colour and morphology, we find that a galaxy’s present-day colour tells us more about its historical contribution to the cosmic star formation history than its current morphology. We show that downsizing effects are greatest among galaxies currently in the blue cloud, but that the level of downsizing in galaxies of different morphologies depends quite sensitively on the morphological classification used, due largely to the difficulty in classifying the smaller low-mass galaxies from their ground-based images. Nevertheless, we find agreement that among galaxies with stellar masses $M_{\star } \gt 6\times 10^{9}\, \mathrm{ M}_{\odot }$, downsizing is most significant in spirals. However, there are complicating factors. For example, for more massive galaxies, we find that colour and morphology are predictors of the past star formation over a longer time-scale than in less massive systems. Presumably this effect is reflecting the longer period of evolution required to alter these larger galaxies’ physical properties, but shows that conclusions based on any single property do not tell the full story.

Peterken, Thomas↗

DOE OSTI2021

Star formation in CALIFA survey perturbed galaxies – II. Star-formation histories and oxygen abundances

ABSTRACT Galaxy evolution is generally affected by tidal interactions. First, in this series, we reported several effects that suggest that tidal interactions contribute to the regulation of star formation (SF). To confirm this, we now compare stellar mass assembly histories and SF look-back time annular profiles between CALIFA survey tidally and non-tidally perturbed galaxies. We pair their respective star-forming regions at the closest stellar mass surface densities to reduce the influence of stellar mass. The assembly histories and annular profiles show statistically significant differences so that higher star-formation rates characterize regions in tidally perturbed galaxies. These regions underwent a more intense (re)activation of SF in the last 1 Gyr. Varying shapes of the annular profiles also reflect fluctuations between suppression and (re)activation of SF. Since gas-phase abundances used to be lower in more actively than in less actively star-forming galaxies, we further explore the plausible presence of metal-poor gas inflows able to dilute such abundances. The resolved relations of oxygen (O) abundance with stellar mass density and with total gas fraction show slightly lower O abundances for regions in tidally perturbed galaxies. The single distributions of O abundances statistically validate this. Moreover, from a metallicity model based on stellar feedback, the mass rate differentials (inflows−outflows) show statistically valid higher values for regions in tidally perturbed galaxies. These differentials, and the metal fractions from the population synthesis, suggest dominant gas inflows in these galaxies. This dominance and the differences in SF through time confirm the previously reported effects of tidal interactions on SF.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2023

The star-formation history in the last 10 billion years from CIB cross-correlations

ABSTRACT The cosmic infrared background (CIB) traces the emission of star-forming galaxies throughout all cosmic epochs. Breaking down the contribution from galaxies at different redshifts to the observed CIB maps would allow us to probe the history of star formation. In this paper, we cross-correlate maps of the CIB with galaxy samples covering the range z ≲ 2 to measure the bias-weighted star-formation rate (SFR) density 〈bρSFR〉 as a function of time in a model independent way. This quantity is complementary to direct measurements of the SFR density ρSFR, giving a higher weight to more massive haloes, and thus provides additional information to constrain the physical properties of star formation. Using cross-correlations of the CIB with galaxies from the DESI Legacy Survey and the extended Baryon Oscillation Spectroscopic Survey, we obtain high signal-to-noise ratio measurements of 〈bρSFR〉, which we then use to place constraints on halo-based models of the star-formation history. We fit halo-based SFR models to our data and compare the recovered ρSFR with direct measurements of this quantity. We find a qualitatively good agreement between both independent data sets, although the details depend on the specific halo model assumed. This constitutes a useful robustness test for the physical interpretation of the CIB, and reinforces the role of CIB maps as valuable astrophysical probes of the large-scale structure. We report our measurements of 〈bρSFR〉 as well as a thorough account of their statistical uncertainties, which can be used to constrain star-formation models in combination with other data.

Astronomy & Astrophysics↗

DOE OSTI2020

Code package for calculating modified cosmic ionization and thermal histories with dark matter and other exotic energy injections

Here we present a new public Python package, DarkHistory, for computing the effects of dark matter annihilation and decay on the temperature and ionization history of the early universe. DarkHistory simultaneously solves for the evolution of the free electron fraction and gas temperature, and for the cooling of annihilation/decay products and the secondary particles produced in the process. Consequently, we can self-consistently include the effects of both astrophysical and exotic sources of heating and ionization, and automatically take into account backreaction, where modifications to the ionization/temperature history in turn modify the energy-loss processes for injected particles. We introduce a number of worked examples, demonstrating how to use the code in a range of different configurations, in particular for arbitrary dark matter masses and annihilation/decay final states. Possible applications of DarkHistory include mapping out the effects of dark matter annihilation/decay on the global 21 cm signal and the epoch of reionization, as well as the effects of exotic energy injections other than dark matter annihilation/decay. The code is available at https://github.com/hongwanliu/DarkHistory with documentation at https://darkhistory.readthedocs.io. Data files required to run the code can be downloaded at https://doi.org/10.7910/DVN/DUOUWA.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗