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At least 163 records · Page 9

Demonstration of event position reconstruction based on diffusion in the NEXT-white detector

Noble element time projection chambers are a leading technology for rare event detection in physics, such as for dark matter and neutrinoless double beta decay searches. Time projection chambers typically assign event position in the drift direction using the relative timing of prompt scintillation and delayed charge collection signals, allowing for reconstruction of an absolute position in the drift direction. In this paper, alternate methods for assigning event drift dis tance via quantification of electron diffusion in a pure high pressure xenon gas time projection chamber are explored. Data from the NEXT-White detector demonstrate the ability to achieve good position assignment accuracy for both high and low-energy events. Using point-like energy deposits from 83m Kr calibration electron captures (E ~ 45 keV), the position of origin of low-energy events is determined to 2 cm precision with bias < 1 mm. A convolutional neural network approach is then used to quantify diffusion for longer tracks (E ≥ 1.5 MeV), from radiogenic electrons, yielding a precision of 3 cm on the event barycenter. The precision achieved with these methods indicates the feasibility energy calibrations of better than 1% FWHM at Q ββ in pure xenon, as well as the potential for event fiducialization in large future detectors using an alternate method that does not rely on primary scintillation.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Cosmic ray nuclear composition above 20 GeV/nucleon

In three balloon flights during 1971 and 1972 a scintillator-Cerenkov counter telescope was exposed for a net total of 7.6 sq m-ster-hr to measure the charge composition of cosmic-ray nuclei. The telescope includes two gas Cerenkov counters for energy measurements above 20 GeV/nucleon. In this energy range about 3400 nuclei between Li and Fe have been detected and analyzed. The resulting charge composition and energy spectra are presented. The nuclear composition has been found to change with energy. The flux of galactic daughter nuclei decreases faster with increasing energy than the flux of source nuclei. The carbon/oxygen abundance ratio is significantly reduced as compared to low-energy measurements, and iron seems to exhibit a flatter energy spectrum than other nuclei.

Juliusson, E.↗

Estimation of Fission Product Transport Parameters for Cesium in the AGR-3/4 TRISO Fuel Experiment

A one-dimensional (1D) finite-element model of fission product transport in the AGR-3/4 experiment has been developed using the Multiphysics Object Oriented Simulation Environment (MOOSE) framework and implemented in the fuel performance code, BISON. The model resolves capsule-specific geometries, materials, and temperature histories and simulates radial migration of fission products from the fuel compact through the inner ring, outer ring, and into the sink ring. Model parameters governing diffusion and sorption were estimated for key fission products – cesium (Cs), and europium (Eu) – by simultaneously fitting modeled isotopic concentration profiles and total ring inventories to a post-irradiation experimental measurement. These data include gamma scanning, liquid scintillation for Sr-90, radial deconsolidation leach-burn-leach analysis, tomographic reconstructions, and destructive physical sampling. A mortar-based interfacial sorption framework was implemented to enforce physically consistent mass transfer and flux conservation across gas gaps. Two classes of parameter sets were derived: a least-squares best-fit, and a safety-oriented conservative-fit, what applies strong penalties for underprediction of sink inventories. Across all twelve capsules, the model successfully reproduces the dominant radial transport trends for Cs, Sr, with decreasing concentrations from the compact outward through successive rings. Cs behavior is captured most consistently, while strontium predictions reveal systematic trade-offs between compact accuracy and conservative sink-ring bounding. The results demonstrate that sink ring weighted calibration provides conservative, safety relevant bounds on low temperature fission product transport, but at the cost of underpredicting compact inventories for Sr isotopes. These discrepancies highlight the need for additional physics, including fast-slow diffusion model, incorporating trapping mechanism in the transport behavior. Overall, this work establishes a robust, capsule-specific modeling framework for AGR-3/4 fission product transport and provides a defensible basis for parameter selection in source-term and fuel performance analyses for high temperature gas-cooled reactors.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Experimental determination of cosmic ray charged particle intensity profiles in the atmosphere

Absolute cosmic-ray free air ionization and charged particle fluxes and dose rates throughout the atmosphere were measured on a series of balloon flights that commenced in 1968. Argon-filled ionization chambers equipped with solid-state electrometers, with different gas pressures and steel wall thicknesses, and a pair of aluminum-wall Gm counters have provided the basic data. These data are supplemented by measurements with air-filled and tissue equivalent ionization chambers and a scintillation spectrometer. Laboratory experiments together with analyses of the theoretical aspects of the detector responses to cosmic radiation indicate that these profiles can be determined to an overall accuracy of + or - 5 percent.

Lowder, W. M.↗

Density fluctuations in solar wind flow types at 1 AU: Comparison to Doppler scintillation measurements

Density fluctuations with periods 10 minutes to 1 hour have been investigated in ISEE 3 plasma measurements of solar wind flows at l AU. Coronal hole, interstream, plasma sheet, coronal mass ejection, and interaction region flow types are considered. The ISEE 3 results support the interpretation of the large-scale variations in density fluctuations observed by Doppler scintillation measurement techniques inside 0.2 AU. The highest absolute and relative density fluctuations occur ahead of and within the plasma from coronal mass ejections, with the maximum values occurring between the associated interplanetary shocks and the driver gas. For the quasi-stationary solar wind, density and relative density fluctuations are highest around the heliospheric current sheet and lowest in the high-speed coronal flow. Superposed epoch analysis shows that the region of enhanced density fluctuations and its abrupt boundaries observed in the vicinity of the heliospheric current sheet near the Sun persists to l AU, providing further support for the filamentary nature of the extensions of coronal streamers. The results of this study confirm the advantages of using density fluctuations rather than density as a tracer of solar wind flows with differing origins at the Sun and as a detector of propagating interplanetary disturbances.

Huddleston, D. E.↗

Large area position sensitive detector for thermal neutrons

Large area thermal neutron detectors are applied in many fields including industrial imaging, nuclear safeguarding, neutron scattering, and fundamental science. Historically, these detectors were based on 3 He gas proportional counters despite the limitations of 3 He detectors such as high cost, limited supply, non-uniform spatial resolution, and depth of absorption problems. Two alternatives to 3 He detectors are 6 Li-loaded glass scintillators, and powdered ZnS(Ag) scintillators mixed with 6LiF neutron converters. The 6 LiF/ZnS(Ag) scintillator has advantages over 6 Li glass as it is less expensive and can be produced in larger areas, although its self-absorption presents a problem. In this work, we developed a large area thermal neutron detector based on 6 LiF/ZnS(Ag) scintillator coupled with wavelength shifting fibers. The detector uses resistive charge divider-based position encoding. We further modified and improved the method by 2D segmentation of the detector using modular multichannel readout electronics. This segmentation approach allows for a combination of large detector area, improved spatial resolution, and increased count rate. Furthermore, spatial resolution can be variable across the detector area by adjusting the segment size.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Solid, structured composite neutron detectors with high dynamic range capability

Neutron detectors are essential across disciplines such as fundamental science, nuclear security, safeguards, and civilian applications. While 3 He-filled gas proportional counters have long been revered for their efficacy in detecting thermal neutrons and praised for their efficiency, neutron/gamma discrimination, and stability, the scarcity of 3He has spurred a search for alternatives. Here, we explore a solid structured scintillating particle composite (SPC) consisting of 6 Li-containing scintillating glass particles within an acrylic matrix as a neutron detector for high dynamic range applications. We show for the first time that an SPC neutron detector can boast an intrinsic detection efficiency of 0.261% for pure 252 Cf fission neutrons and an overall neutron detection efficiency of (0.546 ± 0.003)% at the Neutron Free-in-Air facility while being able to function in an intense gamma-ray environment. We also show that the SPC neutron detector supports fast neutron capture times and enables a dual-readout scheme that extends the detector dynamic range to high incident neutron fluxes. A scalable fabrication process allows for tailoring the SPC detector properties to the requirements of specific applications. Good agreement is found between the experimental results taken with a National Institute of Standards and Technology traceable 252 Cf source and the coupled MCNP6 and optical-ray-tracing simulations.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Cosmic ray telescope for OGO 2 and 4 spacecraft

The construction and subsequent flight are described of a cosmic ray telescope aboard the OGO-2 and 4 Spacecraft. This instrument was a combination Cerekov-scintillation counter telescope designed to measure the cosmic ray energy spectrum from 1-15 GV and charge composition from Z=1-8. OGO-2 was launched in October 1965; however, attitude control problems caused a rapid loss of control gas, so that after approximately 2 weeks it was no longer possible to point the spacecraft. This mission was officially declared a failure. The cosmic ray instrument appeared to work well during this time. OGO-4 was launched in July 1967, with a similar telescope aboard. It operated successfully approximately one year. The details of the experiment, its operation, and the results are given.

Webber, W. R.↗

Detection of scintillation light in noble gases with wavelength-shifting optical fibers

Wavelength-shifting (WLS) techniques enable particle detectors based on noble gases, whose scintillation light is predominantly emitted in the vacuum-ultraviolet. We investigate WLS fibers coated with tetraphenyl butadiene (TPB) for scintillation light detection in gaseous xenon and argon at pressures up to 8.5 bar, motivated by future high-pressure xenon time-projection chambers of the NEXT program. Two detector configurations are studied: an elongated high-pressure vessel with four PTFE panels equipped with WLS fibers read by temperature-stabilized SiPMs, and a compact box-shaped detector operated at 1 bar Xe with WLS fibers read out by PMTs. Both operate with continuous gas purification. The detector response is characterized using cosmic muons and alpha particles from a $^{241}$Am source. With the SiPM setup, we measure a light collection efficiency (LCE) of ${1.18 \pm 0.01~\mathrm{(sta.)}~^{+0.07}_{-0.09}~\mathrm{(sys.)}~\%}$ for xenon and ${1.07 \pm 0.01~\mathrm{(sta.)}~^{+0.06}_{-0.08}~\mathrm{(sys.)}~\%}$ for argon. With PMT readout, we measure a LCE of ${0.45 \pm 0.01~\mathrm{(sta.)} \pm 0.05~\mathrm{(sys.)}~\%}$ in xenon, in agreement with the SiPM result once photon detection efficiency is accounted for. Average scintillation waveforms in xenon and argon are studied to assess the time structure of the emitted light. Cosmic-muon measurements yield a mean energy required to produce a scintillation photon $45\pm7~\mathrm{(sta.)}~^{+4}_{-5}~\mathrm{(sys.)}~\mathrm{eV}$ at 1.5 bar, in agreement with the literature. The results demonstrate that TPB-coated WLS fiber systems can reliably detect scintillation light in high-pressure gaseous noble detectors, with a LCE representing an upper limit for realistic large-scale TPCs, where additional photon losses from materials and fiber attenuation are expected.

Soleti, S. R. [Donostia Intl. Phys. Ctr., San Seba↗

An instrument to measure the spectrum of cosmic ray iron and other nuclei to above 100 GeV/nucleon

A balloon-borne instrument system for the study of cosmic ray composition in the energy region beyond 100 GeV/nucleon is described. The large area detector incorporates an ionization spectrometer or calorimeter to determine the energy of the incident particles which is calibrated in flight by a gas Cerenkov counter filled with freon 12 at 20 psi. Calibration of calorimeter response indicates that the effects of ionization energy loss and nucleon fragmentation are correctly accounted for in a Monte Carlo simulation. A charge measuring module consisting of five scintillators and a lucite Cerenkov counter is used to determine the charge and position of the incoming particles. A spatial resolution of 5 to 10 cm has been obtained by using the ratios of pulse heights in different photomultiplier tubes aimed at the same scintillators within the module. The detector represents the heaviest cosmic ray experiment that can be flown over 30 km using the dynamic launching technique commonly employed.

Arens, J. F.↗

The occultation of Epsilon Geminorum by Mars - Analysis of McDonald data

An analysis of observations of the occultation of Epsilon Gem by Mars on April 8, 1976, is presented. The data were obtained by three neighboring telescopes at McDonald Observatory. Intensity fluctuations on time scales of the order of 100 ms were observed simultaneously at the three telescopes. As the observations compare well with predictions of turbulent scintillation theory, it is concluded that such fluctuations were probably largely the effect of stellar scintillations in the Martian atmosphere. The stellar diameter is included as a parameter in the theory but in a way which differs from previously published interpretations of occultations of extended sources by planetary atmospheres. Scintillations govern the experimental uncertainty in the deduction of the scale height of the high Martian atmosphere. A density scale height of 9.9 + or - 2.5 km is obtained at an altitude of 74 + or - 8 km above the mean surface. For CO 2 gas, this result corresponds to a temperature of 190 + or - 50 K.

Africano, J.↗

Observation of EAS using a large water tank

Using a large water tank (30 m in diameter, 4.5 m in depth) transition of extensive air showers (EAS) was investigated at Taro (200 m above sea level). There are set 150,0.4 sq m proportional counters on the bottom of the water tank. A conventional EAS array of 25 plastic scintillation detectors was arranged within several tens meter from the water tank. A proportional counter (10x10x200 cc x2) is made of a square shaped pipe of iron. Tungsten wire (100 mu m phi) is stretched tight in the center of the counter. A gas mixture of 90% argon and 10% methane is used at 760 mmHg. About 3000 EAS were obtained through 1 m of water since 1984.

Inoue, K.↗

The energy spectrum of primary cosmic ray electrons from 2 GeV to 200 GeV.

Use of a balloon-borne counter telescope with a gas Cerenkov counter to measure the energy of primary cosmic ray electrons between 2 and 200 GeV. Electrons are identified by the characteristic electron-photon shower which they produce in a 15 radiation length deep stack of high-Z material interleaved with scintillation counters. Calibrations with monoenergetic electrons up to 14 GeV and monoenergetic protons up to 28 GeV from accelerators are used to develop criteria to statistically separate electrons from proton-induced events. The results from six balloon flights (total exposure time 63 hours) are combined to obtain the electron energy spectrum. Up to about 30 GeV, the spectrum measured in this experiment can be directly checked with calibrations and agrees well with results from other experiments. Above this energy, the flux reported in the present work is somewhat higher than the determinations reported by most other authors. An apparent flattening of the energy spectrum above 50 GeV is not regarded as significant. There is no evidence for a steepening of the spectrum at energies below 200 GeV.

Fanselow, J. L.↗

SiPM-matrix readout of two-phase argon detectors using electroluminescence in the visible and near infrared range

Proportional electroluminescence (EL) in noble gases is used in two-phase detectors for dark matter searches to record (in the gas phase) the ionization signal induced by particle scattering in the liquid phase. The “standard” EL mechanism is considered to be due to noble gas excimer emission in the vacuum ultraviolet (VUV). In addition, there are two alternative mechanisms, producing light in the visible and near infrared (NIR) ranges. The first is due to bremsstrahlung of electrons scattered on neutral atoms (“neutral bremsstrahlung”, NBrS). The second, responsible for electron avalanche scintillation in the NIR at higher electric fields, is due to transitions between excited atomic states. In this work, we have for the first time demonstrated two alternative techniques of the optical readout of two-phase argon detectors, in the visible and NIR range, using a silicon photomultiplier matrix and electroluminescence due to either neutral bremsstrahlung or avalanche scintillation. The amplitude yield and position resolution were measured for these readout techniques, which allowed to assess the detection threshold for electron and nuclear recoils in two-phase argon detectors for dark matter searches. To the best of our knowledge, this is the first practical application of the NBrS effect in detection science.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

A portable and monoenergetic 24 keV neutron source based on 124Sb-9Be photoneutrons and an iron filter

A portable monoenergetic 24 keV neutron source based on the 124Sb-9Be photoneutron reaction and an iron filter has been constructed and characterized. The coincidence of the neutron energy from SbBe and the low interaction cross-section with iron (mean free path up to 29 cm) makes pure iron specially suited to shield against gamma rays from 124Sb decays while letting through the neutrons. To increase the 124Sb activity and thus the neutron flux, a >1 GBq 124Sb source was produced by irradiating a natural Sb metal pellet with a high flux of thermal neutrons in a nuclear reactor. The design of the source shielding structure makes for easy transportation and deployment. A hydrogen gas proportional counter is used to characterize the neutrons emitted by the source and a NaI detector is used for gamma background characterization. At the exit opening of the neutron beam, the characterization determined the neutron flux in the energy range 20–25 keV to be 6.00±0.30 neutrons per cm2 per second and the total gamma flux to be 245±8 gammas per cm2 per second (numbers scaled to 1 GBq activity of the 124Sb source). A liquid scintillator detector is demonstrated to be sensitive to neutrons with incident kinetic energies from 8 to 17 keV, so it can be paired with the source as a backing detector for neutron scattering calibration experiments. This photoneutron source provides a good tool for in-situ low energy nuclear recoil calibration for dark matter experiments and coherent elastic neutrino-nucleus scattering experiments.

Dark Matter detectors (WIMPs, axions, etc.)↗

X-ray Scintillating Lanthanide-Based Coordination Polymers

Reported are the syntheses and characterization of 25 lanthanide-containing coordination polymers exhibiting four structure types: type I′: [Ln(TFTP) 1.5 (bpy)] (Ln = La 3+ –Nd 3+ ), type I: [Ln(TFTP) 1.5 (bpy)(H 2 O)] (Ln = Sm 3+ –Lu 3+ ), type II′: [Pr(TFTP) 1.5 (phen)], and type II: [Ln(TFTP) 1.5 (phen)(H 2 O)] (Ln = Nd 3+ –Yb 3+ , excluding Pm). These compounds feature lanthanide metal cations bound to tetrafluoroterephthalate linkers (TFTP) and either, 2,2′-bipyridine (bpy) or 1,10-phenanthroline (phen) capping ligands. Initial calculations using crystallographic data revealed large void spaces, ranging from 86 Å 3 in type I to 333 Å 3 in type II. Yet, adsorption isotherm data indicate very little gas uptake of both materials with a BET surface area of 9 m 2 /g for I-Tb (8) and 19 m 2 /g for II-Tb (20). X-ray irradiation of I-Eu (6), II-Eu (18), I-Tb (8), and II-Tb (20) produced visible red and green emission, respectively. Furthermore, radioluminescence studies of both type I and II with Sm 3+ , Eu 3+ , and Tb 3+ metal centers indicate that both structure types featuring Tb 3+ are brighter than those with Eu 3+ or Sm 3+ . Notably, structure type I with Tb 3+ is the brightest scintillator with a relative luminosity of 1.7× that of bismuth germanate (BGO).

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

An experiment to study the nuclear component of primary cosmic rays

An apparatus has been designed and is being fabricated to study the charge composition, fluxes, and energy spectra of light nuclei in the energy region from 1 GeV to 100 GeV. The apparatus essentially consists of an array of a large number of particle detectors operated in coincidence and serving as a charged particle telescope. A mosaic silicon semiconductor detector, a plastic scintillation counter and a lucite Cerenkov detector are used to measure the charges of the incident nuclei. Two one-inch thick CsI detectors are used to study low energy particles. An ionization spectrometer is utilized to measure primary energies in the 1 to 100 GeV energy interval. A gas Cerenkov counter is being designed to distinguish between electrons and protons. It is planned to calibrate the apparatus at an accelerator using particles of known energy.

Paul, J. M.↗

Studies of Light and Charge Produced by Alpha-Particles in High-Pressure Xenon

The results of measurements of scintillation light induced by alpha-particles in high-pressure Xe are presented. The ratio of N(sub ex)/N(sub i) and the intensity and time characteristics of the luminescence signal have been measured for different densities up to 0.74 g/cc. The role and mechanisms of the electron-ion recombination in high-pressure gas have been investigated. The existence of clusters and self-trapped excitons above 0.6 g/cc has been observed and discussed. This work is a part of a development program of high-pressure Xe detectors for low-energy gamma rays.

Bolotnikov, Aleksey↗