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All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

Benchmarking of X‐Ray Fluorescence Microscopy with Ion Beam Implanted Samples Showing Detection Sensitivity of Hundreds of Atoms

Abstract Single impurities in insulators are now often used for quantum sensors and single photon sources, while nanoscale semiconductor doping features are being constructed for electrical contacts in quantum technology devices, implying that new methods for sensitive, non‐destructive imaging of single‐ or few‐atom structures are needed. X‐ray fluorescence (XRF) can provide nanoscale imaging with chemical specificity, and features comprising as few as 100 000 atoms have been detected without any need for specialized or destructive sample preparation. Presently, the ultimate limits of sensitivity of XRF are unknown – here, gallium dopants in silicon are investigated using a high brilliance, synchrotron source collimated to a small spot. It is demonstrated that with a single‐pixel integration time of 1 s, the sensitivity is sufficient to identify a single isolated feature of only 3000 Ga impurities (a mass of just 350 zg). With increased integration (25 s), 650 impurities can be detected. The results are quantified using a calibration sample consisting of precisely controlled numbers of implanted atoms in nanometer‐sized structures. The results show that such features can now be mapped quantitatively when calibration samples are used, and suggest that, in the near future, planned upgrades to XRF facilities might achieve single‐atom sensitivity.

36 MATERIALS SCIENCE↗
DOE OSTI2022

Autoencoders for semivisible jet detection

The production of dark matter particles from confining dark sectors may lead to many novel experimental signatures. Depending on the details of the theory, dark quark production in proton-proton collisions could result in semivisible jets of particles: collimated sprays of dark hadrons of which only some are detectable by particle collider experiments. The experimental signature is characterised by the presence of reconstructed missing momentum collinear with the visible components of the jets. This complex topology is sensitive to detector inefficiencies and mis-reconstruction that generate artificial missing momentum. With this work, we propose a signal-agnostic strategy to reject ordinary jets and identify semivisible jets via anomaly detection techniques. A deep neural autoencoder network with jet substructure variables as input proves highly useful for analyzing anomalous jets. The study focuses on the semivisible jet signature; however, the technique can apply to any new physics model that predicts signatures with anomalous jets from non-SM particles.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2023

Probing an MeV-scale scalar boson in association with a TeV-Scale top-quark partner at the LHC

Searches for new low-mass matter and mediator particles have actively been pursued at fixed target experiments and at e + e - colliders. It is challenging at the CERN LHC, but they have been searched for in Higgs boson decays and in B meson decays by the ATLAS and CMS Collaborations, as well as in a low transverse momentum phenomena from forward scattering processes (e.g., FASER). We propose a search for a new scalar particle in association with a heavy vector-like quark. We consider the scenario in which the top quark (t) couples to a light scalar φ' and a heavy vector-like top quark T. We examine single and pair production of T in pp collisions, resulting in a final state with a top quark that decays purely hadronically, a T which decays semileptonically (T → W + b → ℓ ν b), and a φ' that is very boosted and decays to a pair of collimated photons which can be identified as a merged photon system. The proposed search is expected to achieve a discovery reach with signal significance greater than 5σ (3σ) for m(T) as large as 1.8 (2) TeV and m(φ') as small as 1 MeV, assuming an integrated luminosity of 3000 fb -1 . This search can expand the reach of T, and demonstrates that the LHC can probe low-mass, MeV-scale particles.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2025

Search for Higgs boson decays into a pair of pseudoscalar particles in the γγτhadτhad final state using pp collisions at s = 13 TeV with the ATLAS detector

A search for exotic decays of the 125 GeV Higgs boson into a pair of new spin-0 particles, H → aa, where one decays into a photon pair and the other into a τ-lepton pair, is presented. Hadronic decays of the τ-leptons are considered and reconstructed using a dedicated tagger for collimated τ-lepton pairs. The search uses 140 fb−1 of proton-proton collision data at a centre-of-mass energy of s$$ \sqrt{s} $$ = 13 TeV recorded between 2015 and 2018 by the ATLAS experiment at the Large Hadron Collider. The search is performed in the mass range of the a boson between 10 GeV and 60 GeV. No significant excess of events is observed above the Standard Model background expectation. Model-independent upper limits at 95% confidence level are set on the branching ratio of the Higgs boson to the γγττ final state, B$$ \mathcal{B} $$(H → aa → γγττ), ranging from 0.2% to 2%, depending on the a-boson mass hypothesis.

Aad, G↗
DOE OSTI2022

Search for a heavy resonance decaying into a top quark and a W boson in the lepton+jets final state at $\sqrt{s}$ = 13 TeV

A search for a heavy resonance decaying into a top quark and a W boson in proton-proton collisions at $\sqrt{s}$ = 13 TeV is presented. The data analyzed were recorded with the CMS detector at the LHC and correspond to an integrated luminosity of 138 fb -1 . The top quark is reconstructed as a single jet and the W boson, from its decay into an electron or muon and the corresponding neutrino. A top quark tagging technique based on jet clustering with a variable distance parameter and simultaneous jet grooming is used to identify jets from the collimated top quark decay. The results are interpreted in the context of two benchmark models, where the heavy resonance is either an excited bottom quark b* or a vector-like quark B. A statistical combination with an earlier search by the CMS Collaboration in the all-hadronic final state is performed to place upper cross section limits on these two models. The new analysis extends the lower range of resonance mass probed from 1.4 down to 0.7 TeV. For left-handed, right-handed, and vector-like couplings, b* masses up to 3.0, 3.0, and 3.2 TeV are excluded at 95% confidence level, respectively. The observed upper limits represent the most stringent constraints on the b* model to date.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2023

Jet thermalization in QCD kinetic theory

We perform numerical studies in the framework of QCD kinetic theory to investigate the energy and angular profiles of a high energy parton — as a proxy for a jet produced in heavy ion collisions — passing through a Quark-Gluon Plasma (QGP). We find that the fast parton loses energy to the plasma mainly via a radiative turbulent quark and gluon cascade that transports energy locally from the jet down to the temperature scale where dissipation takes place. In this first stage of the system time evolution, the angular structure of the turbulent cascade is found to be relatively collimated. However, when the lost energy reaches the plasma temperature it is rapidly transported to large angles w.r.t. the jet axis and thermalizes. We investigate the contribution of the soft jet constituents to the total jet energy. We show that for jet opening angles of about 0.3 rad or smaller, the effect is negligible. Conversely, larger opening angles become more and more sensitive to the thermal component of the jet and thus to medium response. Our result showcases the importance of the jet cone size in mitigating or enhancing the details of dissipation in jet quenching observables.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Search for high-mass $Wγ$ and $Zγ$ resonances using hadronic $W/Z$ boson decays from 139 fb –1 of $pp$ collisions at $\sqrt{s}$ = 13 TeV with the ATLAS detector

A search for high-mass charged and neutral bosons decaying to $Wγ$ and $Zγ$ final states is presented in this paper. The analysis uses a data sample of $\sqrt{s}$ = 13 TeV proton-proton collisions with an integrated luminosity of 139 fb –1 collected by the ATLAS detector during LHC Run 2 operation. The sensitivity of the search is determined using models of the production and decay of spin-1 charged bosons and spin-0/2 neutral bosons. The range of resonance masses explored extends from 1.0 TeV to 6.8 TeV. At these high resonance masses, it is beneficial to target the hadronic decays of the $W$ and $Z$ bosons because of their large branching fractions. The decay products of the high-momentum $W/Z$ bosons are strongly collimated and boosted-boson tagging techniques are employed to improve the sensitivity. No evidence of a signal above the Standard Model backgrounds is observed, and upper limits on the production cross-sections of these bosons times their branching fractions to $Wγ$ and $Zγ$ are derived for various boson production models.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2025

A robust search for lepton flavour violating axions at Mu3e

We propose a search at Mu3e for lepton flavor violating axion(-like) particles in μ → 3e + a decays. By requiring an additional e+e− pair from internal conversion, one can circumvent the calibration challenges which plague the μ → e + a channel for axions lighter than 20 MeV. Crucially, the corresponding reduction in signal rate is to a large extent compensated for by Mu3e’s ability to resolve highly collimated tracks. For phase I of Mu3e, we project a sensitivity to decay constants as high as 6 × 109 GeV which probes uncharted parameter space in scenarios of axion dark matter. The sensitivity to axions which couple primarily to right-handed leptons can be further improved by leveraging the polarisation of the muon beam.

Knapen, Simon↗
DOE OSTI2026

Measurement of the jet mass in hadronic decays of boosted W bosons at 13 TeV and extraction of the W boson mass

The jet mass of W bosons decaying to a quark-antiquark pair is measured in W+jets events from proton-proton collisions at a center-of-mass energy of 13 TeV. The data used were collected by the CMS experiment at the CERN LHC and correspond to an integrated luminosity of 138 fb −1 . Hadronic decays of W bosons with high momenta produce strongly collimated decay products due to the large Lorentz boost, and are reconstructed as single large-radius jets. These jets have a characteristic substructure that is exploited to distinguish them from the large background of quark- and gluon-initiated jets. The jet mass is computed using the soft-drop algorithm, which suppresses soft wide-angle radiation that leads to a broadening of the jet mass distribution. For the first time, unfolded measurements are presented of the double-differential W+jets cross section as a function of the jet transverse momentum and soft-drop mass. From these distributions, the W boson mass is obtained, with a value of 80.83 ± 0.55 GeV in a scheme with mass-dependent width, achieving the smallest uncertainty available today from an all-jets final state at a hadron collider.

hadron-hadron scattering↗
DOE OSTI2020

Search for a light pseudoscalar Higgs boson in the boosted $\mu\mu\tau\tau$ final state in proton-proton collisions at $\sqrt{s}=$ 13 TeV

A search for a light pseudoscalar Higgs boson (a) decaying from the 125 GeV (or a heavier) scalar Higgs boson (H) is performed using the 2016 LHC proton-proton collision data at $ \sqrt{s} $ = 13 TeV, corresponding to an integrated luminosity of 35.9 fb$^{−1}$, collected by the CMS experiment. The analysis considers gluon fusion and vector boson fusion production of the H, followed by the decay H → aa → μμττ, and considers pseudoscalar masses in the range 3.6 < m$_{a}$< 21 GeV. Because of the large mass difference between the H and the a bosons and the small masses of the a boson decay products, both the μμ and the ττ pairs have high Lorentz boost and are collimated. The ττ reconstruction efficiency is increased by modifying the standard technique for hadronic τ lepton decay reconstruction to account for a nearby muon. No significant signal is observed. Model-independent limits are set at 95% confidence level, as a function of m$_{a}$, on the branching fraction (ℬ) for H → aa → μμττ, down to 1.5 (2.0) × 10$^{−4}$ for m$_{H}$ = 125 (300) GeV. Model-dependent limits on ℬ(H → aa) are set within the context of two Higgs doublets plus singlet models, with the most stringent results obtained for Type-III models. These results extend current LHC searches for heavier a bosons that decay to resolved lepton pairs and provide the first such bounds for an H boson with a mass above 125 GeV.[graphic not available: see fulltext]

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2020

Jet substructure from dark sector showers

We examine the robustness of collider phenomenology predictions for a dark sector scenario with QCD-like properties. Pair production of dark quarks at the LHC can result in a wide variety of signatures, depending on the details of the new physics model. A particularly challenging signal results when prompt production induces a parton shower that yields a high multiplicity of collimated dark hadrons with subsequent decays to Standard Model hadrons. The final states contain jets whose substructure encodes their non-QCD origin. This is a relatively subtle signature of strongly coupled beyond the Standard Model dynamics, and thus it is crucial that analyses incorporate systematic errors to account for the approximations that are being made when modeling the signal. We estimate theoretical uncertainties for a canonical substructure observable designed to be sensitive to the gauge structure of the underlying object, the two-point energy correlator $ {e}_2^{\left(\beta \right)} $ , by computing envelopes between resummed analytic distributions and numerical results from Pythia. We explore the separability against the QCD background as the confinement scale, number of colors, number of flavors, and dark quark masses are varied. Additionally, we investigate the uncertainties inherent to modeling dark sector hadronization. Simple estimates are provided that quantify one’s ability to distinguish these dark sector jets from the overwhelming QCD background. Such a search would benefit from theory advances to improve the predictions, and the increase in statistics using the data to be collected at the high luminosity LHC.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2024

The metamorphosis of semi-classical mechanisms of confinement: from monopoles on ℝ 3 × S 1 to center-vortices on ℝ 2 × T 2

There are two distinct regimes of Yang-Mills theory where we can demonstrate confinement, the existence of a mass gap, and the multi-branch structure of the effective potential as a function of the theta angle using a reliable semi-classical calculation. The two regimes are deformed Yang-Mills theory on ℝ 3 × S 1 , and Yang-Mills theory on ℝ 2 × T 2 where the torus is threaded by a ’t Hooft flux. The weak coupling regime is ensured by the small size of the circle or torus. In the first case the confinement mechanism is related to self-dual monopoles, whereas in the second case self-dual center-vortices play a crucial role. These two topological objects are distinct. In particular, they have different mutual statistics with Wilson loops. On the other hand, they carry the same topological charge and action. We consider the theory on ℝ × T 2 × S 1 and extrapolate both the monopole and vortex regimes to a quantum mechanical domain, where a cross-over takes place. Both sides of the cross-over are described by a deformed ℤ N TQFT. On ℝ 2 × S 1 × S 1 , we derive an effective field theory (EFT) of vortices from the EFT of monopoles in the presence of a ’t Hooft flux. This construction is based on a two-stage Higgs mechanism, reducing SU(N) to U(1) N−1 in 3d first, followed by reduction to a ℤ N EFT in 2d in the second step. This result shows how monopoles transmute into center-vortices, and suggests adiabatic continuity between the two confinement mechanisms. The basic mechanism is flux fractionalization: the magnetic flux of the monopoles splits up and is collimated in such a way that 2d Wilson loops detect it as a center vortex.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Scalable Detector Design for a High-Resolution Fast-Neutron Radiography Panel

Development of a scalable flat-panel neutron radiography device is needed to meet the nondestructive testing needs of a growing industrial market. Flood field images from a Cs-137 gamma source and a Cf-252 fission neutron source were generated using a detector composed of a 3-mm-thick sheet of EJ-200, and 3-mm-thick sheet of acrylic light spreader, an 8 $\times$ 8 array of SensL MICROFJ-60035-TSV SiPMs, and an IDEAS ROSSPAD readout module. The readout module can be tiled together with similar systems to create a panel of any size, and is only limited by the number of available Ethernet ports in a switching system. A collimated gamma line image demonstrated a 90% spatial resolution of approximately 0.47 line pairs per centimeter and a 10% spatial resolution of approximately 2.32 line pairs per centimeter. A neutron edge image demonstrated a 90% spatial resolution of approximately 0.70 line pairs per centimeter and a 10% spatial resolution of approximately 3.35 line pairs per centimeter. Both of these images show the ability to generate radiographs with sub-SiPM spatial resolution. Using these readout modules, a large-scale radiographic panel can be developed by tiling ROSSPAD modules together.

36 MATERIALS SCIENCE↗
DOE OSTI2021

Radiation damage of a two-dimensional carbon fiber composite (CFC)

Carbon fiber composites (CFC) are, among other applications, already in use as low-impedance collimating elements for intercepting TeV-level protons machines, like the CERN Large Hadron Collider. Towards a comprehensive understanding of these materials’ properties and behavior, a series of radiation damage campaigns have been undertaken in order to quantitively investigate the response of AC-150 K CFC to high proton fluences. The CFCs dimensional changes, stability, micro-structural evolution, and structural integrity below and above 5 × 10 20 p/cm 2 fluence threshold were studied. The irradiating particles were protons of kinetic energies in the range of 130–200 MeV. The effects of the irradiation temperature (~90–180°C and 280–500°C) combined with the proton fluence on the dimensional stability and the microstructural evolution of this anisotropic two-dimensional composite structure were studied using precision dilatometry and X-ray diffraction. Our results shed light on the fluence-based limitations for these composite materials. Furthermore, we compare these results with reference unirradiated graphite, and we discuss the similarities and differences in the dimensional changes and post-irradiation annealing properties.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Quantitative investigation of sooting dynamics in droplet combustion using an automated image analysis algorithm

This paper reports an image analysis approach using a newly-developed open-source program to extract quantitative measurements of soot volume fraction (SVF) from digital video images of burning n-heptane droplets. The automated program developed in this work can analyze images of fixed and untethered droplets to quantify sooting dynamics. The images analyzed in the program were taken from experiments carried out in the Multi-user Droplet Combustion Apparatus (MDCA) onboard the International Space Station (ISS). In these experiments, video imaging of burning droplets was obtained using backlighting by a laser diode with a wavelength of 653 nm. Here, the light was collimated before it passed through the droplet and soot-containing region, after which the light was then attenuated and projected onto the camera’s sensors. This technique facilitates the measurements of SVF based on the principles of the full field light extinction method (FFLEM). The measurements provide quantitative data that reveal the sooting dynamics of liquid fuels during droplet combustion processes. The analyses of a soot-attenuating image (ISS n-heptane, untethered droplet) at an instant during the burning show that the SVF distribution has a peak at the soot shell location. It then decreases due to soot oxidation when the location is further away from the burning droplet. Regarding temporal effects on the maximum SVF (SVF max ), results show that SVF max first increases after the burning is initiated until a peak value is reached, after which SVF max decreases. The SVF max values identified in this study for n-heptane are quantitatively consistent with previously reported values for fiber-supported droplets and are reached relatively early in the burning history. n-Heptane images are also analyzed to show the effects of initial droplet sizes on the maximum soot volume fraction. Results show that SVF max decreases with increasing initial droplet size, which is consistent with visual observations of less soot formed and dimmer flame brightness as Do increases.

42 ENGINEERING↗
DOE OSTI2024

Cobalt-60, Barium-133, Cesium-137, and Europium-152 migration from cementitious sources through sediment under field conditions

Safe and effective storage of radioactive waste is essential to protect human and environmental health. Due to the potential for accidental releases and the severity of the associated risks, it is imperative to further understand radionuclide transport should an accident occur. This study was the second set of measurements conducted in 2022 of an ongoing experiment that has analyzed the vadose zone migration of radionuclides from cementitious wasteforms at the Savannah River Site over the last ten years. The radionuclides introduced within the sources are prominent constituents of radioactive waste or analogs for other groups or series of radionuclides. Lysimeters were first analyzed in 2016 using a collimated high-purity germanium gamma-ray spectrometer to non-destructively measure the concentration of each radionuclide in the sediment column as a function of depth. Following these measurements, the lysimeters were redeployed for another 4 years. All radionuclides in all lysimeters were observed to transport further during the redeployment period; however, the extent of migration varied with the material used for introduction. Except for 137Cs, migration through the sediment control system increased with decreasing ionic potential (ionic charge/radius); migration order: 152Eu<137Cs<60Co<133Ba. Overall, the cementitious wasteforms were observed to decrease radionuclide migration extent relative to natural vadose zone conditions. In both cementitious wasteforms, the migration extent increased in the order 152Eu<133Ba<60Co<137Cs. However, less migration was measured when the radionuclides were incorporated into a reducing grout wasteform. The novelty of this paper is the demonstration of a technique capable of creating non-destructive measurements over decade time scales. Ultimately, this work provides insight into the long-term migration of alkali, alkali earth, divalent transition metal, and trivalent (e.g., lanthanide and actinide element) isotopes.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2023

$In-situ$ synchrotron x-ray diffraction and thermal expansion of TiB2 up to ~3050 °C

There is an increasing interest in understanding the performance and properties of ultra-high temperature ceramics due to their high melting points (<3000 °C) that make them promising for extreme environment applications. In-situ high temperature X-ray diffraction experiments were performed on TiB 2 beads up to ~3050 °C. For these experiments, TiB 2 powders were fabricated into spherical beads via gel casting methods and densified in a high temperature graphite furnace. These sample beads were then levitated in a conical nozzle levitator with reducing atmosphere (3% H 2 -Ar) while being heated using a 400 W CO 2 laser. During levitation a collimated synchrotron X-ray source was used to perform in-situ, temperature-dependent structural characterizations. The anisotropic coefficients of thermal expansion of TiB 2 were characterized as a function of temperature up to ~3050 °C. Elucidation of these properties are critical for the advancement of TiB 2 ceramics and other transition metal di-borides for use in high temperature applications such as hypersonic platforms, nuclear reactors, and atmospheric re-entry.

36 MATERIALS SCIENCE↗
DOE OSTI2022

Persistent mysteries of jet engines, formation, propagation, and particle acceleration: Have they been addressed experimentally?

Here, the physics of astrophysical jets can be divided into three regimes: (i) engine and launch (ii) propagation and collimation, (iii) dissipation and particle acceleration. Since astrophysical jets comprise a huge range of scales and phenomena, practicality dictates that most studies of jets intentionally or inadvertently focus on one of these regimes, and even therein, one body of work may be simply boundary condition for another. We first discuss long standing persistent mysteries that pertain the physics of each of these regimes, independent of the method used to study them. This discussion makes contact with frontiers of plasma astrophysics more generally. While observations theory, and simulations, and have long been the main tools of the trade, what about laboratory experiments? Jet related experiments have offered controlled studies of specific principles, physical processes, and benchmarks for numerical and theoretical calculations. We discuss what has been accomplished on these fronts. Although experiments have indeed helped us to understand certain processes, proof of principle concepts, and benchmarked codes, they have yet to solved an astrophysical jet mystery on their own. A challenge is that experimental tools used for jet-related experiments so far, are typically not machines originally designed for that purpose, or designed with specific astrophysical mysteries in mind. This presents an opportunity for a different way of thinking about the development of future platforms: start with the astrophysical mystery and build an experiment to address it.

79 ASTRONOMY AND ASTROPHYSICS↗