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At least 163 records · Page 9

Chemical consequences of the initial diffusional growth of cloud droplets - A clean marine case

A simple microphysical cloud parcel model and a simple representation of the background marine aerosol are used to predict the concentrations and compositions of droplets of various sizes near cloud base. The aerosol consists of an externally-mixed ammonium bisulfate accumulation mode and a sea-salt coarse particle mode. The difference in diffusional growth rates between the small and large droplets as well as the differences in composition between the two aerosol modes result in substantial differences in solute concentration and composition with size of droplets in the parcel. The chemistry of individual droplets is not, in general, representative of the bulk (volume-weighted mean) cloud water sample. These differences, calculated to occur early in the parcel's lifetime, should have important consequences for chemical reactions such as aqueous phase sulfate production.

Twohy, C. H.↗

Modeling the Impact of Drizzle and 3D Cloud Structure on Remote Sensing of Effective Radius

Remote sensing of cloud particle size with passive sensors like MODIS is an important tool for cloud microphysical studies. As a measure of the radiatively relevant droplet size, effective radius can be retrieved with different combinations of visible through shortwave infrared channels. MODIS observations sometimes show significantly larger effective radii in marine boundary layer cloud fields derived from the 1.6 and 2.1 pm channel observations than for 3.7 pm retrievals. Possible explanations range from 3D radiative transport effects and sub-pixel cloud inhomogeneity to the impact of drizzle formation on the droplet distribution. To investigate the potential influence of these factors, we use LES boundary layer cloud simulations in combination with 3D Monte Carlo simulations of MODIS observations. LES simulations of warm cloud spectral microphysics for cases of marine stratus and broken stratocumulus, each for two different values of cloud condensation nuclei density, produce cloud structures comprising droplet size distributions with and without drizzle size drops. In this study, synthetic MODIS observations generated from 3D radiative transport simulations that consider the full droplet size distribution will be generated for each scene. The operational MODIS effective radius retrievals will then be applied to the simulated reflectances and the results compared with the LES microphysics.

Platnick, Steven↗

Cloud properties as deduced from satellite observation

The three major accomplishments of this project are presented. The first was the simultaneous observations from both satellite and in situ aircraft of the effects of ship exhaust on cloud microphysics and the consequent changes in cloud reflectivity. Second, the satellite observations collected during the FIRE marine stratocumulus intensive field operation (IFO) were analyzed to reveal differences in the reflectivities of uniform and broken clouds. Third, the relationship between liquid water path and cloud reflectivity was examined.

Coakley, James A., Jr.↗

Statistical Analyses of Satellite Cloud Object Data from CERES: Comparison with Cloud-Resolving Model Simulations of Tropical Convective Clouds - Part III

The present study evaluates the ability of a cloud-resolving model (CRM) to simulate the physical properties of tropical deep convective cloud objects identified from a Clouds and the Earth s Radiant Energy System (CERES) data product. The emphasis of this study is the comparisons among the small-, medium- and large-size categories of cloud objects observed during March 1998 and between the large-size categories of cloud objects observed during March 1998 (strong El Ni o) and March 2000 (weak La Ni a). Results from the CRM simulations are analyzed in a way that is consistent with the CERES retrieval algorithm and they are averaged to match the scale of the CERES satellite footprints. Cloud physical properties are analyzed in terms of their summary histograms for each category. It is found that there is a general agreement in the overall shapes of all cloud physical properties between the simulated and observed distributions. Each cloud physical property produced by the CRM also exhibits different degrees of disagreement with observations over different ranges of the property. The simulated cloud tops are generally too high and cloud top temperatures are too low except for the large-size category of March 1998. The probability densities of the simulated top-of-the-atmosphere (TOA) albedos for all four categories are underestimated for high albedos, while those of cloud optical depth are overestimated at its lowest bin. These disagreements are mainly related to uncertainties in the cloud microphysics parameterization and inputs such as cloud ice effective size to the radiation calculation. Summary histograms of cloud optical depth and TOA albedo from the CRM simulations of the large-size category of cloud objects do not differ significantly between the March 1998 and 2000 periods, consistent with the CERES observations. However, the CRM is unable to reproduce the significant differences in the observed cloud top height while it overestimates the differences in the observed outgoing longwave radiation and cloud top temperature between the two periods. Comparisons between the CRM results and the observations for most parameters in March 1998 consistently show that both the simulations and observations have larger differences between the large- and small-size categories than between the large- and medium-size, or between the medium- and small-size categories. However, the simulated cloud properties do not change as much with size as observed. These disagreements are likely related to the spatial averaging of the forcing data and the mismatch in time and in space between the numerical weather prediction model from which the forcing data are produced and the CERES observed cloud systems.

Luo, Yali↗

Microphysical development of a pulsating cumulus tower - A case study

In-cloud microphysical data collected within a 22-minute period during seven consecutive passes at the -13 C sampling level of a deep (base +22 C) convective cloud provide observational evidence for a secondary ice production mechanism at work in the Florida environment. The observed microphysical characteristics of the convective tower, particularly the spatial distribution and habit of the ice phase relative to the updraft, are consistent with a rime-splintering hypothesis for secondary ice production. It is shown that the cloud's updraft structure is critically important in governing the timing of the ice production by controlling the flux of graupel particles through the critical temperature zone (-3 C to -8 C). The importance of the cloud's pulsation growth dynamics on the microphysics is emphasized, particularly as it relates to rapidly glaciating cumuli.

Keller, V. W.↗

Cirrus clouds and climate feedback: Is the sky falling and should we go tell the king

It is widely believed that thin cirrus clouds act to enhance the greenhouse effect owing to a particular combination of their optical properties. It is demonstrated how this effect is perhaps based on inadequate resolution of the physics of cirrus clouds and that the more likely impact of cirrus clouds to climate change remains somewhat elusive. These conclusions are developed within the context of a specific feedback mechanism incorporated into a simple mechanistic climate model. A specific scientific question addressed is whether or not the observed relationship between the ice water content and temperature of cirrus provides any significant feedback to the CO2 greenhouse warming. A related question also examined concerns the specific role of cloud microphysics and radiation in this feedback. This raises several pertinent issues about the understanding of cirrus clouds and their likely role in climate change as there presently exists a considerable uncertainty about the microphysics of these clouds (size and shape of ice crystals) and their radiative influences.

Stephens, Graeme L.↗

Simulations of Aerosol Microphysics in the NASA GEOS-5 Model

Aerosol-cloud-chemistry interactions have potentially large but uncertain impacts on Earth's climate. One path to addressing these uncertainties is to construct models that incorporate various components of the Earth system and to test these models against data. To that end, we have previously incorporated the Goddard Chemistry, Aerosol, Radiation, and Transport (GOCART) module online in the NASA Goddard Earth Observing System model (GEOS-5). GEOS-5 provides a platform for Earth system modeling, incorporating atmospheric and ocean general circulation models, a land surface model, a data assimilation system, and treatments of atmospheric chemistry and hydrologic cycle. Including GOCART online in this framework has provided a path for interactive aerosol-climate studies; however, GOCART only tracks the mass of aerosols as external mixtures and does not include the detailed treatments of aerosol size distribution and composition (internal mixtures) needed for aerosol-cloud-chemistry-climate studies. To address that need we have incorporated the Community Aerosol and Radiation Model for Atmospheres (CARMA) online in GEOS-5. CARMA is a sectional aerosol-cloud microphysical model, capable of treating both aerosol size and composition explicitly be resolving the aerosol distribution into a variable number of size and composition groupings. Here we present first simulations of dust, sea salt, and smoke aerosols in GEOS-5 as treated by CARMA. These simulations are compared to available aerosol satellite, ground, and aircraft data and as well compared to the simulated distributions in our current GOCART based system.

Colarco, Peter↗

New Concepts for Refinement of Cumulus Parameterization in GCM's the Arakawa-Schubert Framework

Several state-of-the-art models including the one employed in this study use the Arakawa-Schubert framework for moist convection, and Sundqvist formulation of stratiform. clouds, for moist physics, in-cloud condensation, and precipitation. Despite a variety of cloud parameterization methodologies developed by several modelers including the authors, most of the parameterized cloud-models have similar deficiencies. These consist of: (a) not enough shallow clouds, (b) too many deep clouds; (c) several layers of clouds in a vertically demoralized model as opposed to only a few levels of observed clouds, and (d) higher than normal incidence of double ITCZ (Inter-tropical Convergence Zone). Even after several upgrades consisting of a sophisticated cloud-microphysics and sub-grid scale orographic precipitation into the Data Assimilation Office (DAO)'s atmospheric model (called GEOS-2 GCM) at two different resolutions, we found that the above deficiencies remained persistent. The two empirical solutions often used to counter the aforestated deficiencies consist of a) diffusion of moisture and heat within the lower troposphere to artificially force the shallow clouds; and b) arbitrarily invoke evaporation of in-cloud water for low-level clouds. Even though helpful, these implementations lack a strong physical rationale. Our research shows that two missing physical conditions can ameliorate the aforestated cloud-parameterization deficiencies. First, requiring an ascending cloud airmass to be saturated at its starting point will not only make the cloud instantly buoyant all through its ascent, but also provide the essential work function (buoyancy energy) that would promote more shallow clouds. Second, we argue that training clouds that are unstable to a finite vertical displacement, even if neutrally buoyant in their ambient environment, must continue to rise and entrain causing evaporation of in-cloud water. These concepts have not been invoked in any of the cloud parameterization schemes so far. We introduced them into the DAO-GEOS-2 GCM with McRAS (Microphysics of Clouds with Relaxed Arakawa-Schubert Scheme).

Sud, Y. C.↗

What does Reflection from Cloud Sides tell us about Vertical Distribution of Cloud Droplet Sizes?

Cloud development, the onset of precipitation and the effect of aerosol on clouds depend on the structure of the cloud profiles of droplet size and phase. Aircraft measurements of cloud profiles are limited in their temporal and spatial extent. Satellites were used to observe cloud tops not cloud profiles with vertical profiles of precipitation-sized droplets anticipated from CloudSat. The recently proposed CLAIM-3D satellite mission (cloud aerosol interaction mission in 3-D) suggests to measure profiles of cloud microphysical properties by retrieving them from the solar and infrared radiation reflected or emitted from cloud sides. Inversion of measurements from the cloud sides requires rigorous understanding of the 3-dimentional(3-D) properties of clouds. Here we discuss the reflected sunlight from the cloud sides and top at two wavelengths: one nonabsorbing to solar radiation (0.67 microns) and one with liquid water efficient absorption of solar radiation (2.1 microns). In contrast to the plane-parallel approximation, a conventional approach to all current operational retrievals, 3-D radiative transfer is used for interpreting the observed reflectances. General properties of the radiation reflected from the sides of an isolated cloud are discussed. As a proof of concept, the paper shows a few examples of radiation reflected from cloud fields generated by a simple stochastic cloud model with the prescribed vertically resolved microphysics. To retrieve the information about droplet sizes, we propose to use the probability density function of the droplet size distribution and its first two moments instead of the assumption about fixed values of the droplet effective radius. The retrieval algorithm is based on the Bayesian theorem that combines prior information about cloud structure and microphysics with radiative transfer calculations.

Marshak, A.↗

What Does Reflection from Cloud Sides Tell Us About Vertical Distribution of Cloud Droplet Sizes?

Cloud development, the onset of precipitation and the effect of aerosol on clouds depend on the structure of the cloud profiles of droplet size and phase. Aircraft measurements of cloud profiles are limited in their temporal and spatial extent. Satellites were used to observe cloud tops not cloud profiles with vertical profiles of precipitation-sized droplets anticipated from Cloudsat. The recently proposed CLAIM-3D satellite mission (cloud aerosol interaction mission in 3D) suggests to measure profiles of cloud microphysical properties by retrieving them from the solar and infrared radiation reflected or emitted from cloud sides. Inversion of measurements from the cloud sides requires rigorous understanding of the 3-dimensional (3D) properties of clouds. Here we discuss the reflected sunlight from the cloud sides and top at two wavelengths: one nonabsorbing to solar radiation (0.67 micrometers) and one with liquid water efficient absorption of solar radiation (2.1 micrometers). In contrast to the plane-parallel approximation, a conventional approach to all current operational retrievals, 3D radiative transfer is used for interpreting the observed reflectances. General properties of the radiation reflected from the sides of an isolated cloud are discussed. As a proof of concept, the paper shows a few examples of radiation reflected from cloud fields generated by a simple stochastic cloud model with the prescribed vertically resolved microphysics. To retrieve the information about droplet sizes, we propose to use the probability density function of the droplet size distribution and its first two moments instead of the assumption about fixed values of the droplet effective radius. The retrieval algorithm is based on the Bayesian theorem that combines prior information about cloud structure and microphysics with radiative transfer calculations.

Marshak, Alexander↗

Atmospheric Cloud Physics Laboratory thermal control

The paper presents the development background and the present status of the Atmospheric Cloud Physics Laboratory (ACPL) thermal control capability. The ACPL, a Spacelab payload, is currently in the initial flight hardware development phase for a first flight scheduled in June 1981. The ACPL is intended as a facility for conducting a wide variety of cloud microphysics experimentation under zero gravity conditions. The cloud chambers, which are key elements of the ACPL, have stringent thermal requirements. Thus the expansion chamber inner walls must be uniform to within + or - 0.1 C during both steady-state and transient operation over a temperature range of +30 to -25 C. Design progression of the expansion chamber, from early in-house NASA-MSFC concepts (including test results of a prototype chamber) to a thermal control concept currently under development, is discussed.

Moses, J. L.↗

A global radiative-convective feedback

We have investigated the sensitivity of the intensity of convective activity and atmospheric radiative cooling to radiatively thick upper-tropospheric clouds using a new version of the Colorado State University General Circulation Model (CSU GCM). The model includes a bulk cloud microphysics scheme to predict the formation of cloud water, cloud ice, rain, and snow. The cloud optical properties are interactive and dependent upon the cloud water and cloud ice paths. We find that the formation of a persistent upper tropospheric cloud ice shield leads to decreased atmospheric radiative cooling and increased static stability. Convective activity is then strongly suppressed. In this way, upper-tropospheric clouds act as regulators of the global hydrologic cycle, and provide a negative feedback between atmospheric radiative cooling and convective activity.

Fowler, Laura D.↗

Remote Sensing of In-Flight Icing Conditions: Operational, Meteorological, and Technological Considerations

Remote-sensing systems that map aircraft icing conditions in the flight path from airports or aircraft would allow icing to be avoided and exited. Icing remote-sensing system development requires consideration of the operational environment, the meteorological environment, and the technology available. Operationally, pilots need unambiguous cockpit icing displays for risk management decision-making. Human factors, aircraft integration, integration of remotely sensed icing information into the weather system infrastructures, and avoid-and-exit issues need resolution. Cost, maintenance, power, weight, and space concern manufacturers, operators, and regulators. An icing remote-sensing system detects cloud and precipitation liquid water, drop size, and temperature. An algorithm is needed to convert these conditions into icing potential estimates for cockpit display. Specification development requires that magnitudes of cloud microphysical conditions and their spatial and temporal variability be understood at multiple scales. The core of an icing remote-sensing system is the technology that senses icing microphysical conditions. Radar and microwave radiometers penetrate clouds and can estimate liquid water and drop size. Retrieval development is needed; differential attenuation and neural network assessment of multiple-band radar returns are most promising to date. Airport-based radar or radiometers are the most viable near-term technologies. A radiometer that profiles cloud liquid water, and experimental techniques to use radiometers horizontally, are promising. The most critical operational research needs are to assess cockpit and aircraft system integration, develop avoid-and-exit protocols, assess human factors, and integrate remote-sensing information into weather and air traffic control infrastructures. Improved spatial characterization of cloud and precipitation liquid-water content, drop-size spectra, and temperature are needed, as well as an algorithm to convert sensed conditions into a measure of icing potential. Technology development also requires refinement of inversion techniques. These goals can be accomplished with collaboration among federal agencies including NASA, the FAA, the National Center for Atmospheric Research, NOAA, and the Department of Defense. This report reviews operational, meteorological, and technological considerations in developing the capability to remotely map in-flight icing conditions from the ground and from the air.

Ryerson, Charles C.↗

Radiative Impacts of Cloud Heterogeneity and Overlap in an Atmospheric General Circulation Model

The radiative impacts of introducing horizontal heterogeneity of layer cloud condensate, and vertical overlap of condensate and cloud fraction are examined with the aid of a new radiation package operating in the GEOS-5 Atmospheric General Circulation Model. The impacts are examined in terms of diagnostic top-of-the-atmosphere shortwave (SW) and longwave (LW) cloud radiative effect (CRE) calculations for a range of assumptions and parameter specifications about the overlap. The investigation is conducted for two distinct cloud schemes, the one that comes with the standard GEOS-5 distribution, and another which has been recently used experimentally for its enhanced GEOS-5 distribution, and another which has been recently used experimentally for its enhanced cloud microphysical capabilities; both are coupled to a cloud generator allowing arbitrary cloud overlap specification. We find that cloud overlap radiative impacts are significantly stronger for the operational cloud scheme for which a change of cloud fraction overlap from maximum-random to generalized results to global changes of SW and LW CRE of approximately 4 Watts per square meter, and zonal changes of up to approximately 10 Watts per square meter. This is because of fewer occurrences compared to the other scheme of large layer cloud fractions and of multi-layer situations with large numbers of atmospheric being simultaneously cloudy, conditions that make overlap details more important. The impact on CRE of the details of condensate distribution overlap is much weaker. Once generalized overlap is adopted, both cloud schemes are only modestly sensitive to the exact values of the overlap parameters. We also find that if one of the CRE components is overestimated and the other underestimated, both cannot be driven towards observed values by adjustments to cloud condensate heterogeneity and overlap alone.

Oreopoulos, L.↗

TPSAS-NF1676L-32084-DND

We present aerosol and cloud observations obtained from the satellite-, aircraft- and ship-based measurements of the North Atlantic Aerosols and Marine Ecosystems Study (NAAMES). The data span three seasons (November 2015, May 2016, and September 2017), which correspond to substantial variation in ocean ecosystem characteristics, continental long-range transport, and local aerosol-cloud microphysics and meteorology. For example, below-cloud aerosol number concentrations in November 2015 were of order 10-50 cm-3, while concentrations observed in May and September were of order 100-500 cm-3. Here, we focus on 20 cloud sampling flight modules carried out during NAAMES, which encompass approximately 27 flight hours of the more than 220 NAAMES project flight hours. The nominal cloud module pattern consists of a series of 5-6 vertically-stacked, horizontal flight legs of 10-15 minute duration (~50-90 km in length) that profile the near-surface (300 ft. altitude) and below-cloud aerosol characteristics, the cloud properties near cloud base and top, the aerosol properties above cloud, and finally a high-altitude remote sensing leg that characterizes the cloud top and above-cloud atmosphere. Ship-based aerosol and ceilometer measurements provide the below-cloud context over time, while GOES satellite imagery and cloud retrieval products fill in the above-cloud story.

Richard H Moore↗

Cirrus microphysics and infrared radiative transfer: A case study

Coincident measurements of cirrus cloud microphysical properties such as particle size distribution and particle shape and morphology, and measurements of infrared intensity and flux were made. Data was acquired nearly simultaneously in space and time by a KingAir in cloud and by an ER-2 at an altitude of 19 km. Upwelling infrared intensities and fluxes measured from the ER-2 and observations of cloud particle size distributions and particle phase and morphology made from the KingAir are discussed. Broad-band flux measurements were available both in and below the cirrus layer from the KingAir.

Ackerman, Thomas P.↗

Sensitivity of Boreal-Summer Circulation and Precipitation to Atmospheric Aerosols in Selected Regions: The Americas - Part 2

Aerosol perturbations over selected land regions are imposed in Version-4 of the Goddard Earth Observing System (GEOS-4) general circulation model (GCM) to assess the influence of increasing aerosol concentrations on regional circulation patterns and precipitation in four selected regions: India, Africa, and North and South America. Part 1 of this paper addresses the responses to aerosol perturbations in India and Africa. This paper presents the same for aerosol perturbations over the Americas. GEOS-4 is forced with prescribed aerosols based on climatological data, which interact with clouds using a prognostic scheme for cloud microphysics including aerosol nucleation of water and ice cloud hydrometeors. In clear-sky conditions the aerosols interact with radiation. Thus the model includes comprehensive physics describing the aerosol direct and indirect effects on climate (hereafter ADE and AIE respectively). Each simulation is started from analyzed initial conditions for 1 May and was integrated through June-July-August of each of the six years: 1982 1987 to provide a 6-ensemble set. Results are presented for the difference between simulations with double the climatological aerosol concentration and one-half the climatological aerosol concentration for three experiments: two where the ADE and AIE are applied separately and one in which both the ADE and AIE are applied. The ADE and AIE both yield reductions in net radiation at the top of the atmosphere and surface while the direct absorption of shortwave radiation contributes a net radiative heating in the atmosphere. A large net heating of the atmosphere is also apparent over the subtropical North Atlantic Ocean that is attributable to the large aerosol perturbation imposed over Africa. This atmospheric warming and the depression of the surface pressure over North America contribute to a northward shift of the inter-Tropical Convergence Zone over northern America, an increase in precipitation over Central America and the Caribbean, and an enhancement of convergence in the North American monsoon region.

Wilcox, E. M.↗