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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 163 records · Page 9
All sourcesNASA NTRSDOE OSTI
DOE OSTI2020

Random Polymerization Strategy Leads to a Family of Donor Polymers Enabling Well‐Controlled Morphology and Multiple Cases of High‐Performance Organic Solar Cells

Abstract Developing high‐performance donor polymers is important for nonfullerene organic solar cells (NF‐OSCs), as state‐of‐the‐art nonfullerene acceptors can only perform well if they are coupled with a matching donor with suitable energy levels. However, there are very limited choices of donor polymers for NF‐OSCs, and the most commonly used ones are polymers named PM6 and PM7, which suffer from several problems. First, the performance of these polymers (particularly PM7) relies on precise control of their molecular weights. Also, their optimal morphology is extremely sensitive to any structural modification. In this work, a family of donor polymers is developed based on a random polymerization strategy. These polymers can achieve well‐controlled morphology and high‐performance with a variety of chemical structures and molecular weights. The polymer donors are D–A1–D–A2‐type random copolymers in which the D and A1 units are monomers originating from PM6 or PM7, while the A2 unit comprises an electron‐deficient core flanked by two thiophene rings with branched alkyl chains. Consequently, multiple cases of highly efficient NF‐OSCs are achieved with efficiencies between 16.0% and 17.1%. As the electron‐deficient cores can be changed to many other structural units, the strategy can easily expand the choices of high‐performance donor polymers for NF‐OSCs.

Liang, Jiaen↗
DOE OSTI2023

A Superconducting Micro-Magnetometer for Quantum Vortex in Superconducting Nanoflakes

Superconducting quantum interferometer device (SQUID) plays a key role in understanding electromagnetic properties and emergent phenomena in quantum materials. The technological appeal of SQUID is that its detection accuracy for the electromagnetic signal can precisely reach the quantum level of a single magnetic flux. However, conventional SQUID techniques normally can only be applied to a bulky sample and do not have the capability to probe the magnetic properties of micro-scale samples with small magnetic signals. Here, in this paper, it is demonstrated that, based on a specially designed superconducting nano-hole array, the contactless detection of magnetic properties and quantized vortices in micro-sized superconducting nanoflakes is realized. An anomalous hysteresis loop and a suppression of Little–Parks oscillation are observed in the detected magnetoresistance signal, which originates from the disordered distribution of the pinned vortices in Bi 2 Sr 2 CaCu 2 O 8+δ . Therefore, the density of pinning centers of the quantized vortices on such micro-sized superconducting samples can be quantitatively evaluated, which is technically inaccessible for conventional SQUID detection. The superconducting micro-magnetometer provides a new approach to exploring mesoscopic electromagnetic phenomena of quantum materials.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2023

Design and Synthesis of Cubic K 3−2 x Ba x SbSe 4 Solid Electrolytes for K–O 2 Batteries

Developing K-ion conducting solid-state electrolytes (SSEs) plays a critical role in the safe implementation of potassium batteries. In this work, a chalcogenide-based potassium ion SSE is reported, K 3 SbSe 4 , which adopts a trigonal structure at room temperature. Single-crystal structural analysis reveals a trigonal-to-cubic phase transition at the low temperature of 50 °C, which is the lowest among similar compounds and thus provides easy access to the cubic phase. The substitution of barium for potassium in K 3 SbSe 4 leads to the creation of potassium vacancies, expansion of lattice parameters, and a transformation from a trigonal phase to a cubic phase. As a result, the maximum conductivity of K 3−2x Ba x SbSe 4 reaches around 0.1 mS cm −1 at 40 °C for K 2.2 Ba 0.4 SbSe 4 , which is over two orders of magnitude higher than that of undoped K 3 SbSe 4 . This novel SSE is successfully employed in a K–O 2 battery operating at room temperature where a polymer-laminated K 2.2 Ba 0.4 SbSe 4 pellet serves as a separator between the oxygen cathode and the potassium metal anode. Effective protection of the K metal anode against corrosion caused by O 2 is demonstrated.

25 ENERGY STORAGE↗
DOE OSTI2026

Complete Phase Transformation of Ir Nanowire Network into Defect-Rich Oxide Catalyst for High-Performance PEM Water Electrolysis

Iridium-based catalysts remain the most reliable option for the oxygen evolution reaction (OER) in proton exchange membrane water electrolyzers (PEMWEs). However, their high cost and limited performance represent critical barriers to the commercialization of this green hydrogen production technology. Herein, we report the creation of a metallic Ir nanowire network (IrNWN), which exhibits superior OER performance through its in-situ transition into an oxide structure with high intrinsic activity. At a low loading of 0.25 mgIr/cm2 in PEMWEs, IrNWN achieved a current density of 3.13 A/cm2 at a cell voltage of 1.8 V, outperforming the commercial Ir-based catalyst and surpassing the Department of Energy (DOE) 2026 technical target. Moreover, the high activity of IrNWN was maintained for 900 hours in a durability test at 2 A/cm2, showing a low degradation rate of 0.042 mV/hour. Structural analysis of the electrochemically oxidized IrNWN revealed the presence of mixed Ir oxidation states and a high density of surface terminal oxygen groups (μ1-O), which contributed to a reduced energy barrier for the rate-determining O-O coupling step.

oxygen evolution reaction↗
DOE OSTI2024

Measurement of prompt D + and ${D}_s^{+}$ production in p Pb collisions at $\sqrt{s_{NN}}$ = 5.02 TeV

The production of prompt D + and $D^+_s$ mesons is studied in proton-lead collisions at a centre-of-mass energy of $\sqrt{^{S}NN}$ = 5.02 TeV. The data sample corresponding to an integrated luminosity of (1.58 ± 0.02)nb –1 is collected by the LHCb experiment at the LHC. The differential production cross-sections are measured using D + and $D^+_s$ candidates with transverse momentum in the range of 0 < p T < 14 GeV/c and rapidities in the ranges of 1.5 < y* < 4.0 and –5.0 < y* < –2.5 in the nucleon-nucleon centre-of-mass system. For both particles, the nuclear modification factor and the forward-backward production ratio are determined. These results are compared with theoretical models that include initial-state nuclear effects. In addition, measurements of the cross-section ratios between D + , $D^+_s$ and D 0 mesons are presented, providing a baseline for studying the charm hadronization in lead-lead collisions at LHC energies.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2024

Measurement of the Z boson production cross-section in pp collisions at $ \sqrt{s}$ = 5.02 TeV

The first measurement of the Z boson production cross-section at centre-of-mass energy $\sqrt{s}$ = 5.02 TeV in the forward region is reported, using pp collision data collected by the LHCb experiment in year 2017, corresponding to an integrated luminosity of 100 ± 2 pb –1 . The production cross-section is measured for final-state muons in the pseudorapidity range 2.0 < η < 4.5 with transverse momentum p T > 20 GeV/c. The integrated cross-section is determined to be ${\sigma}_{Z\to \mu +\mu -}=39.6\pm 0.7\left(\textrm{stat}\right)\pm 0.6\left(\textrm{syst}\right)\pm 0.8\left(\textrm{lumi}\right)\textrm{pb}$ for the di-muon invariant mass in the range 60 < M μμ < 120 GeV/c 2 . This result and the differential cross-section results are in good agreement with theoretical predictions at next-to-next-to-leading order in the strong coupling constant. Based on a previous LHCb measurement of the Z boson production cross-section in pPb collisions at $\sqrt{s_{NN}}$ = 5.02 TeV, the nuclear modification factor RpPb is measured for the first time at this energy. The measured values are ${1.2}_{-0.3}^{+0.5}$ (stat) ± 0.1(syst) in the forward region (1.53 < ${y}_{\mu}^{\ast }$ < 4.03) and ${3.6}_{-0.9}^{+1.6}$ (stat) ± 0.2(syst) in the backward region (–4.97 < ${y}_{\mu}^{\ast }$ < –2.47), where ${y}_{\mu}^{\ast }$ represents the muon rapidity in the centre-of-mass frame.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2022

Study of charmonium and charmonium-like contributions in $\mathrm{B}^+$ → $\mathrm{J/ψηK^+}$ decays

A study of B+ → J/ψηK + decays, followed by J/ψ → μ + μ – and η → γγ, is performed using a dataset collected with the LHCb detector in proton-proton collisions at centre-of-mass energies of 7, 8 and 13 TeV, corresponding to an integrated luminosity of 9 fb –1 The J/ψη mass spectrum is investigated for contributions from charmonia and charmonium-like states. Evidence is found for the B + →(ψ2(3823) → J/ψη)K + and B + → (ψ(4040) → J/ψη)K + decays with significance of 3.4 and 4.7 standard deviations, respectively. This constitutes the first evidence for the ψ 2 (3823) → J/ψη decay.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2023

Measurement of CP asymmetries in ${D}_{(s)}^{+}\to \eta {\pi}^{+}$ and ${D}_{(s)}^{+}\to {\eta}^{\prime }{\pi}^{+}$ decays

Searches for CP violation in the decays ${D}_{(s)}^{+}\to \eta {\pi}^{+}$ and ${D}_{(s)}^{+}\to {\eta}^{\prime }{\pi}^{+}$ are performed using pp collision data corresponding to 6 fb –1 of integrated luminosity collected by the LHCb experiment. The calibration channels ${D}_{(s)}^{+}\to \phi {\pi}^{+}$ are used to remove production and detection asymmetries. The resulting CP-violating asymmetries are $\mathcal{A}^{CP} = (D^+ \to ηπ^+) = (0.34 ± 0.66 ± 0.16 ± 0.05)$ %, $\mathcal{A}^{CP} = (D^+_s \to ηπ^+) = (0.32 ± 0.51 ± 0.12)$ %, $\mathcal{A}^{CP} = (D^+ \to η'π^+) = (0.49 ± 0.18 ± 0.06 ± 0.05)$ %, $\mathcal{A}^{CP} = (D^+_s \to η'π^+) = (0.01 ± 0.12 ± 0.08)$ %, where the first uncertainty is statistical, the second is systematic and the third, relevant for the D + channels, is due to the uncertainty on ${\mathcal{A}}^{CP}=\left({D}^{+}\to \phi {\pi}^{+}\right)$. These measurements, currently the most precise for three of the four channels considered, are consistent with the absence of CP violation. A combination of these results with previous LHCb measurements is presented.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2022

Observation of the doubly charmed baryon decay $Ξ_{cc}^{++}$ →$Ξ_c^{'+}π^+$

The $Ξ_{cc}^{++}$ →$Ξ_c^{'+}π^+$ decay is observed using proton-proton collisions collected by the LHCb experiment at a centre-of-mass energy of 13 TeV, corresponding to an integrated luminosity of 5.4 fb –1 . The $Ξ_{cc}^{++}$ →$Ξ_c^{'+}π^+$ decay is reconstructed partially, where the photon from the $Ξ_c^{'+}$ →$Ξ^+_cγ$ decay is not reconstructed and the $ρK^-π^+$ final state of the $Ξ^+_c$ baryon is employed. The $Ξ_{cc}^{++}$ →$Ξ_c^{'+}π^+$ branching fraction relative to that of the $Ξ_{cc}^{++}$ →$Ξ_c^+π^+$ decay is measured to be 1.41 ± 0.17 ± 0.10, where the first uncertainty is statistical and the second systematic.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2022

Search for the decay $B^0$ → $\phiμ^+μ^–$

A search for the decay $B^0$ → $\phiμ^+μ^–$ is performed using proton-proton collisions at centre-of-mass energies of 7, 8, and 13 TeV collected by the LHCb experiment and corresponding to an integrated luminosity of 9 fb –1 . No evidence for the $B^0$ → $\phiμ^+μ^–$ decay is found and an upper limit on the branching fraction, excluding the $\phi$ and charmonium regions in the dimuon spectrum, of 4.4 × 10 –3 at a 90% credibility level, relative to that of the $B^0_s$ → $\phiμ^+μ^–$ branching fraction and assuming a phase-space model, the absolute branching fraction of the $B^0$ → $\phiμ^+μ^–$ in the full q 2 range is determined to be less than 3.2 x 10 –9 at a 90% credibility level.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2024

Measurements of the branching fraction ratio $$ \mathcal{B}\left(\phi \to {\mu}^{+}{\mu}^{-}\right)/\mathcal{B}\left(\phi \to {\textrm{e}}^{+}{\textrm{e}}^{-}\right) $$ with charm meson decays

Abstract Measurements of the branching fraction ratio$$ \mathcal{B}\left(\phi \to {\mu}^{+}{\mu}^{-}\right)/\mathcal{B}\left(\phi \to {e}^{+}{e}^{-}\right) $$ B ϕ → μ + μ − / B ϕ → e + e − with$$ {D}_s^{+}\to {\pi}^{+}\phi $$ D s + → π + ϕ andD + → π + ϕdecays, denoted$$ {R}_{\phi \pi}^s $$ R ϕπ s and$$ {R}_{\phi \pi}^d $$ R ϕπ d , are presented. The analysis is performed using a dataset corresponding to an integrated luminosity of 5.4 fb −1 ofppcollision data collected with the LHCb experiment. The branching fractions are normalised with respect to theB + →K + J/ψ(→e + e − ) andB + →K + J/ψ(→μ + μ − ) decay modes. The combination of the results yields$$ {R}_{\phi \pi}=1.022\pm 0.012\left(\textrm{stat}\right)\pm 0.048\left(\textrm{syst}\right). $$ R ϕπ = 1.022 ± 0.012 stat ± 0.048 syst . The result is compatible with previous measurements of theϕ→ℓ + ℓ − branching fractions and predictions based on the Standard Model.

Physics↗
DOE OSTI2023

Measurement of the Z boson production cross-section in proton-lead collisions at $\sqrt{s_{\textrm{NN}}}$ = 8.16 TeV

This article presents the first measurement of the differential Z-boson production cross-section in the forward region using proton-lead collisions with the LHCb detector. The dataset was collected at a nucleon-nucleon centre-of-mass energy of $\sqrt{s_{NN}}$ = 8.16 TeV in 2016, corresponding to an integrated luminosity of 30.8 nb –1 . The forward-backward ratio and the nuclear modification factors are measured together with the differential cross-section as functions of the Z boson rapidity in the centre-of-mass frame, the transverse momentum of the Z boson and a geometric variable $\phi$*. The results are in good agreement with the predictions from nuclear parton distribution functions, providing strong constraining power at small Bjorken-x.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2023

Amplitude analysis of the $D^+$ → $π^-π^+π^+$ decay and measurement of the $π^-π^+$ S-wave amplitude

An amplitude analysis of the $D^+$ → $π^-π^+π^+$ decay is performed with a sample corresponding to 1.5 fb -1 of integrated luminosity of $pp$ collisions at a centre-of-mass energy $\sqrt{s}$ = 8 TeV collected by the LHCb detector in 2012. The sample contains approximately six hundred thousand candidates with a signal purity of 95%. The resonant structure is studied through a fit to the Dalitz plot where the $π^-π^+$ S-wave amplitude is extracted as a function of $π^-π^+$ mass, and spin-1 and spin-2 resonances are included coherently through an isobar model. The S-wave component is found to be dominant, followed by the $ρ(770)^0π^+$ and $f_2(1270)π^+$ components. A small contribution from the $ω$(782) → $π^-π^+$ decay is seen for the first time in the $D^+$ → $π^-π^+π^+$ decay.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2023

Search for the lepton-flavour violating decays B0 → K *0 μ ± e ∓ and ${B}_s^0$ → Φμ ± e ∓

A search for the lepton-flavour violating decays B 0 → K *0 μ ± e ∓ and \( {B}_s^0 \) → Φμ ± e ∓ is presented, using proton-proton collision data collected by the LHCb detector at the LHC, corresponding to an integrated luminosity of 9 fb - 1 . No significant signals are observed and upper limits of $$ {\displaystyle \begin{array}{c}\mathcal{B}\left({B}^0\to {K}^{\ast 0}{\mu}^{+}{e}^{-}\right)<5.7\times {10}^{-9}\left(6.9\times {10}^{-9}\right),\\ {}\mathcal{B}\left({B}^0\to {K}^{\ast 0}{\mu}^{-}{e}^{+}\right)<6.8\times {10}^{-9}\left(7.9\times {10}^{-9}\right),\\ {}\mathcal{B}\left({B}^0\to {K}^{\ast 0}{\mu}^{\pm }{e}^{\mp}\right)<10.1\times {10}^{-9}\left(11.7\times {10}^{-9}\right),\\ {}\mathcal{B}\left({B}_s^0\to \phi {\mu}^{\pm }{e}^{\mp}\right)<16.0\times {10}^{-9}\left(19.8\times {10}^{-9}\right)\end{array}} $$ are set at 90% (95%) confidence level. These results constitute the world’s most stringent limits to date, with the limit on the decay \( {B}_s^0 \) → Φμ ± e ∓ the first being set. In addition, limits are reported for scalar and left-handed lepton-flavour violating New Physics scenarios.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2023

Measurement of the ${\Lambda}_c^{+}$ to D 0 production ratio in peripheral PbPb collisions at $\sqrt{s_{\textrm{NN}}}$ = 5.02 TeV

We report on a measurement of the ${\Lambda}_c^{+}$ to D 0 production ratio in peripheral PbPb collisions at $\sqrt{s_{\textrm{NN}}}$ = 5.02 TeV with the LHCb detector in the forward rapidity region 2 < y < 4.5. The ${\Lambda}_c^{+}$ (D 0 ) hadrons are reconstructed via the decay channel ${\Lambda}_c^{+}$ → pK – π + (D 0 → K – π + ) for 2 < p T < 8 GeV/c and in the centrality range of about 65–90%. The results show no significant dependence on p T , y or the mean number of participating nucleons. They are also consistent with similar measurements obtained by the LHCb collaboration in pPb and Pbp collisions at $\sqrt{s_{\textrm{NN}}}$ = 5.02 TeV. The data agree well with predictions from PYTHIA in pp collisions at $\sqrt{s}$ = 5 TeV but are in tension with predictions of the Statistical Hadronization model.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2023

Search for the lepton-flavour violating decays B 0 → K *0 τ ± μ ∓

A first search for the lepton-flavour violating decays B 0 → K*0 τ ± μ ∓ is presented. The analysis is performed using a sample of proton-proton collision data, collected with the LHCb detector at centre-of-mass energies of 7, 8 and 13 TeV between 2011 and 2018, corresponding to an integrated luminosity of 9 fb –1 . No significant signal is observed, and upper limits on the branching fractions are determined to be B (B 0 → K* 0 τ + μ – ) < 1.0(1.2) x 10 –5 and B(B 0 → K* 0 τ – μ + ) < 8.2(9.8) x 10 –6 at the 90% (95%) confidence level.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2023

Study of exclusive photoproduction of charmonium in ultra-peripheral lead-lead collisions

The cross-sections of exclusive (coherent) photoproduction J/ψ and ψ(2S) mesons in ultra-peripheral PbPb collisions at a nucleon-nucleon centre-of-mass energy of 5.02 TeV are measured using a data sample corresponding to an integrated luminosity of 228 ± 10 µb -1 , collected by the LHCb experiment in 2018. The differential cross-sections are measured separately as a function of transverse momentum and rapidity in the nucleus-nucleus centre-of-mass frame for J/ψ and ψ(2S) mesons. The integrated cross-sections are measured to be $σ^{coh}_{J/ψ}$ = 5.965 ± 0.059 ± 0.232 ± 0.262 mb and $σ^{coh}_{ψ(2S)}$ = 0.923 ± 0.086 ± 0.028 ± 0.040 mb, where the first listed uncertainty is statistical, the second systematic and the third due to the luminosity determination. The cross-section ratio is measured to be $σ^{coh}_{ψ(2S)}$/$σ^{coh}_{J/ψ}$ = 0.155 ± 0.014 ± 0.003, where the first uncertainty is statistical and the second is systematic. These results are compatible with theoretical predictions.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2023

Measurement of the ratio of branching fractions $\mathcal{B}\left({B}_c^{+}\to {B}_s^0{\pi}^{+}\right)/\mathcal{B}\left({B}_c^{+}\to J/\psi {\pi}^{+}\right)$

The ratio of branching fractions of ${B}_c^{+}\to {B}_s^0{\pi}^{+}$ and ${B}_c^{+}\to J/\psi {\pi}^{+}$ decays is measured with proton-proton collision data of a centre-of-mass energy of 13 TeV. The data were collected with the LHCb experiment during 2016–2018, corresponding to an integrated luminosity of 5.4 fb –1 . The ${B}_s^0$ mesons are reconstructed via the decays ${B}_s^0\to J/\psi \phi$ and ${B}_s^0\to {D}_s^{-}{\pi}^{+}$. The ratio of branching fractions is measured to be $\mathcal{B}\left({B}_c^{+}\to {B}_s^0{\pi}^{+}\right)/\mathcal{B}\left({B}_c^{+}\to J/\psi {\pi}^{+}\right)=91\pm 10\pm 8\pm 3$ where the first uncertainty is statistical, the second is systematic and the third is due to the knowledge of the branching fractions of the intermediate state decays.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗