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At least 163 records · Page 9
All sourcesNASA NTRSDOE OSTI
DOE OSTI2022

Multi‐Layered Systems for Permanent Geologic Storage of CO 2 at the Gigatonne Scale

Abstract The effectiveness of Carbon Capture and Storage (CCS) as an imperative decarbonization technology relies on the sealing capacity of a fine‐grained caprock to permanently store CO 2 deep underground. Uncertainties in assessing the caprock sealing capacity increase with the spatial and temporal scales and may delay CCS deployment at the gigatonne scale. We have developed a computationally efficient transport model to capture the dynamics of basin‐wide upward CO 2 migration in a multi‐layered setting over geological time scales. We find that massive capillary breakthrough and viscous flow of CO 2 , even through pervasively fractured caprocks, are unlikely to occur and compromise the storage security. Potential leakage from the injection reservoir is hampered by repetitive layering of overlying caprocks. This finding agrees with geologic intuition and should be understandable by the public, contributing to the development of climate policies around this technology with increased confidence that CO 2 will be indefinitely contained in the subsurface.

58 GEOSCIENCES↗
NASA NTRS1976

Definition study for photovoltaic residential prototype system

A parametric sensitivity study and definition of the conceptual design is presented. A computer program containing the solar irradiance, solar array, and energy balance models was developed to determine the sensitivities of solar insolation and the corresponding solar array output at five sites selected for this study as well as the performance of several solar array/battery systems. A baseline electrical configuration was chosen, and three design options were recommended. The study indicates that the most sensitive parameters are the solar insolation and the inverter efficiency. The baseline PST selected is comprised of a 133 sg m solar array, 250 ampere hour battery, one to three inverters, and a full shunt regulator to limit the upper solar array voltage. A minicomputer controlled system is recommended to provide the overall control, display, and data acquisition requirements. Architectural renderings of two photovoltaic residential concepts, one above ground and the other underground, are presented. The institutional problems were defined in the areas of legal liabilities during and after installation of the PST, labor practices, building restrictions and architectural guides, and land use.

Imamura, M. S.↗
NASA NTRS2007

Microbial Extremophiles in Aspect of Limits of Life

During Earth's evolution accompanied by geophysical and climatic changes a number of ecosystems have been formed. These ecosystems differ by the broad variety of physicochemical and biological factors composing our environment. Traditionally, pH and salinity are considered as geochemical extremes, as opposed to the temperature, pressure and radiation that are referred to as physical extremes (Van den Burg, 2003). Life inhabits all possible places on Earth interacting with the environment and within itself (cross species relations). In nature it is very rare when an ecotope is inhabited by a single species. As a rule, most ecosystems contain the functionally related and evolutionarily adjusted communities (consortia and populations). In contrast to the multicellular structure of eukaryotes (tissues, organs, systems of organs, whole organism), the highest organized form of prokaryotic life in nature is the benthic colonization in biofilms and microbial mats. In these complex structures all microbial cells of different species are distributed in space and time according to their functions and to physicochemical gradients that allow more effective system support, self-protection, and energy distribution. In vitro, of course, the most primitive organized structure for bacterial and archaeal cultures is the colony, the size, shape, color, consistency, and other characteristics of which could carry varies specifics on species or subspecies levels. In table 1 all known types of microbial communities are shown (Pikuta et a]., 2005). In deep underground (lithospheric) and deep-sea ecosystems an additional factor - pressure, and irradiation - could also be included in the list of microbial communities. Currently the beststudied ecosystems are: human body (due to the medical importance), and fresh water and marine ecosystems (due to the reason of an environmental safety). For a long time, extremophiles were terra incognita, since the environments with aggressive parameters (compared to the human body temperature, pH, mineralization, and pressure) were considered a priori as a dead zone.

Pikuta, Elena V.↗
DOE OSTI2025

Identifying Potential Geochemical and Microbial Impacts of Hydrogen Storage in a Deep Saline Aquifer

Hydrogen is valuable commodity and a promising energy carrier for variable energy production. Storage of hydrogen may occur through injection of hydrogen or a hydrogen/methane gas blend in subsurface reservoirs. However, the geochemical and biological reactions that may impact the stored hydrogen are not yet understood. Therefore, we collected samples from a deep storage aquifer located in the St. Peter Formation in southern Illinois. The reservoir material was primarily quartz with sulphur and iron deposits, while the major constituents of the fluid were chloride and sulphate. 16S rRNA gene amplicon sequencing revealed a low biomass microbial community that contained no obvious hydrogen-consuming bacteria. Next, we enriched a field sample to increase the biomass and completed a metagenomic analysis, finding a low number of genes present that are associated with hydrogen consumption. Then, we completed a series of reactor experiments under reservoir conditions with 15% H2/85% CH4 gas simulating a short-term hydrogen storage, high withdrawal scenario. We found minimal changes in the geochemistry or microbiology for the reactor experiments. This work suggests that short-term storage may be highly successful, although significant additional work needs to be completed in order to accurately evaluate the risks associated with long-term hydrogen storage scenarios. It is essential we continue to expand our understanding of the dynamics present in saline aquifers and provide new insights into how hydrogen storage may impact underground geological storage environments.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1998

Gale Crater: An Amazonian Impact Crater Lake at the Plateau/Plain Boundary

Gale is a 140-km diameter impact crater located at the plateau/plain boundary in the Aeolis Northeast subquadrangle of Mars (5S/223W). The crater is bordered in the northward direction by the Elysium Basin, and in eastward direction by Hesperian channels and the Aeolis Mensae 2. The crater displays a rim with two distinct erosion stages: (a) though eroded, the south rim of Gale has an apparent crest line visible from the north to the southwest (b) the west and northwest rims are characterized by a strong erosion that, in some places, partially destroyed the rampart, leaving remnant pits embayed in smooth-like deposits. The same type of deposits is observed north, outside Gale, it also borders the Aeolis Mensae, covers the bottom of the plateau scarp, and the crater floor. The central part of Gale shows a 6400 km2 subround and asymmetrical deposit: (a) the south part is composed of smooth material, (b) the north part shows spectacular terraces, streamlines, and channels. The transition between the two parts of the deposit is characterized by a scarp ranging from 200 to 2000 in high. The highest point of the scarp is at the center of the crater, and probably corresponds to a central peak. Gale crater does not show a major channel directly inflowing. However, several large fluvi systems are bordering the crater, and could be at the origin of the flooding of the crater, or have contributed to. One fluvial system is entering the crater by the southwest rim but cannot be accounted alone for the volume of sediment deposited in the crater. This channel erodes the crater floor deposit, and ends in a irregular-shaped and dark albedo feature. Gale crater shows the morphology of a crater filled during sedimentation episodes, and then eroded Part of the lower sediment deposition contained in Gale might be ancient and not only aqueous in origin. According to the regional geologic history, the sedimentary deposit could be a mixture of aeolian and pyroclastic material, and aqueous sedimentary material that can originate both from drainage of the regional subsurface aquifer, and/or from surface flood. The central deposit shows three main levels: (a) the current crater floor (north of Gale), (b) an ancient level about 200 rn higher (south of Gale), and (c) the massive terraced deposits. A crater statistics on the 15,400 kM2 area of the crater floor and deposit [3,41 gave: 259+/-112.4 craters, most of them partly embayed in the sedimentary deposit, and all inferior to 5-km diameter. For superimposed crater population only, the result is 194+/-112. The deduced relative ages ranges from Early to Middle Amazonian. The population of craters are comparable for the three levels, implying that the last sedimentation/erosion episode on Gale was recent and affected the whole crater. The streamlined morphology of the border of the deposit, the layering, the channels, and the terraces are compatible with a significant fluvio-lacustrine history of the site. Multiple levels may suggest different episodes, but the common statistical age of the three levels shows that the last episode involved the whole crater. The origin of the lake water in Gale may have varied in time. Three major contributions have been proposed: (a) the drainage of the regional underground aquifer by Gale crater over an area of 110-km radius around the crater which would have provided approximately 1,600 cubic km of water, (b), surface drainage entering Gale by the south and north rims. In the south, a 250-km long system originates in the cratered uplands in a Noachian crater material plain (Nc), and crosses Hesperian and Amazonian crater material plains (AHc) northward [1]. Several fluvial systems originate in the Aeolis Mensae, east of Gale. They may had two functions in time: to recharge, the underground aquifer in the region of Gale, and to supply surface water in the crater by overspilling the northern rim, and (c) surface floods that originated from the rising of the water level in the Elysium Basin. According to the Amazonian age of Gale's floor, and the erosion direction in the crater, a flood from Elysium Basin is the most likely event to explain the material observed in Gale, and the formation of the last lake. This last flood may have been important enough to flood the central deposit up to about 1400 m above the crater floor, leaving two islands (non stream lined features) at the center of the deposit. Terrace spacing suggests a regular drop of the lake level in time. Fractures in terraces perpendicular to the shoreline can be interpreted either as: (a) the result of the drainage systems during the waning of the lake, or (b) traces of the pressure of an ice-covered sheet associated with subglacial drainage. The presence of a lake of such volume during the Amazonian period is one more evidence that water was still active on Mars relatively recently. Gale crater offers the rare opportunity to unveil a key-period of the martian history. The Amazonian might proved not as cold and dry as previously thought. The presence of large lakes and basins (Elysium Basin is large as the Mediterranean Sea), reinforces the model of an extensive water activity during the Amazonian that has still to be understood in the context of an assumed cooling and drying planet. The sediments and rocks that were left of this period in Gale keep the record of the climatic conditions of the Amazonian and the clues that are missing to understand the climatic evolution of Mars. In addition, Gale crater presents the advantage to be located at the plateau/plain boundary, which has never been studied and contains information about the two main martian geological units. As a conclusion, we propose a table that summarizes the worthiness of a mission in Gale crater, and the expected science return relative to the objectives to be met by the Surveyor Program. Additional information contained in the original.

Cabrol, N. A.↗
DOE OSTI2024

How Rains and Floods Become Groundwater: Understanding Recharge Pathways With Stable and Cosmogenic Isotopes

Anthropogenic climate change leads to increased precipitation intensity and exacerbated droughts in California, challenging the reliability and drought resiliency of water supply. Storing floodwater underground via managed aquifer recharge can mitigate these effects through direct infiltration or streambed infiltration. Seasonally dry streams (arroyos) already play an important part in managing groundwater recharge to the Livermore basin (CA). Understanding how, when and where stormwater and arroyo water infiltrate is critical to effectively utilise this strategy. To track water from recent storms (water year 2022–2023, WY23) into the Livermore Valley Groundwater Basin, we analysed stable water isotopes (δ 18 O and δ 2 H) in combination with naturally occurring radioactive isotopic tracers, sulphur-35 ( 35 S, t ½ = 87 days) and tritium ( 3 H, t ½ = 12.3 years). By comparing measurements of δ 18 O, 35 S and 3 H in arroyos to precipitation and groundwater, we classified the relative age and identified source of recharge to 16 wells near two arroyos. Two wells contained water with recent recharge (from WY23) from local precipitation. One well had recent recharge from variable (precipitation and imported water) sources. One well contained imported water recharge. Three wells contained water from mixed recent and older (pre-WY23) waters, from local precipitation sources. Two wells contained recent recharge from local mine settling ponds. Seven wells had older recharge from local precipitation sources. This combination of isotopes allows us to delineate where local and imported water recharges in this highly managed basin and identify locations where managed aquifer recharge is contributing to rapid groundwater infiltration. Our combined interpretation of isotopic water ages and sources in the context of land use shows that local infiltration of precipitation in open spaces is an important recharge mechanism, in addition to the managed arroyo recharge. Finally, a broader familiarity with 35 S will enable more extensive research on the infiltration of urban floodwaters.

58 GEOSCIENCES↗
NASA NTRS1988

Cultural systems for growing potatoes in space

Higher plants are being evaluated for life support to provide needed food, oxygen and water as well as removal of carbon dioxide from the atmosphere. The successful utilization of plants in space will require the development of not only highly productive growing systems but also highly efficient bioregenerative systems. It will be necessary to recycle all inedible plant parts and all human wastes so that the entire complement of elemental compounds can be reused. Potatoes have been proposed as one of the desirable crops because they are 1) extremely productive, yielding more than 100 metric tons per hectare from field plantings, 2) the edible tubers are high in digestible starch (70%) and protein (10%) on a dry weight basis, 3) up to 80% of the total plant production is in tubers and thus edible, 4) the plants are easily propagated either from tubers or from tissue culture plantlets, 5) the tubers can be utilized with a minimum of processing, and 6) potatoes can be prepared in a variety of different forms for the human diet (Tibbitts et al., 1982). However potatoes have a growth pattern that complicates the development of growing the plants in controlled systems. Tubers are borne on underground stems that are botanically termed 'rhizomes', but in common usage termed 'stolons'. The stolons must be maintained in a dark, moist area with sufficient provision for enlargement of tubers. Stems rapidly terminate in flowers forcing extensive branching and spreading of plants so that individual plants will cover 0.2 m2 or more area. Thus the growing system must be developed to provide an area that is darkened for tuber and root growth and of sufficient size for plant spread. A system developed for growing potatoes, or any plants, in space will have certain requirements that must be met to make them a useful part of a life support system. The system must 1) be constructed of materials, and involve media, that can be reused for many successive cycles of plant growth, 2) involve a minimum quantity of media, 3) contain media that is essentially inert and not oxidize or degrade with use, 4) utilize a recirculating nutrient solution to permit regulation of pH and nutrient concentrations, and 5) be capable of complete automation of all planting, maintenance and harvesting procedures.

NASA Discipline Number 61-10↗
DOE OSTI2020

Recovery and Calibration of Legacy Underground Nuclear Test Seismic Data from the Leo Brady Seismic Network

The Leo Brady Seismic Network (LBSN, originally the Sandia Seismic Network) was established in 1960 by Sandia National Laboratories to monitor underground nuclear tests (UGTs) at the Nevada National Security Site (NNSS, formerly named the Nevada Test Site). The LBSN has been in various configurations throughout its existence, but it has generally been comprised of four to six stations at regional distances (~150–400 km) from the NNSS with approximately evenly spaced azimuthal coverage. Between 1962 and the end of nuclear testing in 1992, the LBSN—and a sister network operated by Lawrence Livermore National Laboratories—was the most comprehensive United States source of regional seismic data of UGTs. Approximately 75% of all UGTs performed by the United States occurred in the predigital era. At that time, LBSN data were transmitted as frequency-modulated (FM) audio over telephone lines to a central location and recorded as analog waveforms on high-fidelity magnetic audio tapes. These tapes have been in dry temperature-stable storage for decades and contain the sole record of this irreplaceable data; full waveforms of LBSN-recorded UGTs from this era were not routinely digitized or otherwise published. We have developed a process to recover and calibrate data from these tapes. First, we play back and digitize the tapes as audio. Next, we demodulate the FM “audio” into individual waveforms. We then estimate the various instrument constants through careful measurement of “weight-lift” tests performed prior to each UGT on each instrument. Finally, these coefficients allow us to scale and shape the derived instrument response of the seismographs and compute poles and zeros. Finally, the result of this process is a digital record of the recorded seismic ground motion in a modern data format, stored in a searchable database. To date, we have digitized tapes from 592 UGTs.

58 GEOSCIENCES↗
DOE OSTI2026

Seismic Event Characterization Using Full Moment Tensors on the Hypersphere

Moment tensor solutions provide insights into the deformation that has occurred in the source region of a seismic event and are therefore of great value in identifying different types of seismic sources, such as when monitoring for underground nuclear tests. Despite this utility, inversion of waveforms recorded by seismometers for their full seismic moment tensor is not yet routine, and development of robust methods to classify events based on this information is in its infancy. Here, we assemble an inventory of 1405 full moment tensor solutions that include explosive, earthquake, and collapse events, and investigate the use of anisotropic probability distribution functions on the 5D hypersphere to discriminate between these sources. Using a Bayesian classifier, we obtain optimal success rates of 98.4% across all events and demonstrate that modification of the prior probabilities provides a natural way to alter the balance between not missing desirable events (such as explosions) versus misclassifying large numbers of undesired events (such as earthquakes). The approach is specifically designed to progress from traditional, bipolar event screening metrics to more generalized event identification across multiple types of seismic sources. Despite current databases containing insufficient numbers of events to definitively demonstrate at present, we also find intriguing evidence of subgroupings within individual source populations on the hypersphere, for example, between chemical and nuclear explosions, raising the potential possibility of discriminating between these event types in the future.

Geosciences↗
DOE OSTI2024

Leveraging Existing Assets for Long Duration Energy Storage

Increased renewables penetration to electrical grid is necessary to reduce overall emissions from the electrical power generation sector. Nonetheless, its integration creates challenges to grid operators who must match the power being generated by intermittent renewables and other traditional energy sources with the demand from consumers, while ensuring the reliability and power quality for the entire system. Energy storage has been proposed as an alternative to natural gas peaking plants and a form to deliver excess renewable energy generation at times of peak demand. For energy storage to provide benefits to end customers (energy consumers), it must be reliable, efficient, and cost effective. The Illinois Sustainable Technology Center (ISTC), one of the surveys that integrate the Prairie Research Institute (PRI), aims to develop a Center for Energy Storage at Existing Assets (CESEA) at UIUC with the participation of Waste Pressure Corp and Ecotek Engineering USA LLC. CESEA will focus on LDES systems that can integrate to existing infrastructure in a manner that reduces the initial capital expenditure and demonstrates the ability to repurpose fossil assets that would otherwise become stranded, to serve the energy transition. CESEA aims to leverage UIUC’s unique facilities to validate LDES systems performance at a relevant operating environment. UIUC’s facilities include a 85-MW combined heat and power (CHP) power plant, two (2) solar PV plants totaling over 18 MWdc of installed capacity, an electrical grid along with a substation at transmission and distribution voltages, a 22-mile gas pipeline network operating at two pressure levels, along with steam and chilled water distribution networks. The new LDES systems will connect to the existing UIUC grid through a new test electrical station, which will have the capacity to accommodate additional connections to test new devices and technologies as part of future CESEA R&D activities. The test electrical station will contain meters, instrumentation, and controls to accurately capture data and allow optimization of control algorithms. CESEA will initially focus on technologies that: i) utilize existing equipment or facilities to perform at least one of the process steps in LDES (charging, storage, or discharging), ii) leverage mature or commercially available components or controls, iii) show potential for cost-leadership in 10+ hour storage at a commercial scale. Initial technologies that were identified to meet these criteria include Compressed Gas Energy Storage (CGES), and TES. CGES stores electricity by raising the pressure of a compressible gas inside a control volume and converting the stored energy to electricity via expansion-generation. CGES is a generalization of CAES that covers any working gas (not just air). A successful CGES demo will help to circumvent many challenges faced by CAES (long development times due to site prospecting, high cost of compression and storage, heat recovery management, etc.) by: 1) utilizing existing infrastructure (compressors, pipelines, underground storage or pressure vessels) used in the transportation and storage of industrial gases for LDES charging and storage; 2) deploying over sites already-developed for industrial applications with minor additional work; 3) leveraging the price structure of commercial industrial gas to cover the costs of electricity used during charging. A previous DOE-sponsored conceptual study (DE-FE-0032018) estimated the levelized cost of energy of a 1.1 MW / 17 MWh CGES system at $0.08/kWh, with a commercial 10x scale system cost estimated at <$0.04/kWh (Giardinella, 2022). The pilot-sized system was estimated to avoid up to 2693 tons of CO2/year.

25 ENERGY STORAGE↗
DOE OSTI2021

EGS Collab Experiment 2: Core Photographs and Descriptions

This submission contains photographs of rock core collected from EGS Collab Experiment 2 (and 3) boreholes. Cores were generally photographed in about 1-foot sections using Nikon D3300 DSLR cameras from two angles about 90 degrees apart, wet and dry. Core photos are provided here in .zip files for each well, organized in subfolders by depth interval. Panoramic photographs of the rock cores as well as description and anomaly logs are also available here.

15 GEOTHERMAL ENERGY↗
DOE OSTI2021

All in the timing: epigenetic control of greening

During germination, the emerging seedling relies on a limited supply of energy and nutrients stored within itself and the seed. This often occurs underground in darkness where seedlings undergo skotomorphogenesis, characterized by hypocotyl elongation, reduced root growth, and small closed cotyledons forming an apical hook to protect the shoot apical meristem as the seedling grows though the soil towards sunlight. Such long and pale dark-grown seedlings are commonly referred to as etiolated (from the French étiolier (to make pale)). However, a seedling must eventually find sunlight and make an irreversible shift to photoautotrophic growth (photomorphogenesis or de-etiolation). This leads to a dramatic change in physiology, including reduced hypocotyl elongation, increased root growth, expansion and unfolding of the cotyledons, and the biogenesis of photosynthetic plastids (i.e. chloroplasts). Furthermore, this shift is accompanied by a massive change in gene expression, with about one-third of genes being reprogrammed. A large amount of the transcriptional response is regulated by the plant photoreceptors (phytochromes and cryptochromes) that activate transcriptional networks. Furthermore, this involves the rapid degradation of PHYTOCHROME INTERACTING FACTORS (PIFs), which are basic helix-loop-helix domain-containing transcription factors that repress photomorphogenesis in the dark.

59 BASIC BIOLOGICAL SCIENCES↗
DOE OSTI2020

Scaling the training of particle classification on simulated MicroBooNE events to multiple GPUs

Measurements in Liquid Argon Time Projection Chamber (LArTPC) neutrino detectors, such as the MicroBooNE detector at Fermilab, feature large, high fidelity event images. Deep learning techniques have been extremely successful in classification tasks of photographs, but their application to LArTPC event images is challenging, due to the large size of the events. Events in these detectors are typically two orders of magnitude larger than images found in classical challenges, like recognition of handwritten digits contained in the MNIST database or object recognition in the ImageNet database. Ideally, training would occur on many instances of the entire event data, instead of many instances of cropped regions of interest from the event data. However, such efforts lead to extremely long training cycles, which slow down the exploration of new network architectures and hyperparameter scans to improve the classification performance. We present studies of scaling a LArTPC classification problem on multiple architectures, spanning multiple nodes. The studies are carried out on simulated events in the MicroBooNE detector. We emphasize that it is beyond the scope of this study to optimize networks or extract the physics from any results here. Institutional computing at Pacific Northwest National Laboratory and the SummitDev machine at Oak Ridge National Laboratory’s Leadership Computing Facility have been used. To our knowledge, this is the first use of state-of-the-art Convolutional Neural Networks for particle physics and their attendant compute techniques onto the DOE Leadership Class Facilities. We expect benefits to accrue particularly to the Deep Underground Neutrino Experiment (DUNE) LArTPC program, the flagship US High Energy Physics (HEP) program for the coming decades.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
NASA NTRS2011

Asia from Space: New Ideas for Exploration

Megafans, also known (incorrectly) as inland deltas, are partial cones of fluvial sediment with radii >~100 km. Each is generated by a formative river avulsing across a lowland. The alluvial tract (channel, levee, overbank, etc.) is the building block for megafans. Planform and sectional analyses, based on SRTM data, reveal their conical, low-angle morphology. Megafans are not geologically rare as often assumed but a normal feature in the hierarchy of fluvial features that is slowly beginning to be understood. Our global survey contains a total of >150 examples worldwide, in all tectonic basin types, with a majority of smaller, more easily distinguished megafans occupying classic foreland basins (54%) which may explain the general view that megafans only form in Himalaya-like foreland basins, especially since the Kosi Megafan in the Indogangetic Plain is one of the best known in the geological literature. Recent research has shown that all actively alluviating basins are occupied by fanlike sediment masses, from the well known smaller and steeper alluvial fan (level 8 in Miall s hierarchy of fluvial forms), to the much larger megafan feature (level 9). A close relationship exists between upland basin size and fan size and slope. Larger upland drainage basins give rise to low-slope megafan sedimentation, which can cover very large areas where the receptacle basin exists individual megafan areas are 10(sup 3-5) square kilometers, and collectively cover 1.2 million square kilometers in South America, for example. The habitat of megafans is now sufficiently well understood that prediction of some modern cryptic megafan locations has been successfully achieved. Underground prediction therefore seems possible, where sufficient data exists. It seems necessary to distinguish megafans from (i) steep, coarse-grained mountain-front alluvial fans which are overwhelmingly coarse-grained, (ii) deltas, since megafans lack distal shoreline processes), and (iii) confined floodplains which lack radial drainage. Numerous other differences can be identified. As a normal component of the modern fluvial environment, megafans must exist in the subsurface. Megafan size, predictable channel patterns of the formative river, and the gradation from coarser to finer sediments from apex to toe of megafans are characteristics that ought to assist in understanding subsurface patterns of hydrocarbon host rocks, and possibly source rocks as well. We show examples from various producing basins. A roughness map of Asia, based on an algorithm developed for Mars, shows megafan landscapes to be dominated by short baseline roughness and low slopes, consistent with megafan-dominated plains worldwide. Interestingly, this a unique signature for a larger continental landform.

Wilkinson, M. Justin↗
DOE OSTI2022

Two-Phase Flow Mechanisms Controlling CO2 Intrusion into Shaly Caprock

Abstract Geologic carbon storage in deep saline aquifers has emerged as a promising technique to mitigate climate change. CO 2 is buoyant at the storage conditions and tends to float over the resident brine jeopardizing long-term containment goals. Therefore, the caprock sealing capacity is of great importance and requires detailed assessment. We perform supercritical CO 2 injection experiments on shaly caprock samples (intact caprock and fault zone) under representative subsurface conditions. We numerically simulate the experiments, satisfactorily reproducing the observed evolution trends. Simulation results highlight the dynamics of CO 2 flow through the specimens with implications to CO 2 leakage risk assessment in field practices. The large injection-induced overpressure drives CO 2 in free phase into the caprock specimens. However, the relative permeability increase following the drainage path is insufficient to provoke an effective advancement of the free-phase CO 2 . As a result, the bulk CO 2 front becomes almost immobile. This implies that the caprock sealing capacity is unlikely to be compromised by a rapid capillary breakthrough and the injected CO 2 does not penetrate deep into the caprock. In the long term, the intrinsically slow molecular diffusion appears to dominate the migration of CO 2 dissolved into brine. Nonetheless, the inherently tortuous nature of shaly caprock further holds back the diffusive flow, favoring safe underground storage of CO 2 over geological time scales.

58 GEOSCIENCES↗
DOE OSTI2022

A Project Lifetime Approach to the Management of Induced Seismicity Risk at Geologic Carbon Storage Sites

The geologic storage of carbon dioxide (CO 2 ) is one method that can help reduce atmospheric CO 2 by sequestering it into the subsurface. Large-scale deployment of geologic carbon storage, however, may be accompanied by induced seismicity. We present a project lifetime approach to address the induced seismicity risk at these geologic storage sites. This approach encompasses both technical and nontechnical stakeholder issues related to induced seismicity and spans the time period from the initial consideration phase to postclosure. These recommendations are envisioned to serve as general guidelines, setting expectations for operators, regulators, and the public. They contain a set of seven actionable focus areas, the purpose of which are to deal proactively with induced seismicity issues. Although each geologic carbon storage site will be unique and will require a custom approach, these general best practice recommendations can be used as a starting point to any site-specific plan for how to systematically evaluate, communicate about, and mitigate induced seismicity at a particular reservoir.

58 GEOSCIENCES↗
DOE OSTI2020

Small to Full Height Scale Comparisons of Cesium Ion Exchange Performance with Crystalline Silicotitanate

The U.S. Department of Energy’s (DOE) Hanford Site houses 56 million gallons of high-level radioactive waste generated from plutonium production from 1944 to 1988. The supernatant waste, currently stored in underground tanks, is intended to be vitrified following filtration and 137 Cs removal at the Hanford Waste Treatment and Immobilization Plant (WTP) Low-Activity Waste (LAW) Vitrification Facility. The WTP Pretreatment Facility will not be operational for several years. The Tank Side Cesium Removal (TSCR) system is a technology demonstration that will remove cesium from tank waste supernate to support directly feeding LAW to the vitrification facility. The 137 Cs removal is important to meet the WTP LAW contract specification and ultimately for creating a contact-handled waste form. The waste acceptance criteria (WAC) limit for the WTP LAW Facility is <3.18E-5 Ci 137 Cs per mole Na. The TSCR system is skid mounted and employs two key technologies: dead end filtration for solids removal and ion exchange (IX) for cesium removal. Filtration is necessary to protect the functionality of the IX columns. The IX process utilizes sodium form crystalline silicotitanate (CST) IX media produced by UOP Honeywell, LLC (Des Plaines, IL) under the product name IONSIV R9140-B, 18 x 50 mesh, in a lead-lag-polish column configuration. Each column contains a CST bed height of 92 inches and a volume of approximately 157 gallons of CST IX media. The full-scale TSCR operation will run at a residence time of 1.9 bed volumes (BV)/h, which results in a superficial velocity of 7.3 cm/min and a flowrate of ~5 gal/min. Column testing at small (2.5% of the full bed height), medium (12% of the full bed height), and full-height scales has been previously conducted to evaluate process variables and scale up performance of Cs exchange onto the CST. Cesium load performances from various sieve cuts at the small scale indicated that a 30-mesh sieve cut be tested to determine if it better reflects the 12% and full-height column performances at the small scale. Two process flowrates were tested in the small-column configuration with <30-mesh CST and simulant solutions. These tests were compared to full-height column tests at the same residence times to assess CST particle size effect on column scaling. Table S.1 summarizes the observed column performance determined for the two flowrates juxtaposed to the previous work with 5.6 M Na simulant at higher scales (used as benchmarks). The WAC breakthroughs between the small and full-height tests at 1.3 BV/h differed by ~59 BVs. The WAC breakthroughs for small, medium, and full-height tests at 1.8 BV/h were consistent at 240 BVs. The 50% Cs breakthroughs were nominally equivalent for all column tests. The common transition zones and onsets of Cs breakthrough at the 1.8 BV/h tests indicated that the Cs mass transfers were equivalent and thus the <30-mesh CST Cs load performance at the small scale successfully modeled that of the full-height system. It is recommended that the <30-mesh CST be used in subsequent 10-mL CST bed tests.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
DOE OSTI2022

Search for NuMI $\mu$DAR Electron Neutrinos in MicroBooNE

Muon Decay-at-Rest ($\mu$DAR) produces electron-neutrinos ($\nu_e$) in the $0$ to $53$ MeV energy range. The given range is especially interesting for its similarity to Supernovae-produced $\nu_e$. The Deep Underground Neutrino Experiment (DUNE) has as one of its main goals to measure Supernovae neutrinos on the occasion of a Galactic Supernova burst. To optimize the chances of detection, a low-energy neutrino-LAr cross-section (XS) measurement is a piece of important information to have at hand. MicroBooNE presents a good opportunity to explore the low-energy $\nu$-LAr detection and XS using the $\mu$DAR neutrinos and therefore develop the tools necessary for DUNE to in is a LArTPC that has been collecting neutrino data since October 2015 from the Booster Neutrino Beam (BNB) and off-axis to the Neutrinos at the Main Injector (NuMI) beam, both copious sources of $\mu$DAR neutrinos. esis, we present a first attempt to measure MeV-scale neutrinos in a LArTPC. To do that, we use specifi c MeV-scale reconstruction tools combined with other traditional reconstruction tools used in MicroBooNE. We discuss the tool's performance, limitations, and provide suggestions on how to improve them. zes looks for $\mu$DAR neutrino- argon charged current interactions in the NuMI Run1 data, that contains $2\times 10^{20}$ POT. We observed $9,176$ signal candidates. The number of expected background events is $8,776$, the majority from cosmic rays. We establish a XS upper limit of $<\sigma> = 1.99\times10^{-37} \textrm{cm}^2 / \textrm{Ar}$, which corresponds to $551.9$ times the nominal prediction from MARLEY, the neutrino generator used in this work. Despite the lack of sensitivity, this work is the first of its kind and sets the foundation for future similar analysis in the future. In the conclusions, we discuss how this results can be further improved in MicroBooNE.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗