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At least 163 records · Page 9

NUMERICAL VERIFICATION OF THE RELAP-7 CORE CHANNEL SINGLE-PHASE MODEL

The RELAP-7 code is the next generation of nuclear reactor system safety analysis code being developed at the Idaho National Laboratory (INL). All the physics in RELAP-7 are fully coupled and the errors resulted from the traditional operator-splitting approach are eliminated. By using 2nd order methods in both time and space and eliminating operator-splitting errors, the numerical error of RELAP-7 can be minimized. Numerical verification is the process to verify the orders of numerical methods. It is an important part of modern verification and validation process. The core channel component in RELAP-7 is designed to simulate coolant flow as well as the conjugated heat transfer between coolant flow and the fuel rod. A special treatment at fuel centerline to avoid numerical singularity for the cylindrical heat conduction in the continuous finite element mesh is discussed. One steady state test case and one fast power up transient test case are utilized for the verification of the core channel model with single-phase flow. Analytical solution for the fuel pin temperature and figures of merit such as peak clad temperature and peak fuel temperature are used to define numerical errors. These cases prove that the mass and energy are well conserved and 2nd order convergence rates for both time and space are achieved in the core channel model.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

FUEL PERFORMANCE STUDIES AT IDAHO NATIONAL LABORATORY MAKING USE OF THE BYRON FUEL SHIPMENT

In December of 2023 a shipment of commercially irradiated fuel rods from the Byron Generating Station in Illinois was successfully shipped to the Materials and Fuels Complex (MFC) at Idaho National Laboratory (INL). The make-up of the rods includes a mix of cladding types from traditional ZirloTM, advanced zirconium alloys, and chrome coated ZirloTM. Burnups range from regular end of life values to over 70 GWd/MTU rod average. The R&D plan for the rods involves multiple projects from developing licensing data for new claddings to integral transient tests to support burnup extension efforts in the United States. The R&D began in early 2024 with the nondestructive examinations of the rods after which they will be sectioned for microscopy, mechanical testing, and analytical chemistry. Additionally, many rod segments will be refabricated into new test pins and inserted into a static water capsule for integral Reactivity Initiated Accident (RIA) and Loss of Coolant Accident (LOCA) testing at the TREAT reactor.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

TREAT neutronics analysis and design support, Part I: Multi-SERTTA

Experiment vehicle design is necessary in preparation for Transient Reactor Test (TREAT) facility restart and the resumption of transient testing to support Accident Tolerant Fuel (ATF) characterization and other future fuels testing requirements. Currently the most mature vehicle design is the Multi-SERTTA (Static Environments Rodlet Transient Test Apparatuses), which can accommodate up to four concurrent rodlet-sized specimens under separate environmental conditions. Robust test vehicle design requires neutronics analyses to support design development, optimization of the power coupling factor (PCF) to efficiently maximize energy generation in the test fuel rodlets, and experiment safety analyses. Calculations were performed to support analysis of a near-final design of the Multi-SERTTA vehicle, the design process for future TREAT test vehicles, and establish analytical practices for upcoming transient test experiments. Models of the Multi-SERTTA vehicle containing typical PWR-fuel rodlets were prepared and neutronics calculations were performed using MCNP6.1 with ENDF/B-VII.1 nuclear data libraries. Calculation of the PCF for reference conditions of a PWR fuel rodlet in clean water at operational temperature and pressure provided results between 1.10 and 1.73 W/g-MW depending on the location of the four Multi-SERTTA units with the stack. Basic changes to the Multi-SERTTA secondary vessel containment and support have minimal impact on PCF; using materials with less neutron absorption can improve expected PCF values, especially in the primary containment. An optimized balance is needed between structural integrity, experiment safety, and energy deposition in the experiment. Type of medium and environmental conditions within the primary vessel surrounding the fuel rodlet can also have a significant impact on resultant PCF values. The estimated reactivity insertion worth into the TREAT core is impacted more by the primary and secondary Multi-SERTTA vehicle structure with the experiment content and contained environment having a near negligible impact on overall system reactivity. Additional calculations were performed to evaluate the peak-to-average assembly powers throughout the TREAT core, as well as the nuclear heat generation for the various structural components of the Multi-SERTTA assembly. Future efforts include the evaluation of flux collars to shape the PCF for individual Multi-SERTTA units during an experiment such as to achieve uniformity in test unit environmental conditions impacted by the non-uniform axial flux/power profile of TREAT. Upon resumption of transient testing, experimental results from both the Multi-SERTTA and Multi-SERTTA-CAL will be compared against calculational results and methods for further optimization and design strategies. (authors)

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

TREAT Neutronics Analysis and Design Support, Part I: Multi-SERTTA

Experiment vehicle design is necessary in preparation for Transient Reactor Test (TREAT) facility restart and the resumption of transient testing to support Accident Tolerant Fuel (ATF) characterization and other future fuels testing requirements. Currently the most mature vehicle design is the Multi-SERTTA (Static Environments Rodlet Transient Test Apparatuses), which can accommodate up to four concurrent rodlet-sized specimens under separate environmental conditions. Robust test vehicle design requires neutronics analyses to support design development, optimization of the power coupling factor (PCF) to efficiently maximize energy generation in the test fuel rodlets, and experiment safety analyses. Calculations were performed to support analysis of a near-final design of the Multi-SERTTA vehicle, the design process for future TREAT test vehicles, and establish analytical practices for upcoming transient test experiments. Models of the Multi-SERTTA vehicle containing typical PWR-fuel rodlets were prepared and neutronics calculations were performed using MCNP6.1 with ENDF/B-VII.1 nuclear data libraries. Calculation of the PCF for reference conditions of a PWR fuel rodlet in clean water at operational temperature and pressure provided results between 1.10 and 1.74 W/g-MW depending on the location of the four Multi-SERTTA units with the stack. Basic changes to the Multi-SERTTA secondary vessel containment and support have minimal impact on PCF; using materials with less neutron absorption can improve expected PCF values, especially in the primary containment. An optimized balance is needed between structural integrity, experiment safety, and energy deposition in the experiment. Type of medium and environmental conditions within the primary vessel surrounding the fuel rodlet can also have a significant impact on resultant PCF values. The estimated reactivity insertion worth into the TREAT core is impacted more by the primary and secondary Multi-SERTTA vehicle structure with the experiment content and contained environment having a near negligible impact on overall system reactivity. Additional calculations were performed to evaluate the peak-to-average assembly powers throughout the TREAT core, as well as the nuclear heat generation for the various structural components of the Multi-SERTTA assembly. Future efforts include the evaluation of flux collars to shape the PCF for individual Multi-SERTTA units during an experiment such as to achieve uniformity in test unit environmental conditions impacted by the non-uniform axial flux/power profile of TREAT. Upon resumption of transient testing, experimental results from both the Multi-SERTTA and Multi-SERTTA-CAL will be compared against calculational results and methods for further optimization and design strategies.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

TREAT Neutronics Analysis and Design Support, Part II: Multi-SERTTA-CAL

Experiment vehicle design is necessary in preparation for Transient Reactor Test (TREAT) facility restart and the resumption of transient testing to support Accident Tolerant Fuel (ATF) characterization and other future fuels testing requirements. Currently the most mature vehicle design is the Multi-SERTTA (Static Environments Rodlet Transient Test Apparatuses), which can accommodate up to four concurrent rodlet-sized specimens under separate environmental conditions. Robust test vehicle design requires neutronics analyses to support design development, optimization of the power coupling factor (PCF) to efficiently maximize energy generation in the test fuel rodlets, and experiment safety analyses. In integral aspect of prior TREAT transient testing was the incorporation of calibration experiments to experimentally evaluate and validate test conditions in preparation of the actual fuel testing. The calibration experiment package established the test parameter conditions to support fine-tuning of the computational models to deliver the required energy deposition to the fuel samples. The calibration vehicle was designed to be as near neutronically equivalent to the experiment vehicle as possible to minimize errors between the calibration and final tests. The Multi-SERTTA-CAL vehicle was designed to serve as the calibration vehicle supporting Multi-SERTTA experimentation. Models of the Multi-SERTTA-CAL vehicle containing typical PWR-fuel rodlets were prepared and neutronics calculations were performed using MCNP6.1 with ENDF/B-VII.1 nuclear data libraries; these results were then compared against those performed for Multi-SERTTA to determine the similarity and possible design modification necessary prior to construction of these experiment vehicles. The estimated reactivity insertion worth into the TREAT core is very similar between the two vehicle designs, with the primary physical difference being a hollow Inconel tube running down the length of the calibration vehicle. Calculations of PCF indicate that on average there is a reduction of approximately 6.3 and 12.6%, respectively, for PWR fuel rodlets irradiated under wet and dry conditions. Changes to the primary or secondary vessel structure in the calibration vehicle can be performed to offset this discrepancy and maintain neutronic equivalency. Current possible modifications to the calibration vehicle include reduction of the primary vessel wall thickness, swapping Zircaloy-4 for stainless steel 316 in the secondary containment, or slight modification to the temperature and pressure of the water environment within the primary vessel. Removal of some of the instrumentation within the calibration vehicle can also serve to slightly increase the PCF. Future efforts include further modification and optimization of the Multi-SERTTA and Multi-SERTTA-CAL designs in preparation of actual TREAT transient testing. Experimental results from both test vehicles will be compared against calculational results and methods to provide validation and support additional neutronics analyses.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

TREAT neutronics analysis and design support, Part II: Multi-SERTTA-CAL

Experiment vehicle design is necessary in preparation for Transient Reactor Test (TREAT) facility restart and the resumption of transient testing to support Accident Tolerant Fuel (ATF) characterization and other future fuels testing requirements. Currently the most mature vehicle design is the Multi-SERTTA (Static Environments Rodlet Transient Test Apparatuses), which can accommodate up to four concurrent rodlet-sized specimens under separate environmental conditions. Robust test vehicle design requires neutronics analyses to support design development, optimization of the power coupling factor (PCF) to efficiently maximize energy generation in the test fuel rodlets, and experiment safety analyses. An integral aspect of prior TREAT transient testing was the incorporation of calibration experiments to experimentally evaluate and validate test conditions in preparation of the actual fuel testing. The calibration experiment package established the test parameter conditions to support fine-tuning of the computational models to deliver the required energy deposition to the fuel samples. The calibration vehicle was designed to be as near neutronically equivalent to the experiment vehicle as possible to minimize errors between the calibration and final tests. The Multi-SERTTA-CAL vehicle was designed to serve as the calibration vehicle supporting Multi-SERTTA experimentation. Models of the Multi-SERTTA-CAL vehicle containing typical PWR-fuel rodlets were prepared and neutronics calculations were performed using MCNP6.1 with ENDF/B-VII.1 nuclear data libraries; these results were then compared against those performed for Multi-SERTTA to determine the similarity and possible design modification necessary prior to construction of these experiment vehicles. The estimated reactivity insertion worth into the TREAT core is very similar between the two vehicle designs, with the primary physical difference being a hollow Inconel tube running down the length of the calibration vehicle. Calculations of PCF indicate that on average there is a reduction of approximately 6 % for PWR fuel rodlets irradiated under both wet and dry conditions. Changes to the primary or secondary vessel structure in the calibration vehicle can be performed to offset this discrepancy and maintain neutronic equivalency. Current possible modifications to the calibration vehicle include reduction of the primary vessel wall thickness, swapping Zircaloy-4 for stainless steel 316 in the secondary containment, or slight modification to the temperature and pressure of the water environment within the primary vessel. Removal of some of the instrumentation within the calibration vehicle can also serve to slightly increase the PCF. Future efforts include further modification and optimization of the Multi-SERTTA and Multi-SERTTA-CAL designs in preparation of actual TREAT transient testing. Experimental results from both test vehicles will be compared against calculational results and methods to provide validation and support additional neutronics analyses. (authors)

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Study on the mechanism of diametral cladding strain and mixed-oxide fuel element breaching in slow-ramp extended overpower transients

Cladding strain caused by fuel/cladding mechanical interaction (FCMI) was evaluated for mixed-oxide fuel elements subjected to 70–90% slow-ramp extended overpower transient tests in the experimental breeder reactor II. Calculated transient-induced cladding strains were correlated with cumulative damage fractions (CDFs) using cladding strength correlations. In a breached high-smeared density solid fuel element with low strength cladding, cladding thermal creep strain was significantly increased to approximately half the transient-induced cladding strain that was considered to be caused by the tertiary creep when the CDF was close to the breach criterion (=1.0), with the remaining strain due to instantaneous plastic deformation. In low-smeared density annular fuel elements, FCMI load was significantly mitigated and resulted in little cladding strain. The CDFs of the annular fuel elements were lower than 0.01 at the end of the overpower transient, indicating a substantial margin to breach. A substantial margin to breach was also maintained in a high-smeared density fuel element with high strength cladding.

99 GENERAL AND MISCELLANEOUS↗

Design of separate-effects In-Pile transient boiling experiments at the $\mathrm{TREAT}$ Facility

The cladding-to-coolant heat transfer during rapid power excursions, such as reactivity-initiated accidents, remains a crucial area of uncertainty in nuclear reactor safety. This uncertainty impacts the ability to accurately predict fuel performance behavior for these conditions. Improving our understanding of transient cladding-to-coolant heat transfer will enhance our ability to model design basis accidents and could increase design and improve safety margins for the current commercial fleet and advanced reactors. To address these issues, the Critical Heat Flux Static Environment Rodlet Transient Test Apparatus (CHF-SERTTA) experiment uses a novel approach with a borated stainless-steel heater rodlet that can replicate cladding temperatures experienced during a design-basis reactivity-initiated accident. The rodlet and experiment is instrumented to provide temperature and thermal-hydraulic conditions throughout the transient. The design of the rodlet allows for separate effect testing that eliminates complexities with a fuel and cladding specimen. We report the experiments have provided data that will be used to improve our understanding of boiling behavior, specifically critical heat flux, under transient conditions.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Preliminary Analysis of Damage to MPFDs Caused by Reactor Pulses

The need for next-generation, accident-tolerant fuels has generated significant interest in the restart of domestic fuels testing at the Transient Reactor Test (TREAT) facility. The TREAT reactor is designed to produce large, transient fluxes that replicate the effects of a wide variety of accident conditions on an irradiated fuel sample. Peak powers generated during short pulses approach 20 GW with a neutron flux of approximately 10{sup 17} n cm{sup -2} s{sup -1}. As part of the restart effort, new vehicle designs are being explored for sample irradiation, including the Static Environment Rodlet Transient Test Apparatus (SERTTA) and variants. As part of the SERTTA designs, micro-pocket fission detectors (MPFDs) are being explored for localized flux measurements before, during, and after transient operations. These detectors are also being considered as part of future, core-wide instrumentation for the TREAT reactor. However, the high fluxes associated with the pulses in the TREAT core present certain thermodynamic concerns given their intensity and the amount of energy they will release within the MPFDs within such a short amount of time. Assuming each fission that occurs in a MPFD results in a fission fragment depositing 85 MeV of energy in the substrate on average and each MPFD has 0.5 μg of natural uranium deposited on it, a 100 ms long pulse in the TREAT reactor at 1017 n cm{sup -2} s{sup -1} flux will produce approximately 4.6 x 10{sup 6} fissions in an MPFD. This pulse deposits 6.3 x 10{sup -5} J in the substrate over a 100 ms duration. That amount of energy is sufficient to melt roughly 33% of the Pt under the UO{sub 2} deposition or a circular spot with a diameter of approximately 860 μm. Of course, the above estimate makes a number of simplifying assumptions and ignores heat transfer, but does serve to illustrate the point that this rapid heating effect could be detrimental to the integrity and life of these in-core MPFDs. To study how these layers are affected by large transient neutron fluxes, five samples were prepared, pre-analyzed, and then subjected to a pulse in the central thimble of the Kansas State University TRIGA Mark II reactor to a peak power of 1.58 GW. After being allowed to decay to safer radiation levels, the sample substrates and coatings were inspected using scanning electron microscopy (SEM) to identify any changes to their surface morphology. Indeed, certain changes were found and are discussed in greater detail in this paper.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Implementation of Weighted Delta-Tracking with Scattering in the Serpent 2 Monte Carlo Code

Serpent 2, a continuous-energy Monte Carlo Reactor physics burnup code developed at the VTT Technical Research Centre of Finland, uses a common rejection sampling technique, known as Woodcock delta-tracking. This method improves the efficiency of Monte Carlo in the complicated geometric layout of nuclear reactors and is widely used despite drawbacks that make it inefficient in specific cases, such as in the presence of strong absorbers. At present, Serpent actively uses delta-tracking, falling back to a surface tracking option in situations where delta-tracking is inefficient to partially offset these weaknesses. Morgan and Kotlyar introduced a Weighted Delta Tracking (WDT) routine to address these issues, replacing the rejection sampling of absorption events with an implicit event. In this research, we examine the theoretical basis for rejection sampling and implicit events, and how they relate to WDT. We then discuss implementation of a routine that extends the WDT routine to include scattering events. The routine is implemented and tested within Serpent. We examine various test cases including a Boiling Water Reactor (BWR) pin cell, and homogenous fuel media based on the content of the fuel of the Transient Test Reactor (TREAT) at Idaho National Lab (INL)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Advanced Fuel Cycle Technology: Special Session in Honor of Dr. Michael Lineberry

The US DOE recently initiated an effort to develop accident tolerant fuel designs for potential use in commercial power reactors. Evaluation of various fuel design concepts will require a broad array of testing that will include performance attributes at both steady state and transient irradiation conditions. The first stage of the transient testing program is intended to establish the relative performance limits of each proposed concept and to support development of first-draft fuel performance models. It is anticipated that this data can subsequently be used as the basis for larger scale qualification testing. This initial stage of the testing program is outlined in this paper.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

High-temperature oxidation and quenching of chromium-coated zirconium alloy ATF cladding tubes with and w/o pre-damage

Chromium-coated zirconium alloys are one of the promising candidates for accident-tolerant fuel cladding (ATF) tubes for light water reactors (LWRs). In this study, the high temperature oxidation and degradation of two types of Cr coatings (cold spray and physical vapor deposition) with and without pre-damage by scratches were investigated on prototype rod segment samples filled with ZrO 2 pellets and tightly sealed with welded end caps. Isothermal tests at 1100 and 1200 °C were terminated by quenching with water; transient tests were performed up to 1500–1600 °C until complete coating failure. The positive effect of both types of Cr coatings was observed in all tests. Pre-damaged specimens showed only locally increased oxidation of the scratched zone, but no negative effects on the adjacent Cr coating. Finally, the behavior of the two types of coatings is compared and the degradation mechanisms are discussed based on hydrogen release data, extensive metallographic post-test examinations, and the current state of global research.

36 MATERIALS SCIENCE↗

Code validation of SAM using natural-circulation experimental data from the compact integral effects test (CIET) facility

The primary objective of this study is to validate the system analysis code, SAM, using experimental data from the Compact Integral Effects Test (CIET) experimental loop. SAM is a modern system analysis code being developed at Argonne National Laboratory for safety analysis of designs for advanced non-light water reactors (non-LWRs), such as sodium-cooled fast reactors, high-temperature gas-cooled reactors, and fluoride salt-cooled high-temperature reactors (FHRs). To support SAM code development for the wide range of non-LWR applications, it is of paramount importance to validate the code against experiments highly relevant to these reactor concepts. Additionally, the CIET facility, which was designed to reproduce the thermal-hydraulics response of FHRs under both forced- and natural-circulation conditions, has been identified and selected as one of the benchmark test facilities for SAM code validation. In this study, two sets of available CIET tests were selected for SAM code validation purposes, namely, power step change transient tests and steady-state natural-circulation tests. For all selected tests, SAM-predicted results show very good agreement with experimental data. The successful validation of SAM against these selected CIET experiments demonstrates that the computer code is well suited for thermal-hydraulics analysis of FHR designs.

42 ENGINEERING↗

SAM Code Validation using the Compact Integral Effects Test (CIET) Experimental Data

The primary objective of this study is to validate the system analysis code, SAM, using experimental data from the Compact Integral Effects Test (CIET) facility. The System Analysis Module (SAM) is an advanced and modern system analysis tool being developed at Argonne National Laboratory under the U.S. DOE Office of Nuclear Energy’s Nuclear Energy Advanced Modeling and Simulation (NEAMS) program. Originally aiming at supporting sodium fast reactor (SFR) design, it is now extended to cover other non-light water reactor (non-LWR) concepts, such as high-temperature gas-cooled reactor (HTGR) designs, molten salt-fueled, and molten salt-cooled reactor designs. To support SAM code development for the wide range of non-LWR applications, it is of paramount importance to validate the code against experiments relevant to these reactor concepts. The Compact Integral Effects Test (CIET) facility, which was designed to reproduce the thermal-hydraulics response of fluoride salt-cooled high-temperature reactors (FHR) under both forced- and natural-circulation conditions, has been identified and selected as one of benchmark test facilities for SAM code validation. Among available CIET experiments, three sets of them with distinctive characteristics were selected for SAM code validation purpose. The three sets experiments are: 1) Power step change transient tests; 2) DHX-DRACS natural circulation tests; and 3) heater frequency response tests. For all tests, steady-state or transient, SAM-predicted results show very good agreement with experimental data. The successful validation of SAM against these selected CIET experiments demonstrates that the computer code is well suited for thermal-hydraulics analysis of FHR designs.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Comparative post-irradiation examination of high burnup U-19Pu-10Zr: Assessing steady-state irradiation behavior against historical and modeled fuel performance

Here, the development of next-generation sodium-cooled fast reactors necessitates comprehensive research on metallic fuels to maximize economic performance while ensuring safe operation. In this study, we investigated the steady-state irradiation behavior of two high burnup U-19Pu-10Zr fuel pins, DP-36 and DP-40, in preparation for planned safety testing. Post-irradiation examination (PIE) was performed to quantify fuel column elongation, regions of low-density at the top of the fuel column, pin deformation, fission product distribution, fractional fission gas release, microstructural evolution, and fuel constituent redistribution. Benchmarking against existing PIE data from U-19Pu-10Zr fuel pins irradiated in EBR-II revealed consistent patterns in fuel column elongation and cladding diametral strain. However, both pins exhibited longer low-density structures, and destructive examination of DP-36 revealed more complex constituent redistribution patterns compared to previously reported data for ternary fuel pins. The steady-state irradiation of both pins was also modeled using BISON. Comparisons of PIE results with modeled predictions showed overall agreement in fractional fission gas release but consistent overestimation of axial and radial swelling due to gaseous and solid swelling models. These findings underscore the critical importance of pre-test characterization on test and sibling pins to accurately capture steady-state fuel behavior ahead of transient testing, thus establishing a baseline for post-test comparison. Additionally, these analyses identified key data gaps that warrant further investigation to improve the understanding and prediction of fuel swelling, thereby enhancing the synergy between modeling and experimental efforts in supporting accident testing.

BISON↗

Specifications of Cladding Diameter Measurements Conducted at AGHCF

Fuel element diameter data was collected on-site at the Alpha-Gamma Hot Cell Facility (AGHCF) before and after out-of-pile furnace transient tests of fuel elements. Available data records have been collected and preserved in the Out-of-Pile Transient Database (OPTD). This data is used to determine the transient-induced changes in fuel element diameter, or cladding strain, for the Whole Pin Furnace (WPF) tests. Fuel element diameter was measured by contact profilometry along the length of the fuel pin at specified rotational orientations and/or by a manually operated micrometer at several discrete axial locations along the pin. The Alpha-Gamma Hot Cell Facility Operations Manual details the way the facility operated, organizational and oversight responsibilities, and procedures for examination of samples. The working version of the manual at the time of the whole pin furnace tests and the test pin examinations is Doc. No. IPS-2-00-00, dated June 1989. This specification was developed using the operations manual and recovered measurement records in consultation with subject matter experts (SMEs). The measurement methods, format of the available post-test examination (PTE) data, and recommended methods for use and interpretation of that data are summarized. Section 2 describes the available diameter measurement data for the WPF tests with guidance for interpretation and usage, and Section 3 describes the instrument measurement procedures and calibration methods.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Advanced Multiscale Microscopy Characterization of High Burnup LWR UO 2 Before and After LOCA Testing

Previous microscopy work within the campaign has observed increased porosity coupled with subgrain formation in the mid-radial region of the fuel. However, examinations of high burnup fuel taken from multiple reactors with different operating conditions have shown that this structure can move radially inward depending on the fuel operating conditions. It is currently theorized that inter- and intragranular fission gas bubble nucleation is precursory to the grain subdivision observed in the mid-radial and central regions of the fuel. Characterization of samples after loss-of-coolant accident (LOCA) testing has revealed that these restructured regions with a high density of bubbles and subgrains pulverize during the transient test. It appears that the increase in fission gas bubbles coupled with grain subdivision renders the fuel mechanically weaker during a LOCA transient and thus susceptible to fuel fragmentation relocation and dispersal (FFRD). Work this past fiscal year has prioritized understanding this behavior by using advanced microscopy to investigate fission gas behavior in the as-irradiated and post-LOCA state. Additional work has been performed to verify the theory described above by analyzing multiple post-LOCA optical micrographs and comparing that to as-irradiated microstructural data. This document reports progress in the post-irradiation characterization of high burnup nuclear fuel with emphasis on the restructured fuel regions, particularly how microstructural features influence FFRD and fission gas release behavior in LOCA conditions.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Design of a Loss of Coolant Blowdown Capsule for Remote Assembly with High Burnup Fuel

The Transient Water Irradiation System is an enhanced capability capsule type irradiation vehicle designed to support fuel safety research for light water reactor specimens in the Transient Reactor Test Facility and is designed to simulate loss of coolant and reactivity-initiated accidents. The capsule was designed, deployed, and commissioned with fresh fuel specimens to validate instrumentation and prepare for previously irradiated high burnup specimens. The irradiation system features an extensive in-situ instrumentation package to detect phenomena typical to light water reactor fuels. To accommodate the assembly with high burnup specimens inside the Hot Fuel Examination Facility, and to ensure instrumentation integrity is maintained throughout assembly, the design was updated to support remote handling. The updated design features a hinge mechanism which allows for remote pre-irradiated specimen loading and assembly while protecting sensitive instrumentation by relocating during loading. Fixtures and equipment have been developed to handle the experiment capsule and components in cell, and to support remote assembly. The experiment module also includes radiation shielding and contamination control to support operations after removal from the hot cell.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗