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At least 163 records · Page 9

Rapid depletion analysis of flowing-pebble reactor systems at equilibrium using SCALE

Several high-temperature gas-cooled reactor concepts (and more recently, salt-cooled designs such as the fluoride salt-cooled high-temperature reactor) feature core designs employing continuously circulating fuel pebbles. These reactor designs permit both continuous online refueling of fuel elements as well as higher overall achievable discharge burnups. However, rapid calculation of time-dependent fuel isotopic inventories proves challenging for this class of dynamic systems with current analysis tools. While iterative approaches employing coupled neutron transport have been developed to solve this issue, rapid depletion analysis techniques are needed to calculate time-dependent inventories for individual pebbles and batches (and thus the construction of full- core inventory at equilibrium). We propose a depletion analysis strategy for this type of system for cores at equilibrium. Drawing upon previous neutronic analysis of the PBMR-400 equilibrium core, we demonstrate the viability of developing collapsed one-group cross section libraries suitable for performing rapid depletion analyses with SCALE. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Light Water Reactor Sustainability Program Modeling of Cu Precipitate Contributions to Reactor Pressure Vessel Steel Microstructure Evolution and Embrittlement

This report summarizes the lower-length-scale effort during FY 2017 in developing simulation capabilities for the mesoscale: models for microstructure evolution and plasticity in reactor pressure vessel steels. During operation, reactor pressure vessels undergo hardening and embrittlement caused by irradiation induced defect accumulation and irradiation enhanced solute precipitation. Both defect production and solute precipitation initiate on the atomic scale and manifest their eventual effects as degradation in the engineering scale properties. To predict the engineering scale property degradation, multiscale modeling and simulation capabilities are needed to better understand the microstructure evolution and to connect the microstructure feature evolution to the engineering scale material properties. In this report the development of coupling across different length scale models to understand the multi-physics property dedgration problem is discussed. The development of coupling a lattice kinetic Monte Carlo code to cluster dynamics to capture irradiation enhanced diffusion in the formation of defects is summarized. The implementation of a cluster dynamics model with Grizzly to predict Cu percipitate formation is discussed. A summary of the coupling of crystal plasticity and cluster dynamics to predict the effect on reactor pressure steel hardening is given.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Reactor System Safety: A case for New and Advanced Reactors

This presentation covers a generic overview of reactor system safety testing, analysis, and related research and development (R&D) focusing on new and advanced reactor systems. This presentation is prepared for graduate-level student seminar talks. No specific reactor design information is provided. Only publicly available information and related published articles and book contents are utilized.

21 - SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLAN↗

Multiscale model based design of an energy–intensified novel adsorptive reactor process for the water gas shift reaction

In this work, an adsorptive reactor (AR) process is considered that can energetically intensify the water gas shift reaction (WGSR). To best understand AR process behavior, a multiscale, dynamic, process model is developed. This multiscale model enables the quantification of catalyst and adsorbent effectiveness factors within the reactor environment, obliviating the commonly employed assumption that these factors are constant. Simulations of the AR's alternating adsorption-reaction/desorption operation, using the proposed model, illustrate rapid convergence to a long-term periodic solution. The obtained simulation results quantify the influence of key operating conditions and design parameters (e.g., reactor temperature/pressure, W cat /F CO , W ad /F CO , F H2O /F CO ratios, and pellet size) on the AR's behavior. Finally, they also demonstrate, for pellet diameters used at the industrial scale, significant temporal and axial variation of the catalyst/adsorbent pellet effectiveness factors. Finally, the energetic intensification benefits of the proposed AR process over conventional WGSR packed-bed reactors are quantified.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Enhancing the Chemical Energy Flux in a High-Temperature Tubular Counterflow Solid Fuel Synthesis Reactor Using a Bypass

Redox reactions of metal oxides offer a path towards using intermittent renewable resources for high-density thermochemical energy storage. Thermochemical energy storage often involves the flow of a particulate media. We describe a novel method to increase the throughput in a gravity-driven high-temperature thermochemical storage reactor flowing pelletized MgMnO. The moving bed reactor operates under counter-flow conditions and encounters particle flowability problems at temperatures of 1500 °C leading to sintering of the bed. Inertial forces of a counter-flowing gas can overcome the gravitational forces on the particles and limit the chemical energy storage rate of the reactor. We found that the insertion of a gas bypass (a slotted tube) into the reactor results in a 100% increase of the flow rates and achieved a 50% higher chemical energy storage flux compared to the operation without a bypass tube while mitigating the effects of sintering on the particles. As a result, the higher solid flow rates require a longer heated zone to reach a comparable residence time and extent of reduction compared to the lower flow rates.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Design and construction of a cascading pressure reactor prototype for solar-thermochemical hydrogen production

Recent work regarding the efficiency maximization for solar thermochemical fuel production in two step cycles has led to the design of a new type of reactor—the cascading pressure reactor—in which the thermal reduction step of the cycle is completed in multiple stages, at successively lower pressures. This approach enables lower thermal reduction pressures than in single-staged reactors, and decreases required pump work, leading to increased solar to fuel efficiencies. In this work we report on the design and construction of a prototype cascading pressure reactor and testing of some of the key components. We specifically focus on the technical challenges particular to the design, and their solutions.

14 SOLAR ENERGY↗

Design Studies for the Optimization of 238 Pu Production in NpO 2 Targets Irradiated at the High Flux Isotope Reactor

Efforts to reestablish a domestic 238 Pu production capability in support of National Aeronautics and Space Administration mission objectives are ongoing throughout the U.S. Department of Energy complex. The Plutonium-238 Supply Project (PSP) was initiated in response to a report published by the National Research Council in 2011 stating that “without a restart of 238 Pu production, it will be impossible for the United States, or any other country, to conduct certain important types of planetary missions after this decade.” The PSP is targeting a sustained, constant production rate of 1.5 kg/year of heat source PuO 2 for several years. Design and optimization studies of 237 Np-bearing targets are underway at Oak Ridge National Laboratory (ORNL). It is anticipated that targets will be irradiated in ORNL’s High Flux Isotope Reactor (HFIR) and in the Advanced Test Reactor (ATR) at Idaho National Laboratory. A variety of target materials, containments, arrangements, and irradiation histories have been analyzed, and the results indicate that a sufficient quantity of 238 Pu can be produced in HFIR and ATR to fulfill the PSP’s constant production rate target. This paper focuses on the design and optimization of new target configurations containing pellets that are (1) ~93% of the theoretical density of NpO 2 , (2) loaded into pins of cladding materials that can be handled as solid waste following postirradiation 238 Pu recovery operations, (3) irradiated in various vertical experiment facility (VXF) locations in the HFIR permanent beryllium reflector, and (4) rotated within and/or moved to another VXF location following each HFIR operational cycle to maximize 238Pu production and minimize peak heat generation rates.

07 ISOTOPE AND RADIATION SOURCES↗

Experimental and modeling study of chemical-based strategies for mitigating dust formation in fusion reactors [Plasma Flow Reactor Chemical Kinetics: A Method Toward Optimizing Nano-Manufacturing and Laser Inertial Fusion Energy Strategies]

We studied carbon/hydrogen/oxygen chemical kinetics at time scales and thermal conditions relevant to fusion energy applications using a custom-built plasma flow reactor to investigate chemical-based strategies for eliminating carbon dust formation in fusion reactors. Acetylene and oxygen gases under varying conditions of initial concentrations are injected into an inductively coupled argon plasma where complete molecular dissociation occurs. The evolution of chemical species is investigated along the plasma flow reactor as a function of temperature and residence time. Atomized species of C, H, and O cool from 5000 K to 1000 K within 30 ms at atmospheric pressures. We employed optical emission and infrared absorption spectroscopy to measure the reaction intermediates (e.g. C 2 ) and products (e.g. C 2 H 2 ). Chemical equilibrium models are inadequate to describe the evolution of carbon molecular products, and thus a chemical kinetics model is developed. In both experiments and kinetic modelling, we find that the addition of oxygen in 1:1 proportion to carbon strongly favors the formation of CO, preventing the formation of acetylene (an important soot precursor) in less than 10 milliseconds. The kinetics model is also used to perform a reaction sensitivity and a rate of production analyses to identify the rate determining steps and the major chemical pathways that control the acetylene production/consumption. The results demonstrate the feasibility of chemical-based strategies for eliminating the formation of carbonaceous particles in fusion energy reactors.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Light Water Reactor Sustainability Program: Technical and Economic Considerations for Uprate of Existing Nuclear Reactors with Cogeneration

The United States nuclear reactor fleet consists of 63 pressurized water reactors and 31 boiling water reactors and is a pivotal component in the nation's energy infrastructure, supplying approximately 97 GW e of clean power. With the country's commitment to decarbonization by 2050, these reactors are not only instrumental in decarbonizing the electricity grid but also play a critical role in decarbonizing industrial processes, producing clean fuels, and scaling up CO 2 removal. This report delves into the potential for power uprates in the existing fleet to contribute to these decarbonization efforts, focusing on the expansion of capacity for applications such as hydrogen production and carbon capture and sequestration. Building on previous research, the report explores regional market demands for hydrogen, oxygen, and carbon dioxide, financial implications of oxygen and CO 2 sales from high-temperature steam electrolysis systems, and the potential for direct air capture systems paired with uprated nuclear plants.

29 ENERGY PLANNING, POLICY, AND ECONOMY↗

Heat Pipe Reactor Dynamic Response Tests: SAFE-100 Reactor Core Prototype

The SAFE-I00a test article at the NASA Marshall Space Flight Center was used to simulate a variety of potential reactor transients; the SAFEl00a is a resistively heated, stainless-steel heat-pipe (HP)-reactor core segment, coupled to a gas-flow heat exchanger (HX). For these transients the core power was controlled by a point kinetics model with reactivity feedback based on core average temperature; the neutron generation time and the temperature feedback coefficient are provided as model inputs. This type of non-nuclear test is expected to provide reasonable approximation of reactor transient behavior because reactivity feedback is very simple in a compact fast reactor (simple, negative, and relatively monotonic temperature feedback, caused mostly by thermal expansion) and calculations show there are no significant reactivity effects associated with fluid in the HP (the worth of the entire inventory of Na in the core is .<el, so fluid movement and temperature changes will cause very minor effects). In previous SAFE-100 tests, the point kinetics model was based on core thermal expansion via deflection measurements. It was found that core deflection was a strung function of how the SAFE-100 modules were fabricated and assembled (in terms of straightness, gaps, and other tolerances). To remove the added variable of how this particular core expands as compared to a different concept, it was decided to use a temperature based feedback model (based on several thermocouples placed throughout the core).

Bragg-Sitton, Shannon M.↗

Summary of the Workshop on Molten Salt Reactor Technologies Commemorating the 50th Anniversary of the Startup of the Molten Salt Reactor Experiment

A workshop on Molten Salt Reactor (MSR) technologies commemorating the 50th anniversary of the Molten Salt Reactor Experiment (MSRE) was held at Oak Ridge National Laboratory on October 15–16, 2015. The MSRE represented a pioneering experiment that demonstrated an advanced reactor technology: the molten salt eutectic-fueled reactor. A multinational group of more than 130 individuals representing a diverse set of stakeholders gathered to discuss the historical, current, and future technical challenges and paths to deployment of MSR technology. This paper provides a summary of the key messages from this workshop.

Greenwood, Michael Scott↗

Summary of thermocouple performance during advanced gas reactor fuel irradiation experiments in the advanced test reactor and out-of-pile thermocouple testing in support of such experiments

High temperature gas reactor experiments create unique challenges for thermocouple-based temperature measurements. As a result of the interaction with neutrons, the thermoelements of the thermocouples undergo transmutation, which produces a time-dependent change in composition and, as a consequence, a time-dependent drift of the thermocouple signal. This drift is particularly severe for high temperature platinum-rhodium thermocouples (Types S, R, and B) and tungsten-rhenium thermocouples (Type C). For lower temperature applications, previous experiences with Type K thermocouples in nuclear reactors have shown that they are affected by neutron irradiation only to a limited extent. Similarly, Type N thermocouples are expected to be only slightly affected by neutron fluence. Currently, the use of these nickel-based thermocouples is limited when the temperature exceeds 1000 deg. C due to drift related to phenomena other than nuclear irradiation. High rates of open-circuit failure are also typical. Over the past 10 years, three long-term Advanced Gas Reactor experiments have been conducted with measured temperatures ranging from 700 deg. C - 1200 deg. C. A variety of standard Type N and specialty thermocouple designs have been used in these experiments with mixed results. A brief summary of thermocouple performance in these experiments is provided. Most recently, out-of-pile testing has been conducted on a variety of Type N thermocouple designs at the following (nominal) temperatures and durations: 1150 deg. C and 1200 deg. C for 2,000 hours at each temperature, followed by 200 hours at 1250 deg. C and 200 hours at 1300 deg. C. The standard Type N design utilizes high purity, crushed MgO insulation and an Inconel 600 sheath. Several variations on the standard Type N design were tested, including a Haynes 214 alloy sheath, spinel (MgAl{sub 2}O{sub 4}) insulation instead of MgO, a customized sheath developed at the University of Cambridge, and finally a loose assembly thermocouple with hard-fired alumina insulation and a molybdenum sheath. The most current version of the High Temperature Irradiation Resistant Thermocouple, based on molybdenum/niobium alloys and developed at Idaho National Laboratory, was also tested. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Demonstration of MOOSE-based Griffin reactor physics, code for heterogeneous lead-cooled fast reactor analysis

The MOOSE-based reactor physics code Griffin was assessed on a heterogeneous pin-resolved model of a prototype lead-cooled fast reactor assembly. This model was developed in preparation for future use in MOOSE-based multiphysics calculations for computing hot channel factors. Heterogeneous multigroup cross sections were prepared using the fast reactor multi-group cross section processing code MC{sup 2}-3 using a two-step method. Griffin simulations were performed using the DFEM-SN solver on 576 cores on Argonne's LCRC cluster. Diffusion-based acceleration methods were applied (NDA and CMFD). Reference solutions were generated with continuous energy MCNP and the hybrid MOC/finite element solver PROTEUS-MOC for code-to-code comparison. Space-angle convergence studies were conducted to observe convergence in k-eigenvalue and axial pin power distributions. The fully resolved Griffin calculation was within 68 pcm of the MCNP eigenvalue and exhibited max 1.2% relative error in the axial pin power distribution. Griffin produced nearly identical results to PROTEUS-MOC when using the same 9-group multigroup cross-section set. Griffin demonstrated favorable scaling in wall-clock time and memory usage when using diffusion-based acceleration methods. Griffin is capable of simulating the pin-resolved heterogeneous LFR assembly with good accuracy and performance, and is suitable for future use in coupled high-fidelity hot channel factor simulations. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Multiscale thermal hydraulic coupling methods for boiling water reactor simulation

During the last two years, the Virtual Environment for Reactor Applications (VERA) has been extended to simulate boiling water reactors (BWRs). The thermal hydraulic effects present in BWRs are far more complex than those in pressurized water reactors (PWRs). Therefore, the runtime is significantly increase and convergence behavior worse compared to PWRs. Most of the additional runtime is spent during the first few coupled iterations, when the power shape is still rapidly evolving, dramatically affecting the thermal hydraulics (TH). To alleviate the increased computational expense, a multiscale TH coupling approach was developed in VERA in which a highly efficient, simplified TH model is solved for several coupled iterations until the power shape is partially converged. The simplified solution is used to inform the assembly-wise flow distribution in the high-fidelity TH solver CTF, reducing the amount of work required to properly balance the pressure drop in each channel and reducing runtime for the couple calculation. Because the final TH calculations are performed with CTF, there is ultimately no impact on the accuracy of the converged solution. This paper presents the details of this multiscale TH coupling approach, along with results for a 4x4 array of GE-14 fuel bundles and whole-core coupled simulations of the Hatch core. These two cases show that the multiscale approach dramatically reduces the runtime of coupled BWR simulations. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Microstructural Examinations of Reactor Pressure Vessel Surveillance and Test Reactor Irradiated Materials

The reactor pressure vessel (RPV) in a light-water reactor (LWR) represents the first line of defense against a release of radiation in case of an accident. Thus, regulations that govern the operation of commercial nuclear power plants require conservative margins of fracture toughness, both during normal operation and under accident scenarios. In the unirradiated condition, the RPV has sufficient fracture toughness such that failure is implausible under any postulated condition, including pressurized thermal shock (PTS) in pressurized water reactors (PWR). In the irradiated condition, however, the fracture toughness of the RPV may be severely degraded, with the degree of toughness loss dependent on the radiation sensitivity of the materials. As stated in previous progress reports, the available embrittlement predictive models, e.g. [1], and our present understanding of radiation damage are not fully quantitative, and do not treat all potentially significant variables and issues, particularly considering extension of operation to 80y. The major issues regarding irradiation effects are discussed.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Preliminary Demonstration Reactor Point Design for the Fluoride Salt-Cooled High-Temperature Reactor

Development of the Fluoride Salt-Cooled High-Temperature Reactor (FHR) Demonstration Reactor (DR) is a necessary intermediate step to enable commercial FHR deployment through disruptive and rapid technology development and demonstration. The FHR DR will utilize known, mature technology to close remaining gaps to commercial viability. Lower risk technologies are included in the initial FHR DR design to ensure that the reactor can be built, licensed, and operated within an acceptable budget and schedule. These technologies include tristructural-isotropic (TRISO) particle fuel, replaceable core structural material, the use of that same material for the primary and intermediate loops, and tube-and-shell heat exchangers. This report provides an update on the development of the FHR DR. At this writing, the core neutronics and thermal hydraulics have been developed and analyzed. The mechanical design details are still under development and are described to their current level of fidelity. It is anticipated that the FHR DR can be operational within 10 years because of the use of low-risk, near-term technology options.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Core follow calculation with the nTRACER numerical reactor and verification using power reactor measurement data

The nTRACER direct whole core transport code employing the planar MOC solution based 3-D calculation method, the subgroup method for resonance treatment, the Krylov matrix exponential method for depletion, and a subchannel thermal/hydraulic calculation solver was developed for practical high-fidelity simulation of power reactors. Its accuracy and performance is verified by comparing with the measurement data obtained for three pressurized water reactor cores. It is demonstrated that accurate and detailed multi-physic simulation of power reactors is practically realizable without any prior calculations or adjustments. (authors)

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

The international research reactor conversion effort and its contribution to the validation of reactor physics and thermal-hydraulics codes

Full text of publication follows. With about 200 reactors in operation, civilian Research and Test Reactors (RTRs) represent approximately a third of the global nuclear fleet. RTRs make use of core designs that are drastically different from commercial power plants to perform a wide variety of non-power applications that greatly benefit society. Because they often rely on high neutron fluxes, RTRs are designed with relatively compact cores and as a result, prior to the 1980's, were often deployed using Highly Enriched Uranium fuel (HEU, {sup 235}U/U = 20 wt. %). Due to proliferation concerns, the international community aims at eliminating the use of HEU in civilian facilities and favor instead the use of Low Enriched Uranium fuel (LEU, {sup 235}U/U < 20 wt. %). A program to support conversion of the world's RTRs to LEU fuel has been initiated in 1978 by the U.S. Department of Energy (DOE). This program is still alive today and has achieved more than 103 conversion metrics. Today, the program focuses heavily on the conversion of so-called high-performance RTRs, which are far more challenging than previous conversions as they require new fuel element designs and the use of new, higher density LEU fuel forms. Development and qualification of new LEU fuel elements is ongoing and requires extensive engineering analysis and testing. Both activities require the development and validation of codes and methods for reactor physics, thermal-hydraulics, and multi-physics, which in turn rely on experiments performed in RTRs or other experimental facilities. This talk will present the collection of RTR experimental data and benchmark analyses from the international conversion program that contribute to the validation of computer codes and methods.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗